Probabilistic Fracture Mechanics Analyses of Reactor Pressure Vessel Under PTS Transients

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Probabilistic Fracture Mechanics Analyses of Reactor Pressure


Vessel under PTS Transients

Kunio ONIZAWA

, Katsuyuki SHIBATA

, Daisuke KATO

and Yinsheng LI

The probabilistic fracture mechanics (PFM) analysis code PASCAL has been developed
in JAERI. This code can evaluate the conditional probabilities of crack initiation and fracture
of a reactor pressure vessel (RPV) under transient conditions such as pressurized thermal
shock (PTS). Based on the temperature and stress distributions in the vessel wall for four
cases of PTS transients in a typical 3-loop PWR, parametric PFM analyses were performed
using PASCAL on the variables such as pre-service inspection method, crack geometry, frac-
ture toughness curve and irradiation embrittlement prediction equation. The results showed
that the Arakawas model for a pre-service inspection had a signicant eect on the fracture
probability and reduced it by more than 3 orders of magnitude compared with no inspec-
tion case. The fracture probability calculated by the fracture toughness estimation method in
Japan was about 2 orders of magnitude lower than that by the USA method. It was found
that the treatment of a semi-elliptical crack after its initiation in PASCAL reduced the con-
servatism in a conventional method where it is transformed into an innite length crack.
Key Words: Reactor Pressure Vessel, Probabilistic Fracture Mechanics, Pressurized Ther-
mal Shock, Non-Destructive Examination, Irradiation Embrittlement, Fracture
Toughness
1. Introduction
Prevention of non-ductile fracture of a reactor pres-
sure vessel (RPV) is one of the most important items to
assure the integrity of primary loop pressure boundary of
a light water reactor. Therefore, stringent design criteria
are prescribed in the codes and standards, such as fracture
toughness requirements and surveillance programmethod.
One of the major aging degradation mechanisms of a
RPV is the fracture toughness degradation due to neutron
irradiation, that is, the irradiation embrittlement of RPV
steel around the beltline region. For pressurized water re-
actors, pressurized thermal shock (PTS) events are a major
safety concern considering the irradiation embrittlement.
Regarding the integrity assessment of the RPV for PTS
events, a specic rule and a regulatory guide were estab-

Received 4th September, 2003 (No. 03-4111)

Department of Reactor Safety Research, Japan Atomic


Energy Research Institute, 24 Shirakata, Tokai-mura,
Ibaraki 3191195, Japan.
E-mail: konizawa@popsvr.tokai.jaeri.go.jp

Science Solution Group, Fuji Research Institute Corpo-


ration, 23 Kanda Nishikicho, Chiyoda-ku, Tokyo 101
8443 Japan
lished in the U.S.A.
(1), (2)
and afterwards in some countries.
The PTS rule prescribes the screening criterion for the
reference temperature of fracture toughness curve. When
the reference temperature is predicted to reach the crite-
rion, additional analysis by means of probabilistic fracture
mechanics (PFM) is required according to the regulatory
guide to assess the risk due to PTS events for the operation
of the plant with the reference temperature above the cri-
terion. The OCA-P
(3)
and VISA-II
(4)
codes are referred to
in the regulatory guide as the representative PFM analysis
codes.
Since the PTS rule was established, there have been
advancements in relevant technologies associated with the
physical phenomena involved in PTS events that may im-
pact the RPV integrity assessment. Based on the advance-
ments, the level of conservatism in the screening criterion
may be reduced without aecting the level of safety
(5)
.
The PTS re-evaluation project was therefore initiated to
revisit the technical basis for the current PTS rule and
to possibly propose to revise the rule that would reduce
any unnecessary level of conservatism in the current rule
within the framework established by modern probabilistic
risk assessment (PRA) techniques
(6)
. The improved mod-
els have been implemented into the FAVOR code
(7)
. Some
Series A, Vol. 47, No. 3, 2004 JSME International Journal
487
PFM analysis codes have also been developed in the other
countries, such as PROFMAC-II
(8)
and OPERA
(9)
codes.
In JAERI, the PFM analysis code PASCAL (PFM
Analysis of Structural Components in Aging LWR) has
been developed
(10), (11)
. This code can evaluate the con-
ditional probabilities of crack initiation and failure of a
RPV under transient conditions such as PTS events. The
probabilistic simulation methods used in this code are
the importance sampling Monte Carlo and stratied sam-
pling Monte Carlo methods. PASCAL has some methods
proposed in Japan, such as the crack detection capabil-
ity formula on a pre-service inspection method, fracture
toughness K
IC
curve and irradiation embrittlement pre-
diction equation as well as those in the USA. The initial
crack size, chemical composition, neutron uence, frac-
ture toughness and ductile to brittle transition temperature
are treated as probabilistic variables.
The PTS transients analyzed in the study were three
cases of loss of coolant accident (LOCA) and one case of
main steam line break for a typical 3-loop PWR. These
were selected from many transients considering the sever-
ity on the crack initiation and fracture. Based on the re-
sults of thermal hydraulic analyses of the transients, the
stress distributions in the vessel wall were calculated with
the nite element analysis tool in PASCAL.
The objective of this study is to conrm the eect
of variables important to the integrity assessment of a
RPV. In the study, we performed parametric PFM analyses
on some important models and parameters including pre-
service inspection models, fracture toughness curves and
irradiation embrittlement prediction equations. A RPV
having a semi-elliptical surface crack or an innite length
surface crack in the axial direction was analyzed. The
Marshall exponential model
(12)
was used to simulate the
distribution of an initial crack depth. This paper summa-
rizes the description of the PTS transients selected for this
study and the results of PFM analyses on several important
methods and parameters. Since the overall PTS impacts
on the RPV integrity are to be evaluated with all possi-
ble transients through PRA procedure taking into account
their respective occurrence frequencies, this study is con-
sidered as a scoping analysis on the important features in
conditional fracture probability. The comprehensive PTS
analyses are to be performed in the next step.
2. Analysis
2. 1 Thermal hydraulics analysis
PTS analyses are performed for an RPV of 3-loop
PWR. Referring to the analysis results performed for the
H. B. Robinson reactor
(13)
, four out of more than 20 se-
quences were selected, considering the frequency of the
event and likelihood of crack initiation during each event.
The selected four PTS sequences are as follows:
1 ) Small break LOCA at hot 0% power condition
(SEQ 1)
2 ) Small break LOCA at hot 0% power condition
(Auxiliary feed water not stopped) (SEQ 2)
3 ) Main steam line break at hot 0% power condition
(SEQ 3)
4 ) Medium break LOCA at full power (SEQ 4)
For SEQ 1 to SEQ 3, thermal hydraulics analyses in
the primary loop were performed by using the TRAC-PF1
code for approximately one hour after the event occur-
rence
(14)
. The temperature of the coolant at the down-
comer region inside the RPV shell, primary loop pressure,
and heat transfer coecient obtained from the thermal hy-
draulics analyses are plotted as a function of time in Figs. 1
to 3. The SEQ 4 corresponds to the sequence 2.1 in the
PTS analysis report for the H. B. Robinson
(15)
. The tem-
perature, pressure and heat transfer coecient for SEQ 4
are those shown in the report. The time histories of these
parameters were extrapolated until two hours in order to
conrm the termination of the thermal stress during the
sequence.
2. 2 Stress analysis
A RPV was modeled by a cylindrical shell with the
inside radius of 1 994 mm and the thickness of the vessel
wall of 197 mm including 5 mm of overlay cladding at the
inner surface. Physical and mechanical properties of the
weld metal and cladding used in the thermal stress anal-
Fig. 1 Coolant temperature at the downcomer region during
PTS transients
Fig. 2 Primary loop pressure during PTS transients
JSME International Journal Series A, Vol. 47, No. 3, 2004
488
Fig. 3 Heat transfer coecients (HTC) during PTS transients
Table 1 Physical and mechanical properties used in the analy-
ses
(a) Weld metal
(b) Overlay cladding
yses are listed in Table 1. The temperature dependence
of the properties is considered by linear interpolation be-
tween listed values.
A thermal stress analysis for the whole period of each
sequence was performed by a FEM program attached to
the PASCAL code. To calculate the thermal stratication
of low temperature coolant injected from the emergency
core cooling system (ECCS) when a natural circulation is
terminated, it is necessary to perform a thermal mixing
analysis. In this study, however, the coolant temperature
histories in the downcomer region from the analyses by
the TRAC-PF1 were used for simplicity. The results of
the thermal stress analysis for SEQ 2 are shown in Fig. 4
(a) Temperature distribution in the wall of an RPV
(b) Circumferential stress distribution in the wall of an RPV
Fig. 4 Results of thermal stress analysis for SEQ 2
as an example. At 40 minutes after the transient initia-
tion, the circumferential stress at the inside region of weld
metal becomes highest during the transient. At that time,
the stress at the inside region reached the yield strength
of weld metal as seen in Fig. 4. When the level of stress
is compared among the sequences, SEQ 2 results in the
highest, while SEQ 4 is the lowest.
2. 3 Probabilistic fracture mechanics analysis
A single crack in the weld metal was modeled in axial
direction of the RPV and assumed to be an innite length
crack or a semi-elliptical crack at the inner surface. No
combination of multiple cracks was considered. A distri-
bution of the size of crack is a major factor for fracture
mechanics analysis. The distribution was simulated using
the Marshall distribution
(12)
that was expressed as an ex-
ponential type equation. For the semi-elliptical crack, the
aspect ratio (depth / length: a/c) was assumed to follow
a log-normal distribution where the probability of aspect
ratio less than 0.2 was approximately 1%.
Non-destructive examination (NDE) was considered
only for a pre-service inspection (PSI). To study the ef-
fect of the NDE, the ultrasonic testing model proposed by
Arakawa
(16)
and the NDE model developed at LLNL
(17)
were applied in the present study. The Arakawa model
was developed for advanced ultrasonic testing methods
based on theoretical considerations and laboratory experi-
Series A, Vol. 47, No. 3, 2004 JSME International Journal
489
ments. The LLNL model was developed for the ultrasonic
testing of nuclear piping and applied to a PFM analysis
code, PRAISE.
Neutron uence at the vessel inner surface was var-
ied up to 10 10
19
n/cm
2
(E > 1 MeV) by considering
an extended operation beyond the design basis plant life-
time. The decrease in fracture toughness due to neutron
irradiation was evaluated by the shift of transition tem-
perature in the fracture toughness curve according to ei-
ther the method prescribed in the JEAC 4206
(18)
or the
method used in the USA. For the JEAC method, the tran-
sition temperature shift of RPV steel is estimated by the
Japanese embrittlement prediction equation in the JEAC.
The chemical compositions, such as Cu, Ni, P and Si in the
material important to the irradiation embrittlement were
set to correspond to those in a typical old-type RPV weld
metal. Fracture toughness was evaluated by means of the
Japanese K
IC
curve established for the generic PTS anal-
ysis prescribed in the JEAC 4206. On the other hand,
Regulatory Guide (R. G.) 1.99 revision 2
(19)
and the K
IC
and K
Ia
curves based on the ASME code
(20)
were used
for the USAs method. Since the K
IC
and K
Ia
curves in
the code are dened as a lower bound ones for a deter-
ministic analysis, the stochastic models developed for the
IPTS study
(3)
was applied in the PASCAL code. In the
JEAC 4206, the K
Ia
curve is not prescribed. Therefore,
the K
Ia
curve for the JEAC method was dened by using
the JEAC K
IC
curve and the temperature dierence be-
tween the stochastic models for the K
IC
and K
Ia
curves.
The attenuation of neutron uence and the degree of em-
brittlement were estimated by using the exponential type
equation provided by R. G. 1.99 rev.2. The initial condi-
tion of the fracture toughness of the RPV steel is dened
by the reference temperature, RT
NDT
. Therefore, the ini-
tial RT
NDT
value was set to 50

C for a relatively new


material and 17.8

C for an old one, respectively.


For PFM analyses, several parameters are considered
as probabilistic variables with a normal distribution. Ta-
ble 2 lists the variables with their respective mean, stan-
dard deviation, and limits used in this study. In this study,
a total of eight cases of the combinations of parameters
mentioned above were analyzed for each sequence as in-
dicated in Table 3.
Using the PASCAL code, the conditional probabil-
ities of crack initiation and fracture were calculated as-
suming a crack subjected to the transient for all cases. A
stratied Monte Carlo simulation is applied to the cases
woth a semi-elliptic crack while a Monte Carlo simula-
tion is applied to the cases with an innite length crack.
The maximum number of sampling in the simulations was
2.710
8
times for the cases of a semi-elliptical crack and
110
8
times for the cases of an innite length crack. The
warm pre-stress eect was not considered in this study.
The deviation from the mean of the fracture toughness
Table 2 Probabilistic variables for PFM analyses
Table 3 PFM analysis cases studied

: Initial T
0
value instead of initial RT
NDT
was used for the case
of JEAC K
IC
curve.
was calculated only once before crack initiation in the
Monte Carlo simulation based on the benchmark exer-
cises for PFM analyses
(21), (22)
. The detail information on
the other functions for fracture mechanics analysis is de-
scribed elsewhere
(23)
. In this study, the fracture is dened
as the propagation of a crack through 100% of the wall
thickness.
3. Results and Discussion
3. 1 Comparison of fracture probability on tran-
sients
The conditional fracture probabilities for base cases
1-0 and 2-0 are summarized in Table 4. These results were
obtained from the analyses with applying the Arakawas
NDE method to PSI. When the probabilities are compared
among the transients, those of SEQ 1 and SEQ 2 are al-
most the same values each other and larger than the other
transients. The transient of SEQ 3 was the least severe,
and no fracture was calculated for case 1-0 in the simu-
lations. These results can be understood from the coolant
temperature of the transients as was shown in Fig. 1. Since
the nal coolant temperature for SEQ 3 is highest, al-
JSME International Journal Series A, Vol. 47, No. 3, 2004
490
Table 4 Comparison of conditional fracture probability as a
function of neutron uence
(a) Case 1-0
(b) Case 2-0
though the initial cooling is rather rapid and there is re-
pressurization, thermal stress could be very lowfor a crack
to propagate through the wall. Since the results of SEQ 1
transient are almost similar to those of SEQ 2 transient and
the results of SEQ 3 is less important, the following dis-
cussion, the transients of SEQ 2 and SEQ 4 are used for
the comparison of the results.
3. 2 Eect of NDE
The conditional fracture probabilities obtained here
are very low as indicated in Table 4. This can be due to
high capability of crack detection in the PSI based on the
Arakawa model. In Fig. 5, the conditional fracture prob-
ability by applying the Arakawa model and LLNL model
as the PSI are compared with no PSI case. When the ef-
fects of NDE are compared, it is obvious that the fracture
probability by the Arakawa model is lower than the others
by more than 3 orders of magnitude as shown in Fig. 5.
The dierence between the Arakawa and LLNL models
is 2 orders for a semi-elliptical crack and 3 orders for
an innite length crack. This result is similar to the result
of the literature
(24)
. The probabilities for no crack detec-
tion for the Arakawa model, LLNL model and VISA-II
model are plotted in Fig. 6. The curves for the LLNL and
VISA-II methods are plotted in two patterns varying the
parameter. Clearly the Arakawa model results in the low-
est probability of no crack detection. When the fracture
probabilities as a function of crack size are concerned, the
results may be explained by practically the good NDE per-
formance by the Arakawa model. Figure 7 shows the re-
sults of case 1-d for SEQ 2 transient at the neutron uence
of 1010
19
n/cm
2
(E >1 MeV) when the Arakawa model
was applied. From Fig. 7, it is found that a crack larger
than 9% of the wall thickness does not contribute the frac-
ture in this case. The crack size of the highest probability
of fracture in this case was 3% of the wall thickness, that
(a) Semi-elliptical crack: case 1-0
(b) Innite length crack: case 2-0
Fig. 5 Eect of NDE for SEQ 2 transient
Fig. 6 Comparison of NDE models on the probability of no
crack detection
Fig. 7 Fracture probability as a function of crack size for Case
1-d at neutron uence of 1010
19
n/cm
2
(E>1 MeV)
is, 6 mm.
3. 3 Eect of fracture toughness
Initial fracture toughness is dened by the initial
Series A, Vol. 47, No. 3, 2004 JSME International Journal
491
Fig. 8 Eect of initial RT
NDT
(The JEAC prediction equation
and the ASME K
IC
curve were used.)
Fig. 9 Eect of fracture toughness curve
value of the reference temperature, RT
NDT
. As mentioned
in section 2.3, two cases of initial RT
NDT
values, 17.8

C
and 50

C, were used in this study. Figure 8 shows the


comparison of fracture probabilities for SEQ 2 and SEQ 4
transients. The dierence of 32

C in initial RT
NDT
value
results in 3 to 20 times of dierence depending on the
amount of neutron uence and the transient condition.
The dierence tends to decrease as the neutron uence in-
creases.
When the fracture toughness curve is changed from
the curve corresponding to the ASME code to that of the
JEAC, the fracture probability is signicantly decreased
as indicated in Fig. 9. The K
IC
curve corresponding to the
JEAC used in the PASCAL code was dened by the sim-
ilar method to the ASME curve with an assumption of a
normal distribution. For SEQ 2 transient, the dierence in
the probability is more than one order of magnitude, indi-
cating very low value for JEAC curve. This is because the
fracture toughness K
IC
in the JEAC is higher than that in
the ASME code.
3. 4 Eect of embrittlement prediction equation
Neutron irradiation embrittlement is predicted as a
transition temperature shift using an equation established
through a statistical analysis of surveillance database. The
equations applied in this study are those used in the
USA and Japan. For the material studied here is a weld
metal having relatively high copper (0.20 wt%) and nickel
(1.0 wt%) as compared to actual RPV welds of PWRs in
Fig. 10 Comparison of embrittlement prediction equations
between the JEAC and NRC regulatory guide
Japan. For the chemical composition of the weld, the R.
G. 1.99 rev.2 gives higher shift of transition temperature of
188

C at neutron uence of 1010


19
n/cm
2
(E >1 MeV),
while the JEAC equation gives 134

C at the same u-
ence. The dierence of these shift values directly leads
to the dierence in the fracture probability as shown in
Fig. 10. For SEQ 2 and SEQ 4 transients, the dierences
in the probabilities are factors of 2.5 and 4.5, respectively.
The dierences are not so large as compared to the ef-
fect of NDE mentioned above. There exists the dierence
in the database used to establish the prediction equations
between in the USA and in Japan. The level of copper
content of material studied here is slightly higher than the
range of Japanese RPV welds, while the nickel content is
higher than the range of the USA RPV welds. It is also
noted that the equation in R. G. 1.99 rev.2 is based on
the analysis of the surveillance data in the USA available
in 1984. Since then, a large number of surveillance data
have become available, and the understanding of embrit-
tlement mechanisms has advanced. The improved corre-
lations have recently been developed in the USA. Further
comparisons using the improved equations are necessary.
3. 5 Eect of fracture toughness estimation method
In the previous two subsections, the dierences in
fracture toughness curves and embrittlement prediction
equations were separately compared. However, the esti-
mation of fracture toughness after neutron irradiation is
practically performed in the combination of these meth-
ods. Figure 11 shows the results of the comparisons for a
semi-elliptical crack and an innite length crack for SEQ
2 and SEQ 4 transients. It is found from the gure that
the fracture probability by the USA method is two orders
of magnitude higher than that by the JEAC method, indi-
cating the signicant conservativeness of the USA method
in the analyzed case. This trend is clearer from the com-
parison of the results in the case of innite length crack
as shown in Fig. 11 (b). The dierence of the probabilities
by the two methods becomes three orders of magnitude.
As mentioned in 3.3 subsection, the dierence in fracture
toughness curve aects the fracture probability by two or-
JSME International Journal Series A, Vol. 47, No. 3, 2004
492
(a) Semi-elliptical crack
(b) Innite length crack
Fig. 11 Comparison of fracture toughness estimation methods
between Japan and the USA
ders of magnitude. Therefore it can be concluded that the
large part of the dierence in Fig. 11 comes from the dif-
ference in fracture toughness curve.
3. 6 Eect of crack geometry
When a semi-elliptic crack is subjected to higher
stress at the surface point than the deepest point, the crack
initiates towards the length direction. In the VISA-II
code
(4)
and the FAVOR code
(7)
, the crack geometry is
transformed to an innite length crack in such case. How-
ever, in the PASCAL code, the function to simulate the
increment of crack length at the surface has been incorpo-
rated in the same manner as the deepest point of the crack.
Using the function, the eect of crack geometry between
a semi-elliptic crack and an innite length crack on the
fracture probability was studied. Figure 12 compares the
fracture probabilities for a semi-elliptical crack and an in-
nite length crack. The probability for an innite length
crack is 7 to 20 times, approximately one order, higher
than that for a semi-elliptical crack for both the JEAC and
USA methods. The method to calculate the initiation and
subsequent propagation of a crack at the surface as well as
the deepest point may be more realistic than the method
that transforms a semi-elliptical surface crack into an in-
nite length surface crack. Therefore, this calculation per-
formed in PASCAL reduces the conservatism due to the
use of an innite length crack in PFM analysis.
(a) JEAC fracture toughness estimation method
(b) Fracture toughness estimation method in the USA
Fig. 12 Eect of crack geometry
4. Conclusion
The PFM analysis code PASCAL has been developed
in JAERI to analyze the failure probability of the RPVdur-
ing PTS transients for a typical 3-loop PWR. Paramet-
ric PFM analyses under PTS transients were performed
mainly focusing on the dierence in the methodologies
between Japan and the USA using the PASCAL code. The
results showed the following conclusions:
When the good performance NDE model proposed
by Arakawa for pre-service inspection is applied, the frac-
ture probability is reduced by more than 3 orders of mag-
nitude.
Due to the dierence in the equations, the fracture
toughness estimation method in Japan gives about 2 or-
ders of magnitude lower values of fracture probability than
those of the USAs method for the cases studied.
The calculation method for a semi-elliptical sur-
face crack used in PASCAL reduces the conservatism in
the method assuming an innite surface crack transformed
from an elliptical crack.
Acknowledgements
The authors thank to Drs. M. Suzuki and M. Hirano,
JAERI for their helpful discussion and supports. They
also appreciate the help and comments by Dr. M. Hirano,
JAERI who kindly supplied the information on the PTS
transients.
Series A, Vol. 47, No. 3, 2004 JSME International Journal
493
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