IFW Dresden, Germany , ,

ARPES view of low energy electronic interactions in superconducting cuprates

Alexander Kordyuk

IFW Dresden, Germany IMP Kiev, Ukraine

Navigation
Introduction to ARPES Introduction to HTSC physics The advantages of our group Electronic band structure Antinodal region Nodal region

Introduction to ARPES
the most direct tool to explore the momentum-energy space of the electrons in solids

Photoemission Spectrum

Angle-Resolved Photoemission (ARPES)

Energy

Angle

Angle Resolved Analyser

Energy

Angle

ARPES with Synchrotron Light

Damascelli RMP 2003

Basics: electron dispersion

Photocurrent geometrical prefactor momentum and energy resolution

A(k,)
matrix elements Fermi cutoff extrinsic background

I(k,) - Energy Distribution Map

I(k,) - Momentum Distribution Curve

I(k,) - Energy Distribution Curve

I(kx,ky,) - Momentum Distribution Map

Borisenko PRB 2001

Precise Cryo-Manipulator

0.1 precision

15 K < T < 400 K

UHV

Fermi-surface map
(,) (0,0) (,0) X M Z

Aebi PRL 1994

Momentum-energy space
ky
m (
-1

tu n e m o M

kx

EF

EF
Binding energy (eV) 0.5 eV

2 M X M Y
min

X M (,0)
max
Borisenko PRB 2001

X (,)

Momentum Distribution Map

300 K, 21.2 eV

Kordyuk 2000

Momentum-energy space explorer today

+
SLS

hv
BESSY

ELETTRA

more synchrotrons

...travelling chamber

The advantages of our group

why Bi(Pb)-2212 is the best of the cuprates to be explored by ARPES

Bi2Sr2CaCu2O8+ BSCCO Bi-2212

e ee e e e

Pb or not Pb?

Introduction to HTSC physics

what ARPES said, what people believed it had been saying, and what we believe it is saying today

Generic phase diagram of cuprates Bi2Sr2CaCu2O8+

Fermi surface

Damascelli RMP 2003

Borisenko PRL 2000

Bogdanov PRL 2000

Kordyuk PRB 2002

Fermi surface:
Nature of the Shadow Band (SB) Stripes ...

Borisenko PRL 2000

Peak-Dip-Hump

Quasiparticles?

100 K

Evidence for MFL

Time reversal symmetry breaking?

In what we believe today

Electronic band structure

A set of superstructure-free Bi(Pb)-2212 in a wide doping range...

Kordyuk PRB 2002

A set of superstructure-free Bi(Pb)-2212 in a wide doping range with known doping level

Kordyuk PRB 2002

Band structure: TBF

( k x , k y ) = 2t (cos k x + cos k y ) + 4t cos k x cos k y 2t (cos 2k x + cos 2k y )

0.4 eV t 0.4 eV t 0.1 eV t 0.05 eV

OD 69K
Kordyuk PRB 2003

Bare band structure

A, EDCmax , Tc

100 80 60 40 20 0 0.05 0.10 0.15 0.20 0.25 0.30

x
Kordyuk PRB 2003

High precision Fermi surface mapping

OD <Tc

OP <Tc

UD <Tc

Bilayer splitting in OP Bi-2212 in normal state

Momentum

Momentum

T<Tc Energy Energy

T>Tc

Momentum

Momentum

Key regions

UD77K 27 eV 30 K

OD69K 38 eV 30 K

Energy

Momentum

Energy

Momentum

Saddle point

(,0)

Excitation energy variation: PDH in OD

Kordyuk PRL 2002

Excitation energy variation: PDH in OD

Kordyuk PRL 2002

Antinodal region (XMY)

Antinodal or "XMY cut"

Interaction with a mode

d
0.0

-0.1

OD69K hv = 21.2 eV -0.2 T = 30 K

0.2 0.1 0.0

OD69K hv = 38 eV T = 30 K
0.2 0.1 0.0 -0.1 -0.2

OD76K hv = 50 eV T = 30 K
0.2 0.1 0.0 -0.1 -0.2

g Energy (eV)
0.0

-0.1

UD77K hv = 25 eV -0.2 T = 30 K
0.2 0.1 0.0

UD77K hv = 38 eV T = 30 K
0.2 0.1 0.0 -0.1

UD76K hv = 55 eV T = 30 K
0.2 0.1 0.0 -0.1 -0.2

j
0.0

-0.1

UD77K hv = 21.2 eV -0.2 T = 120 K

0.2 0.1 0.0

UD77K hv = 38 eV T = 120 K
-0.1 0.2 0.1 0.0 -0.1
-1

UD77K hv = 50 eV T = 120 K
0.3 0.2 0.1 0.0 -0.1 -0.2 )

Momentum (

Borisenko PRL 2003

Interaction with a mode

Kim PRL 2003

Antinodal electrons couple to ...

Doping dependence: UD OD Temperature dependence: <Tc Energy ~ 40 meV k-dependence:

spin fluctuations

Nodal direction (GX)

Kinks

Kaminski PRL 2001 Bogdanov PRL 2000

Johnson PRL 2001

Lanzara Nature 2001

Kinks

Zhou Nature 2003

Zhou cond-mat 2004

One complication: nodal splitting

c
1

ky ( )

-1

X
-1

-2

-1
-1

kx ( )

Kordyuk PRB 2004

Nodal splitting

k = 0.012 1/ = 50 meV (bare!)

27 eV

17.5 eV

Kordyuk PRB 2004

Bare dispersion

Kordyuk cond-mat/0405696

Self-energy approach

Kordyuk cond-mat/0405696

Self-energy approach

'() = KK ''()

Kordyuk cond-mat/0405696

Kramers-Kronig transform

'() = KK ''()

Kordyuk cond-mat/0409483

Bare dispersion

Kordyuk cond-mat/0405696

Bare dispersion
Self-consistency: LDA + self-energy Well defined quasiparticles Kink phenomenology

Kordyuk cond-mat/0405696

Kinks

Kaminski PRL 2001 Bogdanov PRL 2000

Johnson PRL 2001

Lanzara Nature 2001

Phenomenology of the kink

Kordyuk cond-mat/0409483

Scattering rate kink

Kordyuk PRL 2004

Scattering rate

Kordyuk PRL 2004

Scattering rate kink

Kordyuk PRL 2004

Parity

Circular dichroism in nodal region

Kinetic energy (eV)

46.0

45.8

45.6
T

0 -2 Angle (deg)

-4

(, )

Borisenko 2004

Circular dichroism in nodal region

Kinetic energy (eV)

46.0

45.8

45.6
T

0 -2 Angle (deg)

-4

(, )

Borisenko 2004

Circular dichroism in nodal region

(, )

Borisenko 2004

Odd scattering
~ antibonding ~ bonding

Im (ab. un.)

x10

50 40 30 20 10 -0.20 -0.15

Antibonding Bonding

-0.10 Energy (eV)

-0.05

0.00

Borisenko 2004

Nodal electrons couple to ...

Doping dependence: UD OD Temperature dependence: < Tc for OD < T* for UD Parity: odd boson

spin fluctuations

Conclusions
The spectral function analysis is applicable to the ARPES spectra from HTSC cuprates. Along the nodal direction well defined quasiparticles exist even for the underdoped Bi-2212 in the pseudogap state. Two channels in the scattering rate can be distinguished. The main doping independent contribution to the scattering can be well understood in terms of the conventional Fermi liquid model... ...while the additional doping dependent contribution has a magnetic origin. The magnetic contribution essentially increases with underdoping becoming dominant for the rest of the Brillouin zone and therefore determines the unusual properties of the cuprates in the superconducting and pseudo-gap phases.

Thanks to:
Spectroscopy Group IFF, IFW Dresden
Sergey Borisenko

Thanks to:
Spectroscopy Group IFF, IFW Dresden
Sergey Borisenko, Timur Kim, Andreas Koitzsch, Vladimir Zabolotny, Jochen Geck, Roland Hbel, Martin Knupfer, Jrg Fink ,

Single Crystals
Helmut Berger Chengtian Lin, Bernhard Keimer S. Ono, Yoichi Ando EPFL Lausanne MPI Stuttgart CRIEPI Tokyo

Synchrotron Light
Rolf Follath Stefano Turchini, Cesare Grazioli Ming Shi, Luc Patthey BESSY Berlin ELETTRA Trieste SLS Villigen

THE END