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Quantum Fluctuations of A Coulomb Potential As A Source of Flicker Noise
Quantum Fluctuations of A Coulomb Potential As A Source of Flicker Noise
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Quantum Fluctuations of a Coulomb Potential as a Source of Flicker Noise
Kirill A. Kazakov
A
0
|in, in|
A|in. In the
Schwinger-Keldysh formalism [10, 11], they are given by
in|
|in =
_
D
_
D
+
A
+
exp{iS[
+
] iS[
]} , (2)
where the subscript + () shows that the time argument of the integration variable runs from to + (from +
to ). Integration is over all elds satisfying
A
+
0 ,
+
+
0
, (
)
+
0
)
+
for t ,
+
=
for t +, (3)
where collectively denotes the fundamental elds of the theory, = {A
, ,
}, the components ,
describing
the charged particle which for simplicity will be assumed scalar,
0
is the given particle state, D the invariant
integral measure, and S = S[] the action functional of the system. Assuming that the gradient invariance of the
theory is xed by the Lorentz condition
G
= 0 , (4)
the action takes the form
S[] = S
0
[] + S
gf
[] ,
S
0
[] =
_
d
4
x
_
(
+ ieA
)(
ieA
) m
2
1
4
_
d
4
xF
,
S
gf
[] =
1
2
_
d
4
x G
2
, F
. (5)
Diagrammatics generated upon expanding the integral (2) in powers of the coupling constant e consists of the following
elements. There are four types of pairings for each eld A
(x, y) =
_
D
++
(x, y) D
+
(x, y)
D
+
(x, y) D
(x, y)
_
=
_
iT
A
(x)
A
(y)
0
i
(y)
A
(x)
0
i
(x)
A
(y)
0
i
T
A
(x)
A
(y)
0
_
,
D(x, y) =
_
D
++
(x, y) D
+
(x, y)
D
+
(x, y) D
(x, y)
_
=
_
iT
(x)
(y)
0
i
(y)
(x)
0
i
(x)
(y)
0
i
T
(x)
(y)
0
_
,
where the operation of time ordering T (
T) arranges the factors so that the time arguments decrease (increase) from
left to right, and
0
denotes vacuum averaging. The propagators D
(x, z)D
(z, y) = e
(4)
(x y) , G
(x, y) = i
2
S
(2)
A
(x)A
(y)
, (6)
_
d
4
z G(x, z)D(z, y) = e
(4)
(x y) , G(x, y) = i
2
S
(2)
(x)(y)
, (7)
where S
(2)
is the free eld part of the action, e, i are 2 2 matrices with respect to indices +, :
e =
_
1 0
0 1
_
, i =
_
1 0
0 1
_
.
As in the ordinary Feynman diagrammatics of the S-matrix theory, the propagators are contracted with the vertex
factors generated by the interaction part of the action, S
int
[] = S[] S
(2)
[], with subsequent summation over
(+, ) in the vertices, each vertex coming with an extra factor (1). This can be represented as the matrix
multiplication of D
3
S
A
(x)(y)
(z)
=0
,
where the indices i, j, k take the values +, , and s
ijk
is dened by s
+++
= s
0
_
, r
= (
0
,
0
),
satisfying
_
d
4
z G(x, z)r(z) =
_
0
0
_
,
_
d
4
x r
(x)|in calculated using the ordinary Feynman rules. This is natural because we are concerned here with
a one-point function whose matrix element is evaluated between one-particle states for which |in is essentially the
same as |out. The things change, however, if we want to determine the eld uctuation. In the Schwinger-Keldysh
formalism, the expectation value of the product
A
(x)
A
(x
(x)
A
(x
)|in =
_
D
_
D
+
A
(x)A
+
(x
) exp{iS[
+
] iS[
]} , (9)
1
Below, Gothic letters are used to distinguish quantities representing columns, matrices etc. with respect to indices +, .
4
The corresponding tree diagrams are shown in Fig. 2. We see that these diagrams dier from those we would have
obtained applying the ordinary Feynman rules to the quantity out|
(x)
A
(x
(x, x
) = in|
(x)
A
(x
)|in in|
(x)|inin|
(x
)|in. (10)
The rst term in this denition is usually written in a symmetrical form thus rendering the function C
(x, x
) real.
However, this makes no dierence for what follows because it will be shown below that the leading low-frequency term
of the correlation function is contained entirely in its disconnected part [the second term in Eq. (10)].
We are concerned with the power spectrum of correlations in the values of the electromagnetic elds measured at
two distinct time instants (spatial separation between the observation points, |x x
(x, x
) with respect to (t t
)
C
(x, x
, t
, ) =
+
_
dtC
(x, x
)e
i(tt
)
. (11)
To complete the present section, we write out explicit expressions for various pairings of the photon and scalar elds
D
D
0
, D
0
D|
m=0
,
D
++
(x, y) =
_
d
4
k
(2)
4
e
ik(xy)
m
2
k
2
i0
, D
(x, y) =
_
d
4
k
(2)
4
e
ik(xy)
k
2
m
2
i0
,
D
+
(x, y) = i
_
d
4
k
(2)
3
(k
0
)(k
2
m
2
)e
ik(xy)
, D
+
(x, y) = D
+
(y, x) . (12)
III. EVALUATION OF THE LEADING CONTRIBUTION
Evaluation of the low-frequency asymptotic of the correlation function proceeds in two steps. First, we will prove
in Sec. III A that the low-frequency asymptotic of the connected part of C
)
(k p)
2
,
which does not involve the particle mass at all. Taking into account that each external scalar line gives rise to the
factor (2
q
)
1/2
, where
q
=
_
m
2
+q
2
m, we see that the contribution of the diagram 2(g) is proportional to
1/m. Hence, on dimensional grounds, this diagram is proportional to . The same is true of all other diagrams without
internal matter lines.
The sum of diagrams (a)(e) in Fig. 2 has the following symbolic form
I
+ I
tr
, I
=
1
i
_
D
_
r
DV
_
+
,
where the superscript tr means transposition of the indices and spacetime arguments referring to the points of
observation: , + , x x
reads
I
(x, x
) = ie
2
__
d
4
zd
4
z
_
+ D
0
++
(x, z)
_
0
(z)
D
++
(z, z
0
(z
)
_
D
0
+
(z
, x
)
D
0
++
(x, z)
_
0
(z)
D
+
(z, z
0
(z
)
_
D
0
(z
, x
)
D
0
+
(x, z)
_
0
(z)
D
+
(z, z
0
(z
)
_
D
0
+
(z
, x
)
+ D
0
+
(x, z)
_
0
(z)
(z, z
0
(z
)
_
D
0
(z
, x
)
_
,
(13)
where
.
Contribution of the third term in the right hand side of Eq. (13) is zero identically. Indeed, using Eq. (12), and
performing spacetime integrations we see that the three lines coming, say, into z-vertex are all on the mass shell,
which is inconsistent with the momentum conservation in the vertex. Taking the Fourier transform of I
(x, x
),
(x, x
, t
, ) =
+
_
dtI
(x, x
)e
i(tt
)
,
the remaining terms in Eq. (13) take the form
(x, x
, t
, ) = e
2
__
d
3
q
(2)
3
d
3
p
(2)
3
a
(q)a(q +p)
_
2
q
2
q+p
e
ip
0
(t
t0)+ipx
(p, q, x x
, ) , (14)
p
0
=
q+p
q
,
where
(p, q, x x
, ) = i
_
d
3
k
(2)
3
e
ik(xx
)
(2q
+ k
)(2q
+ k
+ p
_
D
0
++
(k)D
++
(q + k)D
0
+
(k p) D
0
++
(k)D
+
(q + k)D
0
(k p)
+D
0
+
(k)D
(q + k)D
0
(k p)
_
k
0
=
. (15)
Here
q
=
_
q
2
+ m
2
is the particles energy, m, e, q
= |x
x
0
|, are such that r q 1, r
q 1, where q =
_
q
2
is the particle momentum variance (note that q is
time-independent for a free particle). To the leading order of the long-range expansion, p
, k
.
6
Let us now show that the low-frequency asymptotic of
J
is weaker than 1/. The rst and the third terms in the
integrand in Eq. (15) give rise to a contribution which is nite at = 0. We have for the third term
_
d
3
k e
ik(xx
)
D
0
+
(k)D
(q + k)D
0
(k p)
k
0
=0
=
_
d
2
o
_
0
d|k|
k
2
e
ik(xx
)
2i(k
2
)
[2(qk) i0][p
2
+ 2(pk) i0]
=
i
4|q|p
2
_
dd sin
cos + i0
=
3
2|q|p
2
.
Similarly,
_
d
3
k e
ik(xx
)
D
0
++
(k)D
++
(q + k)D
0
+
(k p)
k
0
=0
=
_
d
2
o
_
0
d|k|
k
2
e
ik(xx
)
2i(p
0
)
_
(p
0
)
2
(k p)
2
_
[k
2
i0][k
2
+ 2(qk) i0]
is also nite for all p and q = 0 [the singularity at q = 0 or p = 0 in these expressions is inessential as it is removed
by the factors q
2
and p
2
in the integral measure in Eq. (14)]. The second term in the integrand, however, leads to a
divergence at = 0. This divergence comes from integration over small |k|. Hence, it is the same as the divergence of
the integral
_
d
2
o
_
0
d|k|
k
2
(
2
+ 2m k
2
2(qk))
[
2
+k
2
i0][p
2
i0]
=
|q|p
2
q
2
+
2
+2m+|q|
_
q
2
+
2
+2m|q|
udu
2
+ u
2
i0
.
The latter integral diverges for 0 only logarithmically.
B. Low-frequency asymptotic of the disconnected part of correlation function
Let us turn to the disconnected part of the correlation function. To nd its Fourier transform, we have to evaluate
the following integral
+
_
dt in|A
(x)|ine
i(tt
)
= q
e
it
I(r, ) , (18)
where
I(r, ) =
+
_
dt
_
e
it
__
d
3
q
(2)
3
d
3
p
(2)
3
e
ipr
p
2
e
ip
0
(tt0)
b
(q)b(q +p)
_
, r = x x
0
.
Substituting
p
0
(p +q)
2
2m
q
2
2m
gives
I(r, ) = 2e
it0
__
d
3
q
(2)
3
d
3
p
(2)
3
_
p
2
+ 2pq
2m
_
e
ipr
p
2
b
(q)b(q +p) .
For a spherically-symmetric charge distribution, b(q) = (q
2
),
I is actually a function of r = |r|,
I(r, ) =
I(r, ),
and hence, averaging over directions of r, one can write
I(r, ) = 2e
it0
__
d
3
q
(2)
3
d
3
p
(2)
3
_
p
2
+ 2pq
2m
_
sin(pr)
p
3
r
(q
2
)(q
2
+ 2m)
=
me
it0
2r
_
d
3
q
(2)
3
(q
2
)(q
2
+ 2m)
_
0
d
sin sin(ur)
u
_
q
2
cos
2
+ 2m
,
u = |q| cos +
_
q
2
cos
2
+ 2m , (19)
7
where is the angle between the vectors p, q , and it is assumed that > 0. Taking u as the integration variable
yields
I(r, ) =
me
it0
8
3
r
+
_
0
dq
2
(q
2
)(q
2
+ 2m)
q
2
+2m+|q|
_
q
2
+2m|q|
du
sin(ur)
u
2
. (20)
To further transform this integral, it is convenient to dene a function (q
2
, ) according to
(q
2
, ) =
1
4
2
+
_
q
2
dz
I(r, ) =
me
it0
2r
+
_
0
d|q|
(q
2
, )
_
q
2
+ 2m
_
sin(ur)
u
u=
q
2
+2m+|q|
+
sin(ur)
u
u=
q
2
+2m|q|
_
. (22)
Finally, integrating
I by parts once more, we nd
I(r, ) =
e
it0
2r
+
_
0
d|q| sin
_
r
_
q
2
+ 2m
_
_
2cos(|q|r) +
1
r
|q|
sin(|q|r)
_
. (23)
This exact expression considerably simplies in the practically important case of low and large r. Namely, if is
such that
q
mr
0
, (24)
and also
r q 1
(and therefore, q
2
/m), then the rst term in
I turns out to be exponentially small ( e
r q
) because of the
oscillating product of trigonometric functions. Replacing sin
2
(qr) by its average value (1/2) in the rest of
I gives
I(r, ) =
e
it0
4r
2
+
_
0
d|q|
|q|
=
e
it0
(0, 0)
4r
2
=
e
it0
16
3
r
2
+
_
0
dz|(z)|
2
. (25)
Substituting the obtained expression into the dening equations (18), (10), (11), we thus obtain the following expres-
sion for the low-frequency asymptotic of the correlation function
C
00
(x, x
, t
, ) = e
i(t0t
)
e
2
16
3
r
2
+
_
0
dz|(z)|
2
__
d
3
q
(2)
3
d
3
p
(2)
3
e
ip(x
x0)
p
2
(q
2
)((q +p)
2
) ,
(26)
all other components of C
such that r, r
D
t
,
where D
t
is a characteristic linear dimension of the particle charge distribution (for instance, variance of the particle
coordinates), Eq. (26) simplies to
C
00
(x, x
, t
, ) = e
i(t0t
)
e
2
64
4
r
2
r
+
_
0
dz|(z)|
2
. (27)
8
In applications to microelectronics, varies from 10
6
Hz to 10
6
Hz, the relevant distances r are usually 10
5
cm to
10
2
cm, q /d, where d 10
8
cm is the lattice spacing, and m is the eective electron mass, m 10
27
g, hence,
0
10
10
Hz, so the conditions r d,
0
are always well-satised.
Equation (27) represents an individual contribution of a conduction electron to the electric potential uctuation.
Considering a large number of uncorrelated electrons in a sample, one should take into account that the corresponding
time instants t
0
are distributed uniformly. Because of the oscillating exponent e
i(t0t
)
, the magnitude of the total
noise remains at the level of the individual contribution independently of the number of electrons. Therefore, summing
up all contributions amounts simply to averaging over x
0
:
C
tot
00
(x, x
, )
=
e
2
64
4
||
+
_
0
dz|(z)|
2
_
d
3
x
0
r
2
r
, (28)
where is the sample volume. To visualize it, one can say that various uncompensated individual contributions
icker in various points of the sample.
It is clear from the above discussion that the distribution of the noise magnitude around the value C
tot
00
is Gaussian,
by virtue of the central limiting theorem. Thus, the quantum eld uctuations in a sample possess the above-mentioned
property 2).
Next, let us consider the case when the sample is in an external electric eld, E. Under the inuence of the external
eld, both the electron wave functions and the statistical probability distribution are changed. It turns out, however,
that in practice, the change of the wave functions is negligible. Namely, a direct calculation shows that the relative
value of the correction is of the order
q
=
2
me|E|
q
4
L
,
where L is the smallest linear dimension of the sample. Using the above estimates for q, L in the condition
q
1
gives |E| 10
10
, in the cgs system of units. In applications to microelectronics, the eld strength is usually |E| 1,
so
q
10
10
. On the other hand, the relative change of the statistical distribution function, given by the kinetic
theory, is of the order
s
=
e|E| l
,
where l is the electron mean free path, and its mean energy,
2
/md
2
.
s
is generally not small. Furthermore,
the statistical distribution is generally analytic in E in a vicinity of E = 0, and hence the leading correction to the
scalar quantity C
00
is proportional to E
2
[property 3)].
Because of collisions with phonons and impurities in the crystal, evolution of the conduction electrons usually cannot
be considered free. It is important, however, that in view of the smallness of the electron mass in comparison with
the mass of the lattice atoms, these collisions may often be considered elastic. In such collisions, the electron energy
is not changed, and therefore, so is time evolution of the electron wave function. Hence, the above results concerning
dispersion of the electromagnetic eld uctuations remain essentially the same upon account of the electron collisions,
except that now they must be expressed in terms of the electron density matrix, rather than wave function. Denoting
the momentum space density matrix of the electron by (p
2
, q
2
), Eq. (28) thus takes the form
C
tot
00
(x, x
, )
=
e
2
0
16
2
||
_
d
3
x
0
r
2
r
,
0
1
4
2
+
_
0
dz(z, z) . (29)
The quantity denoted here by
0
is nothing but the expectation value of the inverse particle momentum:
0
=
_
d
3
q
(2)
3
(q
2
, q
2
)
|q|
=
_
1
|q|
_
.
Hence, by the order of magnitude,
0
1/ q (in the ordinary units,
0
/ q.)
In practice, one is interested in uctuations of the voltage, U, between two leads attached to a sample. Using the
above results, it is not dicult to write down an expression for the voltage correlation function, C
U
(x, x
, ). We
have
in|U(x, x
, t)|inin|U(x, x
, t
)|in = in|A
0
(x, t) A
0
(x
, t)|inin|A
0
(x, t
) A
0
(x
, t
)|in
= in|A
0
(x, t)|inin|A
0
(x, t
)|in +in|A
0
(x
, t)|inin|A
0
(x
, t
)|in
in|A
0
(x
, t)|inin|A
0
(x, t
)|in in|A
0
(x, t)|inin|A
0
(x
, t
)|in . (30)
9
Fourier transforming and applying Eq. (27) to each of the four terms in this expression, we obtain the low-frequency
asymptotic of the overall voltage uctuation across the sample
C
tot
U
(x, x
, )
=
e
2
0
G
16
2
||
, (31)
where
G
_
d
3
x
0
_
1
r
3
+
1
r
3
1
r
2
r
1
r
2
r
_
. (32)
Let us discuss the role of the sample geometry in somewhat more detail. Consider two geometrically similar samples,
and let n be the ratio of their linear dimensions (see Fig. 3). Such samples are characterized by the same value of
the G-factor. Indeed, the voltage across each sample is measured via two leads attached to its surface. Hence, the
radius-vectors of the leads drawn from the center of similitude scale by the same factor n, and therefore,
_
2
d
3
x
0
r
2
r
=
_
n
3
1
d
3
x
0
|nx x
0
|
2
|nx
x
0
|
=
_
1
n
3
d
3
(x
0
)
|nx nx
0
|
2
|nx
nx
0
|
=
_
1
d
3
x
0
|x x
0
|
2
|x
x
0
|
=
_
1
d
3
x
0
r
2
r
,
and likewise for the other terms in Eq. (32). Thus, it follows from Eq. (28) that for geometrically similar samples, the
noise level is inversely proportional to the sample volume [property 1)].
It is worth also to make the following comment concerning Eq. (32). The integrand in this formula involves the
terms 1/r
3
and 1/r
3
which give rise formally to a logarithmic divergence when the observation points approach the
sample. In this connection, it should be recalled that the above calculations have been carried out under the condition
r q 1, hence, r, r
cannot be taken too small. Furthermore, one should remember that in any eld measurement
in a given point, one deals actually with the eld averaged over a small but nite domain surrounding this point,
i.e., the voltage lead in our case. Thus, for instance, the quantity A
0
(x, t) appearing in the expression (30) is to be
substituted by
A
0
=
1
L
_
L
d
3
xA
0
(x, t) ,
where
L
is the voltage lead volume. As the result of this substitution, the term 1/r
3
takes the form
1
2
L
__
L
d
3
xd
3
x
|x x
0
|
2
| x x
0
|
.
This is nite however the lead is attached to the sample. Equation (32) is recovered in the case when r, r
are much
larger than the sample size.
C. A preliminary comparison with experiment
For a preliminary comparison of the noise level given by Eq. (31) with experimental data, let us use the results of the
classic paper by Voss and Clarke [5] where the 1/f-noise in continuous Bi and Au lms was measured. The bismuth
and gold samples had dimensions 1000