Professional Documents
Culture Documents
EPA01635 Foldtani Kozlony 2000 130 2
EPA01635 Foldtani Kozlony 2000 130 2
Budapest, 2000
Fldtani Kzlny
A Magyarhoni Fldtani Trsulat Bulletin of the Hungarian Geological
folyirata Society
Budapest
ISSN 0015-542X
F tmogat Sponsors
MOL Hungarian Oil and Gas Co., Budapest
M O L Magyar Olaj- s Gzipari Rt., Budapest
PIROS Olga, 1443 Budapest, Pf. 106. Olga PIROS, 1443 Budapest, PO. box 106.
Fldtani Kzlny is abstracted and indexed in GeoRef (Washington) Pascal Folio (Orleans)
Zentralblatt fr Palontologie (Stuttgart), Referativny Zhurnal (Moscow) and Geolgiai s
Geofizikai Szakirodalmi Tjkoztat (Budapest)
Fldtani Kzlny 130/2 177-192 (2000) Budapest
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178 Fldtani Kzlny 130/2
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Bevezet szavak
A ma geolgija a holnaprt"
Jnius 21
Plenris ls
IKS, .: Repositories for high-level radioactive waste in crystalline rocks, geological key questions
ORMAI, R , FRIGYESI, F.: Status of low and intermediate level radioactive waste repository programme
in Hungary
BALLA, Z . : Geological exploration for low and intermediate level radioactive waste disposal in
Hungary
TTH, Gy., HORVTH, I.: Hydrodinamics and hydrogeochemistry of the Mrgy Granite Complex
MAROS, Gy., PALOTS, ., RUSCH-FELGENHAUER, E.: Tectonic evaluation of the Mrgy Granite with
Imageo Mobile Corescan System
KOVCS, L., CSICSK, J., BERTA, Z S . : Main results of the qualification programme of the Boda Siltstone
Formation
HMOS, G . - FOLDING, G. - MAJOROS, Gy. - KONRD, Gy.: T h e role of geological research in the
qualification programme of the Boda Siltstone Formation
RKAI, P , BALOGH, ., DEMNY, A., FRIZS, I., MTH, Z . , NAGY, G.: Study of composition, diagenetic and
post-diagenetic alterations of the albitic Boda Siltstone Formation
CHIKN, G.: The role of geological mapping in radioctive waste disposal in Hungary
194 Fldtani Kzlny 130/2
Junius 22
A szekci: Geological aspects of radioactive waste disposal
BREWITZ, W : Longterm safety of underground radioactive waste repositories - key issue for research
and development
BODVARSSON, G. S.: Geological consideration for the flow and transport model of Yucca Mountains,
Nevada
D E CRAEN, M . , DELLEUZE, D., VOLCKAERT, G., SNEYERS, . , , M . : U - T h series disequilibrium studies on
Boom Clay, a natural analogue of radionuclide migration in argillaceous sediments
BIRKHUSER, E , ROTH, E , NEUF, H., STAMPFLI, G.: Application of 3D seismic for radioctive waste disposal
in the Swiss Sedimentary Site Characterization Programme for HLW disposal in sedimentary
rocks
SHESTOPALOVA, O.: Future perspective clay formations usage for hazardous waste isolation in
Carpathian Region
DURDUN, I., MARUNTEANU, C- Romanian LILW disposal - site selection, characterization and
investigation programme
ANTTILA, E : Geological disposal of nuclear waste in Finland
BRUER, V , BORNEMANN, .: Geoscientific investigations at the Gorleben Salt Dome - the potential
German repository site for radioactive waste
WOLLER, : Siting of deep geological repository in the Czech Republic: history and current situation
LALIEUX, P.: International co-operation regarding site characterization and site evaluation for
repository systems of long-lived radioactive waste
ERIKSSON, L. G.: The M D design: an integrated earth sciences and geoengineering approach to safe
geological disposal of long-lived waste
AITMATOVA, D.: Radioactive wastes disposal and ecological safety problems on the Territory of
Kyrgyzstan
MARCINKEVICIUS, V , KANOPIENE, R.: The possibilities of deep repository of radioactive waste in
Lithuania
SHESTOPALOV, V , ZAIONTS, I. O., BONDARENKO, Ya. I., STETSENKO, . D., RUDENKO, YU. F.: Structural-
geodynamical and hydrogeological zoning to reveal geological structures most perspective for
depth isolation of radioactive wastes
OPHORI, D.: Simulating large-scale groudwater flow for waste disposal purposes
KESSER, Z S . : Aquifers and mines at interacting risks: prevention principles for sedimentary
environment
TTH, J . , SHENG, G.: Using the recharge area concept as a strategy to enhance the safety of nuclear
waste disposal
LEBEDYNETS, M . , SPRYNSKY, M . : Subsurface water pollution by nitrate-ions contry-side in West Ukraine
VELICIU, S.: Consequences on the aquifers of the subterranean combustion in an oil field
KENNEDY, . , MLLER, I.: Improving ground water protection strategy by using documentes
Contaminant/Tracer Transport Rates
"A ma geolgija a holnaprt" konferencia eladsai 195
GONDI, E , LOEBEL, E.: An alternative approach for aquifer protection risk-based decision matrix
OGNIANIK, N . S., PARAMONOVA, N . K.' The problems of estimating the unsaturated zone contamination
with hydrocarbons and determining protective properties of the unsaturated zone
BOSCH, F. E , MLLER, I.: Groundwater vulnerability mapping in fissured rocks using continuously
recording, non contact, radio-frequency electromagnetic ( R F - E M ) instruments
SRs, L . , GULYS, A., OCSENS, P.: Ground geoelectrical methods in hydrogeological exploration
HAVAS-SZILGYI, E . , LIEBE, E : Problems and solutions of aquifer protection in Hungary
Zr ls
NARASIMHAN, T. N . : Protection of subsurface aquifers: a broader context
NEERDAEL, . , D E CRAEN, M . : Repositories for high-level waste in argillaceous formations geological
key questions
HALMAI, J.: Closing word
Fldtani Kzlny 130/2 197-206 (2000) Budapest
1
Lszl KOVCS - Gbor H M O S - Jzsef C S I C S K
(4 Figures)
Trgyszavak: Bodai Aleurolit Formci, telephely minsts, nagy aktivits hulladk, Magyarorszg,
vgleges elhelyezs, Rvidtv Program
Abstract
Since 1993 an extensive geological research programme has been carried out in an attempt to
characterise the BSE The aim of the programme is to prepare for the final disposal of HLW produced
at the Paks Nuclear Power Plant. At the beginning of 1999 the final report was completed the
professional results of the three-year programme (Short-Term Project). O n the basis of the
investigations done so far, there is no evidence demonstrating the unsuitability of the BSF (indicating
that no further research is necessary). Besides the introduction of the most significant facts of final
report, the article gives a brief description of the three-year-project, including the economic,
regulatory and public acceptance background, project-specific professional circumstances, and the
possibility for making further progress.
sszefoglals
1993 ta kiterjedt geolgiai kutatsi program irnyult a Bodai Aleurolit Formci megkutatsra,
aminek clja a Paksi Atomermben keletkezett nagy radioaktivits hulladkok elhelyezsnek
elksztse. 1999 elejn elkszlt a hrom ves (rvidtv) program szakmai eredmnyeket
bemutat zrjelentse. A mr elvgzett kutatsok alapjn semmi olyan bizonytk nem merlt fel,
ami kizrn a Bodai Aleurolit alkalmassgt vagy megkrdjelezn a kutatsok folytatsnak
szksgessgt. A zrjelents lnyegnek ismertetse mellett rviden lerjuk a hrom ves
programot, belertve a gazdasgi, a szablyozsi s a lakossgi elfogadsi htteret, a program
specifikus szakmai krlmnyeket s az elrelpsi lehetsgeket.
Introduction
1
MECSEKRC Environmental, Pcs, Esztergr L. str. 19. H-7633, Hungary e-mail:
< surename > < forename > @mecsekerc.hu
198 Fldtani Kzlny 130/2
-p| 1 Boda Siltstone Fornation (claystone, slltstone Underground Research Laboratory in BSF
with thin layers of dolonltlc narl, dolonite> a t the level of-700 n (not in scale)
T h e plan for the Short-Term Project was prepared in co-operation with AECL.
Its main aim is to provide essential information for answering the following
questions:
- Geological evolution (sedimentation, diagenetic and post-diagenetic
processes, tectonic history, etc.).
- Geometrical suitability, homogeneity, possibility of spatial extrapolation of
the results.
- Primary isolation capabilities of the formation.
KOVCS, L. et al: Actual state of the site characterisation programme of the Boda Fm 201
Fig. 2 Map of the exploring tunnels and more important underground boreholes of URL
LEGEND:
Fig. 3 Geological cross-section in the vertical plane of the Alpha-1 exploratory tunnel
c o m p l e t e d during the second half of last year. It consists of 9 Volumes (about 1600
pages in total). T h e following sections provide brief information on the key issues
of this report.
Geological evolution
Geometric suitability
Geotechnical features
Fig. 4 Geometry of the installed measuring devices in the Complete Instrumental Array
Conclusion
1 1
W e r n t B R E W I T Z - Ulrich N O S E C K
(3 figures)
Key words: radioactive waste, repositories, safety concepts, long-term safety assessment
Abstract
Concepts for the final disposal of radioactive waste include, among others, disposal in under
ground cavities and, in specific cases, disposal in deep geological formations. In several countries
provisions have been made in the national regulatory framework for the adoption of such waste
disposal concepts. The basic idea is to isolate waste from ground surface and meteoric water as long
as required for the sustainable preservation of the environment. T h e time-frame depends on the
toxicity of the radioactive materials as well as on durability of the waste containers. Both are essential
parameters for the selection of appropriate underground cavities or deep geological strata for the
construction of such repositories. One of the most challenging tasks for scientists and engineers is to
forecast the long-term behaviour of the repository and the assessment of potential adverse conditions
on the basis of sound geological data and realistic evolution models (scenarios).
For very good reasons many countries are pursueing radioactive waste disposal in deep geological
formations. The principal advantage is that deep repositories are covered by thick geological barriers,
in many cases with separated aquifers and without effective hydraulic pathways which could be
potential travelling ways for toxic substances. That means that under normal conditions the isolation
capacity of deep repositories should be in the range of geological time-frames. Potential host rocks are
granite, rock salt, argillaceous rocks and others, depending on favourable site-specific conditions.
With respect to the operational safety rock mechanic aspects are the most important factors. This
is w h y various parameters, such as rock stresses and tensile strength, have to be investigated. In
addition, field measurements may help to characterise the rock mass stability and the changes which
may be induced by the repository. For post-operational safety hydrogeological and geochemical
research is mainly needed in order to produce data on radionuclide mobilisation and groundwater-
transport. These are input parameters for generic as well as site-related performance assessment
models. An engineering task is the development of adequate backfilling and sealing measures for the
underground cavities and the access shafts. In Germany a comprehensive R & D programme has been
devised to cover these issues. The main objective is to improve both the data-base and methodology
for the long-term safety assessment of underground waste repositories.
1
Gesellschaft fr Anlagen- und Reaktorsicherheit (GRS) mbH, Repository Safety Research Divison,
38011 Braunschweig, Postfach 2126
208 Fldtani Kzlny 130/2
sszefoglals
A radioaktv hulladkok vgs elhelyezsre irnyul tervek kztt - egyb megoldsok mellett -
fldalatti regek, s klnleges esetekben mlysgi fldtani kpzdmnyek is szerepelnek. A nemzeti
jogszablyozs keretben tbb orszgban ilyen hulladkelhelyezsi koncepcit fogadtak el. Az
alapgondolat az, hogy a hulladkot mindaddig elszigeteljk a felszntl s a csapadktl, amg azt a
krnyezet vdelme megkveteli. A szksges id hossza a radioaktv anyagok mrgez tulaj
donsgtl s a hulladktartlyok tartssgtl fgg. Mindkett fontos tnyez a trol ptshez
megfelel fldalatti regek vagy felsznalatti fldtani kpzdmnyek kivlasztsban. A tudsok s a
mrnkk szmra az egyik legnagyobb kihvs a trol hossztv viselkedsnek elrejelzse s a
lehetsges kedveztlen esemnyek becslse a fldtani adatok s a fejldsi modellek alapjn.
Jl rthet okokbl szmos orszg trekszik a radioaktv hulladkok mlyen fekv fldtani
kpzdmnyekben val elhelyezsre. Lnyeges elny, hogy a mlysgi trolkat vastag fldtani gt
fedi, sok esetben elklnl vzad rteggel, s nincsenek hatkony ramlsi plyk, amik egyben a
mrgez anyagok lehetsges szlltsi tvonalai lehetnnek. Ez azt is jelenti, hogy normlis
krlmnyek kztt a felsznalatti trolk szigetel hatsa fldtani idkben mrhet. A lehetsges
befogad kzetek kztt van a grnit, a ks, az agyagok s a telephely sajtos krlmnyeitl
fggen ms kzetek.
A biztonsgos zemeltets szempontjbl a kzetmechanikai jellegek a legfontosabbak, ezrt meg
kell hatrozni a kzetfeszltsget s a hzszilrdsgot. A terepi mrsek hozzsegthetnek a kzet
stabilitsnak, s a tervezett trol ltal ltrehozott vltozsoknak a jellemzshez. Az zemeltets
utni biztonsgossghoz a hidrogeolgiai s a geokmiai kutats a legszksgesebb, mivel ezekbl a
radioaktv elemvndorlsrl s a talajvzmozgsrl nyernk adatokat, amik az ltalnos s a
telephelykzeli modellek bemen adatai. Mrnki feladat a fldalatti regek s az aknk megfelel
tmedkelse s a zrrtegek kiptse. Nmetorszgban tfog K&F (Kutatsi s Fejlesztsi)
program kszl ezeknek a problmknak a megoldsra. A f cl a felsznalatti trolk hossztv
biztonsgi becslsnek alapjul szolgl adatbzis s a mdszertan fejlesztse.
Introduction
In G e r m a n y rock salt was selected as a ' d r y ' disposal formation for all
categories of radioactive waste at a very early stage of t h e G e r m a n waste
m a n a g e m e n t programme. T h e first experiences with LLW/ILW-disposal were
m a d e in the ASSE salt m i n e in 1972 - 1977 (GSF 1982). For ILW a special disposal
technique for 200 1 drums without over-packs w a s developed a n d tested. A total
of about 1300 drums containing an inventory of 5 000 T B q , mainly of short-lived
3
radionuclides, was emplaced in rock salt in a small c h a m b e r of about 9000 m and
p e r m a n e n t l y sealed off from the mine workings. The m a x i m u m surface dose rate
of t h e d r u m s was about 30 Sv per hour a n d was mainly caused b y Cobalt 60. This
radiation level required transport a n d handling techniques to b e carried out
u n d e r p e r m a n e n t radiation shielding. T h e LLWALW-disposal operation in t h e
ASSE-mine w a s terminated in 1977. With respect to operational safety, the
following results can be given:
- t h e ILW-drums w e r e safely e m p l a c e d b y routine o p e r a t i o n s while a
p e r m a n e n t radiation shield was maintained,
- t h e radiation exposure of the staff was v e r y low c o m p a r e d with that of t h e
e m p l a c e m e n t of unshielded LLW-Drums,
- within 2 0 years of p e r m a n e n t emplacement the concentration of hazardous
c o m p o n e n t s in t h e chamber's atmosphere remained far below a n y set safety limit,
- the radiation level decreased as expected from the half-lives of the radio
nuclide inventory.
With respect to the post operational safety of radioactive waste disposal in rock
salt several case studies were performed within the scope of national and
i n t e r n a t i o n a l R & D - p r o j e c t s (BUHMANN et al. 1995; BUHMANN 1996; HIRSEKORN et al.
1991; STORCK et al. 1988). In the PAGIS-project (co-funded b y the EU) different
host rock formations were evaluated for their isolation potential for H L W
(STORCK et al. 1988). In t h e PACOMA project the long-term effects of conceptual
u n d e r g r o u n d repositories for intermediate-level and a - c o n t a m i n a t e d wastes
w e r e c o m p a r e d with those of HLW-repositories (HIRSEKORN et al. 1991). T h e
calculated radionuclide release into the biosphere, as a c o n s e q u e n c e of a brine
7
intrusion scenario, resulted in a dose rate of about 10" Sv/year a n d n o release for
HLW repositories. If, shortly after operation, a considerable n u m b e r of disposal
c h a m b e r s a n d drifts is affected b y brine intrusion the total dose rates for both will
4 6
be in t h e range of 1 0 " to 1 0 " Sv/year. With reference to t h e long-term
c o n s e q u e n c e s o f H L W a n d spent fuel disposal in rock salt a n u m b e r o f sensitivity
BREWITZ, W. & NOSECK, U.: The long-term safety of underground waste repositories 211
Fig. 1 Schematic concept of a repository for HLW, spent fuel and ILW in salt formations
cast iron and normal 5 ft and 10 ft containers have b e e n selected for LLW and
2
ILW. The containers will be emplaced in 40 m wide drifts by m e a n s of the
stacking technique. T h e remaining open space will be backfilled before the drifts
are sealed off.
The long-term safety assessment of the repository is based on a hydro-
geological m o d e l covering an area of 40 km from north to south and 14 k m from
east to west (STORCK 1988). The hydraulic rock parameters and, in particular, the
rock mass conductivity were either directly measured or determined from
geological analogues. From the experiences gained in the K O N R A D m i n e itself
and in the entire mining district of Salzgitter, it was concluded that a considerable
water intrusion will not occur during the operational phase. After s h u t d o w n the
repository will slowly be filled with high saline, deep groundwater and this will
take up to several thousand years. O n l y then will the regional groundwater flow
b e c o m e effective again, but at a greater depth. Due to the uniform geological
structure and the absence of deep cutting tectonic faults only three possible
pathways w e r e identified for radionuclide transport (these are s h o w n in Fig. 2).
After s h u t d o w n of the repository the total radionuclide inventory will a m o u n t to
6
1 0 TBq, of which 9 7 % will be beta/gamma- and 3% alpha-emitters. Iodine-129
amounts to 0.15 TBq. Although the density of the high saline g r o u n d w a t e r was
not taken into account, the calculated groundwater travelling times ranged from
0.3 to 1.1 million years. T h e calculation of individual doses as a function of time
224 Fldtani Kzlny 130/2
p r o v e d that for up to 10 000 years and more there will be no contamination of the
biosphere. Hypothetical calculations for individual radionuclides revealed that
after more than 300 000 years I o d i n e - 1 2 9 could cause some m i n o r exposure in a
r a n g e w h i c h is a natural level of exposure to man.
It has to be stressed that due to the most favourable site conditions, the great
d e p t h a n d the almost complete lack of groundwater in the mine, major side
effects will not occur. In particular, the corrosion of containers a n d waste is of no
great importance in the operational phase of the repository. In the post-
operational phase corrosion gases (which m a y be generated as a c o n s e q u e n c e of
w a t e r seepage into the disposal drifts) can migrate along the excavation damage
zone so that no gas pressure build up has to be considered. This m a y be
completely different at other sites with larger volumes of g r o u n d w a t e r present or
freely available from adjacent rock masses. However, for a repository taking
advantage of the 'dry' site conditions, adequate backfilling and sealing measures
in drifts a n d shafts are of utmost importance in order to preserve these
conditions for as long as required.
Summary
References
BALTES, . 1995: Sicherheitskriterien fr Endlager, ATW, 9 5 / 3 .
BfS 1995: Morsleben Erfahrungen, Morsleben-Info, 3 .
BRENNECKE, E, KUGEL, K. & NOACK, W. 1997: Endlagerungsbedingungen Morsleben, ATW, 4.
BUHMANN, D., BRENNER, J. & STORCK, R. 1995: Long Term Safety Assessment of Disposal Concepts for
HLW and Spent Fuel in Rock Salt. - In: Proc. of the Fifth International Conference on Radioactive
Waste Management and Environmental Remediation (ICEM), Berlin, 03-09. 09. 1995, 617-623,
Berlin.
BUHMANN, D. 1996: Relevance of near field and far field effects to the release of radionuclides from
repositories with low level waste. - Intern. Symp. on Experience in the Planning and Operation
of Low Level Waste Disposal Facilities, 405-416, IAEA, Vienna, 17-21. June.
BUHMANN, D., NIES, A. & STORCK, R. 1991: Analyse der Langzeitsicherheit von Endlager-konzepten fr
wrmeerzeugende radioaktive Abflle. - GSF-Bericht 2 7 / 9 1 . GSF - Forschungszentrum fr
Umwelt und Gesundheit mbH, Braunschweig.
DECAMPS, F. 1996: Overview of radwaste repositories in Europe. - Nuclear Europe Worldscan, 3/4.
EBEL, . 1991: Das Endlager Morsleben fr LLW und MAW, ATW, 1 1 .
GSF 1982: The Asse Salt Mine - Research for the Final Disposal -, GSF Mnchen.
HIRSEKORN, R.-E, NIES, A., RAUSCH, H. & STORCK, R. 1991: Performance Assessment of Confinements for
Medium-Level and Alpha-Contaminated Waste (PACOMA), Rock Salt Option, EUR 13 634 EN. -
GSF-Bericht 1 2 / 9 1 , Kommission der Europischen Gemeinschaften, GSF-Forschungszentrum fr
Umwelt und Gesundheit GmbH, Brssel-Luxemburg.
IAEA 1991: Shallow Ground Disposal of Radioactive Wastes. A Guidebook. - Safety series 5 3 , Vienna.
LHRMANN, L . , NOSECK, U., STORCK, R. 2000: Spent Fuel Performance Assessment (SPA) for a
Repository in Crystalline Formations in Germany, GRS Nr-154, Gesellschaft fr Anlagen- und
Reaktorsicherheit mbH, Braunschweig.
PAPP, R. 1997: GEISHA - Gegenberstellung von Endlagerkonzepten in Salz und Hartgestein. FZKA-
PTE Nr. 3, Forschungszentrum Karlsruhe GmbH, Karlsruhe.
Posiva O y 1996: Nuclear Waste Management of Olkiluoto and Loviisa Power Plants, annual review.
RTHEMEYER, H. 1994: Langzeitsicherheit von Endlagern, ATW, 2 .
STORCK, R. 1988: Performance Assessments for the Disposal of Low-level Wastes into an Iron-Ore
Formation. - In: Near Field Assessment of Repositories for Low and Medium Level Waste,
Proceedings of an NEA/OECD Workshop, Organization for Economic Co-Operation and
Development, Paris.
STORCK, R. & PREUSS, J. 1997: Langzeitsicherheitsnachweis fr das erste bundesdeutsche Endlager
Morsleben, Felsbau, 1 5 / 6 .
STORCK, R., ASCHENBACH, ] . , HIRSEKORN, R.P, NIES, A. & STELTE, N. 1988: Performance Assessment of
Geological Isolation Systems for Radioactive Waste (PAGIS): Disposal in Salt Formations. EUR 11
778 EN GSF-Bericht 23/88. Commission of the European Communities, Gesellschaft fr Strahlen-
und Umweltforschung mbH Mnchen, Brussels-Luxembourg.
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WITHERSPOON, P A . 1996: Geological Problems in Radioactive Waste Isolation, LBNL-38915, UC-814.
Fldtani Kzlny 130/2 219-228 (2000) Budapest
1 1 1
M i e k e D E C R A E N - D o m i n i q u e D E L L E U Z E - Geert V O L C K A E R T -
1 1
Alain S N E Y E R S - Martin P u t
(4 Figures, 1 Plate)
Key words: natural analogue, argillaceous formation, U-Th series disequilibrium studies
Abstract
In 1996 the Belgian Nuclear Research Centre ( S C K ' C E N ) started a natural analogue study on
Boom Clay. T h e aim of this study is to increase confidence in the barrier function of argillaceous
sediments by investigating long-term geological processes. A detailed mineralogical and geochemical
investigation enables a study to be made of the natural distribution of the uranium and thorium in
the clay deposit. U-Th series disequilibrium studies are applied to study the mobility of U-Th-Ra
isotopes in Boom Clay. The first results indicate that variations in U-Th concentration are mainly
primary in origin, and relate to lithological variations. No indication for radionuclide mobility has
been observed in Boom Clay, with the exception of one layer with a coarser grain size, and therefore,
it is a zone of potentially higher permeability and pore water mobility.
sszefoglals
A Belga Atomkutat Kzpont ( S K C ' C E N ) 1996-ban kezdett bele a termszetes analgia kutatsba
a Boomi Agyagban. A kutats clja az agyagos ledkek gtknt val viselkedsnek tovbbi
megerstse hossz tv geolgiai folyamatok tanulmnyozsa ltal. A rszletes svnytani s
geokmiai kutats lehetv teszi az urn s a trium termszetes eloszlsnak tanulmnyozst az
agyagban. A nemegyenslyi U-Th sorozat tanulmnyozsa lehetv teszi az U-Th-Ra izotpok
mozgsnak megfigyelst a Boomi Agyagban. Az els eredmnyek arra utalnak, hogy az U-Th
koncentrcikban fellp eltrsek elsdlegesen a kzet keletkezsekor jnnek ltre, s kzettani
vltozatokhoz kapcsoldnak. A Boomi Agyagban nincs jele radioaktv elemvndorlsnak, egy
durvbb szemcsemret, valsznleg permebilisabb s prusvzzel tjrt rteg kivtelvel.
Introduction
1
Belgian Nuclear Research Centre ( S C K ' C E N ) Waste and Disposal Department, Boeretang 200,
B-2400 Mol - Belgium
220 Fldtani Kzlny 130/2
Photo 1 Cyclic alternation of silry clays and clayey silts. Boom Clay quarry at Rumst, 30 km north of
Brussels
1 foto Kzetlisztes agyag s agyagos kzetliszt ciklikus vltakozsa a Boomi Agyag fejtsben Rumstnl,
Brsszeltl 30 km-re szakra
Fig. 1 Present-day outcrops of Rupelian Boom Clay in Belgium. To the north of the outcrops, the Boom Clay is present in the subsurface. The natural analogue
study has been performed on samples from the Mol-l borehole where the Boom Clay is present at a depth of 190 to 293 m
1. bra A rupeli Boomi Agyag jelenlegi felszni elfordulsa Belgiumban. A feltrstl szakra a Boomi Agyag a felszn alatt tallhat. A termszetes analgia kutatst a Mol-l
frs mintin vgeztk, ahol a Boomi Agyag 190-293 m-ben tallhat
222 Fldtani Kzlny 130/2
Methods
Putte
Member
lerhagen
Mpmhfir
Belsele-Waas qq
Member
Ruisbroek
sands
U (ppm)
. Th (ppm)
U-Th series disequilibrium studies have been performed to study the mobility
of natural U and Th in the B o o m Clay on a geological time scale. The
radiochemical da'ta of the solid samples of the M o l - l borehole are presented in
Figure 3. T h e error bars in the figure represent 2 a standard deviation un
certainties due to counting statistics only.
In the entire B o o m Clay profile, the 234TJ/238TJ t i v i t y ratios are all close to
ac
2 3 4
unity within the 2 a uncertainty, although there might be some evidence for U
2 3
excess in some samples. The 234TJ/238TJ data are c o m p l e m e n t e d b y the ^ T h / ^
activity ratios; these are generally indicative of radiometric equilibrium although
2 3 0 2 3 4
some ratios are rather low (ratios b e t w e e n 0.8 and 1). S u c h low T h / U activity
ratios are indicative of 'geologically recent' U uptake from the pore water,
2 3 4
m e a n i n g that local mobile U has b e e n immobilised. The U excess in these
precipitates can be explained by a-recoil. Pore water is often characterised by
2 3 4
U excess as a result of a-recoil, either by recoil injection into surrounding fluids
or by injection into neighbouring solids, followed by leaching (FLEISHER 1988).
After the uranium has been immobilised, the precipitate will be in equilibrium
2 3 4 2 3 8
with the pore water, and h e n c e it will also have U / U activity ratios > 1.
2 2 6 2 3 0
From the R a / T h activity ratios, it is apparent that Ra isotope mobility in
B o o m Clay is considerably more widespread than that of U. Although the
2 2 6 2 3 0
uncertainties of Ra activities are rather large, significant variations in R a / T h
2 3 8 2 3 2
Fig. 3 Isotope activity ratios for isotopes of the U and T h decay chains in solid samples of the Mol-1 borehole ( S C K ' C E N domain, Mol, Belgium)
2 38 232
3. bra Az l - s Th bomlsi sor izotpjaira vontakoz izotp aktivitsi arny a Mol-1 frs szilrd kzetmintiban (SCK'CEN kutatsi terlet, Mol, Belgium)
D E C/MEN, M. et al: U-Th series disequilibrium studies on Boom Clay 225
Conclusions
13 Z31
4. bra U-Th koncentrci a Putte Tagozat bzisnl tv U-gazdag intervallum szilrd mintiban (Mol-1. frs) s a "U , Th hasadsi sor izotp/ra vonatkoz,
kapcsold izotp aktivitsi hnyados.
DE CRAEN, M. et ai: U-Th series disequilibrium studies on Boom Clay 227
the B o o m Clay, at least for the last million years. O n e exception is present in the
'double band' which consists of two silty layers, and which is a z o n e of higher
permeability and pore water mobility. This probably caused the preferential
2 3 0 2 3 4
leaching of uranium and radium, as indicated by the T h / U and ^ R a / ^ T h
isotope activity ratio, which is significantly larger than 1 a n d smaller than 1
respectively.
In the Eigenbilzen Formation and the Ruisbroek sands, aquifers over- and
underlying the B o o m Clay, respectively, there is some evidence of Ra mobility.
This m a y be a result of pore water mobility and associated leaching of radio-
nuclides in the aquifers.
This study gives a general picture of the distribution and mobility of U and Th
in the B o o m Clay. A next step is the investigation of separated mineral phases, in
order to b e able to understand better the distribution and mobility of U and Th
on a microscale. Chemical sequential leaching separation will result in different
phases (e.g. ion-exchangeable, absorbed, crystalline, a m o r p h o u s Fe/Mn oxides,
a n d resistant), from w h i c h the isotopic distribution can b e s u b s e q u e n t l y
m e a s u r e d . T h e latter will b e refined b y additional m i n e r a l o g i c a l a n d
p e t r o g r a p h i c a l investigation a n d associated m i c r o - a n a l y s i s (e.g. optical
microscopy, S E M , B S E M , E D X ) . Together with the results of the pore water
analyses, these data should enable to better understanding of the distribution
a n d mobility of U and Th in the B o o m Clay.
Acknowledgements
References
CUTTELL, J. C . 1 9 8 3 : Application of uranium and thorium series isotopes to the study of certain British
aquifers. - University of Birmingham, Unpublished PhD Thesis in Geology, 2 6 9 p.
FLEISHER, R. L . 1 9 8 8 : Alpha-recoil damage: Relation to isotopic disequilibrium and leaching of
radionuclides. - Geochim. Cosmochim. Acta 5 2 , 1 4 5 9 - 1 4 6 6 .
IVANOVICH, M . & MURRAY, A. 1 9 9 2 : Spectroscopic methods. - In: IVANOVICH, M . & HARMON, R. S. (Eds):
Uranium-series disequilibrium: Applications to Earth, Marine, and Environmental Sciences. Second
edition Chap. 5 , 1 2 7 - 1 7 3 . Clarendon Press, Oxford.
LALLY, A.E. 1 9 9 2 : Chemical procedures. - In: IVANOVICH, M . & HARMON, R. S. (Eds): Uranium-series
disequilibrium: Applications to Earth, Marine, and Environmental Sciences. Second edition Chap. 4 ,
9 5 - 1 2 6 . Clarendon Press, Oxford.
VANDENBERGHE, N. 1 9 7 8 : Sedimentology of the Boom Clay (Rupelian) in Belgium. - Verhand. Kon. Acad.
Wetenschappen Blgi 4 0 , 1 4 7 , 1 3 7 p.
VANDENBERGHE, N. & VAN ECHELPOEL, E. 1 9 8 7 : Field Guide to the Rupelian Stratotype. - Bulletin van de
Belgische Vereniging voor Geologie 9 6 / 4 , 3 2 5 - 3 3 7 .
228 Fldtani Kzlny 130/2
1 2
Ion D U R D U N - Cristian M R U N T E A N U
(3 Figures)
Key words: Low and intermediate level radioactive waste, surface repository, geological barrier,
site investigation
Kulcsszavak: kis- s kzepes radioaktivits hulladk, felszni trol, fldtani gt, telephely kutats
Abstract
The first reactor of the Cernavoda N P P was commissioned in 1996, but the radioactive waste
programme started in 1992. Geological investigation works have been initiated to select and describe
the location for a low and medium radioactive waste final disposal facility. The selection of a surface
repository type has taken into consideration the experience of other countries, such as France and
Spain, whose positive practice in this field is applicable in Romania as well. IAEA guidelines were also
used in this process. The site selection process included 37 potential sites, 2 - 3 candidate sites and one
preferred site (Saligny) and was based on specific criteria: lithological, tectonical, seismological,
hydrogeological, climatic, transport facilities and public acceptance (DURDUN & MARUNTEANU 1997).
Starting in 1996, a complex and detailed site and laboratory investigation programme has been in
progress with the purpose of determining the characteristics of the site and selecting the best area for
the construction of the disposal units.
sszefoglals
A Cernavoda Atomerm els reaktort 1996-ban helyeztk zembe, de a radioaktv hulladk
program mr 1992-ben elkezddtt. A fldtani kutats clja a kis- s kzepes radioaktivits
hulladkok vgs elhelyezsre szolgl telephely kivlasztsa s jellemzse volt. A felszni tpus
trolra m s orszgok, pl. Franciaorszg s Spanyolorszg tapasztalatainak figyelembevtelvel esett
a vlaszts, akiknek az ilyen terleten szerzett gyakorlata Romniban is alkalmazhat. Az eljrs
sorn a Nemzetkzi Atomenergia gynksg irnyelveit kvettk. A telephely kivlasztsakor 37
esetleges helysznt, 2 - 3 lehetsges helysznt s egy alkalmas objektumot (Saligny) vlasztottak ki
specilis kritriumok - kzettan, tektonika, szeizmolgia, hidrogeolgia, klma, szlltsi lehetsgek
s lakossgi elfogads - alapjn (DURDUN & MARUNTEANU 1997). Az 1996-ban elkezddtt komplex s
rszletes telephely- s laboratriumi vizsglat programnak az a clja, hogy meghatrozza a telephely
jellegzetessgeit s kivlassza a trolhely megptshez legmegfelelbb terletet.
1
Institute for Geotechnical and Geophysical Studies - GEOTEC Bucharest, Str. Vasile Lascar,
No. 5-7, 70211, Bucharest, Romania, e-mail: geotec@pcnet.ro
2
University of Bucharest, Str. Traian Vuia, No. 6, 70139, Bucharest, Romania, e-mail:
cristian@gg.unibuc.ro
230 Fldtani Kzlny 130/2
Introduction
Disposal system
Site selection
DOBROGEA REGION
G E N E R A L F I E L D INVESTIGATION 1 9 9 3 - 1 9 9 4
3 drillings 1-2 refraction sections
H laboratory tests, chemical a n d d e u t e r i u m analyses
C O L L A B O R A T I O N : I.N.R. PITESTI, B U C H A R E S T UNIVERSITY, C I T O N ( R E N E L P R O G R A M M E
g C O O R D I N A T O R ) . I.T.I.M. CLUJ
DETAILED INVESTIGATIONS 1 9 9 7 - 1 9 9 8
Fig. 171LW near surface repository for the Cernavoda NPP Geotec Investigation Programme
1. bra A Cernavodai Atomerm kis- s kzepes aktivits radioaktiv hulladknak felsznkzeli trolsra
vonatkoz Gcotechnikai Kutatsi Programja
232 Fldtani Kzlny 130/2
Hydrogeology
Unsaturated zone:
- water infiltration in natural and compacted loessoid soil by lisimetric
measurement;
- permeability tests in boreholes and laboratory tests;
- suction tests on borehole samples.
Saturated zone:
- 50 drillings in the area for the identification of local aquifers and a main
aquifer;
- permeability tests on each borehole;
- chemistry of the groundwater;
- 5 drillings for the measurement of the groundwater level in local aquifers;
- 3 drillings for Eocene aquifer;
- 5 specially equipped drillings measuring for the groundwater level in the
main aquifers;
- estimation of groundwater flow velocity and direction;
- the inventory of water users;
Geoengineering
Ftg. 3 Variation of some physical parametes of the geological formation and of the distribution coefficient for specific radionuclides in the drilling FC23
3. bra A fldtani kpzdmnyek nhny fizikai paramternek s nhny radioaktv izotp eloszlsi egytthatjnak vltozsa az FC23-as frsban
DURDUN, I. & MRUNTEANU, : Romanian LILW disposal 235
Computational modelling
LEGEND
1 - Unsaturated zone II - Saturated zone
a - loess 2 middle S = 0.2-0.4 prequaternary clays with sand lenses
3 lower S = 0.8 III - Main aquifer - barremian limestone
b - quaternary- red clay S = 0.9-1.0 Compacted loess effect (3 m thickness)
- prequaternary clays Natural conditions
GV/L Underground water level
5. bra A H szennyezds
3 maximlis elterjedse a Saligny telephelyen (CHAIN-ID software, keresztmetszet)
DURDUN, I. & MRUNTEANU, : Romanian LILW disposal 237
Conclusions
R a t h e r t h a n c o n c l u s i o n s , o n e result o f o u r r e s e a r c h w h i c h h a s to b e
e m p h a s i s e d is that the behavior of the geological e n v i r o n m e n t as geological
barrier must be considered an important criterion of acceptance for the facilities
of a LILW repository.
Reference
DURDUN, I., MARUNTEANU, C . & GHEORGHE, A. 1 9 9 7 : O n the radioactive waste final disposal in
geological formations from Romania. Proceedings International Symposium "Engineering
Geology and the Environment", Athens, Greece, June 2 3 - 2 7 , 1 9 9 7 , 1 7 9 9 - 1 8 0 3 , A. A. BALKEMA,
1997.
Fldtani Kzlny 130/2 239-249 (2000) Budapest
1
Philippe L A L I E U X
Abstract
This general paper is principally aimed at providing examples of O E C D Nuclear Energy Agency
initiatives in the field of the characterisation and evaluation of potential sites for the geological
disposal of long-life radioactive waste. The examples focus on the geoscientific aspects of geological
disposal and the added value of addressing them in an international context. Most of the initiatives
chosen have resulted, or will soon result, in open publications. Following introductory information
on the O E C D Nuclear Energy Agency, the paper also presents an overview of some of the key
challenges that are, or will have to be, faced in the implementation of the geological disposal of long-
life waste.
sszefoglals
This paper does not intend to detail all actual and potential, technical and non
technical challenges that are, or will have to be, faced in the various decision
m a k i n g and implementing steps of geological disposal. However, in order to put
the specific geoscientific aspects of disposal into perspective, it is worthwhile
summarising some of these k e y challenges.
In recent years, waste m a n a g e m e n t programmes have focused on the technical
aspects of deep underground disposal of long-life radioactive waste. Today, a
c o n s e n s u s exists b e t w e e n experts in various countries w h i c h accepts that that
sites can be properly identified a n d characterised, that geological repositories can
be designed so that no short-term detriment to populations will result from the
waste disposal, and that an acceptable level of safety is provided for times far into
the future (OECD/NEA 1991, 1999a). There also exists a consensus, a m o n g the
experts, that the current generation, which has benefited from the nuclear energy
produced, should provide future generations with the m e a n s to dispose of the
waste p e r m a n e n t l y ( O E C D / N E A 1995). R e c e n t setbacks in disposal p r o g r a m m e s
have not b e e n based on technical arguments, but rather political and societal
aspects. T h e waste m a n a g e m e n t c o m m u n i t y must therefore find n e w w a y s to
address the concerns of all stakeholders in the repository d e v e l o p m e n t process.
A m o n g the general strategic challenges linked with the above consideration are
the following:
- the establishment of, and confidence-building in the entire step-wise process
of decision-making; this should take into account technical aspects of repository
d e v e l o p m e n t a n d more qualitative arguments, as well as consider the active
i n v o l v e m e n t of all stakeholders, including the general public;
- the assessment of the place of waste disposal within the broader debate on
environmental and sustainability issues, including the demonstration that safe
and environmentally acceptable strategies can be applied;
- the comparison of the principles of radioactive and non-radioactive waste
m a n a g e m e n t and of the evaluation of their impacts; and
- the evaluation of the impact of financial pressures on waste m a n a g e m e n t
p r o g r a m m e s - e.g. due to deregulation of electricity markets - as well as the
impact of waste m a n a g e m e n t on the continued e c o n o m i c sustainability of
nuclear power.
From a more technical point of view, some of the k e y challenges could be
synthesised as follows:
- the establishment of technical confidence in long-term safety assessment in
the presence of uncertainties inherent in natural systems and very l o n g time-
scales;
- the adequate consideration of the interfaces b e t w e e n the various natural and
m a n - m a d e c o m p o n e n t s of the repository system; and
- the appropriate consideration of site-specific geoscientific information in the
preparation of a safety case; this includes (i) the avoidance of over-conservatism
w h i c h m a y lead to the effective disregard of the geosphere as a barrier, a n d also
242 Fldtani Kzlny 130/2
to bias in the sensitivity analysis, and (ii) the use of large a m o u n t s of soft"
information*.
Introduction
* Hard" data are quantitative measurements that have a clear relationship to disposal safety-
relevant features and processes represented in assessment models (e.g. hydrogeological data from the
testing in boreholes and tunnels). Soft" data include both qualitative information (such as expert
judgement and geological experience) and also quantitative information that is either weakly
correlated to the attributes of interest in assessment models (e.g. geophysical and geochemical data),
or describes the attribute of interest through constitutive equations (e.g. hydraulic heads to hydraulic
conductivity).
LALIEUX, P.: International co-operation regarding site characterisation 243
Underground testing
The main objectives of the initiatives below are to assess the perturbation
induced in the geosphere by the repository and to promote the understanding of
the interactions with the geosphere w h e n defining repository components.
In u n d e r g r o u n d repositories for radioactive waste, significant quantities of
gases m a y be generated as a result of several processes - notably the interaction
of groundwaters and brines with waste and engineered materials placed in
disposal systems. The gases m a y migrate through the engineered barrier system
and the natural geological barrier. The potential impact of gas generation,
accumulation and migration on the long-term safety of a repository will be
d e p e n d e n t u p o n the waste types, the repository concept, the host geological
e n v i r o n m e n t and the scenarios for the long-term evolution of the system. It is
r e c o m m e n d e d that the potential impact of gas accumulation and migration on
the performance of the various barriers should be addressed and assessed in the
development of safety cases for radioactive waste repositories.
Significant efforts have been, and continue to be, expended in n u m e r o u s
national and international programmes in analysing the potential impacts of gas
in u n d e r g r o u n d repositories. In light of these efforts, and in order to help focus
further work, the European Commission and the NEA have jointly undertaken a
review of the knowledge gained so far in order to establish the current status of
the basic understanding of the topics concerned ( R O D W E L L et al. 1999). The
review report covers most underground repository concepts presently being
considered. Amongst the repository concepts that are reviewed in the report, that
for the Yucca Mountain is unique in that disposal is envisaged in unsaturated
rock in an arid region. The consequence for this concept is that two-phase flow
issues are absolutely central to repository performance analysis, and have
therefore c o m m a n d e d m o r e resources and attention than gas migration in
repository concepts developed for saturated locations. For other repository
concepts - i.e. those involving emplacement in saturated rocks - the scenarios
involving substantive gas migration issues vary in line with the repository
concept.
Argillaceous media
initiatives set up u n d e r the Clay Club auspices help to assess the commonalities
a n d differences b e t w e e n various argillaceous formations; t h e r e f o r e , t h e y
facilitate the transferability of the information gained - notably in u n d e r g r o u n d
testing facilities - and foster international and multilateral co-operation.
A m o n g these initiative is the elaboration of a catalogue of Features, Events and
Processes specific to argillaceous media (FEPCAT Project). T h e catalogue, which
is p l a n n e d for the end of 2000, will provide, for each post-closure FEP, an up-to-
date, critical overview of conclusions and k e y references related to current
u n d e r s t a n d i n g and potential impact o n the long-term p e r f o r m a n c e of the
g e o s p h e r e barrier, and also information on ongoing and p l a n n e d work. In
addition to systematically exploring the commonalities and differences a m o n g
argillaceous media, it should help provide a sound, realistic a n d defensible
international basis for further long-term safety assessments.
Conclusions
References
ANSTO, 1997: Analogue studies in the Alligator Rivers Region. - Six Monthly Report, 1st July to 31st
December 1996.
HORSEMAN, S., H I C G O , J. ALEXANDER, J. & HARRINGTON, J. 1996: Water, gas and solute movement
through argillaceous media, OECD/NEA.
LALIEUX, P, PESCATORE, C. & SMITH, P 1999: Preliminary lessons from GEOTRAP, the OECD/NEA
International Project on Radionuclide Transport in Actual, Geological Media, Transactions of the
ENS Topseal '99 Conference - Radioactive Waste Management: Commitment to the Future
Environment, Antwerp, Belgium, 10-14 October 1999, ENS.
OECD/NEA 1991: Can long-term safety be evaluated? - An international collective opinion
OECD/NEA 1995: The environmental and ethical basis of geological disposal. - A collective opinion
of the NEA Radioactive Waste Management Committee.
OECD/NEA 1998a: Modelling the effects of spatial variability on radionuclide migration. -
Proceedings of a GEOTRAP Workshop, Paris, France, 9-11 June 1997
OECD/NEA 1998b: Use of hydrogeochemical information in testing groundwater flow models. -
Proceedings of a SEDE Workshop, Borgholm, Sweden, 1-3 September 1997.
OECD/NEA 1998c: Fluid flow through faults and fractures in argillaceous formations. - Proceedings
of a Joint NEA/EC Workshop, Bern, Switzerland, 10-12 June 1996.
OECD/NEA 1999a: Geological disposal of radioactive waste: Review of developments in the last
decade.
OECD/NEA 1999b: Water-conducting features in models of radionuclide migration. - Proceedings of
a GEOTRAP Workshop, Barcelona, Spain, 10-12 June 1998.
OECD/NEA (in preparation): Confidence in models of radionuclide transport for site-specific
performance assessment. - Proceedings of a GEOTRAP Workshop, Carlsbad, NM, United States,
14-18 June 1999.
LAUEUX, P.: International co-operation regarding site characterisation 249
OECD/NEA & EC 1 9 9 7 : Field tracer experiments: Role in the prediction of radionuclide migration. -
Proceedings of a GEOTRAP Workshop, Cologne, Germany, 2 8 - 3 0 August 1 9 9 6 .
OECD/NEA & SKB 1 9 9 3 : International Stripa Project 1 9 8 0 - 1 9 9 2 , 3 Volumes, Overview Volume I -
Executive S u m m a r y (FAIRHURST, C , GERA, F., GNIRK, F , GRAY, M. & STILLBORG, .) Overview
Volume II - Natural Barriers (GNIRK, P.), Overview Volume III - Engineered Barriers (GRAY, M . S )
OECD/NEA & SKI 1 9 9 6 : The International INTRAVAL Project - Developing groundwater flow and
transport models for radioactive waste disposal - Final results.
RODWELL, W , H A R R I S , A . , HORSEMAN, S., LALIEUX, E, MLLER, W., O R T I Z AMAYA, L. & PRUESS, K. 1 9 9 9 : Gas
migration and two-phase flow through engineered and geological barriers for a deep repository
for radioactive waste. - A joint EC/NEA Status Report published by the European Commission,
European Commission Report EUR 1 9 1 2 2 EN.
SACCHI, E. J . , MICHELOT, L. & PITSCH, H . 1 9 9 9 : Extraction of water and solutes from argillaceous rocks
for geochemical characterisation: methods and critical evaluation, OECD/NEA, (in press)
THURY, M & BOSSART, E 1 9 9 9 : "The Mont Terri Rock Laboratory, a new international research project in
a Mesozoic shale formation, in Switzerland". - Engineering Geology, 5 2 , 3 4 7 - 3 5 9 .
Fldtani Kzlny 130/2 251-261 (2000) Budapest
R o m a K A N O P I E N E - Vytautas M A R C I N K E V I C I U S
(3 Figures)
Abstract
The majority of radioactive waste in Lithuania is accumulating at the Ignalina Nuclear Power Plant
(INPP); the latter is located in the northeastern part of Lithuania, near lake Drukshiai. The project of
INPP construction was started in 1972; exploitation of the first reactor began in 1983, and in the
second began in 1987. There are two RMBK-1500 reactors with a total electric power capacity of 2600
MW and a thermal power output of 8400 MW in INPP
The radioactive wastes of INPP are separated into 3 categories according to the respective levels of
4 6
their radioactivity. The waste of the first (I) category has a low radioactivity level- 7.4 x 1 0 - 3.7 x 1 0
6 9
Bq/kg. The waste of the second (II) category is the intermediate activity level 3.7 x 1 0 - 3.7 x 1 0
9
Bq/kg waste. The waste of high radioactivity level is more than 3.7 x 1 0 Bq/kg - such as control rods
3
(pivots) and spent nuclear fuel elements - are ascribed to the third (III) category. 1400 m of the
3 3
category I , about 330 m of category II and about 180 m of category III waste have been forming in
3
INPP every year. There is about 30 000 m of radioactive waste accumulated in INPP. This volume
3
could reach about 50 000-100 000 m before the end of NPP exploitation.
Safe management and repositories for radioactive waste represent a new problem for Lithuania,
because in the Soviet Union these problems were solved by central institutions in Moscow.
Since 1996 the Law on Nuclear Energy" of the Republic of Lithuania has been the general order
for radioactive waste disposal. The preparation of the Law on radioactive waste management is going
on now. Lithuania signed The Joint Convention on the Safety of Spent Fuel Management and on the
Safety of Radioactive Waste Management" in 1997.
According to the recent waste management plan, the I and the II categories of radioactive waste
from INPP can be disposed in landfill repository, but for the III category waste a deep geological
repository must be constructed.
The geological structure of Lithuania could be suitable for a deep repository for radioactive waste.
The territory of Lithuania is in the northeastern part of the East European platform. A crystalline
basement occurs at depth of between 200-2300 metres below the land surface. The sedimentary cover
consists of the deposits of all geological systems (Fig. 2). Vendian and Cambrian deposits are
terrigenous (e.g. claystone, clay, gravelstone, sandstone, siltstone); Ordovician and Silurian deposits
are of a carbonate type and clayey (e.g. limestone, marl, dolomitic marl, dolomite, claystone, clay);
Devonian deposits are also of a carbonate type, sandy and clayey (e. g. sandstone, sand, clay,
dolomitic marl, dolomite, etc.); Carboniferous deposits are sandy and clayey; Permian deposits are
represented, in general, by limestone, anhydrite and rock-salt; Triassic deposits are clayey; Jurassic -
clay, siltstone, sandstone; Palaeogene and Neogene - sand, silt, clay; and Quaternary deposits are till,
sand and gravel.
sszefoglals
Litvnia radioaktv hulladknak legnagyobb rsze Litvnia K-i rszn, a Drukshiai-t mellett
fekv Ignalina Atomermben (INPP) kpzdik. Az INPP ptse 1972-ben kezddtt, az els
reaktort 1983-ban, a msodikat 1987-ben adtk t. A kt RMBK-1500-as reaktor teljes villamosenergia
kapacitsa 2600 MW, a henergia termels 8400 MW.
Az INPP radioaktv hulladka a radioaktivits mrtke szerint hrom osztlyba sorolhat. Az els
4 6
(I) kategriba a kis radioaktivits hulladkok kerlnek ( 7 , 4 x l 0 - 3 , 7 x l 0 Bq/kg). A kvetkez (II)
6 9 9
kategrba a kzepes aktivits ( 3 , 7 x l 0 - 3 , 7 x l 0 Bq/kg), mg a harmadik (III) kategriba ( > 3 , 7 x l 0
Bq/kg) a nagy aktivits hulladkok, pldul a szablyzrudak s a kigett ftelemek tartoznak.
3 3 3
vente 1400 m I, kb. 330 m II s kb. 180 m III kategrij hulladk keletkezik az INPP-ben, ami a
3
mai napig sszesen kb. 30 000 m radioaktv hulladk felhalmozdst jelent. Az atomerm
3
bezrsig a teljes mennyisg elrheti az 50 000-100 000 m -t.
A radioaktv hulladk biztonsgos kezelse s trolsa jkelet problma Litvniban, mivel a
Szovjetuni idejben az ilyesfajta problmkat a moszkvai kzponti intzetekben oldottk meg.
1996-ben a Litvn Kztrsasg atomenergia trvnyben fektette le a radioaktv hulladklerakssal
kapcsolatos ltalnos szablyokat. Jelenleg a radioaktv hulladkkezelssel kapcsolatos trvny
elksztse folyik. Litvnia 1997-ben alrta A kigett ftelemek kezelsnek biztonsgrl s a
radioaktv hulladkok kezelsnek biztonsgrl szl kzs egyezmny"-t.
A jelenlegi hulladkkezelsi tervek szerint az INPP-bl kikerl I s II kategriba tartoz
radioaktv hulladkok elhelyezse trtnhet felszni krlmnyek kztt, a III kategriba tartozkat
viszont mlysgi trolban kell elhelyezni.
Litvnia fldtani szerkezete lehetv teszi mlysgi trol ltestst. Litvnia a kelet-eurpai
platform K-i rszn fekszik, ahol a kristlyos aljzat 200-2300 m mlysgben kezddik. Az ledkes
takar a legklnflbb fldtani kpzdmnyekbl tevdik ssze (1. bra). A vendi s a kambriumi
ledkek szrazfldi keletkezsek (agyagk, agyag, konglomertum, homokk, aleurolit), az
ordovciumi s a szilur ledkek karbontosak s agyagosak (mszk, mrga, dolomitos mrga,
dolomit, agyagk, agyag), a devon ledkek karbontosak, homokosak s agyagosak (homokk,
homok, agyag, dolomitos mrga, dolomit, stb.), a karbon ledkek homokosak s agyagosak, a permi
ledkeket ltalban mszk, anhidrit s ks reprezentlja, a triszban agyagos ledkek, a jurban
agyag, aleurolit s homokk, a paleognben s a neognben homok, aleurit s agyag, mg a
kvarterban till, homok s kavics rakdott le.
A fldtani kutatsok eredmnyei szerint a kvetkez fldtani formcik alkalmasak mlysgi
radioaktv hulladktrol ltestsre: 1) kristlyos aljzat; 2) als-kambriumi agyag; 3) permi szulftos
ledkek; 4) permi ks; 5) als-trisz agyag. A mlysgi trol brmelyik formciban trtn
elhelyezse fgg a megfelel tektonikai, hidrogeolgiai s mrnkgeolgiai adottsgoktl, a
nemzetkzi elvrsoktl, valamint Litvnia trvnyeitl.
6 9 3
II intermediate level 3.7 x 1 0 - 3.7 x 10 Bq/kg 330 m
9 3
III high level > 3.7 x 1 0 Bq/kg 180 m
Project at L G T
The project for the first stage (prospective (review) investigations) of this long-
term w o r k w a s a p p r o v e d and started at the L G T this year (1999). T h e title of this
project is Evaluation of the territory of Lithuania according to the suitability for
the d e e p repository for radioactive waste".
According to international recommendations (IAEA 1981, 1989; S A V A G E 1995), a
safe d e e p repository for radioactive waste disposal can b e constructed only in a
deep-lying (depth > 2 0 0 m) geological formation. T h e long-term safety of high
level radioactive waste disposal has to be based on the multibarrier c o n c e p t to
avoid the m o v e m e n t o f radionuclides from the repository to the e n v i r o n m e n t .
These barriers h a v e to be: engineered barriers, the host rock and the geological
environment. It is, nevertheless, recognised that the geological barrier plays the
major role in assuring long-term safety. Therefore the site selection for a deep
geological radioactive waste disposal repository is a primary and complex task.
T h e requirement for selecting radioactive waste disposal repository is to assure
long-term (not less t h a n 10 000 years) h u m a n a n d e n v i r o n m e n t a l safety
(protection) from radioactive pollution (SAVAGE 1995).
Given international r e c o m m e n d a t i o n s and the data of similar investigations
from foreign countries specialists of Geological S u r v e y of Lithuania decided to
select a geological formation for a deep R W repository using 3 groups of criteria:
1, geological,
2, radiation (radiological) safety,
3, territorial.
The criteria for the first and the second group have already b e e n d e t e r m i n e d
quite clearly.
1, T h e major geological criteria are: structure of the formation, density of
tectonic faults, hydrogeological situation, geochemistry of the rocks a n d others
(see Table II)
256 Fldtani Kzlny 130/2
Assessing the suitability of the geological formations for high level radioactive
waste repository construction the following data about the territory must be
evaluated:
- Geographical conditions;
- Tectonic, neotectonic conditions and seismic situation;
- H y d r o g e o l o g i c a l c o n d i t i o n s (stratification o f h y d r o g e o l o g i c a l section,
h y d r o d y n a m i c and hydrochemical properties of low permeability layers and
aquifers, w a t e r exchange b e t w e e n the aquifers, h y d r o d y n a m i c relationships
b e t w e e n shallow and g r o u n d w a t e r etc.);
- C o m p o s i t i o n of geological formation, its physical, chemical a n d mechanical
properties (conductivity, porosity, solubility, absorption properties, radioactivity,
t h e r m a l conductivity a n d capacity, temperature gradient etc.);
- O c c u r r e n c e of geological processes;
- E n v i r o n m e n t a l geological situation.
KANOPIENE, R. & MARCINKEVICIUS, V. Possibilities of radioactive waste repository in Lithuania 257
All the data about the geological structure of Lithuania are h a v e b e e n collected
by the at LGT. This information can be divided in to four m a i n groups:
1) borehole data,
2) geological, geophysical m a p p i n g data,
3) raw material prospecting and exploration data,
4) results of special geological investigations.
T h e r e are data about more than 2600 deep boreholes (depth m o r e than 200 m )
in the computerised State geological information system. Geological m a p p i n g on
a scale o f 1: 200 000 covers all the territory of Lithuania. This scale was selected as
a working scale for the graphical information in the project. S o m e geological
formations (systems) w e r e investigated in detail during the prospecting and
exploration project for oil, rock salt, anhydrite and other mineral resources. The
reports o f different geological investigations will be used (as well as the archive
data) for the selection of the geological formation for the H L R W repository.
Finally, to compare the suitability of different geological formations and to
s h o w graphically the results of the project GIS technologies and Maplnfo
software will be used.
mNN 4 2 6
\ 1385m ^
O i [V]4 Q 5 H
Fig-. 2 Geological section of Pagirai anhydrite deposit. 1 aquitard, 2 medium permeability, 3 aquifer,
4 gypsum, 5 banded anhydrite, 6 spotted anhydrite
2. bra Pagirai anhidrit lelhely fldtani szelvnye. 1. vzzr, 2. kzepesen tereszt, 3. vztereszt, 4. gipsz,
5. szalagos anhidrit, 6. foltos anhidrit
The oldest part of the Lower Cambrian - i.e. Baltija group - consists of a
c o m p a c t clay formation. This formation occurs in Eastern Lithuania at a depth of
3 0 0 - 5 0 0 and m o r e metres. T h e clay is very compact and consists of hydromica
(from 6 0 - 6 5 to 8 5 - 9 0 % , kaolinite (from 3 - 5 % to 2 5 - 3 0 % and chlorite (from 3 - 5 %
to 1 0 - 1 5 % ) minerals ( P A S K E V I C I U S 1 9 9 9 ) . There is some intercalation of sandstone
in the L o w e r Cambrian clay.
KANOPIENE, R. & MARCINKEVICIUS, V. -.Possibilities of radioactive waste repository in Lithuania 259
The entire layer of these deposits is 4 0 - 6 0 m thick and occurs in the Southern
2
and South-western parts of Lithuania covering an area of more than 1 2 0 0 0 k m .
This layer lies at a depth of 1 5 0 - 7 9 0 m. Most of these deposits ( 7 0 - 8 0 % ) consist of
anhydrite. Permian gypsum which 5 - 8 m thick occurs above the anhydrite layer
and g y p s u m which is 3 - 5 m thick lies below the anhydrite. In the Kaunas district
i.e. the Pagiriai deposit (Fig. 2 ) the exploration of anhydrite has b e e n carried out.
Resources of 8 1 . 5 million, tonnes of anhydrite have b e e n evaluated there. The
project for the exploitation of anhydrite by underground mining has been
prepared. According to this project, the free underground cavities after the
exploitation of anhydrite can be used for a repository for radioactive waste
(KADUNAS 1993).
Permian rock-salt
Expected results
- will provide the information for further stages of geological investigations for
d e e p R W r e p o s i t o r y site selection.
Conclusions
We h a v e a p r o b l e m in Lithuania - T h e Ignalina N u c l e a r P o w e r P l a n t a n d
3
414 m of solid h i g h activity Radioactive Wastes.
We c o u l d solve this p r o b l e m b y using a geological formation in L i t h u a n i a
w h i c h is suitable for a d e e p R W repository.
We h a v e to give the clear a n s w e r to this question.
This is w h y w e h a v e to carry out the project w h i c h r e p r e s e n t s the first stage of
geological investigations - to evaluate the territory of L i t h u a n i a a c c o r d i n g to its
suitability for a d e e p R W repository.
References
International Atomic Energy Agency 1981: Underground disposal of radioactive wastes. Basic
guidance, - Safety Series 54, IAEA, Vienna, 56 p.
International Atomic Energy Agency 1989: Safety principles and technical criteria for the
underground disposal of high level radioactive wastes. IAEA safety standards - Safety Series 99,
IAEA, Vienna, 28 p.
KADNAS, V. 1993: Ecogeological appreciation of the Upper Permian anhydrite seam from the point of
arrangement of depositories. - Geologija 15, Vilnius, 27-31.
LOMTADZE, V. 1978: (Ingenernaia geolgia. Specialnaia ingenernaia geolgia) Engineering geology.
Special engineering geology., Leningrad., Nedra, 496 p.
MARFIN, S., MIKSYTS, R . . , MOTUZA, G., & SKRIPKINA, T 1982: The structure of the Marcinkonys granitic
massif and properties of rocks. - Geologija 3 , Vilnius 3-16.
PASKEVICIUS J. 1999: Stratigraphy of Vendian, lower and middle Paleozoic and its problems. (Lietuvos
mokslas. Geomokslai. Monografija) Science of Lithuania. Geosciences. Monograph. Vilnius;
96-129.
SAULENAS, V , GASIUNIENE, V. E., & KRALIKAUSKAITE R . 1997: Whether we will extract Lithuanian rock-
salt? - Information publication. Geological Survey of Lithuania. Vilnius.
SAVAGE, D. (Ed.) 1995: The scientific and regulatory basis for the geological disposal of radioactive
waste. Wiley, Chichester, 438 p.
SUVEIZDIS E 1994: Triassic; (Triasas. Lietuvos geologija. Monografija) Lithuania's geology. Monograph,
Vilnius, 132-138.
Fldtani Kzlny 130/2 263-273 (2000) Budapest
D u k e U. O P H O R I
(4 Figures)
Key words: Modelling, groundwater flow, particle tracking, waste disposal, Canada
Abstract
Atomic Energy of Canada Limited (AECL) has developed a concept for the disposal of Canada's
nuclear fuel waste in a vault, deep (500 m to 1000 m) in low-permeability plutonic rocks of the
Canadian Shield. In the concept, the low-permeability rock mass is expected to provide a natural
barrier to the release and migration of wastes from the vault. An understanding of groundwater flow
can be used to enhance the role of the rock mass as a barrier in the overall disposal system. Therefore,
AECL has developed large-scale groundwater flow models of some candidate sites that are used to
identify potential vault locations within the sites which have the longest groundwater flow times
from prospective disposal vault depths to ground surface.
One candidate site that has been studied by AECL is the Whiteshell Research Area (WRA) in
southeastern Manitoba. At this site, a regional groundwater flow model has been developed for a 1050
2
k m area in order to evaluate alternative locations for a hypothetical nuclear fuel waste disposal vault
that maximizes retention of vault contaminants in the rock. A conceptual model of the hydrogeologic
conditions was constructed using information obtained from field investigations at the WRA between
1977 and 1994. Simulations of flow were performed using AECL's three-dimensional finite-element
code, MOTIF.
First, average values of hydraulic parameters obtained from an analysis of the field data were used
in the simulations. Simulated average groundwater recharge did not compare favorably with the
recharge rate that was estimated from field data independently. Model calibration was performed by
modifying the hydraulic parameters and total dissolved solids distribution of the fluids in a series of
consecutive simulations. The simulated recharge rate for the final calibrated model was 4.8 mm/yr.
which compared well with the field-based rate of 5 mm/yr. The simulated freshwater heads for this
simulation also compared reasonably well with measured heads in the network of boreholes at the
WRA. Most of the groundwater flow occurred in local systems between the ground surface and the
depth of 2000 m relative to less flow in the intermediate and region systems at greater depth.
A particle tracking code, TRACK3D was used to determine the travel times, pathways and exit
locations of particles released from different depth horizons in the groundwater velocity field of the
calibrated model. These were used to select a location for a hypothetical nuclear fuel waste disposal
vault that maximizes the retention of vault contaminants in long, slow groundwater flow pathways.
Montclair State University, Upper Montclair, NJ 07043 USA, Phone: 973-655-7558; Fax: 973-655-4072
264 Fldtani Kzlny 130/2
sszefoglals
A Canada Ltd Atomenergia gynksge (Atomic Energy of Canada Limited - AECL) terve szerint
Kanada kigett nukleris ftelemeit a Kanadai Pajzs mlyen fekv boltozatnak (500-1000 m
kztti), kis teresztkpessg mlysgi kzeteibe vgott regben kellene elhelyezni. A tervben a kis
teresztkpessg kzettmegtl azt vrjk, hogy termszetes mdon akadlyozza az regbl
kiszk s elvndorl szennyezanyagokat. A talajvzramlsi rendszer jobb megrtse segtheti
tisztzni a kzettmegnek a lerakrendszerben elfoglalt gt szerept. Ezrt az AECL elksztette
nhny szmbajv terlet talajvzmodelljt, amelyek alapjn azonosthatak azok a lehetsges
telephelyek a kivlasztott terleten bell, amikhez a leghosszabb talajvzramlsi idk tartoznak a
vrhat lerakhelytl a felsznig.
Az egyik AECL ltal tanulmnyozott lehetsges telephely a Whiteshell Kutatterlet (WRA),
2
Manitoba DK-i rszn. Ezen a telephelyen modelleztk a regionlis talajvzramlst egy 1050 km -es
terletre, hogy tbb szbajhet helysznt rtkeljenek egy leend elhasznlt nukleris ftelem
lerakhely szmra, ami maximlisan visszatartja az regben elhelyezett szennyez anyagot. A
hidrogeolgiai krlmnyek/felttelek koncepcis modelljt ksztettk el, azoknak az adatoknak a
felhasznlsval, amiket a WRA 1977-1994 kztti terepi megfigyelseibl nyertek. Az ramls
modellezsre az AECL hromdimenzis vges-vltozs programjt, a MOTIF-ot alkalmaztk.
Elszr a terepi adatok rtkelsbl nyert hidraulikus paramterek tlagos rtkeit hasznltk a
modellhez. A modellezett tlagos talajvz utnptlds nem hasonltott elgg a terepi adatokbl
kzvetlenl becslt rtkekhez. A modell helyesbtse gy trtnt, hogy egy sorozat modellben
fokozatosan mdostottk a folyadkok hidraulikus paramtereit s a teljesen feloldott
szilrdanyagok eloszlst. Az utols modellben az utnptlds mennyisge 4,8 mm/v volt, ami jl
egyezett a terepi becsls 5,0 mm/vvel. A modellezett desvz nyomsok ebben az utols modellben
szintn megfelel mrtkben hasonltottak a WRA-n teleptett kthlzatban mrtekhez. A
vzramlsok tbbsge a helyi rendszerekben a felszn s 2000 m kztt tallhat a nagyobb
mlysgben megjelen tmeneti s regionlis rendszerek kis ramlsval szemben.
Egy rszecske-kvet rendszert, a TRACK3D-t alkalmaztk a kalibrlt modell talajvz ramlsi
felsznnek klnbz mlysgszintjrl indul rszecskk ramlsi idejnek, ramlsi tvonalnak
s kijutsi helynek meghatrozsra. Ezeket az rtkeket hasznltk az elmleti nukleris ftelem
lerakhely boltozat megfelel helynek kivlasztshoz, ami maximlja a boltozatban lv szennye
zanyagok ksleltetst hossz, lass talajvz ramlsi tvonalakon.
Introduction
Fig. 1 Map of the Whiteshell research area showing lineaments (fracture zones), model area and
locations of deep boreholes (Grid areas)
1. bra A Whiteshell Kutatsi Terlet trkpe a trses znkkal, a modell terlettel s a mlyfrsok helyvel
(hls terletek)
Fig. 2 Geologie Framework, Surface Structure and Finite-Element Mesh of the Whiteshell Research
Area. Section A-A' is a Line Joining Point A to Point A'.
2. bra A Whiteshel Kutatsi Terlet fldtani felptse, felszni szerkezete s vges vlts hlja
W i t h i n the WRA, the water table is a subdued replica of the surface topography
w h i c h has a moderate regional slope of about 0.002 from southeast to northwest.
The w a t e r table elevation was used as the top b o u n d a r y condition. T h e Winnipeg
River was assumed to provide stable hydrological boundaries on m o s t sides of
the area, except the northeastern part of the m o d e l area w h i c h is b o u n d e d by a
major fault referred to as the F - F fault. Because there is sufficient local topo
graphic relief around it to capture groundwater flow from considerable depth,
the W i n n i p e g River was assumed to be a no-flow hydrogeologic boundary. T h e
major fault along the northeastern part of the area was also a s s u m e d to b e a n o -
flow boundary. The bottom b o u n d a r y o f the m o d e l at a d e p t h o f 4000 m was
a s s u m e d to be impermeable. Trends in available field permeability data suggest
2 1 2
that permeability at this depth could be 1 0 " m or lower, essentially im
p e r m e a b l e . It was demonstrated that changing these lateral a n d lower b o u n d a r y
conditions does not affect the convective transport of solutes from the selected
locations of a hypothetical vault at 500 m to 1000 m depth to the groundwater
discharge locations in the biosphere ( O P H O R I et al. 1 9 9 6 ) . T h e s e b o u n d a r y
conditions w e r e the same as u s e d in an earlier m o d e l of the W R A ( D A V I S O N et al.
OPHORI, D . U.: Simulating large scale groundwater flow for waste disposal purposes 267
1994) except that the elevation of the water table has b e e n substituted for the
topographic elevation for the top b o u n d a r y condition of the m o d e l .
Permeability data exist from straddle packer tests a n d p u m p i n g tests in
boreholes to depths of 1000 m at the W R A . T h e s e data w e r e analysed in detail b y
S T E V E N S O N et al. (1995). T h e values of permeability used in the simulation for the
rock mass and fracture zones are s h o w n in Table 1. For the rock mass, horizontal
15 2 2 1 2
permeability decreased from 1 x 1 0 " m at the surface to 1 x 1 0 " m at a depth
of 1000 m. T h e anisotropy in the rock was represented b y assigning vertical
permeabilities o n e order of magnitude higher than horizontal permeabilities
b e t w e e n the ground surface a n d 300 m for the granite, and also b e t w e e n 300 a n d
1000 m for the gneiss. Below this depth, the rock mass was assigned a constant
2 1 2
permeability of 1 x 1 0 " m . T h e fracture zones were a s s u m e d isotropic with
13 2 16 2
permeability varying from 1 x 1 0 " m at the surface to 1 x 1 0 " m at a depth of
1000 m. Below 1000 m, the fracture zones were assigned gradually decreasing
1 9 2
permeabilities reaching 7.52 x 1 0 " m at the bottom of the m o d e l (4000 m ) . The
permeability values w e r e derived from the analysis b y S T E V E N S O N et al. (1995).
Porosity values were estimated from field and laboratory data b y S T E V E N S O N et
al. (1996a). T h e s e r a n g e d from 0.003 to 0.001 for the rock mass, a n d form 0.05 to
0.005 for the fracture z o n e s (Table 1).
Flow simulation
* Gneiss
* Granite
* * G r a n i t e u n d e r TDS dome
X Ti
Hypothetical vault location
code, particles were released on a regular grid at different depths into the
g r o u n d w a t e r velocity field of the calibrated model and tracked to their exit points
at surface. T h e advective travel times of the particles w e r e also determined. Three
different particle release depths, 500-, 750- and 1000 m, w e r e analysed in detail.
The travel times of particles released at a depth of 750 m to their exit locations
at the ground surface are depicted in Fig. 4. These travel times w e r e used to select
a location for a hypothetical disposal vault at a depth of 750 m in the modeled
area.
O t h e r aspects that w e r e c o n s i d e r e d in c h o o s i n g t h e l o c a t i o n for the
hypothetical vault were:
6
1. the location should have long travel times ( m i n i m u m 1 0 a),
2. the location should be an area of at least 2 k m b y 2 k m in size containing no
regional fracture zones at the d e p t h of the vault,
3. the location should have a reasonable level of field data control (i.e. borehole
control within or near the location), and
4. the depth of the hypothetical vault should be within 500 m to 1000 m below
g r o u n d w a t e r surface.
The selected location for the hypothetical disposal vault is indicated in Figure
4. T h e site is about 5 km northeast of the location of the U n d e r g r o u n d Research
Laboratory (URL). Details of the selection process are p r e s e n t e d in O P H O R I et al.
(1996) and D A V I S O N et al. (1996).
Summary
Fig. 4 Travel times of particles released from model depth horizon of 750 m
Acknowledgements
I t h a n k N. W S C H E I E R , . C. D A V I S O N , A. B R O W N , M . G A S C O Y N E a n d D . R .
S T E V E N S O N for their constructive c o m m e n t s and helping to improve this paper.
This w o r k was p e r f o r m e d for the Canadian Nuclear Fuel Waste M a n a g e m e n t
Program, w h i c h is jointly funded b y AECL and Ontario Hydro u n d e r the
auspices of the C a n d u O w n e r s Group.
272 Fldtani Kzlny 130/2
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CHAN, T., REID, J.A.K. &. GUVANASEN, V 1997: Numerical modelling of coupled fluid, heat and solute
transport in deformable fractured rock. - In: CHIN-FU TSANG (Ed): Coupled Processes Associated
with Nuclear Waste Repositories, Academic Press, Inc., Orlando, Florida, 605-625.
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NAKKA, B. W., O ' C O N N O R , P A., O P H O R I , D. U., SCHEIER, N. W , SOONAWALA, N. M , STANCHELL, F.
W., STEVENSON, D. R., THORNE, G. A., VANDERCRAPF, T. X VILKS, R & WHITAKER, S. H. 1994: Xhe
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Conference, September, 1996, Winnipeg, Manitoba, Canada, 7 p.
GUVANASEN, V. 1984: Development of a finite-element code and its application togeoscience research.
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modelling in the geosphere: description and user's manual.- Atomic Energy of Canada Limited
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OPHORI, D. U. 1996: Regional groundwater flow in the Atikokan Research Area: Model Development
and calibration. - Atomic Energy of Canada Limited Report, AECL-11081, COG-94-183, Pinawa,
Manitoba, Canada.
OPHORI, D. U. 1999: Constraining permeabilities in a large-scale groundwater system through model
calibration. - Jour, of Hydrology 2 2 4 , 1 - 2 0 .
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1 8 3
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O P H O R I , D. U., B R O W N , A.,. CHAN, X, DAVISON, C. C , GASCOYNE, M., SCHEIER, N. W , STANCHELL, F. W. &
STEVENSON, D. R. 1996: Revised model of regional groundwater flow of the Whiteshell Research
Area. - Atomic Energy of Canada Limited Report, AECL-11435, COG-95-443, Pinawa, Manitoba,
Canada.
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N. W., STANCHELL, F. W., XHORNE, G. A. & XOMSONS, D. K. 1995: A revised conceptual
hydrogeological model of a crystalline rock environment, Whiteshell Research Area,
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STEVENSON, D. R., B R O W N , A., DAVISON, C. C , GASCOYNE, M., M C G R E G O R , R. G., O P H O R I , D. U., SCHEIER,
N . W , STANCHELL, F. W , XHORNE, G. A. & XOMSONS, D. K. 1996a: A revised conceptual
hydrogeological model of a crystalline rock environment, Whiteshell Research Area,
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Fldtani Kzlny 130/2 275-289 (2000) Budapest
1 2
Grant S H E N G - J z s e f T T H
(2 Figures, 2 Tables)
Abstract
The Recharge Area Concept is the proposition that in Canadian-Shield type natural environments
recharge areas of regional groundwater flow systems are superior for high-level nuclear waste
repositories to other types of groundwater flow regimes, especially to areas of groundwater
discharge. This conclusion is reached from an analysis of basinal groundwater flow models. The
calculations were made for a two-dimensional flank of a fully saturated topographic basin, 20 km long
and 4 km deep, in which groundwater is driven by gravity. Variants of hydraulic-conductivity
distributions were considered: 1) homogeneous; 2) stratified; and 3) stratified-faulted. The faults
attitudes were changed by steps from vertical to horizontal for different variants. The model is
assumed conceptually to represent the crystalline-rock environment of the Canadian Shield.
The hydrogeologic performances of hypothetical repositories placed 500 m deep in the recharge
and discharge areas were characterized by thirteen parameters. The principal advantages of recharge-
over discharge-area locations are: 1) longer travel paths and return-flow times from repository to
surface; 2) robustness of predicted values of performance parameters; 3) field-verifiability of
favourable hydrogeologic conditions (amounting to an implicit validation of the calculated minimum
values of return-flow times); 4) site acceptance based on quantifiable and observable flow-controlling
parameters; and 5) simple logistics and favourable economics of site selection and screening. As a by
product of modelling, it is demonstrated that the presence of old water is not an indication of
stagnancy.
'Faculty of Environmental Studies, York University, 4700 Keele Street,Toronto, Ontario, M3J 1P3,
Canada
2
D e p a r t m e n t of Earth and Atmospheric Sciences, University of Alberta, Edmonton, Alberta, T6G
2E3, Canada
276 Fldtani Kzlny 130/2
sszefoglals
Az utnptldsi terlet koncepci (Recharge Area Concept) lnyege az, hogy a Kanadai pajzs
tpus termszetes krnyezetekben a regionlis felszn alatti vzramlsi rendszerek utnptldsi
terletei alkalmasabbak nagy radioaktivits hulladktrol kiptsre ms tpus felszn alatti
vzrendszereknl, klnsen a megcsapolsi terleteknl. Erre a kvetkeztetsre a medence mret
vzramlsi modellek elemzsbl juthatunk. A szmtsokat egy 20 km hossz, 4 km mly
topogrfiai medence tkletesen teltett ktdimenzis szelvnyre vgeztk el, ahol a talajvizet a
gravitci mozgatja. A kvetkez vzvezetkpessg-eloszlsi eseteket vettk figyelembe: 1)
homogn; 2) rtegzett; 3) rtegzett s trses. A vetk helyzett a klnbz esetekre lpsenknt
vltoztattuk a fgglegestl a vzszintesig. A modellbe koncepcionlisan a Kanadai Pajzs kristlyos
kzetekbl ll krnyezett ptettk be. Az utnptldsi s megcsapolsi terleteken 500 m
mlysgben elhelyezett kpzeletbeli trolk hidrogeolgijt tizenhrom paramterrel jellemeztk.
Az utnptldsi terleten lv trol leglnyegesebb elnyei a megcsapolsihoz kpest: 1) hosszabb
vndorlsi tvonalak s elrsi idk a troltl a felsznig; 2) sokkal jobb vrhat paramterrtkek;
3) a kedvez hidrogeolgiai felttelek terepi ellenrizhetsge (ami az elrsi idk szmtott
minimum rtkeinek egyrtelmstshez vezet); 4) a telephelynek a mennyisgileg meghatrozhat
s szlelhet ramlsi paramtereken alapul elfogadsa; valamint 5) a telephely kivlaszts s szrs
tlthat logisztikja s a kedvez gazdasgi felttelek. A modellezs mellktermkeknt az is
kiderlt, hogy az ids vizek jelenlte nem utal az ramls hinyra.
Introduction
Technical issues
Since the overriding concerns of this disposal endeavour are to ensure safety
of h u m a n s and protection of the environment both n o w and far into the future,
a convincing demonstration of the safety of the disposal system primarily
involves technical issues. T h e first is associated with the capability to make
forecasts of far-future events (especially those geologically related), and the
second, with the extent that such forecasts can be confirmed" in some fashion
SHENC, G. & TTH, J.: Using the Recharge Area Concept 277
With respect to the first technical issue, m u c h effort and resources have b e e n
devoted by the international community to geologic and geotechnical R & D w o r k
because of the c o n c e p t ' s heavy reliance on the geology to act as a natural barrier
( S H E M I L T & S H E N G 1983; S H E N G et al. 1993a). It is axiomatic to v i e w g r o u n d w a t e r
always as the negative agent that transports contaminants to the surface, and
fractures as the conduits through which the groundwater d o e s the transport.
These assumptions stem from an implicit world-view that w e must s o m e h o w
create a water-tight box" to confine the contaminants. Although there is
a c k n o w l e d g e m e n t that absolute c o n f i n e m e n t m a y n o t b e p o s s i b l e , it is,
nevertheless, the idealized goal, as indicated b y use of terms such as waste
isolation", multi-barriers", etc. T h e box" is to be m a d e water-tight" with a
series of m a n - m a d e (container, buffer, backfill, vault) and natural barriers (host
geologic medium, and associated features). Thus, the major research effort
internationally is directly or indirectly focused on h o w to k e e p groundwater (a)
from intruding into the vault, (b) away from the waste, (c) from exiting the vault,
(d) a w a y from fractures; and (e) studying the influence of fracture a n d fracture-
associated p h e n o m e n a on the m o v e m e n t of groundwater. B o t h (d) and (e) have
been, a n d continue to b e , the main focus of R & D w o r k u n d e r the present vision
of waste disposal.
However, m a n y years of intense research d o c u m e n t e d in publications such as
G E O V A L ( 1 9 8 7 , 1 9 9 0 ) h a v e shown the great difficulties associated with items (d)
and (e). There are at least two underlying factors that give rise to this situation:
(1) an inherent characteristic of fractures is that they are essentially d i s
continuous" on the scale relevant to site characterization and, (2) although
various theories exist to explain the formation and propagation of fractures, the
p h e n o m e n o n is so c o m p l e x that accurate predictions or forecasting of their future
behaviour, even in the short-term, is not yet within the realm of our present
understanding a n d technology. Furthermore, as pointed out in S H E N G et al.
( 1 9 9 3 a ) , e v e n if it w e r e possible to do such accurate p r e d i c t i o n s a n d
characterizations, there is no guarantee that n e w fractures will not form during
the time period that the disposal vault is required to remain effective. T h e s e are
but several of the most salient and fundamental issues that the current disposal
c o n c e p t have yet to resolve.
278 Fldtani Kzlny 130/2
With respect to the second technical issue, the extent with w h i c h the forecasts
from models can be confirmed (or to use the popular term in this field:
validated") obviously has a great bearing on the degree of confidence one places
on the models a n d their results. However, demonstration of the safety of the
disposal system is problematical in this situation w h e r e the ultimate performance
of the system at some distant point in the future c a n n o t be ascertained.
Adequate/satisfactory performance must be inferred based on a combination of:
(a) our present understanding of natural processes, (b) k n o w l e d g e about relevant
system parameters, (c) our ability to design, and have confidence in, the
e n g i n e e r e d systems and (d) our ability to extrapolate this collection of k n o w l e d g e
far into the future.
C o m p u t e r i z e d simulation is the only m e a n s w e h a v e to c a r r y out
systematically a n d quantitatively such an extrapolation u p o n w h i c h to base an
inference of satisfactory system performance so far into the future. While this
paper presents the results of such a simulation study, the specifics of validating
the underlying m o d e l must be dealt with in detail in another paper in accordance
with a framework proposed by S H E N G et al. (1993b).
The Recharge Area Concept is developed from two basic arguments. First, it is
recognized that the favourable combination of maximum groundwater flow-path
lengths with minimum flow velocities, ensuring m a x i m u m travel times and
m a x i m u m dilution of contaminants, is most likely to occur along flow lines that
originate in regional recharge areas. Second, for recharge positions it appears
possible to confirm calculated travel times, i.e. to confirm model calculations to
the extent n e e d e d for the guaranteed safety of a repository. T h e second point
implies the assertion that minimum travel times can be established which cannot
possibly be negated by u n k n o w n deviations from assumed geologic conditions
such as, for instance, undetected fractures or fault zones. Such an assurance
cannot, on the other hand, be given for other basinal areas, including those of
groundwater discharge. Furthermore, adoption of the RAC as a guiding principle
facilitates and rationalizes the practical procedural aspects of the selection,
screening and evaluation of a repository location. Although e c o n o m y and
logistical ease are not specifically considered in this paper, the great advantages
conferred in these respects by a siting strategy based on the RAC should not be
ignored.
Figure 1
Recharge
Areas
System
I ' " I' f ' I " I
5 10 15 20
Valley Flank (arbitrary length units)
Fig. 1 Distribution of flow, hydraulic heads, and principal hydraulic regions in drainage basins with
sinusoidally undulating water table superimposed on a linear regional slope (Composite Basin) (from
T T H & SHENG 1 9 9 6 , Figure 1, p. 6 )
UK
Distance in km
Fig. 2 Calculated distributions of hydraulic heads, groundwater flows lines, and isochrones of
groundwater travel-time between water divide and valley bottom, in a basin of homogeneous matrix
hydraulic conductivity (from TTH & SHENG 1 9 9 6 , Fig. 3 , p. 1 1 )
model is. In this present example, the application of the RAC to repository siting,
the goal is to demonstrate the safety performance of the disposal system by
calculating a minimum travel time" (MTT) for the contaminated groundwater to
reach the surface. The M T T is the shortest (or equivalently, the fastest) time that
the groundwater can possibly re-surface at the discharge zone. It is calculated
based o n an estimation of the shortest path length that the water can take from
the repository to the surface in a regional groundwater flow system. The flow
distribution and other associated characteristics of groundwater in such a system
can be derived from the surface topography by applying the fundamental
principle of groundwater flow as first elucidated by TTH (1963).
. The M T T derived from a particular set of topographic and subsurface geologic
conditions can, in the first instance, be compared with the half-life of any specific
radionuclide of concern. Should the M T T be significantly greater than the half-
life of a particular radionuclide (say ten times) then clearly that radionuclide can
be d e e m e d to pose n o potential harm in the future. S h o u l d the half-life be greater
than the MTT, then the m a x i m u m amount of the radionuclide that can possibly
reach the surface can be calculated based on its initial inventory in the repository
together with its half-life. The maximum possible dose from such a radionuclide
can be calculated by estimating its concentration at the point of discharge at the
surface. The surface area n e e d e d to estimate the concentration is u p w a r d l y
b o u n d e d by the lateral extent of the discharge area which can be estimated from
the particular set of topographic and subsurface geologic conditions used in the
simulation study or, alternatively, based on actual m e a s u r e m e n t s if a specific site
is being investigated. The estimated dose figure can then be c o m p a r e d with the
regulatory limit to decide if a particular hypothetical or actual site is safe.
The practical approach to achieve the ultimate objective of safe waste disposal
by employing the RAC m a y be summarized in the following seven basic steps:
1) Selection of a repository location from which groundwater travel times to
prohibited points are assumed (from general considerations, experience and/or
scoping calculations) to be sufficiently large.
2) Calculation of possible travel times by site-specific models of regional
groundwater flow.
3) Calculation of measurable fluid-dynamic parameters of the groundwater
flow regime.
4) Installation of exploratory instrumentation at k e y points in the basin.
5) Verification of the appropriateness (i.e. applicability) of the m o d e l by
comparing the calculated fluid-dynamic parameters with their field determined
values.
6) Acceptance/rejection of the model, depending on the degree of a g r e e m e n t
b e t w e e n calculated and observed values of the dynamic parameters.
7a) If m o d e l is rejected, construction of n e w one and repeating of the process
from Step 3.
282 Fldtani Kzlny 130/2
T h e spatial and temporal distributions, the fluid dynamic properties and the
wide array of natural manifestations, i.e. the general characteristics of gravity-
i n d u c e d regional groundwater flow have b e e n studied extensively over the last
three decades ( T T H 1963, 1984; B R E D E H O F T et al. 1982). Also, these issues are
routinely treated in modern texts on hydrogeology (e.g. F R E E Z E & C H E R R Y 1979).
For the p r e s e n t p u r p o s e s it is n e c e s s a r y to r e v i e w briefly o n l y those
characteristics w h i c h are directly relevant to the problem of nuclear waste
disposal in the Canadian Shield.
descending limb, i.e. recharge portion, of the regional system, whereas at Site 3
local recharge is underlain by the regional discharge area.
Additional complications m a y be introduced into the pattern of basinal
groundwater flow by permeability variations. The effects on the flow patterns of
heterogeneities, such as fault zones and fractures, depend on their degree, areal
extent, orientation with respect to flow lines, and elevation of outcrop regions.
The two basic arguments upon which the RAC has been developed, as stated
earlier, are: 1) that a position in a regional recharge area ensures the m a x i m u m
degree of dilution and m a x i m u m possible travel times back to the land surface (as
c o m p a r e d with other positions in a basin of similar hydrogeologic properties) for
contaminants possibly escaping from a repository, and 2) that it is recharge
e n v i r o n m e n t s w h e r e the g r o u n d w a t e r flow-characteristics are sufficiently
insensitive to discrepancies b e t w e e n actual hydrogeologic conditions and
conditions assumed for purposes of calculations, to allow the construction of
adequately robust flow models and their validation. Clearly, the above reasoning
is relativistic: it compares the effects of different positions in topographically
defined drainage basins on those hydrogeologic attributes w h i c h play a role in
r e g i o n a l g r o u n d w a t e r flow. T h e greatest contrasts in the basinal scale
hydrogeologic attributes can be expected to exist b e t w e e n regional recharge and
discharge areas, which represent opposite end-members of basinal flow- and
transport-conditions ( T T H 1984). It is logical, therefore, that a comparison
b e t w e e n the relevant key characteristics of regional g r o u n d w a t e r low in
recharge-and discharge-areas should provide an adequate test of the validity of
the above arguments and, thus, of the Recharge Area Concept.
M o d e l calculations
repository to the land surface; 2) repository-age of water", tr, or the travel time
of water from the land surface to the repository; 3) return route", Is, i.e. the
length of flow line leading from the repository to the land surface in the direction
of flow; a n d 4) fault route", If, or the total length of that flow line inside of a
h i g h l y c o n d u c t i v e fault w h i c h passes also t h r o u g h a repository. T h e s e
characteristics w e r e determined with reference to a point 500 m below the land
surface and 1 k m distant from the lateral boundaries of the basin (Fig. 2 ) . T h e
point is considered to represent the upper edge of a repository. T h e repository
extends over a surface area of 2x2 k m (size of the reference repository in the
Canadian disposal concept) a n d its centre coincides with the basin's lateral
boundaries at both the water divide (recharge side) a n d valley bottom (discharge
side).
T h e general p u r p o s e of the modelling e x p e r i m e n t s w a s to establish a
conceptual reference framework of the key characteristics of regional ground
water flow for the Canadian Shield. To this e n d , basinal patterns of hydraulic
heads, flow lines a n d travel times were c o m p u t e d for a variety of basin-
permeability configurations using geologic data a n d field conditions typical of
Shield conditions.
T h e g e o m e t r y of the modelled basin is constant for all variants. It simulates o n e
flank of a centrally symmetrical depression as, for instance, o n e side of a river
valley (TTH 1963). T h e width of the modelled basin's flank is 20 k m a n d it's
d e p t h at the valley is 4 k m . T h e flow domain is enclosed by i m p e r m e a b l e
boundaries o n the two sides a n d the bottom, a n d b y a sinusoidal water table, (i.e.
a sinusoidal distribution of the fluid potential) along the top (Fig. 2 ) . T h e water
table is h i g h e r b y 4 0 0 m at the divide than at the valley bottom.
Two basic, or reference, distributions of basin permeability are used, namely:
o n e h o m o g e n e o u s (Fig. 2) a n d o n e stratified into three horizontal d e p t h ranges
of different p e r m e a b i l i t i e s . T h e latter case w a s further m o d i f i e d b y t h e
introduction of highly permeable fault zones w h i c h lead with a slope from points
of fixed depths at the lateral basin boundaries to outcrops at the land surface or
horizontally, to the opposite lateral b o u n d a r y thus abutting against it without
outcropping. T h e purpose of introducing the faults w a s to examine the potential
effects o n travel times a n d flow-path lengths of highly permeable conduits
located at or n e a r a repository that might remain undetected, a n d thus ignored,
while modelling real life situations. In the different model variants, the attitude
of the faults w a s c h a n g e d b y discrete steps b e t w e e n a vertical position at the
b o u n d a r y a n d the horizontal. T h e various characteristics a n d conditions of the
m o d e l are s u m m a r i z e d in Table I.
T h e key flow properties were determined by visual interpolation from the
model's direct outputs, w h i c h are: basinal patterns of equipotentials (hydraulic
heads), flow lines, travel times (indicated b y time-step beads on flow lines) and
isochrone lines of the travel time. Specifically, travel times were estimated b y
interpolation b e t w e e n c o m p u t e d isochrone values, a n d travel distances were
expressed as relative lengths along flow lines passing through the reference
point. T h e calculations were performed b y the code F L O W N E T , developed b y
v a n E L B U R G et al., ( E N G L E N & J O N E S 1986). F L O W N E T m o d e l s t w o - d i m e n s i o n a l
SHENG, G. & TTH, ].; Using the Recharge Area Concept 285
Table 1 - /. tbla
lault: none
HDiO
" rep.: discharge N. A N. A. 9,5 X 1 0 4
3,4 X 106
fault: none
SReO stratified rep.: recharge N. A. N. A. e x 10 1,25 X 10$
fault: none
SDiO ~~~ rep.: discharge N. A N. A. 1,1 X 10b 8,0 x
6
fault: none
SRe5/1,6 stratified recharge 500 1600 3 x 106 2,0 X i o 5
SReS/13,6 500 13600 1 . 3 X 10*> 3,2X104
SRe5/2O,0 ' 500 20000 8,3 X 10b 3,0 X *
SRe5/h - 500 horizontal (3,5 to 8,7) X 105 3.0 X 10*
SRe 10/2,6 stratified recharge 1000 2600 2,96 X 106 6,5 X io*
SRe10/11,4 - 1000 11400 1,17X106 2,8 X 104
SRe10/20,0 - 1000 20000 9,5 X 105 2,7X10*.
SRe10/h ' - 1000 horizontal (1,83to5,0)xio5 2,7X10*
SD5/2.8 stratified discharge 500 2800 1,8 X 10b 2,6 X 106
SDiS/11.2 - " 500 11200 2,7 X 1 0 * 1,26 X 106
SD5/20.0 " " 500 20000 2,3 X 1 0 4
8,5 X IQ5
S0i5/h * " 500 horizontal 2,7X10" 6,5 X I Q 5
SDi 10/2,6 stratified discharge 1000 2600 6,3 X 10
4
3,0 X 106
SDi 10/11,4 " 1000 11400 2,8 X * 1.15X 10&
SOilO/20,0 " 1000 20000 2,5X104 7,0 X io5
souom 1000 honzontal 2,5 X 104 4,2 X IQ5
* general conditions
" conditions in reference (unratified and stralified) basin
discharge area, o n the other hand, b y virtue of its high age, an 8x106 year old
water could be mistaken to indicate stagnancy, yet it is only 1.1x105 years away
from the surface.
All the above n u m b e r s are modified by the presence of faults. Nevertheless, all
the parameters h a v e m i n i m u m values that can b e evaluated for realistic
conditions.
T h u s , faults c a n r e d u c e the r e t u r n - r o u t e l e n g t h to a m i n i m u m o f
approximately 20 k m for a recharge-area repository, but c a n n o t c h a n g e the 500 m
in a discharge area. Similarly, the return travel times can be significantly reduced
by faults in recharge areas: from 8x106 to 0.18x106 years in the absolute extreme
(the m i n i m u m value o f the error bar), but more likely only to approximately
0.8x106 years (Table 11, Items 7 , 8 , 9). An important point h e r e to n o t e is that, with
the exception of those recharge area faults w h i c h r u n the full l e n g t h of the basin
and outcrop in the valley bottom, n o n e of the faults can c o n v e y water directly
from the vicinity of the recharge divide to the land surface. B u t even in these
extreme cases, water that descends from the surface within o n e kilometre of the
basin's crest is forced to m o v e across these faults d o w n into the low velocity or
the stagnant z o n e of the basin and then travel its full width, largely through the
low permeability b a s e m e n t , to emerge in the discharge area s o m e 107 years later!
All these n u m b e r s can b e increased purposefully further b y selecting a basin
configuration with a lower elevation difference b e t w e e n valley a n d the upland,
a longer flank and a broader divide than those in the present model. Faults m a y
reduce the return travel times in discharge areas also. In the calculated cases
(Table 11, Items 7, 8 , 9 ) the reduction is from 1.1x105 to 2.3x104 years. (Actually, the
upper limit obtained for a n e a r vertical fault is ~ 4x105 years.) However, because
return times and return-route lengths are controlled b y local conditions in
discharge positions, modifying the regional basin characteristics, n a m e l y b y the
choice o f the basin, will have little or no effect on these parameters.
S u m m a r y and c o n c l u s i o n
1) A n e w a p p r o a c h in d e m o n s t r a t i n g the safety p e r f o r m a n c e o f an
u n d e r g r o u n d nuclear waste disposal facility is proposed. Based on the R e c h a r g e
Area Concept, it e m b o d i e s the view that a clear understanding of regional
groundwater flow patterns can be exploited so as to have g r o u n d w a t e r delay the
transport of escaped contaminants to the surface through either e n t r a p m e n t in
stagnant zones of no-flow or through transport along a very long flow trajectory.
This passive 'safe-fail' system can be seen as adding another barrier" to the
planned system of engineered/geologic multi-barriers as envisioned in the
existing general disposal concept adopted internationally.
2) In addition to the e n h a n c e m e n t of total system safety, a siting strategy based
o n the RAC m a k e s it possible to c o n f i r m m o d e l l i n g results w i t h field
m e a s u r e m e n t s that can be extrapolated far into the future.
3) From the v i e w p o i n t of contamination transport b y groundwater, recharge
areas are superior to discharge areas for the siting of high level nuclear waste
288 Fldtani Kzlny 130/2
Acknowlegdements
C o m m i t t e e for its support of this work; and to its m e m b e r s for their valuable
c o m m e n t s a n d discussions in refining the RAC. T h e research was also supported
by a Natural Sciences and Engineering Research Council grant to G. S H E N G .
References
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United States; historical perspectives. - Geological Society of America Special Paper 1 8 9 , 297-316.
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in Ecology, Vol. IV, Academic Press, 313-325.
ENGELEN, G. B . & . JONES, G. P (Eds) 1986: Development in the analysis of groundwater systems. -
International Association of Hydrogeological Sciences, Publication Number 1 6 3 , 1 2 7 - 1 4 0 .
FREEZE, R. A. &. CHERRY, J. A 1979: Groundwater. - 604 p., Prentice-Hall Inc., New Jersey.
GEOVAL 1987: A symposium on validation of geosphere flow and transport models organized by the
Swedish Nuclear Power Inspectorate, SKI, in cooperation with OECD/NEA. Stockholm.
GEOVAL 1990: A symposium on validation of geosphere flow and transport models organized by the
Swedish Nuclear Power Inspectorate, SKI, in cooperation with OECD/NEA. Stockholm, May
14-17.
SHENC, G. & TTH, ].: Using the Recharge Area Concept 289
IAEA 1960: Disposal of radioactive wastes. - Proceedings of a conference held in Monaco, Nov. 1959.
International Atomic Energy Agency, Vienna.
National Research Council, 1957: Publication 91, National Academy Press, Washington, D.C.
NEA/IAEA/CEC 1991: Disposal of radioactive wastes. Can long-term safety be evaluated? A collective
opinion of the Radioactive Waste management Committee, Advisory Committee, International
Atomic Energy Agency. - OECD Nuclear Energy Agency, Paris.
SHEMILT, L. W. & SHENG, G. 1983: An Overview of nuclear waste management. - Energy, Exploration,
and Exploitation, 2/1, 42-55.
SHENG, G., LADNYI, . & SHEMILT, L. W 1993a: Canada's High-Level Nuclear Waste Disposal Concept:
The evaluation process and a review of some aspects of the research work. - Energy Studies
Review, 5 / 3 , 1 6 5 - 1 7 9 .
SHENG, G., ELZAS, M. S. E REN, . I. & CRONHJORT, . T. 1993b:, Model validation: A systemic and
systematic approach. - Reliability Engineering and System Safety 42, 247-259.
TTH, J. 1963: A theoretical analysis of groundwater flow in small drainage basins. - Journal of
Geophysical Research 68/16, 4795-4812.
TTH, J. 1984: The role of regional gravity flow in the chemical and thermal evolution of groundwater.
- In: HITCHON, B. & WALLICK, E. I. (Eds): Proceedings, First Canadian/American Conference on
Hydrogeology; Practical applications of groundwater chemistry, Banff, Alberta, Canada, June
2 2 - 2 6 , 1 9 8 4 , Worthington, Ohio, National Water Well Association, 3-39.
TTH, J. & SHENG, G. 1996: Enhancing safety of nuclear waste disposal by exploiting regional
groundwater flow: The Recharge Area Concept. - Hydrogeology Journal 4/4, 4 - 2 5 .
Fldtani Kzlny 130/2 291-322 (2000) Budapest
A bizonytalansg rtkelse a
fldtudomnyokban
1 2 3 3
B R D O S S Y Gyrgy - F O D O R Jnos - M O L N R Pter - T U N G L I Gyula
( 8 bra, 4 tblzat)
Key words: bootstrap methods, error, fuzzy sets, reserve estimation, uncertainity
Abstract
The aim of this article is to review the main problems of uncertainty in the Earth's Sciences,
particularly in geology and to propose methods for their handling. The term error is applied in this
paper for quantified uncertainty. That is, the error is the difference between a true value and an
estimate of that value. The error consists of the following main components:
- The natural variability of geologic objects and processes.
- T h e error of measurements, where measurement bias and random deviations should be
distinguished.
- The limited possibility to sample geologic objects in space and time.
Mathematical methods are used to quantify uncertainty. Unfortunately, the theory of probability has
certain limitations when applied to geological problems:
- The additivity axiom does not allow gradual transitions from one population to the other.
- Several statistical methods prescribe repeated experiments, impossible to perform in many
geological investigations, e.g. repeated drilling of borehole sets with small changes of location.
The statistical study of closed systems" leads in several cases to spurious results.
For the handling of uncertainties and error the authors suggest the application of some up to date
mathematical methods, such as:
- Geostatistics, that is the theory of regionalized variables.
- Interval analysis.
- Fuzzy set theory (see Figure 1).
- Bootstrap methods.
- Jacknife methods.
- Cross validation.
In the next section the authors review generalized steps of the geologic investigations respective to
uncertainty and error. The following steps are discussed:
- Representative sampling of geologic objects in space and time.
- Measurements and observations on geologic objects.
- Descriptive statistical evaluation of the data obtained.
- Inferential evaluation and modelling.
1
1055 Budapest, Kossuth L. tr 18
2
llatorvostudomnyi Egyetem Biomatematikai s Szmtstechnikai Tanszk 1078 Budapest,
Istvn t 2.
3
Golder Associates Hungary, 1021 Budapest, Hvsvlgyi t 54.
292 Fldtani Kzlny 130/2
Four tables were constructed containing the main subjects of the topics listed above, the reasons of
uncertainty for each case and the suggested mathematical methods to solve the problems. The spatial,
the temporal and the complex predictions are discussed separately and methods are suggested for the
solution of each problem. The most difficult task is to perform predictions for complex systems, such
as reserve estimations of mineral deposits, environmental impact statements for constructions in and
on geologic objects, safety assessments for the disposal of toxic and radioactive waste etc. According
to our knowledge, only traditional deterministic and stochastic methods were applied so far to handle
the above listed tasks.
Unfortunately, the meaning and role of uncertainty, error, random events and risk are often
confounded in the articles dealing with these problems. Therefore, definitions and explanations of
these notions are presented in this paper.
The fuzzy methods are considered by the authors to be particularly efficient in solving the
problems of uncertainty and error in geology. Four examples are presented to illustrate the
application of the method:
Differential thermogravimetry is suitable to detect the mineral composition of rock and soil
samples. The M O M derivatograph with an attached computer measures the phase composition with
an average 10% weight error. The limit of detection varies from 1 to 5%, depending on the chemical
and mineral compositions of the sample. 36 rock samples, collected from the late Permian Boda
Claystone Formation (southern Hungary) were measured and evaluated first by the traditional
method, furnishing crisp values and in a second step by the fuzzy method. It is of top importance that
the calculation of the fuzzy numbers occurred jointly by the thermoanalist, the geologist and the
mathematician, thus assuring a maximum level of measurement and geologic experiences. The results
of a selected sample are presented on Figure 2. The statistical evaluation of the fuzzy numbers of all
samples opened the possibility to distinguish the natural variability of the formation from the errors
of measurement. Ranking the minerals according to the amount of measurement error (expressed by
the fuzzy numbers) furnished new information about the methodology of the measurements and the
properties of the formation. The results of these evaluations will be published in a separate paper.
A similar evaluation was carried out on 36 samples collected from the same formation, by using
X - r a y diffractometry and X-ray spectrometry. The average error of the phase analysis was 10% and
the limit of detection varied from 0.5 to 5%. Figure 3 illustrates the crisp and fuzzy results of the phase
analysis of one rock sample. Here again a statistical study of the crisp and fuzzy numbers was carried
out. The results were correlated with different rock features. These results will also be published in a
separate paper.
The measurement of water transmissivity in fractured rocks is a particularly complex and difficult
problem. 32 packer measurements from boreholes in the above mentioned Boda Claystone Formation
were evaluated by traditional and fuzzy methods. Additionally 104 packer measurements from
boreholes in the granite massif of Mrgy, southern Hungary, were also evaluated. The results of
some measurements represented by fuzzy numbers are shown on Figures 4. 5. and 6.
The identified mineral deposits are of particular geologic and economic interest. Experiences show
that in many places the following basic mathematical rules are not observed when calculating ore
reserves:
- Ranges of influence are not calculated for the main parameters of the calculations.
- Normality of the main features is not checked by corresponding normality-tests, however non
normal, highly asimmetric distributions are frequent. In such cases robust M-estimators or non-
parametric methods should be applied.
- The results of the reserve calculations are presented in the form of point-estimates, instead of
interval estimates, referring to an adequately chosen level of confidence.
In the above cases the ore reserves are significantly biased. Furthermore, the traditional methods
do not allow sufficient insight into the uncertainties and errors of the calculations. To eliminate these
shortcomings, a new methodology is presented by the authors, based on the fuzzy set theory:
Determination of the area of the reserves. First the geologically most probable contours are
constructed, taking into account all available geological and geophysical information about the
deposit.The minimum area is then determined for the case when all features (circumstances) take
BRDOSSY Gy. et al: A bizonytalansg rtkelse a fldtudomnyokban 293
most unfavourable values. In a third step the maximum area is calculated for the most favourable
values. Figure 7 represents an example of these extreme boundaries, taken from the Halimba bauxite
deposit (Hungary). Finally a triangular fuzzy number is constructed by these three results.
Determination of the average thickness. First normality tests are performed and the corresponding
methods are applied to calculate the average thickness. The standard error of the mean is taken for
the core" of a trapezoidal fuzzy number. A confidence interval is calculated, using 95 % level of
confidence. This interval corresponds to the Support" of the fuzzy number, representing the average
ore thickness.
Determination of the average bulk density of the ore. First step is the determination of the
analytical error of the bulk density determinations. Normality test for the distribution of analytical
results follow. The standard error of the mean gives the core, the confidence interval at 95% level of
confidence the support of the resulting trapezoidal fuzzy number.
Calculation of the reserves. The three fuzzy numbers are multiplied following the rules of fuzzy
arithmetic. The resulting fuzzy number represents the ore reserves (Figure 8). The minimum and
maximum values of the support indicate only the two extreme situations, with the best and worst
conditions. The real range of possibility is indicated by the core of the fuzzy number.
Calculation of ore quality occurs in the same way as for the quantity of ore.
Recoverable ore reserves can be also calculated when taking into account the planned mining
losses and contaminations. The errors of these two parameters are included into the construction of
the corresponding fuzzy number.
Commercial reserves can be calculated by taking into account the corresponding technical and
economic parameters. The errors of these parameters serve as input values for the construction of the
corresponding fuzzy number. These fuzzy numbers allow the calculation of the probability and of the
amount (consequences) of investement and mining risk.
For the detection of undiscovered mineral deposits - in known districts - special probabilistic
methods have been developed, such as the weights-of-evidence, the weighted logistic regression
(ACTERBERG et al.1993) and the probabilistic neural networks methods (SINGER & KOUDA 1997,1999).
Conclusion. A systematic study of uncertainty and error is suggested by the authors for all steps of
geologic investigations. A great advantage of the fuzzy approach is the interdisciplinary cooperation
of the geologist, the mathematician and the expert of the given field of study. The application of the
above listed new mathematical methods should take place in as many fields of geology as possible.
sszefoglals
Alapvet fogalmak
HAGYOMNYOS MDON
FUZZY TAGSGFGGVNYEKKEL
Idbeli elrejelzsek
P l d k a fuzzy m d s z e r alkalmazsra
Termikus mdszer.
Rntgendiffraktomteres mdszer
V i l g s z e r t e s z m o s m d s z e r t h a s z n l n a k a kvantitatv r n t g e n o g r f i a i
fzisanalzisre. Az ltalunk vizsglt m d s z e r t az MTA G e o k m i a i Kutat
Laboratriumban (GKL) dolgoztk ki a h e t v e n e s vekben. Ez a m d s z e r mind
az adott s v n y o k relis szerkezett, mind a minta vegyi sszettelt figyelembe
veszi. Az elmlt v e k b e n a Bodai Aleurolit Formci kzeteibl, a fed s fek
kzetekbl vett kzel 100 mintn vgeztek a GKL-ben kvantitatv rntgenogrfiai
fzisanalzist R K A I Pter akadmikus vezetsvel. Vele n z t k t a vizsglati
e r e d m n y e k e t s ksztettk el 36 k z e t m i n t a tagsgfggvnyeit. rtkes
segtsgrt e h e l y e n fejezzk ki hls ksznetnket. A vizsglati e r e d m n y e k
1 0 % hibahatr kztt mozognak. Az egyes svnyok kimutathatsgnak
hatra 0,5-tl 5%-ig terjed. A mrsi hibk e mdszernl h r o m tnyezbl
fakadnak:
308 Fldtani Kzlny 130/2
HAGYOMNYOS KIRTKELS
Fig. 2 Mineral composition obtained by derivatograph study. Above crisp numbers, below fuzzy numbers. Albitic
claystone from the Upper Permian Boda Siltstone Formation. Borehole Number BAT-10, 85.7 m depth
3. bra Rntgendiffraktomteres vizsglattal nyert svnyos sszettel brzolsa hagyomnyos (crisp) s fuzzy szmokkal. Albitfszkes agyagk a ks-perm
kor Bodai Aleurolit Formcibl. BAT-4 frs 1169,2 mterbl
Fig. 3 Mineral composition obtained by X-ray dijfractometry. Albitic claystone from the Upper Permian Boda Siltstone Formation. Borehole BAT-4, 1169.2 m depth
BRDOSSY Gy. et al: A bizonytalansg rtkelse a fldtudomnyokban 311
r e p e d s r e n d s z e r e k irnyrl, a k k o r a b i z o n y t a l a n s g o t l e g i n k b b azzal
cskkenthetjk, ha ragaszkodunk a fggleges frsokhoz.
A n a g y m r t k vltozkonysg miatt k n n y e n elfordulhat, h o g y a frlyuk
e g s z e n rvid szakaszhoz igen magas vzvezet kpessg tartozik. Ezrt a
leghelyesebb, ha a frlyuk teljes hosszt szkennelsszeren vgigvizsgljuk,
e g y m s t a szleken kis mrtkben tfed, lehetleg egyforma hosszsg,
1 0 - 2 5 m-es vizsglati szakaszokkal.
A repedsrendszerek tbbfle orientcija s sszekapcsoldottsga miatt
ltalban n e m tudjuk, hogy mekkora a mrs hattvolsga, azaz h o g y az adott
v z v e z e t k p e s s g m i l y e n i r n y b a n m i l y e n tvolsgra t e r j e s z t h e t ki.
Rendszerint m g nagy frssrsg esetn sem lehet a vzvezet kpessget az
egyes frsok kztt korrellni. Ez annl is inkbb gy van, mivel a vzvezet
k p e s s g m g e g y e t l e n k o n k r t r e p e d s skja m e n t n is akr h r o m
n a g y s g r e n d e t vltozhat, a r e p e d s szlessgnek, ill. a r e p e d s k i t l t s e k
llapotnak fggvnyben. Ezrt a frsok szmt, vagyis a vizsglt szakaszok
sszhosszt csak olyan mrtkig clszer nvelni, h o g y a transzmisszivitsok
eloszlst megfelelen tudjuk jellemezni. A frsok kztti interpolcihoz
ltalban a tektonikai s geofizikai vizsglatok e r e d m n y t is figyelembe kell
v e n n i , illetve valamely frs ktvizsglatval egyidejleg a kzelben lv tbbi
frsban is szlelseket kell vgezni (egymsrahats-vizsglat).
A k t v i z s g l a t o k sorn valamilyen j l kontrolllhat m d o n - pldul
szivattyzssal (termeltetssel) v a g y vzbesajtolssal (nyeletssel), illetve a
termeltets v a g y nyelets megszntetsvel - hatst gyakorolunk a vztroz
k p z d m n y e k r e . Az erre a szablyozott jelre kapott vlasz (nyomsvltozs,
v z h o z a m v l t o z s ) alapjn k v e t k e z t e t h e t n k a k p z d m n y e k v z v e z e t
k p e s s g r e . A j e l a d s szablyozsi m d j a alapjn tbbfle ktvizsglati
m d s z e r t klnbztethetnk meg. Pldul az lland h o z a m tesztek sorn a
termelt vagy besajtolt vzhozamot a kt szjnl lland rtken tartjuk, s a
vizsglt szakaszban mrjk a nyomsvltozst.
Az lland h o z a m teszt bizonytalansgnak egyik forrsa, h o g y mennyire
tudjuk a vzhozamot lland szinten tartani. Alacsony vzvezet kpessgek
esetn m g viszonylag kisebb vzhozam-ingadozsok is m e g n e h e z t h e t i k a teszt
k i r t k e l s t . E b i z o n y t a l a n s g c s k k e n t s n e k az a l e g j o b b m d j a , ha
h u z a m o s a b b idej vztermels vagy nyelets utn a kutat hirtelen lezrjuk, azaz
a v z h o z a m o t zrusra vltoztatjuk, s mrjk a vizsglati szakaszon a nyoms
felfutst, ill. cskkenst.
Az l l a n d h o z a m tesztek b i z o n y t a l a n s g n a k e g y m s i k forrsa a
n y o m s m r s pontossga. M a mr igen nagy rzkenysg, kzvetlenl a
vizsglati szakaszba t e l e p t h e t n y o m s s z o n d k llnak r e n d e l k e z s r e . Az
a l a c s o n y v z v e z e t k p e s s g r e p e d e z e t t kristlyos k z e t e k , v u l k n i t o k ,
aleuritok vizsglathoz szksg van ilyen pontos s kltsges mszerekre, a
porzus k p z d m n y e k tbbsge esetben azonban kisebb rzkenysg
n y o m s m r k is megfelelnek, st, nyitott kutakban szmos esetben elegend a
megfelel srsg vzszintmrs.
A ktvizsglat sorn mrt nyomsadatokbl n e m lehet kzvetlenl meg
h a t r o z n i a k p z d m n y e k transzmisszivitst. Az szlelt adatok ugyanis csak
312 Fldtani Kzlny 130/2
A szilrd svnyvagyonbecsls
Fig. 6 Fuzzy membership functions of the tests performed in the Delta-6 borehole
Fig. 7 The smallest and the largest possible extent of the Halimba 11/SW bauxite ore body
Bakonyi Bauxitbnya Kft. hivatalos vagyonszmtsa
8. bra A Halimba II/DNY bauxit rctest fldtani vagyonnak kiszmtshoz felvett fuzzy szmok A: alapterlet, B: tlagos bauxitvastagsg, C: tlagos bauxit
trfogatsrsg, D: fldtani vagyon. Fggleges vonal: a hagyomnyos vagyonszmts eredmnyei
Fig. 8 Fuzzy numbers applied to the bauxite ore reserve estimation of the Halimba WSWore body A extent, average bauxite thickness, average bulk density, Dore tonnage.
The vertical lines represent the results of the traditional ore reserve estimation
320 Fldtani Kzlny 130/2
Kvetkeztetsek
J a v a s o l j u k , h o g y a j v b e n m i n d a t u d o m n y o s , m i n d a z alkalmazott
fldtudomnyi kutatsoknak legyen szerves rsze a bizonytalansg vizsglata,
szmszerstse ill. a hibahatrok cskkentse
M i n l t b b s z a k t e r l e t e n ki k e l l e n e p r b l n i a t a n u l m n y b a n emltett
mdszereket, elssorban a fuzzy elmlet mdszereit
M e g k l n b z t e t e t t fontossgot tulajdontunk az svnyvagyon becslsek s a
biztonsgi e l e m z s e k korszerstsnek, hibahatraik m e g h a t r o z s n a k
A bizonytalansg cskkentsnek ltalunk javasolt mdja interdiszciplinris
e g y t t m k d s t kvn a fldtudomny, a matematika s a szmtstechnika
szakemberei kztt
Javasoljuk, h o g y az egyetemi oktatsban is kapjon szerepet a bizonytalansg,
valamint a hibahatrok kiszmtsa
BRDOSSY Gy. et al: A bizonytalansg rtkelse a fldtudomnyokban 321
Ksznetnyilvnts
Irodalom - References
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Fldtani Kzlny 130/2 323-336 (2000) Budapest
Hrek, ismertetsek
Helyreigazts
Knyvismertets
15. A kutatsi programok fldtani zrjelent vagy dolga akadt klfldi (karszt)bauxitkutat
sek s vzfldtani jelentsek elksztsben r intzmnyek dokumentcijval, Jamaiktl
demben rszvevk nvsora (abc sorrendben) Grgorszgon s Irnon t Vietnamig. (A later
16. A frt aknk egyes adatai itbauxit-kutats felttelei s kvetelmnyei
17. A bauxitipar szervezete s fgeolgusai 1950 kzismerten egszen msok.) Mindez vilgosan
s 1997 kztt bizonytja, hogy a dicsretesen nirnikus nt
18/a Bauxittermels s felhasznls (1926-1998) val ellenttben: AI2O3. x H 0 " egyltaln nem
2
18/b A bauxittermels terletenknti megosz csak ennyit tud egy jlnevelt bauxitkutat."
lsa (1926-1998) Vgl a Bauxitkutat Vllalat egy olyan jel
19. Magyarorszg bauxittermelse 1926 s 1998 legzetessgt szeretnm megemlteni, amely
kztt kt-ban mgis hinyzik VIZY Bla feldolgozsbl. Nem
20. Magyarorszg bauxitvagyona (1950-1996) rhat fel neki, mert nem szakmai termszet.
21. Magyarorszg ismert bauxitkszletnek Arrl van sz, hogy a Magyar-Szovjet Bauxit-
alakulsa (1950-1996) Alumnium RT Bauxitkutat Expedcija s
22. A fontosabb esemnyek Kronolgija utdja, a mr tisztn magyar Bauxitkutat
Vllalat 1950-tl az 1960-as vek vgig politikai
Idzem az sszefoglalsbl: Haznk mindig a menedkhely is volt, ahol nyugodtan s meg
bauxitipar lvonalban volt... A kutats j o becsltn dolgozhattak olyan mszaki s kutat
gosultsgt s eredmnyessgt bizonytja, hogy szakemberek, akiket akkoriban egyetemeken
1926-tl napjainkig 103 milli tonna bauxitot ter vagy/s tudomnyos kutatintzetekben nem
meltek ki bnyinkbl, amelynek tbb mint lttak szvesen. Ez a kderpolitika bevlt: ezek a
ktharmadt hazai timfldgyraink dolgoztk szakemberek legjobb kpessgeik szerint dol
fel... A kitermelt bauxit 70%-a kerlt ki mly- goztak feladataikon, s mint az adatokbl vil
mvelses bnykbl... 60 milli tonna bauxitot gosan kitnik, nem is eredmnytelenl.
3
sszesen 4,7 millrd m vz kiemelsvel lehetett
csak megoldani..." Az itt jrt francia bauxitgeo Ezrt (is) ksznettel tartozunk az akkori
lgusok szerint ez olyan, mint tenger all ter vezetknek.
melni bauxitot.
Hoz kell tenni ehhez, hogy a kutats doku DUDICH Endre
mentlsa mindvgig rendkvl alapos s pon
tos volt, olykor a (nha bizony bosszant) pe
dnssgig menen. A zrjelentsek tartalma a
nemzetkzi sszehasonltsban is pldaszer:
legfeljebb a tlzottnak vlt rszletessg kpez
hette kritika trgyt. Errl meggyzdhetett - s
egyrtelmen meg is gyzdtt - minden ma
gyar bauxitgeolgus, aki klfldn is dolgozott
326 Fldtani Kzlny 130/2
Jubill tagtrsaink
B r e z s n y n s z k y Kroly
az M F T elnke
85 ves
N a g y Lszln
(1914. jl. 5.)
80 ves
K U N Bla P r d y Mihly*
(1919. jl. 2.) (1919 jl. 25)
80 ves
URBANCSEK J n o s SZEPESHZY K l m n
(1919. okt. 2 3 . ) (1919. okt. 2 5 . )
KoTSis Tivadar
(1919. dec. 30.)
328 Fldtani Kzlny 130/2
75 ves
J H E L Y I Gyrgyn
(1924. okt. 25.)
70 ves
70 ves
P A P A J C S I K Mrtonn F B I N Gyula
(1929. nov. 11.) (1929. nov. 16.)
330 Fldtani Kzlny 130/2
A mlt
A jelenlegi helyzet
Tisztelt Elnk r!
Tisztelt Miniszter r!
Tisztelt Elnk r!
Tisztelt Kpvisel r!
Tisztelettel:
Budapest, 1999. jnius 14.
POKORNI Zoltn
oktatsi miniszter
sszelltotta : P I R O S O l g a
Haas, J. 1999: Genesis of Late Cretaceous Basin. - Berichte der Deutschen Miner-
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Tartalom - Contents
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Bevezet szavak A ma geolgija a holnaprt" cm konferencin elhangzott eladsok el . 193
Lszl KOVCS - Gbor HMOS - Jzsef CSICSK: Actual state of the site characterisation
programme of the Boda Siltstone Formation - A Bodai Aleurolit Formci telephely-
jellemzsi programjnak jelenlegi llapota 197
Wernt BREWITZ - Ulrich NOSECK: The long-term safety of underground waste repositories
- A key issue for research and development - Felsznalatti hulladktrolk hossztv
biztonsga - kutats s fejleszts 207
Mieke De CRAEN - Dominique DELLEUZE - Geert VOLCKAERT - Alain SNEYERS - Martin : U - T h
series disequilibrium studies on Boom Clay - A natural analogue of radionuclide
migration in argillaceous sediments - A nemegyenslyi U-Th sorozat tanulmnyozsa a
Boomi Agyagban - a radioaktv elemvndorls termszetes analgija agyagos ledkekben 219
Ion DURDUN - Cristian MRUNTEANU: Romanian LILW disposal - site selection, characterization
and investigation programme - Kis- s kzepes radioaktivits hulladklerak
Romniban - telephely kivlasztsi, jellemzsi s kutatsi program 229
Philippe LALIEUX: International co-operation regarding site characterisation and site evaluation
for geological repository systems for long-life radioactive waste - Hossz lettartam
radioaktv hulladkok fldtani trolrendszereinek telephely-jellemzsre s rtkelsre
vonatkoz nemzetkzi egyttmkds 239
Roma KANOPIENE - Vytautas MARCINKEVICIUS: Possibilities for developing deep radioactive
waste repository in Lithuania - Mlysgi radioaktv hulladktrol teleptsnek
lehetsgei Litvniban 251
Duke U. OPHORI: Simulating large scale groundwater flow for waste disposal purposes -
Nagylptk talajvzramls modellezse hulladkelhelyezsi clbl 263
Grant SHENG - Jzsef TTH: Using the Recharge Area "Concept as a strategy for siting
underground nuclear waste repositories - Az utnptldsi terlet koncepci (Recharge
Area Concept) stratgiai alkalmazsa felszn alatti radioaktv hulladktrol kutatsban . . . 275
BRDOSSY Gyrgy - FODOR Jnos - MOLNR Pter - TUNGLI Gyula: A bizonytalansg rtkelse
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Hrek, ismertetsek - News and reviews 323
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