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Environ. Sci. Technol.

2011, 45, 666–672

Optical Remote Sensing to Quantify tracked vehicles ranged from 8.3 to 72.5 kg PM/km for PM10
and 1.1 to 17.2 kg PM/km for PM2.5, and there was no obvious
Fugitive Particulate Mass Emissions correlation between PM emission and vehicle speed. The
emission factor for the helicopter flying at 3 m above the ground
from Stationary Short-Term and ranged from 14.5 to 114.1 kg PM/km for PM10 and 5.0 to 39.5
Mobile Continuous Sources: Part II. kg PM/km for PM2.5, depending on the velocity of the helicopter
and type of soil it flies over. Fugitive PM emissions by an
Field Applications airborne helicopter were correlated with helicopter speed for
a particular soil type. The results from this range-resolved
KE DU* ORS method were also compared with the data obtained with
Institute of Urban Environment, Chinese Academy of Sciences, another path-integrated ORS method and a Flux Tower
Xiamen, China method.

WANGKI YUEN, WEI WANG, AND 1. Introduction


MARK J. ROOD
Fugitive particulate matter (PM) emissions into the atmo-
Department of Civil and Environmental Engineering, sphere have been characterized with emission factors for a
University of Illinois, 205 N. Mathews Ave, Urbana, variety of activities such as traveling vehicles on roads (1),
Illinois 61820, United States
agriculture activities (2) (3), and natural wind erosion (4).
These dust plumes are of interest due to their ability to reduce
RAVI M. VARMA visibility and the need to characterize their emission proper-
Department of Physics, National Institute of Technology ties for PM emission inventories. Particles with diameters
Calicut, Calicut 673601, India <10 µm (PM10) were shown to reduce visibility from local (5)
(6) to global scales (7).
RAM A. HASHMONAY Military training and testing operations at the United
ENVIRON, 88 VilCom Circle, Suite 185, Chapel Hill, North States Department of Defense (DoD) facilities in desert areas
Carolina 27514, United States generate fugitive dust plumes (8). The dust generating
activities studied in this research included back blast from
BYUNG J. KIM AND MICHAEL R. KEMME firing artillery, movement of tracked vehicles, and airborne
U.S. Army Engineer Research and Development Center, helicopters. Many DoD installations are close to Federal Class
Construction Engineering Research Laboratory, 2902 I areas. PM emissions from training and testing activities
Newmark Dr., Champaign, Illinois 61826-9005, United States within those installations have caused concerns about
compliance with the Regional Haze Rule. In addition,
Received June 4, 2010. Revised manuscript received quantification of emission factors for these sources is
October 15, 2010. Accepted November 14, 2010. important to develop emission inventories as well as to serve
as the source term for air quality modeling to predict the
ambient PM concentrations at and near DoD facilities.
Therefore, characterizing fugitive PM emissions from military
Quantification of emissions of fugitive particulate matter training and testing activities is among the top priorities of
(PM) into the atmosphere from military training operations is the environmental quality/compliance technology research
and development of DoD.
of interest by the United States Department of Defense. A new
range-resolved optical remote sensing (ORS) method was Improvements in optical remote sensing (ORS) technolo-
gies and methodologies have led to the development of new
developed to quantify fugitive PM emissions from puff sources
methods to characterize fugitive PM emissions. In a study
(i.e., artillery back blasts), ground-level mobile sources (i.e., to quantify PM10 emissions from agricultural tilling in
movement of tracked vehicles), and elevated mobile sources California, light detection and ranging (lidar) profiles were
(i.e., airborne helicopters) in desert areas that are prone to used to verify the heights and shapes of plumes that were
generating fugitive dust plumes. Real-time, in situ mass derived from a point-sampling method (9). Vertically scan-
concentration profiles for PM mass with particle diameters ning lidar measurements were also compared with the results
<10 µm (PM10) and <2.5 µm (PM2.5) were obtained across the from point measurement coupled inverse modeling for
dust plumes that were generated by these activities with this determining emission rates from point and diffuse area
new method. Back blasts caused during artillery firing sources. The comparison showed good agreement (10). Also,
were characterized as a stationary short-term puff source an open path-laser transmissometer (OP-LT) was coupled
with vertically distributed dust monitors to determine the
whose plumes typically dispersed to <10 m above the ground
dust mass fluxes across a vertical plane (11).
with durations of 10-30 s. Fugitive PM emissions caused by
A novel ORS method was developed with this research
artillery back blasts were related to the zone charge and ranged using a vertically scanning micropulse lidar (MPL, National
from 51 to 463 g PM/firing for PM10 and 9 to 176 g PM/firing Aeronautical and Space Administration, Model Type 4, Sigma
for PM2.5. Movement of tracked vehicles and flying helicopters Space Corp.) mounted on an automated positioner (AL-4011-
was characterized as mobile continuous sources whose 1E, Orbit Communication Systems Inc.), two open path-
plumes typically dispersed 30-50 m above the ground with Fourier transform infrared spectrometers (OP-FTIR, IMACC,
durations of 100-200 s. Fugitive PM emissions caused by moving Inc., and Midac, Inc.), two OP-LTs (IMACC Inc.), and
anemometers (R.M. Young Inc., Model 09101) to characterize
* Corresponding author phone: +86-592-6190767; e-mail: dust plume geometry and to quantify PM mass concentra-
kdu@iue.ac.cn. tions and emission factors for select military activities. This
666 9 ENVIRONMENTAL SCIENCE & TECHNOLOGY / VOL. 45, NO. 2, 2011 10.1021/es101906v  2011 American Chemical Society
Published on Web 12/13/2010
ORS method was previously described but is succinctly larger the charge zone number, the more energy is transferred
described here for clarity (12). The MPL signals were to the ground when the artillery fires the projectile.
processed to describe time-dependent one-dimensional (1- 2.2. Fugitive PM Emissions from Ground-Level Mobile
D) and then two-dimensional (2-D) PM light extinction Sources (i.e., Movement of Tracked Vehicles). The same
profiles across the dust plumes. OP-FTIRs and OP-LTs ORS systems that were used to measure fugitive PM emissions
determined the particle size distributions of the PM and the from artillery back blasts were also deployed to measure dust
PM’s light extinction mass extinction efficiencies (12). The emissions from the movement of tracked vehicles at YTC.
light extinction profiles and the light extinction efficiencies However, the MPL was mounted on a positioner for the MPL’s
were used to compute the 2-D real-time dust mass con- laser beam to scan radially in the vertical direction through
centrations along the entire optical path of the MPL when the plumes. The MPL was operated parallel to the paths
intersecting the plumes. The PM mass emissions were then of the tracked vehicles and was located 30 m downwind from
calculated by integrating the real-time 2-D mass concentra- the vehicle path and 300 m away from the two sets of OP-
tion profiles with the concurrent wind speed and direction FTIRs/OP-LTs (Figure 3, ref 13). A 1.2 m high × 2.4 m wide
measurements. In addition, the plume’s properties, such as metal mesh was used instead of the previously described
its dimensions, were characterized based upon the 2-D real- metal pole as the reflective target to provide a larger and
time PM mass concentration profiles. more stable target for the MPL. This reflective target was
located on the opposite side of the plumes from the MPL so
2. Site Locations, Emission Source Types, and Field that backscatter signals from the reflective target and plume
Sampling Methods did not overlap. Two anemometers were located on the scissor
lift at the same location as the retroreflectors. Two sets of the
Fugitive PM plumes generated by back blast from firing OP-FTIR/OP-LT systems were operated parallel and within
artillery, movement of tracked vehicles, and airborne heli- 1 m of the MPL’s optical path but were offset 300 m from the
copters are described here. The types of sources and ground MPL so they were located within the dust plumes. Two
surfaces were selected to represent the frequently used retroreflectors were aligned at a horizontal distance of 90 m
operational conditions that generate fugitive dust at DoD away from their respective OP-FTIR/OP-LT systems. One
training and testing facilities. For each activity, the plumes retroreflector was 1.5 m above the ground and the other one
were characterized, and emission factors were determined was 10 m above the ground (Figure 3, ref 13). The ORS systems
under select operating conditions with the range-resolved continuously collected data during the movement of the
ORS (RR-ORS) method (13). Results are presented in this tracked vehicles. Two types of ground surfaces were evaluated
paper and are compared with the results obtained with the during this field campaign. One surface had an unimproved
path-integrated ORS (PI-ORS) (14) and Flux Tower (15, 16) road with bare soil on the road and the other one was initially
methods to quantify fugitive PM emissions. covered with desert vegetation, but the vegetation cover was
removed, and the bare soil was exposed after a few trips of
This RR-ORS method is with a spatial resolution of up to
tracked vehicle movement along the desert vegetation.
15 m and temporal resolution up to 1 s. The MPL was located
2.3. Fugitive PM Emissions from an Elevated Mobile
300-500 m away from the plume, and its optical path was
Source (i.e., Airborne Helicopter). The field configuration
scanned radially in the vertical direction with the positioner
of the ORS systems to measure fugitive PM emissions from
to characterize plumes that were up to 40 m high and up to
an airborne helicopter was similar to that used for the tracked-
100 m wide (13). vehicle field campaign. A Bell 210 helicopter flew parallel to
2.1. Fugitive PM Emissions from Puff Sources (i.e., Back the optical paths of the ORS instruments at 100-150 m
Blasts during Firing of Artillery). The MPL operated in a upwind of their optical paths. When approaching the test
weatherproofed and temperature-controlled trailer that was site, the helicopter first descended to a height of 3 m above
located 400 m away from the two OP-FTIR/OP-LT systems. the ground and flew over the test site at a constant speed for
The OP-FTIR/OP-LT systems were set up 50 m downwind at least 100 m and then withdrew. Two types of sites were
from the artillery and directed toward the retroreflectors. evaluated during this field campaign. One site is called “Desert
One OP-FTIR/OP-LT system had a horizontal optical path Pavement,” which was covered with gravel. The other site is
collinear with the MPL’s laser path. The other OP-FTIR/OP- called “Disturbed Soil,” which was covered with a 2-5 cm
LT system had an optical path in the same vertical plane but thick layer of dry loose soil.
with a slant angle. The retroreflectors for the OP-FTIR/OP- The MPL was deployed parallel to the two OP-FTIR/OP-
LT systems were located 100 m horizontally from the OP- LT systems, which had a horizontal optical path of 130 m.
FTIR/OP-LT systems but on the opposite side of MPL. The However, the MPL was operated 300-500 m away from the
retroreflectors were 1.5 m above the ground and 10 m above OP-FTIR/OP-LT systems to compensate for the MPL’s optics
the ground (ref 13, Figure 2). The centerline of the plume requirements (13), with the OP-FTIR/OP-LT systems located
was located between the OP-FTIRs/OP-LTs and their re- in the plumes. The MPL’s reflective mesh target was located
spective retroreflectors (Figure 2, ref 13). Each corner of the 700 m from the MPL along the optical path of the MPL so
trailer was lifted with a hydraulic jack to stabilize the trailer that backscatter signals from the MPL and plume did not
and the optical path of the MPL’s laser. The direction of the overlap. One OP-FTIR/OP-LT system operated horizontally
MPL’s optical path was fixed in the horizontal direction and while the other system operated at a slant angle with its
directed perpendicular to the wind’s direction. A 1.3 cm wide retroreflector located 10 m above the ground. The ORS
and 2.4 m high metal pole was used as the reflective target continuously collected data during the helicopter tests
and was located 600-1000 m away from the MPL and in the (Figure 4 in ref 13).
optical path of the MPL so that the backscatter signals from Three research groups participated in this field campaign.
the reflective target and plume did not overlap. Two Each of the three groups simultaneously measured the PM
anemometers were located on the scissor lift at the same mass emission for the same source using a different method.
location as the retroreflectors. The MPL and OP-FTIR/OP- University of Illinois in collaboration with a consulting
LT systems continuously collected data during the firing of company, ARCADIS, and Construction Engineering Research
the artillery. Dust emissions from the firing of two artillery Lab (CERL) of the U.S. Army Engineer Research and
with projectile models M549A1 and M107 were measured Development Center, developed the “RR-ORS” method.
for charge zones 2 and 8S, respectively. Charge zones were ARCADIS developed a method based on path-integrated
selected based on how far the projectiles were to travel. The measurements with two sets OP-FTIRs/OP-LTs to determine

VOL. 45, NO. 2, 2011 / ENVIRONMENTAL SCIENCE & TECHNOLOGY 9 667


the optical properties of the plume, two anemometers to reasons could be the difference in detected portion of the
determine the wind’s velocity and direction, and the MPL to plumes. Flux tower method relied on the sensors installed
determine the geometry of the plume to quantify PM10 and on the 10-15 m high towers. With the high sensor density
PM 2.5 fluxes and mass emission factors (12) and is referred of one sensor per two meters, Flux Tower method provides
to here as the “PI-ORS” method. The Desert Research Institute measurements at much higher spatial and temporal resolu-
(DRI) used up to three flux towers with extractive point tion than ORS method in the lower part of the plumes, whose
measurements devices mounted on the towers. Two 15 m scanning paths are 10-15 m apart and scanning cycles are
and one 9 m tall towers were typically located 50 m downwind 10-15 s long. However, the plumes were detected with the
from the source (17). Five pairs of calibrated PM10 and PM2.5 MPL as high as 50 m, which can be seen from both profiles
samplers (TSI 8520 DustTraks) were installed at five levels in manuscript Part I. Another possible influence in the results
on each of the towers to measure the PM mass concentrations. is the degree of data filtering that occurred for each method.
These mass concentrations were then combined with The ORS technique used all test results unless there was a
measured wind speed and direction values and the duration clear physical justification to not include the results in the
for each event to determine PM mass emission factors. This report (e.g., wind direction or scanning angle caused the
method is referred to here as “Flux Tower” method. plume to miss the MPL’s measurement plane), which may
not be the same as Flux Tower method. Both methods have
3. Results and Discussion advantages as well as drawbacks, and we cannot say which
3.1. Fugitive PM Emissions from Back Blasts during Firing one is better. It might be better to use Flux Tower method
of Artillery. PM emission factors for artillery back blasts with for low altitude plumes and ORS method for high altitude
select projectile type, charge model, and charge zone are and/or elevated plumes.
described in Table 1. The larger charge zone, with more power Figure 2 describes how PM10 mass emission factors vary
dissipated upon firing, provided more PM due to the back with vehicle speed during the events that the tracked vehicles
blast. The arithmetic mean ( standard deviation for PM10/ traveled. Statistical hypothesis tests show that there is no
PM2.5 emission factors for the M107 projectile, with M3A1 significant linear dependence of PM emission factor on
propelling charge, and 2 charge zone was 192 ( 65 g PM/ vehicle speed for all three types of tracked vehicles at the
firing/62 ( 200 g PM/firing, respectively. The arithmetic mean confidence level of 95% (0.68 < p < 0.95). The average emis-
( standard deviation for PM10/PM2.5 emission factors for the sion factors for each type of vehicle are 1.25 × 103 g PM10/km
M549A1 projectile, with M203A1 propelling charge, and 8S for the BFV, 4.74 × 103 g PM10/km for the M1A1, and 2.10 ×
charge zone was 301 ( 67 g PM/firing/109 ( 155 g PM/firing, 103 g PM10/km for the M113.
respectively. Figure 2 also compares the results obtained with the three
PM mass emission factors for PM10 and PM2.5 were also PM mass emission measurement methods. For PM10, the
obtained with the PI-ORS (14) and Flux Tower methods (17) average emission factor determined with RR-ORS and PI-
for these artillery operations and compared in Figure 1. The ORS consistently agreed with each other within an absolute
vertical bars in Figure 1 are the arithmetic means, and the difference of 12%. Statistical hypothesis tests show that there
lines on the bars are standard deviations of the PM emission is no statistical difference for the average emission factors
factors for the artillery back blasts. All three measurement determined with the RR-ORS and PI-ORS methods at the
methods show a similar trend of PM emissions with respect confidence level of 95% (0.12 < p < 0.96). The results obtained
of charge zone (i.e., the larger the charge zone, the more PM with the Flux Tower method are presented in Figure 2. Overall,
is emitted). All three groups of measurements show similar the average PM emissions for all vehicle speeds for the Flux
ratios between the mean emissions of PM10 and PM2.5 with Tower are 100% larger than for the RR-ORS. However, as
mean ( standard deviations for PM2.5/PM10 of 0.34 ( 0.24 indicated before, the Flux Tower results were obtained at the
for charge zone 2 and 0.41 ( 0.13 for charge zone 8S. However, same base but at different times than the ORS measurements.
the PM emission results provided by the ORS methods are Figure 3 describes the dependence of PM2.5 mass emission
larger than for the Flux Tower measurements for six of the factors on vehicle type and speed for the two ORS measure-
eight tests. It is also important to note that the relative ment methods. As with the PM10 emission factors, the PM2.5
standard deviations (standard deviation/mean) for the PM emission factors did not show strong correlation with the
emission factors were larger for the ORS techniques than the vehicle speed. Statistical hypothesis tests show that there is
Flux Tower technique with all relative standard deviations no significant linear dependence of PM emission factor on
> 0.5, possibly due to the uncertainties in wind direction, vehicle speed for all three types of tracked vehicles at the
local turbulence, heterogeneous, and fast-changing profiles confidence level of 95% (0.26 < p < 0.84). The average emission
through the plumes, especially for the upper heights of the factors for each type of vehicle are 2.66 × 103 g PM2.5/km for
plumes. the BFV, 9.32 × 103 g PM2.5/km for the M1A1, and 5.15 × 103
3.2. Fugitive PM Emissions from Movement of Tracked g PM2.5/km for the M113. Statistical hypothesis tests for PM2.5
Vehicles. The tracked vehicles that were tested as part of this emission factors show that there is no statistical difference
field campaign were the M113 tank, Bradley Fighting Vehicle for the average emission factors determined with the RR-
(BFV), and M1A1 tank. Data obtained from measurements ORS and PI-ORS methods at the confidence level of 95%
by the ORS systems and the anemometers were integrated (0.30 < p < 0.82). PM emission results for the Flux Tower
using the method described in ref 13 to calculate the PM method were not included in this comparison because the
emission factors for each vehicle type, vehicle speed, and PM2.5 emission factors were not examined using the Flux
surface type. Tower method (15).
The mass emission factors of PM10 obtained with RR-ORS Large variations were observed in the mass emission
method were compared with those obtained with PI-ORS factors for PM10 and PM2.5 that were obtained with both ORS
method (14) in Figure 2 for all the three vehicles. Fugitive PM methods. For example, the relative standard deviations for
emissions from the same sources were also measured using PM10 and PM2.5 are both 70% for the range-resolved ORS
Flux Tower method but during different days (15) and are method, and 40 and 90% for PM10 and PM2.5, respectively,
also compared to results from the ORS results in Figure 2. for path-integrated ORS method. Factors that could cause
It should be noted that some discrepancies exist between such large fluctuation in PM emission factors include the
the results from ORS method and Flux Tower method. Testing following: (a) variable local winds; (b) inhomogeneous surface
dust emissions at different times is one of the reasons for of the ground so that the vehicle did not travel exactly along
disagreement between the two methods. Other possible the same path during each test; and (c) changing surface

668 9 ENVIRONMENTAL SCIENCE & TECHNOLOGY / VOL. 45, NO. 2, 2011


TABLE 1. Fugitive PM Mass Emission Factors for Artillery Back Blast, Movement of Tracked Vehicles, and an Airborne Helicopter as Determined with the Range-Resolved ORS Method
PM emission factor and standard deviation
PM10 PM2.5
wind speed wind direction operating parameter
(standard deviation) (standard deviation) (charge zone or vehicle/ emission factor standard
PM generator test condition m/sec degree from North helicopter speed) no. of tests unit mean standard deviation mean deviation
projectile model:M107 3.3 (0.5) 303.1 (9.2) charge zone ) 2 2 192.3 64.7 62.4 200.4
artillery back blast g PM/firing
projectile model:M549A1 3.3 (1.2) 278.1 (22.4) charge zone ) 8S 7 301.4 67.3 109.2 154.9
8 km/h 1.4 × 104 1.3 × 104 2.2 × 103 2.0 × 103
24 km/h 1.3 × 104 -a 1.8 × 103 -a
bradley 3.0 (1.2) 256.1 (43.2) 7 g PM/km
32 km/h 1.4 × 104 7.6 × 103 3.0 × 103 1.3 × 101
40 km/h 1.4 × 104 4.3 × 102 3.2 × 103 7.6 × 102
8 km/h 1.7 × 104 1.4 × 104 1.1 × 103 1.3 × 102
16 km/h 5.8 × 104 5.3 × 104 9.1 × 103 1.0 × 104
tracked vehicle M1A1 7.2 (1.2) 291.5 (14.5) 24 km/h 14 g PM/km 7.2 × 104 6.2 × 104 1.7 × 104 1.3 × 104
32 km/h 1.4 × 104 4.3 × 102 3.2 × 103 7.6 × 102
40 km/h 1.1 × 104 -a 2.9 × 103 -a
16 km/h 8.3 × 103 6.3 × 103 2.3 × 103 2.2 × 103
24 km/h 9.5 × 103 -a 2.2 × 103 -a
M113 2.8 (1.2) 228.5 (32.7) 7 g PM/km
32 km/h 1.0 × 104 -a 2.3 × 103 -a
40 km/h 3.7 × 104 3.0 × 104 8.9 × 103 9.0 × 103
15 km/h 6.1 × 104 2.0 × 104 2.1 × 104 7.0 × 102
desert pavement 4.8 (1.4) 163.1 (19.5) 30 km/h 25 g PM/km 4.3 × 104 3.0 × 104 1.5 × 104 1.1 × 103
60 km/h 1.4 × 104 1.5 × 104 5.0 × 103 5.2 × 102
helicopter 15 km/h 1.1 × 105 6.1 × 104 4.0 × 103 2.2 × 103
25-30 km/h 7.8 × 104 7.9 × 104 2.7 × 104 2.7 × 103
disturbed soil 3.7 (1.8) 219.2 (48.1) 42 g PM/km
35 km/h 6.8 × 104 3.5 × 104 2.4 × 104 1.2 × 103
45-60 km/h 2.2 × 104 1.7 × 104 7.6 × 103 5.9 × 102
a
Indicates no data available.

VOL. 45, NO. 2, 2011 / ENVIRONMENTAL SCIENCE & TECHNOLOGY


9 669
FIGURE 1. Comparison of fugitive PM emission factors
determined by range-resolved ORS, path-integrated ORS (14),
and Flux Tower (17) based measurements.

FIGURE 4. Comparison of PM10 emission factors that were


determined with range-resolved ORS, path-integrated ORS (14),
and Flux Tower (16) methods for an airborne helicopter
traveling over desert pavement and disturbed soil surfaces.

FIGURE 5. Comparison of PM2.5 emission factors that were


determined with range-resolved ORS, path-integrated ORS (14),
FIGURE 2. Comparison of PM10 emission factors that were and Flux Tower (16) based methods for an airborne helicopter
determined with range-resolved ORS, path-integrated ORS (14), traveling over desert pavement and disturbed soil surfaces.
and Flux Tower (15) based methods for three tracked vehicles.
dust generated by the vehicle. Dust materials were incor-
porated into the track as the track pressed down on the surface
and then were lifted into the air when that tracks reached
the rear of the vehicle.
3.3. Fugitive PM Emissions from an Airborne Helicop-
ter. The rotary aircraft tested during this research is a Bell
210 helicopter. PM10 and PM2.5 emissions from the airborne
helicopter were quantified for the two types of surfaces using
the RR-ORS method with a vertically scanning MPL, PI-ORS
method with fixed two-beam OP-FTIR/OP-LT (14), and the
Flux Tower method (16). The emission factors were grouped
based on the helicopter’s speed (Figures 4 and 5) for desert
pavement and disturbed soil surface conditions, respectively.
The vertical lines on the top of vertical bar in Figures 4 and
5 are standard deviations of the emission results for the same
helicopter speed and surface type. Statistical hypothesis tests
show that there is significant linear dependence of PM10 and
PM2.5 emission factors on helicopter speed for both surface
types at the confidence level of 95% (p < 0.05). The correlation
coefficients between the emission factor and helicopter speed
are high with the R2 of 0.995 and 0.992 for desert pavement
and disturbed soil surfaces, respectively. The decreasing
emission factor with increasing helicopter speed is reasonable
FIGURE 3. Comparison of PM2.5 emission factors that were
because (a) a slower helicopter had a longer time period to
determined with range-resolved ORS, and path-integrated ORS
(14) methods for three tracked vehicles. entrain PM from the earth’s surface than for a faster helicopter
for the same horizontal distance traveled; and (b) the surface
condition after each trip of the tracked vehicle. Furthermore, shear stress increased with decreasing helicopter speed (16),
the patterns of the track may also impact on the amount of which resulted in higher PM emissions.

670 9 ENVIRONMENTAL SCIENCE & TECHNOLOGY / VOL. 45, NO. 2, 2011


TABLE 2. Data Regressions for PM Emission Factors (EF, g PM/km) Versus Vehicle/Helicopter Speed (v, km/h) or Momentum (mv,
kg m/s)
range of data used for
dust generator test condition particle diameter range regression R2 regression
PM10 EF ) 13 647v0.0014 0.00
Bradley
PM2.5 EF ) 1329.7v0.2038 0.31
PM10 EF ) 35 484v-0.0433 0.00
M1A1
PM2.5 EF ) 387.04v0.8698 0.25
tracked vehicle 8 < v < 40 km/h
PM10 EF ) 1111.7v0.8596 0.56
M113
PM2.5 EF ) 396.4v0.729 0.41
PM10 EF ) 115.33(mv)0.4177 0.22
all three vehicles combined
PM2.5 EF ) 7.6638(mv)0.5068 0.25
PM10 EF ) -1016.1v + 74 868 0.995
desert pavement
PM2.5 EF ) -351.73v + 25 916 0.995
helicopter 15 < v < 60km/h
PM10 EF ) -2417.6v + 14 9213 0.992
disturbed soil
PM2.5 EF ) -836.86v + 51 651 0.992

PM emission results from the two ORS methods compare and surface types using recently developed RR-ORS and PI-
well with the differences in PM10 emission factors of 14 and ORS methods. In terms of showing plume PM mass distri-
10% for desert pavement and disturbed soil, respectively, for bution profiles, RR-ORS is the preferred method because it
the low helicopter speed (i.e., 15 km/h), when the largest directly detects dust at different locations along the optical
plumes were generated. As the helicopter speed increased, paths, while the PI-ORS detects the total extinction along
the relative difference between the results obtained with the the optical paths and relies on bivariate Gaussian model to
two methods also increased. Statistical hypothesis tests show map the 2-D distribution. The PM-generating mechanisms
that there is no statistically significant difference for the were different for these three military activities, which resulted
average emission factors determined with the RR-ORS and in different plume characteristics and emission factors. Back
PI-ORS methods for desert pavement (p ) 0.11) at the blasts during artillery firing generated PM by transferring
confidence level of 95%. However, there is a statistically the force generated by the detonation of the propellant to
significant difference for disturbed soil (p ) 0.03). The RR- the soil surface. The soil at the gun position was compressed
ORS method yielded larger emission factors than the PI-ORS by the force and then rebounded. PM was injected into the
method for disturbed soil surface. The same statistical air and transported by the wind. Therefore, the amount of
hypothesis tests for PM2.5 emissions indicate no statistically dust emission from a single short-term puff depended on
significant difference for the average emission factors the surface character and the force generated by the back
determined with the RR-ORS and PI-ORS methods for desert blast. Artillery firing plumes typically lasted for 10-30 s, and
pavement (p ) 0.69) at the confidence level of 95%. However, the heights were less than 10 m. The larger amount of energy
there is statistically significant difference for disturbed soil exerted onto the ground caused a larger amount of PM to
(p ) 0.014). Higher emission factors were determined with be entrained into the air. (i.e., charge zone of 8S versus charge
the RR-ORS method than the PI-ORS method for disturbed zone of 2).
soil surface. Nevertheless, all three methods showed the same Mobile tracked vehicles and airborne helicopters con-
trend of decreasing PM emission factors with increasing tinuously generated PM plumes when traveling and conse-
helicopter speed. Figures 4 and 5 also demonstrate that quently produced long-lasting and larger-sized plumes
disturbed soil is a larger PM source than desert pavement. comparing to those generated by short-term “puff” artillery
The disturbed soil surface has PM emission factors 50-88% back blasts. The plumes generated by moving tracked vehicles
larger than desert pavement surface for PM10 and PM2.5 at and airborne helicopters lasted for 100-200 s or even longer
each helicopter speed category. Data regressions for PM10 for these field campaigns, and the plumes reached up to
and PM2.5 emission factors for tracked vehicles and airborne 50 m above the ground. Tracked vehicles emitted PM by
helicopters are described in Table 2. entraining the soil that was attached to the links of the tracks
An exponential model was used for data regression for when they reached the rear of the vehicle. The amount of
tracked vehicles, while a linear model was used for the PM emitted per unit distance the vehicle traveled depended
helicopter in Table 2. This is because the dust emission more on the type of tracked vehicle and type of soil surface
mechanism is more complicated for tracked vehicles than than the speed of the vehicle.
for the helicopters. The exponential model provided higher
However, the airborne helicopter did not physically
R2 values than the linear model for tracked vehicle results.
contact the surface of the soil like the tracked vehicles. The
In addition, AP-42 also uses empirical expressions for
helicopter generated dust emissions by blowing the topsoil
emission factors for vehicles traveling on unpaved roads with
through its rotary wings (16). Therefore, the emission rates
an exponential format for vehicle speed. Therefore, an
depended on the surface properties of the soil and the
exponential model was used for data regression for tracked
duration of the event. The duration of the event was linearly
vehicles. However, helicopters ave different dust-generating
correlated to the inverse of the helicopter speed. Field results
mechanism from tracked vehicles. The increased PM emis-
show good correlation (R2 > 0.99) between the emission factor
sion factors at lower helicopter speeds result from the longer
and the helicopter speed for each surface type.
duration of exposure of the dust to the downward wind from
the rotor blades. The duration is linearly proportional to the
speed of the helicopter. Therefore, a linear model should be Acknowledgments
used for the helicopter, which is confirmed by the high R2 The authors thank the supporting staff from Yuma Proving
values of the regression. Ground and Yakima Training Center for coordinating the field
campaigns, and the following agencies that provided funds/
4. Discussion support for this research: Strategic Environmental Research
Fugitive PM emission factors from three types of military and Development Program (Project SI-1400); Fujian Science
activities were determined for typical operating conditions and Technology Commission (No. 2010Y0056), Xiamen Dis-

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