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Synthesis of 119 Superheavy Elements Using Ca-And Ti-Induced Reactions
Synthesis of 119 Superheavy Elements Using Ca-And Ti-Induced Reactions
Synthesis of 292−303 119 superheavy elements using Ca- and Ti-induced reactions
The synthesis of superheavy element Z = 119 in the fusion evaporation reactions 42,44,46,48 Ca + 252−255 Es and
46−50
Ti + 246−249 Bk in the 3n-, 4n-, and 5n-channels leading to 294−303 119 and 292−299 119, respectively, is evaluated.
It is observed that the 3n-channel (952.173 fb) cross section is larger for the reaction 48 Ca + 252 Es → 300 119; the
4n- (155.026 fb) and 5n- (23.11 fb) channel cross sections are larger for 48 Ca + 254 Es → 302 119. For the reaction
50
Ti + 249 Bk → 299 119, the experimental upper limit of the cross section was about 50 fb, which is very close to
our calculated value (40.86 fb for the 4n-channel). Also, the isotopic dependence of both projectile and target
for the production cross section is discussed. These studies will be useful for the experimentalists to produce
isotopes of element Z = 119.
DOI: 10.1103/PhysRevC.96.034610
with ξ = z/b, where the width (diffuseness) of nuclear surface where E ∗ is the excitation energy of the compound nucleus, EB∗
b ≈ 1 fm and Ci is the Susmann central radii, denotes the excitation energy of the compound nucleus when
b2 the center-of-mass beam energy is equal to the Coulomb and
Ci = Ri − . (7) proximity barriers, is an adjustable parameter ( = 4 MeV),
Ri2
and xeff is the effective fissility defined as
For Ri , we use the semiempirical formula in terms of mass
number Ai as
(Z 2 /A)
−1/3 xeff = [1 − α + αf (K)], (14)
Ri = 1.28Ai
1/3
− 0.76 + 0.8Ai . (8) (Z 2 /A)crit
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SYNTHESIS OF 292−303 119 SUPERHEAVY . . . PHYSICAL REVIEW C 96, 034610 (2017)
with (Z 2 /A)crit , f (K), and K is given by barrier height Bf can be determined as the sum of the liquid
2 drop (LD) fission barrier and shell correction terms,
(N − Z)
(Z 2 /A)crit = 50.883 1 − 1.7826 , (15) Bf (E ∗ ) = BfLD + S exp(−E ∗ /ED ), (21)
A
4 where ED is the shell damping energy given by
f (K) = , (16)
K2 + K + 1
K
+ 1
K2 ED = 5.48A1/3 /(1 + 1.3A−1/3 ) MeV. (22)
K = (A1 /A2 ) 1/3
, (17)
The liquid drop fission barrier is very low or equal to zero for
where Z, N, and A represent the atomic number, the neutron heavy elements with Z > 109 [52,53]. So the fission barrier in
number, and the mass number, respectively. A1 and A2 are the heaviest nuclei is defined mainly by shell corrections, and
the mass numbers of the projectile and the target, respectively. its value depends on the excitation energy. The shell correction
xthr , c are adjustable parameters, and α = 1/3. For the best S is taken from Ref. [54].
fit for the cold fusion reaction, the values of c and xeff are
136.5 and 0.79, respectively. For the hot fusion reaction, the III. RESULTS AND DISCUSSION
best fits for xeff 0.8 are c = 104 and xthr = 0.69; whereas
for xeff 0.8, the values are c = 82 and xthr = 0.69. These With the methodology described previously, we have
constants are suggested by Loveland [46]. evaluated the production cross section of SHE Z = 119 in
the fusion reactions 42,44,46,48 Ca + 252−255 Es and 46−50 Ti +
246−249
3. Evaporation residue cross section Bk leading to 294−303 119 and 292−299 119, respectively.
The Coulomb barrier and barrier position are calculated taking
The cross section of SHE production in a heavy-ion fusion the Coulomb and proximity potentials as the interacting
reaction with the subsequent emission of x neutrons is the potential. The capture cross section is calculated using the
product of the capture cross section, the fusion probability, well-known formula of Wong [42]. The probability of CN
and the survival probability [47–49], formation PCN and fission barrier Bf are calculated using
∞
xn π xn
the energy-dependant formulas. Fusion and ER cross sections
σER = (2 + 1)T (E,)PCN (E,)Wsur (E ∗ ,), (18) for the synthesis of isotopes of Z = 119 are evaluated
k 2 =0
systematically.
The survival probability Wsur is the probability for the The calculated maximum value of the evaporation residue
compound nucleus to decay to the ground state of the final cross section (in the 3n-, 4n-, and 5n-channels) and the
residual nucleus via the evaporation of light particles and a γ corresponding excitation energy for these reactions are listed in
ray for avoiding the fission process. Table I. It is found that, among the reactions 42 Ca + 252−255 Es
Survival probability. The survival probability under the leading to 294−297 119 the highest cross section is obtained
evaporation of x neutrons is for the reaction 42 Ca + 253 Es → 295 119 in the 4n-channel
(4.766 fb at 47 MeV). Also among these, the 3n-channel
imax
=x
∗ n cross section (1.226 fb at 44.48 MeV) is larger for the
Wsur = Pxn (ECN ) , (19) reaction 42 Ca + 252 Es → 294 119, and the 5n-channel cross
i=1
n + f i,E ∗
section (2.167 fb at 52.89 MeV) is larger for the reaction
where the index “i” is equal to the number of emitted neutrons,
42
Ca + 254 Es → 296 119.
Pxn is the probability of emitting exactly xn neutrons [50], E ∗ The ER cross section of 44 Ca + 252−255 Es leading to
296−299
is the excitation energy of the compound nucleus, n and f 119 in the 3n-, 4n-, and 5n-channels is evaluated.
represent the decay width of neutron evaporation and fission, Among these, the maximum cross section obtained is for
respectively. To calculate n /f , Vandenbosch and Huizenga the 4n-channel (39.213 fb at 43.3 MeV) for the reaction
[51] have suggested a classical formalism,
44
Ca + 255 Es → 299 119. The 3n-channel cross section is larger
(25.038 fb at 38.77 MeV) for 44 Ca + 252 Es → 296 119, and the
n 4A2/3 af (E ∗ − Bn ) 5n-channel cross section (7.627 fb at 49.68 MeV) is larger
= 1/2
f K0 an 2af (E ∗ − Bf )1/2 − 1 for 44 Ca + 254 Es → 298 119. Among 46 Ca + 252−255 Es leading
to 298−301 119, the largest cross section obtained is 476.381 fb
× exp 2an1/2 (E ∗ − Bn )1/2 − 2af (E ∗ − Bf )1/2 ,
1/2
at 33.82 MeV for the reaction 46 Ca + 252 Es → 298 119 in the
(20) 3n-channel, and the next highest cross section for the same
channel obtained is 321.161 fb for 46 Ca + 254 Es → 300 119.
where A is the mass number of the nucleus considered, E ∗ The 4n-channel cross section is larger (137.672 fb) for the
is the excitation energy, and Bn is the neutron separation reaction 46 Ca + 255 Es → 301 119.
energy. The constant K0 is taken as 10 MeV. an = A/10 and The ER cross section using the 48 Ca-induced reaction
af = 1.1an are the level-density parameters of the daughter on 252−255 Es targets is presented in Fig. 1. For the reaction
nucleus and the fissioning nucleus at the ground state and 48
Ca + 254 Es → 302 119, the obtained maximum values of the
saddle configurations, respectively. Bf is the fission barrier, ER cross section in the 3n-, 4n-, and 5n-channel cross sections
and this height is a decisive quantity in the competition are 722.331, 155.026, and 23.108 fb, respectively. The 3n-
between processes of neutron evaporation and fission. Fission and 4n-channel cross sections for 48 Ca + 253 Es → 301 119 are
034610-3
K. P. SANTHOSH AND V. SAFOORA PHYSICAL REVIEW C 96, 034610 (2017)
TABLE I. Predicted maximum value of the ER cross section obtained for the synthesis of SH element Z = 119 using Ca- and Ti-induced
reactions.
601.494 and 140.425 fb, respectively, and for 48 Ca + 255 Es → projectile for SH element synthesis, which is heavier than a Ca
303 projectile.
119 are 215.442 and 145.943 fb, respectively. It is found
that, among all the Ca-induced reactions on 252−255 Es, the re- So for the synthesis of SHE Z = 119, we also have
action 48 Ca + 252 Es → 300 119 has the largest ER cross-section calculated an ER cross section using Ti-induced reactions
value obtained in the 3n-channel (952.173 fb at 30.17 MeV). on Bk targets. For computing an ER cross section, isotopes
46−50
The 4n- and 5n-channel cross sections for the same reaction Ti are used as projectiles and 246−249 Bk are used as
is 61.595 and 9.437 fb, respectively. The half-lives of the targets. Among the reactions 46 Ti + 246−249 Bk leading to
292−295
einsteinium isotopes 252−255 Es are 471, 20, 275, and 40 119, the highest ER cross section obtained is 1.994 fb
days, respectively, sufficient to be used as target material. for the reaction 46 Ti + 249 Bk → 295 119 in the 4n-channel.
However, for the moment, it is impossible to accumulate Among the reactions 47 Ti + 246−249 Bk leading to 293−296 119,
and prepare the required amount of the target material. The the highest cross section of 3.772 fb is obtained for the reaction
isotopes of Es are extremely difficult to produce, however,
47
Ti + 248 Bk → 295 119 for the 4n-channel.
these targets could be made available in the near future. Thus The reaction for which the highest cross section obtained
to synthesize elements with Z > 118, Ti is the most promising among the reactions 48 Ti + 246−249 Bk leading to 294−297 119
034610-4
SYNTHESIS OF 292−303 119 SUPERHEAVY . . . PHYSICAL REVIEW C 96, 034610 (2017)
034610-5
K. P. SANTHOSH AND V. SAFOORA PHYSICAL REVIEW C 96, 034610 (2017)
TABLE II. Comparison of predicted maximum values of the evaporation residue cross sections σER (3n) and σER (4n) for 50 Ti + 249 Bk →
299
119, 48 Ca + 252 Es → 300 119, and 48 Ca + 254 Es → 302 119 with other theoretical predictions.
50
Ti + 249 Bk → 299 119 48
Ca + 252 Es → 300 119 48
Ca + 254 Es → 302 119 Reference
E∗ σER E∗ σER E∗ σER E∗ σER E∗ σER E∗ σER
(MeV) 3n (fb) (MeV) 4n (fb) (MeV) 3n (fb) (MeV) 4n (fb) (MeV) 3n (fb) (MeV) 4n (fb)
27.5 640 35.0 350 [24]
36 210 42 3160 36 80 42 1700 [25]
35 260 40 160 33 410 37 1300 [26]
41 40 43.5 55 [27]
35 170 41 570 [28]
33 35 43 35 [29]
36 60 46 110 [30]
36.5 480 43.5 310 [31]
37 33 46 15 [32]
34.5 12 46.5 64 34 590 44 960 [33]
38 40 50 150 37 45 47 180 [34]
30 340 40 160 30 2750 38 160 27 4040 35 1230 [35]
35.5 30 47.5 36 33 80 43 220 32 4 41 16 [36]
32.6 105.1 40.1 40.9 30.2 952.2 38.7 61.6 29.6 722.3 38.1 155.0 This paper
maximum values of the ER cross section obtained are 601.494 sections. From the isotopic trend in the Ti-induced reactions on
and 140.425 fb in the 3n- and 4n-channels, respectively. For the Bk targets, with the increase in neutron number of the projectile
synthesis of 302 119 and 303 119, the studied combinations are and target, the production cross section is found to be increas-
48
Ca + 254 Es and 48 Ca + 255 Es, respectively. The maximum ing. In this case, the reactions 50 Ti + 249 Bk in the 4n-channel
value of the ER cross section obtained in the 3n- and and 50 Ti + 248,246 Bk in the 3n-channel gave the maximum
4n-channels for 48 Ca + 254 Es are 722.331 and 155.026 fb, production cross sections for the synthesis of Z = 119.
respectively, and for 48 Ca + 255 Es are 215.442 and 145.943 fb, Among all the reactions mentioned, the 3n-channel cross
respectively. section is larger for 48 Ca + 252 Es → 300 119; the 4n- and 5n-
In Table II, we compared our results with other theoretical channel cross sections are larger for 48 Ca + 254 Es → 302 119.
studies for the reactions 50 Ti + 249 Bk, 48 Ca + 252 Es, and Thus we have predicted the production cross section for the
48
Ca + 254 Es, and in most of the cases our values agree synthesis of isotopes of element Z = 119 and the favorable
with other theoretical predictions. The difference observed in projectile-target pair using Ca- and Ti-induced reactions. We
various theoretical predictions is due to the different methods would like to mention that, in the present paper, we have
used for calculating the probability of CN formation and predicted the production cross section for the synthesis of iso-
survival probability. Also the use of different mass tables topes 292−299 119 using the reactions 42,44,46,48 Ca + 252−255 Es
in different theoretical approaches gives different values and 46−50 Ti + 246−249 Bk, whereas the other theoretical studies
of binding energy, and the corresponding changes will be are based on the 48 Ca- and 50 Ti-induced reactions only. We
reflected in the calculations. Theoretically many studies have hope our studies will be a guide for future experiments to
been performed using the reaction 50 Ti + 249 Bk than the synthesize the SH element Z = 119, which is not synthesized
other two reactions (48 Ca + 252 Es and 48 Ca + 254 Es), and an so far.
experimental attempt also is performed using the 50 Ti + 249 Bk In order to check the reliability of the present calculations,
reaction. By analyzing our results and other theoretical studies we have calculated the fusion excitation functions for the re-
(Table II), it is found that the highest cross section obtained is actions leading to superheavy elements Z = 114 to Z = 118,
for the 48 Ca-induced reaction and hence it is the best reaction which have already been measured in the experiments. The
to synthesize SHE Z = 119. So, we look forward to new predicted ER cross sections and the corresponding excitation
experimental investigations using the 48 Ca + 252,254 Es reaction energies are compared with the experimental values and are
as it is found to be the most feasible combination. shown in Table III. Our predictions of the ER cross sections
While analyzing Table I, it also is found that, with the agree with the experimental values. For these calculations on
increase in neutron number of target 252−255 Es (for a particular Z = 114−118, we have used the same model with the same set
Ca projectile on odd-A and even-A targets), the production of parameters which are described in Sec. II. We would like to
cross section is found to be decreasing for the 3n-channel and mention that, for the SHEs Z = 117 [45] and Z = 120 [44],
increasing for the 4n-channel. With the increase in neutron we already have performed the calculations using the same
number of the projectile as 42,44,46,48 Ca, the production cross model with the same set of parameters. We were successful
section is found to be increasing. The result shows that the in reproducing the experimentally measured cross sections for
targets 252 Es in the 3n-channel, 254 Es in the 4n-channel, and the SHEs Z = 114−118 which clearly shows the validity of
the projectile 48 Ca in both channels have the largest cross our calculations and hence we are confident in predicting the
034610-6
SYNTHESIS OF 292−303 119 SUPERHEAVY . . . PHYSICAL REVIEW C 96, 034610 (2017)
TABLE III. Comparison of the calculated evaporation residue cross section and the corresponding excitation energy with that of experiments
for the SHEs with Z = 114−118.
fusion excitation functions for the synthesis of SHEs, which the 3n-channel. For the reaction 50 Ti + 249 Bk, our calculated
are not synthesized so far. maximum value (40.86 fb) for the 4n-channel is very close to
the predicted experimental upper limit of the cross-sectional
IV. CONCLUSION value (50 fb). The isotopic dependence of the projectile and
target for the production cross section leading to the CN
We have evaluated the ER cross section in the 3n-, 4n-, Z = 119 also are studied, and these studies will be helpful
and 5n-channels of the fusion reaction 42,44,46,48 Ca + 252−255 Es for experimentalists to conduct experiments with optimum
and 46−50 Ti + 246−249 Bk leading to the CN 292−303 119. Our energy.
result shows that 48 Ca + 252 Es → 300 119 and 48 Ca + 254 Es →
302
119 in the 3n-channel and the 4n-channel, respectively,
ACKNOWLEDGMENT
should be the favorable projectile-target pair for the syn-
thesis of Z = 119. Among the 46−50 Ti-induced reactions on One of the authors (V.S.) would like to thank the University
246−249
Bk targets, the promising projectile-target pairs for Grants Commission (UGC), Government of India, for financial
which the maximum production cross section obtained is support in the form of a Moulana Azad National Fellowship
for 50 Ti + 249 Bk in the 4n-channel and 50 Ti + 248,246 Bk in (MANF).
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