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Art 13
Art 13
Review
a r t i c l e i n f o a b s t r a c t
Article history: The flux assisted GTAW or A-TIG process developed at the Paton Welding Institute in 1960. Despite
Received 5 January 2016 capable of offering a penetration up to 5–6 mm in a single pass weld, it could not find enough space in
Received in revised form 4 March 2016 industrial applications, primarily due to few inherent unfavorable features: (a) two-step nature of the
Accepted 21 March 2016
process, (b) poor weld-bead and (c) poor electrode life. High penetration capability of A-TIG process has
fascinated researchers and renewed the research interest in last one decade. In the present work, attempts
Keywords:
have been made to analyze and review the literature published with respect to (a) advancement of various
A-TIG
hypotheses to explain the reasons for high penetration achieved using A-TIG, (b) effect of input process
Flux
Weld bead geometry
parameters related to GTAW and A-TIG, (c) effect of chemical composition and various alloying elements
Review paper in steel on penetration achieved by A-TIG, (d) feasibility studies of A-TIG on ferrous and non-ferrous
metals and (e) technological problems associated with A-TIG. In light of the above, the present review
will help in (a) highlighting the future scope of research in A-TIG to enhance its industrial application
and (b) to develop systematic understanding of various technological factors determining the capability
of this process.
© 2016 The Society of Manufacturing Engineers. Published by Elsevier Ltd. All rights reserved.
Contents
1. Introduction . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 212
2. Mechanism of A-TIG . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 212
2.1. Reversal of the Marangoni convection . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 213
2.2. Arc constriction . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 214
3. Methods opted for flux deposition . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 215
4. Factors affecting the A-TIG performance . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 215
4.1. Forces acting in A-TIG welding . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 215
4.2. Welding related process parameters . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 216
4.2.1. Welding current . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 216
4.2.2. Welding speed . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 216
4.2.3. Arc length . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 216
4.2.4. Electrode geometry . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 218
4.2.5. Shielding gas composition . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 219
4.3. Properties of the metal to be welded . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 220
4.3.1. Thickness of the plate . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 220
4.3.2. Composition of metal . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 221
4.4. Flux . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 223
5. Recent development in TIG process to enhance the depth of penetration . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 224
6. Conclusions . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 225
References . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 226
http://dx.doi.org/10.1016/j.jmapro.2016.03.012
1526-6125/© 2016 The Society of Manufacturing Engineers. Published by Elsevier Ltd. All rights reserved.
212 R.S. Vidyarthy, D.K. Dwivedi / Journal of Manufacturing Processes 22 (2016) 211–228
that surface tension gradient (d/dT) across the weld pool could
other responsible mechanism for increased depth of penetration. affect the convective flow in the weld pool. The presence of surface
Then after reversal of Marangoni flow come into consideration in A- active elements like sulfur and oxygen in the steel causes the alter-
TIG welding. After a thorough exercise on the probable forces that ations in surface tension () in the weld pool illustrated in Fig. 3.
can affect the penetration, it was concluded that the higher penetra- It reverses the surface tension gradient (d/dT) in the weld pool
tion could be due to changes in fluid flow direction [11–14,25,92]. which makes the surface tension higher at the center of weld pool
Thereafter, reversal of Marangoni convection and arc constriction that decreases gradually towards outer section [25].
evolved as the most accepted phenomena for higher penetration Roper et al. [95] correlated the effect of a small amount of sur-
depth during flux assisted TIG welding. face active elements on the surface properties of the weld pool with
interfacial energy. Heiple et al. [96] studied the effect of the surface
2.1. Reversal of the Marangoni convection active elements with the fluid flow motion in the weld pool. And
developed a theory that the direction and the magnitude of thermo
Marangoni convection, also known as surface-tension driven capillary forces decide the fluid flow direction in the weld pool
convection or thermo capillary convection, can have a dramatic consequently affect the depth of penetration. The thermo-capillary
effect on the penetration depth of the weld. This phenomenon was forces can be controlled by the concentration of the surface active
first proposed by James Thomson in 1855 [93]. The phenomenon elements such as sulfur and oxygen in the metal. It was observed
got its name on the name of Carlo Marangoni who further investi- that as the concentration of the surface active elements exceed a
gated it in 1865 [7]. According to this theory, the direction of fluid particular amount (about 50 ppm), the temperature coefficient of
flow depends on the surface tension gradient in the fluid. Fluids surface tension (d/dT) changes from negative to positive value.
flow from low surface tension region towards the high surface ten- Since the flow of fluid in weld pool occurs from lower surface ten-
sion region. The strength of thermo-capillary flow is determined sion () region to higher surface tension () region, triggers the
by the Marangoni number (Ma), which is non-dimensional and circulation flow in the molten weld pool as shown in Fig. 4. In case
expressed by Eq. (1) where dT/dx is the temperature gradient, is of pure metals, including steels and other iron alloys, with low sul-
the viscosity, a is the thermal diffusivity and L is the characteristics fur and oxygen contents the surface tension decreases with increase
length [25]. in temperature that is a negative surface tension gradient (d/dT).
It promotes the molten metal surface flow in a radially outward
d dT L2
Ma = (1) direction which in turn makes the weld bead shallow and wider as
dT dx a
shown in Fig. 4A.
The effect of Marangoni forces was first proposed in welding to Keene et al. [97] studied the relation between surface tension
understand the problems encountered in the case of “cast to cast” and molten metal flow direction in weld pool and indicated that
variations or variable penetration. The problem “variation in pene- all systems exhibit a maximum positive surface tension gradi-
tration” observed during autogenous tungsten inert gas welding of ent (d/dT) at some temperature. Further increase of temperature
stainless and ferritic steel was first identified in 1960. This problem results gradual decrease in the surface tension, combination of
was severe in case of robotic welding due to requirement of higher these produces a complex flow similar to that shown in Fig. 5. Simi-
weld penetration and repetitive work. It was reported that welds on lar type of study done by other researchers, and reported increased
some batches of steel exhibit lower penetration than normal while penetration depth using A-TIG, the same was attributed to reversal
other batches exhibit higher, despite all batches were meeting the of Marangoni convection in the weld pool [6,30,35].
material specification requirements [25]. The above discussion suggests that the trace presence of the
A number of attempts had been made to co-relate the “cast to minor alloying elements in the weld pool can reverse the surface
cast” variation and systematic variations in the concentrations of tension gradient in the weld pool; this effect is described by the
specific minor or impurity elements in the metal. It was suggested name of reversal of Marangoni convection in published literature.
that a small amount of impurities or elements in composition of Reversal in Marangoni convection promotes molten metal’s fluid
steel can result in large changes in arc characteristics and the sur- flow from the fusion boundary to the center of the weld pool. A
face properties of the weld pool [14,23,91]. Ishizaki [94] proposed combination of fluid flow from the fusion boundary towards the
214 R.S. Vidyarthy, D.K. Dwivedi / Journal of Manufacturing Processes 22 (2016) 211–228
Fig. 4. Proposed fluid flow on and below the weld pool surface: (A) negative surface tension temperature coefficient; (B) positive surface tension temperature coefficient.
center and the pressure of the arc turn it in the direction of the
arc as shown in Fig. 4B. These forces combine and work together
to increase penetration by transferring heat from top to bottom
effectively. Further, it was observed that this reversal of Marangoni
convection is effective only up to a limit of temperature after which
complex behavior of fluid is expected in the weld pool.
Fig. 6. Schematic illustration of arc constriction.
Fig. 9. Marangoni convection in (a) Conventional TIG and (b) A-TIG welding process.
Fig. 7. Variation in partial pressure of electron gas and negative ions of Halides (1
and 5 with “KCl” flux, 2 with “Ti”, 3 and 4 with “KF” flux). Fig. 10. Direction of (a) Electromagnetic or Lorentz force and (b) Buoyancy force in
molten weld pool.
activated fluxes during welding offers two effects (due to the more
electron affinitive character): other Alcoholic Liquors” [93]. Subsequently Carlo Marangoni did his
doctoral work on this force and explained that ‘fluid always flows
(a) Reduction in number of charged particles in arc. from low surface tension region to high surface tension region’ [82].
(b) Pushing of the arc column radially inward by more electroneg- Due to Marangoni force in weld pool, fluid flow in the centrally out-
ative charged vapor. ward direction and thus transfer a maximum of its heat to the wall
of the weld pool rather than bottom as shown in Fig. 9. This action
Both these factors in turn lead to arc constriction. leads it to the high width and low depth of penetration during TIG
welding [14,23,25,91,93,99–101].
3. Methods opted for flux deposition Electromagnetic or Lorentz force: Electromagnetic force is caused
by the interaction of the induced magnetic field and that of the
The activating fluxes of micro size are mixed with either acetone current passes through a conductor. The welding current induces a
or ethanol to form a paste, which is applied on the surface of the magnetic field around the conductor. Resulting Lorentz force acts
material to be welded. The paste can be applied with a brush or with toward the weld pool center in the direction of current flow shown
an aerosol applicator like a spray shown in Fig. 8(b) [27,92]. Patent in Fig. 10(a).
filed by Matthew et al. [98] used a polymeric binder and suggested Buoyancy force: Buoyancy force is caused by the density differ-
that it can be applied to the weld zone as a hot melt, paint, tape, ence of the molten metal in the weld pool. Molten metal density
adhesive, rod, wire or a stick. decreases with the temperature rise. Due to buoyancy force, the
fluid tends to flow from high density to low density (Fig. 10(b)).
4. Factors affecting the A-TIG performance During A-TIG welding, it always acts toward the surface of the weld
pool. However, buoyancy forces are generally less effective as com-
4.1. Forces acting in A-TIG welding pared to other forces during TIG welding of plate up to a thickness
of 10 mm.
Four types of forces have been so reported to affect the pen- Aerodynamic drag: Aerodynamic drag forces produced by the
etration during A-TIG welding, namely, (a) Marangoni forces; (b) action of the arc plasma flowing over the surface of weld pool which
Electromagnetic or Lorentz forces; (c) Buoyancy forces; and (d) induce an outward flow along the surface of the weld pool shown
Aerodynamic drag forces [23,25,91,93]. in Fig. 11.
Marangoni forces: James Thomson (1855) proposed this force in However, the fluid flow in the weld pool is extremely com-
his article “On certain curious Motions at the Surfaces of Wine and plicated because, Marangoni, electromagnetic, buoyancy and
Fig. 8. Techniques for applying the activating flux in the A-TIG process (a) a brush and (b) a spray.
216 R.S. Vidyarthy, D.K. Dwivedi / Journal of Manufacturing Processes 22 (2016) 211–228
Fig. 12. (a) Surface tension variation with temperature. (b) Weld depth to width ratio of weld as function of welding current for 304 type stainless steel and 304 doped with
sulfur or selenium.
Fig. 13. Variation in weld fusion zone geometry “(a) depth of penetration, (b) weld width” with current, of 304LN austenitic stainless steel welds.
Fig. 14. Effect of weld travel speed on weld geometry with (a) different surface active elements and (b) weld current.
the arc plasma also increases (due to more convection and radi- away from the cathode tip on the arc central axis, the electron
ation) hence the overall efficiency () will decrease. Tanaka et al. temperature was constant value (22,000 K) irrespective of the arc
[40] founded that arc voltage were also increased during TIG weld- length. However, the electron temperature recorded at the anode
ing with increases in arc length shown in Fig. 15. In the same work, spots was decreased with higher arc length. Matsunawa et al. [107]
Tanaka et al. also reported that at a fix position (assumed 1 mm) proposed that out of all these four forces aerodynamic drag forces
218 R.S. Vidyarthy, D.K. Dwivedi / Journal of Manufacturing Processes 22 (2016) 211–228
Fig. 15. (a) Schematic of a self-stabilized arc and its root area with anode and (b) Photographs of TIG Arc at 100 A with different arc length.
Fig. 16. Relation between weld ratio d/w and arc length for (a) 304 type stainless steel and 304 doped with sulfur or selenium [28] and (b) various steel casts; each symbol
represents a different steel.
will play dominating role in case of larger arc length (for exam- 5.5 mm of arc length and a current value of 100 A. And stated
ple 8 mm). Later Okada et al. [104] experimentally established this through his finding (Figs. 17 and 18) that although the heat distribu-
and stated that at higher arc length beneficial effect of sulfur on tion area increased with increase in electron tip angle, but that was
penetration became less effective. The effect of arc length on pene- a slight increment (14%) in the heat distribution area over a wide
tration has been further studied by Burgardt et al. [18] and Ishizaki change of electrode tip angle (30◦ –120◦ ). With this Tsai et al. con-
et al. [103] the results being shown in Fig. 16(a) and (b), respec- cluded that theoretically the electrode tip angle should not affect
tively, which corroborate that the d/w ratio decreased with larger the heat distribution area significantly. However, Tanaka et al. [40]
arc length. examined the axial temperature in the arc plasma, anode spot area
With increase in arc length welding voltage, anode root area and and the heat density on the anode surface variation with the elec-
heat loss from the arc column increases. Increase in welding voltage trode tip angle; and reported that the electron temperature and the
strengthens the heat flux density; however, the increase in anode weld cross sectional area attained a maximum value for electrode
root area weakens it. Initially effect of increase in welding voltage tip angle of 45◦ , but a fall in electron temperature was recorded
dominates over the effect of anode root area and the heat loss from for either increase or decrease in electrode tip angle (30◦ and 60◦ ),
the arc column, but after an optimum arc length further increase while the current density changes were little for all three (30◦ , 45◦
in arc length shows that the combine effect of anode root area and and 60◦ ) electrode tip angles taken.
the heat loss from arc column dominate over the welding voltage.
Fig. 17. Electron temperature and the cross sectional area with the electrode tip angle.
Fig. 19. Current density obtained with conical tipped and frustum shaped elec-
trodes.
Fig. 18. Heat and the mass distribution with the electrode tip angle.
depends on the arc length. However, the arc pressure was found
maximum at 45◦ in almost all case.
nium doped). Burgardt et al. reported that the D/W ratio of the pure
AISI 304 without doping reduced with higher percentage of helium, the pure argon and reported that, at the same parameters; depth of
whereas the D/W ratio of the doped AISI 304 (with sulfur and sele- penetration and weld area for both cases (conventional as well as
nium) stainless steels increased with increased helium as shown activating GTAW process) increased with the addition of hydrogen
in Fig. 22. Huang [2,3] added the hydrogen as well as nitrogen in as well as nitrogen shown in Figs. 23 and 24.
220 R.S. Vidyarthy, D.K. Dwivedi / Journal of Manufacturing Processes 22 (2016) 211–228
Fig. 21. Wb/Wf as function of arc voltage obtained with various shielding gases for Inconel 800.
Fig. 22. Weld ratio d/w as function of helium content of torch gas for 304 type
stainless steel and 304 doped with 76 ppm Sulfur or 47 ppm Selenium.
Fig. 23. Effect of nitrogen addition on the penetration and cross-sectional area of
weld.
The results obtained in the former cases are consistent with the 4.3. Properties of the metal to be welded
proposal that the enhanced heat input caused increased tempera-
ture gradients and thermo-capillary flows [M(+) and M(−)], which 4.3.1. Thickness of the plate
resulted in further divergence of the d/w ratios for high and low It has been seen that the thickness of the plates to be welded also
sulfur steels. affect the depth and width of the weld. Pollard [19] investigated the
Fig. 24. Penetration and weld area vs hydrogen content in argon shielding gas.
R.S. Vidyarthy, D.K. Dwivedi / Journal of Manufacturing Processes 22 (2016) 211–228 221
Fig. 28. Effect of sulfur content on aspect ratio of weld pool d/w for 304 and 316
type stainless steels.
Fig. 30. Effect of SO2 concentration in shield gas on aspect ratio of weld pool d/w
for 21Cr–6Ni–9Mn stainless steel.
Fig. 31. Effect of various dopant concentrations on aspect ratio of weld pool d/w for
Fig. 29. Effect of oxygen concentrations in shield gas on aspect ratio of weld pool 21Cr–6Ni–9Mn stainless steel.
d/w for 21Cr–6Ni–9Mn stainless steel.
Fig. 32. Variation of aspect ratio of weld pool d/w with aluminum content in
21Cr–6Ni–9Mn stainless steel.
Fig. 34. Variation of aspect ratio of weld pool d/w with oxygen content in shield gas
for low and high S samples of Inconel IN 718.
et al. [42] and also with other gases by different researchers Fig. 39. Double electrode TIG welding torch.
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