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Economic Potential of Leachate Evaporation by Using Landfill Gas A Systemdynamics Approach
Economic Potential of Leachate Evaporation by Using Landfill Gas A Systemdynamics Approach
A R T I C L E I N F O A B S T R A C T
Keywords: A system dynamics (SD) approach that models the economic potential of a regional incineration plant by using
System dynamics landfill gas to evaporate waste leachate is proposed in this study. A case study is provided to demonstrate
Incineration plant application of the proposed approach, which takes an incineration plant and an adjacent sanitary landfill located
Leachate evaporation at Chengdu City, China into account. Two scenarios are divided by different ratios of leachate evaporation and
Landfill gas
landfill gas utilization to examine the economic revenues obtained by the incineration plant. The optimal
scenario with the best economic performance is identified to incorporate into future waste management practice.
The limitations of this approach are discussed, laying a foundation for further work.
1. Introduction than 0.3, the biological treatment is ineffective due to the high
concentrations of biorefractory contaminants, fulvic acids, ammonium
With population growth, municipal waste disposal has become a nitrogen etc (Hermosilla et al., 2009; Kalčíková et al., 2014). For the
primary issue during urbanization (Pires et al., 2011; Marshall and physic-chemical approaches, such as flotation, coagulation-floccula-
Farahbakhsh, 2013). Despite great efforts have been made in waste tion, adsorption, stripping etc., it is usually considered as pre-treat-
reduction by reuse or recycle, a large number of municipal waste is ments or post-treatments, in light of leachate stabilization through
disposed in landfill sites, maintaining a comparatively high proportion, aging of the landfill site (Zhu and Liu, 2008; Torres-Socías et al., 2015).
around 60% (Mian et al., 2016). Thermal treatments, e.g. evaporation, distillation, vitrification etc., are
Leachate is generated during biochemical process of waste disposal, used to separate humic suspensions from leachate, concentrate leachate
including suspended solids, dissolved components from degradation of into a small volume at or close to crystallization point, thus to reduce its
the waste by various micro-organisms (Renou et al., 2008; Mohan and contained toxicity and non-biodegradability (Yue et al., 2007; Schiopu
Gandhimathi, 2009; Puig et al., 2011). Because of its complex and and Gavrilescu, 2010). Although the thermal treatments are challenged
harmful compounds, waste leachate may pose a substantial risk to by volatile organic compounds (VOCs), ammonia condensate with
publics (Zhao et al., 2012; Toufexi et al., 2013). Thus, leachate exhaust vapor, high inorganic salt concretion etc., it is still suitable to
treatment is considered as one of the most difficult issues in waste- treat various categories of waste leachate, especially in advantage of
water treatment, which has aroused greater attentions in waste disposal reducing volume of the leachate, and saving total cost (Atabarut and
(Demirabas, 2011). Generally, there are a number of approaches Ekinci, 2006; Schiopu and Gavrilescu, 2010; Zhao et al., 2012).
regarding its treatment, including biological, physic-chemical treat- As energy supply plays a critical role in the thermal treatment of
ment, thermal treatment etc (Zou et al., 2014). waste leachate, using landfill gas (LFG) as an alternative energy source
Biological treatment is deemed as the conventional treatment for has been proposed by a number of researchers (Themelis and Ulloa,
leachate, which aims to degrade organic compounds by using micro- 2007; Hao et al., 2008; Dudek et al., 2010; Johari et al., 2012). LFG,
organisms to carbon dioxide under aerobic conditions, and to biogas mainly constituted by methane and carbon dioxide, if not recovered,
under anaerobic conditions (Ahmed and Lan, 2012). However, the has a global warming potential on climate change (Tan et al., 2014; Liu
biological process is easily inhibited by toxic pollutants within the et al., 2017). On the contrary, LFG is also deemed as a renewable
leachate (Gotvajn et al., 2011; Torres-Socías et al., 2015). In the case of energy source, which has been given greater attentions to its develop-
older leachate, with lower COD, TOC and BOD5, and a BOD5/COD less ment of recovery and utilization, e.g., extraction for power generation
⁎
Corresponding author.
E-mail address: ruizhaoswjtu@gmail.com (R. Zhao).
http://dx.doi.org/10.1016/j.resconrec.2017.04.010
Received 8 December 2016; Received in revised form 19 April 2017; Accepted 20 April 2017
0921-3449/ © 2017 Elsevier B.V. All rights reserved.
R. Zhao et al. Resources, Conservation & Recycling 124 (2017) 74–84
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R. Zhao et al. Resources, Conservation & Recycling 124 (2017) 74–84
Fig. 1. Causal loop diagram of the combined system for leachate evaporation.
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R. Zhao et al. Resources, Conservation & Recycling 124 (2017) 74–84
Table 1
Key variables in the stock-flow diagram.
operation, indicated as two stocks. The investigated landfill is in charge d time for duration of waste life, years;
of recovering the LFG in-site, which is exported to the incineration D (t ) annual landfill gas production rate, m3/y t;
plant through pipeline transport. The incineration plant purchases the F the landfill gas production rate of landfill, m3/a;
LFG to substitute coal as the alternative combustion promoter, and
evaporates the waste leachate. The SD model further hypothesizes that Ti the stock of waste in the ith layer, tonne
the purified LFG is provided by the landfill continuously, as well as The sub-system of incineration plant operation mainly focuses on its
there is no significantly technical challenges on the leachate evapora- associated economic revenue. The major income are sourced from the
tion. Once the landfill is in the stage of closure, the integrated operation power generation, municipal waste incineration, cost saving of combus-
is expected to come to an end, and the incineration plant returns to use tion promoter and government subsidy, whilst the main expenditures
coal as the major combustion improver. are the cost of waste incineration, leachate treatment, LFG purchase,
The sub-system of the LFG generation is based upon the Marticorena annual maintenance and construction investment of pipelines transpor-
Dynamics Model, which is a first-order dynamic equation, and has been tation.
widely applied to prediction of LFG production (Bilgili et al., 2009; The power generation by incineration is mainly determined by the
Bicheldey and Latushkina, 2010). The model is given as follows calorific value of waste (Lombardi et al., 2015; Wang et al., 2016a). LFG
(Marticorena et al., 1993): may increase the waste calorific, but the leachate sprayed to the
incinerator may give rise to the decrease of calorific value. Thus, the
⎛ t⎞ purchased LFG α is ensured to a keep a high waste calorific value. With
MP = MP0·exp ⎜ − ⎟
⎝ d⎠ (1) regard to the leachate evaporation β, it should be set within an
appropriate range. Otherwise, excessive leachate may result in reduc-
dMP MP0 ⎛ t⎞ tion of calorific value and production of toxic pollutants.
D(t) = − = ·exp ⎜ − ⎟
dt d ⎝ d⎠ (2)
3. Data collection and quantification
t t ⎡ MP ⎛ t − i ⎞⎤
F= ∑ Ti ·D (t − i ) = ∑ Ti ⎢ 0 ·exp ⎜− ⎟⎥ A municipal solid waste (MSW) incineration plant and a solid waste
i i
⎣ d ⎝ d ⎠⎦ (3)
sanitary landfill located in Chengdu, China are taken as the case study
where: to obtain the data for the proposed SD model. The sanitary landfill is
MP Landfill gas produced by municipal waste (MSW) degradation, about 6 kilometers apart from the incineration plant, and their
m3/tonne; geographic locations are shown in Fig. 3. The designed treatment
MP0 Landfill gas produced from fresh waste, m3/tonne; capacity of the incineration plant is 1200 t per day. There are about
t time, years; 300m3 of fresh leachate produced per day due to waste degradation.
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R. Zhao et al. Resources, Conservation & Recycling 124 (2017) 74–84
Table 2
Input data related to the key variables.
MP0 MP0 of landfill is 85 m3/t, in which the average ratio of the dry organic matter is about 30% in terms of 85 m3/tonne
municipal waste (Wang et al., 2001)
d The duration of landfill waste d is assigned as 4 years in terms of its stabilization, which is derived by analogy 4 years
to Wang et al. (2001).
Ti By field investigation 1.02 million tonne/y
Cost of conventional leachate treatment By field investigation 60 Yuan/tonne
Purchasing price of purified LFG As there is no precise price of the purified LFG, it is thus converted by the industrial price of natural gas, set its 3.00 Yuan/m3
benchmark as 3.14 Yuan/m3 (Wang and Lin, 2014). The conversion is depended upon the equivalent calorific
value of purified LFG in contrast to the natural gas, in which the former is about 22,360 kJ/m3, whilst the latter
is 37,260 KJ/m3.
Waste incinerated annually The annual waste disposal by incineration is measured by the predicted population of Chengdu city multiplied 380,000–600,000 t/y
by waste production per capita per day (Li et al., 2015).
Governmental subsidy to the Due to a high maintenance cost of the incineration plant, local government is intended to give subsidy to 180 Yuan/tonne
incineration plant support its operation (Xin-gang et al., 2016).
Annual utilization of combustion The mass ratio of municipal waste and combustion improver is set as 0.8:0.2 (MOHURD, 2009) 100,000 t/y
improver
The price of standard coal The initial price is set by analogy to Cheng et al. (2007) 310 Yuan/t
Feed-in Tariff of incineration By field investigation 0.583 Yuan/kwh
Cost of waste incineration By field investigation 70 Yuan/tonne
Storage ratio of fresh leachate By investigation 20%
Cost of LFG pipeline construction According to the field investigation, the construction fee for LFG pipeline is 500 Yuan/m, and the distance 300,000 Yuan/y
between landfill and incinerator is 6KM. Thus, the one-off investment is 3 million Yuan with 10 years lifespan
of the pipeline. The annual fee equals to 300,000 Yuan.
Maintenance cost of incineration By investigation 100 Yuan/tonne
The leachate is pre-treated in-site by using physical method, and then validity. The common practice is to check whether the simulation
transferred to a municipal sewage treatment plant for advanced results of certain quantitative variables are in agreement with the
treatment. The sanitary landfill has started to receive municipal waste corresponding historical data (Li et al., 2014). This verification is
in 1993, and become the primary landfill for waste disposal in performed by comparing the relative error between the historical data
Chengdu. The landfill has an average reception of 959,368 t of waste and simulation results. However, the proposed system has not been
annually, and its associated LFG has not taken into account for the brought into implementation. It is difficult to compare the model
recovery, but emitted after torching, which poses a substantive risk to outcomes directly with the actual economic performance. Especially,
the public health and regional environment (Wu and Zheng, 2012). the filed investigation reflects that the project manager is not likely to
The input data to the key variables are mainly derived from field reveal the actually annual revenue of the investigated incineration
investigation and relevant studies, which are listed in Table 2. plant, which has been commissioned in 2008. In such case, the study
selects one of the key variables, i.e., landfill gas production, to validate
the model by comparing its historic generation with the simulation
4. Model validation
result. As the investigated landfill has been commissioned for waste
disposal in 1993, the actual LFG production from 1995 to 2015 are in
To ensure the model accuracy, it is necessary to verify the extent to
contrast with the simulation result, shown in Table 3. The relative error
which the model is consistent with actual situation. In this study,
of the tested variable is lower than 18%, with an average error of
behavior sensitivity is used for model validation, by which variables
3.91%, which reflects that the simulation result is approached to the
highly sensitive to the system is identified. Moreover, the system
actual generation, indicated that proposed SD model is valid to reflect
behavior is examined to judge its reasonability, once calibrating the
the real-world situation. Thus, further simulation can be conducted to
value corresponding to the identified sensitive variables (Talyan et al.,
investigate the possible variation in economic returns from changes in
2007; Wang et al., 2012). The ratio of purchased LFG and the ratio of
the purchased proportion of LFG and the proportion of leachate
leachate evaporation, which have a certain degree of subjectivity in
evaporation.
further scenario analysis, are considered as two of the most critical
variables affecting the economic performance of the incineration plant.
The sensitivity is calculated by the slope between −20% and +20% of 5. Simulation results and discussion
the variance in the two variables, to measure their influences on the
annual revenue of the investigated incineration plant. The larger the 5.1. Baseline scenario
slope is, the higher the sensitivity of the variables obtains.
By using the x-axis to indicate the purchased ratio of LFG, its change To investigate the possible impact of the purchased proportion of
to influence the annual revenue (indicated by the y-axis) is examined. LFG α and the proportion of leachate evaporation β on the annual
The evaporation ratio decreased by 20% gives rise to an increase of revenue of the investigated incineration plant, a benchmark revenue is
1.6% of the annual revenue, whilst the ratio increased by 20% results in determined by the independent operation of the municipal landfill and
a decrease of 1.5% of the annual revenue, shown in Fig. 4. incineration plant, as shown in Fig. 6. The simulation period of the
Similarly, using the x-axis to indicate the evaporation ratio, its established model is set to 30 years, which is consistent with the
variance to influence the annual revenue is also examined. The possible situation of LFG production. If the revenue of the integrated
purchased proportion of LFG decreased by 20% gives rise to an increase system is lower than the benchmark revenue, the attempt of interaction
of 1.0% of the annual revenue, while increasing by 20% it causes a is deemed as inapplicable. In such case, the incineration plant is still
decrease of 1.1% of the annual revenue, shown in Fig. 5. This result intended to use coal instead of LFG as the combustion improver.
indicates the availability of the proposed model, which can rationally Additionlly, if the calorific value is lower than the average waste
predict the outcomes when changes in system behavior occur. calorific value of Chengdu City, i.e., 5631.6 KJ/kg offered by Yang
Historical data comparison is also implemented for the behavioral (2014), the leachate evaporation process will be stopped.
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The initial value of α is transformed by using the principle of heat incineration plant with the changes of β, three options are considered:
conservation based on the purpose of substituting LFG for coal (1) the leachate evaporation keeps a constant-growth rate, and
combustion improver. It has been calculated that 100,000 t of standard considers β growing in a linear function; (2) the growth of evaporation
coal can be substituted by 80,000 cubic metre LFG (Zhao et al., 2012), if rate decreases gradually, and considers β growing in a convex function;
the integrated operation has been in application. Thus, the minimum (3) the growth of evaporation rate increases gradually, and considers β
value of α is set as to 0.0042. For the evaporation ratio β, the initial growing in a concave function. In each option, the interval of α is
value is set as zero due to the conventional treatment for the leachate. divided into 50 points by taking 0.02 as the step-length, fixed as 0.02,
The interval of α and β is determined as [0.0042, 1], [0,1] respectively. 0.04, 0.06, ultimately as1.0. Each α is given an input value for the SD
For seeking the optimal range of α and β, two scenarios are built by the simulation, to seek for the maximum annual revenue of the incineration
division of the above intervals. plant, and its corresponding β. On this basis, the maximum annual
revenues of the three options are obtained, by which the optimum LFG
purchased proportion is determined.
5.2. Simulation results of the scenario 1 By Taking α = 0.02 as a typical example, Fig. 7 shows the SD
simulation result of the annual revenue. The x axis represents the
In this scenario, the purchased proportion of LFG α is taken as a simulation time (year), whilst the y axis indicates the annual revenue of
fixed value, whilst the proportion of leachate evaporation β is set by the incineration plant (million Yuan). It is apparent that the annual
using a table function provided by the Stella Software Package. In order revenues corresponding to the three options are above the benchmark
to examine influences on the annual revenue of the investigated
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R. Zhao et al. Resources, Conservation & Recycling 124 (2017) 74–84
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R. Zhao et al. Resources, Conservation & Recycling 124 (2017) 74–84
revenue of the incineration plant of the Option 3 reaches the maximum Especially, it is even inferior to the benchmark revenue at the 13th
as 110.92 million Yuan, the greatest amount of the leachate evapora- time node, which indicates the Option 2 is not economically feasible for
tion is 41%. By taking both economic revenue and leachate treatment practical operation. Compared with the Option 3 and the Option 1, the
into account, it is implied that the Option 3 is optimal for further former revenue is higher than that of the latter, which can be deemed as
managerial implementation. When input α as 0.04, 0.06, 0.08… etc., the optimal scenario for further managerial implementation. When
into the SD model, the similar results can be obtained, which still input β as 0.04, 0.06, 0.08… etc., into the SD model, the similar
indicates the Option 3 is superior to the other two options. simulation results can be obtained. In case β = 0.12, the maximum
By taking β = 0.02 as an example in the Scenario 2, the annual revenue for the incineration plant is received as 105.71 million Yuan in
revenue of the Option 2 is the lowest among the three options. the Option 3, with its optimal purchase ratio of LFG as 10%.
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R. Zhao et al. Resources, Conservation & Recycling 124 (2017) 74–84
Based on the above analysis, the Option 3 in both the Scenario 1 and 2015; Hettiaratchi et al., 2015). However, the empirical models for
the Scenario 2 is identified as the optimal alternatives for possible prediction of LFG production, e.g., the Marticorena Dynamics Model
implementation. Fig. 9 further demonstrates the variation of the annual used in this study, Mexico LFG model, IPCC prediction model, multi-
revenue related to the two optimal options, which reflects that the phase prediction model etc., may be not sufficient enough to discrimi-
optimal option of the Scenario 1 has a better economic performance nate whether the landfill is at the stage of intensive gas production or
than that of the Scenario 2. not, thus may give rise to uncertainties of prediction (Cakir et al.,
As far as the treatment of leachate is concerned, the optimal option 2016). The second issue is that, evaporation itself, as a single process,
of the Scenario 1 is obviously superior to that of the Scenario 2, may not be effective to treat different types of leachate. For instance,
indicated by a larger proportion of the leachate evaporation, i.e. 4 times the relationship between leachate dosage and evaporation efficiency
bigger of the amount of evaporation, as shown in Fig. 10. may bring uncertainties in simulation results. There needs a careful
While giving both considerations to the economic and environ- design regarding leachate evaporation, particularly in its associated
mental performances, Scenario 1 is deemed as the optimal operation volatile components control, and reduction of high inorganic salt
scenario for further implementation, in which the incineration plant is concretion on the incinerator furnace wall (Zhao et al., 2012). It is
capable of purchasing 7% of the purified LFG, and evaporating 41% of thus recommended to combine the evaporation with other alternative
the in-site leachate. Ultimately, the annual revenue is expected to be treatment facilities. Specifically, leachate is generally divided into the
more than 110 million Yuan, 35% above the independent operation. young and mature leachate, according to age of landfill (Nair et al.,
Although the simulation results show that the integrated mode for 2014). The former may have higher BOD and COD contents than that
leachate thermal treatment has a great potential for future implementa- the latter has, by which the biological process coupled with evaporation
tion due to a substantial economic performance, there are still a number is expected to have a good performance on the leachate treatment
of uncertainties in evaluating the sustainable treatment system. With (Martin-Utrillas et al., 2015). With regard to the mature leachate, due
regard to the model, the uncertainty may result from any of the to its low biodegradability, refractory organics consisting of dissolved
quantitative expressions. For instance, the LFG in the model is organic matter (DOM), evaporation integrated with reverse osmosis
hypothesized as a stabilized alternative energy source for the combus- (RO), ultrafiltration etc., is recommended as the solution to reduce its
tion substitute of the incineration plant. The actual LFG generation is a organic and ammonia level (Wang et al., 2016b). From the perspective
complex progress, which may be influenced by considerable factors, of data uncertainty, it may come from its acquisition and reliability,
e.g. waste characteristics (density, biodegradation, moisture etc.), e.g., there is a lack of statistic data related to the economic performance
content of micro-organisms, conditions of either aerobic or anaerobic, of the investigated incineration plant, since it is newly built, thus may
the degree of initial compaction etc (Yang et al., 2013; Burnley et al., not validate the model robustly.
6. Conclusion
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