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Powder Technology: Mohammad Goharkhah, Armia Salarian, Mehdi Ashjaee, Mahmoud Shahabadi
Powder Technology: Mohammad Goharkhah, Armia Salarian, Mehdi Ashjaee, Mahmoud Shahabadi
Powder Technology
journal homepage: www.elsevier.com/locate/powtec
a r t i c l e i n f o a b s t r a c t
Article history: The effects of constant and alternating magnetic field on the laminar forced convective heat transfer of water
Received 26 August 2014 based magnetite (Fe3O4) ferrofluid in a heated tube are studied experimentally. The ferrofluid flows in a uniform-
Received in revised form 13 January 2015 ly heated tube with 9.8 mm diameter and 2680 mm length and is influenced by a magnetic field generated by
Accepted 18 January 2015
four electromagnets. The local convective coefficients are measured at both thermally developing and fully devel-
Available online 24 January 2015
oped regions for three different volume fractions of φ = 1, 1.5 and 2 % and in the Reynolds number range of
Keywords:
400–1200. The magnetic field and the resulting magnetic force distributions are also simulated to get further in-
Heat transfer sight into the heat transfer augmentation. In the absence of a magnetic field, results show that using magnetite
Forced convection ferrofluid with φ = 2 % improves the average convective heat transfer up to 13.5% compared to the DI-water
Magnetite at Re = 1200. This value grows up to 18.9% and 31.4% by application of constant and alternating magnetic
Nanofluid field with intensity of B = 500 G, respectively. The heat transfer is shown to be increased with the Reynolds num-
Alternating magnetic field ber, ferrofluid concentration, and the intensity of the magnetic field. Under the constant magnetic field, migration
Tube of nanoparticles to the tube surface increases the local thermal conductivity and consequently the heat transfer
near the electromagnets. Moreover, disruption of the thermal boundary layer and increased flow mixing seem to
be the possible reasons for the heat transfer enhancement by the alternating magnetic field.
© 2015 Elsevier B.V. All rights reserved.
http://dx.doi.org/10.1016/j.powtec.2015.01.031
0032-5910/© 2015 Elsevier B.V. All rights reserved.
M. Goharkhah et al. / Powder Technology 274 (2015) 258–267 259
increases up to 27.6% at low Reynolds numbers by an alternating magnet- circulating the nanofluid, tube test section, magnetic field generation
ic field. and control system, and data acquisition system for temperature
Recently, Azizian et al. [19] studied the effect of a constant magnetic recording.
field on the laminar convective heat transfer and pressure drop of mag-
netite nanofluid in a vertical tube and reported large enhancement in 2.2.1. Fluid circulation system
the local heat transfer coefficient against only a 7.5% increase of pressure Ferrofluid is circulated in a loop from a reservoir tank by a 24 V DC
drop. They also showed that the convective heat transfer enhancement pump driven by a DC power supply. Volumetric flow rate passing
increases with the magnetic field intensity and gradient. through the loop is measured using a calibrated flow meter, and can
The aim of this paper is to experimentally investigate the effects be varied by changing the voltage of the DC power supply of the
of constant and alternating magnetic field on forced convective pump. There is also a fluid collection tank for measuring and calibrating
heat transfer of Fe3O4 nanofluid in a long heated tube. For this pur- flow rates. The constant temperature bath (F10-Hc Julabo) is located
pose, the convective heat transfer coefficients have been measured upstream of the pump to control the inlet temperature. The exit heated
at both thermally developing and fully developed regions at different ferrofluid from the tube passes through a spiral copper tube which is
Reynolds numbers, magnetic nanoparticle concentrations, and mag- submerged in the thermal bath reservoir. Ferrofluid is cooled due to
netic field intensities. The results will be compared with those of no the heat transfer to the cold water inside the constant temperature
magnetic field. bath. Therefore, nanofluid inlet temperature to the tube can be con-
trolled by the thermal bath reservoir temperature.
2. Experimental method
2.2.2. Tube test section
2.1. Ferrofluid synthesis procedure The main part of the tube test section is a 2680 mm long straight alu-
minum tube with inner and outer diameters of 9.8 mm and 11.8 mm, re-
The ferrofluid samples are synthesized using the conventional spectively. The tube has a heat transfer section of 2380 mm. The
coprecipitation process. Briefly, stochiometric amounts of FeCl2.4H2O 100 mm entry and 200 mm exit lengths of the tube are unheated in
and FeCl3.6H2O equivalent to the chemical composition of Fe3O4 are dis- order to eliminate the end effects in the measurements. A constant
solved in DI-water and degassed via argon gas purging. Then, NH4OH heat flux is provided by passing electric current through a 3 mm thick
solution is gradually added into the iron solution under the mechanical flat-wire element. The heater is wounded on the entire tube surface
stirring until pH reaches 12. The black precipitate is removed from the and is connected to an AC power supply through a variac. It does not
liquid phase via centrifugal and magnetic separation and washed sever- contain any ferric material to prevent the distortion of the inner
al times by acetone and DI-water. The obtained solid product is magnetic field in the tube. The tube and heater are insulated with low
redispersed in DI-water and TMAH is added to the solution under stir- thermal conductivity elastomeric foam of 10 mm thickness. Two
ring in a manner that the desired volume fraction values of 1%, 1.5% polyurethane bushings are lathed and placed on the inlet and outlet of
and 2% are achieved. The stirring process is continued for an additional the aluminum tube to diminish the heat flow in the axial direction. A
1 h until the stable ferrofluid is obtained. SEM image of the synthesized small mixing chamber is located at the exit of the heat transfer
sample is presented in Fig. 1. section for the purpose of the accurate measurement of fluid exit
As seen in Fig. 1, nanoparticles with various shapes are aggregated temperature.
and formed larger agglomerates. The mean particle size is 30 nm. The surface temperature of the tube at the heat transfer section is
measured by 20 thermocouples coated with a compound of copper
powder and thermal paste. The thermocouples are installed on the
2.2. Experimental apparatus aluminum tube surface with an equal spacing of 125 mm. Also, locat-
ed in the inlet and outlet of the test section are two K-type thermo-
An experimental setup has been designed, implemented, and used couples to measure the inlet and exit temperatures of the fluid. All
to study the effects of constant and alternating magnetic fields on lam- the thermocouples used in this study are calibrated and the uncer-
inar forced convection characteristics of Fe3O4 ferrofluid in a heated cir- tainty of the temperature measurement is estimated to be less than
cular tube. The setup is presented schematically in Fig. 2. The main 1%. The thermocouples are connected to two data connected to a
components are: a constant temperature bath in a closed loop for PC such that all the temperature values can be monitored and re-
corded simultaneously.
The DC power supply is connected to a signal generator which is de- Teslameter has been used to measure the magnetic field strength during
signed to produce the alternating magnetic field with specific frequency the experiments.
and phase shift. It converts the input DC current to rectangular pulses
for driving the windings. With the help of its microcontroller, the digital 3. Data processing
circuit of the signal generator has the ability to adjust the frequency of
the pulses and their relative phase shifts. An oscilloscope is used to The local convection heat transfer coefficient on the tube surface is
monitor the wave form of the generated pulses. Furthermore, a HT201 calculated from:
q}
hðxÞ ¼ ð1Þ
T s ðxÞ−T m ðxÞ
where q" is the imposed constant heat flux to the aluminum tube and
Ts(x) and Tm(x) are the surface and bulk fluid temperatures, respective-
ly. Ts(x) is measured at 20 equally spaced points on the heat transfer sec-
tion of the tube surface. Through the energy balance, Tm(x) is calculated
from:
qx
T m ðxÞ ¼ þ T mi ð2Þ
L m Cp
where L is the length of heated section of the tube, ṁ is the mass flow
rate, q is the total heat flow and Tmi is the inlet temperature of the
fluid. The surface heat flux has been calculated from the net heat trans-
fer to the fluid using the following equation:
} m C p ðT mi −T m0 Þ
q ¼ ð3Þ
A
The heat flux can also be calculated from the total electric power
transferred to the aluminum tube divided by the surface area as follows:
} VI
q ¼ ð4Þ
A
where V and I are electric voltage and current, respectively, and A is the
surface area of the tube.
Fig. 3. (a) Magnetic field generation and control system; (b) dimensions of the A maximum discrepancy of 8% is observed between the two values
electromagnets. which is mainly due to the heat leaks through the insulations.
M. Goharkhah et al. / Powder Technology 274 (2015) 258–267 261
Table 1 The following equations have been used for calculation of nanofluid
Uncertainty of the measured parameters. bulk density and specific heat [20].
Quantity Uncertainty
Finally, using the obtained local convection heat transfer coefficients, where ρp is the particle density, ρf is the base fluid density and cp,p and
the average value is calculated from: cp,f are the particle and the base fluid specific heats, respectively.
Z The viscosity and thermal conductivity of the ferrofluid samples
L
1 at different volume fractions of φ = 1, 1.5 and 2 % have been
havg ¼ hðxÞdx ð5Þ
L measured by a viscometer (Antoon Paar Lovis 2000 M) and a KD2
0
pro device (Decagon Devices Inc.) for the temperature range of
4. Uncertainty analysis 20 − 600C.
In order to verify the accuracy of the transport properties measure-
Uncertainty of the experimental data may originate from the measur- ments, primary tests have been carried out for DI-water and the results
ing errors of quantities such as heat flux or temperature. The uncertainty have been compared with that of Incropera [21]. Viscosity and thermal
of the local convection heat transfer coefficient is calculated as follows: conductivity of the DI-water are shown in Fig. 4.
sffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi Fig. 4 indicates the reliability of the data obtained from the measure-
2 2 ments. Maximum deviations of 2.9% and 1.89% from the experimental
∂h } 2 ∂h ∂h
δh ¼ }
δq þ δT s þ δT m ð6Þ results of ref. [21] have been obtained for the thermal conductivity
∂q ∂T s ∂T m
and viscosity, respectively.
Then,
sffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi
} 2 2 2
δh δq δT w ∂T m
¼ }
þ þ δT m ð7Þ
h q T s −T m T s −T m
mp
ρp
φ¼ m mf ð8Þ
p
þ
ρp ρf
Fig. 4. Measured values of DI-water thermal conductivity and viscosity in comparison with Fig. 5. Variation of the measured ferrofluid (a) viscosity and (b) thermal conductivity with
data of Incropera and Dewitt [21]. concentration and temperature.
262 M. Goharkhah et al. / Powder Technology 274 (2015) 258–267
Measurements of nanofluid viscosity and thermal conductivity for Note also a large magnetic flux density gradient near the electro-
different concentration at various temperatures are shown in Figs. 5(a), magnet tips. Thus, large magnetic forces are expected in these regions.
(b), respectively. The magnetic force can be calculated from the magnetic flux density dis-
As shown, the dependence of nanofluid viscosity on temperature is tribution as follows [22,23]:
significant for all the concentrations. Decrease of nanofluid viscosity is
due to the decrease of the base fluid (DI-water) viscosity with temper- * χi * *
FM ¼ Vp B∇B ð11Þ
ature. Moreover, it is clear from Fig. 5(b) that the thermal conductivity μ0
increases with both temperature and concentration. The thermal con-
*
ductivity ratio of the ferrofluid to the DI-water increases from 10% to a where Vp is the nanoparticle volume and χi, μ0, and B are the magnetic
maximum of 16% at volume fraction of 2% as the temperature increases susceptibility of the magnetite nanoparticle, magnetic permeability of
from 20 to 60oC. This is due to the increasing Brownian motion of the free space, and magnetic flux density, respectively. Fig. 7 shows the cal-
nanoparticles at higher temperatures. culated x and z components of the magnetic force across the tube
centerline.
6. Magnetic field simulation Equation of motion for a single magnetic nanoparticle can be written
as follows:
Distributions of the magnetic field and the resulting Kelvin's mag-
netic body force for the given configuration of the electromagnets d2r * * *
have been simulated using COMSOL. Fig. 6(a) illustrates the magnetic m ¼ F M þ F Hydro þ m g ð12Þ
dt 2
flux density distribution B in the xz-plane obtained for an electric cur-
rent of I = 2A in the copper windings. Where, x is measured from the *
where r is the position vector of the particle and the first and second
tube inlet. Furthermore, the horizontal and vertical components (Bx,
terms are the magnetic and hydrodynamic drag forces, respectively.
Bz) and the magnitude of the magnetic flux density (B) along the tube
The opposing Stokes drag force on a spherical particle is given by:
centerline are plotted in Fig. 6(b).
Fig. 6(a) shows that the maximum magnetic field intensity exists *
near the tips of the electromagnets. As a result, the magnetic flux densi- F Hydro ¼ 6πμr p V r ð13Þ
ty B, has eight peaks of 700 G along the tube centerline, as shown in
Fig. 6(b). It can also be inferred from Fig. 6(b) that Bz has an alternating. where μ is the dynamic viscosity of the fluid, rp radius of a nanoparticle.
This is due to the opposite direction of the electric current in the wind- Vr is the relative velocity between the nanoparticle and the fluid with an
ings of each electromagnet. order of magnitude of 0.1m/s.
Fig. 6. (a) Magnetic flux density distribution in longitudinal plane; (b) variation of the magnitude of the magnetic flux density B and its horizontal and vertical components along the tube
centerline.
M. Goharkhah et al. / Powder Technology 274 (2015) 258–267 263
Fig. 8. Measured values of local convective heat transfer coefficient for DI-water flow in Fig. 9. Variations of local convective heat transfer coefficient along the tube for different
the channel compared with the predictions of Shah [23]. concentrations at (a) Re = 400 and (b) Re = 1200.
264 M. Goharkhah et al. / Powder Technology 274 (2015) 258–267
Fig. 12. Effect of a constant magnetic field on the local convective heat transfer coefficient
Fig. 11. Effect a constant magnetic field on the tube surface temperature. along the tube length for φ = 2 and Re = 600.
M. Goharkhah et al. / Powder Technology 274 (2015) 258–267 265
Fig. 13. Effect of an alternating magnetic field on the tube surface temperature. coefficients for the nanofluid and base fluid, respectively. The effects
Fig. 14. Effect of an alternating magnetic field on the local convective heat transfer coeffi- Fig. 15. Effects of constant and alternating magnetic fields on the average heat transfer co-
cient along the tube length for φ = 2 and Re = 600. efficient for (a) φ = 1 and (b) φ = 2.
266 M. Goharkhah et al. / Powder Technology 274 (2015) 258–267
of the constant and alternating magnetic field on the heat transfer en-
hancement are shown in Figs. 16(a), (b) and (c) for concentrations of
φ = 1, 1.5 and 2, respectively.
As Fig. 16 shows, the heat transfer enhancement increases with the
Reynolds number. This can be explained by the possible increase in
the flow mixing due to the formation of the magnetic aggregates in
proximity of the electromagnets. The increase of the heat transfer
with the nanoparticle volume fraction can also be justified considering
the mechanism described previously. The amount of the accumulated
particles near the tube walls increases with the increase of the volume
fraction. This leads to higher local thermal conductivity near the electro-
magnets. Moreover, further magnetic nanoparticles participate in the
disruption of the thermal boundary layer.
It should also be noted that the thermal entry length grows with the
Reynolds number and covers the entire tube length at high Reynolds
numbers of Re = 1000 and 1200. Therefore, the increase of the heat
transfer enhancement with Reynolds number implies that the effect of
magnetic field is more pronounced at the thermally developing region.
8. Conclusion
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