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Plasma Split Ring
Plasma Split Ring
Magnetic and surface plasmon resonances for periodic lattices of plasmonic split-ring resonators
Ruey-Lin Chern*
Institute of Applied Mechanics, National Taiwan University, Taipei 106, Taiwan, Republic of China
共Received 31 January 2008; revised manuscript received 9 July 2008; published 12 August 2008兲
In this study, the author investigates magnetic and surface plasmon resonances for periodic lattices of
plasmonic split-ring resonators by the use of the interface matching method. Magnetic resonance is character-
ized by a special frequency branch and illustrated with the localized eigenmode patterns. The basic features
associated with magnetic resonance are present at the long wavelength as well as at the Bloch wavelength
comparable to the size of a unit cell with minor distinctions. Near the surface plasma frequency, a large number
of highly resonant branches appear and surface plasmon resonance gradually becomes the dominated feature.
By varying the ratio of lattice constant to plasma wavelength, the influence of plasmonic property on magnetic
resonance is examined for rather small and large skin depths.
I. INTRODUCTION and lattice resonance.22 The former refers to the local re-
resonator1
Split-ring has been the essential element in the sponse of an individual element and the latter to the system
design of electromagnetic metamaterials2 in recent years. In- behavior due to the periodicity of the structure. At the long
tensive works were devoted to the studies of various split- wavelength, the local response dominates the dispersion
ring structures.3–6 Due to the adverse magnetic response,7–9 characteristics and can be well studied by the quasistatic
split-ring structures may exhibit a negative effective perme- approximation.1,23 At the Bloch wavelength comparable to
ability 共at the long wavelength兲,1,10 which is not available in the size of a unit cell, the local response and system behavior
naturally occurring materials. This unusual property is useful are intermixed to cause a somewhat complex phenomenon. A
in building a composite medium with simultaneously nega- more general analysis would involve a link between the local
tive permeability and permittivity11 and to demonstrate a and system responses.24
For plasmonic materials, the free-electron motion ac-
negative index of refraction.12,13 Based on split-ring resona-
counts for the dispersion and gives rise to frequency depen-
tors, left-handed coplanar waveguides,14 low-power micro-
dence of the dielectric property. The underlying problem is
wave plasma sources,15 and compact band pass filters16 can formulated as an eigensystem with the frequency as un-
also be realized. In fact, the split ring is itself a high Q known. Due to the evanescent nature of electromagnetic field
resonator17 and has been used in the design of electron-spin in plasmonic materials, the problem demands a delicate treat-
resonance spectroscopy18 and in measuring the microwave ment of boundary conditions at the interface. The interface
surface resistance.19 matching method is proposed for this purpose. This approach
Magnetic response of the split-ring structure is attributed is aimed to resolve the fields and related physical quantities
to resonance20,21 in which the ring acts as an inductor and the according to their surface-linking nature. On one hand, the
gap as a capacitor. The split-ring element is therefore consid- fields may exhibit a drastic change or rapid variation across
ered an analog of the LC circuit and serves to induce the the interface at which they are nondifferentiable or even dis-
magnetic activity in a structure composed of nonmagnetic continuous. A straightforward manner to deal with the prob-
materials. In order to seek for a large effect, very inhomoge- lem may lead to a nonlinear problem25 accompanied with
neous fields inside the structure are required,1 which indi- unstable or even inaccurate solutions. On the other hand, the
cates that the currents and charges would be significant when dominated physical quantities 共such as surface charge兲 are
the electromagnetic waves approach the resonance condition closely related to the property of interface.26 The matching
and have strong interactions with the medium. process at the interface brings in a linear formulation that can
For plasmonic split-ring structures, surface plasmon reso- be dealt with standard eigenvalue solvers.
nance serves as another distinguished feature. This type of In this study, magnetic and surface plasmon resonances
resonance comes from collective excitation of electric for plasmonic split-ring structures are investigated with em-
charges in the plasmonic material coupled with the electro- phasis on the dispersion characteristics. The frequency
magnetic fields. As the frequency approaches the surface branch associated with magnetic resonance is identified and
plasma frequency sp, surface plasmon resonance may occur. compared with the acoustical and optical branches that occur
The two types of resonances associated with the plasmonic for most periodic structures. Basic features of magnetic reso-
split-ring structure result from the interaction of waves with nance are illustrated with the corresponding localized eigen-
the medium, which is usually described in terms of disper- mode patterns in terms of fields, currents, charges, magnetic
sion. As split-ring elements are arranged to form a periodic moment, and effective permeability. On one hand, the prop-
lattice, the resonance features are contained in the dispersion erties based on the effective-medium theory1 are recaptured
relations = 共k兲 in which the variations of electromagnetic and integrated together to depict the magnetic resonance
fields in time and in space are correlated. from several aspects based on a more rigorous theory. On the
In periodic lattices, two scales of resonances are embed- other hand, magnetic resonance is explored at the conditions
ded in the overall dispersion characteristics: site resonance other than the long wavelength. In particular, basic features
The interface matching method is designed to solve the 共r + ai兲 = eik·ai共r兲, 共3兲
eigenvalue problem for dispersive materials when the fre-
applying at the unit-cell boundary where is either E or H
quency is considered as unknown.26 This approach is particu-
field, k is the Bloch wave vector, and ai 共i = 1 , 2兲 are the
larly useful in resolving the plasmon-dominated problem,
lattice translation vectors. The schematic of the unit cell is
where surface modes are essential to the overall dispersion
shown in Fig. 1. Using the Drude model 共兲 = 1 − 2p / 共2
characteristics. The basic idea of the interface matching
+ i␥兲 as the dielectric function of the metal and d as the
method is to separately deal with the wave equations in the
dielectric constant of the background material, Eqs. 共1兲 and
strict insides of the dielectric and plasmonic materials and
共2兲 are formulated as eigensystems with the frequency as
connect the two equations by matching the boundary condi-
unknown, where p is the bulk plasma frequency and ␥ is
tion at the interface. Equations in the separate regions 共di-
the damping constant. As appears in the differential opera-
electric and plasmonic兲 as well as at the interface are com-
tor, the eigensystems in Eqs. 共1兲 and 共2兲 become nonlinear in
bined together to yield a mixed formulation. The original
frequency.25
nonlinear problem25 is recast into a linear eigensystem with
The first step is to deal with the equations in the strict
standard format and can be efficiently solved by standard
insides of the two different media 共where the interface is
algorithms.27,28 A similar approach based on an auxiliary in-
excluded兲 so that the equation in either region can be rear-
terfacial variable has been proposed to deal with the prob-
ranged as
lems of plasmonic crystals,29 polaritonic crystals,30 and nega-
tive index crystals.31 In the present approach, the interfacial
variable is not applied and the problem is formulated with a
more direct manner.
−
1 2
d
ⵜ = 冉冊
c
2
, 共4兲
modes 共with time dependence e−it兲 are described in terms of for in the dielectric and metal regions, respectively. The
the field component along the column axis as32 above two equations are then connected by matching the
1
冉冊
− ⵜ 2E =
2
E, 共1兲
boundary conditions at the interface. Continuity of the tan-
gential H and E fields across the interface gives
冋 册 冋 册
c
E 1 H
−·
1
冉 冊冉冊
H =
c
2
H, 共2兲 n S
= 0,
n S
for transverse magnetic 共TM兲 and transverse electric 共TE兲 in the strict insides 关Eqs. 共4兲 and 共5兲兴 as well as at the inter-
polarizations, respectively. Here, TM 共TE兲 is referred to the face 关Eq. 共6兲兴 are arranged together to yield a generalized
case where the H 共E兲 field lies completely on the SRR plane. linear eigensystem that can be efficiently solved by standard
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MAGNETIC AND SURFACE PLASMON RESONANCES FOR… PHYSICAL REVIEW B 78, 085116 共2008兲
0.8
optical
Frequency (ωa/2πc)
0.6
(a)
0.4 magnetic
upper
lower
0.2
acoustical TM modes
TE modes
0
Γ X M Γ
Wave vector (k)
(b)
FIG. 2. 共Color online兲 Dispersion relations for the periodic lat-
tice of plasmonic split rings with w / a = 0.6, t / a = 0.1, s / a = 0.2, and FIG. 3. 共Color online兲 Magnetic-field vectors 共Re关H兴兲 of the TE
a / p = 10. The shaded region corresponds to the complete band gap eigenmodes for the plasmonic split-ring structure in Fig. 2. 共a兲 the
and the left and right circular dots denote the upper and lower band second mode at the point ⌫ 共upper band edge兲 and 共b兲 the first mode
edges, respectively. The inset shows four 共2 ⫻ 2兲 unit cells of the at the point M 共lower band edge兲.
structure. Dashed lines are results for the closed ring structure 共s
= 0兲 with the same thickness and width. increasing the Bloch wave number k and becoming flattened
near the point X关k = 共 / a , 0兲兴 or M关k = 共 / a , / a兲兴. On the
eigenvalue solvers without resorting to nonlinear techniques. other hand, the optical branch begins with a cut-off fre-
Details of the interface matching method can be found in quency and goes down as k increases in the range ⌫ − X or
Ref. 26. ⌫ − M.
2. Resonance branch
III. RESULTS AND DISCUSSION
Between the acoustical and optical branches, a special TE
Both the magnetic and surface plasmon resonances occur frequency branch 共the second band兲 appears, which is attrib-
in TE polarization, where the magnetic field aligns normal to uted to magnetic resonance associated with the split-ring
the lattice plane. This is because for TM polarization, the structure. For comparison, the dispersion curves for the
electric fields are parallel to the metal surface and continuous closed ring structure 共s = 0兲 with the same width and thick-
across the interface between the dielectric and plasmonic ma- ness are overlaid in Fig. 2 共in dashed lines兲 in which the
terials. As a result, no surface charges exist to excite the resonance branch is absent. Basic features related to the reso-
resonances. For plasmonic materials, the plasma wavelength nance branch will be identified from several aspects includ-
p = 2 / k p = 2c / p is a characteristic length scale associ- ing the field pattern, current and charge distribution, resultant
ated with the free-electron oscillation and is also a measure magnetic moment, and effective permeability. The resonance
of the skin depth for electromagnetic field.33 In the periodic branch begins with a cut-off frequency 共substantially lower
structure with lattice constant a, the ratio a / p = pa / 2c than that for the optical branch兲 and draws near to the optical
then serves as a plasmonic parameter to describe the signifi- branch as k increases. A complete band gap is opened be-
cance of plasmonic behavior. The dielectric constant d of tween the acoustical and resonance branches.
the surrounding dielectric is unity. Unless specified, the
damping constant ␥ is assumed to be zero. 3. Localized modes
In Fig. 3共a兲, the eigenmode on the resonance branch at the
A. Magnetic resonance point ⌫ is illustrated with the magnetic-field vectors. The
fields are intense inside the split ring, while outside the field
1. Dispersion relation
amplitude is substantially reduced and the field orientation is
Figure 2 shows the dispersion relations = 共k兲 for the even reversed. This inhomogeneous field pattern depicts a
periodic lattice of plasmonic split rings with w / a = 0.6, t / a local response of the individual element where the fields are
= 0.1, and s / a = 0.2. The plasmonic parameter is given as concentrated inside the split ring and the interaction between
a / p = 10 so that the ring thickness is comparable to the skin adjacent elements is weak. Localization of the fields within
depth; that is, t / p = 1. The first and the third TE modes individual elements prevents the electromagnetic energy
display a common feature for most periodic structures. They from being transferred across the unit cells and indicates the
are qualitatively similar to the acoustical- and optical-phonon existence of a complete band gap in the dispersion diagram
branches in the two-atoms crystal.34 The acoustical branch 共cf. Fig. 2兲. This feature consists with the negative value of
has a relatively lower frequency range, starting from zero the effective permeability1 and the low transmission in the
frequency at the point ⌫关k = 共0 , 0兲兴, growing up linearly with corresponding frequency range.11,35,36
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RUEY-LIN CHERN PHYSICAL REVIEW B 78, 085116 共2008兲
(a)
(b) (a)
4. Band edges
The point ⌫ on the resonance branch 关where the eigen-
mode in Fig. 3共a兲 is shown兴 corresponds to the upper band
edge and is considered as the long-wavelength condition. As
the Bloch wave number k increases, the resonance branch
gradually deviates from the band gap and begins to loses its
magnetic-resonance nature. Meanwhile, the acoustical
branch gradually approaches the lower band edge at the point
M. This is the condition where the Bloch wavelength is com-
parable to the size of a unit cell. The corresponding eigen-
mode in Fig. 3共b兲 shows a similar field pattern within the (b)
unit cell, except that the fields outside the split ring have an
antisymmetric distribution on opposing sides, in contrast to FIG. 5. 共Color online兲 Surface charge strengths 共Im关兴兲 and
the symmetric pattern in Fig. 3共a兲. This difference comes polarization current vectors 共Re关J p兴兲 of the TE eigenmodes for the
from the phase modulation by the Bloch wave vector and is plasmonic split-ring structure in Fig. 2: 共a兲 upper and 共b兲 lower
consistent with the Bloch condition 关Eq. 共3兲兴 that has to be band edges, respectively. The red 共dark gray兲 and green colors 共light
satisfied at the unit-cell boundary. As the fields are intense gray兲 correspond to positive and negative charges, respectively.
inside the split ring, the localized nature associated with
magnetic resonance still appears with a difference of the energy conversion between the electric 共stored in the gap兲
resonance frequency. The frequency difference between the and magnetic energies 共stored in the ring兲 has been initiated.
long wavelength 共resonance branch at the point ⌫兲 and the Inhomogeneous as well as localized fields thus serve as the
Bloch wavelength comparable to a unit cell 共acoustical typical feature of magnetic resonance associated with the
branch at the point M兲 makes up the band-gap width caused split-ring structure. Note that the distinction between Fig.
by magnetic resonance. 4共a兲 共upper band edge兲 and Fig. 4共b兲 共lower band edge兲 be-
comes less significant except at the portion near the cell
5. Electric fields boundary.
E= 冉
i Hz
y
x̂ −
Hz
x
冊
ŷ . 共7兲
tinuity of normal electric field at the surface as
= 0关n̂ · E兴S, where 关¯兴S denotes the jump across the inter-
face S and n̂ is the unit vector normal to the interface. As the
As the magnetic fields have significant changes from inside electric fields for the upper and lower band edges 关Figs. 4共a兲
the split ring to outside, the electric fields in the gap region and 4共b兲兴 share a very similar pattern near the interface, the
共the passage between inside and outside兲 are strongly en- surface charges shown in Figs. 5共a兲 and 5共b兲 are nearly iden-
hanced. The electric energy is raised and a mechanism of tical. Accumulation of surface charges illustrates the function
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MAGNETIC AND SURFACE PLASMON RESONANCES FOR… PHYSICAL REVIEW B 78, 085116 共2008兲
1
of a capacitor imbedded in the split-ring element as magnetic
resonance occurs.
0.8
7. Polarization currents
ωsp
Frequency (ωa/2πc)
In another aspect, the polarization fields P = 共 − 0兲E in-
0.6
duced in the plasmonic split-ring structure produce the po-
larization currents J p = Pt . These volume currents circulate
along the split ring and give rise to a magnetic moment 共per 0.4
085116-5
RUEY-LIN CHERN PHYSICAL REVIEW B 78, 085116 共2008兲
1
prevents most of the fields from penetrating into the plas-
monic material, the fields of surface plasmon mode become
0.8 highly localized at the interface and rapidly decay in either
ωsp the dielectric or plasmonic material.41 This feature consists
Frequency (ωa/2πc)
3. Large ratio
(a)
In another aspect, Fig. 10 shows the variation of
magnetic-resonance frequency range at large a / p, which
corresponds to relatively small skin depths. It is shown that
magnetic-resonance frequency approaches an asymptotic fre-
quency 共on the scale of a / 2c兲 at very large a / p, which is
identified as the result for perfect metal. In this situation, the
plasmonic behavior becomes less important and magnetic
resonance is mostly determined by the split-ring geometry.
(b)
4. Magnetic moment
FIG. 8. 共Color online兲 共a兲 Magnetic-field vectors 共Re关H兴兲 and
共b兲 electric-field vectors 共Im关E兴兲 of a typical surface plasmon mode Finally, the effect of plasmonic property is displayed with
for the plasmonic split-ring structure in Fig. 6. the dependence of magnetic moment on the plasmonic pa-
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MAGNETIC AND SURFACE PLASMON RESONANCES FOR… PHYSICAL REVIEW B 78, 085116 共2008兲
0.3 0.4
Upper edge
Lower edge
Gap ratio 0.3
0.2
0.2
0.1
0.1
0
moment
frequency
0 -0.1 -2
0 0.5 1 1.5 2 10 10-1 100 101 102
(a) a/λp a/λp
共at the upper band edge兲 with a / p 共in logarithm scale兲 for
the plasmonic split-ring structure with w / a = 0.6, t / a = 0.1,
and s / a = 0.2. For small a / p 共⬍0.2兲, the magnetic moment
0.1
increases linearly with the plasmonic parameter. In this
range, the polarization current strengths are relatively weak.
At large a / p 共⬎10兲, the magnetic moment tends to ap-
Upper edge
0 Lower edge
proach a constant value where the currents are highly local-
Gap ratio ized at the interface. A local maximum of the magnetic mo-
ment is located at an intermediate a / p 共⬇2.5兲. In this
0 0.2 0.4 0.6 0.8 1
(b) w/a situation, the plasmonic property exhibits a most favorable
contribution for sustaining the magnetic moment. Mean-
FIG. 9. 共Color online兲 Variation of magnetic-resonance fre- while, the magnetic-resonance frequency 共in dashed line兲 in-
quency range for the plasmonic split-ring structure 共a兲 with fixed creases monotonically with the plasmonic parameter until it
geometry: w / a = 0.5, t / a = 0.1, and s / a = 0.3 for various a / p and is saturated.
共b兲 with fixed a / p = 0.1 for various w / a 共t / a and s / a are changed
accordingly兲.
IV. CONCLUDING REMARKS
085116-7
RUEY-LIN CHERN PHYSICAL REVIEW B 78, 085116 共2008兲
number of highly resonant branches gathered around sp. for the prefect metal structure and magnetic resonance is
Band flattening, band broadening, and expected infinite num- mostly determined by geometric property.
ber of surface modes bear a close resemblance to those in
plasmonic crystals. The influence of plasmonic property on ACKNOWLEDGMENTS
magnetic resonance was also examined by altering the the The author thanks Ding-Ping Tsai at National Taiwan
ratio of lattice constant to plasma wavelength. For small ra- University and Pi-Gang Luan at National Central University
tios 共relatively large skin depths兲, the kinetic energy of free for their helpful discussions. This work was supported in part
electrons increases its importance and the resonance fre- by National Science Council of the Republic of China under
quency reaches a saturated value. For large ratios 共relatively Contracts No. NSC 96-2221-E-002-190-MY3 and No. NSC
small skin depths兲, the resonance frequency approaches that 96-2120-M-002-017.
Pendry, D. N. Basov, and X. Zhang, Science 303, 1494 共2004兲. Rev. B 72, 205112 共2005兲.
8 30 R. L. Chern, C. C. Chang, and C. C. Chang, Phys. Rev. B 73,
S. Linden, C. Enkrich, M. Wegener, J. Zhou, T. Koschny, and C.
Soukoulis, Science 306, 1351 共2004兲. 235123 共2006兲.
9 N. Katsarakis, G. Konstantinidis, A. Kostopoulos, R. S. Penciu, 31 R. L. Chern, C. C. Chang, and C. C. Chang, Phys. Rev. B 74,
085116-8