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To cite this version: Selle, Laurent and Poinsot, Thierry and Ferret,
Bernard Experimental and numerical study of the accuracy of flame-speed
measurements for methane/air combustion in a slot burner. (2011)
Combustion and Flame, vol. 158 (n° 1). pp. 146-154. ISSN 0010-2180
a b s t r a c t
Measuring the velocities of premixed laminar flames with precision remains a controversial issue in the
combustion community. This paper studies the accuracy of such measurements in two-dimensional slot
burners and shows that while methane/air flame speeds can be measured with reasonable accuracy, the
method may lack precision for other mixtures such as hydrogen/air. Curvature at the flame tip, strain on
the flame sides and local quenching at the flame base can modify local flame speeds and require correc-
tions which are studied using two-dimensional DNS. Numerical simulations also provide stretch, dis-
Keywords:
placement and consumption flame speeds along the flame front. For methane/air flames, DNS show
Laminar flame speed
Slot burner
that the local stretch remains small so that the local consumption speed is very close to the unstretched
Water addition premixed flame speed. The only correction needed to correctly predict flame speeds in this case is due to
the finite aspect ratio of the slot used to inject the premixed gases which induces a flow acceleration in
the measurement region (this correction can be evaluated from velocity measurement in the slot section
or from an analytical solution). The method is applied to methane/air flames with and without water
addition and results are compared to experimental data found in the literature. The paper then discusses
the limitations of the slot-burner method to measure flame speeds for other mixtures and shows that it is
not well adapted to mixtures with a Lewis number far from unity, such as hydrogen/air flames.
doi:10.1016/j.combustflame.2010.08.003
strongly varying and sophisticated interpolation methods are the paper (Section 8) discusses the limitations of the slot-burner
needed to find the flow speed at the flame location and deduce a method. Numerous effects (buoyancy, instabilities, non-unity Lewis
flame speed. Moreover, the stagnation-point flame is stretched number, etc.) that may impact the precision of the measurement are
and a model for the effects of stretch on flame speed is required discussed to try and define the type of flames for which the slot-bur-
to extrapolate the flame speed at zero stretch. The same problem ner technique may be a good choice for flame-speed measurements.
arises in Method 3 where the spherical flame is obviously growing A DNS of hydrogen/air flames is used to demonstrate that the slot-
and therefore stretched. Moreover, the precision of flame-speed burner method is difficult to apply for mixtures having a Lewis num-
measurements in spherical flames is the source of multiple contro- bers far from unity.
versies [20,33] because the front may not remain perfectly spher- The setup chosen here is a rectangular slot rather than circular
ical and is continuously submitted to a varying stretch [34–36]. as often found in the literature. The reasons for this are twofold: (1)
One great advantage of method 4 is that it does not require a model in this 2D slot burner, the flame sheets are perfectly planar in the
for stretch or curvature effects on the flame speed. Its accuracy measurement area and no curvature effect has to be taken into ac-
basically depends on the precision of temperature measurements. count (except at the flame tip unlike in the axisymmetric case
The slot-burner technique of Method 5 is probably the simplest where all flame sheets are curved) [29,30] and (2) simulations
one and this paper focuses on its capacities and limitations. First, are easier as well as velocity measurements.
methane/air flames stabilized on a slot burner are studied using
three approaches: 2. Experimental set-up
an experimental measurement in the slot-burner set-up (using The experiment used to measure the flame speed of a methane/
two methods to evaluate the flame length), air mixture is presented in Fig. 1. Flow rates are controlled and
a numerical calculation in a one-dimensional configuration measured using Bronkhorst flow meters. The temperature is regu-
using COSILAB and a full scheme for methane (GRI-Mech 3.0 lated to ensure a constant value in the plenum. Air is injected tan-
[37]) which gives a flame speed called s0L ðGRIÞ and gentially in the plenum where it mixes with methane jets. The flow
a two-dimensional calculation of the exact experimental set-up is then laminarized by an array of small balls, a honeycomb section
using a Direct Numerical Simulation (DNS) code [38,39] and a and a converging nozzle. The slot used to stabilize the flame is
simplified two-step chemical scheme (called 2SCM2) used in h = 10 mm wide and L = 100 mm long. The slot is water cooled
previous LES studies [40]. The same code is also used to com- and its surface temperature was measured around 350 K.
pute the laminar flame speed s0L ð2SCM2Þ for a one-dimensional Example of flames observed along the y axis are given in Fig. 2
flame with 2SCM2 to be used as a reference for two-dimen- for an equivalence ratio / of 0.8 (left) and 1 (right). The flame is
sional cases. thin, its length is easy to measure and changes strongly when /
varies making flame-speed measurements straightforward. A small
Using these three methods together allows to quantify the sys- quenched zone is observed at the flame base while its tip exhibits
tematic errors associated with the measurement of methane/air significant curvature: these effects are quantified in Section 5.
flame speeds using the length of a flame stabilized on a two-dimen- A view of the flame along the x axis is presented in Fig. 3 for / =
sional slot. In Section 2 the experimental set-up is presented; then 0.8: all measurements are performed in the central part of the slot
the methodology and potential sources of errors are discussed in (rectangular box of Fig. 3), where the flame is almost perfectly two-
Section 3. Section 4 presents the numerical tools: 1D code for flames dimensional. The side effects on the flame shape at y = 0 and y = L
(COSILAB) and two-dimensional DNS code. The results are described are discussed in Section 6.
first by investigating the flame structure revealed by DNS (Section To illustrate the method used to measure the flame length, a
5), then evaluating systematic measurement errors using DNS data typical image of the flame obtained for a bulk velocity Ub of
(Section 6) and comparing the experimental results with the COSI- 1.7 m/s and an equivalence ratio / of 0.8 is given in Fig. 4. This im-
LAB data and literature results (Section 7). All tests are performed age is used to evaluate the flame length Lf using two methods. In
for a methane/air flame at atmospheric pressure (1 bar) and stan- the first one (TRIANG), the flame is assumed to be a perfect triangle
dard temperature (300 K) over a range of equivalence ratio /, going and its length Lf is evaluated as LTf ¼ 2x where x is the triangle side
from 0.8 to 1.2 (Section 7.1). To illustrate the potential of the method, length. In the second method (IMAGE), the line corresponding to
it is finally used in Section 7.2 to study the influence of water vapor the maximum reaction rate is extracted from the flame image
addition on flame speed for a stoichiometric flame. The last part of (Fig. 4) and its length LIf is measured using image analysis.
Fig. 1. Slot burner with a square cross section for methane/air flames: (a) cross section of the whole burner, (b) zoom on the outlet section where the flame is stabilized.
was uniform at the outlet of the slot so that the flame angle could
be directly related to the flame speed. This approximation is rarely
valid and a different approach is used here. Consider the central
section of the flame (i.e. y = L/2) where the flow is 2D: the inte-
grated consumption of the flame ðqY F sL Lf Þ balances the fresh gases
flow rate (qYFU h) so that the mean consumption speed sL averaged
along the flame length is given by:
Uh
sL ¼ ð1Þ
Lf
Fig. 4. Flame images obtained experimentally superimposed with the flame length detection method (bold line). Center: raw image. Left: TRIANG method (a triangle is fitted
on the flame). Right: image processing is used to measure the flame length Lf.
gravity even though the burnt gases mix differently downstream Table 1
the flame front with and without gravity. Rate constants for the 2SCM2 scheme used in the two-dimensional DNS code: the
activation energies are in cal/moles and the preexponential constants in cgs units.
Of course, the measurement of the flame length Lf can also be
affected by other uncertainties and great care was used to identify A1 nCH
1
4
nO
1
2 Ea1 A2 nCO
2 nO
2
2
nCO
2
2 Ea2
the isoline of the images which tracks the reaction-rate zone. In a 210 15
0.9 1.1 34,500 210 9
1 0.5 1 12,000
first step, however, we will concentrate on the systematic errors
(a) to (c) and see if these errors are significant and must be ac-
counted for. If they are, our objective is to see whether Eq. (1) 0.5
can be corrected to use sL as a measure of s0L . To do this, the ratio
2SCM2
s0L =sL is measured in the DNS and the correction factor for system-
GRI-Mech 3.0
atic errors (a) to (c) is introduced as a factor g1:
R h=2
for a laminar flow in a rectangular duct (which is a good approxi- uðx; y ¼ L=2Þdx
exp ÿh=2
mation for the present case). These authors solved the Poisson g2 ¼ R h=2 ð10Þ
equation for the axial velocity field in a rectangular duct using ÿh=2
uPoi ðxÞdx
Legendre polynomia. They show that transverse velocity profiles This evaluation yields gexp
2 ¼ 1:054, which is close to the value ob-
(u(x,y) at fixed y) remain parabolic and they provide a simple fit tained analytically (gana ¼ 1:067 using Eq. (8). The experimental va-
2
(valid for a slot aspect ratio a P 3) linking the maximum velocity lue g2 = 1.054 was kept for the evaluation of s0L .
in the channel, u(x = 0, y = L/2), as a function of the bulk velocity
Ub and the aspect ratio a of the duct: Ub/u(x = 0, y = L/2) = 2/
7. Application
3 ÿ 0.4201/a. From this relation, the g2 factor can be obtained
using U = 2/3 u(x = 0, y = L/2):
Sections 5 and 6 can be summarized as follows: in the slot bur-
1
gana
2 ¼ ð8Þ ner of Fig. 1, the unstretched laminar flame speed s0L can be ob-
1 ÿ 0:6301=a tained from the averaged flame speed sL in a transverse plane by
Here, the aspect ratio a is 10 so that gana is 1.067. correcting it by two factors g1 and g2: g1 integrates the effect of
2
To verify this evaluation of g2, Pitot tube measurements were quenching at the flame base, strain and curvature effects. It is a
also performed on the experiment to evaluate the axial velocity small correction, estimated from a two-dimensional DNS as
along two lines: y = L/2 and x = 0 (cf. Fig. 1). As expected, two g1 = 1.010 for method TRIANG and 1.005 for method IMAGE. g2 is
boundary layers are observed at the extremities y = 0 and y = L of due to boundary effects at each extremity of the slot which lead
the slot (Fig. 8b) but the axial velocity profile in the transverse to a flow acceleration at the center of the slot where the flame
direction (Fig. 8a) is not perfectly parabolic, indicating that the shape is visualized and used to measure sL . This factor depends
flow is not fully established. The correction factor g2 can be evalu- only on the aspect ratio of the rectangular duct and is of the order
ated using the velocity measurements of Fig. 8b. For a very long of g2 = 1.054 for the present channel.
slot (i.e. large a), the velocity profile at the center of the slot
(y = L/2) is given by the Poiseuille solution: 7.1. Methane/air flames
3
x2
uPoi ðxÞ ¼ U b 1 ÿ ð9Þ The final result s0L ¼ g1 g2sL is now used to post process experi-
2 l
mental results for a methane/air flame at atmospheric pressure
For a finite A slot like in the present experiment, the Pitot tube mea- and temperature (T0 = 300 K). The method used to measure the
surements provide the axial velocity profile (Fig. 8a) and the correc- flame length is method IMAGE but method TRIANG leads to almost
tion factor g2 is simply expressed as identical values. Flame speed (s0L ) measurements are compared
Fig. 8. Axial velocity profiles obtained experimentally. (a) Transverse direction: u(x, y = L/2); (b) longitudinal direction: u(x = 0, y).
over a range of equivalence ratios with various other results: the 0.6
T=300 K (GRI)
numerical output of COSILAB in the same conditions is used as a
T=300 K (Exp)
reference but other experimental data are also introduced for com- 0.5 T=330 K (GRI)
parison [12,50–52,28,53]. Figure 9 displays flame speed values
T=330 K (Exp)
from / = 0.8 to 1.2. The only numerical result in Fig. 9 is the COS- 0.4 T=370 K (GRI)
ILAB data obtained with GRI-Mech 3.0. Measurements were per-
(m/s)
formed in the slot-burner set-up using an outlet bulk velocity
0.3
Ub = 1.9 m/s. The effect of this velocity was verified by changing
Ub from 1.2 to 1.9 m/s: such changes lead to variations in s0L smaller
than 0.3%. The present measurements agree well with COSILAB re- 0.2
sults. They are slightly higher than other experiments for lean
flames (except for the data of Gu et al. [51]) and slightly below 0.1
them for rich flames (except for the data of Halter et al. [54]). Con-
sidering the error bars on all flame-speed measurements (see for 0.0
example a summary of measured values for methane/air flames 0 50 100 150 200 250
in [28]), it is difficult to determine which method is the best but SH (g/kg)
the present one obviously gives reasonable results and matches
GRI-Mech 3.0 results very well. Fig. 10. Laminar flame speed s0L vs. specific humidity sH at 1 bar for a stoichiometric
flame. Symbols are experimental results, lines correspond to simulations with
COSILAB and GRI-Mech 3.0. Simulations at 300 K and 330 K are conducted up to the
saturation point of water vapor in air.
7.2. Methane/air flames with water vapor
This section presents an application of the slot-burner method a limited amount of water can be added to air at 300 K and the
to measure flame speeds of methane/air mixtures where the air flame speed is mildly affected: s0L is reduced by less than 15%. How-
contains water vapor. In most practical applications of combustion ever, at 330 K s0L can be divided by two, which may have a signifi-
in air, significant amount of water vapor may be present in the air cant impact on the operation of the engine. For these two
stream, either because of natural atmospheric conditions or conditions, the measurements closely match the numerical simula-
through intentional water addition. For example, in gas turbines tions of COSILAB. For engines that may have a much higher inlet
water is added to lower emission levels; in piston engines when temperature together with direct water addition or EGR, a numer-
Exhaust Gas Recirculation (EGR) is used, water present in the com- ical simulation at 370 K shows that the flame speed can be reduced
bustion products modifies the flame speed by changing the heat by 90%. These effects are important and must be incorporated in
capacity of the mixture, but also its kinetics. Measuring these ef- models used for combustion in piston engines and gas turbines.
fects is of interest and the slot burner methodology was applied
to the combustion of methane in air containing water vapor. Since
the Lewis number of water vapor is close to unity, the local effects 8. Extension to other flames and limitations
of stretch and curvature are expected to match those of the meth-
ane/dry-air flame. Consequently, the correction factor g1 derived in The previous sections have shown that the slot burner was a
Section 5 is retained. The factor g2 solely depending on the burner reasonably accurate and inexpensive technique to measure flame
geometry is also kept constant. The water-vapor content is quanti- speeds for methane/air mixtures. Similar methods are routinely
fied by the specific humidity sH, defined as the ratio of the mass of used in the literature to measure flame speeds and an interesting
vapor to the total mass of humid air (air plus water). At a given question that came out during this work is the validity of the
temperature, the specific humidity is bounded by the saturation approach in a more general framework: can this method be used
of water in air: typically, at T = 300 K, the saturation specific for all mixtures? The answer is negative because of multiple
humidity is ssat sat
H ¼ 21:8 g=kg and at T = 330 K, sH ¼ 112 g=kg. The factors:
measurements of laminar flame speed s0L at stoichiometry for three
fresh-gases temperature are presented in Fig. 10, together with 1. Very slow flames will be submitted to buoyancy effects.
numerical simulations using COSILAB and GRI-Mech 3.0. The two 2. Slot flames are also known to be highly unstable, exhibiting
lower temperatures correspond to operating conditions of an air- strong pulsations. In most cases, these pulsations are due to
breathing engine in standard to extreme conditions. Because acoustic coupling mechanisms between the flame and the ple-
saturation occurs for smaller sH values at lower temperatures, only num [55–57].
3. Flames with non-unity Lewis number are strongly affected by
40
preferential diffusion where the reaction zone is curved. For a
(cm/s)
slot flame, both the tip and the shoulder are curved potentially
35 affecting the average flame speed and leading to non-unity val-
Present experiment ues for the correction factor g1 defined in Eq. (2). This effect is
Laminar flame speed,
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