Download as pdf or txt
Download as pdf or txt
You are on page 1of 8

Nuclear Engineering and Design 374 (2021) 111066

Contents lists available at ScienceDirect

Nuclear Engineering and Design


journal homepage: www.elsevier.com/locate/nucengdes

Study on strategy construction for dismantling and radioactive waste


management at Fukushima Daiichi Nuclear Power Station
Akira Asahara *, Daisuke Kawasaki , Satoshi Yanagihara
University of Fukui, 1-3-33 Kanawa-cho, Tsuruga-shi, Fukui 914-0055, Japan

A R T I C L E I N F O A B S T R A C T

Keywords: Upon the commencement of the phase-three decommissioning of Fukushima Daiichi Nuclear Power Station
Radioactive waste management (FDNPS), strategy construction is a necessary step for effective radioactive waste management as well as safe
Decommissioning project implementation. In this study, we evaluate safety and environmental detriment (SED) score of radioactive
SED score
materials in the expected major stages of the project for the strategy construction. Following assumptions are
Fukushima Daiichi Nuclear Power Station
made for the evaluation. The phase-three decommissioning, which is defined as active decommissioning, pro­
ceeds in the order of fuel debris retrieval, core component removal, piping & equipment dismantlement, and
building structures demolition. The radioactive waste management proceeds in the order of pre-treatment,
treatment, and conditioning. SED scores are calculated for each of the four groups of objects (object-base) and
their total (plant-base) at a specific point of time during the active decommissioning, considering the progress of
the radioactive waste management. The calculation results indicate following suggestions for strategy con­
struction. First, treatment and conditioning of fuel debris and core components make a large contribution for
reducing plant-base SED score during the active decommissioning. Second, nearly 90% of achievable amount of
reduction in plantbase SED score could be realized without piping & equipment dismantlement and building
structures demolition. Third, since plant-base SED score could be hugely influenced by physical form of fuel
debris, it may be necessary to consider work plan from the viewpoint of cutting and containing methods. Those
perspectives would be useful input to construct active decommissioning strategies together with project man­
agement parameters such as staffing, technical capability, and financial readiness.

1. Introduction been made toward starting the phase three especially for characteriza­
tion of the core part; robotic systems have been deployed to survey the
The decommissioning project of Fukushima Daiichi Nuclear Power conditions inside primary containment vessel (PCV) of damaged units
Station (FDNPS) has been steadily progressing under the Mid-and-Long- (IRID and IAE, 2018; Yamashita et al., 2020). Also, scenarios of fuel
Term Roadmap towards the Decommissioning of TEPCO’s Fukushima debris retrieval have been studied, which include top access with sub­
Daiichi Nuclear Power Station Units 1–4 (The Inter-Ministerial Council mersion, top access with partial submersion and side access with partial
for Contaminated Water and Decommissioning Issues, 2019). The submersion to retrieve fuel debris by remote handling technologies
roadmap defines three phases in the decommissioning project; phase (NDF, 2019). However, the detailed plan of the phase three after fuel
one is for preparation of spent fuel removal from spent fuel pool; phase debris retrieval have not been described in the roadmap. On the other
two is for spent fuel removal and preparation of fuel debris retrieval; hand, current efforts on radioactive waste management have been
phase three is major part of the decommissioning project, in which the devoted mainly for managing the radioactive wastes generated until
fuel debris is retrieved, structures, systems, and components of facilities now, estimating radionuclide composition in the wastes, and planning of
are dismantled and removed, and finally the buildings are demolished to treatment of radioactive wastes to be generated within around 10 years
complete the decommissioning project. Those activities are defined as ahead (Sugiyama et al., 2019; TEPCO, 2019).
active decommissioning in this paper. Up to the present, progress has Strategy construction is a necessary step for planning of radioactive

Abbreviations: TEPCO, Tokyo Electric Power Company; FDNPS, Fukushima Daiichi Nuclear Power Station; SED, Safety and environmental detriment; RHP,
Radiological hazard potential; FD, Facility descriptor; WUD, Waste uncertainty descriptor; FF, Form factor; CF, Control factor.
* Corresponding author.
E-mail address: aasahara@u-fukui.ac.jp (A. Asahara).

https://doi.org/10.1016/j.nucengdes.2021.111066
Received 30 September 2020; Received in revised form 30 December 2020; Accepted 6 January 2021
Available online 29 January 2021
0029-5493/© 2021 The Authors. Published by Elsevier B.V. This is an open access article under the CC BY license (http://creativecommons.org/licenses/by/4.0/).
A. Asahara et al. Nuclear Engineering and Design 374 (2021) 111066

waste management in the active decommissioning. Prioritization of the 2.2. Radioactive waste management
active decommissioning is one of the significant challenges in strategy
construction for the decommissioning project. UK Nuclear Decom­ During each of the above-mentioned stages of the active decom­
missioning Authority (NDA) has developed a prioritization measure missioning, radioactive materials are generated by removing from their
called Safety and Environmental Detriment (SED) score for effective original places and they need to be managed as radioactive waste. Ac­
decommissioning and site remediation, including decontamination, cording to the IAEA, radioactive waste management could be catego­
dismantling, waste management, etc. (NDA, 2011). Since calculation of rized into six steps: pre-treatment, treatment, conditioning, interim
SED scores considers both the intrinsic properties of a material and the storage, transport and disposal. Interim storage must be provided for
current conditions of the material and its confining facility, it could be untreated/unconditioned waste as well as for conditioned waste (IAEA,
applied to decommissioning, site remediation, radioactive waste man­ 2017). In this study, an SED score is calculated for each radioactive
agement where hazardous materials will be treated. We can see some material before pre-treatment (defined as ’as-it-is’) and in storages after
applications in literature (Jarjies et al., 2013; Utkin and Linge, 2019). each of the three steps: pre-treatment, treatment, and conditioning,
Nuclear Damage Compensation and Decommissioning Facilitation Cor­ respectively. Pre-treatment consists of removal of the materials from its
poration of Japan (NDF), which has a responsibility to develop technical original place by cutting/dismantling/demolishing/segregating and
strategic plan, has applied SED scores for prioritizing on-site activities to placement of the removed materials into temporary containers. Treat­
reduce various radiation risk relating to such as spent fuel, fuel debris, ment consists of desiccation process or volume reduction process and
secondary waste arising from treatment of contaminated water, and packaging into storage containers. Desiccation is applied to fuel debris
concrete rubbles (NDF, 2019). However, its application is limited only to and core components, while volume reduction applied to piping &
D&D activities for the time being. equipment and building structure. Conditioning is solidification or sta­
In this study, we have studied SED scores in order to obtain useful bilization process for onsite long-term storage. Vitrification is assumed
input to strategy construction of active decommissioning and radioac­ as a conditioning method for fuel debris because it is applied to high
tive waste management of FDNPS. Since the main purpose of this study level radioactive waste produced by reprocessing of spent fuel in Japan.
is to see the applicability of SED scores as a prioritization measure, only Similarly, cementation is assumed for core components and piping &
reactor building of unit 1 is considered as a case study. The active equipment as it is applied to low-level radioactive waste. The condi­
decommissioning is assumed to consist of fuel debris retrieval, core tioning is not applied to building structure, which is to be packaged into
components removal, piping & equipment dismantlement, and building flexible containers after being demolished. In this paper, we focus on the
structures demolition. The radioactive waste management is categorized activities that are likely to be done within the site of FDNPS, and we
into pre-treatment, treatment, and conditioning. Details of the active exclude the transport and disposal.
decommissioning and radioactive waste management are explained in
the following section. By modifying evaluation criteria for the applica­ 2.3. SED score calculations
tion to FDNPS, SED scores are calculated for each of the four groups of
objects (object-base) and their total (plant-base) at a specific point of SED score consists of three attributes: the intrinsic properties of a
time during the active decommissioning, considering the progress of material, the current conditions of the material, and the current condi­
radioactive waste management. The analysis of SED scores would be tions of a facility that contains it. It can be therefore generally used as a
useful to construct active decommissioning strategies together with prioritization measure in the active decommissioning and radioactive
project management parameters such as staffing, technical capability, waste management. The scores are calculated using the following
and financial readiness. equation:

2. Methods SEDscore = RHP × (WUD × FD)n , (1)

This section describes how SED scores are calculated for unit 1 of where RHP denotes the degree of hazard originating from radionuclides
FDNPS. First, assumptions are made on how the active decommissioning in materials, WUD the potential for dispersion of the radioactive mate­
and radioactive waste management proceed. Then, the process of SED rial due to degradation with time, FD the degree of confinability by the
score calculations are described. After that, assumptions about radio­ facility containing radioactive materials. RHP is calculated based on the
active materials and confining facilities for them are made as an input total radioactivity in materials and estimated to range from 100 to 1012
for calculating SED scores. in the case of FDNPS. WUD and FD are scored ranging from 100 to 102,
respectively. The n is a balancing factor so that effect of WUD and FD
2.1. Four stages in active decommissioning becomes dominant on prioritization. SED score is a multi-attribute
scoring method that takes account of potential impact of stored mate­
Generally speaking, decommissioning process proceeds from ’hot to rials being released into the environment, not only simple radiotoxicity
cold’, namely from higher radioactivity to lower radioactivity. The four or surface radiation dose. In this study, SED scores are calculated for
stages in this assumption are made based on this approach. The active each object, namely, fuel debris, core components, piping & equipment,
decommissioning proceeds in the following order of four stages: fuel and building structure.
debris retrieval, core components removal, piping & equipment RHP is derived from the following equation:
dismantlement, and building structures demolition. The objects of those ∑
RHP = Ai × Pi × FF × CF − 1 , (2)
four stages are fuel debris, core components, piping & equipment and all nuclides i
building structures, respectively. The fuel debris is defined as fuel as­
sembly, control rod and structures inside reactor that have melted and where, Ai denotes the radioactivity (TBq) of radionuclide i, Pi the
solidified together (NDF, 2019). The core components are equivalent to amount of water required to dilute radionuclide i for safe drinking (m3/
equipment and structures inside the PCV such as reactor pressure vessel, TBq), FF (Form Factor) the fraction of radionuclides being released if its
steam dryer, shroud, etc. The piping & equipment are components confinement is completely lost, and CF (Control Factor) the length of
located outside PCV but inside reactor building. The building structures time a material itself can maintain the current stabile state if safety
are mainly made of reinforced concrete that makes up biological measures against its chemical or radiological properties such as flam­
shielding and reactor building. mability, reactivity with air or water, heat generation, etc. are
completely lost. The worst and the best FF are 100 and 10− 6, respec­
tively. The worst FF is given to radionuclides in the form of gas or liquid,

2
A. Asahara et al. Nuclear Engineering and Design 374 (2021) 111066

100% of which could be dispersed, while the best FF in the form of large dispersed if their containment is lost in as-it-is. After pre-treatment
monolithic solid or activated component, almost 0% of which could be where piping & equipment and concrete structure are cut into pieces,
dispersed. The worst and the best CF are 100 and 105, respectively. The their FF becomes 10− 3 as their internal surface contamination becomes
worst CF is given to radionuclides that become unstable in ‘hours’ if its dispersible.
safety measure is lost, while the best CF to radionuclides that maintain CF is set based on the reactivity with other materials, considering
its stability for ‘decades (more than 87,600 h ≈ 105 h)’. Pi of each hydrogen and hazardous gas production due to radiation decomposition
radionuclide has been calculated using an equation in the NDA report of water and metallic corrosion. Fuel debris in both as-it-is and pre-
(NDA, 2010). Tables for FF and CF are provided in Appendices. treatment have possibility to produce hydrogen because of existing
Evaluation criteria of WUD and FD have been modified to meet the cooling water, and droplet adhered to the materials after segmentation.
conditions of FNDPS 10 years after the accident, rather than legacy Desiccation in treatment reduces probability of hydrogen production by
nuclear sites that NDA are targeting. For scoring WUD in this study, reducing the amount of water contents. The possibility of hydrogen
considered evaluation criteria are a) generation of hazardous gases, b) production remains low after the treatment. CF represent the frequency
dispersion due to physical degradation, c) lack of containers, and d) lack of human intervention such as monitoring or ventilation, namely, 100
of monitoring. For scoring FD, considered evaluation criteria are a) for fuel debris in as-it-is, 101 in pre-treatment, 102 in treatment, and 105
presence of significant defects, b) unsatisfaction of safety standards, c) in conditioning, respectively. CF of core components in as-it-is is set as
insufficient layers of boundary, d) excess of remaining building life, and 103 considering the possibility of hazardous gas production due to
e) loss of its boundary by failures of neighbouring facilities. Tables 1 and metallic corrosion. Desiccation in treatment reduces probability of
2 show evaluation criteria and the corresponding numbers of WUD and hazardous gas production by reducing the amount of water contents.
FD, respectively. Therefore, CF of core components in pre-treatment, treatment, and
The value of n is determined so that RHP and WUD × FD have the conditioning is set as 104, 105, and 105, respectively. CF of the other
same contributions to SED scores in average as a whole process of objects is set as 105 because they do not have probability of hydrogen or
radioactive waste management, using the following equation: hazardous gas production.
∑N=4 ∑M=4 log(RHPi )
n= /(N × M) (3) 2.5. Radioactive inventory
j=step log(WUD
i ) + log(FDi )
i=object

Radioactivity of all objects in as-it-is is estimated at 10 years after the


where N is the number of objects i and M the number of radioactive
accident, when the active decommissioning is planned to begin. For
waste management steps, respectively.
estimating radioactive inventory of fuels, burnup calculation results for
unit 1 of FDNPS are referred (Nishihara et al., 2012). For the other ob­
2.4. FF and CF jects, the radioactive inventory is considered to be from two sources:
activation and contamination. Radioactive inventory due to activation is
FF is set depending on physical form of object. The physical form of referred from the calculation of a reference BWR reactor (Oak et al.,
fuel debris in as-it-is is assumed to be either sludge, powder, or discrete 1980) and that due to contamination is referred from the study on
solid. That of core components is discrete solid and large monolithic release fraction of radionuclides from the reactor core (Shibata, et al.
components. That of piping & equipment and building concrete is large 2016). According to the reference, core shroud, piping in the primary
monolithic components. system, and biological shielding have the dominant radioactivity in each
Physical form can be changed in some steps in radioactive waste of the three objects, respectively. The radioactive inventory of the three
management. The physical form of fuel debris does not change by pre- objects is extracted from that of those dominant components.
treatment, while those of the other objects change from large mono­ As a source of contamination, Cs-137 is taken into account as the
lithic components to discrete solid by pre-treatment. The physical form dominant radionuclide released from the fuels. For estimating its
of all objects does not change by treatment and change into large radioactivity, the assumption is made that the contamination distribu­
monolithic solid by conditioning. In the case of building structure, tion is 0.3, 0.2, and 0.1 among core components, piping & equipment,
however, its physical form does not change by conditioning where and building structure, respectively, considering the closer the object to
crushed concrete rubbles are packaged into flexible containers. the fuel, the higher the degree of contamination with Cs-137. Further­
FF represent the size of the physical form (NDA, 2010), namely 10− 1 more, the release fraction of Cs-137 from the core is estimated to be 60%
for sludge and powders, 10− 5 for relatively large (< 1 ton) solid, and (Sugiyama et al., 2019). Table 3 shows radioactivity and specific toxic
10− 6 for very large (> 1 ton) components. FF of fuel debris in as-it-is is potential (Pi) of the radionuclides that have dominant contribution to
conservatively assumed to be 10− 1. FF of core components in as-it-is are SED scores of each object.
assumed to be 10− 3 since there is external surface contamination that is
more dispersible than discrete solid but less than powder. FF of piping & 2.6. Confining facilities for radioactive materials
equipment and concrete structure is assumed to be 10− 6 although they
are contaminated on their internal surface that is unlikely to be The potential of loss of confinement is evaluated as FD in SED cal­
culations. The confining facilities are specified by postulating that new
Table 1 facilities for confining the objects will be constructed in the process of
WUD evaluation criteria and corresponding numbers. the active decommissioning. An auxiliary building adjacent to the
reactor building will to be constructed prior to fuel debris retrieval for
Criteria Categories
receiving pieces of fuel debris, core components, and pipes & equip­
1 2 3 4 5 6 7 8 9 10 ment. A covering structure will be installed as a containment for
a) Generation of Y Y Y Y N N Y Y N N building structures prior to demolition. Waste storage facilities will be
hazardous gases constructed to receive wastes that have been treated or conditioned.
b) Potential impact Y Y N N Y Y Y N Y N
Table 4 lists those facilities for each object.
of degradation
c) Lack of packaging Y Y Y Y Y Y N N N N
d) Lack of Y N Y N Y N N N N N
monitoring
WUD 100 90 74 50 30 17 9 5 3 2

Y = yes, N = no.

3
A. Asahara et al. Nuclear Engineering and Design 374 (2021) 111066

Table 2
FD evaluation criteria and corresponding numbers.
Criteria Categories

1 2 3 4 5 6 7 8 9 10

a) Presence of significant defects L L U U L U U U U U


b) Unsatisfaction of safety standards L L L L L L U U U U
c) Insufficient layers of boundary L P L P U U U U U U
d) Excess of remaining building life L L L L L L L P U U
e) Loss of its boundary by failures of neighbouring facilities L L L L L L L L L U
FD 100 91 74 52 29 15 8 5 3 2

L = likely, P = possible, U = unlikely.

Table 3 Table 5
Radioactivity and specific toxic potential of dominant radionuclides of FDNPS FF, CF and RHP of objects in different steps of radioactive waste management.
unit-1. Objects Steps of radioactive FF CF RHP
Objects Radionuclides Radioactivity (Ai) Specific toxic potential waste management
(TBq) (Pi) (m3/TBq)
Fuel debris As-it-is 1.00E- 1.00E+00 4.69E+11
Fuel debris Pu-238 4.72E+03 1.38E+08 01
Pu-241 1.38E+05 2.88E+06 Pre-treatment 1.00E- 1.00E+01 4.69E+10
Am-241 3.37E+03 1.20E+08 01
Sr-90 1.18E+05 1.68E+07 Treatment 1.00E- 1.00+02 4.69E+09
Cs-137 1.61E+05 7.80E+06 01
Core Fe-55 8.90E+03 1.98E+05 Conditioning 1.00E- 1.00E+05 4.69E+01
components Co-60 1.23E+04 2.04E+06 06
Ni-63 1.13E+04 9.00E+04 Core As-it-is 1.00E- 1.00E+03 4.05E+05
Cs-137 4.83E+04 7.80E+06 components 03
Piping & Co-60 1.97E+01 2.04E+06 Pre-treatment 1.00E- 1.00E+04 4.05E+04
equipment Cs-134 1.06E-01 1.14E+07 03
Cs-137 3.22E+04 7.80E+06 Treatment 1.00E- 1.00E+05 4.05E+03
Building Fe-55 3.49E-01 1.98E+05 03
structure Co-60 2.77E-02 2.04E+06 Conditioning 1.00E- 1.00E+05 4.05E+00
Eu-152 9.46E-03 8.40E+05 06
Cs-137 1.61E+04 7.80E+06 Piping & As-it-is 1.00E- 1.00E+05 2.51E+00
equipment 06
Pre-treatment 1.00E- 1.00E+05 2.51E+03
03
Table 4 Treatment 1.00E- 1.00E+05 2.51E+03
Facilities confining objects in different steps of radioactive waste management. 03
Conditioning 1.00E- 1.00E+05 2.51E+00
Objects Steps of radioactive waste Confining facilities 06
management Building As-it-is 1.00E- 1.00E+05 1.26E+00
Fuel debris As-it-is PCV structure 06
Pre-treatment Auxiliary building Pre-treatment 1.00E- 1.00E+05 1.26E+03
Treatment Waste storage 03
facility Treatment 1.00E- 1.00E+05 1.26E+03
Conditioning Waste storage 03
facility Conditioning 1.00E- 1.00E+05 1.26E+03
Core components As-it-is PCV 03
Pre-treatment Auxiliary building
Treatment Waste storage
facility debris and core components, RHP steadily decrease by ten and five or­
Conditioning Waste storage ders of magnitude from as-it-is to conditioning, respectively. On the
facility other hand, RHP of both piping & equipment and building structure does
Piping & As-it-is Reactor building
equipment Pre-treatment Auxiliary building
not decrease by completing waste management up to conditioning. As
Treatment Waste storage for fuel debris and core components, the decrease in RHP from as-it-is to
facility treatment is a change in CF because of the reduction in the amount of
Conditioning Waste storage water surrounding those objects by their retrieval from the core and the
facility
desiccation process, while the decrease from treatment to conditioning
Building structure As-it-is Covering structure
Pre-treatment Covering structure is a change in FF as a result of solidification process. As for the other two
Treatment Waste storage objects, the increase in RHP by completing pre-treatment is a change in
facility FF because of their surface contamination becoming dispersible by
Conditioning Waste storage segmentation. RHP of building structure does not change by condi­
facility
tioning because the process does not change its physical form. In addi­
tion, by completing conditioning, RHP of core components, piping &
3. Results and discussion equipment, and building structures are almost the same order of
magnitude as that of fuel debris. This is because Cs-137 originating from
3.1. RHp the accident has the dominant contribution in radioactive inventory of
the former three objects. In other words, RHP of piping & equipment and
RHP is calculated for all objects with different in radioactive waste building structures in as-it-is after planned shutdown are three and six
management. The calculation results are shown in Table 5. As for fuel orders of magnitude less than the case of FDNPS, respectively.

4
A. Asahara et al. Nuclear Engineering and Design 374 (2021) 111066

3.2. WUD and FD connection with reactor building for transporting those objects.
Covering structure of reactor building will meet safety standards as a
WUD is set assuming characteristics of objects. The setting is made by storage facility for demolished concrete but will be temporarily pre­
whether each criterion is judged as yes or no by referring Table 1. pared to demolish reactor building and likely to have limited design life
The characteristics of the objects in as-it-is are postulated as follows. as a storage facility. The other confining facilities are supposed to have
Fuel debris and core components have a possibility of physical degra­ sufficient protections of wastes and not potential to be affected by fail­
dation due to contact with water. Piping & equipment are not expected ures of other on-site facilities. Consequently, for the PCV, a) presence of
to progress significant physical degradation, which is expected in significant defects is figured as likely, and c) insufficient layers of
building structures due to physical damage at the time of the accident. boundary as possible, and FD is set as 91. For reactor building and the
Consequently, WUD of each object in as-it-is is given as follows. Fuel auxiliary building, 15 is set because criteria a) presence of significant
debris and core components are given 90 because of the criteria a) defects and c) insufficient layers of boundary are figured as unlikely with
generation of hazardous gases, b) dispersion due to physical degrada­ b) unsatisfaction of safety standards being likely. For covering structure,
tion, and c) lack of waste containers being figured as yes with d) lack of 8 is set because a) presence of significant defects and b) unsatisfaction of
monitoring being no. Piping & equipment is given 2 because of a) safety standards are figured as unlikely and d) excess of remaining
generation of hazardous gases, b) dispersion due to physical degrada­ building life is likely. For the other confining facilities, 2 is set because a)
tion, and c) lack of waste containers being figured as no. Building presence of significant defects, b) unsatisfaction of safety standards, d)
structures is given 17 because of b) dispersion due to physical degra­ excess of remaining building life, and e) loss of its boundary by failures
dation and c) lack of waste containers being figured as yes and a) gen­ of neighbouring facilities are figured as unlikely. The setting results of
eration of hazardous gases and d) lack of monitoring being no. FD are shown in Table 6.
By completing pre-treatment, WUD of both fuel debris and core
components decrease to 9 because of providing temporary containers. 3.3. SED scores
WUD of building structures decrease to 3 because of the same reason as
in the case of fuel debris and core components. By completing condi­ Based on the calculation of RHP and the setting of FD and WUD
tioning, WUD of fuel debris and core components decrease to 2 because described in Sections 3.1 and 3.2, n value is calculated to be 3.30. Fig. 1
of solidification or stabilization process. The setting results of WUD are shows SED scores of each object. SED scores of fuel debris and core
shown in Table 6. components have relatively high in as-it-is but hugely decrease in each
FD setting is done by assuming the confinability by the facility step of radioactive management. On the other hand, those of the other
containing radioactive materials. The setting is made by whether each two objects have relatively low in as-it-is, even lower than that of fuel
criterion is judged as likely, possible, or unlikely by referring to Table 2. debris in conditioning, and increase in pre-treatment. As for the effect of
The confinability of facilities is postulated as follows. PCV has been radioactive waste management, SED scores of fuel debris decreases by
damaged to have a possible leak of radioactive nuclides but the release 21 orders of magnitude (from 24 to 3) with the process from as-it-is to
of radionuclides from PCV could be to some extent contained in the conditioning, while those of building structure decrease by 2 orders of
reactor building. Reactor building and the auxiliary building do not magnitude (from 7 to 5) only. This is due to higher FF, lower CF, higher
meet safety standards as a storage facility for the objects to be removed FD, and higher WUD of fuel debris and core components.
from reactor building because part of reactor building is open due to Plant-base SED score is calculated by summing up SED scores of each
spent fuel retrieval operation and the auxiliary building has a object, considering two cases where different steps of radioactive waste
management are reached. Fig. 2 shows the case where each object after
Table 6
completing pre-treatment in the process of radioactive waste manage­
FD and WUD in different steps of radioactive waste management. ment. Plant-base SED score decreases by the order of 7 (from 24 to 17)
and its value remained whether the active decommissioning proceeds or
Objects Steps of radioactive waste Confining WUD FD
management facilities
not. This is because that fuel debris and core components own large SED
scores in as-it-is, and plant-base SED score could not be decreased by
Fuel debris As-it-is PCV 90 91
progress of active decommissioning, where piping& equipment and
Pre-treatment Auxiliary 9 15
building building structure contribute little to decreasing plant-base SED score.
Treatment Waste storage 3 2 Fig. 3 shows the case where each object after completing conditioning in
facility the process of radioactive waste management. Plant-base SED score
Conditioning Waste storage 2 2 further decreases by the order of 19 (from 24 to 5) with progress of
facility
Core As-it-is PCV 90 91
radioactive waste treatment and conditioning for fuel debris and core
components Pre-treatment Auxiliary 9 15 components.
building Comparison between the two cases indicates that core components
Treatment Waste storage 3 2 removal could reduce a relatively large amount of plant-base SED score
facility
under the conditions that treatment and conditioning of fuel debris are
Conditioning Waste storage 2 2
facility done. When stabilization of radioactive waste is realized by condition­
Piping & As-it-is Reactor building 2 15 ing, nearly 90% of achievable amount of reduction in plant-base SED
equipment Pre-treatment Auxiliary 2 15 score will take place during stage 1 and 2. It indicates that fuel debris
building and core components have inherent higher RHP than that of the other
Treatment Waste storage 2 2
facility
objects, which could be minimized if robust confinement of the con­
Conditioning Waste storage 2 2 tainers is provided after retrieval. Therefore, the priority may be given
facility fuel debris retrieval and core components removal as early as possible in
Building As-it-is Covering 17 8 the active decommissioning from the viewpoints of keeping plant-base
structure structure
SED score minimum.
Pre-treatment Covering 3 8
structure In addition, physical size of radioactive materials is expected to
Treatment Waste storage 3 2 change in the process of pre-treatment. Taking fuel debris as an example,
facility SED scores of fuel debris is calculated hypothesizing that all the fuel
Conditioning Waste storage 3 2 debris becomes discrete solids and powders (Fig. 4). It is shown that
facility
plant-base SED score in the case of powder form is four orders of

5
A. Asahara et al. Nuclear Engineering and Design 374 (2021) 111066

Fig. 1. SED scores of each object in different steps of radioactive waste management.

Fig. 2. SED scores of each object after completing pre-treatment in the process of radioactive waste management.

Fig. 3. SED scores of each object after completing conditioning in the process of radioactive waste management.

6
A. Asahara et al. Nuclear Engineering and Design 374 (2021) 111066

active decommissioning compared with the core components


removal. This is due to inherent large RHP of the fuel debris, which
could be minimized by robust confinement by the containers after
retrieval.
2) Since nearly 90% of achievable amount of reduction in plant-base
SED score could be realized by fuel debris retrieval and core com­
ponents removal without addressing piping & equipment and
building structure, the priority will be given the efforts to deal with
the fuel debris and core components as early as possible in the whole
decommissioning period.
3) Plant-base SED score will be hugely influenced by physical form of
fuel debris. It may be necessary to consider for developing work plan
from the viewpoints of cutting and containing methods.
Fig. 4. SED scores of fuel debris with different physical form after completing 4) These perspectives would be useful to construct active decom­
pre-treatment in the process of radioactive waste management. missioning strategies together with project management parameters
such as staffing, technical capability, and financial readiness.
magnitude higher than that of discrete solid. This means physical form
of fuel debris will hugely impact plant-base SED score. It may be CRediT authorship contribution statement
therefore necessary to consider work plan for fuel debris retrieval from
the viewpoints of cutting and containing methods. Akira Asahara: Conceptualization, Methodology, Writing - original
draft, Software, Investigation. Daisuke Kawasaki: Writing - review &
4. Conclusions editing. Satoshi Yanagihara: Writing - review & editing, Supervision.

The calculation of SED scores indicates the following suggestions for Declaration of Competing Interest
strategy construction.
The authors declare that they have no known competing financial
1) Treatment and conditioning of fuel debris retrieved make a large interests or personal relationships that could have appeared to influence
contribution for reducing plant-base SED score under proceeding the the work reported in this paper.

Appendix I

FF of each physical form

FF (Release fraction) Physical form

1 Gas
1 Liquid
1
10− Powder
1
10− Sludge
5
10− Discrete solid
6
10− Large monolithic, activated component

Appendix II

CF of each length of time that represents the frequency of human intervention

CF Length of time

1 Hours (0 – 24 h)
1
10− Days (24 – 168 h)
2
10− Weeks (168 – 720 h)
3
10− Months (720 – 8760 h)
4
10− Years (8,760 – 87,600 h)
5
10− Decades (87,600 h –)

References NDA, 2011. NDA Prioritisation – Calculation Of Safety And Environmental Detriment
Scores, EGPR02, Revision 6.
NDA, 2010. Instruction for the calculation of the Radiological Hazard Potential, EGPR02-
IAEA, 2017. Selection of Technical Solutions for the Management of Radioactive Waste.
WI01, Revision 3.
IAEA TECDOC 1817.
NDF, 2019. Technical Strategic Plan 2019 for Decommisioning of the Fukushima Daiichi
IRID, IAE, 2018. Upgrading of the Comprehensive Identification of Conditions inside
Nuclear Power Station of Tokyo Electric Power Company Holdings, Inc.
Reactor.
Nishihara, K., Iwamoto, H., Suyama, K., 2012. Estimation of fuel compositions in
Jarjies, A., Abbas, M., Fernandes, H.M., Wong, M., Coates, R., 2013. Prioritization
Fukushima-Daiichi Nuclear Power Plant. JAEA-Data/Code 2012–2018.
methodology for the decommissioning of nuclear facilities: a study case on the Iraq
Oak, H.D., Holter, G.M., W. E. Kennedy, J., Konzek, G.J., 1980. Technology, Safety and
former nuclear complex. J. Environ. Radioact. 119, 70–78. https://doi.org/10.1016/
Costs of Decommissioning a Reference Boiling Water Reactor Power Station,
j.jenvrad.2012.01.001.
NUREG/CR–0672-Vol.2.

7
A. Asahara et al. Nuclear Engineering and Design 374 (2021) 111066

Shibata, A., Koma, Y., Ohi, T., 2016. Estimation of the inventory of the radioactive The Inter-Ministerial Council for Contaminated Water and Decommissioning Issues,
wastes in Fukushima Daiichi NPS with a radionuclide transport model in the 2019. Mid-and-Long-Term Roadmap towards the Decommissioning of TEPCO’s
contaminated water. J. Nucl. Sci. Technol. 53, 1933–1942. https://doi.org/10.1080/ Fukushima Daiichi Nuclear Power Station.
00223131.2016.1196625. Utkin, S.S., Linge, I.I., 2019. Decommissioning strategy for liquid low-level radioactive
Sugiyama, D., Nakabayashi, R., Koma, Y., Takahatake, Y., Tsukamoto, M., 2019. waste surface storage water reservoir. J. Environ. Radioact. 196, 164–170. https://
Development of calculation methodology for estimation of radionuclide composition doi.org/10.1016/j.jenvrad.2016.11.011.
in wastes generated at Fukushima Daiichi nuclear power station. J. Nucl. Sci. Yamashita, T., Sato, I., Honda, T., Nozaki, K., Suzuki, H., Pellegrini, M., Sakai, T.,
Technol. 56, 881–890. https://doi.org/10.1080/00223131.2019.1595765. Mizokami, S., 2020. Comprehensive Analysis and Evaluation of Fukushima Daiichi
TEPCO, 2019. Solid Waste Storage Management Plan [in Japanese]. Nuclear Power Station Unit 2. Nucl. Technol. 1–21 https://doi.org/10.1080/
00295450.2019.1704581.

You might also like