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Journal of Power Sources: Kailong Liu, Kang Li, Cheng Zhang
Journal of Power Sources: Kailong Liu, Kang Li, Cheng Zhang
Journal of Power Sources: Kailong Liu, Kang Li, Cheng Zhang
h i g h l i g h t s
a r t i c l e i n f o a b s t r a c t
Article history: Battery temperature is a primary factor affecting the battery performance, and suitable battery tem-
Received 16 March 2016 perature control in particular internal temperature control can not only guarantee battery safety but also
Received in revised form improve its efficiency. This is however challenging as current controller designs for battery charging have
16 December 2016
no mechanisms to incorporate such information. This paper proposes a novel battery charging control
Accepted 12 February 2017
strategy which applies the constrained generalized predictive control (GPC) to charge a LiFePO4 battery
based on a newly developed coupled thermoelectric model. The control target primarily aims to maintain
the battery cell internal temperature within a desirable range while delivering fast charging. To achieve
Keywords:
LiFePO4 battery
this, the coupled thermoelectric model is firstly introduced to capture the battery behaviours in
Constrained generalized predictive control particular SOC and internal temperature which are not directly measurable in practice. Then a controlled
Coupled thermoelectric model auto-regressive integrated moving average (CARIMA) model whose parameters are identified by the
Battery internal temperature recursive least squares (RLS) algorithm is developed as an online self-tuning predictive model for a GPC
Battery charging process controller. Then the constrained generalized predictive controller is developed to control the charging
current. Experiment results confirm the effectiveness of the proposed control strategy. Further, the best
region of heat dissipation rate and proper internal temperature set-points are also investigated and
analysed.
© 2017 The Authors. Published by Elsevier B.V. This is an open access article under the CC BY license
(http://creativecommons.org/licenses/by/4.0/).
http://dx.doi.org/10.1016/j.jpowsour.2017.02.039
0378-7753/© 2017 The Authors. Published by Elsevier B.V. This is an open access article under the CC BY license (http://creativecommons.org/licenses/by/4.0/).
146 K. Liu et al. / Journal of Power Sources 347 (2017) 145e158
round trip efficiency, energy and power capability, cycle life, reli- charging currents for battery thermal management. Klein et al. [19]
ability and charge acceptance [3]. Both the surface temperature and used a nonlinear model predictive control (MPC) method to mini-
internal temperature may exceed permissible levels when batteries mize a battery charging time based on the complex electrochemical
charge or discharge at prevailing conditions or at high ambient model. Marcelo et al. [20] applied constrained MPC to generate
temperature, which is detrimental for battery operation safety and battery CCCV charge current profile to charge a Li-ion battery cell as
will dramatically decrease the battery performance. On the other fast as possible. In these papers, MPC strategy has been successfully
hand, if the battery temperature exceeds a certain minimum applied to BMS, but they mainly consider constraints on the
threshold, it starts to generate heat uncontrollably while in oper- charging current and voltage, as well as average shell temperature
ation [4]. The battery capacity will be lost irreversibly if charging of battery, the temperatures especially the internal temperature of
battery at low temperature due to poor charge transfer at the battery are not considered. This battery internal temperature con-
electrode/electrolyte interface [5]. Therefore, suitable battery trol is however crucial in many prevailing battery application
thermal management which monitors and controls the battery conditions. When batteries are charged with high current in order
temperature is indispensable in EV applications [6]. to reach the specified SOC as quickly as possible in high power
To date, the reasonable working temperature suitable for most applications, both the battery shell and internal temperature will
current Li-ion batteries is to charge between 0 and 45 C and increase noticeably. When the battery temperature exceeds the
discharge between -20 and 60 C based on the instruction manuals reliable operating range, battery performance will be severely
from most battery manufacturers. A number of effective ap- damaged and even lead to battery failures and safety problems.
proaches have been proposed to estimate, monitor and control the Further, there exists large difference between the battery surface
temperature and to guarantee Li-ion battery operation safety [3]. In and internal temperature during charging process (e.g., sometimes
terms of battery materials, novel electrolytes materials, and anode greater than 10 C in high power applications [21]). The battery
and cathode materials which can improve operation safety for Li- internal temperature usually increases to a critical temperature
ion batteries under high temperature circumstance have been point earlier than the battery surface temperature. Therefore, the
researched. Maleki et al. [7] researched high thermal Li-ion con- battery temperature especially the internal temperature has to be
ductivity cells based on negative electrode material with high taken into account when batteries are charged with high currents
thermal conductive property. Kise et al. [8] presented a novel in high power applications. In other word, the battery internal
electrode which can improve safety for Li-ion batteries at high temperature has to be controlled within certain range during the
temperatures. For battery packages, researches are mainly focused charging process.
on developing passive (i.e., using ambient environment) or active One approach to achieve this is through the implementation of
(i.e., an embedded source provides heating or cooling) systems to the generalized predictive control (GPC) assisted with a proper
control the battery temperature under different situations. Based battery model which can not only reflect the battery electric be-
on the medium used, these systems can be further grouped as haviours but also the surface and internal temperature. GPC is a
thermal management system using air [9], liquid [10], phase self-adapted control algorithm widely used in industrial applica-
change materials [11], and combination of these mediums [12]. tions [22]. According to ‘look-ahead’ strategy in GPC, the future
Furthermore, some researchers focus on the development of outputs can be predicted at each sampling instant effectively. More
electronical circuits and a temperature management function is importantly, GPC is able to calculate the suitable control increments
often embedded in the circuits. Park et al. [13] proposed a dynamic with the constraints imposed on both the inputs and the outputs.
thermal model for the Li-ion battery system using the finite- This implies that hard constraints such as voltage, current and
volume approach. The thermal model is a two-state lumped current increment limits which affect the battery performance can
model where the Joule heat is applied to calculate the heat gener- be incorporated into the battery thermal control strategy directly.
ation. A battery cooling system with the cooling fan was then On the other hand, many researchers have focused on devel-
developed under the battery charging and discharging processes. In oping various battery thermal-electrical models to estimate the
Ref. [14], the relationship between the Li-ion BMS and charging temperature distribution of battery. A. Samba et al. [23] proposed a
strategies with temperature was analysed, and it has been shown two dimensional thermal model to predict the cell temperature
that the battery temperature has a significant impact on the distribution over the surface of battery and the ANSYS FLUENT
charging strategy design. A Li-ion battery protection approach was software was used to solve the models. In Ref. [24], a thermal
then proposed based on the existing integrated circuit (IC) condi- swelling model was proposed to address the dependence of the
tions. Kim et al. in Ref. [15] analysed the effect of power re- equivalent coefficient of thermal expansion and also reflect the
quirements and temperature change on the electrical states of temperature distribution through the cell. Then the thermal
battery cells, and a battery thermal management architecture to swelling at a variety of C-rates can be predicted. L. Song et al. [25]
heat/cool battery cells timely and selectively was proposed to presented an electrochemical-thermal coupling model to investi-
improve the efficiency of the BMS. gate the thermal behaviour of the Li-ion battery. And the temper-
To design effective control strategies for battery management ature distributions inside battery during charging/discharging
has been another active research topic. Jiang et al. [16] proposed to process were simulated by the finite element approach. These
adjust the charging current acceptance with different battery state developed models have significantly improved the understanding
of charge (SOC) stages using a constant-polarization-based fuzzy- of the battery behaviours and temperature distributions during
control charging method to shorten the charging time. Liu et al. [17] charging and discharging processes, though most of them are
presented an optimal five-step charging strategy for Li-ion batteries generally too complex to be used in real-time control. In this paper,
based on consecutive orthogonal arrays. Hu et al. [18] developed a we aim to develop advanced control method for battery charging,
dual-objective optimal charging strategy for lithium nickel- with particular consideration of the battery internal temperature
manganese-cobalt oxide (LiNMC) and lithium iron phosphate for safety operation. Therefore, a proper and simplified battery
(LiFePO4) batteries which optimally trades off the conflict between thermoelectric model plays a vital role in designing a highly effi-
the energy loss and charging time. cient control strategy and should be adopted. Our previous work
It is clear that most control strategies adapt the charging current [26] has shown a successful development of a coupled battery
acceptance with battery SOC stages. However, little has been done thermoelectric model. With some improvements of this thermo-
so far to apply advanced control strategies that manipulate electric model and the proposed constrained GPC strategy, the
K. Liu et al. / Journal of Power Sources 347 (2017) 145e158 147
battery behaviours under a given internal temperature and SOC, LiFePO4 battery, in particular their temperature constraints are
which are often difficult to measure directly can now be estimated presented firstly, followed by the illustration of the improved bat-
and controlled, and real world constraints on the battery operation tery coupled thermoelectric model.
can all be incorporated.
In summary, for the proposed strategy, the constrained GPC is 2.1. Basics of LiFePO4 battery
first used to charge a battery from an initial SOC to a targeted state
as quickly as possible, while keeping the battery internal temper- LiFePO4 battery uses nano-scale phosphate cathode materials to
ature within an acceptable range during the charging process so as offer good electrochemical performance with low resistance.
to enhance the battery safety and to avoid damages caused by Particular characteristics of LiFePO4 battery are shown in Table 1.
overheating. Further, both battery electrical and thermal con- LiFePO4 is more tolerant to full charge condition and is less stressed
straints including SOC, voltage, current and temperature during than other Li-ion systems if being kept charging at high voltage.
operation are also incorporated into the control strategy. The main LiFePO4 battery is now widely used in electric vehicles to replace
contributions of this work are summarized as follows: (1) The the lead acid battery. Eqs. (1)e(2) describe the chemical reactions
proposed fast charging control strategy considers the battery in- occur during charging process. It should be noted that it is vital to
ternal temperature which is important for safe operation and control the LiFePO4 battery charging process as it directly impacts
control of electric vehicles, particularly in some high power appli- the battery safety and performance.
cations where the difference between surface temperature and
internal temperature can be quite large. (2) The improved battery Charge
LiFePO4 ! yLiþ þ ye þ Li1y FePo4 for positive electrode
thermoelectric model in the charging control strategy can guar-
antee both charging efficiency and control of internal temperature (1)
rising to prolong battery service life. (3) The CARIMA model
structure is optimized by a fast recursive algorithm (FRA). This Charge
xLiþ þ xe þ Li1x C6 ! LiC6 for negative electrode (2)
brings extra benefits in that the model complexity is optimized so
that the CARIMA model used in the GPC can be simplified with Conventional charging methods include current control, voltage
good performance and the computation time can be shortened in control and Mas Law control [27]. Current control uses a small
the implementation of the GPC controller. (4) The correlation be- current to charge battery to avoid sharp increase in both battery
tween battery cooling cost and charging time during the charging temperature and voltage. However, this method is difficult to
process is analysed to identify the most appropriate region of heat generate a suitable charging current rate for battery capacity
dissipation rates. (5) The effect of internal temperature set-points balancing and to further ensure operation safety. For voltage con-
on both charging time and energy loss is investigated to identify trol method, battery is charged at a constant voltage in order to
the proper internal temperature set-points. avoid overvoltage problem which may occur at the end of charging
The remainder of this paper is organized as follows. Section 2 process. The disadvantage of this method is that the current at the
first introduces relevant basics of Li-ion battery especially LiFePO4 beginning of charging process may be too high, which can harm the
battery, in particular their temperature constraints, then the battery life. The Mas Law method calculates the current to charge
improved coupled thermoelectric model is presented. Section 3 the battery by ‘Mas Three Laws’, but it is only designed for lead-acid
develops the constrained GPC algorithm, especially the predictive batteries, not for Li-ion batteries.
model identification and constraints formulation. Details to The constant-current-constant-voltage (CCCV) method in-
formulate the battery charging control objectives, coupled ther- tegrates current control and voltage control method to shorten
moelectric model identification, and battery charging control charging time as well as to improve charging performance and
strategy are presented in Section 4. Section 5 gives the experiment safety [28]. In this method, battery is first charged at a constant
results to demonstrate the efficacy of the proposed approach. The current and the voltage increases due to the charge current. When
most appropriate region of heat dissipation rates and battery in- the battery terminal voltage reaches the maximum safe value, the
ternal temperature set-point are also investigated and analysed. battery begins to be charged at a constant voltage until the battery
Finally, section 6 concludes the paper. capacity meets the goal requirement. Although CCCV is easy to
apply, it is often designed using the voltage limits and thus may not
take full advantage of the actual operating characteristics of bat-
2. Battery coupled thermoelectric model teries. Besides, both the shell and core temperature may exceed
acceptable ranges when the battery is charged in high power ap-
In this section, the relevant basics of Li-ion battery especially plications without any other solutions. It is therefore vital to
include the temperature information when battery is charged using
CCCV method for some high power cases.
Table 1
Characteristics of LiFePO4 battery [21].
2.2. Battery temperature constraints
LiFePO4 battery
Voltage (nominal) 3.20 Ve3.30 V The reasonable ambient temperature limits for various bat-
Charge (C-rate) Charge to 3.65 V (1C): typical 3 h charging time
Discharge (C-rate) 40A pulse; 2.50 V cut-off (lower than
teries during charging or discharging process are shown in
2 V may cause damage) Table 2 [27]. Compared with Lead acid and NiMH/NiCd battery,
Specific energy 90-120 Wh/kg Li-ion batteries have fairly desirable charging performance at
Thermal runaway 270 C (518 F) cooler temperatures within the range of 0e45 C (41e113 F).
Cycle life 1000-2000 (related to depth of discharge,
During the charging process, the battery internal resistance will
temperature)
Applications Stationary and portable needing high usually cause a slight temperature rise within the battery, and
endurance and load currents this temperature rise will be more significant in cold environ-
Comments Low capacity with very flat voltage ment due to the increase of the internal resistance. On the other
discharge curve. One of hand, the battery internal resistance can be reduced by elevating
the safest Li-ion batteries.
the battery temperature, thus increase the Li-ion battery
148 K. Liu et al. / Journal of Power Sources 347 (2017) 145e158
Table 2
Reasonable ambient temperature constraints for various batteries.
Li-ion 0 C to 45 C (32 F to 113 F) 20 C to 60 C (4 F to 140 F) Good charge/discharge performance at higher
temperature but may shorten battery life.
Not permitted for charging below freezing.
Lead acid 20 C to 50 C (4 F to 122 F) 20 C to 50 C (4 F to 122 F) Lower V-threshold by 3mV/oC when hot.
Charging at 0.3C or less below freezing.
NiMH, NiCd 0 C to 45 C (32 F to 113 F) 20 C to 65 C (4 F to 149 F) Charge acceptances at 45 C and 60 C are 70% and 45% respectively.
Charging at 0.1C between 18 C and 0 C.
Charging at 0.3C between 0 C and 5 C.
charging effectiveness slightly, but excessive high temperature V1 is the voltage of the RC network, which is also called the battery
will dramatically reduce the battery life. To achieve the best polarization voltage. Ro represents battery internal resistance.
performance, Li-ion batteries are recommended to be charged The battery SOC is calculated based on the battery nominal ca-
within a narrower ambient temperature range of 10 C and 30 C pacity shown as follows,
(50 F and 86 F).
Apart from the ambient temperature, the internal and surface Ts
socðkÞ ¼ socðk 1Þ *iðk 1Þ (4)
temperatures of Li-ion batteries also impact the battery behaviour Cn
during the charging process. In our previous study [26], it is clearly
shown that the battery internal and shell temperatures are where Cn is the battery nominal capacity which unit is As (3600
distinctively different from ambient temperature during the fast As ¼ 1 Ah) and Ts is the sampling time period which unit is second
charging process. The battery internal temperature is always higher respectively.
and the difference between the internal and shell temperatures can Suppose the terminal load current keeps constant during the
be even more dramatical, which has revealed the importance to sampling period, then, following the dynamics of a RC network, the
effectively control the battery internal temperature in order to battery polarization voltage V1 of RC network could be calculated
prevent Li-ion battery from overheating during the charging as,
process.
DT DT
V1 ðkÞ ¼ exp V1 ðk 1Þ R1 1 exp
R1 C1 R1 C1
2.3. Battery coupled thermoelectric model
iðk 1Þ ¼ a1 *V1 ðk 1Þ b1 *iðk 1Þ
In the battery charging process, some battery internal states (5)
such as SOC and internal temperature are difficult to measure
Combing Eqs. (3)e(5), the battery Thevenin model can be
directly, yet they play vital roles for battery online status control
expressed as follows:
and to ensure safe operation. In this paper, a newly developed
thermoelectric model is used to capture both the battery thermal 8
< socðkÞ ¼ scoðk 1Þ Ts =Cn *iðk 1Þ
and electric behaviours, including voltage, surface temperature,
V1 ðkÞ ¼ a1 *V1 ðk 1Þ b1 *iðk 1Þ (6)
and in particular SOC and internal temperature during battery :
VðkÞ ¼ V1 ðkÞ þ iðkÞ*Ro þ UOCV
charging. Then according to the comprehensive capture of the
battery behaviours using this thermoelectric model, the con-
where Ro and UOCV are dependent on internal temperature and SOC
strained GPC strategy enables simultaneous and efficient control to
respectively shown in Eqs. (7)e(8). Both of them can be obtained
guarantee both battery charging efficiency and internal tempera-
from a look-up table based on linear interpolation algorithm.
ture rising within reasonable ranges, further to prolong the battery
service life. Ro ¼ fR ðTin Þ (7)
where V is the battery terminal voltage and i is the battery current. Fig. 1. Battery Thevenin model.
K. Liu et al. / Journal of Power Sources 347 (2017) 145e158 149
where Ro is the battery internal resistance; Q1 considers the heat Generalized predictive control (GPC) belongs to a wide range
generation is mainly dominated by the ohmic heat generated over of MPC algorithms. It formulates the optimization process of a
internal resistance. Q2 considers the heat generation caused by the suitable cost function concerning the future output errors and
over-potentials and entropy change within battery. Here, i*ðv control actions. Compared with traditional control approach, GPC
UOCV Þ is known as the Ohmic or Joule's heating and offers some advantages such as capability of stabilizing non-
i*Tin *dUOCV =dTin is known as the heat generated or consumed due minimum phase and unstable open-loop processes, and
to the reversible entropy change that is a result of electrochemical handling unknown or variable dead-time and plants with un-
reactions. known orders. Over the years, the GPC strategy has proven to be
Assuming Tðk_ þ 1Þ ¼ z1*TðkÞ ¼ 1 *ðTðk þ 1Þ TðkÞ , the two- highly effective in many industrial applications where the per-
Ts Ts
formance and robustness are difficult to achieve with traditional
stage thermal model for the battery cells can then be formulated as designs. Besides, the hard constraints can be incorporated into
8 the controller directly and solved by a quadratic optimization
>
> k k Ts
>
< Tin ðkþ1Þ¼ 1Ts 1 *Tin ðkÞþTs * 1 *Tsh ðkÞþ *Q problem in GPC.
C1 C1 C1
>
>
> k k þk2 Ts 3.2. Predictive model identification
: Tsh ðkþ1Þ¼Ts * 1 *Tin ðkÞþ 1Ts 1 *Tsh ðkÞþk2 *Tamb *
C2 C1 C2
(12) When applying the constrained GPC strategy for the battery
charging process, the first task is to select a suitable predictive
As the ambient temperature decreases or battery shell tem-
model to represent the controlled dynamic process. In order to
perature rises, k2 will increase accordingly and more heat be
improve the robustness of GPC controller, an online self-tuning
dissipated into the ambience [32], i.e. k2 increases with the tem- predictive model is formulated using the controlled auto-
perature gradient Tsh Tamb . In order to take this effect into regressive integrated moving average (CARIMA) model shown as
consideration and further improve the accuracy of the thermal follows,
model, two cases are considered and compared: 1) constant k2 ; 2)
time-varying k2 : k2 ¼k2;1 þk2;2 *ðTsh Tamb Þ. 1
A z1 yðkÞ ¼ zd B z1 uðkÞ þ C z1 εðkÞ (14)
D
2.4. Battery coupled thermoelectric model where uðkÞ, yðkÞ and εðkÞ are m*1 input vector, n*1 output vector
and n*1 noise vector at sampling time k respectively. The noise in
The battery Thevenin model and the two-stage thermal model CARIMA model is supposed to be a zero mean white noise. d is the
are combined to produce the coupled thermoelectric model as delay factor and D ¼ 1 z1 is a difference operator. Bðz1 Þ is a
follows, n*m polynomial matrix, Aðz1 Þ and Cðz1 Þ are n*n polynomial
150 K. Liu et al. / Journal of Power Sources 347 (2017) 145e158
(1). The battery SOC must meet the EV application demand. 30A iðkÞ 0 A for 3C; (27)
(2). The terminal voltage must be operated within reliable and
safe operating range to avoid high voltage situation which 2:6 V VðkÞ 3:65 V (28)
will accelerate the capacity loss, resulting in internal short
circuits as well as decomposition of the electrolyte. Suppose the charging process starts from initial SOC of 0.1, and
(3). Both the temperatures of battery shell and core must be the targeted state is 0.9, that is
maintained within a desired level to ensure proper and safe
0:1 SOCðkÞ 0:9 (29)
charging, avoiding battery service life being shortened or
terminated and battery thermal runaway caused by over- The main control target is to find a suitable charging current
temperature. profile iðkÞ that could maintain the battery temperature within a
(4). The battery SOC should be charged from initial SOC state to a desired level while driving the SOC from initial state 0.1 to final
specified state as fast as possible under the above mentioned state 0.9 simultaneously. The hard constraints for voltage and
constraints. current should be also considered during the charging process.
According to the constrained GPC strategy, the optimal increment
sequence DiðkÞ of control inputs (charging current) are calculated at
each sampling time. This optimal increment sequence minimizes
the multistage cost function formulated in Eq. (21) within the area
limited by hard constraints on input current, output SOC and ter-
minal voltage simultaneously. Finally, the first value of the optimal
control increment is extracted and the step-wise control input iðkÞ
at each sampling time can be calculated as
Table 3
Battery OCV and SOC relationship.
SOC 0.900 0.798 0.695 0.593 0.491 0.389 0.287 0.186 0.085
OCV(V) 3.330 3.325 3.299 3.292 3.290 3.278 3.251 3.215 3.057
Fig. 2. Constrained GPC for battery charging.
152 K. Liu et al. / Journal of Power Sources 347 (2017) 145e158
Parameter Value
5. Experiments
a1 0.981
b1 1.8e4
The accuracy of the improved thermal sub-model is first vali-
C1 263.8
C2 31.2 dated through a practical battery self-heating test. Then simulation
k1 1.264 tests are conducted to investigate the performance of the con-
k2 0.33 strained predictive controller for battery charging proposed in
k2,1 0.268
section 4.3. In the simulation tests, the sampling time is Ts ¼ 1s, and
k2,2 0.0044
the CARIMA model is used as a predictor. The ambient temperature
is chosen as 27 C and the initial battery shell and interior tem-
peratures are both chosen as 29 C. Three simulation tests are
conducted, including (i) tracking performance test with different
iðkÞ ¼ iðk 1Þ þ DiðkÞ (30) GPC tuning parameters; (ii) test with different heat dissipation
rates; (iii) test with different internal temperature set-points. The
where DiðkÞ ¼ ½1; 0; /; 0½Dik Dikþ1 /DikþNc 1 T . tests are further analysed to identify the most appropriate of the
The constrained GPC strategy for battery control is implemented heat dissipation rates and proper internal temperature set-points
through the following steps at each sampling time: for the designed charging control strategy.
Step 1: Acquire the outputs of electric and thermal behaviours When using CARIMA model as the predictive model in the GPC
based on the thermoelectric model and estimate the parameters of controller, a complex model with a large number of model terms
the CARIMA model using the RLS with forgetting factor. will increase the model complexity and computation time. On the
Step 2: Calculate the j-step predictions based on the online other hand, an oversimplified model suffers from low performance
identified CARIMA model. in terms of both generalization performance and accuracy thus it is
Fig. 3. Battery self-heating test and validation results for battery thermal model.
K. Liu et al. / Journal of Power Sources 347 (2017) 145e158 153
is not measured at the ‘cell core area’, which usually refers to with constant k2 and 2) Q2 with time-varying k2 are conducted to
the core of each individual cell. However, since embedding validate the battery thermal model. The model validation results
micro-temperature sensors within the cell needs additional are then compared.
manufacturing challenges and instrumentation requirements, and The validation results for the thermal models are given in Fig. 3
will further increase cost and complexity significantly [21], so this (c) for Q1 with constant k2 and Fig. 3 (d) for Q2 with a time-varying
measurement approach is also a good indicator of the battery in- k2 , respectively. The validation results are summarized in Table 6.
ternal temperature without advanced micro-temperature sensors. According to Table 6, it is clear that the thermal model accuracy is
The load current and voltage are shown in Fig. 3(a) and the heat improved noticeably when Q2 is used for the calculation of the heat
generation results using two different calculation approaches in Eq. generation while the thermal dissipation rate k2 takes the time-
(11) are compared in Fig. 3(b) respectively. The dUOCV =dTin values varying form. Therefore, Q2 and time-varying k2 are adopted in
given in [34] is applied here. It is clear that Q1 which only considers the battery thermal model.
Joule heat generated by the internal resistance, is smaller than Q2
which considers the heat generation caused by the over-potentials 5.2. Tracking performance test with different control parameters
and entropy change within the battery. To further explore the ef-
fects of these two different heat calculation approaches as well as Parameters in the constrained GPC controller, including pre-
the effect of the two forms of thermal dissipation rate k2 on the diction horizon NP and penalty weight R have huge impacts on the
battery thermal model accuracy, two case studies, including 1) Q1 performance of the proposed battery charging control strategy. In
K. Liu et al. / Journal of Power Sources 347 (2017) 145e158 155
order to test the effects of various parameters on control results and temperature. The surface temperature is also be maintained around
to achieve high efficiency control, NP and R were varied while the 37.5 C. Since the battery surface temperature always reaches to a
control horizon and positive penalty weight for the output are fixed critical temperature more slowly than the internal temperature in
at NC ¼ 2 and Q ¼ 1 respectively in this test. The maximum the charging process, it is sufficient to control the internal tem-
charging current rate is chosen as 3C and the set-points of the perature alone for battery charging thermal management.
battery internal temperature are fixed at 40 C. The tests demonstrated that the control response speed is
The system responses with varying prediction horizon NP are reduced for larger prediction horizon NP . When NP is increased
shown in Fig. 4. These responses include the charge current as the from 15 to 120, the charging profile become less steep and the
control input and the corresponding controlled output variables charge current increment is smaller, and the output values are less
(terminal voltage, internal temperature, shell temperature, SOC). It fluctuated. But the larger NP will require more computing time for
is shown that with the battery internal temperature control, the the GPC controller to calculate the corresponding incurrent in-
total battery charging time to bring SOC from 0.1 to the final tar- crements. To balance the computing time and the fluctuations of
geted state 0.9 has increased to nearly 1500s compared with the the output values, we finally chose NP ¼ 60.
CCCV profile in 1309 s due to the different charging current rate. Fig. 5 illustrates the influence of the penalty weight R choices on
The internal temperature is however maintained around 40 C. This the control increment. Here the control horizon and the prediction
allows the avoidance of the continuous rise of battery internal horizon are fixed at NC ¼ 2 and NP ¼ 60 respectively, only the
156 K. Liu et al. / Journal of Power Sources 347 (2017) 145e158
where Tð:Þ stands for the response charging time with corre-
sponding k2 . Then the change rate of charging time RT can be
defined as,
.
RT ki2 ¼ DT ki2 T ki1
2 (32)
Fig. 7. Relations of charging time with dissipation rates.(a) Charging time (b) Change
rate of charging time. From Fig. 7, the following observations can be reached.
Observation 1: According to Fig. 7(a), it can be observed that for
a fixed set-point Tin , as the dissipation rate k2 increases, the
penalty weight R on the control increment for battery charging response charging time decreases. However, this correlation is
process is varied. The primary role for weight R is to avoid control nonlinear. At a certain point, further increase of the value of k2 will
value change sharply. Reducing the value of R can speed up the have much less effect on reducing the charging time. This result
response for the battery internal temperature. When the control reveals that there exists a best trade-off between the dissipation
weight R is increased from 0.05 to 1, the charging current changed rate k2 and the corresponding charging time.
slowly, leading to a slightly slow response for all output values, Observation 2: In order to find out the most appropriate region
while the charging time with larger control weight R is slightly for k2, the correlation of the change rate of the charging time is
longer, up to 1512s when control weight is chosen as R ¼ 1. It further explored and shown in Fig. 7(b). It is found that the change
should be noted that when the control weight R is decreased below rate is larger than 4% when k2 is less than 0.3. After this value of 0.3,
0.05, the responses for battery charging process are almost the the change rate becomes smaller than 4% which means further
same, further decreasing it will not make any notable difference to increase k2 has insignificant impact on further reducing the
the battery charging performance, therefore R ¼ 0:05 is taken as charging time. Suppose the relation between dissipation rate k2
the lower limit. and the manufacturing cost is linear, the results from Fig. 7(b) can
confirm that improper setting of the dissipation rate will only in-
5.3. Heat dissipation rate test crease the manufacturing cost without any noticeable benefit on
reducing the charging time. The dissipation rate k2 between 0.1 and
The thermal dissipation rate k2 in Eq. (12) stands for the heat 0.3 would be the most appropriate region if we consider 4% as the
conduction between the battery shell and the ambience which can acceptable change rate of the charging time.
be increased by active thermal management including air fan or
liquid cooling system. k2 is a compromise between the cooling cost 5.4. Test of different internal temperature set-points
and the dissipation efficiency (larger k2 usually implies higher
cost). In order to inspect the influence of different dissipation rates Another test is conducted to examine the influence of various
on the performance of the charging control strategy and further to internal temperature set-points on the battery charging process
find out the most appropriate region of k2 for battery charging, the and the results are shown in Fig. 8. Then a cost function considering
k2 is varied while control parameters in GPC being fixed both the charging time and the energy loss is presented to find out
ðNc ¼ 2; NP ¼ 60; R ¼ 0:05Þ in this test. The internal temperature the proper internal temperature target. In this test, five different
set-points are chosen as 40 C. The responses of output variables battery internal temperature set-points (36 C, 37 C, 38 C, 39 C,
and the variation of charge current are shown in Fig. 6. It is evident 40 C) are chosen. All of the five charging profiles show that the
that as k2 decreases from 0.4 to 0.1, both the battery internal and charging time are longer than the CCCV method as the charge
surface temperatures increase more rapidly, and the charging time currents have been changed to keep battery internal temperature
to bring SOC from 0.1 to the 0.9 become noticeably longer. This is within the desirable level. At the beginning of the charging process,
mainly due to the reduced k2 which implies less thermal convec- all charge currents are quite similar with the current profile using
tion occurring between the battery surface and the surrounding CCCV method as an effect to increase the SOC as quickly as possible.
ambient circumstance. The charge current therefore had to be These same charge current profiles will last until the battery in-
smaller in order to maintain internal temperature at a desirable ternal temperatures increase to the targeted temperature. There are
level. It is clear that the thermal dissipation rate has a significant then apparent differences in the charge current for different
K. Liu et al. / Journal of Power Sources 347 (2017) 145e158 157
internal temperature targets. When the internal temperature target battery charging time and energy loss especially in high power
is reduced from 40 C to 36 C, the charging time for different set- applications.
points is 1498s (40 C), 1579s (39 C), 1674s (38 C), 1786s (37 C) Given this consideration, we can use a cost function to evaluate
and 1918s (36 C) respectively. Low targeted internal temperature the performance during battery charging which combines both
prolongs the battery charging time. Internal temperature target is a battery charging time and energy loss
compromise between the battery charging time and energy loss
(larger internal temperature target usually means less charging Z
t¼tf
time but higher energy loss). It is therefore vital to select a proper J ¼ ð1 a1 Þ*tf þ a1 * iðtÞ*ðVðtÞ UOCV ðtÞÞ
internal temperature target in charging process to balance the
t¼0
þ iðtÞ*Tin ðtÞ*dUOCV ðtÞ=dTin ðtÞdt (33)
Table 7
Battery cost function J and its terms under different trajectories Tin . where tf stands for the time when battery reaches its final SOC
T in (oC) 40. 39 38 37 36. level. 0 a1 1 is the weighting factor to balance the two objec-
J 2952.46 2939.03 2933.73 2931.37 2933.81 tive terms (charging time and energy loss).
tf ] 1498.21 1579.73 1674.48 1786.28 1906.36
In the experiment, we use a fixed value a1 ¼ 0:25 , and the cost
Heat[w] 7315.21 7016.75 6711.48 6366.64 6016.16
functions for five charging profiles with different battery internal
158 K. Liu et al. / Journal of Power Sources 347 (2017) 145e158
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