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MSMA Voltage Paper
MSMA Voltage Paper
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Dynamic Magnetic Shape Memory Alloys Responses: Eddy Current Effect and
Joule Heating
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ABSTRACT
1 Introduction
MSMAs are best known for their unique ability to produce Magnetic Field
Induced Strains (MFIS) up to 10% under a magnetic field [1–4]. Some of the
commonly used MSMA material systems are NiMnGa [5–10], FePd [11–15]
∗
Corresponding author. Email: krishnendu@aero.iitb.ac.in
1
and NiMnX, where X = In, Sn, Sb [16–18].Among them, NiMnGa alloys are
widely investigated and will be the main focus of this study. Martensitic
transformations in Ni2 MnGa alloys were first reported by Webster et al. [19].
Zasimchuk et al. [20] and Martynov and Kokorin [21] performed detailed
studies on the crystal structure of martensite in the Ni2 MnGa alloys. Ullakko
et al. [22, 23] are credited with first suggesting the possibility of a magnetic
field-controlled shape memory effect in these materials. The unique magneto-
mechanical coupling makes MSMAs promising materials for multifunctional
structures, actuator and sensor applications [24–28].
The coupled MSMA behaviors can be modeled by considering the mate-
rial as an electromagnetic continuum. Extensive work on different electro-
magnetic formulations had been proposed in the literature [29–33] based on
different notion of breaking up long range and short range forces. A contin-
uum theory for deformable ferromagnetic materials and nonlinear magneto-
elasticity for magneto sensitive elastomers are discussed in [34–37]. On the
other hand, a study of electrostatic forces on large deformations of polariz-
able materials is discussed in[38, 39]. A theory for the equilibrium response of
magneto-elastic membranes is formulated by [40, 41] and a continuum theory
for the evolution of magnetization and temperature in a rigid magnetic body
for ferro/paramagnetic transition could be found in [42]. The variational
formulations for general magneto-mechanical materials have been proposed
by many authors [43–47].
The macroscopically observable MFIS in MSMAs is caused by the mi-
crostructural reorientation of martensitic variants [2, 48], field induced phase
transformation [17, 49–52] or a combination of the two mechanisms. In this
work, we will focus on variant reorientation. In the variant reorientation
mechanism, the variants have different preferred directions of magnetization
and the magnetic field is applied to select certain variants among others,
which results in the macroscopic shape change.
There are two major modeling approaches for variant reorientation mech-
anism. In microstructural based models, the resulting macroscopic strain
and magnetization response are predicted by minimizing a free energy func-
tional. Details on the microstructural based modeling approach can be found
in [1, 11, 53–56]. The second approach to study the material behavior is
through thermodynamics based phenomenological modeling [57–61]. Most
recent model development of variant reorientation in MSMAs and magneto-
mechanical loading analysis is reported in [62–64]. Moreover, a detailed
anisotropic consideration due to single crystal discrete symmetry is recently
presented in [65, 66]. A brief modeling approach for bulk polycrystalline ma-
terials is also mentioned in [65]. In this study, we systematically consider the
time dependent Maxwell equations and the rate forms of the mechanical and
2
magnetization constitutive equations that include single crystal anisotropy
[66].
Voltage generation (∼ 100 [V]) in MSMA due to mechanical impulse (∼
1.4 [m/s]) inside a biased magnetic induction (∼ 1.5 [T]) is reported in [67].
A similar study of stress induced variant reorientation under a fixed biased
magnetic field (1.6 [T]) is discussed in [28]. They found maximum voltage of
280 [mV] with the strain range of 4.9% at 10 [Hz]. Other relevant studies re-
garding voltage generation of MSMAs as sensors are reported in [68, 69]. Best
of our knowledge, effect of eddy current and corresponding Joule heating are
not so far reported for high-frequency actuation condition. Our main contri-
butions in this article are to predict the above mentioned quantities, based
on experimentally verified quasistatic constitutive equations, and to analyze
other field variable responses under dynamic conditions. We also compare
eddy current and Joule heating due to MSMA actuation with the 430-steel
(rigid ferromagnet) and Terfenol-D (magnetostrictive) material responses.
m = b/µ0 − h, d = ε0 e. (1)
3
remaining electromagnetic variables {e
j f , h,
e e f} are written as
b, m
jf = jf ,
e b = b − c−2 (ẋ × e) ≈ b,
e m
f = m, e = h − ẋ × d
h
with respect to the rest frame variables {j f , h, b, m}, where j f is the free
current. The moving frame fields ej f and m
f are decoupled with the velocity
ẋ as there are no free charge qf and electrical polarization p, respectively.
The local form of the Maxwell equations are:
∗ ∗
∇x · d = 0, ∇x · b = 0, ∇x × h
e=e
j f + d, ∇x × e
e = −b, (2)
∗
where, for a general vector α, convective time derivative is denoted by α =
α̇ − Lα + α tr (L) with α̇ as total time derivative. In a moving frame Ohms
law is given by e j f = Ωee = j f , where Ω is the conductivity tensor and
positive definite. We further write
∗
∇x × e
e = −b ⇒ ∇x × e = −∂t b,
∗
∇x × h
e=e j f + d ⇒ Ω−1 ∇x × h = e
e + 0 Ω−1 ∂t e ⇒ ∇x × h = Ωe
e.
Note that 0 ∼ 10−12 and for a conductor |Ω| ∼ 107 . This means the product
0 Ω−1 ∼ 10−19 and thus negligible.
The conservation laws of mass, linear momentum, angular momentum
and energy are:
4
2.1 Thermodynamic framework and constitutive equa-
tions
The constitutive responses with respect to a potential ψ(F , b, s, {ζ}), where
s is the entropy and the set {ζ} represents the collection of internal state
variables, are obtained through Coleman and Noll procedure [70],
0
σ L = ρ∂F ψF T , µ0 m = −ρ∂b ψ, s = −∂T ψ, −∂ζi ψ · ζ˙i > 0. (8)
5
is around 1.5 [T]. In MSMA, however, the magnetic domain wall motion
appears to be associated with a a minimal amount of dissipation. More
detail could be found in [7, 72].
We denote the reorientation strain tensor by E r and internal magneti-
zation vector due to reorientation by M r . ξ denotes the volume fraction of
the reoriented field-favored martensitic variant (variant-2) and the scalar g
is an internal state variable associated with the interaction (mixing) energy
during reorientation [65]. We assume that the reorientation strain rate Ė r ,
the rate of internal magnetization vector Ṁ r and the rate of mixing energy
g obey the following flow rules
˙
Ė r = Λr ξ, ˙
Ṁ r = γ r ξ, ˙
ġ = f r ξ. (10)
The tensors Λr describes the direction and magnitude of the strain generated
during variant reorientation, γ r takes into account the direction and magni-
tude of the internal magnetization due to reorientation respectively and f r
is the hardening function. Expanding the entropy inequality (9d), we get
π Er : Ė r + π M r · Ṁ r + πξ ξ˙ + πg ġ ≥ 0. (11)
π Er : Λr ξ˙ + π M r · γ r ξ˙ + πξ ξ˙ + πg f r ξ˙ ≥ 0, ⇒ π r ξ˙ ≥ 0,
π r = π E r : Λ r + π M r · γ r + πξ + πg f r . (12)
π r − Y r , ξ˙ > 0
(
r r
Φ := , Φ ≤ 0, (13)
−π − Y , ξ˙ < 0
r r
6
reorientation process follows the principle of maximum dissipation and can
be expressed in terms of the Kuhn Tucker type conditions [75]
Φ ξ˙ = 0 .
r r
Φ ≤ 0, (14)
The martensitic phase of Ni2 MnGa has 10M structure with I4/mmm
space group [76]. The classical point group is 4/mmm (D4h ). The discrete
symmetry restrictions for a specific Gibbs free energy potential, constitutive
equations and evolution equations are elaborately discussed in [65, 66]. The
incremental constitutive equations for single crystal anisotropy can be written
in the following forms:
˙ = [L]bEc
bSc ˙ + [K]Ḣ, (15)
˙ + [K0 ]Ḣ.
Ṁ = [L0 ]bEc (16)
Here [L]6×6 is a mechanical tangent stiffness matrix, [K]6×3 and [L0 ]3×6 are
magneto-mechanical stiffness matrices, and [K0 ]3×3 is a magnetic stiffness
matrix. In a general way, half-vectorization of a n × n symmetric matrix A
is denoted by
vech(A) = [A11 , ..., An1 , A22 , ..., An2 , ..., A(n−1)(n−1) , A(n−1)n , Ann ]T
∇·b = 0, ∇ · d = 0, ∇ × h = Ωe e (17)
∇×e = −∂t b, ∇ · σ = ρv̇, skw (σ) = 0 (18)
σ̇ = [L](ε̇) + [K]ḣ (19)
ṁ = [L0 ](ε̇) + [K0 ]ḣ. (20)
7
where, modified Maxwell stress σ h takes the following form
0 µ0
σ h = σ M − µ0 h ⊗ m − (m · m)I
2 i h
h µ0 0 i
= µ0 h ⊗ h − (h · h)I + 0 e ⊗ e − (e · e)I .
2 2
The rate form of the MSMA constitutive relations ((19),(20)) and the com-
ponents of [L], [K], [L0 ] and [K0 ] can be found in [65, 66]. In 2-D
1 ν 0 max
0 −1
E , [K] = E∆Mε
[L] = 2
ν 1 0 + µ0 hy 0 1 ,(21)
1−ν 1 r(1 + ν)
0 0 2 (1 + ν) 0 0
0 0 0 0 0 0 a1 ∆M/r
[L ] = , [K ] = . (22)
0 0 0 0 −b1 ∆M/r
The material parameters a1 = µ0 MxC , b1 = µ0 ∆M = µ0 (M sat − MyC ), where
MxC is the x-component of the magnetization response at forward reorien-
tation start and ∆M = (M sat − MyC ) + µ0 hy is the difference between the
saturation magnetization and the y-component of the magnetization at for-
ward reorientation start . The parameter r = ∂Φ ∂ξ
, is an explicit function
of the internal variable ξ, which depends on the magnetic field hy . The
functional form r(ξ(hy )) depends on the selection of the hardening function.
Thermodynamic force calculation and selection of hardening function are
briefly presented in Appendix A.
8
Figure 1: Schematic representation of the geometry and assumptions on the
field variables. Infinitely extended y and z planes are considered to avoid
electromagnetic edge effects.
The reduced 1-D constitutive equations become (from (19) and (20)):
(a) (b)
Figure 2: Predictions of (a) magnetization and (b) strain responses for variant
reorientation mechanism (after experimental data correction [77]) with an
incremental method.
9
∆Mεmax
0 = ε̇xx + µ0 ḣy , (24)
r
[∆M ][∆M]
ḃy = µ0 1 − µ0 ḣy . (25)
r
We assume that total stress (component σxx ) inside the specimen is con-
stant and is maintained at σ ∗ = −2 MPa to trigger field induced variant
reorientation and so σ̇xx = 0. Equation (24) reads
εmax ∆M εmax ∆M
Z
ε̇xx = ∂x v = −µ0 ḣy , ⇒ εxx = − µ0 dhy (26)
r r
and from (25) we write
Z
[∆M ][∆M]
by = µ 0 1 − µ 0 dhy . (27)
r
We present the quasistatic responses for magnetization and strain, obtained
in an incremental way, in Fig. 2. Comparisons of predicted responses with
experimental data and data corrections due to demagnetization effect are
discussed in [77].
∂x ez = ∂t by [V /m2 ], (29)
∂x hy = Ωeez [A/m2 ]. (30)
Units: It is always helpful to keep track of the units. We have 0 = 8.85 · 10−12 F/m,
1
µ0 = 4π · 10−7 N/A2 and c = 3 · 108 m/s. Note that F=A.s/V and Volt can further be
written as V =N.m/A.s. Electric field e is V/m and magnetic induction b is T=N/A.m.
Magnetization m and magnetic field h have unit A/m. The unit for current density j is
A/m2 . The conductivity Ω is S/m, where Simens S=A/V.
10
Denoting
β1 = c1 /µ0 [A/m.s],
∆Mεmax
β2 = −µ0 [m/A],
r
[∆M ][∆M]
µr = µ0 1 − µ0 [N/A2 ],
r
we solve for ez with a given ∂t by (equation (25)) from the following equation
∂x ez = ∂t by = µr ∂t hy , (31)
∂x v = β2 ∂t hy . (32)
Knowing the velocity we then compute eez = ez + vby , from which we find ĥy
from (30)
∂x ĥy = Ωe
ez . (33)
We solve all the above equations numerically in a staggered way, and the
outline is presented in Tab. 2. Material constants are given in Table. 1. The
µ0 HsM2 = 0.6 [T], µ0 HfM2 = 0.9 [T], µ0 HsM1 = 0.75 [T], µ0 HfM1 = 0.17 [T]
M sat =742 [kA/m], K =0.5 [T]−1 , H C = HsM2 , εmax = 5.65%, E=2.0 [GPa]
Table 1: Used material constants in the analysis. The values of the magnetic
parameters can be found in [66, 77]. The value for conductivity is taken from
[78, 79].
11
1. Given external applied magnetic field h0y = c1 t + c2 .
(1,n) (1,n) (1,n)
2. Initialize v (1,n) = 0, ez = 0, ĥy = 0, ∆ĥy = 0.
We consider a constant rate c(t) = c1 for which the values of c1 and c2 are the
12
same as given in (23). We present two cases where two different lengths are
considered without altering the frequency (25 Hz, equivalent to ts−f =0.02 s)
(a) (b)
In this case, the length of the bar is considered 25 mm and the frequency is
25Hz. The plot for the field induced volume fraction is presented in Fig. 3(a).
The distribution along the length almost remains uniform for the entire time
period. Note that, along the length, each material point has an electric field,
which creates an induced magnetic field ĥy . The induced magnetic field thus
nucleates more field induced variants and an increase in volume fraction is
observed along the length. The velocity distribution along the time axis is
increasing-decreasing by nature Fig. 3(b). This means, the velocity increases
initially with the rate of nucleation of the new field induced variant and then
gradually slows down at the end. Induced magnetic field due to the motion
is presented in Fig. 4(a) and the Maxwell stress is given in Fig. 4(b). Both of
them are significant. The maximum Maxwell stress turns out to be around
0.4 [MPa], 20% of the -2 [MPa] blocking stress. The eddy current density
along the transverse direction is shown in Fig. 5(a). The predicted current
density is large. The current flows along the width of the bar and the body
is heated up due to the resistance. The Joule heating is given in Fig. 5(b)
and is significant too. A comparison with the standard steel will be provided
as the work progress (see Table. 3). This means the increased temperature
13
(a) (b)
Figure 4: (a) Induced magnetic field due to induced electric field and (b)
Maxwell stress in the x-direction.
(a) (b)
Figure 5: (a) Eddy current density and (b) corresponding Joule heating.
14
(a) (b)
to the increase in length (Fig. 6a). The distribution indicates that complete
reorientation (ξ = 1) takes place almost everywhere after half of the length.
Once the complete reorientation takes place, actuation stops and a sharp
instantaneous drop in velocity to zero is observed (Fig. 6b).
(a) (b)
Figure 7: (a) Induced magnetic field due to induced electric field and (b)
Maxwell stress in the x-direction.
The induced magnetic field becomes high, and it reaches its maximum
value around 0.8 [T] (Fig. 7a). Maxwell stress is given in Fig. 7(b). The eddy
15
current density (Fig. 8b) increases almost twice by increasing the length four
times. The Joule heating also increases than the previous case (Fig. 8b).
(a) (b)
Figure 8: (a) Eddy current density and (b) corresponding Joule heating.
One should notice that a sawtooth is created around x=65 mm for both
current and power responses. This is due to the fact that the velocity becomes
zero after this point and so the motional emf drops. This is mainly the part
Ωvx by that disappears due to zero velocity. However, the presence of applied
field rate contributes in the increasing of jf in spite of zero velocity. The
same argument holds true for the power P .
Note that for ĥy , no sharp drop is observed. As ∂∂xĥy
= Ω(ez + vx by ), it
turns out that the contribution from Ωvx by is very small (in the order of
10−2 ) compared to the static part Ωez .
16
(a) (b)
Figure 9: (a) Volume fraction of the field induced martensitic variant and
(b) velocity distribution due to actuation.
and from the known values of the right hand side, we calculate total stress
distributions at 25 Hz and 500 Hz for L=25 mm (Fig. 10). Note that at
(a) (b)
Figure 10: Total stress distribution due to the frequency (a) 25 Hz and (b)
500 Hz for L = 25 mm.
500 Hz, the maximum stress level (0.6 MPa) is nearly 30% of the assumed
biasing stress (2 M P a). However, at low frequency this approximation holds
good (Fig. 10a).
We perform some parametric studies by varying length up to 100 mm
17
and frequency up to 0.5 KHz. The variation of the maximum stress response
is presented in Fig. 11(a). The white dotted line represents the limit below
which the stress level is less than 5% with respect to the blocking stress.
Considering this range as an admissible domain of L and f , we project this
line on the maximum velocity plot (Fig. 11b), eddy current and Joule heating
plots (Fig. 12).
(a) (b)
Figure 11: (a) Variation of maximum total stress and (b) maximum velocity
at different lengths and frequencies. The dotted lines are the threshold above
which the data start to accumulate spurious values due to constant stress
assumption and lack of satisfying conservation of linear momentum.
It is evident from the above study that we need to consider full coupling of
the conservation of linear momentum equation, coupled magneto-mechanical
constitutive equations and Maxwell equations for accurate predictions in a
wide range of length-frequency combinations. At smaller time scale inertia
will undoubtedly play a crucial role in generating stress waves. Since the
MFIS strongly depends on the stress intensity, a highly nonuniform strain
field may be produced. A proper wave propagation study is required to
conclude about the inertia effect, which is not investigated in this study.
However, the presented analysis gives feasible results only at a specific zone
of interest, as mentioned inFig. 11.
Finally, we present some quantitative data for mechanical waves, elec-
tromagnetic waves and skin depth for MSMA conductors, operating under
fluctuating field. The propagation speed of longitudinal
q mechanical waves
along an elastic MSMA rod (1-D) is given by vm = Eρ = 407.23 m/s. On
the other hand, if we assume linear magnetic MSMA material for which
18
(a) (b)
Figure 12: (a) Maximum eddy current density and (b) Joule heating at
different lengths and frequencies.
µ = max {µr (hy )} ≈ 3.5µ0 , then the plane wave propagation speed is given
by
r sr
ω 0 µr Ω 2
ue = , where κ=ω 1+( ) + 1.
κ 2 0 ω
The values at 1 MHz and 1 kHz frequencies are 1.13 · 103 m/s and 35.88 m/s,
respectively. The skin depth, δ = 1/κ, increases from 0.18 mm to 5.7 mm due
to the decrease in frequency. Further decreasing the frequency, e.g. at 100
Hz, ue = 11.34 m/s and δ = 18.1 mm.
19
electrical conductivity (Ω = 1.66 · 106 [S/m]) of Terfenol-D [82] with the 430
steel suggests that both of them will behave almost same in the considered
range of the magnetic field (0.6-0.9 [T]) .
jz [A/mm2 ]
2.5
6
jz [A/mm2 ]
2
4
1.5
1 2
0.5 0
100
0
100 50 1
×10-3
50 0.01 x [mm] 0
2
t [s]
x [mm] 0 0.02 t [s]
(a) (b)
Figure 13: Induced eddy current at (a) 25 [Hz] and (b) 200 [Hz] for a con-
sidered length of 100 [mm].
M2 √
Hf /µ0 tf Ω(HfM2 − HsM2 ) πγ
Z Z
A dt
µ0 dh(0, t) = √ √ =⇒ A = √ . (38)
Hs
M2
/µ0 Ω πγ 0 t 2 tf
20
The plots are given in Fig. 13 for the eddy current at two different finish
time tf = 0.02 [s] and tf = 2.5 · 10−3 [s], which correspond to 25 [Hz] and 200
[Hz], respectively. At low frequency, saturation of eddy current reaches at
the end of the length. However, saturation reaches much earlier for the high
frequency. A similar trend is also observed for the Joule heating. Maximum
values of the eddy current and the Joule heating and a comparison with the
MSMA responses are given in Table 3.
Comparing the responses in Fig. 13(a) and Fig. 8(a), we observe that
eddy current generation in MSMA is higher than the conventional ferro-
magnetic/magnetostrictive materials (see also Table 3). Presence of rate of
change of magnetization and velocity of the material points during variant
reorientation make MSMA responses significant different. However, for a
non-MSMA materials, responses relax quickly with the evolution of time.
Power loss also follows the similar trend as of the eddy current.
Before conclusion, let us have a quick estimation of temperature change
due to the Joule heating by solving a 1-D steady-state heat equation. Con-
sider Fig. 1 and assume that the surface x = 0 is insulated. The temperature
is uniform, and the system is below the martensitic finish temperature Mf . If
g0 is the energy generation and is assumed to be homogeneous for simplicity,
then the heat conduction equation is written as
1
∂xx T + g0 = 0 (39)
k
where k is the thermal conductivity. Thermal analysis with ambient heat
convection could be found in [83]. Let us assume the temperature at x = L
is maintained at Mf and the other boundary condition is ∂x T = 0 at x = 0.
g0 2
The temperature distribution is then given by T (x) = − 2k [x − L2 ] + Mf ,
where L is the length of the slab. From Table. 3, let us consider the case
L = 25 [mm] and 200 [Hz] for which g0 = P max = 19.12 [mW/mm3 ]. The
21
thermal conductivity of Nickel based alloy is nearly equal to that of Nickel,
i.e., k = 91 W/m·K. For the given thermal conductivity, energy generation,
and geometry the temperature at the adiabatic surface becomes T (0) =
98◦ C and quadratically decreases to T (L) = Mf = 32◦ C (Ni50 Mn28 Ga22
composition, [84]). The austenitic finish temperature for the same chemical
composition is Af = 52◦ C. We are now looking for a range of x for which
g0 2
T (x) = − 2k [x − L2 ] + Mf ≥ Af and the solution for the above mentioned
material parameters is x ≤20.6 [mm]. This implies that more than 80% of
the length will be fully transformed to the austenitic phase and the MFIS will
be decreased due to the presence of austenite [83]. However, this is a gross
estimation, and one needs to solve a coupled magneto-thermo-mechanical
system for more precise information.
5 Conclusion
We found that the time dependent part of the Maxwell equations, which
generally omitted in the quasi-static MSMA analysis, is significant for high
frequency analysis. The high actuation strain rate generated due to variant
reorientation cuts the applied magnetic field and produces motional elec-
tromotive force (emf). The total induced emf due to the rate of change of
magnetic field and motional emf generates an eddy current. Additional mag-
netic field due to eddy current adds up with the existing static magnetic field
and helps in variant reorientation. We solved numerically an Initial Bound-
ary Value Problem by using the existing MSMA constitutive equations in
a staggered way to capture electro-magneto-mechanical coupling responses
of different field variables. We found the eddy current and Joule heating
are significant. A comparison of eddy current and Joule heating between
MSMA and rigid-ferromagnetic/magnetostrictive materials reveals that the
differences are significantly high in MSMA. These could be the two essen-
tial parameters for shape and material optimization in device level MSMA
applications.
Acknowledgments
The authors would like to acknowledge the financial support of the Army
Research Office, Grant no. W911NF-06-1-0319 for the initial stages of this
work, NSF-IIMEC (International Institute for Multifunctional Materials for
Energy Conversion) under Grant No. DMR-0844082, and NSF-NIRT, Grant
no. CMMI: 0709283 for the support of the first author during his graduate
22
study at Texas A&M University.
APPENDIX
A Thermodynamic driving force
The four critical magnetic fields are: the start of forward reorientation, HsM2 ,
the end of forward reorientation, HfM2 , the start of reverse reorientation,
HsM1 , and the end of reverse reorientation, HfM1 . The reduced form of the
thermodynamic force (12) is given by
µ0 2 cur
π r = (σ ∗ + H )ε + µ0 ∆M2 H2 + f r . (A-1)
2 y
The hardening function is chosen as [85]
ξ˙ > 0 ,
( A
r
− 2 (1 + ξ n1 − (1 − ξ)n2 ) + B,
f := (A-2)
− C2 (1 + ξ n3 − (1 − ξ)n4 ) + D, ξ˙ < 0 ,
Solving the above five equations (from A-3a to A-5), we get the solutions of
five unknowns, A, B, C, D, Y r . The detailed derivation and the values of the
five parameters can be found in the [66].
23
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