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Analysis Stimulated Raman Scattering Waveguides: Wagner Shhul
Analysis Stimulated Raman Scattering Waveguides: Wagner Shhul
7 OCTOBER, 1965
Abstract-Stokesradiation,excited by a giantpulseradiation h waveguide with open ends (Fig. 1) does not sustain
propagating alonga rectangular waveguide, is analyzed in thispaper. electromagnetic modes inthepure sense of theterm.
Equations are established and solved for an arbitrary shape of the
giant pulse. At high gains the stimulated radiation is emitted at all
However, since theradiation wavelength is short com-
angles. The maximum outputis almost perpendicular to the exciting paredwith the geometrical dimensions and the growth
beam, and it decreases as theforward and backward directions are or decay times are much longer than the period of oscilla-
approached. Forward-backward ratios are sensitive to the detailed tion, it is meaningful to use the term in a “liberal” sense.
shape and magnitude of the laserpulse. The largeforward-backward Pure transverse modes in a long waveguide can be con-
ratio for intense short laser pulses accountsfor the observed results,
sidered as waves bouncing back and forth in a direction
which are illustrated for a square and a parabolic pulse. In practice,
a large number of waveguide modes are simultaneously excited, perpendicular to the laser beam. If the net power input
resulting in intense excitation of vibrational modes in the medium, into these transverse Stokes modes is positive and large,
and enhancement of the inverse Raman effect and of anti-Stokes their amplitude increases for a time which is of the order
generation. of the duration of the giant pulse. On the other hand,
a wave traveling along the waveguide interactswith
the laserbeamduring its transit time, which inmost
I. INTRODUCTION practical cases is shorter thanthe laser duration. It
EOMETRICALCONDITIONSin most experi- follows that modes wit’h a large transverse component
ments of stimulated Raman and Brillouin scat- of their propagation vector are amplified much more than
teringfavor high gainforStokesradiationin thosetravelingin the forwarddirection. It should be
directions parallel to the laser beam. On the ot’her hand, noted, however, that the higher amplification in a trans-
the highestgainforanti-Stokesradiation is nearthe verse mode also could beobtained in a free forward
off-axis angle satisfying the index matching conditions. propagation in a long path. Such a path is impractical
I n practice, the lateral dimensions of the laser beam are because of the inherent angular divergence of the laser
limitedand the anti-Stokesradiation can emerge from beam.
the high-gain region without attaining thehighest possible Asituation in which the laser beampermeates Dhe
amplification. A higher yield Stokes and anti-Stokes radia- waveguide cross section is considered. Boundary conditions
tion is obtained in a waveguide arrangement which re- prohibit a TEM propqation of the laser beam. However,
flects the radiation back into the high-gain region and if the guide’s cross section dimensions is muchlarger
preserves the index matching angles. Such a configuration t,han the radiationwavelength, it is a good approximation
has been used by Dennis and Tannenwald [l]to obtain to disregard theboundary conditions for waves prop-
a 90 degree Itaman Stokes emission, and by Tang and agatinginthe forwarddirection. The beamintensity
Deutsch [a] andatthe HughesResearchLaboratories is therefore assumed to be uniform along the cross section.
to enhance the anti-Stokes radiation. In an arrangement It follows that the gain for the Raman Stokes and the
where the Raman or Brillouin active material is bounded Brillouin scattering will also be uniform dong that cross
by highly reflecting surfaces, stimulated radiation is gen- section.
erated in a large number of propagating modes. The net The transversenonpropagating modes are in fact stand-
overall gain in these nzodes is determined by the laser ing waves withvanishinglinearmomentum along the
power, the polarization, and the geometrical and optical waveguide axis. Consequently, the momentum conserva-
properties of the waveguide. tionrelationsfor the Stokes and Brillouin cases are
Manuscript received July 2, 1965; revised August 20, 1965. represented by the vector relations (Fig. 2),
W. G. Wagner is with Hughes Research Laboratories, R/lalib11;
Calif. E, = 5, f lGou
S. Yatsiv is with Hughes Research Laboratories, Malibl1, Calif.
He is on leave from tbe Hebrew University, Jerusalem, ‘Israel. 5, = ins + En7,.
287
IEEE JOURNAL OB' QUANTUM ELECTRONICL OC'l'OBfCC
XE =
1 aB
c at
where U, = 1 is assumed. The amplitude 8 , ( t ) of the h e r
field
Ji;l(w2) = &,(t)exp [i(qzz - w , t ) ] (41
is actuallytimedependent, following theshape of thc
giant pulse. I f is assumed that the variation during an
optical cycle is small and satisfies the equation
s, << w,E,. (5)
Accordingly, the linearized wave equation can be written
in the approximate form
Equating
the
real
andimaginary
parts, we obtain
The
quantity (hac cos
O/nV) represents
the power
flux caused by quantum noise or the spontaneous Raman
= C-2W:[E + x f E:@)] (9) emission. It is convenient to normalize P interms of
(fiwc cos e/nV) by defining a dimensionless quantity N
and
Pn V
2
k , g f = c- 2 w,x 2 N =
E&). f f
hwc COS e
I n practice, ( g f / 2 ) 2 << ?cf +
k: and X f & : ( t ) << E; con- which represents an effective &mode occupation number.
sequently, the power gain constant is N satisfies the equation
gf = g sec e W,C
-1
XIf &,(t)
2
see e (11)
where
The experimentally measured quantities are the power
e ~ C
I, _ _ fluxes N ( L , 0, t ) and N(0, 8, t ) . Theseoutputssatisfy
(k: + , y 2
COS =
the condition in the forward and backward semicircles:
and 0 is the angle between the normal to a plane wave
generating the mode andthe x axis. Henceforth,this
N ( 0 , e, t ) = 0 for forward emission
will
as be referredand
to a e mode. (17)
The boundary condition for perfect reflectivity is met
N ( L , e, t ) = 0 for backward emission.
when
With these conditions, the solution of the differential
(m integer). equation (16) is
The gain g sec 0 determines the amplification of the wave N ( L , e, t) = exp S, Lse.28
[ g ( t - ux:)- s(e)l dz - 1
in the absence of dissipation. Its time dependence follows
that of the giant pulse. I n practice, g and &: decreases
along the waveguidebecause of theproduction of the
s(e) / i s e c d {exp+ /'
[ g ( t - uz) - s(e)l dx dy (18)
1
Stokes radiation. We shall assume that this attenuation in the forward direction, and
canbe neglected, and we shall discuss thevalidity of
this assumption in a later section.
The dissipation in a metallic waveguide results mainly
N ( 0 , e, t) = exp
Lsec8
[g(t - 1 1
u. - &(e)]dz - I
IO8
lo7
to6
z lo5
io4
Fig. 3. Parabolic gain pulse.
lo3
A. Power an.d En,ergy Outputs in the Forward !Semicircle
The gain of a wave packet traveling in the forward
IO2
direction ( e = 0) is constant, along the path, since both
Stokes and laser radiation travel wit'h the same velocity.
(Dispersion can be neglected in a short guide.) 10'
For angles e larger than ec, the power and energy fa11
off monotonically.
B. Baclcwurd Semicircle
The nlaxirnum outputinthe backward senxicircle is
always at e = R / Z , falling off nlonotonically toward 0 = R .
Its effective interactiontime at a11 angle 6 is smaller
than at the corresponding forward angle. It follows t'hat
the output in a backward direction is lower than that in
the corresponding forward direction, particularly for short
pulses. The curves for the two semicircles join smoothly
at e = a/2 (Fig. 5). The angular behavior and the for-
ward-backward ratios a.re illustrated in the square-step
for e > e,. (24)
case. Because of the exponential eharac%cr of the ampli- Equations (23) and (24) give the emission 1)alterns in
SCATTERIXG I N WAVEGUIDES 291
FORWARD 8 BACKWARD
and
Thedominant large exponential factors rise andfall
nI,
- (see e, - 1) forward off steeply on both sides of the critical angle. It follows
ry
1 = C
(26) from expressions (23a) and (24a), as well as from Figs. 5
and 6, that at high gains the angular width at half max-
nL
--
c
(/see e,I + 1) backward. imumcan be of the order of 1 degree. Consequently,
most of the power and energy are emitted in a narrow
I t is assumed that T is larger thanthetransittime angular width in adirection which is almost perpendicular
nL/c. Curves for the power output N ( t ) at different angles to the laser beam.
and for the angular dependence E(t9) are given in Figs. 4 b) Low gains: Here (g - 6)L << 1. The exponerltials
and 5 . The maxima of N ( t ) and E(8) in t,he forward involving (g - 6)L can be expanded, yielding
semicircle are atthe critical angle 8, in the forward
direction [see (26)].
The interaction time of a wave packet in a 8, mode,
+
L see e- 1
-
6.
+ 16 exp (-
- 6L sec e) 1
startingat x = 0, with the laser beam is T nL/c.
At the end of its interaction time, the wave p d c e t is a t
+ g(T - T,)L see e, e < e, (23b)
z = L. ,4 packet starting a t x = 0 ina 8 (> 8,) mode and
finds itself at a point x < L at, the end of its interaction
time 1' + nx/c, which is smaller than T +
nL/c. Con-
sequently; the amplification and the power out'put a t such
angles are smaller than for e,. I n the backward semicircle .It should be noted thatthe first derivative of E(e)
the Stokes and laser beams aretraveling in opposite vanishes a t 0 = 0, but the second derivative is positive,
directions. Theinteractiontime at the critical angle is indicatingamaxinlumoutput at e f 0 even for small
T - n L / c and is smaller thanthetime T - nx/c for gains.
0 < 0,. I t follows that the maximum power and energy 2 ) Backward-Forward Intensity Ratios: The backward-
outputs fall off monotonically as the angle approaches forward ratio is an important parameter for which widely
the backward e = T direction. different results were obtainedexperimentally [GI. The
1 ) Asymptotic Solutions: A simple asympt'otic form can calculated value for a square pulse is obtained,noting
be obtained for E ( @ at high and low gains. that u = T s = 0 i,n the forward and u = 2n/c, T o =
292 IEEE JOURNAL O F QUANTUM ELECTROKICS OCTOBER
2nL/c in the backward direction. In most practical cases and the forward-backward ratio is
n/(c6) is much smaller than the pulse duration T and T
canbe neglected. At high gains 2n/[c(g - a)] can also 1' - 2nL/c '
be neglected. Withtheseapproximations, the resulting as in the guided wave.
energy outputs are, for high gains,
D. Parabolic Pulse
forward The power and energy outputs for a parabolic pulse
(27) g ( t ) were also computed. The Stokes energy output for
E = LT
g--6
( 2nL)
c exp ( g
- - 6)L backward,three laser pulses of almost equal energy but different
durationsisdrawninFig. 6. The shape of the curves
and for low gains, is similar to those of the square st.ep. It should be noted
E = gTL forward that for high gain and short pulses, the forward-backwmd
ratio becomes exceedingly large. Itattainsthe value
E =
g(T - ?)I- L6 << 1
backward.
2.5 X 10' for 7 = 5 x lo-'' second and g, = 3 em-'.
The large rat,io is explained as follows. In the forward
yTL +
2n
C
(L - i) L6 > 1
direction a Stokes wave packet moves in step with the
laser beam and may have the maximum gain throughout
its motion. A packet moving backward can have a max-
The formard-baclrmard energy ratioat high gainis imum gain only in a very short time. It actually samples
T / ( T - 2nL/c). This is also the ratio obtainedin the the laser pulse shape inan interval2Ln/c, and is, therefore,
absence of dissipation or freepropagation (see Section much weaker when the pulse is short and strong. Since
111-(3-3). It is noteworthy that in actual experiments the giant pulses often possess narrow spikes, we believe this
gain may be so high t'hat an equivalent square-step rep- is the reason for the sonlet,imes large, nonuniform meas-
resentation is determined by small spikes bulging a.bove ured forward-backward ratio [GI. Bloembergen and Shen
the normal level of the gain pulse. Such spikes can be [7] rightly observe that a change of a few percent between
short, and the ratio T / ( T - 2nL/c) becomes exceedingly the forward and backward gains is sufficient to explain
large. the observed results; however, theyattributethe gain
The forward outputs may cease to be dominant over difference to the different, damping of the opt'ical phonons
the backward outputs if theat,tenuation of the laser emitted in the two cases.
beam along the direction of propagation is considered. The frequency of the emitted optical phonon is much
If g - 6 vanishes a t some point in the active medium, higher than that of any acoustical vibration in the liquid
the larger forward amplification in the back 9 - 6 > 0 or solids on hand. It follows that relaxation of an optical
region is offset by the attenuation in the front g - 6 < 0 quantum involves two or more acoustical phonons. I n
region. A baclrward scattered wave is amplified only in this case, we fail to see that the relaxattion is as sensitive
the back g - 6 > 0 region and therefore not subject to to the available volume in momentum spaceas stated
anyattenuation. I n such a case the backward output in [7].The two different views could be resolved by careful
can be larger than the forward output. measurement of the forward-backward ratiowhile monitor-
3) Propagation in theAbsence of Dissipation: In the ing the giant pulse shape.
limit 6 = 0, (23) and (24) take the form It is seen in Fig. 6 that as the duration of the parabolic
pulse increases, the maximum energy output approaches
the 6 = ~ / 2angle. The angular pattern of the Stokes
radiation serves as arough diagnostic tool for the temporal
shape of the gaint pulse
IV. EXPERIMENTAL CONSIDERATIOSS
8 > 8,. (24c) Caution is needed inattemptingto compare experi-
ment'al results with this analysis because t,he power output
The forward and backward emissions become
in the various Stokes modes is very sensitive to the gain
E(0) = T(exp gL - 1), forward g ( l ) . The bxderline is verynarrow between powers a t
which the laser beam is not deplet.ed and those for which
it. is highly drained.
At high gains it is possible to evaluate the integmted
power output as follows. The maximum Stokes emission
power rises steeply as the critical angle 8, is approached.
For st.ill larger angles and in the backward semicircle,
At high gain and for L >> l/g the baclrward emission is
it falls off relatively slowly. Therefore, a good estimate
for the total power output at high gains can be obtained
by integrating over the angle from 0, to ~ / 2 .
1965 WAGNER AND YATSIV : RAMAN SCATTERING I N WAVEGUIDES 293
APPENDIXA
The explicit form of (16) in the forward semicircle is
eg e - I)(L - 2)](1v+ 1)
At high gains the angle 4, is approximatelyequalto
nL/(nL + Tc) and is much larger than n/[(g - 6)TcI.
dN-- see
-
dz [t -:. - (see
Equations (40), (41), (42), and (43) also hold for t,he
backward semicircle, provided that is
defined l‘,
as
T o = nL(1sec 81 +
l ) / c and u = n(1 +
/cos 8l)/c. It
should also be noted that the power outputs N ( t ) are
continuous functions of t and the energies &(e) are con-
tinuous functions of 8.
REFERENCES
N(t) = -
9
J. H. Dennis and P. E. Tannenwald, “Stimulated Raman emis-
g- 6 sion a,t 90” to the ruby beam,” A p p l . Phys. Lett., vol. 5, pp.
58-60, August 1964.
C. L. Tangand T. F. Deutsch.“Generation of anti-Stokes
radiation i n t h e higher order coherent Raman processes,” Phys.
Rev., vol. 138, pp. Al-A8, April 1965.
Y . It. Shen and N. Bloembergen, “Theory of stimulated Bril-
T+Tg<t (40d) louin and Raman scattering,” Phys. Rev., vol. 137, pp. A1787-
81805, March 1965.
N(t) = 0. H. R.L. Lamont, Wuve Guides, 3rd ed., Methuen’s Monographs.
London: Methuen and Co.. Ltd.. 1950.
[5] W.G. Wagner and €3.A. Lengyel, “Evolution of the giant pulse
The energy output is obtained by integrating N ( t ) over in a laser,” J . i l p p l . Phys., vol.34, pp. 2040-2046, July 1963.
+
the entire 0 < t < 1’ T oint.erva1, which yields [6] P. I). Maker and R.W. Terhune, “Study of optical effects due to
an induced polarization third order in theelectric Geld strength,”
Phys. Reo., vol. 137, pp. 801-818, February 1965.
E ( @ = exp [(g - 6)L see 81 [7! N. Bloembergen and Y. R. Shen, “Coupling between vibration
and light, waves inRaman media,” Phys. Bev. Lett. vol. 12,
pp. 504-507, May 1964.
[SI 1). Weiner, S. E. Schwarz, and F. J. McClung, “Comparison of
observed and predicted Raman scattering conversion effi-
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[9] It. Loudon, “Theory of stimulatedRamanscattering from
lattice vibration,” Proc. Phys. Soc. ( L o n d o n ) , vol. 82, pp. 393-
400, September 1963.