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2018 Mizeraczyk Controlled Generation of Single Trichel J Phys D Appl Phys
2018 Mizeraczyk Controlled Generation of Single Trichel J Phys D Appl Phys
2018 Mizeraczyk Controlled Generation of Single Trichel J Phys D Appl Phys
E-mail: jmiz@imp.gda.pl
Abstract
In this paper, a simple method for the controlled generation of a single Trichel pulse or a series
of single Trichel pulses of a regulated repetition frequency in air is proposed. The concept of
triggering a single Trichel pulse or a series of such pulses is based on the precise controlling
the voltage inception of the negative corona, which can be accomplished through the use
of a ramp voltage pulse or a series of such pulses with properly chosen ramp voltage pulse
parameters (rise and fall times, and ramp voltage pulse repetition frequency). The proposal
has been tested in experiments using a needle-to-plate electrode arrangement in air, and
reproducible Trichel pulses (single or in a series) were obtained by triggering them with an
appropriately designed voltage waveform. The proposed method and results obtained have
been qualitatively analysed. The analysis provides guidance for designing the voltage ramp
pulse in respect of the generation of a single Trichel pulse or a series of single Trichel pulses.
The controlled generation of a single Trichel pulse or a series of such pulses would be a
helpful research tool for the refined studies of the fundamental processes in a negative corona
discharge in a single- (air is an example) and multi-phase gaseous fluids. The controlled
generation of a single Trichel pulse or a series of Trichel pulses can also be attractive for those
corona treatments which need manipulation of the electric charge and heat portions delivered
by the Trichel pulses to the object.
1. Introduction after Trichel who observed them for the first time in 1938
[1]. A single regular Trichel pulse has the form of a sharp
It is known that the negative corona discharge in the needle- current increase (usually lasting nanoseconds, followed by a
to-plate electrode arrangement in air at the corona voltage relatively long low-current tail (of hundred nanoseconds) [2].
threshold usually consists of irregular pulses having a repeti- The properties of Trichel pulses have been comprehensively
tion rate in the kilohertz range. A small increase in voltage described in many regular papers, textbooks and reviews
results in the establishment of regular current pulses having [3–7].
their amplitudes in the milliamps range. The frequency of the The younger of these publications, as well as many regular
regular pulses can extend to the megahertz range. These kind papers published after 1974, have referred to a work of Lama
of negative corona current pulses are known as Trichel pulses, and Gallo [8], who analytically summarised and experimentally
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J. Phys. D: Appl. Phys. 51 (2018) 155204 J Mizeraczyk et al
such a discharge. Examples are: a refined corona treatment in 2. Experimental set-up
printing on polymers [23] and non-thermal plasma treatment
of biological materials (e.g. bacteria [24]). The experimental apparatus for the controlled generation of
The use of the single Trichel pulse technique could be single Trichel pulses consisted of a discharge chamber (an
attractive for the investigation of negative coronas not only in acrylic box with a needle-to-plate electrode arrangement
air (a single-phase fluid) but also in gaseous multi-phase fluids inside), a digital signal generator, a high voltage amplifier,
[25]. For example, a single Trichel pulse or a controlled series two voltage probes and a digital oscilloscope (figure 2).
of such pulses could be useful for refined controlling of the
gaseous two-phase flows.
2.1. Discharge chamber
The single Trichel pulse technique does not require a com-
plex apparatus, which may be considered as its technical merit. The discharge chamber (a sealed acrylic box, L:W:H = 600
It worth noting an experimental convenience when studying mm: 120 mm: 50 mm) with the needle-to-plate electrode
the effects of a single Trichel pulse (nanosecond time scale)— arrangement was filled with air at atmospheric pressure.
synchronisation of the single Trichel pulse inception with the Both the needle and the plate electrodes were made of
other equipment used in the experiment is easy. stainless-steel. The negative voltage stressed needle electrode
The successful generation of a single Trichel pulse depends (the discharge electrode) was a rod (1 mm in diameter), the
on the precise control of the inception moment of the negative end of which had a tapered profile with the tip having a radius
corona. Previously, for fixing the negative corona inception of curvature of 75 µm. The inter-electrode gap was 25 mm.
moment, various external methods were used (comprehensive The plate electrode was grounded.
literature on this subject can be found in [26, 27]). They were:
negative corona triggering by soft x-ray pulses, radioactive β
2.2. Power supply and measuring equipment
or γ sources, and UV radiation from mercury lamps, excimer
lamps and lasers. However, these external methods, inconven- The negative high voltage was supplied by a high voltage
ient to use, were unsatisfactory even when aimed at triggering amplifier (Trek, 40/15) which amplified the voltage signal
regular Trichel pulses. delivered by a digital signal generator (Tektronix, AFG 3052
The concept of triggering a single Trichel pulse presented C). The negative high voltage was applied to the needle elec-
in this paper is based on the precise controlling the voltage trode through a 3.3 MΩ resistor. The voltage between the
inception of the negative corona. The precise setting of the needle electrode and the plate electrode was measured using
inception voltage on the discharge electrode can be accom- a high-voltage probe (Tektronix, P6015A) and recorded by
plished through the use of a ramp voltage pulse with properly a digital oscilloscope (Keysight, DSO 9064A, bandwidth
chosen ramp pulse rise and fall times (an example of such a 600 MHz, sampling rate 10 GS s−1). Using a voltage probe
pulse is shown in figure 3). (Agilent, N2873A), the discharge current waveform was mea-
Below, an experiment aimed at the controlled generation of sured as a voltage drop across a 2 kΩ resistor placed between
a single Trichel pulse and a series of single Trichel pulses in the plate electrode and the ground. The voltage drop was
the needle-to-plate electrode arrangement in air is presented. It recorded by the digital oscilloscope.
will be shown that the controlled generation of a single Trichel
pulse and a series of single Trichel pulses can be achieved
3. Results
by triggering the negative corona with an appropriate ramp
voltage pulse waveform. The proposed method and results
3.1. Single Trichel pulse
obtained will be qualitatively analysed. The analysis provides
guidance for designing the voltage ramp pulse in respect of The first part of the experiment was aimed at the generation
the generation of a single Trichel pulse or a series of single of a single Trichel pulse. The idea was to generate the first
Trichel pulses. Trichel pulse and avoid the generation of the next Trichel
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J. Phys. D: Appl. Phys. 51 (2018) 155204 J Mizeraczyk et al
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J. Phys. D: Appl. Phys. 51 (2018) 155204 J Mizeraczyk et al
(2) divE = 0.
Solving equation (2) for the case of the needle-to-plane gap
gives the electric field distribution as follows [28]:
2U ∗
E (x) ∼
= .
(3)
(r0 + 2x) ln 2d
r0
Here, r0 and d are the curvature radius of the needle tip and
length of the inter-electrode gap, respectively. Using the dis-
tribution (3) and the ionisation coefficient αi in Townsend’s
approximation:
Bln 2d
B r0
αi (x) = Aexp − = Aexp − (r0 + 2x) ,
E(x) 2U ∗
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J. Phys. D: Appl. Phys. 51 (2018) 155204 J Mizeraczyk et al
across the corona gap is constant, i.e. U = U* = const. On the 4.2. The time-lag between the first and second Trichel pulse
other hand, this voltage consists of two variable components: and between regular Trichel pulses
U ∗ = Ui (t) + Ud (t), where Ui (t) and Ud (t) are the dimin- The time intervals ∆τ12 and ∆τr between the first and second
ishing voltage drop across the high-conductive ionisation Trichel pulses and two neighbouring, regular Trichel pulses is
area and the growing voltage drop across the rest of the non- determined by the time needed to remove the excess of posi-
ionised gap, which has some electric capacitance C, respec- tive charge from the ionisation area created by the preceding
tively. Based on the above, we can estimate the total diminish- pulse. Both time intervals are proportional to the length of the
ment of Ui for the first Trichel pulse as follows: ionisation area that forms the preceding pulse, i.e. ∆τ12 ∼ xi1
(6) ∆Ui1 ∼
= Ui1 − Ucn ∼ = 1.6 kV − 0.3 kV = 1.3 kV. and ∆τr ∼ ∆lcr . As for the first Trichel pulse, the length xi1
of the ionisation area is determined by the Laplace distribu-
In the course of cathode layer formation, the conductivity
current I(t) flowing through this layer is being supported by tion of the electric field, which sharply decreases ( E(x) ∼ 1x ).
the displacement current flowing through the non-conductive Because of that and of the saturation of αi with the increase
in the electric field, the ionisation area has to be extended in
gap: Ii (t) = C ∂U∂td (t) ≡ −C ∂U∂ti (t). Thus, the first Trichel pulse
order to satisfy the self-sustaining condition (1). Contrariwise,
is being formed by the displacement current through the non- at the presence of the positive space charge in the vicinity of
ionised gap, the amplitude of which is determined by the the needle, the Poisson electric field distribution is smoother
dynamics of the shrinking cathode layer. However, after fin- (close to the linear dependence like E (x) ∼ (1 − ax)) that
ishing the shrinking process of the large ionisation area up to leads to shortening the length ∆lcr of the ionisation area,
the thin needle cathode layer, the Ud (t) magnitude will not whereby the self-sustaining condition (1) is satisfied. This is
increase more, and the non-ionised gap of the corona therefore the reason why the length xi1 appreciably exceeds the length
cannot support the high current formed by the cathode layer. ∆lcr of the subnormal cathode layer under the critical voltage
It leads to the high-current cathode layer decaying into a low- drop Ui∗ , which, in turn, leads to an inequality ∆τ12 > ∆τr .
current subnormal mode. This decay in corona current is being Moreover, the length ∆lcr decreases with an increase in the
accompanied by the expansion of the cathode layer and the average corona current that decreases the period of regular
increase in the Ui (t) magnitude. As soon as Ui (t) reaches the Trichel pulses. Both of these conclusions are consistent with
critical magnitude Ui∗, the restoration of the needle cathode the experimental observations.
layer accompanied by its shrinking and diminishing, the Ui (t)
happens again and a new Trichel pulse is being formed. The
repetition of these events results in the establishment of a reg- 4.3. Reliable reproducibility of the first Trichel pulses
ular sequence of Trichel pulses. with the use of the pulsed-periodical voltage
Note that the second and next Trichel pulses are formed Due to the definition, the first Trichel pulse develops in a
in the presence of the positive space charge created in the gap that is free of any space charge. Therefore, if the pulsed-
vicinity of the needle by the previous pulses. It causes the periodical voltage is used for the excitation of only the first
Ui∗ magnitude to be lower compared to Ui1, corresponding to Trichel pulses, it is necessary to fully remove from the gap the
the case of non-ionised gas around the needle. According to negative space charge created by the preceding Trichel pulse
the numerical calculations of Trichel pulses [17, 29], the Ui∗ before the appearance of the next one. Let us estimate the time
magnitude can be estimated as Ui∗ ∼ = 2Ucn . In such a case, the T needed for full removal of the negative space charge onto
total diminishment of Ui for the regular Trichel pulses will be the anode. For definiteness, we will assume that the applied
lower: voltage is a periodic sequence of saw-tooth pulses. The
(7) ∆Uir ∼= 2Ucn − Ucn ∼ = (0.3 ÷ 0.4)kV. voltage in each saw-tooth pulse linearly increases in time up
to amplitude U0 = 5.2 kV and instantly falls down to zero at
Based on the above, we can estimate the relationship between
t = T: U (t) = U0 Tt . In other words, T is the period of periodic
the current amplitudes of the first I1 and the regular Ir Trichel
sequence of saw-tooth pulses. In order to provide the period-
pulses. We take into account that according to the numerical
ical reproducibility of the first Trichel pulses, each saw-tooth
calculations, the major changes in Ui of the first and regular
pulse has to perform two functions: (1) to remove quickly
Trichel pulses happen before the maximum current appear-
(in time t < T) the charge generated by the preceding Trichel
ance, within the time interval Δτ with a duration of several
pulse onto the anode, and (2) to create near the cathode the
nanoseconds. In such a case, the I1/Ir ratio can be approxi-
negative charge by its own first Trichel pulse at the moment
mated as:
t = T.
I1 ∼ ∂Ui1 (t) ∂Uir (t) ∼ ∆Ui1 /∆τ ∼ ∆Ui1 We can estimate the minimal duration Tmin needed for
= −C / −C = = . execution of the first function. To do that, we assume that
Ir ∂t ∂t ∆Uir /∆τ ∆Uir
(8) the space charge generated by the first Trichel pulse weakly
Using equations (6) and (7), we find that the I1/Ir ratio is: influences the Laplace distribution (3) of the electric field in
the gap. The equation describing the drift of negative ions
I1 ∼ ∆Ui1 ∼
(9)
= = 3 ÷ 4, through the gap can be found from the definition of the ion
Ir ∆Uir drift velocity Vi ≡ dx/dt = µi E (where E is the electric field
which is close to the experimental data presented in figure 1. strength taken from (3)):
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J. Phys. D: Appl. Phys. 51 (2018) 155204 J Mizeraczyk et al
dx 2µi U(t) 1 It means that the duration τ of the pause between two
= · . neighbour saw-tooth pulses can be diminished practically to
(10)
dt 2d
r0 ln r0 1 + 2x
r0 τ ≈ td. As mentioned above, the formation of the first Trichel
Equation (10) was derived under the assumption that the pulse takes a short time compared to the ion drift time across
total thickness of the cathode layer and transition region the gap. Because of that, it is possible to diminish the duration
where electrons are being transformed into negative ions is of saw-tooth pulses and increase the frequency for generation
much smaller compared to the length of the drift region which of the first Trichel pulses up to 475 Hz.
is equal approximately to the gap length, d. Many numerical All of the above serves as evidence that the offered
calculations have confirmed confirm this assumption [30]. In approach for periodical generation of the first Trichel pulses
such a case, we can choose the coordinate x = 0 close to the based on combination of the saw-tooth pulses and the DC bias
cathode surface. The integration of equation (10) gives: is very promising.
d2 · ln 2d r0
(11) Tmin ∼
= . 5. Summary and conclusions
µ i U0
For the specific experimental conditions, the parameters in In this paper, we presented a simple method for the controlled
equation (10) are: generation of a single Trichel pulse and a series of single
Trichel pulses (of regulated repetition rate) in air in a repro-
2d 2d ∼ ducible manner. The controlled generation is based on trig-
= 667; ln = 2.2 · 10−4 m2 V−1 s−1 ;
= 6.5; µi ∼
r0 r0 gering a single Trichel pulse (or a series of such pulses) by an
d = 2.5 cm; U0 = 5.2 kV. appropriately designed voltage waveform. The parameters of
a single Trichel pulse (the pulse current amplitude and wave-
Substituting these parameters in equation (11), we obtain form) generated with the proposed method are similar to those
Tmin ∼= 3.55 ms. of the first Trichel pulse generated spontaneously in a nega-
Note the formation of the first Trichel pulse takes much tive corona in air. Note that the single Trichel pulses produced
shorter time compared to the drift removal of the generated using the proposed method exhibit higher current amplitudes
negative charge onto the anode. It means that maximum fre- and electric charge than those typical of ‘traditional’ regular
quency for periodical sequence of the saw-toothed pulses Trichel pulses. The theoretical background of the proposed
under the specific experimental parameters cannot be higher method has been presented. The results obtained were qualita-
than 280 Hz. tively analysed. A good agreement between the experimental
In principle, it is possible to use another regime for peri- results and the theoretical predictions was found. The analysis
odical generation of the first Trichel pulses, when short provides guidance for designing the voltage ramp pulse in
saw-tooth voltage pulses with T < Tmin are separated from respect of the generation of a single Trichel pulse or a series
each other by a long pause with duration τ > Tmin. In this of single Trichel pulses.
case, the negative charge generated by each short saw-tooth As the main purpose of this paper was to introduce the
voltage pulse has to be removed onto the anode during the essence and justification of the method for the controlled gen-
pause after the voltage pulse. However, in the absence of an eration of a single Trichel pulse and a series of single Trichel
applied voltage during the pause, the duration of pause has to pulses, other data on the method development will be pre-
be long enough to remove the negative charge from the gap sented at a later date.
by the electrostatic field induced by the charge itself. Indeed,
the experiment with T < Tmin showed that even duration of
τ ≈ 100 ms is not enough to remove the negative charge from Acknowledgment
the gap after each saw-tooth pulse and to provide the repro-
ducible periodical generation of the first Trichel pulses. This work was supported by the National Science Centre
The situation can be improved essentially if we use the (Grant No. UMO-2013/09/B/ST8/02054).
combination of the saw-tooth pulses with the DC voltage. In
this case, the negative charge formed by the first Trichel pulse
ORCID iDs
in the preceding saw-tooth pulse will be removed by the DC
voltage during the pause between voltage pulses. Using the
Artur Berendt https://orcid.org/0000-0003-1013-7337
combination of the saw-tooth pulses with the DC voltage gives
Yuri Akishev https://orcid.org/0000-0001-8379-5782
a possibility to diminish the duration τ of the pause between
two neighbour saw-tooth pulses. Indeed, according to equa-
tion (10) with the DC voltage bias U (t) = UDC = 4.4 kV, References
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