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One Hundred Years of Rapakivi Granite
One Hundred Years of Rapakivi Granite
One Hundred Years of Rapakivi Granite
Mineralogy
aDO
Petrology
© Springer-Verlag 1995
Printed in Austria
With 11 Figures
Summary
Rapakivi granites, recently redefined as A-type granites showing rapakivi texture at least
in the larger batholiths, occur on all continents and presumably represent the most
voluminous continental silicic intraplate magmatism on Earth. Most of the rapakivi
granites are Proterozoic (mainly 1.0 to 1.7 Ga) but also Archean (2.8 Ga) and Phaner-
ozoic (0.05 to 0.4 Ga) are known. The magmatic association is bimodal comprising
anorthosite to gabbro, diabase, minor Fe-enriched intermediate rocks, and monzonite,
beside granite; mingling of silicic and mafic magmas is typical. Geochemically and
otherwise, rapakivi granites show the characteristics of the Phanerozoic A-type granites,
except that they encompass relatively few peralkaline rocks and that they may occur as
very large (up to 40,000 km 2) batholiths. Some of the rapakivi granite complexes host
important Sn-polymetallic and Fe-Cu deposits.
The rapakivi granites crystallized from relatively hot, restite-poor magmas at low
(epizonal-subvolcanic) pressure, an2o, and ao2. Mineral assemblages are indicative of a
multiphase crystallization history; the conspicuous mantling of the perthite ovoids with
plagioclase can be explained by changes in magma composition and/or, P, T, and an2o
affecting the stabilities of feldspars. The isotopic composition of rapakivi granites is
generally compatible with a lower crustal protolith. The latter could have been either a
melt-depleted residue or otherwise relatively anhydrous igneous or metaigneous rock.
Melting of the protolith commenced under vapor-absent conditions and was induced
by heat from the contemporaneous mantle-derived marie magmas. The widespread
rapakivi granite magmatism in the Middle Proterozoic may have been related to the
establishment of a major continental mass (supercontinent).
Zusammenfassung
Einhundert J ahre Rapakivi-Granit
Rapakivi-Granite sind A-Typ Granite mit Rapakivi Texturen, die zumindest in den
gr6Beren Batholiten zu erkennen sind. Sie kommen auf allen Kontinenten vor und stellen
wahrscheinlich das umfangreichste Beispiel kontinentalen sauren Intraplate-Magmatis-
130 O.T. Rfim6 and I. Haapala
mus dar. Die meisten Rapakivi-Granite sind proterozoisch (1.0 bis 1.7 Ga), jedoch sind
auch archaische (2.8 Ga) und phanerozoische (0.05 bis 0.4 Ga) Beispiele bekannt. Die
magmatische Assoziation ist bimodal und umfaBt Anorthosit bis Gabbro, Diabas, in
kleinerem Umfang Fe-angereicherte intermedi/ire Gesteine und Monzonit, zusfitzlich zu
Granit. Das gemeinsame Auftreten yon Silizium-reichen und mafischen Magmen ist
typisch. Die geochemischen Charakteristika der Rapakivi-Granite entsprechen phaner-
ozoischen A-Typ Graniten mit der Ausnahme, dab sie relativ wenige peralkaline Gesteine
umfassen und dab sie als sehr groge (bis zu 40.000 km 2) Batholithe vorkommen k6nnen.
Einige Rapakivi-Granite fiihren wichtige Zinn-polymetallische und Fe-Cu Lager-
st/itten.
Die Rapakivi Granite kristallisierten aus einem relativ heiBen, Restit-armen
Magma bei niedrigem (epizonalem bis subvulkanischem) Druck, aH~o und ao~. Miner-
alassoziationen weisen auf eine vielphasige Kristallisationsgeschichte hin; die auffallen-
den Umwachsungen von Perthit-Ovoiden mit Plagioklas k6nnen durch Nnderungen
in der Magmenzusammensetzung und/oder von P, T und an~o erkl/irt werden, die die
Stabilit~ten der Feldspate beeinflussen. Die Isotopen-Zusammensetzung der Rapakivi
Granite entspricht im allgemeinen einem tieferen Krusten-Protolith. Der letztere kann
entweder ein an Schmelze verarmtes Residuum oder auch ein relativ wasserarmes,
magmatisches oder metamagmatisches Gestein gewesen sein. Schmelzen des Protoliths
begann in Abwesenheit yon volatilen Phasen und wurde durch W~irmezufuhr von
gleichaltrigen mafischen Magmen, die aus dem Mantel stammen, herbeigefiihrt. Der weit
verbreitete Rapakivi Granit-Magmatismus im mittleren Proterozoikum dtirfte mit der
Bildung eines Superkontinentes in Beziehung zu setzen sein.
1. Introduction
One hundred years ago, J. J. Sederholrn (1891) published his classic study of rapakivi
granites entitled 'Ueber die finnl~indischen Rapakiwigesteine' in Tschermak's
Mineralogische und Petrographische Mittheilungen (now Mineralogy and Petrol-
ogy). In this pioneering work Sederholrn described the areal distribution, mode of
occurrence, petrography, and chemistry of the Finnish rapakivi granites. Moreover,
he distinguished the terms rapakivi granite and rapakivi texture and showed
that rapakivi granites form an igneous suite with both intrusive and extrusive
characteristics.
The Finnish word "rapakivi" means disintegrated or crumbly rock or stone and
denotes the tendency of certain rapakivi granite types to disintegrate more easily
than other granitic rocks of the region. In the 18th century, rapakivi granite was
mentioned or briefly described in several reports and academic theses of Finnish
and Swedish scientists. Thanks to Sederholrn's paper, the terms rapakivi granite and
rapakivi texture were incorporated into the international geological terminology,
and southern Finland has since then been regarded as the type area of these rocks.
The work of Sederholrn has been continued and amplified by other Finnish geolo-
gists (Walter Wahl, Pentti Eskola, Victor Hackman, Th. G. Sahama, Antti Savolahti,
Atso Vorrna, among others).
Soon after Sederholrn's 1891 paper had been published, rapakivi granites were
found in Sweden and the Ukraine, and later in the 20th century in the Precambrian
of North America, South America, Asia, Australia, and Antarctica. Rapakivi gran-
ites and related anorogenic granites form an integral part of many Precambrian
cratonic areas and their formation has been an essential part of Precambrian
crustal evolution. The purpose of this paper is, together with a separate paper on
One hundred years of Rapakivi Granite 131
in the larger batholiths, of granite varieties showing the rapakivi texture'. This
definition takes into account the mode of occurrence, magmatic association, petrog-
raphy, mineralogy, and chemistry of the granites but does not restrict the absolute
age of the rocks. It does, however, exclude migmatites and S- and I-type granites,
which locally may have alkali feldspar megacrysts mantled by plagioclase.
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One hundred years of Rapakivi Granite 135
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One hundred years of Rapakivi Granite 137
4. Petrography
Beside the conspicuous rapakivi texture, rapakivi granites exhibit a characteristic
mode of occurrence and lithologic association that, combined, distinguish them
from other granite suites. Typically they occur as multiple high-level batholiths and
stocks that sharply cut the surrounding metamorphic bedrock. They are often also
associated with mafic rocks (gabbros to anorthosites, ferrodiorites, diabase dykes,
basalts) and usually evidence no concurrent orogenic movements in their fabric.
Compared to the granitoids of typical calc-alkaline associations, the silicic rocks in
rapakivi granite complexes show less compositional variation and are characterized
by ubiquitous Fe-enriched mafic silicates and by high alkali feldspar content. This
section confines itself to the petrography of the silicic rocks of the rapakivi associa-
tion, first dealing with the classic Finnish rapakivi granites and thereafter with
rapakivi granites elsewhere, focusing on traits not well represented among the
Finnish granites.
[ ~ Archean
:::::::::: 1463 U*Pb '::
REDWINE v~ v
1317±75 (Rb-Sr)~
, 1000 km,
~100 km~:i~ ~
2,; +',~~,~~~~~,~~~~S~~,~~,[ ~;~ ~~~v~~~~S~~~~ 61~
t
tj:i:i i i i i ::::::::::::::::::::::::::::::: ::::::::::::::::::::::::::::::::::
i
s,~¥ ~, :::::::::::::::::::::::::::::::::::::::::::::::::: :::::::::::::::::::::
iiii!i!
= = = (Sn-Be-Cu-Zn)
/~- ", • "'"'"""'"'"':'.'.'.:.
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.... ...~;.. (U-Pb}'~,:.[.:-
..... ~'.'.'.,
/ / ALAND" - -~x ~1b~1540--1570 (U'Pb) ..... :':':':':'''''' "'':':""" :~" [~.~
' lu-e~l'~66-'~76 ~ ~'" veh;~.'.6~o :::: ::::::::::::::::::::::::::::::::::~~" Lake Ladoga
_~-"~ ~ ,-~ . ::::::::::::::::::::::::::::::::::::::::,:::(s~:~n,:
~ t~ x \ ~,_,_,/,/" /
Fig. 2. a Showing the classic Subjotnian (1.54 to 1.65 Ga) rapakivi granite batholiths and
stocks, gabbroic and anorthositic bodies, and diabase dykes of southeastern Fennoscandia
(southern Finland and Russian Karelia). Isotopic ages (in Ma) of the occurrences (Vaasjoki,
1977; Vaasjoki et al., 1988, 1991, 1993; Idman, 1989; Suominen, 1991; Neymark et al., 1994)
and mineralization related to the rapakivi granite plutons are denoted. Modified from R~m6
(1991, fig. 1). b Map showing the Elsonian (1.29 to 1.46 Ga) rapakivi granite--gabbro-
anorthosite intrusions of central Labrador. Also shown are post-Elsonian diabase dykes and
high-level peralkaline granite suites that occur in conjunction with the Elsonian plutons.
Isotopic ages (in Ma) are from Meyers and Emslie (1977), Simmons and Simmons (1987), Hill
and Miller (1990, table 1 and references therein), Ryan et al. (1991), Emslie and Loveridge
(1992), and Birkett et al. (1992). Compiled after Emslie (1980, fig. 3), Halls and Fahrig (1987),
Hill and Miller (1990, fig. 1), and Emslie and Loveridge (1992, fig. 1). The inset illustrates the
location of southeastern Fennoscandia (a) and central Labrador (b) relative to the middle
Proterozoic supercontinent Laurentia-Baltica (Gower et al., 1991, fig. 1)
140 O. T. R/im6 and I. Haapala
(Brazil) where quartz monzonites and quartz monzodiorites intrude biotite granite
(Bettencourt and Dall'Agnol, 1987), and South Greenland where rapakivi-textured
orthopyroxene-amphibole and biotite-amphibole monzonites occur together with
norites (Harrison et al., 1990a). They are also known from the Laramie anorthosite
complex of Wyoming where orthopyroxene and hornblende monzonites are in-
truded by later biotite-hornblende granites (Fountain et al., 1981; Geist et al., 1989)
and from the Salmi batholith of Russian Karelia where monzonites and associated
quartz syenites occur along boundaries between rapakivi granites and gabbronor-
ires in the subsurface southeastern part of the batholith (Amelin et al., 1991;
Neymark et al., 1994).
According to Barker et al. (1975, 1976), the 1.02 Ga Pikes Peak batholith of
Colorado consists of a potassic trend (biotite and biotite-hornblende granites) that
forms 905/ooof the batholith and a minor sodic trend (alkali gabbro to gabbroic
syenite and syenite, quartz syenite, fayalite granite, and riebeckite granite). The 1.32
Ga (Rb-Sr age) Ragunda complex in east-central Sweden (Kornfiilt, 1976) is excep-
tional among the Fennoscan~dian rapakiva granites inasmuch as it contains, besides
approximately equal amounts of mafic and silicic rocks, a substantial volume
of syenite. Minor peralkaline alkali amphibole (riebeckite-arfvedsonite) -bearing
syenite and granite are associated with the syenite. In Brazil, peralkaline granites
are associated with late intrusive phases of rapakivi granite batholiths (Bettencourt
and Dall'Agnol, 1987).
Subalkaline rapakivi granites associated with a major volume of peralkaline
granite have been reported from the Flowers River area in east-central Labrador
(Fig. 2). Collerson (1982) distinguished three coeval felsic plutonic suites: (1)
peralkaline hypersolvus aegirine-alkali amphibole granite and associated syenite
(Rb-Sr whole rock ages 1262 + 7 Ma and 1257 _+ 36 Ma, respectively), (2) subalka-
line hypersolvus fayalite-pyroxene granite (Rb-Sr whole rock age 1261 _+ 87 Ma),
and (3) subalkaline subsolvus hornblende-biotite granite that commonly shows
rapakivi texture (Rb-Sr whole rock age 1262 ± 28 Ma). Hill and Miller (1990) also
describe contemporaneous volcanic rocks (predominantly subalkaline rhyolites) on
top of the peralkaline granite. Brooks in Hill (1982) reports a U - P b zircon age of
1271 _+ 15 Ma for the peralkaline granite; the Flowers River peralkaline suite is thus
slightly younger than the Elsonian (1.29 to 1.46 Ga) AMCG suites of central
Labrador in general (Emslie, 1980; Hill and Miller, 1990).
Reviewing of the middle Proterozoic anorogenic rock associations of central
Labrador, Hill and Miller (1990) list, in addition to the Flowers River suite, a number
of high-level felsic igneous complexes, such as the 1240 Ma ( U - P b age; Birkett et al.,
1992) Strange Lake peralkaline granite hosting significant Z r - Y - N b - B e - R E E
mineralization (Fig. 2b), the 1317_ 75 Ma (Rb-Sr whole rock age) Red Wine
intrusive suite showing both quartz-undersaturated and -oversaturated rocks, the
Upper North River pluton with peraluminous quartz-rich phases, the fluorite-rich
Manvers biotite granite, and the composite (mafic-felsic) Arrowhead pluton includ-
ing metaluminous quartz syenite and alaskite. These complexes are, in any one area,
younger than the spatially associated AMCG suites, but the age difference is variable
(from 300 Ma in northern Grenville Province to less than 50 Ma in central and
northern parts of the Nain Plutonic Suite; see Hill and Miller, 1990, Table 1 and
Fig. 2, and Emslie and Loveridge, 1992). Evidently, more detailed isotopic age data
are needed to constrain the interrelations of the AMCG suites and the peralkaline
high-level suites. Young peralkaline intrusions may turn out to be more common
in the predominantly subalkaline rapakivi granite complexes as more detailed
petrographic data are obtained from them. An example of this are the peralkaline
alkali-feldspar syenite dykes of the Suomenniemi complex (Riim6, 1991).
In many instances, mafic rocks occurring in close spatial association with rapakivi
granites show textural and structural features that unequivocally demonstrate them
to be coeval with the silicic rocks. Further confirmation is provided by isotopic age
determinations.
Gabbroic and anorthositic rocks associated with rapakivi granite complexes are
usually intruded by the silicic rocks. Evidence for these rocks being (roughly) coeval
with the rapakivi granites thus relies mainly on isotopic studies. In Finland where
the interrelations of rapakivi-related mafic and silicic magmas have been studied
lately in considerable detail (e.g., Riim6, 1991; Eklund, 1993; Salonsaari and
Haapala, 1994), field relations suggest that there are mafic dykes both older and
younger than the associated silicic dykes. Occasionally, composite silicic-mafic
dykes occur verifying that both end members were, at least partly, liquid at the same
time at the same place (e.g., Rgtm6, 1989, 1991). In Fig. 3, schematic diagrams
showing the structure of two composite dykes associated with the Suomenniemi
batholith (Fig. 2a) are presented. R~m6 concluded that the sequence of intrusion of
the mafic and silicic components were different in these dykes but that, in both cases,
the two components had coexisted as magmas (see caption of Fig. 3 for details).
It is generally believed to be difficult for two compositionally contrasted magmas
to mix completely and form homogeneous intermediate rocks (see Frost and
Mahood, 1987; Wiebe, 1991). When interaction of mafic and silicic magmas has
occurred the two components are often intermingled to form a hybrid rock in which
the two components are still easily discernible (Fig. 3; see also Wiebe, 1988). If
circumstances were favorable, however, they may have produced an intermediate
hybrid rock for which its mixed origin can only be established by detailed petro-
graphic studies (e.g., Salonsaari and Haapala, 1994).
In general, typical textural features of bimodal (silicic-mafic) mingled and/or
mixed complexes are mafic inclusions with lobed, and occasionally chilled, margins
within a felsic host (e.g., Wiebe, 1980; Harrison et al., 1990b; Ri~m6, 1991; Salonsaari
and Haapala, 1994), net-veined complexes (Wiebe, 1988), alkali feldspar and quartz
xenocrysts within a mafic host (Riim6, 1991; Lindber9 and Eklund, 1992; Salonsaari
and Haapala, 1994), mafic microgranular enclaves (Salonsaari, 1993), quartz pheno-
crysts mantled by amphibole (Eklund et al., 1989; Ri~m6, 1989; Salonsaari and
Haapala, 1994), alkali feldspar phenocrysts with various disequilibrium textures
(Stimac and Wark, 1992), and calcic plagioclase megacrysts within silicic ground-
mass (Haapala, 1989; Lindberg and Eklund, 1992).
One hundred years of Rapakivi Granite 145
~Oi=base ~O~a~-fo,dsparporphy~~Ming,~drock
. . . . . ._. _ o,=odeouot roekgra=to
~ ~ ~ ~ ] feldspar and quartz xenocrysts ]
5 meters
~ Biotiterapakivigra
Biotite-hornblende
mingled rock show- l" ::, ;~q rapakivi granite
6. Geochemistry
In comparison with calc-alkaline granitoid suites, a prominent feature of rapakivi
granite batholiths is their limited mineralogical and compositional variation. For
instance, up to 80~o of the Finnish part of the Wiborg batholith (Vorma, 1976) and
about 70~ of the Wolf River batholith (Anderson and Cullers, 1978) consists of a
largely undifferentiated sequence of rapakivi granite (wiborgite) and related biotite-
hornblende granites. Equally typical of these complexes are, however, volumet-
rically minor occurrences of mafic fayalite (+_pyroxene)-bearing hornblende
granites (e.g., tirilite), various porphyritic or even-grained biotite granites, and
leucocratic, extremely fractionated topaz-bearing microcline-albite granites (Haa-
pala, 1977, 1985; Bettencourt and Dall'Aonol, 1987; Horbe et al., 1991; Riim6, 1991).
A larger compositional range is shown by the AMCG granitoids with their deeper-
level mangeritic members (McLelland and Whitney, 1990; Emslie, 1991).
Excluding the quartz-poor granitoids of the AMCG suites, granites in rapakivi
granite complexes show higher Si, K, F, Rb, Ga, Zr, Hf, Th, U, Zn, and REE (except
Eu), and lower Ca, Mg, A1, P, and Sr abundances than granitic rocks in general
(Vorma, 1976; Haapala, 1977; Anderson, 1983; Emslie, 1991; Riim6, 1991). Features
typical of the entire suite are high Fe/Mg, K/Na, total alkalies, and Zr, as well as
low A1 (Emslie, 1991). The rapakivi granites show the typical compositional features
.~ .~ O
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§ " • • . ~ o ~ _ ,-~~ ~ ~ ~,~ , .~.~,~
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N ~.,l
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2
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~ d o c ~ S c ~ c ; c S d - ~ o c ; d c ~ . . . . odcS~',-,~-~c; o~0o ' ~ c ~ o ' ~ - c ~ ~ '~ ,~ . . . . . . . . . . ~ -;
~ r. =
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i •~ ~ <
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c~ ~ < o o~ o~ o 0~ o . ~ o+ 6
o~.~
148 O. T. R/im6 and I. Haapala
of the Phanerozoic A-type granites and within plate granites (Nurmi and Haapala,
1986; Bettencourt and Dall'Agnol, 1987; Anderson and Bender, 1989; Amelin et al.,
1991; Emslie, 1991; Riim6 and Haapala, 1990). On a global scale, geochemical data
on these rocks are still rather sparse and scattered. Therefore, in the following
emphasis is placed on the classic Finnish rapakivi granites.
70.7~o SiO 2, D.I. 84.9) than the overall average (71.6 +_ 3.4% SiO2, D.I. 86.7). Vorma
(1976) presents an average composition for the Laitila batholith that is more silicic
(72.6 + 2.6~o SiO 2, D.I. 88.3) than the area-weighted mean. The former is biased by
the relatively large number of analyses on felsic late-stage granites that are volumet-
rically minor. Much of the Suomenniemi batholith, on the other hand, consists of
a relatively felsic biotite granite and its hypothetical initial magma composition is
also clearly more silicic (72.3~o SiO 2, D.I. 89.9) than the area-weighted means of the
Laitila and Wiborg batholiths. On the average, the peralkaline granites (72.8 _+ 3.1~o
SiO~, D.I. 90.1) differ from the subalkaline granites in being more leucocratic and
having higher Fe~O~ and N a and lower Mg, Ca, and P contents, whereas the
56 6O 64 68 72 76 80
1.3 I I I I I
c Wolf River
NCNK Laitila batholith o ,, bathofth
1.2 c
o.
Wiborg batholith ~o ~ o
z z c
1.1 O_o~oo~ ~ o o
PERALUMINOUS
1.0
METALUMINOUS
2 C 0 ••~ • •
0.9
2
A
0,8 c
Suomenniemibatholith o*
0.7
13
A K20+Na20
12 &
Suomennierni
batholith
11
Wiborg batholith
10
7 z / Wolf River o
....................... o
6
1.00
FeO* Lait#abatholith ~ g o o°~oo % o
FeO*+MgO • o . ,,o o"*% o % o o
o o oo \
o oo o o
0.95
• "" ,o ° o~ °o %
~ °°~o c ~ , 3 ~ . ~\ o o o
0.90
o o ii
Ao e c° e i/ e
0.85
o River
0,80 AIkah-fe/dsparsyenites(n=7) , o
/ o
t batholith
l • Peralkalinegranites(n=22) i Wiborg batholith
Wiborgbatholith
Suomenniemi
batho/ithSUthmfi~iemi CC
0,75 -
56 60 64 68 72 76 80
SiO2
Fig. 4. Analyses of the Finnish rapakivi granites and related silicic dyke rocks, alkali-feldspar
syenites, and various peralkaline granites plotted in a A/CNK vs. SiO2, b K20 + Na2 O vs.
SiO2, and e FeO*/(FeO* + MgO) vs. SiO2 variation diagrams. Also shown are the area-
weighted mean compositions of the Wiborg and Laitila batholiths (Table 2), initial magma
composition of the Suomenniemi and Wolf River batholiths (Table 2), as well as average
analyses (crosses) of the four main rock types in the Suomenniemi batholith (numbers refer
to the columns in Table 2). A/CNK denotes molecular A1203/(CaO + K20 + Na20) and
Fee* total iron as Fee. Line separating the alkaline and subalkaline fields in (b) is from
Irvine and Baragar (1971)
150 O.T. Rfim6 and I. Haapala
alkali-feldspar syenites (61.6 __ 2.1~ SiO2, D.I. 86.8) have higher F%O 3, Mg, Ca,
Na, and P and lower Si and FeO abundances than the subalkaline granites.
6.2.2 Al-saturation
The Finnish rapakivi granites and silicic dyke rocks straddle the peraluminosity-
metaluminosity boundary (Fig. 4a) and have an average A/CNK (molecular A1203/
[CaO + Na20 + K20]) of 0.99. The area-weighted mean of the Laitila batholith
is slightly oversaturated (A/CNK 1.05) and that of the Wiborg batholith and the
initial magma of the Suomenniemi batholith somewhat undersaturated (A/CNK
0.95 and 0.96, respectively). Rapakivi granites elsewhere also usually plot close to
the peraluminosity-metaluminosity boundary. A few rapakivi-related suites are
more strongly peraluminous with A/CNK around 1.1. This is the case with some of
the Proterozoic anorogenic granites of southwestern U.S.A. (Anderson and Bender,
1989), the rapakivi-textured monzonites of South Greenland (Harrisonet al., 1990a),
and some of the plutons in Mt. Isa Inlier in northwestern Queensland, Australia
(Wyborn et al., 1988). The alkali-feldspar syenites of the Suomenniemi complex are
clearly subaluminous (average A/CNK 0.82) as are the peralkaline granites (average
A/CNK 0.87).
6.2.3 Alkalinity
The Finnish rapakivi granites and related dyke rocks show high contents of alkalies
(Na20 + K20 ranges from 6.4 to 9.9 and averages 8.4) yet none of them is peralka-
Iine. Typical are also high K/Na; these range from 0.86 to 3.8 and average 2.0. In
the alkalies vs. silica diagram (Fig. 4b) they plot almost exclusively in the subalkaline
field, while their agpaitic index (molecular (Na20 + K20)/A1203) varies from 0.58
to 0.97 and averages 0.82. Alkali-enriched yet not peralkaline nature is typical of
many of the rapakivi-related granite associations (e.g., Anderson, 1983, fig. 7). On
the average, the peralkaline granites are slightly more alkalic (Na20 + K20 ranges
from 6.9 to 10.2 and averages 9.2) but only a few of them fall in the alkaline field in
Fig. 4b; the agpaitic index ranges from 0.86 to 1.32 and averages 1.08. By contrast,
the Finnish alkali-feldspar syenites plot distinctly in the alkaline field in Fig. 4b and
show an overall peralkaline character with agpaitic index varying from 0.79 to 1.13
and averaging 0.99.
6.2.4 Fe-enrichment
Fe-enriched nature (i.e., high Fe/Mg) is typical of the Finnish rapakivi granites
and alkali-feldspar syenites (Fig. 4c). For the former, Fe/(Fe + Mg) vary from 0.79
to 1.00 (average 0.92) and for the latter from 0.88 to 0.93 (average 0.91). The
peralkaline granites are even more Fe-enriched: their Fe/(Fe + Mg) vary from 0.90
to 1.00 and average 0.97. The area-weighted means and the Suomenniemi initial
magma composition all have Fe/(Fe + Mg) greater than 0.9 (Table 2, Fig. 4c). Such
high figures have commonly been reported for rapakivi granites worldwide (see
Anderson, 1983; Bettencourt and Dall'Agnol, 1987). The more strongly peralumi-
nous granites of South Greenland (Brown et al., 1992), southwestern U.S.A.
One hundred years of Rapakivi Granite 151
(Anderson and Bender, 1989), and northwestern Queensland (Wyborn et al., 1988)
have lower Fe/(Fe + Mg), generally on the order of 0.75 to 0.85.
1000
IlnitialmagmaoftheSuomenniemi ]
!~!~-'t~'~2,~, b!ahto/Ohti: (La/Yb)N=11.8,Eu/Eu*=0.29~
~ / ~T o ~ p a z - b ~ granit . . . . . . ge.' ]
Fig. 5. Chondrite-normalized
100
rare earth element composi-
tion of the Finnish rapakivi
o
granites and related silicic
0 dyke rocks (as _ 1~ about
/AmreanWeighptedt'
X ~ ° -"() ~ !~;t+,..... ,....... / .......
the average of 33 analyses)
rr
batholith: I ~ )~r. 'l syeniteaverage; compared to that of average
10 (La/Yb)N=8.62 , i ",-'4tI \ (La/Yb)N=8.45,^ alkali-feldspar syenite and
Eu/EE*=0.35 X ~'1~ IEa/Ee+=0.46(n=zjj
I \ \ average topaz-bearing rapa-
Rapakivigranitesendsilicicdyke] kivi granite, area-weighted
V rocks averageof33analyses: I
(La/Yb)N=9.24,Eu/Eu*=0.26 J mean of the Laitila bath-
olith, and the initial magma
I [ I I I I I [ I I i I of the Suomenniemi bath-
La Ce Pr Nd Sm Eu Gd Tb Dy No Er Tm Yb Lu olith (Table 2)
152 O. T. R/im6 and I. Haapala
The late-stage topaz-bearing granites differ from the average rapakivi granite
composition in having higher F (0.39 to 1.53~o, average 0.80~o), Y (59 to 162 ppm,
average 117 ppm), U (7 to 24 ppm, average 12 ppm), Pb (32 to 133 ppm, average 84
ppm), Li (25 to 480 ppm, average 153 ppm), and Ga (20 to 120 ppm, average 48
ppm) abundances and lower contents of Zr (24 to 327 ppm, average 127 ppm), Sr
(< 10 to 100 ppm, average 28 ppm), Ba (10 to 540 ppm, average 183 ppm), and total
REE (average 224 ppm). Characteristic are also very high Rb/Sr, Rb/Ba, and
10000*Ga/A1 (averages 32.7, 10.1, and 6.4, respectively). The topaz-bearing granites
are also less enriched in LREE (average 166 ppm) and show flat REE patterns
(average [La/Yb]N = 1.41) with very pronounced negative Eu anomalies (average
Eu/Eu* = 0.07).
Compared to the silicic rocks, the alkali-feldspar syenites are markedly impov-
erished in F (0.02 to 0.13~o, average 0.06~o) and show higher abundances of Sc (9.5
to 23 ppm, average 15 ppm) and Hf(16 to 30 ppm, average 22 ppm). Also the Rb/Sr,
Rb/Ba, and 10000*Ga/A1 are clearly lower in the alkali-feldspar syenites, averaging
2.6, 0.24, and 2.66, respectively. The peralkaline granites differ from the subalkaline
granites in having distinctly lower Sr (1 to 110 ppm, average 34 ppm), Ba (6 to 671
ppm, average 127 ppm), U (1 to 3 ppm, average 2.3 ppm), Th (6 to 24 ppm, average
15 ppm), and Pb (7 to 31 ppm, average 19 ppm) abundances. On the other hand,
they are strongly enriched in Zn (40 to 660 ppm, average 263 ppm), Zr (100 to 6010
ppm, average 1840 ppm), Be (20 to 75 ppm, average 34 ppm), and REE (La + Yb
averages 429 ppm, whereas for the subalkaline granites their sum is 111 ppm). As
regards fractionation of REE, they are less enriched in LREE than the subalkaline
granites ([La/Yb]N averages 5.04). Compared to the alkali-feldspar syenites, they
have higher F (averages 0.27 vs. 0.06~), Y (226 vs. 99 ppm), and Zr (1840 vs. 582
ppm) abundances and lower contents of Sr (34 vs. 121 ppm) and Ba (127 vs.
1239 ppm).
Many of the trace element characteristics of the Finnish rapakivi granites are
shared by subalkaline rapakivi granite associations elsewhere. Especially typical are
high F and Zr and low Sr abundances, high total REE contents and the LREE-
enriched chondrite-normalized patterns with negative Eu anomalies (see Anderson,
1983; Amelin et al., 1991; EmsIie, 1991; Horbe et al., 1991; Riim6 et al., 1992).
AI • PERALKALINE
1.0 SUBALKALINE batho#th 10
a
0.8 "M-,I-, 8 o~f\,, o o oO o OGT
and S-type l° ° "
0.6 gramtes I ' 'on/t/2olmagma
0.4 • ! 1
30 100 Zr+Nb+Ce+Y (ppm) lOOO 300o
10000*Ga/AI lO
400 2000
.,... , . " "
1000
WPG ,.'" syn-COLG WPG
-n
lOO ~T
:L~:' u~@l • "0
¢3. • ~ ~c~.( Suomenniemi/
' ~ batholith
100
z
lO
VAG o ~
d 10
i I I Illll I I i I I II 7
10 100 1000 20 100 1000
g (ppm) Y+Nb (ppm)
Fig. 6. Analyses of the Finnish rapakivi granites and related silicic dyke rocks (open circles),
alkali-feldspar syenites (triangles), and various peralkaline granites (closed circles) plotted
in a agpaitic index (molecular (K20 + NazO)/AlzO3) vs. 10000*Ga/A1 and b (except
peralkaline granites) (K20 + Na/O)/CaO vs. Zr + Nb + Ce + Y diagrams of Whalen et al.
(1987), and c Nb vs. Y and d Rb vs. Y + Nb tectonomagmatic discrimination diagrams of
Pearce et al. (1984). FG denotes fractionated felsic granites, OGT unfractionated M-, I-,
and S-type granites, ORG ocean ridge granites, VAG volcanic and granites, syn-COLG
syncollision granites, and WPG within plate granites. Composition of the initial magma of
the Suomenniemi batholith is also shown
7. Conditions of crystallization
The mode of occurrence and general textural characteristics indicate that the
rapakivi granites are usually epizonal intrusives, but many of the rapakivi complexes
also contain subvolcanic and volcanic phases. The scarcity of source rock restites
is indicative of high magma temperature. The normative composition of undifferen-
tiated rapakivi granites with a high orthoclase component is compatible with
generation of the magmas in a HzO-deficient environment at pressures of 7 to 10
kb, corresponding to a depth of 25 to 36 km (Anderson and Cullers, 1978; Ri#n6,
1991). This interpretation is based on old and partly preliminary experimental data
(see Luth, 1969), but recent more detailed studies of crystallization of granitic melts
with variable activities of H 2 0 (Johannes and Holtz, 1990) confirm the earlier data.
The bulk chemical composition of the most strongly fractionated intrusive phases
register conditions at the epizonal to volcanic levels of emplacement. The earliest
154 O. T. Rfim6 and I. Haapala
mineral phases are intratelluric megacrysts (possibly accompanied by minor restitic
material), whereas the groundmass of porphyritic granites and quartz-feldspar
porphyry dykes represents rapid in situ crystallization at the level of emplacement.
The rarity of pegmatites and miarolitic cavities and the occurrence of biotite and
amphibole as anhedral grains filling the interstices between quartz and feldspar
crystals indicate that the early and main intrusive phases crystallized from H20-
undersaturated magmas. Only in the latest intrusive phases is there good petro-
graphic evidence (miarolitic cavities, pegmatite pockets and veins, hydrothermal
alteration and mineralization, various subsolidus reactions) for a separate fluid
phase.
Various experimentally calibrated methods have been developed to determine,
utilizing coexisting mineral assemblages, the intensive parameters of crystallization
(T, P, fn2o, and fo2) of granitic magmas. The main difficulty in applying these
methods for rapakivi granites is that the rapakivi granites usually consist of dis-
equilibrium mineral assemblages (minerals crystallized in different generations,
amphibole and biotite commonly later than feldspars and early quartz, etc.). More-
over, the minerals have probably been partially reequilibrated during the slow
cooling under plutonic conditions, and subsolidus reactions may have markedly
changed the mineral compositions. Thus, methods based on the composition of
coexisting minerals must be applied with great care. In favorable circumstances,
however, they can be used to place constraints on the crystallization conditions of
the rapakivi granites.
Because of subsolidus reequilibration, the two-feldspar geothermometer (Stor-
mer, 1975; Fuhrman and Lindsley, 1988) can be used to obtain only minimum
temperatures of crystallization. Applying the diagrams of Stormer (1975), Haapala
(1977) estimated a temperature of 750°C at 2 kb for the fayalite-biotite-hornblende
granite of the Eurajoki stock, southwestern Finland. For the wiborgites of the
Wiborg batholith, two-feldspar temperatures ranging from 750°C (core of the
ovoids) to 650 to 580°C (margin of the ovoids) have been reported (Lintala et al.,
1991; Rundquist et al., 1991). The association quartz-fayalite(-magnetite) in some
rapakivi granites of Finland suggests low oxygen fugacity during crystallization.
Wones (1980) published two-feldspar temperatures of 775 to 550°C for the biotite
rapakivi granite of the Lucerne pluton, Maine, obtaining 'the best estimation of the
feldspar mantling effect' at about 675°C at 1 kb. Correspondingly, Ayuso (1984)
listed a large temperature range (800 to 450°C) for the granites of the Bottle Lake
complex, Maine, and, from the intersection of biotite stability curves and granite
minimum melting curve, estimated the emplacement conditions as 780 to 720°C, 1.8
to 1 kb, and fo2 between the N i - N i O and hematite-magnetite buffer curves.
Anderson and Cullers (1978) and Anderson (1980) used whole rock chemical
compositions and various mineral assemblages (combinations of pyroxenes, fayalite,
hornblende, biotite, magnetite, ilmenite, plagioclase, alkali feldspar, and quartz) to
estimate the intensive parameters of crystallization of monzonites (mangerites) and
granites of the Wolf River batholith, Wisconsin. Anderson (1980) concluded that
the monzonites equilibrated at confining pressures of 5.6 to 8.7 kb (21 to 32 km, i.e.,
at the same depth where the granite magmas were formed by crustal fusion), at
temperatures of 900 to 1000°C and fo~ slightly below the quartz-fayalite magnetite
buffer. Combining various geothermometers and oxygen barometers, Anderson
(1980, 1983) showed that the granites of the Wolf River batholith finally crystallized
One hundred years of Rapakivi Granite 155
at pressures of 0.5 to 1.0 kb (less than 3.8 km), temperatures of 640 to 790°C and fo2
subparallel to and slightly below the quartz-fayalite-magnetite buffer curve.
Fig. 7. Photograph of wiborgite showing, beside mantled alkali feldspar ovoids, a granitic
inclusion rimmed by plagioclase. Erratic boulder from the Wiborg rapakivi granite area,
southeastern Finland. Found by Atso Vorma in Inkoo, Deger6, 20 km west of the Obbn~is
rapakivi granite pluton (Fig. 2a) (Mineralogical Museum of the Geological Survey of
Finland)
156 O. T. Rfim6 and I. Haapala
partly by the radial intergrowth. Not infrequently, the ovoids contain mineral
inclusions (plagioclase, quartz, hornblende, biotite, zircon) in one or several concen-
tric zones. In addition to, or instead of, the ordinary mantles, plagioclase may form
one or several continuous or discontinuous zones inside the alkali feldspar mega-
crysts. Concave quartz inclusions, often associated with plagioclase, are common
within the ovoids. The composition of the alkali feldspar (perthite) is commonly
within the range Ors0_80Abz0_50An0. 5_4 and plagioclase within the range An10-40
(Vorma, 1971; Emslie, 1991; Stimac and Wark, 1992). Mantled and unmantled ovoids
with different internal textures often occur side by side in the same outcrop (e.g.,
Ryan, 1991). Occasionally, rounded granitic enclaves mantled by plagioclase are
found in wiborgite (Wahl, 1925; Vorma, 1976; Fig. 7).
The plagioclase mantle may consist of a single oligoclase-andesine crystal in
optical continuity with the albite lamellae of the perthite ovoid, or of several differ-
ently oriented plagioclase grains. Plagioclase inclusions are common in the outer
part of the ovoids, adjacent to the mantle, and often they have the same orientation
as the mantle and perthite albite, Patchy compositional variation in characteristic
of the plagioclase mantles in some dark wiborgites of the Wiborg batholith. The
mantles may consist of plagioclase only, but often they contain inclusions of
drop quartz or quartz vermicules, sometimes also other minerals. In the hybrid
hornblende-rich granite of the Jaala-Iitti complex, the rounded alkali feldspar
megacrysts are mantled by a micrographic plagioclase-quartz intergrowth (Sa-
lonsaari and Haapala, 1994), differing markedly from the normal plagioclase man-
tles on alkali feldspar ovoids in wiborgites. Occasionally, there are broken alkali
feldspar ovoids where the plagioclase mantles are thinner or absent on the broken
surfaces.
Several rapakivi studies interpreted the ovoidal shape of the alkali feldspar
megacrysts as being due to continuous crystallization from high viscosity melt rather
than to resorption. Sederholm (1891, 1928) writes: 'Every thought of resorption in
so great a measure and with such a regularity appears a priori untenable. Moreover,
neither the outer ring, nor the inner rings ever show any cavities that might be
ascribed to corrosion, but have always regular shapes. The ovoidal shape seems to
have existed during all the time of the growth of the crystal'. Others (e.g., Hibbard,
1981; NekvasiI, 1991; Stimac and Wark, 1992) have explained the ovoidal shape as
a product of magmatic resorption. In detail, the boundary between the mantle and
ovoid is often quite irregular and corrosion or replacement reactions are, indeed, in
many cases obvious.
Sederholm (1928) also explained the plagioclase mantles by crystallization from
a viscous melt. Because of slow diffusion, local decrease of potassium and increase
of calcium and sodium concentrations around the growing alkali feldspar ovoids
led to the crystallization of the plagioclase rims. Another interesting old model is
that of Popoff (1897) who suggested that sinking of newly formed alkali feldspar
crystals to levels of higher temperature and different composition in the magma
chamber caused partial remelting of the crystals and their coating by plagioclase
and other minerals. Convective circulation in the magma chamber could lead to the
development of multiple mantles; it could also explain the occurrence of megacrysts
of different size, form, and internal texture in many rapakivi granites.
Exsolution of albitic plagioclase from the alkali feldspar and its migration to the
grain boundaries has been suggested as one mechanism for formation of the rapakivi
One hundred years of Rapakivi Granite 157
texture (Gates, 1953; Dempster et al., 1991). Although exsolution can well produce
interstitial albite and myrmekite rims between two alkali feldspar grains (e.g.,
Haapala, 1977), it is not likely to produce oligoclase-andesine shells around alkali
feldspar ovoids or multiple mantles or inclusion zones, not to mention plagioclase
mantles around granitic enclaves (Fig. 7).
Several authors have suggested that the mantled ovoids are formed as a result
of magma mixing or assimilation (Volborth, 1973; Hibbard, 1981; Bussy, 1990;
Stimac and Wark, 1992). There is good field and experimental (Wark and Stimac,
1992) evidence that this mechanism, whereby alkali feldspar crystals are brought
into a mafic magma, can produce plagioclase-rich shells around corroded alkali
feldspar grains. Repeated mixing could explain the multiple zones of plagioclase and
other minerals. It is, however, difficult to understand how such huge volumes of
homogeneous wiborgite as in the Wiborg batholith could be formed by magma
mixing alone.
Stability changes related to pressure decrease in the ascending HzO-
undersaturated granitic magma have been suggested to be the reason for the
formation of the plagioclase-mantled ovoids (Whitney, 1975; Nekvasil, 1991). Mod-
eling the crystallization of an alkali feldspar- and plagioclase-saturated and HzO-
undersaturated granitic magma, Nekvasil (1991) suggested that decompression of
the ascending and slowly cooling (5-10°C/kb) magma causes partial dissolution of
the alkali feldspar megacrysts and quartz crystals, but allows crystallization of
plagioclase leading to the formation of mantled ovoids. Some authors (e.g., Cherry
and Trembath, 1978; Abbott, 1978) have suggested that degassing related to the
ascent of the granitic magma would increase the stability field of plagioclase and
cause rapid crystallization producing mantled alkali feldspar megacrysts. Nekvasil
(1991) points out that H20-saturation and degassing prior to or during ascent of
the magma would result in rapid crystallization of the matrix (pressure quench
phenomenon) and would not be accompanied by partial resorption of either alkali
feldspar or quartz.
It is probable that several mechanisms can produce plagioclase rims around
alkali feldspar megacrysts. Small changes in physical conditions (P, T, a,2o) and/or
in chemical composition (increase in calcium and mafic components) change the
stability fields of feldspars so that plagioclase becomes the only crystallizing phase
and nucleates on the alkali feldspar megacrysts. Rapid decrease of pressure and
magma mixing or other changes in composition (accumulation of crystals in compo-
sitionally stratified magma chambers) can also explain the porphyritic texture and
corrosion of alkali feldspar and quartz crystals. We consider these mechanisms the
most cogent in explaining the origin of the rapakivi texture. However, many petro-
logical questions still remain and detailed petrographic and mineralogic studies are
needed to constrain the conditions of crystallization and to understand which
mechanism in each case is the most realistic one.
9. Petrogenesis
The magmatic origin of the rapakivi granites is considered axiomatic today, yet in
a number of relatively recent papers (e.g., Backlund, 1938; Sudovikov, 1967) trans-
formistic views are entertained. Sharp intrusive contacts of rapakivi granite plutons,
ubiquitous magmatic textures and mineral assemblages, as well as spatially and
158 O. T. Rfim6 and I. Haapala
temporally associated subvolcanic and volcanic suites render such views very diffi-
cult to defend. Regarding the petrogenesis of rapakivi granites, current topics of
debate cover the source of the silicic magmas (mantle and/or crust?), composition
and petrology of their protoliths, as well as processes that control their magmatic
evolution (partial melting, fractional crystallization, magma mixing etc.). Under-
standing these items in detail will have an important bearing on the study of the
evolution of the continental crust especially in the Proterozoic. Isotopic and geo-
chemical data on rapakivi granites and related silicic and mafic rocks are summa-
rized below, and the models advanced to explain their genetic interrelations, the
nature of their protoliths, and magmatic evolution are discussed.
9.1 Isotopic constraints on rhe origin of rapakivi granites and related rocks
9.1.1 Sr isotopes
Sr isotopic data are available for rapakivi granites and related silicic rocks from
numerous North American occurrences, as well as for rapakivi granites of Vene-
zuela, Brazil, South Greenland, Finland, Sweden, Russian Karelia, China, and Aus-
tralia. These data and the isotopic evolution of mantle and continental crust are
plotted in a 87Sr/86Sri vs. age diagram in Fig. 8. The Sr isotopic data on North
American rapakivi granite suites comprise a total of 64 initial 87Sr-86Sr ratios that
range from 0.7000 to 0.7488 and average at 0.7087 +_ 0.0095 (lo). About three
quarters of these fall above the average subcontinental mantle evolution, whereas
most of the remainder plot between the two mantle evolution lines. The two data
points below the evolution of the Rb-depleted mantle are somewhat uncertain due
to possible disturbance of the Rb-Sr system (Anderson, 1983). For other areas, the
data are few and plot, excluding the very low initial ratio (0.7004 ___0.0019) of the
Venezuelan Parguaza rapakivi granite (Gaudette et al., 1978) and the relatively low
initial ratio (0.7024 _ 0.0020) of the rapakivi-textured monzonites of South Green-
land (Dempster et ai., 1991), clearly above the evolution line of the average sub-
continental mantle. For the classic Finnish rapakivi granites, only one poorly-
constrained initial ratio (0.706 _ 0.003) is available (Suominen, 1991).
It should be noted that comparison of the data points with the evolution depicted
for mantle and crust should be considered only tentative, because the Rb-Sr isotopic
system is easily affected by open-system processes. However, in terms of the crude
models of Fig. 8, the bulk of the Sr isotopic data favor a crustal origin for the rapakivi
and related granites, but variable amounts of mantle contribution in some of the
suites can not be ruled out. This could be the case for the 1.55 Ga Parguaza rapakivi
granite (Gaudette et at., 1978).
9.1.2 Nd isotopes
Nd isotopic data are available especially for the Fennoscandian and North Ameri-
can rapakivi granites, and also for the suites in South Greenland, China, and
Australia. These data (a total of 94 analyses) are shown in an end VS. age diagram in
Fig. 9. Compared to the Sr evolution diagram in Fig. 8, Fig. 9 constrains the origin
of the various granites more unequivocally. For example, the diagram distinguishes
between granites within Proterozoic crust and those with which Archean crust is
associated. The Finnish rapakivi granites plot within the evolution of the 1.9 Ga
One hundred years of Rapakivi Granite 159
0.715
• Fennoscandia(U~Pbzircon)
7
,q /
• North America (U-Pb zircon) 0.713
0.705 - '
/ cru,,
o "+ 0.703
i I I I I
I
I 0,699
3.5 3 2.5 2 1.5 1 0.5
Age (Ga)
Fig. 8. Strontium isotopic composition (77 data points) of rapakivi granites from Fennoscan-
dia (Kornfgllt, 1976; Welin and Lundqvist, 1984; Halliday et al., 1988; Suominen, 1991; Neymark
et al., 1994), North America (Heath and Fairbairn, 1969; Bickford and Mose, 1975; Van
Schmus et al., 1975; Barker et al., 1976; Emslie, 1978; Anderson, 1983, and references therein;
Geist et al., 1989; Emslie and Loveridge, 1992), South Greenland (Dempster et al., 1991),
South America (Gaudette et al., 1978; Macambira et al., 1987; Janasi and Ulbrich, 1991),
China (Yu et al., 1994), and Australia (Wyborn et al., 1988) plotted in 878r/86Sri vs. age
diagram. Also shown are the evolution lines for average subcontinental mantle (ending at a
present-day 878r/86Sr of 0.704; Faure, 1986) and Rb-depleted mantle (present-day 878r/a6Sr
of 0.702), both starting at BABI (Basaltic Achondrite Best Initial; Papanastassiou and
Wasserburg, 1969) composition (878r/86Sr = 0.699) 4.7 Ga ago. In addition, hypothetical
evolution lines for Sr extracted from the average subcontinental mantle to form continental
crust at 3.0 and 1.9 Ga are shown: the lines with steep slopes represent typical continental
crust with a Rb/Sr of 0.15, the lines with gentle slopes denote lower continental crust with
a smaller Rb/Sr of 0.04. Isotopic methods for the ages used to calculate the initial 878r-S6Sr
ratios are indicated
crust, whereas the Russian Karelian rapakivi granites that occur along the contact
between Proterozoic and Archean provinces (see Fig. 2a), fall clearly below the
evolution of the 1.9 Ga crust. This relationship appears to hold also for the N o r t h
American granites, excluding granitic plutons associated with the Laramie anortho-
site complex that occurs on the flank of the Archean W y o m i n g Province (Geist et
al., 1989, 1990). These granites show initial N d isotopic compositions that conform
to the long-term evolution of an early to middle Proterozoic protolith, and led Geist
et al. (1989) to conclude that the contact between the W y o m i n g Province and
surrounding Proterozoic crust dips away from the Laramie complex and Archean
material was thus not available in the source of the granites. It is also worth noting
that the Finnish and Russian Karelian rapakivi granites do not differ m u c h from
each other in terms of their initial Sr isotopic composition (Fig. 8), even though their
end values are very different.
The majority of data points in Fig. 9 plot clearly below the depleted mantle
evolution line. Samples with N d isot'opic ratios indicating p r o n o u n c e d long-term
160 O.T. R/im6 and I. Haapala
+8
+4
Depleted Mantle
~'Na
, h, , .,8
3.5 3 2.5 2 1 .S 1 0.5
Age (Ga)
Fig. 9. Neodymium isotopic composition (94 data points) of rapakivi granites from Fenno-
scandia (Rgtm6, 1991; Neymark et al., 1994), North America (DePaolo, 1981; Nelson and
DePaolo, 1985; Bennett and DePaolo, 1987; Geist et al., 1989, 1990; EmsIie and Loveridge,
1992), South Greenland (Patchett and Bridgwater, 1984), China (R~m6 et al., 1992), and
Australia (Wyborn et al., 1988) plotted in eNa VS. age diagram. Also depicted is the evolution
of LREE-depleted mantle (DePaolo, 1981) and Chondritic Uniform Reservoir (CHUR,
DePaolo and Wasserbur9, 1976), as well as that of post-Archean average Australian Shale
(PAAS) denoting Archean crust separated from the depleted mantle 3.0 Ga ago (cf. Patchett
and Bridgwater, 1984). The vertical bar at center illustrates the initial composition of the 1.9
Ga Svecofennian crust of southern Finland with ~Nd values ranging from -- 1.2 to + 4.4
(Huhma, 1986; Patchett and Kouvo, 1986), while the two arrows constrain its time-
integrated evolution. Age of the crust hosting the various rapakivi granite occurrences is
indicated
9.1.3 Pb isotopes
Detailed Pb isotopic data are currently available for the Finnish and Russian
Karelian rapakivi granites. These are plotted, together with scattered analyses on
One hundred years of Rapakivi Granite 161
15.9
m • • X
Average Crustal Lead ~m x
15.7
\
15.5
tl. Plumbotectonics / / ~ -- --
g Model Mantle ~ ~ o Fennoscandia(feldspar)
,~ 15.3 I
/ / / . . o=o
hA=.r
.(fo,dopoO
15.1 /A! \ x=o=ho,.o,.od(
ol.r,*l
lie °~B'- Plumbotectonics o China(feldspar) ,
// ModelLowerCrust "Chi.a(wholerock)
the suites of South Greenland, North America, and China, in a 2°Tpb/2°4pb vs.
2°6pb/2°4pb diagram in Fig. 10. Fennoscandian rapakivi granite whole rocks and
feldspar fractions fall into two distinct groups. The Finnish data (as well as the few
analyses from North America and South Greenland) swarm around and along the
continuation of the average crustal Pb growth curve, while the Russian Karelian
data plot considerably below mantle evolution, close to the model lower crust
growth curve. The latter is true also for the Chinese samples. This bimodality of the
data is in agreement with the nature of the crustal environments where the com-
plexes occur: those within Proterozoic domains follow the higher long-term U/Pb
evolution, those associated with Archean crustal domains are characterized by
retarded Pb isotopic evolution.
9 . 1 . 4 0 and H isotopes
Oxygen isotopic data on rapakivi granites are relatively few. Barker et al. (1976)
reported 6180 values ranging from + 7.7 to + 9.5%0 for the silicic rocks of the Pikes
Peak batholith of Colorado, and considered these as indicative of assimilation of
country rocks with somewhat higher 6180 values than that is usually observed for
magmatic rocks (cf. Taylor and Sheppard, 1986) For the Qernertoq granite of South
Greenland, Dempster et al. (1991) presented relatively high 618 0 values for feldspar
(+ 7 to + 11.5%o) and biotite (+ 4.6 to + 8.1%o) fractions, concluding that the rocks
were not subsequently affected by meteoric-hydrothermal systems. Relatively high
162 O. T. R/im6 and k Haapala
6180 vMues (+8.5 to + t0.8%o) were reported for the Wiborg batholith by Hoefs
and Epstein (1969).
For hydrogen isotopes, 6 D values reported for whole rock samples range from
- 1 2 0 to -86%0 (Pikes Peak batholith, Barker et al., 1976), for feldspar fractions
from - 1 0 5 to -56%0 (Qernertoq granite, Dempster et al., 1991), for biotite from
- 9 6 to -54%0 (Qernertoq granite, Dempster et al., 1991) and -81.1 to -65.7%0
(Finnish rapakivi granites, Kuroda et al., 1978), and for hornblende from -82.6 to
-62.7 (Qernertoq granite, Dempster et al., 1991) and - 1 1 9 to - 1 0 0 (Finnish
rapakivi granites, Kuroda et al., 1978). These 6D values fall in the lower part and
somewhat below the range of 6D values encountered for most igneous rocks (cf.
Taylor and Sheppard, 1986) and are suggestive of only minor, if any, meteoric-
hydrothermal alteration. Kuroda et al. (1978) noted that the large difference in 6D
values between hornblende and biotite in the Finnish rapakivi granites is indicative
of a H20-poor magma.
9.1.5 Isotopic characteristics of the mafic rocks associated with rapakivi granites
Isotopic studies have been carried out on the mafic rocks associated with rapakivi
granites mainly in North America and Fennoscandia. Papers on North American
occurrences deal primarily with anorthositic and gabbroic rocks of the Grenville,
Churchill, and Nain Provinces (Heath and Fairbairn, !969; Emslie, 1978, and refer-
ences therein; Patchett et al., 1981; Basu and Pettingill, 1983; Anderson, 1983, and
references therein; Ashwal et al., 1986; Olson, 1992) but some data also exist on the
Laramie complex in Wyoming (Geist et al., 1990) and the Pikes Peak batholith in
Colorado (Barker et al., 1976). Isotopic data on the mafic rocks associated with the
Fennoscandian rapakivi granites are found in Welin and Lundqvist (1984), Rgtm6
(1991), Suominen (1991), and Neymark et al. (1994).
Initial 8~Sr-86Sr ratios of the mafic rocks associated with rapakivi granites are
generally on the order of 0.703 to 0.705, in line with their predicted mantle origin.
Mafic rocks occurring in complexes situated within early Proterozoic crust show
initial Nd isotopic compositions that differ marginally from those of the associated
silicic rocks. For instance, in southeastern Finland the average end (1.64 Ga) value
of 19 mafic rocks (anorthosite to gabbro, diabase dykes) is - 0 . 2 +_ 0.7 (la), whereas
the average end value of 22 silicic rocks is - 1.4 _+ 0.6 (la) (Riim6, 1991). Comparable
differences have been measured for the 1.75 Ga old rapakivi-textured monzonites
and associated norites of South Greenland (Patchett and Bridgwater, 1984). The
rapakivi-age diabase dykes of southeastern Finland show end values from -- 1.2 to
+ 1.6 (Riim6, 1991, fig. 33); these correlate positively with the fractionation index
(e.g., Mg/Fe) of the dykes and can be accounted for by combined assimilation-
fractional crystallization processes. Initial end values ofmafic rocks from complexes
associated with Archean domains are clearly more negative. For instance, the mafic
rocks of the 1.45 Ga Harp Lake complex intruding Archean rocks of the Churchill
and Nain Provinces have more negative initial end values (averaging --4.0) than
rocks from Mealy Mountains complex (averaging + 2.6 at 1.65 Ga) situated within
the Proterozoic Grenville Province (Ashwal et al., 1986) More negative still are the
initial (1.56 Ga) end values of the gabbroic and anorthositic rocks of the Salmi
batholith in Russian Karelia (Neymark et ak, 1994). They range from - 8.2 to - 6.5
and are indistinguishable from those of the granites of the batholith.
One hundred years of Rapakivi Granite 163
9.1.6 Comments
The Nd, Sr, and Pb isotopic data available for rapakivi granites suggest a crustal
origin for most of them. The data also demonstrate the sensitivity with which these
rocks reflect the isotopic composition of their source. This is exceptionally clearly
shown by the very low 2°Tpb-z°4Pb and 2°6pb-2°gpb ratios of the Russian
Karelian and Chinese rapakivi granites (Fig. 10), explained as indicative of an
Archean lower crustal source component with a very low long-term U/Pb (Rgtm6,
1991; Neymark et al., 1994; Riim6 et al., 1993). The initial Sr isotopic composition
of the mafic rocks of the rapakivi granite association indicate a mantle source for
these rocks. The relatively radiogenic Pb isotopic compositions ofmafic rocks within
complexes in Proterozoic crust and the unradiogenic compositions of those asso-
ciated with Archean domains, as well as the unradiogenic Nd isotopic compositions
are not directly attributable to depleted mantle domains, but need to be explained
either by crustal contamination (e.g., Ashwal et al., 1986; Rfim6, 1991) or by invoking
enriched mantle sources (cf. Hamilton and Morse, 1988; Neymark et al., 1994).
~ EMI B.
\ \
\
\,
.ornb,ende gran,te B,ot, e hornblende gran, e Biotite gran,te Topaz beariog granite
m Ftornblende-cljnopyroxene-fayalitgranite
e [~ Alkali-feldsparsyenitedyke ~ Diabasedyke
~ Quartz-feldsparporphyrydyke ~ Silicic-basiccompositedyke ~ Gabbro-anorthositebody
Fig. 11. Simplified geological map of the Suomenniemirapakivi granite batholith, southeast-
ern Finland. The widths of the dyke rocks are exaggerated. Modified from Riim6 (1991,
appendix 4)
168 O. T. R/im6 and ~. Haapala
tion of a bimodal system is likely only if the compositional difference of the end
members is less than 10~ SiO2, or if the mass fraction of the mafic component is
greater than 0.5. Sparks and Marshall (1986) note further that complete hybridiza-
tion is feasible only if the end members behave as liquids at the same temperature,
and that when the proportion of the silicic magma is large, complete hybridization
can occur with evolved (Fe-rich) mafic magmas only.
The interrelations of silicic and mafic magmas in some of the bimodal systems
of the Finnish rapakivi granite complexes contour with these experimental results.
In the two composite dykes described in Fig. 3, more mingling (and mixing) of the
end members is observed in the dyke showing the greater proportion of the mafic
component (Fig. 3a), and, on the other hand, more complete mixing was presumably
prevented by the large compositional gap between diabase and quartz-feldspar
porphyry ( > 2 0 ~ SiO2; Ram;C, 1991). In contrast, in the Jaala-Iitti complex that
shows more advanced mixing of comparable end members, interaction of the
components probably took place deeper in the crust (Salonsaari and Haapala, 1994)
where there was a large reservoir ofmafic magma continuously available and where
chilling of the mafic magma against the silicic magma was not so efficient as in the
upper (cooler) parts of the crust. Certain disequilibrium features in the more mafic
granite phases of the Wiborg batholith and the/~land batholith (Eklund et al., 1994),
e.g., calcic plagioclase phenocrysts, also suggest that mixing of mafic and silicic
magmas may have been involved in their evolution. It is, however, also possible that
such calcic plagioclase grains are of restitic origin.
Neymark et al., 1994), North American (Emstie, 1978; Geist et al., 1989), Siberian
(Latin and Neymark, 1992), and Amazonian (Dall'Agnol et al., 1994) rapakivi com-
plexes occur in Archean crust but nevertheless close to Proterozoic crustal provinces
(Fig. 1). An exception to this is the 1.67 Ga Shachang rapakivi granite near Beijing;
it occurs within the Archean Sino-Korean craton and is not known to be associated
with early Proterozoic orogenic belts (Riim6 et al., 1993). In general, early Proter-
ozoic crust seems to have been necessary for the formation of most Proterozoic
rapakivi granite occurrences, implying that some causal relations between early
Proterozoic orogenic belts and rapakivi granite suites may exist (HaapaIa and Ri~m6,
1990, 1992).
On a global scale, the Proterozoic rapakivi granite complexes typically occur in
metamorphic terranes that were formed a few hundred Ma prior to granite emplace-
ment. For example, the Finnish rapakivi granites are 200 to 350 Ma younger that
the Svecofennian crust (Vaasjokiet al., 1991; Haapala and Riim6, 1992), the rapakivi
granites of the midcontinental U.S.A. are 100 to 250 Ma younger than their orogenic
host (Van Schrnus et al., 1987), and the rapakivi granites of the Mt. Isa Inlier in
northeastern Australia postdate their early Proterozoic basement by about 150 Ma
(McCulloch, 1987; Wyborn et al., 1988). Accordingly, if anorogenic rocks are defined
as those emplaced >100 Ma after orogenic events (Condie, 1991), most of the
rapakivi granites fall in this category. An exception to this are the rapakivi-textured
monzonites of South Greenland. According to Gulson and Krogh (1975) the
Ketilidian metamorphic crust of South Greenland was formed only about 50 Ma
before the intrusion of these monzonites. Harrison et al. (1990a), Dempster et al.
(1991), and Brown et al. (1992) argued that the peak of metamorphism was even
closer to the ages of the monzonites and interpret their emplacement as synorogenic,
having occurred along ductile extensional shear zones. Windley (1991), by analogy
to the Himalayan orogenic belt, interpreted the rapakivi granites of South Green-
land as having been emplaced within thrust-thickened crust. This was considered
unlikely by Brown et al. (1992) who favored a back-arc environment instead.
Although the anorogenic origin of rapakivi granites seems favored, the ultimate
causes that produced most of these rocks during a fairly restricted time interval in
the Proterozoic are only vaguely understood. The profuse nature of this magmatism
during the Proterozoic has resulted in the concept of a single event that is unique
in the geological history, For example, Bridgwater and Windley (1973) suggested
that the emplacement of these rocks was due to global-scale mantle activity and
crustal rifting and coined the expression 'anorthosite event'. Later, Windley (1989)
considered the rapakivi granites of northwestern North America as early manifesta-
tions of the Grenvillian Wilson cycle with an overall duration of 500 Ma. Focusing
on the crust-upper mantle system, Anderson and Bender (1989) formulated a crustal
overturn model and related the genesis of the anorogenic granites to chemical
instability of the newly generated and vertically undifferentiated juvenile crust-
mantle system, and suggested that the unstable setting will eventually result in
considerable crustal reorganization leading to the emplacement of anatectic granitic
magmas within the upper parts of the juvenile crust. In line with this, Haapala and
Riim6 (1992) suggested that, regarding the Fennoscandian rapakivi granites, the
Svecofennian orogeny may have resulted in unstable domains in the subcontinental
mantle (e.g., late relics of subducted oceanic crust) that may have contributed to the
onset of melting in the upper mantle and the subsequent crustal anatexis. This model
One hundred years of Rapakivi Granite 173
11. Conclusions
The numerous rapakivi plutons in Precambrian cratonic areas in different parts
of the world show that rapakivi magmatism has played an important role in the
evolution of the Proterozoic continental crust. Although relevant information on
the rapakivi granites is still fragmentary and each rapakivi pluton has its own special
character, generalized conclusions regarding the age, geotectonic setting, magmatic
association, petrography, geochemistry, metallogeny (Haapala, 1995), and petro-
genesis of the rapakivi granites can be made.
(1) Most of the rapakivi granites are early to middle Proterozoic (mainly 1.0 to
1.75 Ga) but Archean (2.8 Ga), late Proterozoic (0.57 to 0.59 Ga), and Phaner-
ozoic (0.05 to 0.4 Ga) occurrences are also known. The rapakivi granites in the
Aldan shield (Siberia) are 1.7 to 1.9 Ga old, those in the Ukraine and the
rapakivi-textured monzonites of South Greenland are dated at about 1.75 Ga.
1.5 to 1.7 Ga rapakivi granites are known from southeastern Fennoscandia,
central Labrador and the Grenville Province, Venezuela, Amazonas (Brazil),
northern and southern Australia, and China. The ages of the rapakivi granites
and related anorogenic granites of the Trans-North American belt extending
from Labrador to southern California are between 1.0 to 1.46 Ga, and comprise
three groups: 1.02 to 1.08, 1.34 to 1.41, and 1.41 to 1.49 Ga. In Rond6nia,
Amazonian Craton, the ages of the rapakivi granites range from 0.95 to 1.4 Ga
(Rb-Sr age groups 0.95 to 1.05 and 1.18 to 1.4 Ga). Typically, rapakivi granites
intrude 0.1 to 0.35 Ga older early Proterozoic metamorphic crust; in a few cases
Archean crust. An exception are the rapakivi monzonites of South Greenland
that are < 0.05 Ga younger than the surrounding orogenic province.
(2) Graben structures and swarms of subparallel diabase dykes indicate exten-
sional setting during the emplacement of the rapakivi granites. Typically, the
rapakivi plutons are epizonal or subvolcanic intrusions and range from small
stocks to huge batholiths (up to 40,000 km2). The plutons are often zoned
(centered plutons or ring complexes) suggesting a cauldron subsidence em-
placement mechanism. Seismic soundings and gravimetric models indicate that
the rapakivi batholiths of southeastern Fennoscandia are subhorizontal sheet-
like intrusions (laccoliths) located in areas of relatively thin crust (i.e., in areas
where mantle bulges up).
174 O. T. R~rn6 and I. Haapala
(8) Petrochemical models suggests that the protolith of many subalkaline granites
was an intermediate to acid igneous or metaigneous rock in the middle or lower
parts of the crust. The protolith underwent partial melting initiated by break-
down of mafic F-enriched hydrous silicates (biotite, amphibole) to produce
metaluminous/marginally peraluminous initial magmas whose subsequent
evolution was largely controlled by fractionation of feldspars, quartz, and
subalkaline marie silicates. Mixing of marie and silicic magmas may have been
important in the formation of some of the intermediate rocks, and a mantle
component may have contributed to some of the peralkaline rocks associated
with the subalkaline granites. The late-stage topaz-bearing microcline-albite
granites show marked subsolidus reactions and are occasionally thoroughly
hydrothermally altered. Stable isotope (O, H) data suggest that meteoric-
hydrothermal alteration was probably very restricted.
(9) The mode of occurrence, tectonic setting, age relations, magmatic association,
and chemical and isotopic composition of the rapakivi granites are compatible
with a model postulating that the generation of rapakivi granites and asso-
ciated marie rocks involves partial melting of both upper mantle and lower/
middle continental crust. Enhanced partial fusion and upwelling of mantle
material caused partial melting of the felsic-intermediate crust producing
rapakivi granite magmas. Derivatives of the mantle magmas are diabase dykes,
gabbros, and anorthosites, and probably also some intermediate rocks
(ferrodiorites).
(10) Although the overall status of the rapakivi magmatism is anorogenic, its
indirect causal connection to orogeny, via formation of early Proterozoic
orogenic crust, is obvious in most cases. Establishment of an early/middle
Proterozoic supercontinent could have been the reason for the formation of
most of the Proterozoic rapakivi granites. The possibility of convergent pro-
cesses causing chemical changes in the mantle eventually leading to crustal
melting and rapakivi magmatism should form the subject of future studies.
Acknowledgments
It has been a great pleasure for us to meet and discuss with rapakivi granite researchers of
different countries at the inaugural stage of the rapakivi granite IGCP Project. In this
context, we would like to express our thanks especially to R. F. Emslie and A. B. Ryan for
providing us with the latest data on rapakivi occurrences in Canada and L. J. Robb for those
of southern Africa. W. W. Boyd, Jr., A. Kohl, and J. Tarney reviewed the manuscript and
their comments improved (and shortened) it substantially. We would also like to express
our sincere gratitude to E. F. Stumpfl for his editorial comments. R. Fagerstr6m drafted
most of the figures.
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184 O. T. R/im6 and I. Haapala
Authors' address: Dr. O. T. Ri~rn6 and Prof. Dr. I. Haapala, Department of Geology,
University of Helsinki, P.O. Box 11 (Snellmaninkatu 3), FIN-00014 Helsinki, Finland.