Dark Raman Resonances Due To Ramsey Inte

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PHYSICAL REVIEW A 78, 063816 共2008兲

Dark Raman resonances due to Ramsey interference in vacuum vapor cells


Z. D. Grujić, M. Mijailović, D. Arsenović, A. Kovačević, M. Nikolić, and B. M. Jelenković*
Institute of Physics, 11080 Belgrade, Serbia
共Received 9 September 2008; published 9 December 2008兲
We investigate the evolution of the atomic coherence between Zeeman sublevels with ⌬mF = 2 in the region
between pump and probe laser beams, in a Rb vapor cell using the Hanle configuration. The transmission of the
probe beam, placed inside the hollow pump beam, shows the narrowing of the Hanle resonance 共at external
magnetic field B = 0兲 by Ramsey fringes whose separation from the central peak depends on the distance
between the beams. The temporal evolution of the pump induced alignment is evident from the changes of the
probe transmission spectra with increasing the angle between linear polarizations of each beam. Experimental
results are in agreement with the results of the model which calculates probe fluorescence by solving time-
dependent optical Bloch equations, from the time when atom enters the pump beam to the time when it leaves
the probe beam. The results for total excited state populations were averaged over atomic velocities
distribution.

DOI: 10.1103/PhysRevA.78.063816 PACS number共s兲: 42.50.Gy, 42.50.Nn, 42.65.⫺k

I. INTRODUCTION fine levels of the ground state, interact with atoms in Na 关9兴
and Cs 关10兴 atomic beams. Ramsey fringes due to ground-
In coherent population trapping 共CPT兲, laser radiation, ap- state coherences with ⌬mF = 2 were observed in atomic beam
plied to a ⌳ scheme, places atoms in a nonabsorbing or dark of Ca atoms 关11兴. The observation of Ramsey fringes using
state when two light fields are in Raman resonance with the nonlinear Faraday rotation spectroscopy 共NLFR兲 in the Rb
splitting between two lower states 关1,2兴. This process is very atomic beam were given in 关12兴. Experiments 关9–12兴 pre-
efficient because of simultaneous coherent superposition of sented considerably narrower line shapes of EIT and NLFR
the ground states into an absorbing or bright state which is resonances when compared to nonseparated applied pump
strongly coupled to the excited state of the ⌳ scheme 关3–6兴. and probe beam excitations.
CPT is observed in fluorescence as a fluorescence dip. Nar- In several works, Ramsey methods were used on beams in
row gain in laser transmission or electromagnetically in- Raman resonance to excite alkali-metal atoms, contained in a
duced transparency 共EIT兲 can be observed due to the exis- gas cell and mixed with a buffer gas. Linearly polarized
tence of the “dark” state. probe beam, counterpropagating vs spatially displaced pump
In this paper, we study EIT resonances in a vacuum vapor laser beam in sodium vapor, monitors precession of orienta-
Rb cell when we apply Ramsey method 关7兴 of separated tion in atoms pumped by the circularly polarized pump laser
excitation regions. We show that such separation of fields light 关13兴. The manifestation of Ramsey interference effect
plays an important role in line shapes and linewidths of EIT. of radio-frequency Zeeman transitions in atomic vapor due
In the original Ramsey method, long-lived atomic polariza- to collisional velocity diffusion was shown by Buhr and
tion between ground-state hyperfine levels is induced by us- Mlynek 关14,15兴. These experiments apply the Ramsey reso-
nance idea in the domain where atoms with CPT alter both
ing microwaves. The first field creates coherent superposition
their position and velocity. It was shown that multiple colli-
between two levels. In the region between the two fields,
sions between buffer gas atoms and alkali-metal atoms lead
coherence acquires a phase shift which depends on both the to diffusion of alkali-metal atoms back to the laser beam,
frequency of hyperfine splitting and the time of flight. The which leads to diffusion-induced Ramsey narrowing of EIT
absorption of the microwave field in the second interaction 关16,17兴. Temporal Ramsey fringes due to scattering of de-
region is modulated if the phase of the coherence is changed, layed probe beam by coherently prepared Rb atoms were
for example, by changing the detuning of the microwaves in observed in Ref. 关18兴, while Ramsey fringes due to Zeeman
respect to the atomic frequency. Temporal instead of spatial coherence in Rb atoms for temporally and spatially separated
separation of microwave Ramsey pulses allows application laser beams were shown in Ref. 关19兴. High-contrast, sub-
of Ramsey methods to atomic clocks in buffered alkali-metal kHz, Ramsey fringes through Raman resonant beams were
gas cells 关8兴. In our work, we use modified Ramsey method observed using circularly polarized light and double ⌳
in vacuum Rb cell, by applying pump optical photons to scheme in Cs vapor with buffer gas 关20兴. Temporal Ramsey
create alignment in the ground-state hyperfine level in a Rb fringes due to multiple atom reflections from coated walls of
atom, followed by the pair of probe photons to detect in- the Rb cell were measured using both pump and probe
duced alignment. beams, spatially overlapped and separated 关21兴.
Modified Ramsey methods were performed, in several Excitations from the Ramsey method using beams with
cases, on thermal atomic beams. Spatially separated pump Raman resonance in buffered gas cells have found important
and probe laser beams, in Raman resonance with two hyper- applications, particularly for CPT based frequency standards
and atomic clocks, either active 关22,23兴 or passive 关24兴. The
aim of this paper is to further study Ramsey effects through
*zoran.grujic@phy.bg.ac.yu Raman resonance in vacuum gas cells, i.e., to study the effect

1050-2947/2008/78共6兲/063816共7兲 063816-1 ©2008 The American Physical Society


GRUJIĆ et al. PHYSICAL REVIEW A 78, 063816 共2008兲

(a) (b) (c) z B || z


Fe=2 Fe=1 y
m=-1 x Probe
m=0
m=1
Fe=1 Ring shape
pump beam
beam

Fg=2
m=2
m=1
m=0
Fg=1 m=-2
m=-1

Fg=2
FIG. 1. 共a兲 Schematic of atomic energy level diagram for 87Rb D1 line ground and excited levels, 共b兲 the energy level diagram for
magnetic sublevels of the Fg = 2 → Fe = 1 transition, and 共c兲 pump and probe laser beam radial profiles used in the theoretical model. In 共a兲
and 共b兲 solid lines represent laser light coupling energy levels and dotted lines show the deexcitation paths from excited levels.

of the temporal evolution of coherent superposition on the ground-state hyperfine level. Total probe fluorescence was
shape of EIT resonance. Similar studies in vacuum cells were calculated after averaging over atom velocity components
briefly done in Ref. 关19兴. In our work, we use two-photon parallel and perpendicular to the laser beam. Our work is
Raman transitions between Zeeman sublevels of the Fg = 2 relevant to some applications of the CPT, particularly for
ground-state hyperfine level. Both pump and probe beams atomic frequency standards based on CPT, either active
are tuned to the Fg = 2 → Fe = 1 transition in 87Rb and probe 关22,23兴 or passive standards 关24兴. The Ramsey method with
beam transmission is monitored while axial magnetic field is Raman resonance type excitation approach has advantages
scanned around zero. Experimentally, we put the probe beam over the standard Ramsey method for atomic frequency stan-
inside the central region of hollow pump beam. The role of dards, since it eliminates need for large microwave resona-
the pump in this setup is similar to that of an antireflection tors.
wall coating, and to that of buffer gas collisions in the vapor
cell with buffer gas. This setup allows enhanced interaction
of the atomic coherence with the probe beam in comparison II. THEORY
with separated laser beams 关19兴. This experimental geometry
is similar to the geometry used in Ref. 关25兴, where the sub- We used density matrix formalism to analyze the dynam-
Doppler feature was observed in the transmission of the hol- ics of the interaction between Rb atoms and spatially sepa-
low probe, through the very thin 共10 ␮m兲 cell, while the rated pump and probe laser beams. The temporal evolution
pump beam is placed in the probe center. of the density matrix elements for the excited and the ground
The results of our experiment are compared to the results state populations and coherences 共̺eie j , ̺gig j兲 and for optical
of time-dependent optical Bloch equations for density matrix coherence 共̺eig j兲 is obtained from time-dependent optical
elements for atoms in the pump, in the dark, and in the probe Bloch equations for the open Fg = 2 → Fe = 1 transition in
87
region. All the levels interacting with laser light are taken Rb. Figures 1共a兲 and 1共b兲 show Rb atomic level diagrams
into account, as well as population losses to the other with levels coupled and optically pumped by laser light.

̺˙ eie j = ̺eie ji共␻e j − ␻ei兲 +


i

2

ប k=−2
共̺
˜ e g E+g e − E−e g ̺
i k k j i k
˜ g e 兲 − 2⌫L̺e e 兺 具Jg储erជ储Je典2共2F⬘g + 1兲共2Jg + 1兲
k j i j
F ⬘
g
Jg Je 1
Fe F⬘g Ig
再 冎 2
,

˜˙ e g = ̺
̺ i j
˜ e g i关␻ − 共␻e − ␻g 兲兴 +
i j i j
i

冉兺 1

k=−1
̺eiekE−ekg j −
2

兺 E−e g ̺g g
k=−2
i k k j
冊 − ⌫L̺eie j 兺 具Jg储erជ储Je典2共2Fg⬘ + 1兲共2Jg + 1兲
Fg⬘
再 Jg Je
Fe Fg⬘ Ig
1
冎 2

̺˙ gig j = ̺gig ji共␻g j − ␻gi兲 +


i

1

ប k=−1
共̺
˜ g e E−e g − E+g e ̺
i k k j i k k j
J J 1
˜ e g 兲 + 2⌫L具Jg储erជ储Je典2共2Fg + 1兲共2Fe + 1兲共2Jg + 1兲 g e
Fe Fg Ig
再 冎 2

冉 冊冉 冊
1
Fe 1 Fg Fe 1 Fg
⫻ 兺 ̺e
q=−1
i+qe j+q j+q −q −j i+q −q −i
, 共1兲

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DARK RAMAN RESONANCES DUE TO RAMSEY … PHYSICAL REVIEW A 78, 063816 共2008兲

where 



1



zx
E+aia j = − ␮aia j−1E−1+ − ␮aia j1E+1+ − ␮aia j0ei␸ E0z ,




2


1 zx
E−aia j = − ␮aia j−1E−1− − ␮aia j1E+1− − ␮aia j0e−i␸ E0z ,
2 



yx yx



E0x + iei␸ E0y E0x + ie−i␸ E0y
E−1+ = , E−1− = ,
2 冑2 2 冑2

yx yx
− E0x + iei␸ E0y − E0x + ie−i␸ E0y
E+1+ = , E+1− = , 共2兲
2 冑2 2 冑2 



␮aia jq is the matrix dipole element, and ប␻ei and ប␻gi are the



energies of Zeeman sublevels. Fast oscillations at the laser
frequency in Eq. 共1兲 were eliminated by common substitu-
˜ e g e−i␻t. The summation Fg⬘ is over ground states
tion ̺eig j = ̺ i j
Fg = 1 , 2. E0x and E0y are x, y components of the laser’s elec-
tric vector, orthogonal to the beam propagation direction B=290mG
along the z axis. 



Eជ = eជ x cos共␻t兲E0x + eជ y cos共␻t + ␸yx兲E0y + eជ z cos共␻t + ␸zx兲E0z .
共3兲
The identity

再 冎
 
  

2
Jg Je 1 1
兺 共2F⬘g + 1兲 Fe F⬘g Ig
=
2Je + 1
共4兲 FIG. 2. 共Color online兲 Calculated dependence of spontaneous
Fg⬘ emission and of ground state coherence between Zeeman sublevels
as a function of radial position of an atom 共as atom passes through
relates ⌫L in Eq. 共1兲 to the emission rate ⌫
the pump beam, the “dark region,” and the probe region兲 for differ-
2Jg + 1 ent values of B. First column: Spontaneous emission from the ex-
⌫ = 2⌫L具Jg储erជ储Je典2 . 共5兲 cited Fe = 2 hyperfine level. Second column: the real 共solid line兲 and
2Je + 1 imaginary 共dashed line兲 parts of Zeeman coherence induced be-
tween mF = 0 and mF = −2 Zeeman sublevels of Fg = 2. Results are
Here 具Jg储erជ储Je典2 is reduced matrix element of the dipole op-
given for the magnetic field values of 0, 50, 170, and 290 mG, for
erator between the ground and excited states 关26兴.
four rows top to bottom and average pump and probe powers of
As schematically given in Fig. 1共c兲, the probe laser beam 2 mW and 20 ␮W, respectively. Polarizations of the pump and
is in the axis of the hollow pump beam. Both the pump and probe beam are linear and parallel to each other. The results are for
probe beams have the same frequency ␻. Their radial inten- the atom velocity of 260 m / s and its trajectory is along the probe
sity profiles are modeled by beam diameter. The distances which atoms travel through the pump,

E共r兲 =
Erf冉 r − r1
a共r2 − r1兲
冊 冉
− Erf
r − r2
a共r2 − r1兲
,
冊 共6兲
“dark” and probe regions are 3.5, 1.7, 1.5 mm, respectively.

until the atom exits the probe region. The density of the
2 rubidium vapor is low enough, so we can ignore relaxation
of coherence due to the collision processes.
where r1, r2, and a are suitable parameters.
The atom fluorescence is proportional to total excited-
In order to make numerical integration faster, the transi-
state population
tion from the region without the laser light to the region with
light fields is described by the error function, Eq. 共6兲. Exter-
⌸e共t,B, vជ 兲 = 兺 ̺eiei共t,B, vជ 兲, 共7兲
nal magnetic field B, along the beam propagation, splits the i
Zeeman sublevels by the amount 2␮BgFB, where ␮B is the
Bohr magneton and gF is the gyromagnetic factor of the where vជ is atom velocity vector.
level. We assume that each collision with the wall resets the Figure 2 shows the dependence of the atomic fluorescence
state of an atom, therefore, atoms entering the pump beam 共left column兲 and the coherence between Zeeman sublevels
have equal population of Zeeman sublevels in the ground- mF = 0 and mF = −2 of the Fg = 2 共right column兲 on the atom
state hyperfine levels. Numerical integration is carried out location for magnetic field B: 0, 50, 170, and 290 mG. Po-

063816-3
GRUJIĆ et al. PHYSICAL REVIEW A 78, 063816 共2008兲

larizations of the pump and probe beam are linear and par- VNDF
OI BS
allel to each other. As schematically indicated by shaded ar- ECDL M
eas, the atom enters and crosses the pump region, traverses
the “dark region” where not illuminated by either of laser P
fields, and then enters the probe region. Results in Fig. 2 are DDAVLL
BE
for the atom velocity of v = 260 m / s and its trajectory is
along the probe beam diameter. Curves presenting ⌬m I I
D
= ⫾ 2 ground state coherence are real 共solid lines兲 and imagi- M
nary 共dashed lines兲 part of the matrix elements ̺gig j. Only for λ/2 P I
B = 0, during the flight of atoms through the excitation zone, cell walls
the excited state population relaxes to zero and the coherence Helmholtz’s
coils dark region
reaches its steady state value. The atom is pumped either into pump
probe d=1,5mm
the dark state or to the Fg = 1 hyperfine level. For B ⫽ 0, the Digital Trigger Signal
generator
dark state is not ideal. The atom can be excited and then oscilloscope
pumped back again either into the dark state or into un-
coupled Fg = 1 hyperfine level. Hence, it is necessary to deal FIG. 3. Experimental setup. ECDL: external cavity diode laser,
with time-dependent optical Bloch equations not only to take OI: optical isolator, DDAVLL: Doppler free dichroic atomic laser
into account the real radial profiles of the pump and probe lock, BS: beam splitter, I: iris, P: polarizer, VNDF: variable neutral-
beams, but also to achieve a proper description of this open density filter, BE: beam expander, M: mirrors, ␭ / 2: retardation
atomic system. plate, D: photodiode detector.
Motion of atoms in vacuum Rb cell is faster than the
relaxation rates of the ground state coherence and the coher- laser beam, determines the Doppler shift in the laser fre-
ence varies as atoms traverse the pump laser beam. This is in quency seen by an atom:
contrast to buffer gas cells where much slower motion of
atoms allows the atomic coherence to be instantaneously ad- ⌼共B兲 = 兺 兩vជ 兩Ie共B兲Wb共T,兩vជ 兩兲, 共9兲
justed at each part of the laser beam 关16兴. While in the “dark vជ

region,” the phase of the dark state oscillates, which causes where 兩vជ 兩 accounts for atom flux through the laser beam. In
oscillation from dark to bright state. The frequency of the Eq. 共9兲
evolution is equal to the separation between Zeeman sublev-
els, splitted by the 2gF␮B. The frequency of oscillations in-
creases while the amplitudes of modulation decreases with B.
Wb共T, v兲 = 4␲ 冉 冊
M
2␲kT
3/2
v2e−M v
2/2kT
共10兲
In the absence of collisions, the damping rate of the oscilla-
tions is zero. For each value of B, the phase shift of the is the Maxwell-Boltzmann distribution, k Boltzmann con-
atomic coherence at the entrance of the probe region depends stant, T is the temperature of rubidium vapor, and M is the
on the atom transit time, which in turn depends on the atom mass of a 87Rb atom. We have found that the contribution to
velocity and the direction of the atom propagation. Interfer- the total fluorescence ⌼共B兲 comes from atoms with small vz.
ence occurs when the electric field of the probe beam, phase The range of velocities vz contributing to the fluorescence
coherent to the pump beam, interacts with an atom. If the increases with the laser beam intensity. Even for the highest
two oscillators are in phase, the probe beam transmission intensities, laser detuning as seen by the atom with vz is
increases, otherwise decreases. In the cell, the atoms move much smaller then the separation between the hyperfine lev-
with different velocities due to the Maxwell-Boltzmann dis- els of the excited 2 P1/2 state. This justifies why in Eq. 共1兲 we
tribution and travel at different angles in respect to the laser did not include the Fe = 2 hyperfine level of the excited state.
beam. Thus, the atoms for the same B acquire different
phases at the entrance to the probe beam. This results in the
III. EXPERIMENTAL SETUP
lowering of the amplitude or in the washing out of the Ram-
sey fringes in the probe transmission. The laser light is generated by an external cavity diode
Total fluorescence from an atom due to excitation by the laser 共ECDL兲 and locked to the D1 transition in 87Rb using
probe beam is the doppler free dichroic atomic laser lock 共DDAVLL兲 关27兴
technique 共see Fig. 3兲. The laser beam is split into two beams
Ie共B, vជ 兲 = 冕
0
tp
⌸e共t,B, vជ 兲dt, 共8兲 using a nonpolarizing beam splitter. The intensities of the
two beams are adjusted by variable neutral-density filters.
The diameter of one of the beams 共the pump beam兲 is en-
where t p is the atom transit time through the probe beam. larged to ⬃25 mm and the beam is sent through the iris of
This time is determined by the atom trajectory in the probe, 12 mm in diameter. The polarization of the pump beam is
i.e., and by velocity component perpendicular to the laser determined by the linear polarizer. The linear polarization of
beam vx. To calculate the total fluorescence ⌼共B兲 we aver- the probe beam and its orientation in respect to the linear
aged Ie共B , vជ 兲 over atom trajectories, i.e., over incident angles polarization of the pump beam is determined by both the
of an atom on the probe beam and over different atom ve- linear polarizer and a ␭ / 2 retardation plate. The two beams
locities 共vជ summation兲. vz, velocity component parallel with are combined using a 1-in. mirror with a hole in its center

063816-4
DARK RAMAN RESONANCES DUE TO RAMSEY … PHYSICAL REVIEW A 78, 063816 共2008兲

levels as schematically shown in Fig. 1共b兲. Results are given


for two lengths of the “dark region,” 1.7 and 2.7 mm. As
shown in Fig. 4共b兲, substantial narrowing of the central trans-
mission peak 共probe EIT兲 occurs when the pump beam is on.
The probe linewidth is narrower in comparison with the line-
width obtained with the single laser beam whose diameter is
similar to the diameter of the pump beam. Longer length of
the “dark region” gives narrower EIT peak. Zeeman ⌬m
= ⫾ 2 coherence in the Fg = 2 hyperfine level evolves in the
magnetic field 共see oscillations in Fig. 2兲, at the Larmor fre-
quency. The interaction by the probe laser field, in phase
with the pump laser field, enters into the interference with
the atomic coherence carried by the moving atom. The trans-
mission of the probe beam reflects this interference by the
appearance of line shapes with sidebands, i.e., first-order
Ramsey fringes. Due to velocity averaging, obtained probe
FIG. 4. 共Color online兲 Calculated 共a兲 and measured 共b兲 probe transmission profiles do not show higher-order Ramsey
transmission for the Fg = 2 → Fe = 1 transition in 87Rb as a function fringes. As seen in Fig. 4共a兲, the position of fringes slightly
of the axial magnetic field. Dashed and dotted lines are for two changes with the length of the “dark region.” When compar-
inner pump beam diameters 5 and 7 mm 共corresponding to the ing shapes of measured and calculated EIT resonances, one
“dark region” length of 1.7 and 2.7 mm兲, respectively. The broad can see very good agreement for the linewidths, while the
resonance in 共b兲 is for the pump beam turned off 共solid line兲. Both contrast of measured sidebands is somewhat lost. The inclu-
pump and probe beams have the same linear polarization. The probe sion of the influence of the noncoupled ground-state hyper-
laser power is 10 ␮W, while the pump laser power is 0.55 mW. fine level in the optical Bloch equations leads to good agree-
ment for the linewidths. Smaller amplitudes of measured side
关28兴. The diameter of the hole determines the inner diameter bands might be due to the measurement procedure: the mag-
of the pump beam. The probe beam, 1.5 mm in diameter, netic field B was swept constantly while the probe transmis-
passes through the center of the hole. Both beams pass sion was recorded.
through the Rb cell with length of 85 mm and diameter of EIT resonance line shapes in Fig. 4 are for the probe beam
25 mm. intensity weak enough, so that it does not perturb coherences
The Earth’s and laboratory magnetic fields were compen- very much. Since both pump and probe beams couple the
sated by three orthogonal pairs of Helmholtz coils. Measured same transitions and create Zeeman coherence, increase of
residual inhomogeneity of the total magnetic filed was the probe power increases its contribution in observed probe
⬍5 mG over the cell’s length. We generated homogeneous EIT. At higher powers, fringes will disappear and the EIT has
a central transmission peak on wider pedestal. The pedestal
scanning magnetic field B in the direction of the laser beams
is the probe beam EIT, as shown in Ref. 关19兴.
propagation, by a solenoid around the gas cell.
The evidence of temporal evolution of the coherence was
Behind the cell, the probe beam passes through a circular given by measured sensitivity of the probe resonance line
aperture of the same diameter as the probe beam, in order to shape to the phases of oscillations. In Fig. 5, we present the
eliminate the pump beam contribution to the measured signal results for the probe transmission for several angles between
at the photodiode. The signal from the photodiode was re- the electric vectors of linearly polarized pump and probe
corded by the digital oscilloscope while B was scanned beams. The atomic coherence created by linearly polarized
around its zero value. pump beam is proportional to E+p E−p , where E+共−兲 are circular
p
␴+共−兲 components of linearly polarized radiation 关18,29兴. By
IV. DISCUSSION rotating the polarization of the probe beam by the angle ␾,
we change the phase between the circular components of the
In following figures, we compare theoretical and experi- pump beam by 2␾. This changes the phase of the dark state
mental line shapes of the probe Hanle EIT calculated and entering the probe beam for the same amount. For other pa-
measured as a function of the external magnetic field B. The rameters, such as B and atom velocity, interference will give
direction of the magnetic field is along the laser beam propa- either narrow transmission gains 共for 2␾ = 0兲 or absorption
gation. In the experiment, the magnetic field varies slowly peak 共for 2␾ = ␲兲. These two cases are presented by solid and
共50 Hz兲 so that the period of a magnetic sweep is much dashed lines, respectively. For other values of ␾, the trans-
longer than the atom transit time. The assumption made in mission has a dispersivelike shape. As the rotation angle in-
the model is that B is constant, while atom passes through creases, the first transmission peak shifts towards higher val-
three regions 共pump, dark, and probe regions兲. In all figures, ues of B. This is because by increasing the phase of the pump
spatially displaced pump and probe beams have the same beam, the dark state interference will occur at higher B. The
frequency. Figures 4共a兲 and 4共b兲 present calculated and mea- comparison between results in Figs. 5共a兲 and 5共b兲 shows that
sured probe transmission spectra as a function of the axial calculated line shapes are very similar to measured line-
magnetic field B. The polarizations of the pump and probe shapes.
beams are linear and parallel. Two circular components of We use wave forms in Fig. 5 to find the dependence of the
the laser beams interact with two ground-state Zeeman sub- first peak position and its amplitude on the pump beam po-

063816-5
GRUJIĆ et al. PHYSICAL REVIEW A 78, 063816 共2008兲

FIG. 5. 共Color online兲 Theoretical 共a兲 and experimental 共b兲 re-


sults of probe transmission spectra for the Fg = 2 → Fe = 1 transition
in 87Rb, for linearly polarized pump and probe beams and different
probe beam polarization angles in respect to the pump beam polar-
ization 共0° solid, 20° dash-dot-dot, 45° dotted, 70° dash-dot, and
90° dashed lines兲. The probe and pump powers are 20 ␮W and FIG. 6. Theoretical 共a兲 and experimental 共b兲 values of B re-
1.8 mW, respectively. quired to obtain the first transmission peak as a function of the
angle of the probe beam polarization. Solid lines are used to guide
the eye. Theoretical 共c兲 and experimental 共d兲 variation of EIT am-
larization angle. Figure 6 shows calculated 共a兲 and measured plitude as a function of angle of the probe polarization.
共b兲 values of B at which this first peak occurs. The results
show that the central maximum of the Hanle transmission
resonance moves towards higher magnetic fields, as we in- flow of atoms in dark state reaching the probe beam. This
crease the rotation angle of the probe polarization. Figures setup can be of importance for CPT and EIT applications
6共c兲 and 6共d兲 show the dependence of the amplitude of this using vacuum alkali-metal cells in magnetometry. When
peak on the probe beam polarization angle. pump and probe are in Raman resonance with the atom
ground states hyperfine splitting, inducing ⌬mF = 0 coherence
between hyperfine levels, this setup may be of interest for
V. CONCLUSION
atomic frequency standards. Atomic clocks based on vacuum
Using the setup of spatially separated, coaxial pump and gas cells are of interest because of temperature sensitive fre-
probe beams we show narrowing of the Hanle EIT reso- quency shift in buffer gas cells.
nances in D1 transition in 87Rb, due to the Ramsey method
with Raman resonance in a vacuum Rb cell. We theoretically
explained the shape and the line-widths of experimentally ACKNOWLEDGMENTS
observed EIT resonances by Ramsey interference effects be-
tween the phase-oscillating dark state and the probe beam The authors thank S. Cartaleva for useful comments and
electric filed. These results are of interest for quantum optics suggestions. This work was supported by the Ministry of
of dark states. Placing the probe inside the hole of cylinder- science and environmental protection of the Republic of Ser-
shaped, large-diameter pump beam we also increased the bia, under Grant No. 141003.

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