Blackwell Characteristics of The Plasma Impedance Probe With Constant Bias 2005

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Characteristics of the plasma impedance probe with constant bias

David D. Blackwell, David N. Walker, Sarah J. Messer, and William E. Amatucci

Citation: Physics of Plasmas (1994-present) 12, 093510 (2005); doi: 10.1063/1.2039627


View online: http://dx.doi.org/10.1063/1.2039627
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PHYSICS OF PLASMAS 12, 093510 共2005兲

Characteristics of the plasma impedance probe with constant bias


David D. Blackwell,a兲 David N. Walker, Sarah J. Messer, and William E. Amatucci
U.S. Naval Research Laboratory, Plasma Physics Division, Washington, DC 20375-5346
共Received 30 June 2005; accepted 1 August 2005; published online 26 September 2005兲
The impedance of a small spherical probe immersed in a uniform plasma is measured by recording
the reflection coefficient of an applied signal using a network analyzer. This impedance has a
resonance at the plasma frequency where the imaginary part goes to zero, a feature that has made
this measurement a good way of determining electron density. When the plasma potential is positive
with respect to the sphere—for example, if the sphere is electrically floating or grounded, a second
resonance occurs at ␻ ⬍ ␻ pe due to the capacitance created by the depleted electron density in the
sheath. A greatly increased power deposition occurs at this lower resonance, whose frequency can
be controlled by applying a dc bias which changes the sheath width. As the bias is increased the
value of this frequency becomes smaller until the resonance disappears completely at Vprobe
= Vplasma. As the bias is further increased past the plasma potential, an electron sheath forms with its
own resonance, which is at a lower frequency than the resonance associated with the ion sheath. The
impedance of the electron sheath can be approximated using sheath transit time perturbation theory
for a space charge limited diode. As with the ion sheath resonance, the largest energy deposition
occurs at the lower of the two resonant frequencies. © 2005 American Institute of Physics.
关DOI: 10.1063/1.2039627兴

I. INTRODUCTION Csh ␳+s


= . 共3兲
The plasma impedance probe is a diagnostic method C0 + Csh ␳ + 2s
which has been used in various forms by several authors.1–6 The impedance from Eq. 共1兲 has two resonant points in fre-
In a previous paper7 we described a method of measuring the quency space where the reactance is zero. These are referred
absolute electron density in a plasma using a network ana- to as the parallel and series resonances and are given by
lyzer to observe the resonant frequencies of the reflected sig-
nal from a probe in a plasma. The probe was a small sphere
whose impedance was determined by measuring the reflected ␻1 ⬇ ␻ pe 冑 C0
Csh + C0
series resonance
power when a radio-frequency 共rf兲 signal was applied. The
共4兲
impedance was found to agree with the theoretical model ␻2 = ␻ pe parallel resonance.
often found in the literature8,9 of a capacitance, representing
the sheath, in series with a tank circuit, representing the bulk It was found that the lowest reflected signal and maximum
plasma, as shown in Fig. 1. The impedance Z of a sphere of energy deposition to the plasma occurred at the series reso-
radius ␳ in a plasma with collision frequency ␯ and plasma nance which is below the electron plasma frequency. It is
frequency ␻ pe can be written as implicit in this model that the probe is biased negatively
enough such that a vacuum sheath forms. In most experi-
1 1 ments the probe is either grounded through an impedance or
Z= + 共1兲
j␻Csh 1 floating, so that the potential is a few volts negative with
j ␻C0 + respect to the plasma potential. Because of the minimum of
R p + j ␻L p
the reflection coefficient, the series resonance is much more
with circuit elements written in terms of the plasma param- visible in a variety of measurement techniques and can easily
eters as be mistaken for the plasma frequency. Such an error would
give an incorrectly low value of the electron density, so it is
C 0 = 4 ␲ ⑀ 0␳ , important that the characteristics of the impedance probe are
well understood.
The value of the sheath capacitance is dependent on the
L p = ␻−2 −1
pe C0 , 共2兲
sheath thickness s. It should be possible to change the ca-
pacitance and tune the resonant frequency by applying bias
R = ␯L p to the probe. Since this sheath resonance frequency is where
the reflection coefficient is minimum, we can control the
and the sheath capacitance a function of the sheath thickness spectrum of rf power deposited into the plasma using a dc
s as voltage.
The purpose of this paper is to investigate how the probe
a兲
Electronic mail: davidb@ccs.nrl.navy.mil impedance and series resonance changes with applied bias.

1070-664X/2005/12共9兲/093510/7/$22.50 12, 093510-1 © 2005 American Institute of Physics


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093510-2 Blackwell et al. Phys. Plasmas 12, 093510 共2005兲

FIG. 1. Circuit model of the plasma-probe impedance from Lieberman 共Ref.


8兲. The second capacitance C represents the sheath capacitance between the
plasma and the walls of the vacuum vessel, which because of its much larger
value can be neglected compared to the probe sheath capacitance.

Particularly we are interested in the impedance characteris-


tics as this bias is changed from negative 共ion sheath兲 to
positive 共electron sheath兲. To our knowledge, experimental
measurements of the rf impedance of a biased probe over
such a voltage range have not been previously published.

II. REVIEW OF THEORY


A. Negatively biased probe
When the probe is negatively biased, the sheath that de-
FIG. 2. Calculated magnitude 共a兲 and phase 共b兲 of the probe-plasma imped-
velops around the probe forms a region depleted of electrons
ance with varying applied negative bias w.r.t. the plasma potential. The
of thickness s共␾兲, with ␾ the negative potential relative to extrema of the magnitude and zero crossings of the phase correspond to the
the plasma potential. The impedance of the depleted layer sheath-plasma 共series兲 and plasma 共parallel兲 resonances. Increasing the bias
can be written as the capacitance between concentric spheres pushes the series resonance closer to the parallel resonance at the plasma
frequency. For all computed curves, the plasma electron density used was
with radii of ␳ and ␳ + s as in Eq. 共3兲. The sheath thickness 4 ⫻ 107 cm−3 and the electron temperature was 0.5 eV.
s共␾兲 can be written as a modified Child–Langmuir law as

s共␾兲 = 共2.5 − 1.87e−0.39␳/␭d兲 冉 冊


e␾
kTe
2/5
␭d 共5兲 conditions is a quite complicated analytical procedure which
is based on a perturbation solution to Llewellyn’s equation:11
with ␭d the Debye length. This expression for the sheath
m ⳵ 3x
thickness is an analytic function fit to the numerical calcula- J共t兲 = ⑀0 . 共6兲
tions of Laframboise.10 This value of s can be substituted e ⳵t3
into 1 to get the total impedance of the sphere in the plasma Equation 共6兲 is successively integrated from t to t0 to get
as a function of potential ␾. Figure 2 shows the calculated expressions for the electron acceleration, velocity, and posi-
impedance at several voltages. Throughout this paper, for all tion. These expressions are then expanded in terms of a per-
calculated plots, the plasma electron density assumed was turbed sheath transit time, such that t − t0 = T + ␦共t兲. The per-
4 ⫻ 107 cm−3 and the electron temperature was 0.5 eV. Both turbed transit time ␦共t兲 is found by assuming that the
of these are typical numbers for the plasmas produced in our perturbation is small enough such that the unperturbed and
space chamber. The sheath plasma resonance, noted by the electron perturbed position x may be taken as equivalent.
minimum of the amplitude or by the first zero phase crossing This perturbed transit time is then used to find the perturbed
as the frequency is increased, can be seen to increase with velocity and acceleration. The impedance can be calculated
increasing negative bias, pushing it closer to the plasma po- by integrating the ac electric field, which can be written as a
tential. Conversely, the series resonance decreases as the bias
is decreased until at the plasma potential it disappears, which
is the physical result expected since the sheath also disap-
pears. The reflection coefficient corresponding to this is
shown as a contour plot in Fig. 3. The narrow dark line
represents a minimum in this coefficient, and a maximum
power deposition, associated with the series resonance.

B. Positively biased probe


When the probe is positively biased, the sheath is no
longer depleted of electrons; in fact it is electron-rich, so the
impedance cannot be considered to be a capacitance. The
best approximation of the impedance of an electron-rich
FIG. 3. Calculated magnitude of the complex reflection coefficient ⌫ = Z
sheath is borrowed from the calculations of the impedance of − Z0 / Z + Z0 vs applied negative bias and frequency. The darkest swath of the
a parallel plate diode. Calculating the impedance under these contour indicates a maximum power deposition around the series resonance.
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093510-3 Characteristics of the plasma impedance probe… Phys. Plasmas 12, 093510 共2005兲

linear function of the acceleration, from the sheath edge to


the probe surface, or equivalently, integrating over the sheath
transit time. The algebraic steps involved in this procedure
are too long to include in this paper, but a good reference
where everything is explicitly worked out can be found in
Chap. 2 of Birdsall’s Electron Dynamics of Diode Regions
共1966兲.12 The result is an expression for the sheath imped-
ance for a probe in terms of the sheath transit time

Z+共␤,T兲 =
T2
2␤
冋 冉

1− 1−
3
12S共␤兲
␤3
冊册 共ve0 + ve兲
4 ␲ ␧ 0␳ 2
共7兲

with

␤ = i␻T, ve0 = 冑 kTe


m
,

ve = 冑 2e␾
m
, ␨=
ve0 − ve
ve0 + ve
, 共8兲

S共␤兲 = 2 − 2e−␤ − ␤ − ␤e−␤ .


The sheath transit time itself can be expressed as a function
of the DC probe bias as FIG. 4. 共a兲 Calculated magnitude of the imaginary part of the probe-plasma

冕 冉 冊
s共␾兲
impedance vs frequency at a bias of ±5 V w.r.t. the plasma potential. 共b兲
−1/2
e⌽共x兲 Real part of the probe impedance for the positively biased probe showing a
T= −1
ve0 1+ . 共9兲 zero crossing at ␻T = 2␲.
0 kTe

The potential ⌽共x兲 is derived from Eq. 共5兲 as

冉 冊
trated more clearly in Fig. 6 where we have plotted the mag-
s共␾兲 + ␳ − x 5/2
nitude of the calculated reflection coefficient ⌫ for the sphere
⌽共x兲 = ␾ . 共10兲
s共␾兲 at both positive and negative bias. The minimum of 兩⌫兩
around this resonance indicates maximum power deposition
For the positively biased sheath, the sheath impedance of Eq. into the plasma. We can see that also that this minimum is
共7兲 takes the place of the sheath capacitance term in Eq. 共1兲, wider and shallower for the electron sheath than it is for the
assuming the sheath is sufficiently thin compared to the the
probe radius such that the parallel plate one-dimensional
analysis is valid. The imaginary part of electron sheath im-
pedance is capacitive in nature but is much smaller than the
ion sheath impedance, as shown in Fig. 4共a兲. Unlike the ion
sheath, the electron sheath impedance also has a real part.
The real part of the electron sheath impedance in Fig. 4共b兲
actually changes signs when the sheath transit time is on the
order of one RF period, 2␲ ⬍ ␻T ⬍ 3␲. This sign change has
been observed in the past in higher density plasmas as a
sheath plasma instability.13
The impedance of the positively biased probe is then the
summation of the sheath impedance and the bulk plasma
impedance:
1
Z = Z+共␤,T兲 + . 共11兲
1
j ␻C0 +
R p + j ␻L p
Equation 共11兲 is plotted for several voltages in Fig. 5. We can
see that the parallel resonance is unaffected by the new
sheath impedance term just as in the negatively biased ion
sheath case. The series resonance is also at a slightly lower
value than it was for the ion sheath. It is important to note
FIG. 5. Calculated magnitude 共a兲 and phase 共b兲 of the probe-plasma imped-
that even with the probe biased positively, the series reso-
ance with varying applied positive bias w.r.t. the plasma potential. The series
nance, instead of disappearing, is essentially very similar to resonance is no longer as sharp due to the resistive component of the elec-
the plasma sheath resonance for negative bias. This is illus- tron sheath impedance.
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093510-4 Blackwell et al. Phys. Plasmas 12, 093510 共2005兲

FIG. 6. Calculated magnitude of the reflection coefficient ⌫ at a bias of


±5 V w.r.t. the plasma potential showing the broader resonance of the elec- FIG. 8. Experimental setup used to measure probe impedance with applied
tron sheath. bias.

B. Measurement of impedance
ion sheath. When we reach the zero crossing in the electron
sheath impedance at ␻T = 2␲, the reflection coefficient be- The complex impedance Z of the probe is obtained by
comes larger than one, but the deviation is very small. Figure using a HP 8753-D network analyzer to measure the complex
7 shows a contour plot of 兩⌫兩 as the sheath bias and driving reflection coefficient ⌫, given by
frequency are varied. Z − Z0
⌫= 共12兲
Z + Z0
with Z0 the internal impedance of the analyzer, which in this
III. EXPERIMENTAL ARRANGEMENT
experiment is 50 ⍀. The impedance that we are interested in
A. Plasma source is that of a sphere in a plasma, but what we initially get is the
impedance of the sphere plus whatever cabling connects the
The Space Physics Simulation Chamber at the U.S. Na-
sphere to the network analyzer. An additional complication is
val Research Laboratory 共NRL兲 has been described in recent
that we also have to apply a dc bias to the probe with a
papers.7,14 The chamber is a 2-m diameter, 5-m-long vacuum
power supply. The network analyzer will see a terminal im-
vessel surrounded by five 3-m diameter magnet coils. In this
pedance of this entire assembly, not just the sphere at the
experiment the magnetic field was kept at very low levels
end, which is a very small part. The extra impedance from
共B ⬍ 5G兲 such that ␻ce Ⰶ ␻ pe , ␻ pi. The chamber is filled to a
the cable and probe shaft can be compensated for by cali-
pressure of p ⬇ 10−4 Torr argon. A weakly ionized 共n ⬇ 107
brating the analyzer to ignore everything up to the very tip
− 109 cm−3兲 plasma is created with a 1-square-meter array of
where the sphere is attached. The probe should therefore be
glowing tungsten filaments biased at −100 V. The electron
constructed such that the sphere is removable and an electri-
density is measured two ways: 1兲 by reading the parallel
cal short or 50 ⍀ load can be put in its place with no addi-
resonance frequency from the impedance measurement; and
tional cabling. One at a time, the operator indicates that there
2兲 with a heated Langmuir probe mounted close to the
is an open circuit 共⌫ = 1兲, a short circuit 共⌫ = −1兲, or a 50 ⍀
sphere. Typical electron and ion temperatures are typically
load 共⌫ = 0兲. The network analyzer then adjusts internal
Te ⬇ 0.5 eV and Ti ⬇ 0.05 eV.
phase and amplitude filters until these values of ⌫ are visible
at the terminal. The setup for the experiment and measure-
ment circuit is shown in Fig. 8.

IV. RESULTS

Figure 9 shows the magnitude and phase of the imped-


ance calculated from the measured reflection coefficient
when the sphere is negatively biased. If we compare this to
Fig. 2 we can see that the most obvious difference between
the theoretical and experimental curves is that experimen-
tally we observe a splitting of the parallel resonance into two
peaks on the impedance magnitude curves. This can be ex-
plained with a slight modification to the theory to include a
presheath region where the density profile gradually rises
FIG. 7. Calculated magnitude of the complex reflection coefficient ⌫ = Z
− Z0 / Z + Z0 vs applied positive bias and frequency, showing a more smeared after the sheath region. The impedance can be found using a
out energy deposition compared to the negatively biased probe. more general expression to include a density gradient:
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093510-5 Characteristics of the plasma impedance probe… Phys. Plasmas 12, 093510 共2005兲

FIG. 9. Measured probe impedance magnitude 共a兲 and phase 共b兲 in an argon
plasma with ne = 1.6⫻ 108 cm−3, P = 0.29 mTorr, and Te = 0.5 eV with vary-
ing applied negative bias.

Z=−
1
j ␻4␲⑀0
冕冉


1−
␻2pe共r兲
␻共␻ − i␯兲
冊 −1
dr
r2
. 共13兲

The effect of this is to add another peak to the impedance


curve as shown in Fig. 10. This multiple resonance behavior
is analogous to the Tonks–Dattner resonances15 in a cylindri-
cal plasma.
The series resonance is easily identifiable in the imped-
FIG. 10. The effect of calculating the impedance using an ion sheath with a
ance curves as either the minimum of the impedance magni- gentler gradient outside the sheath region 共a兲 yields a second parallel reso-
tude or the first zero crossing in phase. There is excellent nance which appears as an extra peak in the magnitude 共b兲 and dip in the
theoretical agreement with the experimental results in that phase 共c兲.
the series resonance moves to the right as more bias is ap-
plied to the probe.
is in agreement with the theory. The relative values of the ion
Figure 11 shows the impedance curves when positive
and electron sheath resonance frequencies and the shape of
bias is applied to the sphere. The more rounded series reso-
the contours are also in excellent agreement with the theo-
nance minimum seen agrees with the predicted theoretical
retical predictions.
curves in Fig. 5. As with the ion sheath, an increase in po-
tential moves this resonance closer to the parallel resonance.
V. CONCLUSIONS
Contour plots of the magnitude of the reflection coeffi-
cient and the phase of the impedance are shown in Figs. Measurements of the impedance of a spherical probe in a
12–14. As the voltage is swept from negative to positive, the plasma as the bias on the probe is changed from negative to
series resonance is identifiable as the region where 兩⌫兩 is positive are presented for the first time. For negative bias, the
minimum. The associated phase crossing 共the white dotted ion sheath creates a sheath-plasma resonance at a frequency
line兲 indicates one crossing at the plasma frequency and one below the plasma frequency where the reflection coefficient
crossing at the sheath plasma resonance. We can see that is minimum and energy absorbed by the plasma is maximum.
when we sweep the voltage through the plasma potential the As the voltage on the probe moves more positive toward the
series resonance disappears completely, but reappears as we plasma potential, the resonance frequency decreases in a
keep increasing the bias to obtain an electron sheath. We also manner consistent with theory, until at the plasma potential it
note that the energy deposition associated with this reso- disappears entirely.
nance on the electron side of the curve is much broader when As the potential is increased more positively, an electron
compared to resonance on the ion side, an observation which sheath takes the place of the ion sheath. The impedance of
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093510-6 Blackwell et al. Phys. Plasmas 12, 093510 共2005兲

FIG. 13. Contour plot of ⌫ 共a兲 and ⬔Z 共b兲 at an electron density of ne


= 2.8⫻ 108 cm−3. The higher plasma frequency is evident when this plot is
compared to Fig. 12.

FIG. 11. Measured probe impedance magnitude 共a兲 and phase 共b兲 in an
argon plasma with under the same conditions as in Fig. 9 with varying
applied positive bias. the electron sheath is calculated using a parallel plate diode
model formulated by Llewellyn and Birdsall.11,12 The imped-
ance has a resistive component as well as a capacitive com-
ponent. Both parts of the impedance are functions of the
electron sheath transit time as well as the other plasma pa-
rameters. The series resonance associated with the electron

FIG. 12. 共a兲 Contour plot of the reflection coefficient 兩⌫兩 vs voltage and
phase showing both the electron and ion sheath impedance characteristics.
共b兲 Contour plot of the phase of the impedance with the dashed line showing FIG. 14. Contour plot of ⌫ 共a兲 and ⬔Z 共b兲 at an electron density of ne
the zero crossings. The higher zero crossing which is unchanging with volt- = 9.7⫻ 108 cm−3. The plasma frequency at this density was off the frequency
age is the parallel plasma resonance. The electron density is ne = 6 calibration scale for the network analyzer but the series resonance is still
⫻ 107 cm−3 with Te = 0.5 eV. easily identifiable.
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093510-7 Characteristics of the plasma impedance probe… Phys. Plasmas 12, 093510 共2005兲

5
sheath yields an energy deposition that is broader and shal- S. G. Bilen, J. M. Haas, F. S. Gulczinski, A. D. Gallimore, and J. N.
Letoutchaia, AIAA-99-2714, 35th Joint Propulsion Conference, Los An-
lower than the ion sheath. Despite these differences, overall
geles, June, 1999.
the impedance characteristics for both positive and negative 6
P. Nikitin and C. Swenson, IEEE Trans. Antennas Propag. 49, 1377
bias are qualitatively similar. 共2001兲.
7
D. D. Blackwell, D. N. Walker, and W. E. Amatucci, Rev. Sci. Instrum.
ACKNOWLEDGMENTS 76, 023503 共2005兲.
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M. A. Lieberman and A. J. Lichtenberg, Principles of Plasma Discharges
The authors thank Dr. Charles Swenson for many useful and Materials Processing 共Wiley Interscience, New York, 1994兲, p. 303.
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discussions and Erik Tejero for technical assistance with data V. P. T. Ku, B. M. Annaratone, and J. E. Allen, J. Appl. Phys. 84, 6536
共1998兲.
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J. G. Laframboise, Ph.D. thesis, University of Toronto, Institute for Aero-
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F. B. Llewellyn and L. C. Peterson, Proc. IRE 32, 144 共1944兲.
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