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Fractal Non-Fermi Liquids From Moir E-Hofstadter Phonons: These Authors Contributed Equally To This Work
Fractal Non-Fermi Liquids From Moir E-Hofstadter Phonons: These Authors Contributed Equally To This Work
Fractal Non-Fermi Liquids From Moir E-Hofstadter Phonons: These Authors Contributed Equally To This Work
totic low-temperature non-Fermi liquid regime remains at prohibitively low temperatures, striking
precursor non-Fermi liquid signatures can be observed, and we propose surface acoustic wave atten-
uation and quantum oscillation transport experiments. We also study the motion of MH acoustic
(MHA)-polarons, which we predict exhibit logarithmically diverging effective mass and unconven-
tional magnetic field scaling for scaling of cyclotron resonance frequency and quantum oscillation
amplitude.
FIG. 1. Magnetic band structure – (a), (b), (c) Magnetic bands structures of spin up valence bands in the magnetic
Brillouin zone for θ = 1.5◦ , ν = 1/3, B = 18.0T , θ = 1.1◦ , ν = 1/2, B = 14.5T and θ = 0.8◦ , ν = 1, B = 15.4T . In (a) and (b)
there is a pair of Dirac points at K, K 0 and an electron pocket at Γ point, whereas in (c) Dirac points at K, K 0 smear out to
oblong hole pockets near M, M 0 , forming a three-fold Fermi surface. The magnetic Brillouin zone is shown as a blue hexagon.
(d), (e), (f) bands structure along the high symmetry path Γ − M − K − Γ − M0 − K for θ = 1.5◦ , ν = 1/3, θ = 1.1◦ , ν = 1/2
and θ = 0.8◦ , ν = 1.
connecting the Dirac points in the two layers, and a is {a1 , qa2 }, and exhibits dispersive Bloch-bands labeled by
the graphene lattice spacing. T (r) represent interlayer magnetic quasi-momenta.
tunneling with the (approximate) spatial periodicity of
the moiré lattice Fig. 1(a) and (d) show the lowest two bands near
X charge-neutrality for θ = 1.5◦ , and B = 18T (ν = 13 ).
T (r) = w e−igj ·r Tj . (2) Apart from having lower bandwidth and spin-splitting,
j the bands resemble those of single-layer graphene in zero-
field. In particular, the conduction (valence) bands ex-
√
3kθ
√ hibits a pair of Dirac points near charge-neutrality at
Here g 0 = 0, g 1,2 = ∓x̂ + 3ŷ are moiré-
2
reciprocal-lattice vectors, and Tj = η + σ2πj/3 are sub- the moiré K, K 0 points, which merge into a single Γ-
lattice matrices. The real-space lattice vectors for the centered hole (electron) pocket at the top of the conduc-
moiré√cell are (for small twist angle, θ 1): a1,2 = tion band (bottom of the valence band), crossing through
a a van-Hove (VH) singularity with nearly-nested hexago-
2θ ∓ 3x̂ + ŷ . For numerical results presented below, nal Fermi-surface at intermediate filling along the way.
we take ~v ≈ 610 meV nm, w ≈ 110 meV, and η ≈ 0.82,
Bands at θ = 1.1◦ (shown in Fig. 1(b) and (e)) exhibit a
which accounts corrugation [20].
similar Fermi surface evolution with doping, and also in-
Varying B produces a fractal “Hofstadter butterfly” herit the zero-magnetic field property of having reduced
energy spectrum [18, 19, 21, 22]. Here, instead, we focus bandwidth near the magic angle [17]. In this case, be-
on fixed B such that number of magnetic flux per moiré cause of strong electron-electron interactions relative to
unit cell is a rational fraction [18] (see also Appendix A): the small bandwidth, correlated insulating and supercon-
√ ducting behaviors have been observed [23]. However, at
3a2 p the magnetic fields that we consider here, the supercon-
ν= = , with p, q ∈ Z, (3)
4πθ2 `2B q ductivity near the magic angle is suppressed [23], and the
√ correlated insulating behavior arises only near integer fill-
and magnetic length `B = 1/ eB. At these com- ings of the flat moiré bands [24, 25], which can be gener-
mensurate fields, the Hamiltonian possesses a peri- ically avoided [26]. Therefore, we expect the correlated
odic magnetic-lattice translation symmetry generated by insulating and superconducting behaviors do not neces-
3
FIG. 2. Electron-phonon coupling – electron-phonon coupling Γm , for x-polarization phonons in the limit of zero momentum
transfer for (a) θ = 1.5◦ , ν = 1/3, (b) θ = 1.1◦ , ν = 1/2 and (c) θ = 0.8◦ , ν = 1.
sarily obscure the non-Fermi liquid physics discussed in on the electronic Hamiltonian can be accounted by dis-
this work. placing the tunneling operators T (r) → T (r −u) by with
At special flat Fermi-surface (FFS) fillings, which oc- a single effective displacement field [17, 28, 29]:
cur near (but not precisely at) VH fillings, the Fermi-
surface curvature vanishes at certain points on the Fermi- ẑ × d
u = ū − , (5)
surface, and remains small over extended patches, which 2 tan θ/2
will enhance electron-phonon interaction effects. Taylor
expanding the dispersion in small momentum displace- since the relative sliding of the two graphene sheets
ments from the center of these flat-patches, the vanishing is equivalent to a translation of the moiré pattern per-
Fermi-surface curvature requires a vanishing quadratic pendicular to the sliding direction. This has two im-
term for the tangential dispersion. Due to mirror symme- portant consequences: First, at small twist angles, the
try around the center of the flat-patch, the next leading coupling to d is enhanced by a factor of ≈ θ−1 [29]. Sec-
term is quartic. Near the flat-patches both the quadratic ond, for a commensurate crystal relative displacements
and the quartic terms contribute to the dispersion: would be gapped optical modes. Instead, for incommen-
surate twist angles uniform d-displacements have no en-
1 2 ergy cost [30, 31] and result in gapless acoustic modes (in
k = vF k ⊥ + k + λkk4 (4)
2m k analogy to the sliding “phason” mode of incommensurate
charge density wave orders [32]).
where k⊥ and kk are patch-momentum components per-
The electron-phonon coupling is conveniently identi-
pendicular and parallel to the Fermi-surface. Away from
fied by changing coordinates to a co-moving frame of
the FFS points, there is a crossover momentum scale
1 the lattice: r ← (r − u(r)) [28], in which the lattice
q∗ = √2mλ , below which the leading dependence on kk is
is restored to its undistorted form. To properly account
k ∼ kk2 and above which it is k ∼ kk4 . for the non-commutivity of magnetic translations, while
In SLG, FFS fillings were predicted to enable corre- manifestly preserving gauge invariance, we implement
lated insulators or superconductors [27], but occur at pro- this frame transformation with the unitary operator:
hibitively high electron density ∼ 1015 cm−2 above charge
neutrality. In moiré systems, the FFS occur at much Wu = e−iu(R)·Π (6)
lower fillings and can be experimentally explored. More-
over, the degree of Ferm-surface nesting (alignment be- where R = r − `2B ẑ × Π is the guiding center coordi-
tween antipodal flat-patches), which controls the compe- nate (whose components all commute with Π). Neglect-
tition between interaction-driven orders, can be adjusted ing subleading terms of order O(∇u, u2 ), this transfor-
by twist-engineering. For example, for the parameters mation effectively restores the moiré tunneling potential:
shown in Fig. 1(c), the FFS fillings exhibit a non-nested Wu† T (r − u(r)) Wu ≈ T (~r), while transforming the ki-
FFS with three-fold rotational symmetry. netic energy by: Wu† ΠWu ≈ Π − eB × u(R), yielding a
direct (gradient-free) electron-phonon interaction:
B. Electron-phonon coupling ~ × σ̂ −θ/2 0
He-ph = ev~u · B ≡ ū · Γm + d · Γr (7)
0 σ θ/2
To describe phonons, we introduce displacement fields:
u` (r) for each layer ` = 1, 2, which are conveniently re- For future convenience, we define the electron phonon
expressed in terms of the mean-displacement of the bi- vertices:
layer: ū = 12 (u1 + u2 ) and relative displacements of the
layers, d = u1 − u2 . Both types of phonon displacements Γn,α,λ (k, q) = hn, k + q|ε̂λ (q) · Γα |n, ki (8)
4
description is:
dωd2 k †
Z
S= ψ (iω − k )ψω,k
(2π)3 ω,k
X dΩd2 q
Z
ρ Ω2 + c2s q 2 |uλ (Ω, q)|2
+ 3
(2π)
λ
X Z dωd2 kdΩd2 q †
+ Γλ (k, q)uλ (Ω, q)ψω+Ω,k+q ψω,k
(2π)6
λ
(9)
FIG. 4. Landau damping energy and SAW attenuation length – (a), (b) Landau damping scale of relative-displacement
phonon ELD,r along path K − Γ − K 0 for twist angle θ = 1.5◦ , θ = 1.1◦ and flux filling ν = 1/3, ν = 1/2. (c) ELD,r along path
M − Γ − M 0 for twist angle θ = 0.8◦ and flux filling ν = 1. (d),(e) SAW attenuation length of relative-displacement phonon
ξr along path K − Γ − K 0 , for twist angle θ = 1.5◦ , θ = 1.1◦ and flux filling ν = 1/3, ν = 1/2 and typical driving frequency
ω/2π = 200MHz ∼ 0.96 × 10−2 K. (f) ξr along path M − Γ − M 0 , for twist angle θ = 0.8◦ , filling ν = 1 and driving frequency
ω/2π = 200MHz
packet made from Bloch states of the bands at commen- The cyclotron motion of MHA-polarons differs
surate filling Bν moving in effective field, ∆B). Oscilla- markedly from that of bare electrons as we now
tions with the reduced field ∆B, rather than the full field show by solving the polaron equation of motion in
B could be measured by standard Shubnikov-de-Haas, Eq. (21) for damped oscillatory cyclotron motion r(t) =
cyclotron resonance, or current-focusing [40] techniques, r0 e−Γc t (cos(ωc t)x̂ + sin(ωc t)ŷ), in an excess field ∆B.
but to our knowledge have not yet been explored. Defining an effective frequency dependent mass mp (ωc ) ≡
eB/ωc we find that the MHA-polaron exhibits a
scale-dependent logarithmically diverging effective mass:
1. Cyclotron motion 2 Λ
mp (ωc ) = m 1 + g log ωc . The cyclotron frequency
scales with an unconventional power of ∆B:
Numerical computation reveals the electron-phonon
coupling is proportional to the band-velocity, so that the ω g 2
c,0 1+g 2
phonon fields couple to the electron velocity, ṙ, where r is ωc = ωc,0 ∼ (∆B) (22)
Λ
the electron coordinate. This velocity coupling is directly
analogous to the coupling between charged-particles and and a ∆B independent decay rate Γc = g 2 Λ. Here
gauge fields. Incorporating this feature into a Schwinger- ωc,0 = e∆Bm is the bare (non-interacting) electron cy-
Keldysh path integral description of a single-electron (or clotron frequency of the MH-bands. For TBG we find
hole) coupled to a zero-temperature
R bath of phonons, we that the g 2 . 10−2 (even close to the VH-fillings), so
obtain an effective action C dtL[r, u] on the closed-time these effects may be challenging to observe. We note,
Keldysh contour C with the Lagrangian: however, that these predictions equally apply to a vari-
ety of analog non-Fermi liquid systems [4, 6, 13–15] where
L[r, u] = Le [r] + Le−ph [r, u(r)] + Lph [u] the polaron coupling constant would not be suppressed
1 by the electron-ion mass ratio and could potentially give
Le [r] = mṙ 2 − eṙ · A(r), appreciable modifications to semiclassical electron mo-
2h
ρ 2 2
i tion.
Lph [u] = (∂t u) − c2s (∇u) ,
2
Le−ph [r, u(r)] = αṙ · u(r). (19)
2. Quantum oscillations
Here, the vector potential A(r) corresponds to the excess
magnetic field (∆B = ∇ × A(r)), and does not include In addition to energy dissipation by phonon radiation,
the constant field used to reach the MH-regime, and α ≡ MHA-phonons cause characteristic dephasing of phase-
m ∂Γ(k,q=0) . sensitive measurements such as periodic-in-1/∆B quan-
∂k
We now integrate out the phonon field by approximat- tum oscillations in density of states and resistivity. As
ing the change of the electron position to be slow com- electrons experience MHA-phonon fields u as an effec-
pared to the wavelengths of the phonons being integrated tive electromagnetic vector potential, zero-point fluctua-
out [41], which leads to a quadratic, non-local in time ef- tions of MHA-phonons give rise to quantum-fluctuating
R
fective action for the MHA polaron coordinate r: geometric (Aharonov-Bohm-like) phase, eiα dt ṙ·u(r(t)) .
Quantum fluctuations in the phonon fields results in
α2
Z ∞ Z ∞
r q (t) · ṙ cl (t0 ) random geometric-phase accumulation that suppress the
Seff = S0 − dt dt0 2 (20) quantum oscillation amplitude.
2πρc2s −∞ t (t − t0 ) We compute the quantum oscillatory contribution to
density of states,N (ε), at energy ε via a semiclassical sum
where rcl/q are the so-called “classical” and “quantum” of the return amplitude for multiple classical cyclotron
combinations of r(t) on the two-time Keldysh contour, orbits of the MHA-polaron, averaged over fluctuating ge-
and S0 is the bare action for an electron in the absence ometric phases due to MHA-phonons [44]:
of phonon degrees of freedom. Varying this effective ac-
tion [42], we find the following semiclassical equation of 1 t
Z
motion (EOM) for r (see Appendix D 1): N (ε) ≈ − dt Im GR (r = r0 ; t)e−iεt
π 0
2πε
X R
≈h e−i ωc n eiα dt ṙ·u(r(t)) iu (23)
t
ṙ(t0 )
Z
F ext 0 n
r̈(t) = − g2 dt (21)
m −∞ (t − t0 )2
where h. . .iu indicates an average over quantum fluctua-
q
m ∂Γ(k,q=0) tions of u. We restrict our attention to zero temperature
where g = 2πρc2s ∂k is a dimensionless measure of here, as finite temperature effects with T ωc do not
electron-phonon coupling strength, and F ext represents effect the scaling form that we identify. These fluctu-
the external force due to the excess magnetic field [43]. ations are approximately quenched on the time-scale of
The second term represents the non-Markovian effects the cyclotron motion since the electrons are fast com-
due to the gapless phonons. pared to the phonons, i.e. we may approximately replace
8
R
dt ṙ · u(r(t)) by Φ(u), the flux of a static effective mag- IV. OUTLOOK
netic field b = ∇ × u through the cyclotron orbit. Within
this approximation, applying the Poisson summation for- We have explored moiré super-lattice structures in high
mula (see Appendix D 2) yields. magnetic fields as potential platforms for simulating non-
Fermi liquid (NFL) physics, due to unusually singular
electron-phonon coupling. While the asymptotic low-
temperature NFL fixed point remains at inaccessibly low
temperature, intermediate scale non-Fermi liquid precur-
sor behavior and unconventional polaron dynamics can
X 2πε 1 2
n2 hΦΦi
be observed at by tuning carrier density near a van-Hove
N (ε) = e−i ωc n e−i 2 α singularity. At or very close to the van Hove filling,
n the NFL physics will compete (or intertwine) with en-
X 1 2 hanced tendency to order with a nested Fermi surface.
= Ac exp − 2 (ε − nωc,0 ) (24)
n
2Γ This competition appears to be controllable by twist-
engineering [45–50], and a more detailed study of the
interplay between exotic interaction-driven orders, and
non-Fermi liquid physics in these systems will be a com-
pelling subject for future investigation.
Acknowledgements – We thank Allan Macdonald, Elaine
Li, Sid Parameswaran, Brad Ramshaw, Isabelle Phinney,
The resulting oscillator contribution to the density of Igor Blinov and Naichao Hu for insightful discussions.
states takes the form of a comb of Gaussian peaks cen- This work was supported by NSF DMR-1653007 (AP),
tered at integer multiples of the cyclotron frequency ωc,0 and by the NSF through the Center for Dynamics and
2g 2
with peak-amplitude Ac ∼ |∆B| and
√ width Γ ∼ (∆B) . Control of Materials: an NSF MRSEC under Coopera-
This contrasts the usual Ac ∼ ∆B scaling expected tive Agreement No. DMR-1720595 (AK). Part of this
from impurity scattering, providing a means to distin- work was performed at the Aspen Center for Physics,
guish these two mechanisms. which is supported by NSF grant PHY-1607611.
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10
In this section, we review the derivation of the magnetic Bloch bands for twisted bilayer graphene. Define the
magnetic lattice translational operators:
Ti = eiK·ai , (A1)
√ √
a 3 1 a 3 1
where i = 1, 2, which perform translation by Moire lattice-vectors: a1 = θ − 2 , 2 and a2 = θ 2 , 2 . Further,
define guiding-center momenta:
y x
Kx = Πx + 2 , Ky = Πy − 2 , (A2)
lB lB
An extended magnetic Brillouin zone (MBZ) is spanned by magnetic-reciprocal lattice vectors: g 1 and g 2 /q (where
g i are the original Moire reciprocal lattice vectors). As we now show, the commensurability integers (p, q), determine
the number of sub-bands, and size of the reduced MBZ. The commutation relations for T1 and T2 give:
implying a set of degenerate states T2j |αki ∼ |α, k + jp q g 1 i (j = 1, 2, . . . , q − 1), which have identical energy since
[H, T (a2 )] = 0. Thus there is a q-fold degeneracy along the g 1 direction. Equivalently, we can consider a reduced
magnetic
Brillouin
zone spanned by g 1 /q and g 2 /q with q-fold degeneracy. In addition, Eq.(A8) implies: Eα (k) =
Eα k + pq g 1 , that is, one period in a magnetic band extends over p MBZ’s in the direction of g 1 . The reduction of
energy bands to one MBZ will yield p different subbands. For convenience, we extend Eα (k) to Eα (k + lg 1 ) ≡ Eαl (k)
where l = 0, 1, . . . , p − 1 represents subbands and k is restricted to the reduced MBZ.
Having identified the distinct magnetic sub-bands and reduced MBZ, we can label states of TBG by: |τ, σ, n, l, ki,
where τ = 1, 2 represents layers, σ = A, B represents sublattices, n represents LL index, and l represents sub-
bands. For completeness we write the wavefunction of the LL states in the Landau gauge: hr|n, ki ∼ eiky y Hn (x +
2 2
2
k y lB )e−(x+ky lB )/2lB . However, the expressions obtained below are general and do not rely on fixing a particular
gauge. Under this basis, the single-layer Hamiltonian reads
√
2v iθ/2 √
h(θ/2) = e n + 1|2, B, n + 1, l, kih2, A, n, l, k| + h.c. (A9)
lB
To calculate matrix elements of the interlayer hopping term under this basis, we first split e−igj ·r as
where
2
Rx x − Πy lB x − ηx
R= = 2 ≡ =r−η (A11)
Ry y + Π x lB y − ηy
2 2
Notice that R = lB (ẑ × K) only acts on |l, ki and η = −lB (ẑ × Π) only acts on |ni, so we have
hn, l, k|e−igj ·r |n0 , l0 , ki = hn|e−igj ·η |n0 ihl, k|e−igj ·R |l0 , ki. (A12)
√
The first term on the right hand side of Eq.(A12) is given by hn|e−igj ·η |n0 i = Fnn0 g j lB / 2 , where
r 0
n ! (−zx + izy )n−n0 e− z2 Ln−n
2 0
(z 2 ) n > n0
n0
n!
Fnn0 (z) = r (A13)
n! (z + iz )n0 −n e− z2 Ln0 −n (z 2 ) n < n0
2
0 x y n
n!
with L being the associated Laguerre polynomial.
The second term on the right hand side of Eq.(A12) can be converted to matrix elements of magnetic translation
2
operators by using e−igj ·R = e−ilB K·(gj ×ẑ) . Specifically:
q q
−p
e−ig1 ·R = T2 and e−ig2 ·R = T1p . (A14)
q
−p
Considering T2 |αki ∼ |α, k − g 1 i and applying the commutation relation between T1 and T2 , we can obtain
q
−p q
T2 |l + 1, ki = e−i p k·a2 |l, ki. (A15)
q q
p ip (k·a1 +2πl)
T1 |l, ki = e |l, ki (A16)
The numerical plots shown in the main text were obtained by diagonalizing this inter-layer hopping matrix truncated
to a sufficiently large range of Landau indices n to achieve well-converged cutoff-independent results. Notice that the
direct truncation in LL basis will introduce √
an artifical zero mode in Eq.(A9). To remove it, we add a penalty term
2Ncutoff v
EP |2, A, Ncutoff ih2, A, Ncutoff | with EP lB to Eq.(A9) in the numerical calculation.
In this section, we derive the MHA electron-phonon coupling. For the convenience, we can write Hamiltonian under
the lattice distortion Hu as Hu = H0 (Π) + Ht (r − u(r)), where
h(−θ/2) 0
H0 (Π) = (B1)
0 h(θ/2)
and
0 T (r − u(r))
Ht (r − u(r)) = . (B2)
T † (r − u(r)) 0
Then we implement the co-moving frame transformation with Wu = e−iu(R)·Π on H0 (Π) and Ht (r−u(r)) respectively.
Since [R, Π] = 0, for small u we have
In this section, we estimate the relevant energy scales for the onset of Landau damping (zb = 3) for the phonons,
and non-Fermi liquid behavior of electrons, using self-consistent one-loop propagators (random phase approximation).
While uncontrolled at asympotitically low-temperatures in the non-Fermi liquid regime, this approximation produces
a reliable estimate of the onset for non-Fermi liquid behavior approaching from the high-temperature perturbative
regime. Unless otherwise specified, all propagators are specified in imaginary time (Matsubara frequency).
The (imaginary time/Matsubara) bare phonon propagator and bare electron propagator are given respectively by
D0−1 (q, Ω) = −ρλ Ω2 + ωq2
(C1)
G−1
0 (k, ω) = iω − εk (C2)
where for the long wave limit the phonon dispersion is ωq ≈ cs |q| and εk is the electron dispersion and λ = m/r is the
label for mean and relative displacement phonon modes respectively.
With electron-phonon interaction, the full phonon propagator depends on the phonon self-energy as D−1 = D0−1 −Π.
At the lowest order of electron-phonon interaction, the one-loop phonon self-energy can be calculated by
Z 2
d kdω
Π(q, Ω) = G0 (k, ω)G0 (k + q, ω + Ω)Γ2α,λ (k, q) (C3)
(2π)3
where α = L/T is the label for longitudinal and transverse mode, ρm = 2ρ, ρr = ρ2 (ρ is the mass density of single
layer graphene). At the limit q → 0, only the nonvanished coupling Γ2α,λ (k, q̂) is left. After performing the integrals
2
kk
for the patch dispersion εk = vF k⊥ + 2m , we can obtain
|Ω|
Π(q, Ω) = γα,λ (C4)
|qk |
13
where qk is the component parallel to the fermi surface and the Landau damping coefficient γα,λ is given by
|m|
Γ2α,λ (k, q̂)q̂kFS
γα,λ (q̂) = (C5)
2πρλ vF
where m is the effective mass of electron. Then, the full phonon propagator reads
1
D(q, Ω) = − . (C6)
ρλ Ω2 + ωq2 + γα,λ |q|Ω|
k|
Using Ω ∼ cs q, the energy scale below which Landau damped modes dominate is
s
√ cs |m|
ELD,α,λ ∼ γα,λ cs = Γ2α,λ (k, q̂) (C7)
2πρλ vF q̂kFS
we can obtain the one-loop electron self-energy at the Fermi level defined by G−1 = G−1 0 −Σ
Z 2
d qdΩ
Σ(ω) = D(q, Ω)G0 (q + kF , Ω + ω)Γ2α,λ (k, q̂)
(2π)3
! 13
Γ4α,λ 2
=i √ 2 2
|ω| 3 sgn(ω) (C9)
2 4
12 3π ρλ vF |m|cs
In this section, we give the propagation intensity of a surface acoustic wave on twisted bilayer graphene, which
is attenuated by the electron-phonon scattering and decaying as e−r/ξ . Here we consider the surface acoustic wave
generated by a line source and the phonon propagator in the direction perpendicular to the source is given by, the
retarded phonon propagator:
Z
R 1 1
D (r, q̂, ω) = dqeiqr 2 ω (C11)
ρλ ω − c2S q 2 − iγ(q̂) |q|
Note that for larger imaginary part of poles, the decaying rate of the integral is larger, thus we want to find the pole
with the smallest positive imaginary part which dominates the attenuation. Solving (x − x3 )2 + λ4 = 0 gives 6 roots:
β ± iα, −β ± iα and ±i2α, where
1 2 1 1 1 2 5
23 η3 − 2 · 33 23 32 η 3 + 2 · 36
α= 2 1 , β= 2 1 (C14)
2·6 η3 3 2·6 η 3 3
√
with η = 12 + 81λ4 + 9λ2 . Hence the smallest positive imaginary part of poles is α and correspondingly the typical
decaying length ξ is given by
r cS λ
ξ= = (C15)
yα ELD α
λ2
When energy scale of acoustic wave is much larger than Landau damping scale, i.e., λ 1, α = 2 + O(λ6 ), thus
2cS 2ω
ξ≈ = (C16)
ELD λ γ
2
2
On the other hand, for energy scale much smaller than Landau damping scale, i.e., λ 1, α = 21 λ 3 + O λ− 3 , thus
13
2cS ELD
ξ≈ (C17)
ELD ω
To compute the electronic life-time for temperatures or frequencies above the Landau-damping scale ELD , we
compute the tree-level electron-phonon quantum and transport scattering rates using the bare (undamped) phonon
propagator, and focus on the relative (interlayer-sliding) phonons which have two orders of magnitude stronger
interactions with electrons.
We work in a patch description of the Fermi-surface, which captures the universal aspects of the leading-order
singularities in the electron-phonon scattering rate, while neglecting smooth, non-singular “background” scattering
processes. We consider an electron at initial momentum k = kx̂ above the Fermi surface in a particular (x) direction
(i.e. k is measured relative to the Fermi-momentum kF x̂). We linearize the electron dispersion near the Fermi energy,
and neglect the curvature of the Fermi-surface, εp ≈ vF px . In this computation, the electron dispersions dominates
the energetics in the x direction parallel to the Fermi-velocity, and the phonon dispersion controls the energetics in
the y (perpendicular) direction, allowing us to neglect the dispersion of the phonons along x: ωq ≈ cs |qy | (formally,
this is justified for cs vF ). For tree-level scattering rates, we may consider the Fermi-sea as Pauli-blocked, since
at this order in perturbation theory, additional virtual electron-hole pairs cannot be excited. These approximations
capture the leading singular behavior of scattering rates in the perturbative intermediate-temperature scale regime.
Writing the relative layer displacement field d in terms of annihilation operators aλ,q that destroy a phonon with
polarization λ and wave-vector q:
X 1
λ,q aλ,q eiq·r + h.c. ,
d= p (C18)
λ,q
2ρλ cs |q|
In the above-described setup, the electron couples only to a single polarization of the phonons, so we may drop the
polarization indices, and write the corresponding electron-phonon coupling interaction coefficient as Γr,λ,k := Γ
We first compute the total electron scattering-rate, which enters the so-called “quantum” scattering rate that effects
quantum-coherent processes such as quantum-oscillations:
Z k Z k
Γ2 Γ2
Z
−1 dqx dqy dqx
τQ = 2π δ (vF qx − cs |qy |) = (C19)
0 2π 2π 2ρr c s |q y | 4πρr cs v F 0 qx
where the δ-function enforces energy conservation, and the integration limits [0, k] on qx reflect momentum conserva-
tion and Pauli exclusion. The integral is logarithmically divergent in the infrared (IR, small q). This effect is directly
analogous to similar infrared singularities arising in soft-photon emission in quantum electrodynamics (QED), where
the logarithmic divergence is physically cutoff by an external IR scale such as the energy resolution of the detector.
15
MFP T2 ( m K 2)
MFP T2 ( m K 2)
104 104 104
FIG. 5. Prefactor of mean free path – l × T 2 versus electron filling for (a) θ = 1.5◦ , ν = 1/3 and (b) θ = 1.1◦ , ν = 1/2
and (c) θ = 0.8◦ , ν = 1.
In this regime we see that the quantum lifetime is dominated by very small angle, low-energy scattering processes.
To properly account for these infra-red divergence, in the following section, we implement a semiclassical treatment
which is equivalent to resumming the divergent soft-collinear radiation processes to infinite order [39].
For transport, small angle scatterings are ineffective at relaxing momentum. A standard cheap way of accounting for
this is to weight the scattering processes by the change in angle, which for small angle scattering can be approximated
2
q
by inserting a factor of kFy into the above integrals. This angle-weighting results in a non-diverging transport
scattering rate:
2
Γ 2 vF
−1 k
τtr = ∼ T2 (C20)
8πρr c3s kF
At temperature T , electrons typically have momentum k ∼ T /vF relative to the Fermi surface, and we see that
the above expression gives a ρ(T ) ∼ T 2 contribution to resistivity. Fig. 5 shows the prefactor of the mean free
path l ∼ T −2 versus electron filling. We emphasize that, despite the Fermi-liquid like scaling of resistivity, the
logarithmically divergent quantum-lifetime signals a breakdown of Fermi-liquid quasi-particles.
In this section, we study the problem of an electron directly coupled to MHA-phonons for intermediate to high
energy regime where the phonons are not yet overdamped (the analogous problem in the asymptotic low-temperature
non-Fermi liquid regime was previously studied using a quantum Boltzmann equation approach [51]). This situation
is relevant not only for MH-polaron problems involving a single electron, but also allows a non-perturbative effective
resummation of divergent radiative corrections due to emission of soft collinear phonons at energy scales exceeding
ELD . By numerical computation, we find that hn, k|σ̂i |n, ki ≈ β kkθi for small ki /kθ with β being a constant. The
electron-phonon vertex is then,
βevF B βevF B
Γn,m,λ (k, q = 0) = ẑ × k, Γn,r,λ (k, q = 0) = k (D1)
kθ θkθ
Because of its enhanced coupling by a factor of 1/θ, we focus on the layer-antisymmetric phonon mode, in the following.
The electron-phonon coupling, using first-quantized notation for the electron coordinate r and momentum k, and
second quantized for the phonon field u, and keeping only the leading term at small phonon momentum q (dropping
gradient coupling terms) is,
α X iq·r α
He-ph (r, k) = e u(q) · k = u(r) · k (D2)
m q m
with α = βevθkF Bm
θ
. The coupling is analogous to the paramagnetic coupling of the particle to a U (1) gauge field. Our
problem is therefore, equivalent to that of a charged particle coupled minimally to a fluctuating gauge field.
For simplicity, we consider the phonon spectrum to be isotropic with a polarization independent velocity, as it will
not effect the universal physics. The effective Feynman Lagrangian for the particle in the presence of a uniform excess
16
The dynamics of the electron is naturally described in the Schwinger-Keldysh path integral formulation [42]. The
corresponding action on the closed-time Keldysh contour C is:
Z
S[r, u] = dtL[r, u] (D4)
C
Decomposing the fields u(r, t) and r(t) in terms of fields residing on the forward time contour – u+ (r, t) and r + (t),
and the backward time contour – u− (r, t) and r − (t), we rewrite the action:
Z ∞
dt L[r + , u+ ] − L[r − , u− ]
S[r, u] = (D5)
−∞
α2 ∞
Z
Seff [r] = Se [r] + dtdt0 ∂t~r̃(t)
2 −∞
(D + DR + DA ) (r + (t) − r + (t0 ), t − t0 ) (DK − DR + DA ) (r + (t) − r − (t0 ), t − t0 )
K
∂ 0~r̃(t0 ) (D9)
(DK + DR − DA ) (r − (t) − r + (t0 ), t − t0 ) (DK − DR − DA ) (r − (t) − r − (t0 ), t − t0 ) t
where
cl
~r̃(t) ≡ 1 1 r (t)
, (D10)
−1 1 r q (t)
17
We now make two simplifying approximations on the effective action. Following Ref. [41], we are interested in electron
motion where its position is changing slowly compared to the relevant wavelengths of the phonons being integrated out
(Lamb-Dicke approximation). This corresponds to replacing e−iq·∆r ≈ 1 in the following expression for the advanced
and the retarded Green’s function components:
dΩd2 q e−iq·∆r e−iΩ∆t
Z
R/A 1
D (∆r, ∆t) =
ρ (2π)3 (Ω ± i0+ )2 − c2s q 2
1 θ(±∆t)
≈∓ (D11)
2πρc2s ∆t
with ∆~r = ~r0 − ~r and ∆t = t0 − t. The effective action [D9] is then quadratic in r:
α2 ∞
0 DA
Z
Seff = Se [r] + dtdt0 ṙ(t) ṙ(t0 ) (D12)
2 −∞ DR DK
Furthermore, we restrict ourselves to semiclassical dynamics of the electron at zero temperature; thus ignoring the
role of thermally excited phonons. In this limit, we can ignore the Keldysh component of the Green’s function DK ,
in which case, the effective action takes the form:
Z ∞ Z ∞ cl q 0
α2 0 ṙ (t) · ṙ (t )
Seff = Se [r] + dt dt (D13)
2πρc2s −∞ t t − t0
Expanding the vector potential A to first order in r q , and integrating the non-local in time term by parts we get,
Z ∞ " Z ∞ cl 0
#
dA(r cl ) α2 q
q cl q cl cl 0 ṙ (t )
Seff = dt −2mr · r̈ − 2r · ṙi ∇Ai (r ) − − r (t) · dt 2 (D14)
−∞ dt 2πρc2s t (t − t0 )
dA(r cl )
We obtain the classical equation of motion of the polaron by integrating over r q , and expanding dt =
ṙi ∂i A(r cl ):
cl
eṙ cl × ∆B
Z t
ṙ cl (t0 )
∂t2 r cl = − − g2 dt0 2 (D15)
m −∞ (t − t0 )
where the dimensionless coupling constant
2
α2 β2 m
2 vF ν
g ≡ = √ (D16)
2πρmc2s 8 3π M cs
We now solve for the cyclotron motion of the polaron: r(t) = r0 (cos(ωt)x̂ + sin(ωt)ŷ) where we have suppressed the
cl label, for convenience. We take into account damping effects by allowing ω to be complex. To solve for ω, we first
express r(t) as a complex variable with the x and y components denoting the real and imaginary parts respectively.
Now, using the polaron equation of motion (Eq. D15), we get:
Z ∞ 0
ieiω(t−t )
ω = ωc,0 − ig 2 dt0 (D17)
t (t − t0 )2
where ωc,0 ≡ eB
m . Defining an effective frequency-dependent mass for the polaron: mp (ω) ≡
eB
ω and introducing a
UV-cutoff the small time differences, we obtain an expression for mp :
Λ Λ
mp (ω) = m 1 + g 2 log − ig 2 (D18)
ω ω
which is enhanced at small frequencies, and furthermore, diverges at ω = 0. A signature of this effect is seen in the
unconventional power law dependence of the cyclotron frequency of the polaron ωc on ∆B, discussed in the main
text, which we obtain by solving for ω using ω = meB
p (ω)
:
Λ
ω = ωc,0 − g 2 ω log
+ ig 2 Λ (D19)
ω
The real and imaginary solutions of ω give ωc and Γc respectively, and have been stated in the main text.
18
The previous section focused on the energy-damping of oscillatory MHA-polaron motion due to radiation of soft-
collinear MHA phonons. The cyclotron line-width computed there is relevant for phase-insensitive transport and
optics cyclotron resonance measurements. For quantum oscillations measurements (e.g. Shubnikov-deHaas (SdH)
oscillations in resistivity or related oscillations in tunneling density of states), the phase-coherence of the electronic
orbit is also important, and these phenomena are affected more strongly by MHA phonons.
To analyze this effect, we employ a semiclassical computation of the density of states for an MHA polaron in an
excess magnetic field ∆B away from commensurate filling, by summing up the “return” amplitudes for a particle to
start at some position, and return to that position time t later, and then Fourier transforming with respect to t.
For cyclotron motion of an electron coupled to MHA-phonons, the electron picks up a Berry phase equal to:
R
eiθB = eiα dt ṙ·u(r(t))
(D20)
This phase has quantum fluctuations due to the quantum fluctuations of u, which give a suppression factor for
α2 2
R
the quantum-oscillation amplitude ∼ e− 2 h[ dtṙ·u(r(t))] iu , where the average is taken over the thermal ensemble of
phonons (we will restrict our attention to zero temperature).
Since the phonons are much slower than the electrons, we can approximate the phonon configuration during a
cyclotron orbit as being static (fluctuations
R of phonon field are approximately quenched on the time scale of cyclotron
motion). In that limit, we can replace dtṙ · u(r(t)) → Φ where (by Stoke’s theorem) Φ is the flux of the effective
“magnetic field”
b=∇×u (D21)
through the cyclotron orbit. This approximation is valid for up to n ∼ vcFs cyclotron orbits, on longer time scales than
2πvF
cs ωc , then we would have to account for the dynamics of the phonons.
Let us begin by computing the huui correlator in real-space. We have a Matsubara action: ρ2 (∂τ u)2 + c2s (∇u)2 ,
in 2 + 1d Euclidean time. At zero temperature, the Green’s function of the phonon will just be the 3d Coulomb
potential in 2 + 1d spacetime:
1 1 1
DM (τ, r) = p ≈ . (D22)
2 2
2πρcs cs τ + r 2 τ r 2πρcs r
The hbbi correlator can be obtained by taking spatial derivatives of this propagator, giving: hbbi = −∇2 huui =
1
2πρcs r 3 . Integrating over the cyclotron orbit, we get a flux-flux correlator:
Rc
Ac Ac
Z Z
1 1 dδr
hΦΦi = ≈ 2π ≈ (D23)
2πρcs 0
r,r ⊂cyc. orbit |r − r 0 |3 4πρcs a δr2 ρcs a
−1 t
Z X 2πε X 2πε 1 2 2
N (ε) = dtImGR (r = r 0 ; t)e−iεt ≈ h e−i ωc n e−iαnΦ(u) iu = e−i ωc n e−i 2 α n hΦΦi
π 0 n n
r 2
X 2πρcs a 1 π ρcs a 2
= 2A
exp − 2 A α2
(ε − nωc ) (D25)
n
α c 2 ω c c
where in the last step, we have used the Poisson summation formula.
This result predicts a comb of Gaussian peaks centered at integer multiples of the cyclotron frequency with peak-
amplitude:
r
πρcs a
Ac ≈ ∝ ∆B (D26)
α2 Ac
19
and width:
ωc2 Ac α2 2g 2
Γ∼ 2
∝ (∆B) . (D27)
π ρcs a
2
By contrast, for elastic impurity scattering, the return probability for n-orbits is e−n (ωc τ ) , and the quantum
q
1
√
oscillation amplitude would scale like 1/(ωc τ ) ∼ ∆B. (Note that the amplitude suppression of multiple scattering
mechanisms combine in parallel not in series, so that the linear-∆B dependence of the MHA-phonon dephasing would
dominate at small ∆B over impurity contributions). Hence, the above linear-∆B scaling provides a signature of the
unconventional MHA polaron dynamics that is qualitatively distinct from conventional contributions from impurities.
We also remark that essentially identical expressions apply for analog systems of electrons coupled to emergent
gauge-like fields, such as the composite fermion liquid of the half-filled Landau level, spinon Fermi surfaces in gapless
U (1) spin liquids, and zero-wavevector quantum critical points in metals.