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Defence Technology 17 (2021) 1269e1288

Contents lists available at ScienceDirect

Defence Technology
journal homepage: www.keaipublishing.com/en/journals/defence-technology

Damage to aircraft composite structures caused by directed energy


system: A literature review
Y.X. Zhang*, Zhi Zhu, Richardson Joseph, Isfakul Jamal Shihan
School of Engineering, Western Sydney University, Kingswood, NSW, 2751, Australia

a r t i c l e i n f o a b s t r a c t

Article history: This paper presents a comprehensive review of the research studies on direct energy system effect on
Received 1 June 2020 aircraft composite structures to develop a good understanding of state-of-the-art research and devel-
Received in revised form opment in this area. The review begins with the application of composite materials in the aircraft
24 July 2020
structures and highlights their particular areas of application and limitations. An overview of directed
Accepted 16 August 2020
energy system is given. Some of the commonly used systems in this category are discussed and the
Available online 26 August 2020
working principles of laser energy systems are described. The experimental and numerical studies re-
ported regarding the aircraft composite structures subject to the effect of directed energy systems,
Keywords:
Aircraft
especially the laser systems are reviewed in detail. In particularly, the general effects of laser systems and
Composite structures the relevant damage mechanisms against the composite structures are reported. The review draws
Damage mechanisms attention to the recent research and findings in this field and is expected to guide engineers/researchers
Direct energy system in future theoretical, numerical, and experimental studies.
Laser system © 2020 China Ordnance Society. Publishing services by Elsevier B.V. on behalf of KeAi Communications
Experiment Co. Ltd. This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/
Numerical studies licenses/by-nc-nd/4.0/).

1. Introduction or atomic or subatomic particles are used to degrade, damage, or


completely destroy the targets. Directed energy systems are
Composite materials have been widely used in aircraft in- broadly classified into three main categories: 1) lasers systems,
dustries due to their excellent strength/stiffness to weight ratio, which use an intensely focused beam of energy to destroy objects
leading to significant weight reduction and strength improvement or to dazzle or to disorient peoples; 2) systems which use elec-
for the aircraft structures. In addition, composite materials offer tromagnetic waves of other wavelengths such as microwaves; and
excellent fatigue and corrosion resistance [1]. Composite materials 3) systems which use particle beams to damage the target. It is
caught attention in military applications before their commercial important to provide adequate guidance and reference for engi-
use [2]. They have been widely used in military aircrafts, and the neers/researchers in analysis and design of composite aircrafts
most desirable aspect of weight reduction would render the aircraft against the attack from direct energy systems.
to carry more weapons and increase its range. To better understand the effect of the direct energy systems on
Directed energy systems are relatively new weapon systems the aircrafts and the relevant damage mechanisms on the com-
that have been developed. These systems have seen applications in posite structures, a large number of research studies have been
battle field, and have been used to attack unmanned air vehicles conducted. This paper presents a comprehensive review of the
(UAVs) and helicopters. With further development, these systems research studies on direct energy system effect on aircraft com-
will be used even more widely. In general, all weapons in one way posite structures to develop a good understanding of state-of-the-
or another are devices that deposit energy in targets to achieve a art research and development in this area. This paper focuses on
certain type of damage. Directed energy systems are defined as the the experimental and numerical studies of aircraft composite
systems in which a beam of concentrated electromagnetic energy structures subject to the effect of laser energy systems. The
experimental studies reported include the studies and experi-
mental techniques investigating the thermos-mechanical response,
the ablation behaviour caused by laser energy dissipating in the
* Corresponding author. plasma layer near the target surface, the interlaminar damage
E-mail address: sarah.zhang@westernsydney.edu.au (Y.X. Zhang).
mechanism and other damage mechanism of various composites
Peer review under responsibility of China Ordnance Society

https://doi.org/10.1016/j.dt.2020.08.008
2214-9147/© 2020 China Ordnance Society. Publishing services by Elsevier B.V. on behalf of KeAi Communications Co. Ltd. This is an open access article under the CC BY-NC-
ND license (http://creativecommons.org/licenses/by-nc-nd/4.0/).
1270 Y.X. Zhang et al. / Defence Technology 17 (2021) 1269e1288

(CFRP, GFRP, etc). The effects from both single laser loading and fibre reinforced composites has potential to reduce the cost of
combined laser and mechanical loading are included. Numerical aircrafts, they have their corresponding advantages and disadvan-
studies reviewed include the thermal-mechanical response, abla- tages. For instance, aluminium alloys offer poor fatigue strength
tion behaviour, interlaminar effects and dynamic response of while fibre-reinforced composites have lower fracture toughness.
composite materials under laser irradiations. This review is ex- In order to overcome the disadvantages of these classes of mate-
pected to guide engineers/researchers for future theoretical, nu- rials, the idea to develop hybrid composite structural material was
merical, and experimental studies. initiated [8]. As a result, FRMLs are developed using the advantages
The paper begins with the introduction of the application of of both alloys and fibre reinforced composites, in which the com-
composite materials in the aircraft structures and their particular posite laminates are adhesively bonded to thin metal sheets [9].
application and limitations as presented in Section 2. An overview FRMLs are broadly classified into two main categories, i.e. 1)
of directed energy systems is given in Section 3, with the commonly FRMLs with aluminium alloys and 2) FRMLs with alternate metal
used systems discussed and the working principles of laser energy alloys. Some of the commonly used FRMLs with aluminium alloys
systems described especially. The experimental studies relating to are Aramid Reinforced Aluminium Laminate (ARAL), Glass Rein-
the laser system effects on the aircraft composite structures are forced Aluminium Laminate (GLARE) and Carbon Reinforced
reviewed in Section 4. The numerical studies using finite element Aluminium Laminate (CARALL). On the other hand, FRMLs with
method to simulate the direct energy system effect on composite alternate metal alloy include titanium based FRMLs and magne-
structures are presented in Section 5. Finally, the review is sum- sium based FRMLs [10]. The most commonly used type of FRML in
marized in Section 6 with recommendations of future research. the aircraft industry is GLARE, which was employed in the bulk
cargo floors on Boeing 777, United airlines Boeing 737 and 757
2. Composite application in aircraft structures aircraft, and all Boeing aircraft at QANTAS. It was also employed in
Midwest Express DC9, explosion hardens LD3 containers, Laser Jet
In general, three groups of composite materials have been 45 forward bulkhead, AT&T aircraft electronics cabinets, and the
developed for aircraft industries [2], including Fibre-Reinforced fuselage on the A380 Airbus [11]. In the context of the military
Plastics (FRPs), Fibre-Reinforced Metal Laminates (FRMLs), and application, in which higher fracture toughness is desirable, GLARE
Metal Matrix Composites (MMCs). was found to exhibit outstanding fracture toughness during bullet
hole calibre penetration [12,13]. FRMLs offer low moisture ab-
2.1. Fibre-Reinforced Plastics (FRPs) sorption, however, the main disadvantage associated with FRLMs is
the weak adhesive and cohesive strength between laminas.
Due to the requirements of high mechanical, chemical and Economically, the cost of FRMLs is five to ten times of that of a
thermal material properties, the demand of fibre-reinforced com- traditional aluminium alloy used in the aircraft industry, but they
posites to replace the metal alloy materials started since the end of can reduce the overall structure weight by 20% [1].
the 1960s. The fibres used are usually carbon, glass, Kevlar or the
combination of these, while thermosetting epoxy is generally used
as the matrix material in fibre-reinforced composites. Fibre- 2.3. Metal Matrix Composites (MMCs)
reinforced composites have been used increasingly in civilian
aircraft applications in recent decades. Extensive applications of MMCs, which are metals or metals alloys that incorporate par-
these types of composites are usually seen in Boeing 757, 767, 777, ticles, whiskers or fibres of different materials, offer unique prop-
787 and Airbus A310, A320, A330, A340 and A350. For example, the erties suitable to specific design needs [14]. In the context of the
fibre-reinforced composites have been used in the fuselage of aircraft industry, the materials with lower specific weights are used
Boeing 787 Dreamliner, and the outer and centre wing box, fuselage as matrix materials such as aluminium, magnesium, copper, silver,
and the empennage from the Airbus A350 XWB airframe [3]. tin, lead, titanium, intermetals (NiAl, Ni3Al, Ti3Al, TiAl, MoSi2), and
Carbon Fibres Reinforced Plastics (CFRPs) and Glass Fibres superalloys. MMCs were used in the 5th generation aircraft
Reinforced Plastics (GFRPs) are used in modern fighter aircrafts Lockheed Martin F-22 Raptor and the heavy transport plane Boeing
such as the Lockheed Martin F-35 Lightning II. Their particular C-17 Globemaster III. MMC composite based on alloy TiAl6V4 and
areas of application are in the load-bearing structures such as continuous fibre made of silicon carbide was used in the turbine
vertical stabilizer, tailplane, flaps and wings skin. Future military aircraft engine. In Ref. [2], the composites were made from the
cargo Airbus A400 M, C17 (USA), JSF or F35 (USA) and EFA (Europe) metal matrix and reinforced with a very fine ceramic or metallic
contains up to 40% of composites in the structural mass, covering particle with a diameter of 0.01e0.1 mm to about 15% of the com-
around 70% of the surface area of the aircraft [4]. Another class of posite volume. MMC composite B-Al (Boron-Aluminium) type of
fibre used in the FRPs is Kevlar, which is known for its extremely laminates was used on the leading edges of main and tail rotor
high strength, low specific weight, outstanding thermal properties blades of helicopters: Sikorsky S-76D, Sikorsky S-92 or Sikorsky S-
and dimensional stability. Kevlar has been used in the rotor blades 70 [15].
of the American helicopter Boeing AH-64 Apache, however, its use MMCs are ideal materials where high strength and excellent
in aircraft industries is rather limited due to the high cost associ- thermal properties are required. They are extremely reliable for
ated with it. components which are subjected to higher thermal and mechanical
Although FRPs offer advantages in terms of weight reductions, loadings. However, the use of MMCs is restricted due to the
corrosion resistance, improved fatigue life and use of fewer number extremely higher cost associated with them. Some of the
of components (lesser no. of fasteners in particular) in the aircrafts, commonly used MMCs configurations are presented in Table 1.
there are some inherent disadvantages, such as environmental
degradation, material and processing costs, impact damage and
damage tolerance [5e7]. 3. Directed energy system (DES)

2.2. Fibre-Reinforced Metal Laminates (FRMLs) The three types of directed energy system and their working
principle are introduced in this section with a focus on the laser
Although the application of advanced aluminium alloys and system.
Y.X. Zhang et al. / Defence Technology 17 (2021) 1269e1288 1271

Table 1
Different fibre-matrix configurations for MMCs [2,14,16].

Matrix Fibres

Continuous Discontinuous Whiskers Particulate

Aluminium Boron, Silicon carbide, Alumina, Graphite Alumina, Alumina- Silicon Silicon carbide, Boron carbide
silica carbide
Magnesium Graphite, alumina Silicon Silicon carbide, Boron carbide
carbide
Titanium Silicon carbide, Coated boron Titanium carbide
Copper Graphite, Silicon carbide, Niobium-titanium (wires), Niobium-tin Silicon carbide, Boron carbide, Titanium
(wires) carbide

3.1. Working principles and types of DES knowledge of the intended target is used to develop a high mi-
crowave source to generate an induced voltage.
3.1.1. Lasers
The acronym laser stands for “light amplification through 3.1.3. Particle beam
stimulating emission of radiation”, and the laser system is consid- In principle, the particle beam systems are close to the con-
ered as a device that produces a highly energetic and intense beam ventional kinetic energy systems in the sense that they rely on
of electromagnetic light. Laser light has the following qualities [16]: kinetic energy. However, instead of the projectile used in the con-
ventional kinetic energy systems, the particle beams are composed
 the light released is monochromatic, i.e. with one specific of small particles of high density moving at the speed of light. The
wavelength, which is dependent on the material of the laser and density is usually of the order of 1011 particles per cubic centimetre
the method of stimulation; [17]. The aim of employing this type of system is to destroy or
 the waves of the emitted electromagnetic radiations are in disrupt the molecular or the atomic structure of the target. The two
phase in both space and time, i.e. the light is coherent; main types of particle beam systems are dependent on the types of
 the emitted light is highly concentrated and strong; and the particles being used either particle possess electrical charge
 it does not disperse over a long distance due to the coherent (electrons or protons) or the electrically neutral particles. Usually,
nature. the electrically charged particles are suitable for application within
the earth’s atmosphere, while the neutral particles are suitable for
Laser light is thus a special case of electromagnetic radiation and space operations. However, the huge cost associated with the po-
is defined by the wavelength, frequency, and speed of light in wer supply and large fixed installations makes them susceptible to
vacuum or some other medium [17]. In the context of military attack and render them of limited military use.
applications of laser system, the type of system is determined based
on the intended target and the operating environment. In partic- 3.2. Laser energy system
ular, the vulnerability of the target and the range that it must be
engaged are two of the main factors in determining the type of laser As previously stated, laser is an intense beam of electromagnetic
to be selected [18]. radiation that is usually defined by the wavelength, frequency,
speed of light and the coefficient of refraction. Some of the most
3.1.2. Microwaves common applications of lasers are range finders, target designators,
Microwaves are another type of electromagnetic radiation with beam riding guidance, laser radar, laser communications and laser
a comparatively much longer wavelength and much lower fre- energy systems [18].
quency than light. Microwaves have been used in various devices
for military applications such as radars, communication links and 3.2.1. Types of laser energy systems
missile seekers [17]. However, the use of intense radio frequency The type of a particular laser system and its properties such as
waves (100 MHze3 GHz) is directed towards military targets to beam energy, wavelength, mode, peak power, and useful engage-
accomplish certain desirable military operations. Such systems can ment, for a particular application, is dependent on the intended
be used to disable electronic systems by inducing a voltage to the target and the operating conditions. In terms of energy levels, the
hardware to destroy or disrupt electronic circuit boards, their lasers are characterised as low-energy, medium-energy, and high-
components and software controls. The four levels of effects are energy laser. The associated power for the low, medium, and high
roughly categorised as [18]: energy laser is in the range of <1 kW, 10 kWe100 kW and >100 kW
respectively, while the energy range is < 1 mJ/cm2, > J/cm2 and
 noise, in which the operating signals generated by the source is >1 kJ/cm2 respectively. The damage linked with the low energy and
not extracted by the receiver; medium laser energy system is usually the destruction of a small
 false information, which is generated via the receiving end; circuit or an electronic device. On the other hand, a high energy
 induced voltage from the source which causes transient upset, laser system is used for aiming the destruction of a structure. In this
i.e. upset the logical operation of the targeted electronic context, the high-energy laser systems are the first choice from a
equipment; and military point of view. Lower energy laser systems may produce a
 induced voltage, which could permanently destroy the target. targeted flash or continuous beam that temporarily blind human
being [16].
In general, depending upon the frequency and waveform, two Lasers are also defined by means of the lasing media, i.e. solid
basic types of high-power microwave systems are available, i.e. the state, liquid or gas. In particular, the high energy laser systems are
narrow band and the wide band system. The selection of different powered by a chemical fuel, electric power, or a generated stream of
combinations of the technologies along with the available an electron. The chemical laser setups may achieve high energy
1272 Y.X. Zhang et al. / Defence Technology 17 (2021) 1269e1288

level lasers, however their use for the military applications is 3.2.2.3. Mechanical effects. Due to the vaporization of the target
limited due to the challenging requirements of volume, weight and material, the momentum transfer into the material’s depth is
fuel logistics, which require large platforms and stationary in- termed as the mechanical effect of laser system onto the target. As
stallations. On the other hand, the solid-state lasers are more stable mentioned above, the reaction forces exerted by the vapour at the
and easily transported but are very low in efficiency as most of the surface serves to deform the target even without physically
energy is lost as heat. Moreover, the free-electron lasers use a removing bulk material. Thus, the energy required for the me-
stream of electrons that passes through alternating magnetic fields chanical damage of the target could be lesser than that for the
to generate high energy laser beams, but their use is restricted due thermal damage, though a higher intensity beam is required for the
to the huge size. mechanical effects. From the military point of view, the pressure
and impulse required to cause the mechanical effect on the struc-
3.2.2. Laser-target interaction ture and its material are dependent on the degree of damage
The laser-target interaction is primarily dependent on the co- required.
efficient of refraction-n and an attenuation coefficient-K, which Overall, it is well understood that the required intensity for the
describes the extent to which the beam flux is reduced as it passes target erosion (melting or vaporization) damage is comparatively
through a specific material. The beam’s intensity is decreased as it less than that for the mechanical damage. On the other hand, the
travels from the source to the target. The beam parameters which mechanical damage may require higher laser intensity but less
may be adjusted to compensate the decremented effects are en- energy to carry on. In several laser-target interaction phenomena,
ergy, pulse width, beam diameter, and the wavelength. From a the plasmas are more likely to occur and influence the interaction
broader perspective, the target effects are either thermal or me- at higher intensities [17].
chanical. The effects are also found to be dependent on the pres-
ence of plasma, which is defined as the state of matter in which the 4. Experimental studies
ionised gaseous molecules become electrically conductive to
deliver long range electrical and magnetic fields, dominating the In this section, the experimental studies of the laser system
matter’s behaviour. effects on aircraft composite structures are reviewed.

4.1. Laser loading only


3.2.2.1. Heating and melting. The most basic laser-target interac-
tion effect is heating. When laser light is incident upon the target 4.1.1. Thermal-mechanical response
surface, some fraction of the energy is absorbed, which is presented Herr et al. [19] investigated the effect of high energy laser sys-
as heat. The heat by itself is not enough to damage the target unless tem (HEL) on CFRP panels and the thermal-mechanical response of
the target is very soft [17]. Hence, from a military point of view, the CFRP panels. A 1.07 -mm, 2-kW continuous wave ytterbium laser
heating alone would not be a desirable effect to damage the target was used to irradiate the CFRP panels of varying thicknesses (1.7,
material and structure. However, when the surface of the target is 2.4, 3.2 mm) with 4, 6 and 8 plies of 6 K 2  2 twill weave carbon
heated, the energy which deposits on the surface will start to fibre fabric based on Bisphenol A diglycidyl ether (DGEBA) epoxy
propagate into the material. The propagation depends on the resin blended polymer matrix. The temperatures at the front and
thermal diffusivity of the material and the time, and as a result the back surface of the irradiated panels were recorded by mid-infrared
surface temperature rises. The target surface may begin to melt if camera, and the spatial and temporal laser beam irradiance varia-
the temperature of the heated region reaches the melting point of tion was recorded by near-infrared (NIR) camera. A 30-Hz visible
the material. At the same time, when the intensity on target is camera was also used to monitor each test which was conducted on
weakened (which reduces the heating as well) other energy loss an open optical table with ceiling mounted ventilation hood. All
mechanisms, such as convection and the re-radiation of energy will test panels were shaped to 10.38 cm  10.38 cm. Laser with 5, 10,
come into play. Similar to the heating, melting alone would not be 36, and 64 W/cm2 output was used to irradiate the 3.2 mm thick-
damage the target in military applications. To cause significant ness panels, and laser with 10 and 36 W/cm2 was used to irradiate
damage, it is necessary for the laser beam to make a hole into the the 1.7 mm and 2.4 mm thickness panels respectively. The laser
target surface, and the rate at which the hole increases in depth is spot diameter was 2.3 cm for the 64 W/cm2 output and 6 cm for all
called the material’s erosion rate. If the molten material is removed others. All tests were run for 2 min or until surface ignition
from the hole, the new material would be exposed to the laser occurred. A FLIR SC6000 MWIR camera was used to record thermal
intensity and hence more damage will occur. However, if the imageries. The recorded data were processed via a thermal model
molten material remains in the hole, more energy would be needed with a single set of temperature-dependent thermal, optical and
for further damage. kinetic parameters based on heat diffusion equation, coupled with
a sequence of visible images, to estimate the CFRP thermal prop-
3.2.2.2. Vaporization. If the molten material remains in the hole, it erties and kinetic parameters during matrix decomposition. Igni-
must be vaporized before the laser causes more damage. Therefore, tion was found to occur at T ¼ 1198 ± 50  C under any
the incident laser intensity on the target surface must be high circumstances, which was found to accord with a laser threshold of
enough to accommodate the energy required for the vaporization. 21 W/cm2. It was found that high energy system (HEL) posed
For faster vaporization of the molten materials and hence further detrimental effects to the CFRPs, albeit being incapable of
damage, the heat vaporization must be faster than the erosion. In completely removing its materials.
general, propagation losses will require the laser fire with much Thermal shock strength of the laminated carbon-carbon (C/C)
greater intensities, in order to hit the target with the intensity composite subjected to laser heating up was investigated by a few
necessary for damage. The vaporization, in turn, would transfer the researchers. The manufacturing process and fibre texture are highly
momentum into the depth thus causing the damage by mechanical associated with the mechanical properties of the C/C composite,
effects. For example, the vapour at the surface would act as a small and the failure mechanisms of the C/C composite was found to be
jet and further exerts reaction forces back to the target which very sensitive to the failure between the two layers with low shear
causes deformation without physically vaporizing the bulk strength, thus entailed the developing of a new method of evalu-
material. ation for thermal shock shear strength of laminated C/C composite
Y.X. Zhang et al. / Defence Technology 17 (2021) 1269e1288 1273

[20e23]. Li et al. [24] evaluated the thermal shock strength of the assessed prior to the decomposition experiments using a non-
laminated C/C composite subjected to laser heating up, and the linear inverse heat conduction method. Following each test, a
acoustic emission (AE) was used to detect fracture which corre- post-decomposition micrographic analysis was conducted from
sponded to the critical power density of the laser to obtain the longitudinal cross sections of the coupons. The highest temperature
thermal shock strength. The fracture was assumed to be initiated by magnitude was observed at the centre of the coupons where the
the induced stress over the shear strength of the material, and the thermal loading at the front side was the highest. No in-plane
critical fracture curve was derived as a function of power density deformation was detected from the IR measurements. However,
and beam diameter. The laminate of eight-harness stain-weave temperature-activated chemical reactions occurred which affected
cloth with 40% overall volume fraction of carbon fibres with 7.8 MPa the resin through a pyrolysis charring process. From 150 s exposure
shear strength, 137.3 MPa compressive strength, and 606 MPa duration, the composite coupons experienced critical temperature
tensile strength, was used in the experiments. CO2 laser with the drops which can reach 60 K as observed for the third text coupon.
maximum power of 1 kW was used to irradiate the rectangular Such sudden decreases in temperature could only result from
specimen (50 mm  50 mm  20 mm). Experimental results breaks within the continuous medium, which caused local thermal
concluded that the shear strength criterion was appropriate for the contact resistances. When the maximum temperature on the cold
evaluation of the thermal shock strength of the C/C composites. surface reached 550 K, delamination was seen onset in all tests.
Additionally, the maximum shear stress was found to occur at the Nevertheless, identical experimental conditions and thermal
periphery of the laser beam and beneath the surface and increase loading resulted in different delamination damage and post-
with the growth of the laser beam diameter and power density. damage behaviours in terms of onset time, suggesting that
Uhlmann et al. [25] studied the thermal damage on the unidi- delamination may depend on many parameters with temperature
rectional (UD) carbon/epoxy laminate caused by laser grooving. The and exposure time strongly correlated. The deepest delamination
laser beam was supplied by two CO2 lasers of 10000 W and 1500 W, cracks were identified as the consequence of the mechanical
respectively with 0.17 mm and 0.25 mm focus spot. Grooving ex- damage induced by high thermal gradients and a non-symmetrical
periments were carried out at beam power ranging from 350 to stacking sequence. Moreover, experimental results confirmed that
1500 W in continuous mode and at scanning velocities of the large resin-rich regions at ply interfaces offered preferential
2.5e110 mm/s, and an N2 gas jet flow coaxially to the laser beam paths for the cracks initiation and propagation of T700GC/M21
was applied to protect the focusing lens from debris and to provide laminates.
an inert environment for beam-material interaction. Thermal Herr [27] measured the emissivity-adjusted surface tempera-
conductivity of the carbon/epoxy was measured at 23  C by the tures from laser irradiated CFRP using a mid-wave infrared thermal
Laser Flashing Method using a Holometrix Microflash instrument, camera. In the study, the CFRP targets were irradiated with a
conforming to the ASTM E146-92. Experimental results showed 1.07 mm ytterbium doped continuous wave fibre laser at irradiances
that the heat affected zone was approximately proportional to the ranging from 5 to 525 W/cm2 and 780-3000 W/cm2, respectively.
specific laser energy density. Also, it was found that less thermal Surface temperatures of the specimens were measured. The CFRP
damage would be produced under higher laser traverse velocity, testing panels were of 10.38  10.38 cm2 and thicknesses of 1.7, 2.4,
evidenced by the fact that the heat affected zone was reduced as 3.1 mm, irradiated by a 2-kW continuous wave IPG Photonics
laser traverse velocity increases. ytterbium doped fibre laser at 1.07 mm. The test set up is shown in
Leplat et al. [26] investigated the thermal response and damage Fig. 1. The panels were manufactured by layering multiple plies of
evolution of composite laminates subjected to laser heating in the 6 K 2  2 twill weave carbon fibre fabric in a mould and injecting
test chamber of the BLADE (Banc Laser de cAracte’risation et de epoxy resin under vacuum. The samples contain 4, 6 and 8 plies. A
Degradation) facility developed at ONERA to analyse the aniso- DGEBA based epoxy resin was used. The 3.1 mm thickness panels
tropic and heterogeneous behaviour of decomposing composite were irradiated at 5, 10, 36, and 64 W/cm2 by the 2.3 cm diameter
laminates. The square (80 mm  80 mm) test coupon (T700GC/M21 laser beam. A beam splitter was used to illuminate a stationary
composite laminate) was heated up by continuous laser (1080 nm scatter plate and the spatial and temporal laser beam variation was
wavelength, maximum power of 50W) inside an air-filled pressure- recorded by a calibrated near-infrared (NIR) camera. Tests were set
and temperature-regulated chamber. Sixteen 260 mm thick M21/ up on an open optical table with ceiling mounted ventilation hood,
35%/268/T700GC unidirectional 268 g/m2 prepreg plies were and thermal imagery was recorded by a FLIR SC6000 MWIR camera
stacked into the composite laminate. Especially, the M21 resin operated with a bandpass filter from 3.8 to 4.0 mm and neutral
demonstrated high tolerance to damage under high energy im- density filter of O.D. 1.0. The spectral emissivity of samples was
pacts. The orientations of the plies in the quasi-isotropic layup were observed from 2 to 25 mm with an SOC-100 HDR (Hemispherical
[0 /45 /90 45 /0 /45 /90 /-45 ]s. The average diameter of fibres Directional Reflectometer).
was 7 mm and the volume fraction of fibres was 0.57. The final Decomposition produced billowing clouds of volatile products
thickness was 4.16 mm. At the unheated side of the test coupon, the with soot beginning at surface temperature of around 430  C.
transient temperature was measured by quantitative infrared Enough volatiles were produced on the backside of the panel which
thermography at 10 Hz acquisition frequency. Additionally, the test was ignited by the front side flames at around 600  C. The radius of
chamber was vacuumed to reach 3 mbar (300 pa) to avoid any visible change ranged from around 2e3.5 cm for 5e35.7 W/cm2
convective heat transfer and volatiles flaming. The quantitative using the 3 cm laser beam radius. No significant mass loss was
infrared thermography technique used a FLIR SC7650 infrared observed for total incident energies of less than 7.7 kJ and 5.2 kJ for
camera equipped with a mid-wave [3e5 mm] high-sensitivity InSb non-ignition and ignition cases, respectively, at 6-cm laser spot
detector. Four different integration time was used with specific diameter. However, no mass loss was observed for total incident
calibrations for each temperature range to precisely cover the energies of less than 2.8 kJ at 2.3-cm laser spot radius. The
response of the test coupon with a dependable temperature reso- appearance of combustion flames increased the mass loss rate by
lution. The orientation of each test coupon in the experiment was 45%. Resin matrix removal resulted from HEL heating was found to
accurately performed upon aligning the fibre direction of the first be incapable of completely compromising the material, however, it
0 - ply along the horizontal plane. The laser-generated a constant did inflict several detrimental effects including fouling optics and
non-uniform heat flux of maximum 220 kW/m2 which exerted 40- electronics, providing a fuel source for combustion, which reduced
W thermal loading on the material front surface. The heat flux was the repressive strength of the CFRP.
1274 Y.X. Zhang et al. / Defence Technology 17 (2021) 1269e1288

Fig. 1. Experimental setup [27].

Berlin et al. [28] carried out an investigation to ascertain the the middle while the second one was placed at the rear surface. In
effects of heat radiation on several polymer composites, including addition, an optical pyrometer was installed to measure the tem-
composites reinforced with carbon fibres and E-glass. Laminates of perature of the front surface. Testing was conducted at several laser
carbon/polyetheretherketone (PEEK), carbon/epoxy and glass/ intensity levels, using a fixed 25 mm beam diameter with variable
epoxy namely Ciba Geigy 914C and 914G were used in the experi- power output. Furthermore, to accommodate the aerodynamic
mental study. Ciba Geigy 914C and 914G are thermosetting matrix cooling effects, Mach 0.3 airflow was applied parallel to the irra-
composites made of epoxy matrix reinforced with T300 carbon fi- diated surface during each test. This research served as the
bres and E-glass fibres, respectively. The specimens were exposed benchmark for several later reported studies.
to radiation on the entrance of an oven set at 800  C with minor Furthermore, Lacroix et al. [30] studied the thermo-mechanical
variation between the specimen and the heat source of approxi- behaviour of carbon epoxy composite under laser irradiation. The
mately 1% at intensities 30 kW∙m2. On the backside, laminates laser matter interaction was assumed to be linear for the heat
were subjected to a heat flux of 8e60 kW,m2. The temperature of transfer process. The Fourier thermal conduction model was used
the specimens was measured using infra-red (IR) pyrometer. A to predict the heat conduction, and the mechanical degradation
microbalance was used to determine the loss in mass after expo- during laser exposure was obtained through an “Equivalent Ablated
sure to radiation. In this study, the deterioration of the mechanical thickness” criteria. This criterion was defined to assess the temporal
properties of carbon-reinforced composite was found to be attrib- progression of the thermal flow inside the material despite the
uted to the delamination. The authors further argued the decay of resistance of the carbon fibres to the laser illumination by means of
composites was preceded by visual defects formed as a result of a cantilever bending test configuration. The experimental setup
exposure to heat radiation. The specimen’s (914C and 914G) dam- consisted of G939/M18-1 carbon/epoxy laminate samples (based
age was found to occur at temperature of approximately 300  C. on 8 wraps of G939 50/50 bi-dimensional prepregs with M18-1
Predicting the general laser-matter interaction demands the epoxy resin), irradiated with 10 kW IPG fibre laser with a 1.07 mm
accurate thermal analysis (as the fundamental element) in pre- wavelength. The illumination area diameter was 2 cm and the
dicting the overall composite structural reliability when subjected power density were supposed to be homogenous. Experimentally,
to rapid high intensity heating. One of the earliest work to study the the carbon fibres were found to withstand approximately 1 kW/
transient thermal response of fibre-reinforced composite plates cm2 of power density with the surface temperature reaching
was conducted by Griffis et al. [29]. In this work, a one-dimensional 3250  C.
heat transfer model was developed to predict heat conduction in
the thickness direction. The area exposed to the laser irradiation 4.1.2. Ablation behaviour
was considered to be significantly smaller than the other charac- It was indicated that a highly concentrated laser energy may
teristics dimensions of the structures. The numerical results of the cause energy waste due to laser energy dissipating in the plasma
thermal analysis (temperature distribution and ablative charac- layer near the target surface as high-power density induced optical
teristics) were compared with the experimental data and employed breakdown [31e33]. Ablation effect was strongly dependent on the
to evolve thermomechanical stress analysis and failure criteria. The deposited energy in the target material, emphasizing the impor-
experiments were conducted on the twenty-ply AS/3501-6 tance of determining the threshold of laser power density to trigger
graphite epoxy laminated composite panels of in-plane dimensions optical breakdown which caused energy dissipation. Wu et al. [34]
5.6 cm  10 cm. The thickness of the panels was set as 2.54 mm and investigated this phenomenon in their study of the laser ablation of
the panels were subjected to rapid heating using the 15 kW, mechanism of CFRP composite. In their study, CFRP specimens
continuous wave, CO2 laser. In order to measure the thermal (T800 plain woven carbon fibre cloth reinforced polymer laminate
response during irradiation, one thermocouple was embedded in of 50 mm  50 mm  4.1 mm) were tested under three groups of
Y.X. Zhang et al. / Defence Technology 17 (2021) 1269e1288 1275

laser irradiation to obtain ablation behaviours and morphologies of composite particles observed in the transition region. The surface
the CFRP. The power density for continuous wave laser, long pulsed morphology of the composite showed that the degradation caused
laser (200 ns pulse duration), and short pulsed laser (10 ns pulse by laser irradiation at different power densities ranged from
duration) was 3.54  106 W/m2, 1.50  1012 W/m2, and 4.77  102 W/cm2 to 12.1  102 W/cm2. An increase in the laser
3.00  1013 W/m2 respectively. All lasers were designed to irradiate energy contributed to ablation of the surface coating because of the
the square CFRP specimens for 10 s with random polarizations. The high temperature at the centre of the lase spot. In addition, the
surface morphologies were photographed by optical microscope composite matrix was decomposed when exposed to strong laser
and then compared to the CAD drawing. Under continuous laser resulting in the exposure of the non-ablated carbon fibre layers. The
irradiation, the CFRP specimen was ablated by several layers fol- damage to the composite was resulted from the high laser tem-
lowed by voids appearing throughout the epoxy layer after 10 s. The perature which reached the decomposition temperature of the
ablation effects on the under-epoxy laminate closely attached to composite material, although it did not reach the melting point of
the top carbon fabric were reduced because laser-induced plasma the composites. As a result, the composite was ablated while carbon
absorbed a large part of the incident laser energy as air breakdown fibres were retained but exposed on the surface of the sample. The
occurred after the surface carbon fibre fabric locally evaporated. ablation centre showed large spherical particles at the ablation
However, long pulsed wave laser drilled a conical hole through the centre which was an oxidation product of the composite material. A
laminate with largest radius around 1 mm which was smaller than high number of large spherical materials were also found to be
the laser beam radius, as compared to that the short-pulsed laser distributed at the ablation edge of the composite coating. As the
only ablated the thin surface carbon fabric of CFRP. laser power on the composite material increased, the boundary
Zhu et al. [35] studied the ablation behaviour T300/AG80 carbon between non-irradiated region and the irradiated region became
fibre reinforced laminate following layup sequence [±45 /0 /90 / clearly visible. Both the carbon fibre and composite matrix surface
0 ]S of a shape of 200 mm  200 mm  1.5 mm, under Nd:YAG were ablated. In addition to complete sublimation of the first layers
generated laser beam with 1064 nm wavelength for 5 s irradiation. of the composite and the matrix, the carbon fibres were also sub-
The laser power density was 50 W/cm2, and the laser beam radius limated. The sublimation temperatures of the silicon carbide and
was 10 mm, 20 mm, and 30 mm respectively. They used a CRONOS- carbon composite were 2700  C and 3550  C, respectively, and the
PL2-DIO dynamic strain meter to measure the specimen response. laser temperature at the centre of the composite material was
At 0 , 45 , and 90 directions at front and back surfaces of the above 3550  C.
specimens, strain foils were attached. Experimental results showed
that the larger the laser beam radius, the greater the thermal shock 4.1.3. Interlaminar effects
exerted upon the specimens. The maximum shocking tensile strain Wu et al. [38] conducted a comprehensive study on the me-
recorded in 20 mm and 30 mm laser beam radius cases are 5.7 and chanical and thermal properties of glass fibre reinforced epoxy
8.4 times the maximum shocking tensile strain in the 10 mm case, composites. The diglycidyl ether of bisphenol F epoxy resin with the
respectively. Generally, the strain value at different locations within epoxy equivalent weight of 164e172 g/mol was used. The curing
the laser spot decreased as it was farther from the centre of the agent was diethyl toluene diamine (DETD, HY5200, Huntsman
spot. Advanced Materials) with an amine weight equivalence of 44.5 g/
Stratoudaki et al. [36] investigated the effect of laser generated mol. The boron free glass fibre cloth was treated by silane coupling
ultrasound on epoxy resins using three different lasers, i.e., TEA CO2 agent. The fabric was 0.2 ± 0.022 mm thick with count of 18 ± 1
(Coherent, Hull, Laserbrand150), Q-swtiched fundamental Nd:YAG threads/cm in the warp and 14 ± 1 threads/cm in the fill. The
(Spectron Laser Systems), and XeCl excimer (Lamda Physik). A prepared composite panel was cut into specimens for the short
Michelson interferometer was used to directly measure the ultra- beam shear test with the dimensions of 24 mm  8 mm  4 mm.
sonic waveforms and record the absolute epicentral displacements 60
Co g-ray with dose rate of 300 Gy/min at ambient temperature
on the opposite side of the sample, and the samples were inspected was applied upon the specimens. The total doses of 1 MGy, 5 MGy
under optical microscope. The generation beam spot size was kept and 10 MGy were applied respectively. Through the short-beam
between 0.02 and 0.03 cm2 throughout the experiment. The carbon shear (SBS) test according to the ASTM D2344, the apparent
fibre reinforced composite (CFRC) had a thin superficial layer of interlaminar shear strength (ILSS) was determined. The specimens
resin with a mean thickness of ~12 mm. Pure epoxy resin samples were dipped inside a cryostat filled with liquid nitrogen to achieve
were prepared using resins commonly used for the manufacture of cryogenic condition. After the SBS tests, a Hitachi S-4300 SEM was
composites, of which the first was a cold-curing epoxy resin, and adopted to observe the fracture surfaces of the specimens. The
the second a warm-curing epoxy resin. The Nd:YAG operated in UVeVis spectra of the specimens were measured by a Cary 5000
TEM00 mode with pulse duration at FWHM was 10 ns and its spot spectrometer. Fourier transform infrared spectroscopy was per-
size was ~0.02 cm2. The FWHM of the TEA CO2 was 50 ns, and the formed on an Excalibur 3100 spectrometer. Distinct failure due to
spot size was ~0.03 cm2. The excimer laser had a ‘top hat’ beam the interlaminar shear was found in all cases. No clear effect of the
profile, and its FWHM was 40 ns and its spot size was ~0.02 cm2. gamma ray irradiation on the interlaminar shear strength was
Results showed that in the case of the Nd:YAG laser, most of the found when the total doses was less than 5 MGy. However, the ILSS
energy was absorbed in the first layer of carbon fibres. In the case of sharply decreased after exposed to the total 10 MGy dose. Two
the excimer laser, the ablation threshold was found to be very low radiation-induced processes, i.e., the molecular chain scission and
but the damage was localized at the superficial resin layer. No crosslinking, were identified to associate with ILSS reduction
exposure of fibres was observed in all three cases. mechanisms. Specifically, the chain scission generally reduced the
Pan et al. [37] investigated the ablation mechanism and the ef- cryogenic strength and stiffness of the matrix which resulted in the
fects of laser parameters in laser ablation of carbon fibre reinforced degradation of the ILSS. After 10 MGy irradiation, the ILSS was
silicon composites. The researchers used six different laser power found being decreased by around 58%. Thermogravimetric analysis
densities and six levels of pulse numbers. Results revealed that showed that the initial degradation temperature (IDT) of the
damage to surface morphology included three areas: the board specimens decreased drastically after the irradiation with a
region, the transition region, and the centre region. As the laser decrease of 18% and 25% in IDT respectively from 5 MGy to 10 MGy
power density increased, the ablation at the centre region compared to that of the non-irradiated specimen. Overall, the
increased significantly with the surface cracking with spherical composite laminate could resist the dose of 5.0 MGy.
1276 Y.X. Zhang et al. / Defence Technology 17 (2021) 1269e1288

Following the work done by Wu et al. [34], Liu et al. [39,40] pulse propagating through the sample thickness to the opposite
further investigated the CFRP composite laminate interacting with surface where it bounced back in tension could induce damage.
infrared wave laser, and interlaminar damage of CFRP laminate Firstly, the experiments were performed on the 4-ply lamina and a
under continuous laser irradiation. The 2 mm thick CFRP lamina delamination threshold for an incident intensity of [0.9e1.03] GW/
synthesized from CCF-700 carbon fibre and BA9916-II resin matrix cm2 was detected. Secondly, the 8-ply lamina was tested under
was autoclave treated and then being irradiated by infrared laser of irradiation of 450 ns pulse duration laser, and the 1.49 GW/cm2
1064 nm wavelength and 200 ns pulse duration repeating at 10 Hz. laser intensity was found to be strong enough to induce delami-
The specimen was compacted by 16 laminates of a thickness of nation. The microtomography X-Tek HMXST 225 was used to
0.125 mm by [45 ,0 ,-45 ,90 ]2s sequence, and then shaped into examine recovered samples. The incident intensity to induce
50 mm  50 mm  50 mm cube with 145±g/m3. The specimen was delamination in the 8-ply case was found higher than that in the 4-
irradiated by the infrared laser of 1064 nm wavelength by pulse ply case, and it was observed that laser-induced stress waves could
duration of 200 ns repeating at 10 Hz. The laser spot radius was produce on-axis tension which caused delamination of the speci-
1.1 mm and the output power were around 1.1 J. Optical microscope mens. The tensile strength of both the 4 and 8 ply lamina was found
was used to observe cut cross sections of the CFRP specimens. It to be around 292 MPa, which was in the same range as the strength
was observed that the longer irradiation would cause wider hole at evaluated by Yu and Gupta [47], and Riedel et al. [48].
the back surface of the specimens after it was penetrated and Laser shock wave techniques have also been used to experi-
around 10 s were required to drill the specimen through. In addi- mentally examine the damage of directed energy on composites
tion, Finite Element model was utilized to investigate the temper- which are widely used in the aerospace industry. Ecault et al.
ature and phase change of the specimens. A wider hole than that [49e51] first examined how laser shock wave impacted on carbon
from the experiment as well as a coarse aperture wall were pre- fibre reinforced polymer (material T800/M21). The T800/M21 is a
dicted from the numerical simulations. common composite material in the aeronautical industry, made
When being exposed to high temperature, CFRP laminates from mon-conventional matrix that is mixed from thermoplastic
became very susceptible to deterioration in mechanical properties, nodules and thermoset epoxy resin whose mechanical character-
and composite gradients are prone to flaming [41,42], and inter- istics are created to improve shock resistance. Besides their
laminar thermal damages induced by ablation could lead to adequate mechanical properties, T800/M21 composite materials
disastrous consequence on CFRP laminate. In theory, it was the are also used in the aeronautics industry because of their light
propagation of the interlaminar cracks that governs the interlam- weight. Characterization of T800/M21 materials for various defects
inar separation of the CFRP and was greatly dependent on the fibre has been achieved in the past using Interferometric Confocal Mi-
lay angles. However, the multi-interlaminar shear failure mode was croscopy, X-ray Radiography, and Optical Microscopy. Ecault et al.
basically attributing to the weak fibre-matrix interface in the CFRP. used Carbon Fibre Reinforced Polymer (CFRP) samples for the
In the work done by Liu et al. [40], the interlaminar damage mor- experiment to assess how laser shock waves impacted on com-
phologies of the CFRP laminate under continuous laser irradiation posite materials. The researchers first conditioned the samples by
was recorded. Acquired interlaminar damage pattern and its spatial shocking them with various laser energy levels to generate diverse
distribution were further analysed. An optical microscope and a levels of internal damage. The samples were then recovered from
scanning electron microscope (SEM) were used in the study. The the set-up for analysis using several diagnostic setups. The first
same specimen in the previous study [39] was used again but was shocks were performed on thin T800/M21 samples measuring
irradiated vertically by continuous wave laser in a cabinet filled of 1.5 mm that were extracted by cutting out from thicker materials.
Nitrogen. The continuous wave laser of 1070 nm wavelength was Optical micrography was used to analyse the samples which were
used to irradiate the specimens for 3 s by output of 500 W, 800 W exposed to laser shock waves. The analysis was used to assess the
and 1000 W respectively. The optical microscope and SEM were correlation between laser intensity and damage characteristics on
used to observe the interface damages at cross section of the the composite material. The second shock waves were done on
specimens. Morphologies at cross section were recorded, illus- thicker materials of 6 mm as shown. Resulting damage was ana-
trating pyrolysis occurring in up to eight laminate from the surface lysed using Interferometric Confocal Microscopy (ICM) and X-ray
layer where fibre fracturing under direct irradiation. Similar to the radiography on the back face of the samples. The obtained data was
phenomenon observed in carbon/carbon composite exposed to used to assess the damage threshold done on the T800/M21 CFRP
elevated temperature [43], the interlaminar cracks were found to because of laser shock dynamic loading. Results from the 1.5 mm
increase in width and length as laser power output rise, and at T800/M21 composite samples revealed that the damage induced by
around the backward surface large interlaminar cracks were seen. laser shock was cone shaped through the sample thickness. The
cone basis was situated at the back of the face.
4.1.4. Damage analysis For the different laser shocks, the sample exhibited a similar
Gay et al. [44] studied the local tensile stress caused by laser- kind of damage despite the laser strength used. Ecault et al. [49e51]
induced shock within CFRP composite laminates involved in aero- also performed laser shocks on 66 mm thick T800/M21 CFRP
nautic and defence industry. They selected the carbon fibres G40- samples. Like the thin samples, four different laser pulse intensities
800-24 K reinforced epoxy Cytec® 5276-1 with 4 and 8 ply lami- were used. Results showed that since the samples were thick, the
nates by layup sequence [0 /90 ]S and [0 /-45 /90 /45 ]S respec- laser did not spall them. The laser shock wave amplitude was
tively as test specimen which were shaped to 15 mm  15 mm with decayed through the material’s thickness as there was a longer
a thickness of 600 mm and 1200 mm respectively. The average distance to close before emerging from the other side of the face.
diameter of the carbon fibres is 5 mm and their volume fraction is The resulting damage was evident in the form of small blisters on
70%. A linear-elastic law [45,46] was used to describe the dynamic the material back face based on the ICM and X-ray radiography
behaviour of the composites. In their adhesion test, the load was measurements. In summation, it was observed that the damage
generated by a Nd:YAG laser which delivered a calibrated pulse resulting from the laser shock wave propagation on composite
with a duration of 9.3 ns at Full Width at Half Maximum (FWHM) materials was resulted from laser intensity. A potential damage
and an energy of 1.5 J with 532 nm wavelength. The high intensity scenario for the T800/M21 composite due to high laser irradiation
pulse drove a compression wave within the specimen to test and was shown revealing the damage tolerance of aircraft composite
was eventually released to relax the material to its initial state. The materials when exposed to high energy laser wave shocks.
Y.X. Zhang et al. / Defence Technology 17 (2021) 1269e1288 1277

Ecault et al. [49e51] then examined composite material damage sample had a blister diameter of 8.5 mm compared to the blister
resulting from laser-induced shock waves on 10 mm long and 5 mm diameter of 10 mm on the FPLA sample. Thus, laser shock created
thick transparent epoxy composites using optical shadowgraphy. more damage to FPLA samples than to the FPP samples. Finally, the
The shock waves from high laser intensity were focused on com- HE composites showed partial blister spallation with a diameter of
posite material for 3 ns pulse duration (1.2e3.4 TW/cm) generating 9.4 mm, while that of the GE composite had a whitened zone of
a pressure of between 44 GPa and 98.9 GPa. Results revealed that 7.7 mm. It was found that composites which were used in the
the shock wave and release wave generated by the laser reverber- aerospace industry exhibited different behaviours when being
ation at the back face was followed by a dark zone. The results exposed to laser impact loading and directed energy sources,
indicated that the shock wave and release wave resulting in dark largely depending on distribution, length, type of fibres, and the
zone at the back face corresponded with the creation of tensile matrix used for composite materials. When the same laser impact
zone due to crossing on the loading axis of the release waves that intensity was used, the composite materials recorded three types of
came from the edge of the impact region. The shock wave setting up damage at the back-face samples. These damages included inside
at t ¼ 0.5 ms and propagation t ¼ 1 ms and 1.5 ms revealed two main delamination, residual blister, and spallation. Short fibres were
shapes. At t ¼ 1 ms there were thin curved black lines which were damaged from the spallation phenomenon which indicated their
the shock wave. At this stage, the composite was compressed low strength. Non-woven fibres indicated residual blisters which
because of the pressure state that contributed to the observed was a composite damage step preceded spallation. In contrast,
darkness. Considering that the shock was short, the pressure was woven fibres showed combined spallation and blister damage, but
released once the loading stopped. The shock wave was followed by woven glass composites showed whitening on back face surface.
a grey area which was a colour that was evident in unloaded areas. Garcia et al. [52] investigated the possibility of lasers defeating
A sizeable black blur behind the first two waves was identified targets without penetration but with heat re-radiating to internal
which traduced a tensile loading due to the geometry of the laser components by using a thin carbon fibre-reinforced polymer (CFRP)
impact. The phenomenon was called the edge effect which relied and a steel disc to represent target skin and internal component,
on the principle of spherically propagating release waves inside the respectively. A FLIR® A325sc infrared camera was used to measure
composite from the edge of the impacted area. Upon reaching the steel disc temperature. Thin carbon fibre composite laminate con-
free surface, the shock waves were reflected releasing a curved grey sisting of 2-, 4-, and 6-ply sheets and having 50% carbon fibre-resin
line, which propagated backwards from right to left and crossed the mass ratio were shaped into 5.08 cm  25.4 cm strip specimens.
black blur which was the incident tensile stressed region. The back The composites were reinforced with a 3K plain-weave, 5.7 oz/yd2
face was progressively loaded with tensile stress in line with the carbon fibre cloth. After being vacuum bagged for 1 h at 1 atm
spallation phenomena and shock wave propagation. Ecault et al. pressure, the composites were further heated to 121  C and cured
[49e51] also investigated the impact of laser shocks on eco- using a 2-ton press for 1.5 h. A YLR-100-AC fibre laser served to
composites to assess how the materials degraded under laser output laser beam with a M2 value of 1.07, maximum 100 W, and 5-
impact loading. The researchers compared the impact of laser shock mm diameter. The actual range of on-target irradiances was be-
induced damage based on back observations of composite samples tween 101.9 W/cm2 and 509.3 W/cm2 due to lab limitations. A 1 cm
for various types of eco-composites. Inside delamination, residual diameter metal disc made from 1008 carbon steel with a nominal
blister and spallation resulting from laser impact on fibre length thickness of 0.15 mm was used to simulate the internal component.
were also tested using the Terahertz technique. The laser was Its temperature was measured by an attached Type K thermo-
focused on the surface of the specimen. Aluminium coating caused couple. In the experimental setup, an IR camera was offset 53 from
the matter/laser interaction to be generated on the sample surface, the plane perpendicular to the sample plate to avoid any damage as
which caused the high-pressure plasma created from the process to laser could potentially penetrate the composite. The setup of the
expand rapidly. Reactions inside the material contributed to a experiment is shown in Fig. 2. High energy laser was placed
generation of shock waves. The directed shock propagated through perpendicular to the sample plate at other side. The specimens
the composite material depending on the geometry and charac- were subjected to five different irradiances of between 152.8 W/
teristics of the samples. Due to impedance mismatch, the incident
shock wave was reflected into the release wave upon reaching the
sample blackface creating a release backward wave propagation.
The release wave crossed the incident release wave which came
from initiation at the end of the loading (returns to the initial state).
The crossing of two release waves contributed to high tensile stress
which could damage the composite material if the threshold was
exceeded. In composites with short fibres such as TWA and WA,
damage resulted from ejection and separation of fragments from
the surface, which was referred to as the spallation phenomenon.
For the WA and TWA composites, the spallation phenomenon was
noted to have variations in its damaging ability where the area of
damage for the TWA was 6.6 mm compared to 4.7 mm damage
recorded in WA composite under the same laser shock. These ob-
servations demonstrated that thermal treatment of spruce fibres
caused high damage due to brittleness of the composite material
when exposed to high energy laser. When considering the com-
posites with flat mat reinforcement, no spallation was recorded. In
this case, the inside damage resulting from laser shock generated
residual relief which caused small blisters on the back-face surface
of the FBB and FPLA composites. The measurement of diameters of
blisters resulting from laser directed shocks on the composites
showed that there were also differences in behaviours. The FPP Fig. 2. Experimental setup from top view [52].
1278 Y.X. Zhang et al. / Defence Technology 17 (2021) 1269e1288

cm2 and 356.5 W/cm2. The resulting temperature was measured at severe thermal irradiation may also induce significant geometrical
the back of the composite. Results confirmed that without com- changes in the structure’s surface ablation or localized burn
plete penetration, the intense local heating caused by laser radia- through. It was well understood that if the surface temperature
tion on a CFRP laminate can damage the internal components. reached the ablation temperature of the composite, the material
Radiation from the heated internal component in turn contributed would undergo a sublimation reaction. The burn-out material
to the development of flames at the back surface of the CFRP. The reduced the structural stiffness of the remaining laminate and
released heat elevated the temperature of the 6-ply CFRP back increased the mechanical stresses, thus degrading the structure’s
surface by 237 K during the 305.6 W/cm2 test and by 240 K during load-carrying capability. Moreover, due to the presence of highly
the 356.6 W/cm2 test. In a typical unmanned aerial vehicle (UAV) non-uniform temperatures over the thickness of the composite
fuselage, the heat gave rise to internal flames that could damage laminate, thermal in-plane forces and bending moments might
flight control systems and ignite the fuel mechanism. arise. Obviously, these thermal loads play an important role in the
In the study conducted by Voisey et al. [53], SEM and Raman change of constitutive relations of a laminate, initially subjected to
spectroscopy were used to investigate the effects of the fibre type mechanical loads. Hence, methods for predicting composite dam-
on the extent of laser-induced fibre swelling in carbon fibre com- age under coupled laser irradiation and mechanical loading have
posites being laser-drilled by pulsed Nd:YAG laser (l ¼ 1.06 mm). been developed by the researchers [55,56,61].
T300, high modulus (HM) and P100 fibres were heat treated for Candan et al. [57] investigated laser threats on fibre-based bal-
12 h at 2000  C prior to the experiment. An average output power listic-resistant composites, and the Spectra Shield SR-3136 com-
of 135 W, M2 value of ~25 with single pulsed of energy 1.0 J and posite material was used in the investigation. Spectra Shield SR-
duration 1.0 ms Nd:YAG laser was adopted. An average power 3136 was a thermoplastic composite made of ultra-high molecu-
density of around 30 kW/mm2 was yielded by the 100 mm focused lar weight polyethylene (UHMW-PE) fibres reinforced with low-
spot diameters. Prior heat treatment was found to have substan- density (LD-PE) fibres. The composite was exposed to a contin-
tially reduced the swelling exhibited by the T300 fibres but had uous wave laser beam at 915 nm of a fibre-coupled diode laser
little effect on other two fibres. The obtained spectra showed laser module. The specimen exposed to the laser beam had a puncture
drilling had rendered the T300 fibres more graphitic and less with significant swelling around the entry hole subjected to tem-
disordered. It was proposed that the rapid heating and high ther- perature of 450  C or more. A full penetration was observed at a
mal gradients generated by laser drilling tended to volatilise non- laser energy of 20 kJ and greater. Furthermore, as a result of the
carbon impurities and create high gas pressures. These high pres- slight tapering induced by asymmetric behaviour close to the
sures could act as a driving force for the new structure to be more entrance, the entry hole had a diameter of 16 mm which was larger
open which was apparently retained after the impurities were than the diameter of the exit hole of 2.4 mm.
driven off. This mechanism explained why fibres containing larger
quantities of residual (volatile) impurities were more prone to 4.2. Combined loading
laser-induced swelling.
Instead of the total failure/destruction of the targeted structure, Allheily et al. [58] investigated the thermo-mechanical behav-
the recent military interest has been shifted to tactical threats, such iour of aeronautic materials (CFRP) subjected to powerful electro-
as cruise missiles and unmanned aerial vehicles (UAVs), which can magnetic fluxes to assess the likely impact of directed energy
be countered with comparatively lower laser irradiance. The idea is systems on aircraft composite structures. The method proposed
to bring the incident laser wavelength to the near Infrared region, was meant to find a way to neutralise unmanned aerial vehicles
which can penetrate the matrix resin of most of the composite that posed threat to defence installations. In the preliminary study
materials. One such study was conducted by Wu et al. [54] in which the authors carried out three tests namely thermal surface char-
it was argued that the weakly absorbed, more deeply penetrating acterization, thermal in-depth characterization, and thermo-
near-IR radiation softened the resin matrix resulting in structural mechanical characterization on G939/M18-1 specimens (Hexcel
failure under load at lower laser intensity than what was required Composites) made of plain-woven carbon fabrics. In all the tests the
for mid-IR lasers. The study used two materials for illustration, i.e. specimens were initially exposed to a homogenous irradiation with
translucent fibreglass composite and opaque carbon composite. a 10 kW fibre laser from IPG. Approximately 3% of the laser energy
Since the study was related to the deep penetration of the laser, the was produced with a beam splitter. Concurrently, the front side of
first step in the experimental program was to determine the ab- the specimen was exposed to gas flow which was applied parallel to
sorption properties in material samples, so that the comparison of the irradiated surface before, during and after the irradiation. The
the results with the theoretical values could be made. Following purpose of gas flow was to assess the carbon fibres combustion
this, the measure of the compressive load strength under near-IR impact on temperature readings by comparing experiments with
laser irradiation was made. The composite plate samples were air or nitrogen. After each experiment the specimens were weighed
held vertically in a hydraulic load machine designed to apply a to determine mass loss based on laser intensity and the irradiation
constant compressive force. A uniform illumination on the samples time.
was achieved by passing light from a 1.5 kW diode laser array and Results show that with growing laser power the temperature of
the wavelength of 0.8 mm through a lens duct and imaging lenses. the irradiated zone increased and reached a maximum value of
Digital and IR cameras were used for recording purposes. The ex- 3300  C for power densities that were greater than 1000 W/cm2.
hausts were provided for the fumes to be exhausted. The research The maximum power recorded aligned with the values recorded by
discovered that the volume heating by direct in-depth absorption other researchers [49e51], and it referred to the sublimation
of laser energy in case of translucent fibreglass composite material temperature of the carbon composite fibres. When observing post
and rapid conduction of surface-deposited energy as in the case of irradiation samples, the same property was also observed while
opaque carbon composite may cause the failure at one to three irradiations with power density of less than 1000 W/cm2 only
orders of magnitude lower than the intensity required to produce a impact on epoxy matrix because the sublimation temperature was
lethal effect by target penetration. lower than that of the carbon material where drilling became
The intense heating produced by the laser system can adversely visible when the composite sample were irradiated using laser
affect the mechanical properties of the composite structures such power density that was greater than the threshold value. The
as the tensile/shear strength and elastic modulus. Meanwhile, evolution of the temperature gradient was evident inside the
Y.X. Zhang et al. / Defence Technology 17 (2021) 1269e1288 1279

composites where the results revealed that CFRP was a good specimens. The laser spot was 15 mm in diameter perpendicularly
thermal insulator since it could take some seconds before the back- focusing on the centre of the specimen with 0.202, 0.492, 0.953 and
face side temperature became significant. The observed thermal 1.935 kW/cm2 power intensity. Specimens with the same thickness
resistance was attributed to strong carbon fibres which could were tested under the same pre-load and same irradiation laser
absorb almost all laser energy in a single fabric layer and sustaining intensity. Laser irradiation was kept on until material completely
high temperatures without resulting in ablation. Once the carbon failed. CO2 CW laser system was used to generate laser with 10.6 mm
ablation conditions were attained, the amount of laser energy wavelength. The failure time was defined as the time from the start
needed to damage the composite material was high because of the of irradiation to the complete fracture of the specimens. Results
substantial carbon ablative enthalpy. All these observations showed that the laser power intensity at 0.202 kW/cm2, pre-stress
explained for the 10 s continuous laser irradiation resulting in very ratio at 0.5 and thickness of specimen at 1.5 mm would cause
high temperatures at the composites’ front face (above 2000  C for complete fracture after 9.90 s irradiation. On the contrary, the
200 W/cm2), while the rear side that was 4 mm in thickness failure time in the compression test is much shorter than that in the
reached only 250  C. In contrast, the pyrolyzes process on the tension test. Additionally, the failure mechanism in tension test
matrix started after irradiation. The side post-irradiation and mainly included fibre drag break, while delamination and buckling
infrared observation revealed an exothermic pyrolysis at between were what caused failures in compression test. The failure time of
300  C and 350  C that preceded the delamination front. The the specimens with the same thickness will be shortened expo-
chemical degradation temperature ranged in line with the thermo- nentially as laser power intensity increased. The relationship be-
gravimetric analysis resulting in pure resin component with an tween the specimen failure time and the main parameters under
inert ambient medium. The composite recorded thickness reduc- tension load combined with laser irradiation and under compres-
tion during irradiation and post-irradiation since the bending sive load combined with laser irradiation are expressed in Eq. (1)
displacement increased even when the irradiation stopped. The and Eq. (2) respectively.
study indicated a good thermal insulation of the composite mate-
rial, which was largely because of the potential of carbon fibres to tT ¼ 6:4411  36:7988sh  5:1239sh2 þ 35:1316se3:1464Is
absorb and support heat fluxes. Furthermore, the delamination of
 28:4074he3:1464Is þ 5:2739h2 e3:1464Is
the composite reduced energy deposition on the specimen.
Zhao et al. [59] conducted an experimental study on the failure (1)
behaviour of CFRP composites subjected to tensile loadings under
thermal environments and laser irradiation. T700/BA9916 epoxy tC ¼ 0:7076  11:1656I  0:3597 þ 10:9637hI  0:3597
prepreg was cured at 180  C, and the ply pattern was [45 /0 /-45 /
90 ]2s. The epoxy and fibres accounted for 0.467 and 0.533  2:1372h2I  0:3597 þ 22:7927r sI  0:3597
respectively in the laminated composites which had a thickness of  22:5215r shI  0:3597 þ 4:7401r sh2I  0:3597 (2)
2.40 mm and width of 20 mm. Electric resistance wire was wound
into a heating band, being set around the specimen to conduct the where tT, tc are the specimen failure time under tensile load and
tensile tests at thermal environments. Thermal couples of NiCr-NiSi compressive load, respectively, h is the thickness of composite
type were installed to monitor the specimen temperature and laminated specimen, rs is the pre-stress ratio, I is the laser power
heating rate, and tensile strain was acquired by a DIC system. The density.
CFRP specimens were irradiated by continuous wave laser by po- Kibler et al. [61] conducted a series of experimental and
wer densities ranging from 1.5 MW/m2 to 12.7 MW/m2 in a nitro- analytical studies on the response of graphite-epoxy composites to
gen protection environment for the sake of avoiding possible continuous-wave CO2 laser radiation. Tensile coupons of one
combustion. The laser source was a YLS 1070 nm fibre laser of 2 kW graphite-epoxy system (Narmco 5208/T300) and one aluminium
provided by IPG Ltd. The defective specimen was further applied alloy (2024 (T81)) were exposed to laser irradiation. Three com-
with tensile loading at 2 mm/min rate in MTS until failure. Results posite laminates, namely (0 /±45 )C, (/±45 /90 )2S, and (90 //
showed that complex thermal damages could happen once CFRP ±45 )2S with 12-ply of nominal thickness of 0.073 mm were used.
composites were exposed to thermal loadings which could lead to In the low power laser experiments, the laser irradiations were
decrease of the Young’s modulus and failure strength. Residual performed with a model 41 Coheren Radiation Laboratory laser
strength was found to decline as target temperature or laser power with incident beam power of 200 W. A Mach 0.2 airflow was
density increased. Besides, residual strength was found falling maintained parallel to the specimen surface. An iron-constantan
drastically before laser power density reached 6.3 MW/m2 after thermocouple at various positions on the back surface of the
which it decreased at a slower rate. However, a temperature specimen was used to monitor the temperature. In the high-power
plateau zone was identified before 200  C, which was the thermal laser experiments, a GTE Sylvania model 971 with incident beam
pyrolysis activation temperature for epoxy resin. Sublimation (the power of 750 W was used for the first series of exposures, and a
phase transition of substance directly from solid to gas) of carbon Mach 0.1 airflow was maintained across the width of the specimen
fibres occurred once temperature reached 3000  C. The turning surface. The 10 Kilowatt ‘flat-top’ laser was used for the second
point at which delamination cracks occurred was found to be at a series of exposures. It was determined that the aluminium was
power density of 2.5 MW/m2. more susceptible than composites to damage at a high laser in-
The failure behaviour of the T700/603 carbon fibre/epoxy tensity, especially, both penetration time and strength retention
composite laminates under pre-load compression or tension and were less for aluminium than for the composites. A strength
laser irradiation was tested to study the effect of main parameters retention in terms of fracture mechanics-based predictions was
including pre-stress ratio, laser power density as well as the proposed for the partially penetrated and laser-damaged compos-
thicknesses of the specimens on failure time [60] of ites. Moreover, specimens loaded in tension and irradiated to fail-
140 mm  10 mm specimens with various thickness consisting of ure were found to fracture at a slightly lower preload than the
0.15 mm thick ply. A Zwick/Roell-Z100 universal testing machine strength retention of specimens irradiated but unloaded.
was employed to apply pre-load of 35% or 50% of the average ul- Laser-induced damage on mechanically loaded laminates in
timate compressive collapse stress and 50%, 65% or 80% of the unmanned aircraft was explored with a view to predict the
average ultimate tensile fracture stress to the composite laminate thermal-mechanical response of the heated panel irradiated by
1280 Y.X. Zhang et al. / Defence Technology 17 (2021) 1269e1288

Table 2a
A summary of experimental studies. Experimental studies on thermo-mechanical responses.

Research Thermo-
focus mechanical
response

Materials CFRP CFRP Composite laminated Unidirectional T700GC/M21 Laminate carbon/ Fibre- G939/ CFRP composite
Composite laminate laminate carbon- (UD) carbon/ Composite laminate polyetheretherketone reinforced M18-1 laminate
carbon (C/ epoxy (PEEK) composite Carbon/
C) laminate plates epoxy
composite laminate
Reference [19] [27] [20e24] [25] [26] [28] [29] [30] [58]

Loadings Laser ytterbium fibre CO2 laser CO2 laser Laser-generated Heat flux of 8 Continuous 10 kW Electromagnetic
(5,10,56,64 W cm2) laser 5 1 kW (10 kW, constant non- e60 kW cm2 wave CO2 IPG fibre fluxes, homogenous
e525 W cm2 1.5 kW) uniform heat flux of laser of laser irradiation with
and 780 maximum 15 kW 10 kW fibre laser.
e3000 W cm2 220 kW cm2
Reference [19] [27] [24] [25] [26] [28] [29] [30] [58]

Table 2b
A summary of experimental studies. Experimental studies on ablation behaviour.

Research Ablation behaviour


focus

Material CFRP T300/AG80 carbon Carbon fibre Carbon fibre reinforced silicon
fibre reinforced reinforced composite composites
laminate (CFRC)
Reference [34] [35] [25] [37]

Loading Continuous wave laser, long pulse laser (200ns pulse duration), short pulsed laser Nd:YAG laser beam TEA CO2 Nd:YAG Laser irradiation
(10ns pulse duration). Laser (3.54  106, 1.1  1012, 1.5  1012 W cm2) 50 W cm2 laser (4.77  102 W cm2,
12.1  102 W cm2)
Reference [34] [35] [25] [37]

laser [62]. The laser damage was assessed on specimens under load. strength reduction for unloaded samples were 22% and 14%
This was achieved by applying bending stress of 100 MPa on the respectively. The tensile strength of specimens was measured
specimens, which was produced by a loading device consisting of a before and after laser irradiation by universal testing machine
load cell and target fixture that was used to fix the specimen. An (UTM). Significant damage occurred under mechanically loaded
evaluation was then undertaken to ascertain the thermal- conditions resulting in resin sublimation. The extent of the damage
mechanical parameters of laser irradiated specimens. The investi- was analysed by assessing the ablated mass of the specimen. It was
gation was carried out on glass fibre reinforced polymer (GFRP) and noted that the ablated mass was more for all the specimens when
Carbon Fibre Reinforced Polymer (CFRP) specimens. The specimens the test samples were irradiated by laser under loaded conditions.
were cut into thin rectangular sheets of 120 mm  45 mm. The test High intense radiation induced significant mass loss as a result of
specimen was subjected to a radiation density of 1 kW/cm2. A resin sublimation.
carbon dioxide laser with an operating wavelength of 10.6 mm was The experimental studies reviewed are summarized in Table 2,
used. The damage of the specimen was studied by LYNX Dynoscope. with the experimental studies on thermo-mechanical responses
At an irradiation of 1 kW/cm2, the CFRP samples had a reduction of listed in Table 2a, experimental studies on ablation behaviour in
72% in bending strength recorded at a bending stress of 20 MPa. Table 2b, experimental studies on interlaminar effects in Table 2c,
Besides, the tensile strength was reduced by 36% for the loaded and experimental studies on damage analysis in Table 2d. A sum-
samples subjected to the bending stress of 100 MPa whilst for GFRP mary of damage mode identified in the experimental studied is
specimens a 31% reduction was obtained. In comparison, the tensile listed in Table 3 with those under single loading only listed in

Table 2c
A summary of experimental studies. Experimental studies on interlaminar effects.

Research Interlaminar effects


focus

Material Glass fibre reinforced epoxy composites CFRP Composite laminate CFRP Composite laminate
Reference [38] [39e42] [40]

Loading 60
Co g-ray with dose rate of 300 Gy/min at Infrared laser of 1064 nm wavelength and 200 ns Continuous wave laser of 1070 nm wavelength at
ambient temperature pulse duration, 10 Hz 500 W, 800 W, 1000 W.
Reference [38] [39,40] [40]
Y.X. Zhang et al. / Defence Technology 17 (2021) 1269e1288 1281

Table 2d
A summary of experimental studies. Experimental studies on damage analysis.

Research Damage
focus analysis

Material CFRP CFRP CFRP Carbon fibre Translucent Fibre-based CFRP composite T700/603 carbon Graphite- Glass fibre
composite composite composite composites fibreglass ballistic- laminate fibre/epoxy epoxy reinforced
laminate laminate laminate composite/ resistant composite composite polymer
(T800/M21) opaque composites laminate (Narmco
carbon 5208/T300)
composite
Reference [44,47,48] [49e51] [52] [53] [54] [57] [59] [60] [61] [62]

Loading Nd:YAG Laser Fibre laser with Nd:YAG fibre laser 1.5 kW Continuous Continuous wave Pre-load Continuous- Bending
laser with irradiation 100W, 5-mm with diode laser wave laser laser (1.5 MW/ compression and wave CO2 stress of
calibrated with 3ns pulse diameter, 30  104 kW mm2 with 0.8 mm beam at m2 to 12.7 MW/ tension. Laser laser 100 Mpa,
pulse with duration (1.2 101.9 W cm2 wavelength 915 nm, m2), tensile irradiation 15 mm irradiation laser
9.3 ns e3.4 TW cm2) and 20 kJ loadings under diameter with (750 W), irradiation
duration at 509.3 W cm2 thermal 0.202, 0.492, 0.953, 10 kW ‘flat- of
1.5 J energy power output environment 1.935 kW cm2 top’ laser 1 kW cm2
Reference [44] [50] [52] [53] [54] [57] [59] [60] [61] [62]

Table 3a and those under combined loading listed in Table 3b. axis symmetric ring model was applied for the finite element
analysis. The laser pulse was modelled with beam diameter of
20 mm, power density of 3.0 W/mm2, with constant distribution
5. Numerical studies
and 1-s duration. Simulation results demonstrated that the tem-
perature rapidly decreased in the surface layer and did not change
5.1. Thermal mechanical response
much below 4 mm depth. The critical power density Pc was
confirmed to be a reliable measure of thermal shock strength for
The finite element analysis (FEA) was conducted for analysing
the laminated C/C composite and was corresponding to the critical
transient heat conduction and thermal stress of laminated carbon-
temperature difference in the traditional quenching test. The
carbon (C/C) composite in Ref. [24]. A cylindrical model of 50 mm
asymptotical value of Pc was found to be around 2 W/mm2 on the
diameter and 12 mm height in MARC program was used to simulate
maximum negative shear stress and 2.8 W/mm2.
the experimental specimen which was irradiated at its upper sur-
The ultrasonic wave generated by short pulse laser could be
face by a laser pulse in the FEA. The material used is laminated C/C
optically absorbed by composite material to cause thermal expan-
composite with 7.8 MPa shear strength, 137.3 MPa compressive
sion, and FEA is very handy in dealing with thermoelastic problems
strength, and 606 MPa tensile strength. The isotropic and homo-
owing to its adaptivity in modelling complex geometry and
geneous material is modified for the laminated C/C composite
obtaining full field numerical solutions. Wang et al. [63] developed
materials assuming that the material is regarded to be equivalently
a finite element model of laser ultrasonic generation in thin
homogeneous. Totally 975 elements with an arbitrary quadrilateral

Table 3a
A summary of damages identified in the experimental studies. A summary of damage mode identified in the experimental studied under single loading.

Laser energy (0.8e6) W$cm2 (5/10/36/64) W$cm2 101.9e509.3 W cm2 30  104 kW cm2 1.49 GW cm2 3.54  104 GW cm2
output

Material PEEK (carbon/epoxy, CFRP (4/6/8 plies) CFRP (2/4/6 plies) T300, P100 CFRP (8 plies) CFRP
glass/epoxy)

Damage Delamination Ignition; combustion; resin matrix Internal flames; ignite fuel Laser-induced Delamination Drilling holes;
removal; mass loss mechanism swelling evaporation
References [28] [19] [52] [53] [44] [34]

Laser energy 50 W 1.1 J 20 kJ


output

Material CFRP CFRP SR-3136 thermoplastic composite

Damage Temperature-activated chemical reactions; pyrolysis charring; Drill through; interlaminar thermal damage; Full penetration; significant swelling
breaks within the continuous medium; delamination cracks ablation; pyrolysis
References [26] [39,40] [57]

Table 3b
A summary of damages identified in the experimental studies. A summary of damage mode identified in the experimental studied under combined loading.

Combined loading 1.27 kW cm2, (0.202/0.492/0.953/1.935) kW$cm2, 10 kW, tension 1 kW cm2,


Tensile load, Tensile and compressive load Bending stress
Thermal environment

Materials CFRP T700/603 Graphite-epoxy composite GFRP

Damage Delamination Complete fracture; fibre drag break; delamination; buckling Penetration Resin sublimation
References [59] [60] [58] [62]
1282 Y.X. Zhang et al. / Defence Technology 17 (2021) 1269e1288

transversely isotropic fibre-reinforced laminate composite to study diameter Gaussian beam with 107 W of total power. Material data
this phenomenon, coupled with thermal conductive equation and related to the thermochemical characteristics experimentally
thermo-elastic mechanism generation equation. Specifically, they determined was used by the model. A mesh was created with 40
studied the structural response of a thin fibre-reinforced composite elements in the radial direction and 180 in the through-thickness
plate to normal-direction laser line irradiation. The transient tem- direction. A numerical technique of varying the material proper-
perature and temperature gradient field were calculated, and the ties was employed to simulate material removal. The model was
laser-generated transient Lamb waves were obtained. The ther- validated by the experiment. A 100-W-nomial power, Yb:YAG fibre-
moelastically generated waves were calculated in a thin fibre- coupled laser produced by IPG Photonics that lases at 1070 nm was
reinforced composite plate (40e400 mm thickness) which was measured using a 5 silica wedge-beam splitter and a Spiricon
meshed by elements by 20 mm in length. The laser energy was SP620U profiler with BeamGage software. Additionally, the CFRP
13.5 mJ and the pulse rise time was 10 ns, and the radius of the laminate was tested for comparison with the theoretical model. It
pulsed laser spot on the sample surface was 300 mm. The material was found that the model was unable to predict the experimentally
properties used in the calculation including thermal conductive observed laser-drilled hole evolution. Also, the model predicted a
coefficient, density, thermal capacity, Young’s modulus, and ther- higher recession rate than experimentally observed result. A
mal expansion coefficient were pre-specified. The results obtained recession rate of 3.06 mm/s in the Acryilite, which was 7.6% greater
from numerical simulation clearly showed that the evolution of the than the experimental results was obtained.
dispersive waveform was a function of the target distance and the Boer et al. [65] modelled the thermo-mechanical responses of
plate thickness. In addition, the velocity of Lamb wave propagating the CFRP laminates to continuous laser irradiation using finite
along the fibre direction was found faster than that normal to the element method in which a technique of coupling and decoupling
fibre direction. The dispersive nature of Lamb waveform in two the Degree of Freedom (DOF) was employed for interlaminar
directions was found to be different. cracking simulation. A quarter CFRP laminate was modelled under
In the numerical study conducted by Leplat et al. [26], a 2D axil- laser irradiation. The laser beam was modelled to be of radius 5 mm
symmetrical approach which neglected edge effects was used. The and perpendicularly irradiating the CFRP laminate, while the sur-
test coupon (80 mm  80 mm) was discretised into a Cartesian face heat flux 6.37  106 W/m2, 10.19  106 W/m2 and
regular mesh composed of 40  16 cells, and the exact same 12.74  106 W/m2 were applied on areas where under direct irra-
boundary conditions as in the experiment were introduced into the diation in the three cases. Numerical results indicated that the in-
computation which took account the laser heating distribution and crease in laser power would only increase the temperature
all surface exchanged with the test chamber. All physical properties magnitudes, and that the high displacement gradient occurred near
of the material including thermal conductivity tensor, specific heat, the edge of the laser spot inducing large shear stress therein. Also,
density, porosity, permeability tensor, spectral emissivity/absorp- the maximum normal stress acted on the interface between adja-
tivity, and model parameters (Arrhenius coefficient for chemical cent laminae was higher than 20 MPa and the maximum shear
reactions kinetics, heat of reactions) were assessed experimentally stress higher than 25 MPa, which was around half the interlaminar
using ONERA facilities. Likewise, the space distribution of the heat strength of the CFRP laminates under room temperature [66]. The
flux density generated by the laser was assessed prior to the ex- progressive cracking was observed at the backward surface of the
periments. The thermal response obtained from the numerical specimen under 800 W laser irradiation during the unloading stage
simulation showed that heat transfer from the exposed face caused and the interface cracks propagate as specimen cooled down.
the temperature of the condensed phase grow to cause pyrolysis of In addition, a 3D thermal model (coded in MATLAB®) was used
the matrix into a considerable depth through the laminate. M21 to interpret the laser-CFRP interaction resulting in heating and
matrix was found to decompose faster than the resin as tempera- decomposition [27]. The model was meshed by 30  30 uniform
ture grew inside the laminate and offered preferential paths for elements in the plane perpendicular to the incoming laser, with an
cracks propagation within resin-rich regions between fibre tows. element for each carbon fibre ply in the parallel direction. The
The numerical simulation involved heat and mass (decomposition changing material properties were assumed first to be a function of
gas) transfer model within homogenised porous media and was evolving CFRP decomposition phase, in proportion to the relative
proved to agree well on thermal response of the laminate subjected amounts of each decomposition phase present in each cell. The
to stead laser flux from experiments, although the delamination incident laser intensity distribution was measured throughout each
cracks interacting with heat diffusion and gas transport processes experiment, combined into an average irradiance map and inputted
were neglected. The transformations of the material were found to into the thermal model. At the laser spot the temperature peaked to
induce the gas-phase creation at high temperature and high pres- 634  C after 30 s at a laser irradiation of 9.9 W/cm2. Working out-
sure because of temperature raised fast enough to active the ward the edges of the panel maintained an average temperature of
thermo-chemical reactions on the exposed surface. 100  C. The overall specimen temperature distribution was radially
Tresansky et al. [64] presented a numerical heat transfer model symmetrical. Modelling CFRP without the endothermic reaction
to capture heat flow and material damage to polymer/carbon fibre- enthalpies or volatile heat capacity increased the final backside
reinforced composites subjected to laser beam irradiation. COMSOL temperatures by 100  C and 90  C at 5 W/cm2 and 10 W/cm2 laser
Multiphysics® numerical modelling program which included intensity, respectively. In all combustion cases, model temperatures
packages for heat transfer, fluid dynamics, electro-optics, solid during cool down were underestimated due to combustion being
mechanics, electricity and magnetism was used to establish the neglected in the heat transfer model.
computational heat transfer model. A 2.5 mm thick, 20 ply carbon
fibre/epoxy laminate was tested using Cytec 5215 prepreg with a 1K 5.2. Ablation behaviour
tow in plain-weave architecture. A 16 inch  16 inch panel was
made by first debulking three sets of six plies under vacuum for Temperature patterns of the CFRP being irradiated by contin-
30 min before curing at 200  C for 3 h under vacuum. A Gaussian- uous wave laser, long duration pulsed wave laser and short dura-
profile, surface heat flux to simulate the laser, forced convection, tion pulsed wave laser were analysed using finite element method
and surface to ambient radiation was applied to the top surface of in the study of Wu et al. [34] in which the specimens were modelled
the selected axisymmetric model. A 1/4-inch-thick sheet of Acrylite axis-symmetrically. An axis-symmetrical finite element model was
GP was modelled as a surface absorber for a 1070 nm, 6.12 mm 1/e2 set up to analyse the thermo-physical responses of the specimens
Y.X. Zhang et al. / Defence Technology 17 (2021) 1269e1288 1283

(50 mm  50 mm  4.1 mm). The flow of the sublimation product subject to laser irradiation with the creating of the finite element
was neglected. The power density for continuous wave laser, long ablation model with variation in boundary conditions. They
pulsed laser (200 ns pulse duration), and short pulsed laser (10 ns selected T300/epoxy resin laminate with 20 plies and 4 mm
pulse duration) was 3.54  106 W/m2, 1.50  1012 W/m2, and thickness. CO2 continuous laser with an intensity of 1.528 kW/cm2
3.00  1013 W/m2 respectively. All lasers were designed to irradiate and 3.82 kW/cm2 was employed to irradiate specimens at a 10 mm
the square CFRP specimens for 10 s. The numerical computation diameter spot. The specimen was shaped in 5 cm  5 cm, and the
was carried out with the minimum time step of 0.25 ns to allow one SEM was used to monitor the ablation. The ablation was assumed to
round of heating and cooling complete in each time step. It was be one-dimensional (only long the thickness of laminate) in the
found that the peak temperature remained stable under continuous cases of high energy lasers irradiating composite laminate for short
laser irradiation, while pulsed wave laser irradiation would result time. ABAQUS software was used to model the two-dimensional
in stable temperature after ultra-high temperature (over 25000 K) parts which was further used to calculate the ablation over thick-
caused by first laser pulse evaporating the surface carbon fibre ness of the laminate. 0.1 mm  4.0 mm rectangular shape was
fabric. The numerical results showed that the laser power density created in ‘part’ mode, and elements were discretised into 10  400
threshold was around 3.0  1013 W/m2 to trigger optical break- with 10 mm DC2D4 elements. Using integrating sphere method and
down hence making the irradiating ineffective. Lambda900 spectrograph, the laser energy absorbing coefficient
A three-dimensional model taking the difference of ablation was measured to be 0.86. The thermal radiation coefficient and
performance along different fibre orientations and the laminated thermal convection coefficient was set to be 0.92 and 187 W/
structure of composites into consideration was established to study (m2$ C), respectively [72]. A python program was designed to
the ablation characteristics, temperature distribution, heat affected realize that thermal load affecting zone varying with time, and
zone (HAZ), and the ablation morphologies of composite laminates control the whole finite element analysis. Results showed the
impacted by laser [67]. Governing equations for energy conserva- temperature gradient was relatively steep at locations near the
tion, mass conservation and momentum conservation were pre- laser spot, and the ablation has reached balance very soon. When
sented in details. An air flow at 0.029 Mach was introduced in this laser irradiation intensity reaches 1.528 kW/cm2, the irradiated
study, erosion was neglected to simplify the problem so that surface surface was ablated at a recession rate of 0.15 mm/s and pyrolysis
ablation could be assumed to be governed mainly by the oxidation thickness was around 0.08 mm. At laser irradiation intensity of
of material. As stated by Deng et al. [68], the oxidation was com- 3.82 kW/cm2, the irradiated surface was ablated at a recession rate
parable with erosion of fibre only when flow velocity was higher of 0.77 m/s and around 0.05 mm pyrolysis thickness.
than 0.5 Mach. The heat flux from the laser beam was modelled by a
circular 2D Gaussian function, and the laser beam was modelled to
normally hit the carbon fibre composites by 38 W power output 5.3. Dynamic response
with the laser radius of 1.25 mm. A quarter of the CFRP laminate of
20 mm  20 mm  0.56 mm was modelled considering the sym- The degradation of material property, burn-out and induced
metry. The models were solved by the FEA and the deformed ge- thermal loading due to rapid laser heating will greatly influence the
ometry of COMSOL was adopted to simulate the interface dynamic responses of the composite laminate. The thermal inter-
migration. The T300 carbon fibre and E-51 epoxy with initial laminar forces and bending moments would be induced when
porosity of 0.06 was chosen, and the volume fraction of fibre and composite laminate was heated nonuniformly and combined with
resin was 0.64 and 0.3 respectively. Computational results indicated other thermal effects it would pose great change in dynamic
the direction of heat transfer within material changed by time behaviour such as vibration amplitude of the composite laminate.
owing to different fibre orientations in adjacent layers, which Chen et al. [73] studied the transient response of laminated plates
created a non-monotonic line of material surface temperature, and to combined mechanical load and laser irradiation. In their study, a
the shape of HAZ changed over time. The deviation of temperature moving organic-matrix composite plate suddenly subjected to
along different axis was distinct within the laser spot and gradually uniform and highly intense laser irradiation was examined.
decreased as ablation time elapsed. Initially, a modified Crank-Nicholson finite difference scheme
A numerical study was further conducted [35] in which com- which incorporated the effects of surface ablation, degradation of
posite laminate (200 mm  200 mm  1.5 mm) was modelled using thermophysical properties and heat loss through radiation and
eight node bilinear secondary hot shell element in ABAQUS. convection was employed to analyse temperature distribution and
Boundary conditions were exactly the same as those in the exper- sublimation reaction. Then mechanical load was combined with
imental study, and Simpson integration method with 3 integration thermal load which was evaluated by the temperature distribution.
points, coupled with external laser loading program coded by The burn-out geometry configuration from previous step was used
Fortan, was used to simulate the laser loading (power density of to conduct forced vibration analysis wherein both small and large
50 W/cm2, laser beam radius of 10 mm, 20 mm, and 30 mm). Elastic deflection composite plate theories were adopted. The specimen
modulus and other thermophysical properties were according to was modelled as a 20-ply graphite/epoxy laminate with
literatures [69,70]. Numerical results revealed the strain value ½±; 90; 03 ; ±; 90; 03 2 sequence and 30.48 cm  2.54 cm  0.25 cm
decreased as further away from the centre of the laser spot, which plate. A nine-node isoparametric plate finite element was
aligned with the experimental findings. In addition, the maximum employed. Laser was irradiating at the top or bottom surface of the
strain occurred at the 90 degree at the concentric circle of the specimen, coupled with transverse loads. Both laser irradiation and
laminate, which was at least 1.5 times of the value at 0 degree. transverse loads were step functions of time. 0.25 kw/cm2, 1.0 kw/
Additionally, the increasing of laser spot radius was found to be cm2, and 2.5 kw/cm2 were applied on the entire top surface of the
capable of exerting a sudden shock upon the laminate, causing the specimen, which was simply supported at its shorter edges having
strain at the same location to increase as well. The maximum de- in-plane motion suppressed. A Mach 0.3 airflow was applied to pass
viation of 18.4% was identified in the 10 mm beam radius test, and over the plate surface. Computational results showed that the
the temperature rise effect in the experiments was 16.9% at most, amplitude of the oscillation was governed by the magnitude and
which suggested the numerical model was reasonably reliable. rise time of the induced thermal bending moments and plate
Chang et al. [71] further investigated the ablation temperature bending rigidity. The most significant oscillation occurred in the
filed and recession rate of the carbon/epoxy composite laminate case of 1.0 kw/cm2 laser irradiation. Also, with the irradiated
1284 Y.X. Zhang et al. / Defence Technology 17 (2021) 1269e1288

surface different from the pressure surface, vibration was elevated. fibre and BA9916-II resin matrix under infrared laser of wavelength
The change in the stiffness and mass density of composite laminate 1064 nm, pulse duration 200ns and repetitive frequency 10 Hz for
was also indicated, and the laser irradiation was found to increase 6 s, 8 s, and 10 s irradiation time by common optical microscope
the peak amplitudes of vibration in all cases. However, the dynamic and 3D microscope. An Arrhenius-Equation based model with
response of composite laminates was influenced by laser intensity multi-step decomposition was employed to describe the mass-loss
with the location of the plate surface being irradiated. Higher laser behaviour of CFRP composite under elevated temperature by Zhao
power ensured neither greater escalation nor reduction of the et al. [56]. Additionally, a mesoscopic to macroscopic model
vibration. including thermal degradation of both matrix and fibres for
Chen et al. [72] studied the effects of laser irradiation on obtaining the thermo-mechanical properties of the CFRP composite
strength reduction and on the dynamic and buckling characteristics under heating, along with a progressive destruction program was
of organic-matrix composite laminates. The heat-transfer process employed for theoretical predictions. Specimens were predicted to
was modelled by a modified Crank-Nicholson finite difference fail in a progressive damage way at elevated temperatures, with the
scheme. In this study, a moving composite plate (20 ply failure sequence of 90 plies, ± 45 plies and 0 plies. Young’s
30.48 cm  2.54 cm  0.254 cm graphite/epoxy laminated com- modulus and residual strength decays predicted by the analytical
posite) was assumed to be suddenly exposed to highly intensive model was in well agreement with experiment observation.
laser irradiation (1.33 kW/cm2 and 2.79 kW/cm2). A Mach 0.3 Zhang et al. [74] developed a parametric program using APDL
airflow was assumed to pass over the lamina. A nine-node iso- language from ANSYS, based on three-dimensional Hashin princi-
parametric plate finite element was employed. Computational re- ple to study the accumulative damage of laminated composites
sults showed that the higher the laser intensity, the faster the under laser erosion. Specifically, the initiation, propagation and
degradation and the ablation of the material property. It also structural damage of the macroscopic failure after laser erosion on
showed that the worsening of material degradation and material the composite laminates containing holes were simulated, yielding
removal did not result in monotonical decreasing of the natural cloud charts of damages of different layers under inner static strain.
frequency. The buckling load was found to have significantly T300/KH304 [75] composite laminates containing hole with
reduced as the laser exposure time increased. different diameter (6.21, 7.97, 6.19, 6.15, 6.22, and 6.21 mm) and ply
angle were selected. The SOLID46 laminate element in ANSYS was
5.4. Damage analysis chosen for discretization, and refinements were applied near the
hole where stress concentration was likely to occur. For unpene-
Complex chemical and physical processes including pyrolysis of trated laser erosion, the part being irradiated drastically decreased
matrix, formation and growth of pores and char, oxidation of re- in strength. Specifically, at erosion depth of 1.24 mm and 0.62 mm,
sidual char and carbon fibres, thermal expansion and contraction, the failure load for composite laminate was calculated to be
matrix cracking, and delamination may occur when CFRP com- 38.39 kN and 50.36 kN, respectively, as compared to the failure load
posite with epoxy matrix was exposed to thermal environment of 63.57 kN when no laser erosion exerted upon composite lami-
[39]. Fig. 3 shows section morphologies and surface topography of a nate. By analysing the damage propagation, it was found that the
2 mm thick autoclave cured CFRP laminate from CCF-700 carbon damage initiated from the ply with the largest angle and

Fig. 3. Cross section morphologies and the surface topography of CFRP laminates bring drilled under pulsed infrared laser [39].
Y.X. Zhang et al. / Defence Technology 17 (2021) 1269e1288 1285

propagated to the ply with the smallest angle. The damages at the 0 laminas. Fibre strength of lamina coordination larger than
plies with larger angles were found to be mostly cracks, as opposed 1.8 mm was maintained at a lower stage (532 MPa). The fibre
to the fractures at the plies with smaller angles. strength of laminas 1.0 mme1.8 mm showed a gradual decline. At
Chang et al. [76] presented a numerical study investigating the this point, the composite strength reduced by 50% although the
progressive damage regulation of graphite fibre/epoxy laminate fibre did not record any ablation activities. The phenomenon can be
under combined effects of laser and mechanical loading. An explained by the fact that under high temperature, the matrix
improved bridging model based on the one-dimensional ablation decomposition was induced by laser irradiation.
model was adopted to calculate the tensile strength of the laminate Ablation was only reported to occur at the 1st lamina. In this
under different laser power density and irradiation time. Repre- case, the composite strength decreased because of the matrix
sentative volume element (RVE) was introduced into their study to decomposition. Liu et al. [77] further noted that the 1e4th laminas
calculate stiffness attenuation and laminate thermal stress. The AS/ were ablation with a residual thickness of irradiation being
3501-6 composite laminate with [45 /-45 /90 /0 /0 /0 /0 /-45 / observed in the region of 2.0 mm. After laser irradiation, only 25% of
45 /0 /0 ]S layup sequence and 0.62 fibre volume fraction was the composite strength remained. Two reasons can explain the
selected. The specimen was modelled into 2.54 cm3 cube. The observations: 1) fibre ablation induced thickness loss of the com-
progressive damage under laser irradiation (1.0 kW/cm2 and posite, and 2) the temperature that increased through the com-
2.5 kW/cm2) for 0.5, 1.0, and 5 s was calculated. Calculation showed posite thickness caused the degradation of the fibre strength. In
that the maximum tensile load the laminate can withstand summation, it was found that the tensile strength of the composite
decreased as irradiation time prolonged, and the decreasing rate plate was controlled by the high strength fibres at the 0 lamina,
was associated with the laser irradiation intensity. At 1.0 kW/cm2 while fibre ablation laminas and matrix decomposition hardly
intensity, the carbon fibre was not fractured thus remained to carry influenced the strength of the composite plate. The findings agreed
most of the loadings. However, at 2.5 kW/cm2, both fibres and resin with those from the previous literatures that carbon fibre ablation
matrices were burned out very quickly, followed by the failure of and epoxy matrix thermal decomposition were the primary dam-
the main load-carrying plies (0 plies) after which the tensile age modes for degrading carbon/epoxy composites under directed
strength plummeted. energy such as laser irradiation [72,73,75]. Carbon fibre ablation
Liu et al. [77] developed a multiscale based bridge model to and epoxy matrix thermal decomposition were the main damage
predict the progressive damage of carbon epoxy composite under modes on composite strength decrease.
the combined laser and mechanical loading. Firstly, the thermal Kujawinska et al. [79] conducted experimental study to inves-
response of the composite plate was evaluated by means of an tigate the interaction of a high power near-IR laser beam and
ablation model. The ablation process was divided into three forms, composite material samples composed of sandwich structures of
i.e. heat exchange, matrix decomposition, and carbon fibre subli- fibre-reinforced polymer, and to determine the symptoms and ef-
mation, based on the different responses of the composite plate fects against UAV’s airframe shell by a laser beam. Specimens of
under laser irradiation. The model was employed to obtain the carbon and glass fabric woven resin shells and carbon reinforced/
ablation temperature field and recession rate of the carbon/epoxy epoxy laminate were irradiated by impulse laser beam Nd:YAG
composite laminate. The numerical results were compared with the laser with 1.06 mm wavelength. The specimen was illuminated with
laser irradiation experiments of the composite material laminates, 10 impulses of 5J each. The laser had a maximum power of 20 kW.
subjected to a high-power CO2 laser with a power density of 3D digital imaging projected the interaction of the specimens and
1.528 kW/cm2 and 3.82 kW/cm2 respectively. The numerical and laser beam as displacement maps and temperature maps. An
experimental results were found to be comparable. Moreover, the infrared camera (FLIR SC 7500) near the back surface of the spec-
bridge model (multiscale bridge model) was revised based on the imen took the maps. Two-100 W LED reflectors were used to
Ramberg Osgood model, using the polynomial strengthening enhance illumination on the specimen. DIC software (VIC 3D) was
model for reducing the input parameters of the matrix. Thus, the used to process the recorded images. The specimens were made of
improved bridge model was found to be capable of dealing with sandwich structures for typical UAVs which composed of two car-
existing thermal stresses in the thickness direction while predicting bon and glass fibre woven fabrics face-sheets reinforced by a foam-
the progressive damage and the ultimate strength of composite core. The results obtained indicated that glass-reinforced sandwich
plate. required a smaller number of laser impulses to start degradation of
The high intensity laser beam may incur damage to the com- the composite structure compared to the carbon-reinforced sand-
posite structure by heat re-radiation even without penetration or wich of the same thickness (5 mm). On the other hand, carbon-
material degradation at the target’s surface. From the military point reinforced sandwich needed approximately twice the number of
of view, this is extremely useful as far as the laser lethality of UAVs laser impulses to disintegrate compared to the carbon reinforced
and helicopters is concerned. In order to explore this possibility, an laminate. Specimens reinforced with a foam-core had a better
explicit uni-dimensional heat transfer model was developed at the strength and resistance to the laser beam pulses. A decrease in the
Naval Research Laboratory to study the heat re-radiation from a thickness of the foam-core, however, resulted in the reduction in
carbon-fibre composite skin to the internal components [78]. strength of the composite structure. A specimen of a 1.5 mm thick
Although this model was a unidimensional model, i.e. it did not core was destructed more severely compared to a sample with a
account for the changing material properties of the carbon fibre 5 mm foam-core.
composite, it did provide useful insights to the researchers inter-
ested in exploring the heat re-radiation laser effects on composite 5.5. Other studies
materials. Mechanical analysis on composite failure revealed that
the tensile strength occurred at the 9th lamina failure. At the 9th Boley et al. [80] developed models of laser interactions with
lamina, the fibre strength was 21000 MPa which revealed the composite materials consisting of fibres embedded within a matrix.
composite’s ultimate tensile strength did not occur at the 0 lamina A detailed ray trace model that can calculate the absorptivity and
breakage moment. The temperature did not change the modulus of energy enhancement of composite materials, starting with the
carbon fibre, but the extent of ablation was associated with com- optical parameters of the constituents and the material structure
posite strength. Under coupled laser, tensile load and composite was established to serve as components of a comprehensive model
strength were influenced by the fibre strength variation of of composite behaviour under the effects of laser radiation. The ray
1286 Y.X. Zhang et al. / Defence Technology 17 (2021) 1269e1288

Table 4
A summary of numerical studies.

Research Focus References Materials Loading Software Failure mode

Transient heat conduction, thermal [24] Carbon-carbon Beam of 3.0 W mm2 power density MARC program Not applicable
stress (C/C)
composite
[73] Graphite/ Laser irradiation with 0.25 kW cm2, 1.0 kW cm2 Not applicable Ablation
epoxy laminate 2.5 kW cm2, transverse loads
Laser ultrasonic generation [63] Thin fibre- Laser with 13.5 mJ and 10 ns pulse duration Not applicable Not applicable
reinforced
composite
plate
Heat flow and material damage [64] Polymer/ 100-W-nomial power, Yb:YAG fibre-coupled laser COMSOL Not applicable
carbon fibre- Multiphysics®
reinforced numerical modelling
composite program
2
[35] T300/AG80 Laser beam, 50 W cm power density, beam radius of 10 mm, ABAQUS software, Not applicable
composite 20 mm, 30 mm. Fortran
laminate
Thermo-mechanical responses [65] CFRP laminate Laser beam of radius 5 mm with heat flux 6.37  106 W m2, Not applicable Progressive
. 10.19  106 W m2 and 12.74  106 W m2 cracking; interface
propagate
[34] CFRP laminate Continuous wave laser, long pulsed laser (200 ns pulse Axis-symmetrical Ablation; epoxy
duration), short pulsed laser (10 ns pulse duration) with finite element model matrix
3.54  106 W m2, 1.50  1012 W m2, and 3.00  1013 W m2 sublimation
respectively
Laser-CFRP interaction [27] CFRP laminate Laser irradiation with 9.9 W cm2 MATLAB® coded 3D Combustion;
thermal model decomposition
Ablation characteristics, [67] CFRP laminate 38 W power output laser beam with 1.25 mm laser radius Finite element Ablation
temperature distribution, heat method and
affected zone (HAZ), ablation Deformed Geometry
morphologies of COMSOL
Ablation temperature field, [71] T300/epoxy CO2 continuous laser with intensity of 1.528 kW cm2 and ABAQUS Ablation; pyrolysis
recession rate resin laminate 3.82 kW cm2
Strength reduction, dynamic and [72] Organic-matrix Laser irradiation (1.33 kW cm2 and 2.79 kW cm2) Not applicable Ablation; material
buckling characteristic composite removal.
laminate
Accumulative damage [74] T300/KH304 Laser irradiation ANSYS Interlaminar
composite cracks
laminates
Progressive damage [76] AS/3501-6 Laser irradiation (1.0 kW cm2 and 2.5 kW cm2) Not applicable Fibre/resin burn
composite out; main load-
laminate carrying plies
failure
[77] Carbon/epoxy High-power CO2 laser (1.528 kW cm2 and 3.82 kW cm2) ABAQUS Progressive
composite damage
laminate

trace model was found to be sufficient for the description of of energy systems. The general damage mechanisms of laser sys-
carbon-based composites. The calculation of the absorptivity of the tems hitting aircraft composite structures, and the failure behav-
composite material for different frequencies of incident radiation iour of composite materials under combined laser and mechanical
and the energy enhancement was presented. It was concluded that loadings are particularly reported.
the ray trace model would be more time consuming when applied The experimental studies reported include the investigation on
to glass fibre-based composites. Additionally, their approach was the thermos-mechanical response, the ablation behaviour caused
able to calculate the energy deposition in the material which could due to laser energy dissipating in the plasma layer near the target
be part of a predictive thermomechanical description of material surface, the interlaminar damage mechanism and other damage
behaviour under the effects of high-power laser radiation. mechanism of various composites (CFRP, GFRP, etc). The effects
A summary of the numerical studies is given in Table 4 with the from both sole laser loading and combined laser and mechanical
loading situation, materials and structured modelled, software loading are included. It was found that most of the reported
used for the modelling and the typical failure mode for each experimental studies were mainly focused on CFRP laminate
research focus. composites-. Laser systems are found generally effective against
target of composites; however, complete destruction of the target
6. Summary will require extremely powerful output and for a considerably long
duration.
In this paper we presented a review of literature on damage to Numerical studies including thermal-mechanical response,
aircraft composite structures caused by directed energy systems. ablation behaviour, interlaminar effects and dynamic response of
We firstly discussed the application of composite materials in the composite materials under laser irradiations are reviewed. These
aircraft structures and the common types of directed energy sys- numerical studies further provide an insight into the damage
tems and the mechanisms of their effect. We then presented a mechanisms of laminate composites under laser irradiation. A va-
detailed literature review on the reported experimental and nu- riety of numerical methods have been employed to simulate and
merical studies of aircraft composite structures subject to the effect analyse the sort of problem, which paves the way of establishing
Y.X. Zhang et al. / Defence Technology 17 (2021) 1269e1288 1287

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