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1 Single-Shot Terahertz Time Profiling Using Curved Wavefront
1 Single-Shot Terahertz Time Profiling Using Curved Wavefront
5, SEPTEMBER 2018
Abstract—We report an improved single-shot electro-optic sam- physical chemistry, and in a number of other fundamental areas
pling (EOS) based detection scheme to measure the time profile of science [11], [12]. An important procedure carried out with
of a terahertz (THz) pulse using inherent curvature of a converg- THz radiation is the THz time-domain spectroscopy (THz-TDS)
ing wavefront. A simple addition to conventional multishot EOS
technique enables single-shot recording of THz time profile. While [13], capable of resolving spectral features of several chemicals
the temporal resolution of the proposed method is limited only [14], drugs [15], and explosives [16]. In THz-TDS, an ultra-
by the duration of the probe laser pulse, the spatial resolution short laser pulse probes the THz field amplitude at successive
can be externally controlled with ease. Our method is easy to im- intervals in time to construct the complete temporal waveform
plement and has the potential to provide better signal-to-noise of the radiation. It is a rather time-consuming process and is
ratio compared to other single-shot methods. An interesting spin-
off of the proposed technique is that the quintessential space-to- prone to large errors when the source itself or the background
time calibration process itself reveals the spatial profile of the THz conditions suffer from significant variations. Moreover, with the
radiation. The technique is simple yet versatile and capable of present-day high-power THz sources based on lasers and accel-
characterizing THz radiation emitted by high-power THz sources erators, the well-known multishot delay scanning methods for
employing ultrashort intense lasers and modern-day particle ac- waveform detection are impractical as they offer low repetition
celerators. As a proof of principle demonstration, we provide
measurement and characterization of the THz pulse emitted rates and are prone to large shot-to-shot fluctuations.
by two-color laser-produced plasma in ambient atmosphere In addition, some experiments require more than one temporal
using 45 fs Ti:sapphire laser pulses. Our method faithfully delay line, like the study of carrier dynamics in semiconductors
reproduces the THz waveform measured by conventional scanning [17] or understanding the contribution of various vibrational,
EOS technique. electronic, and rotational degrees of freedom in the composite
Index Terms—Electro-optic (EO) detection, imaging, laser ap- response of a system subjected to THz radiation [18]. Addition
plications, signal detection, terahertz (THz) radiation, ultrashort of such multiple delay lines further increases the time taken
laser. to record an entire dataset for a single sample. While reading
I. INTRODUCTION reversible processes, the sequential detection of signal suffices
to yield the required information, but the irreversible phenom-
LACUNA in the electromagnetic wave spectrum between
A far infrared and microwaves remained for long in the ab-
sence of efficient electronic or optical methods of generation and
ena demand an accurate single-shot waveform acquisition as a
prerequisite. This desire to record rapid time dynamics of phe-
nomena, e.g., material damage, structural phase transitions, or
detection. This spectral region from 0.1 to 10 terahertz (THz) chemical changes, has led to the growth of a few single-shot
was thereby termed as the “THz gap,” and extensive research waveform detection methods in the THz domain, each having
during the last two decades has been able to almost fill it [1]–[4]. their own merits and demerits [18], [19].
Demand for an intense and brighter source has ever been rising, The most widely used method for single-shot detection of
owing to vast and diversified application areas from medicine THz radiation is spectral encoding [20], wherein the temporal
[5] to security [6], from astronomy [7] to communication [8], profile of the THz pulse is encoded on a sufficiently long tempo-
and from basic research in material science [9] to crucial in- rally chirped probe pulse, as they pass through an electro-optic
vestigations like cancer diagnosis [10]. Static and time-resolved (EO) crystal. However, an additional system for the introduction
spectroscopy, along with imaging in the THz regime, has proved of temporal chirp in the laser beam is required, and the knowl-
to be a powerful research tool in condensed matter physics, edge of its exact frequency-to-time calibration is crucial. Despite
its popularity, this method has an inherent temporal resolution
Manuscript received April 1, 2018; revised June 2, 2018 and June 21, 2018; limit [21] given by the square root of the product of chirped pulse
accepted June 22, 2018. Date of publication June 27, 2018; date of current
version September 10, 2018. (Corresponding author: Suman Bagchi.) time duration and the Fourier transform limited pulse duration.
S. Saxena, S. Bagchi, P. A. Naik, and J. A. Chakera are with Raja Ramanna Therefore, it is not suitable for measuring very short duration
Centre for Advanced Technology, Indore 452013, India (e-mail:,sonals@rrcat. THz radiation pulses. This problem was somewhat addressed by
gov.in; sbagchi@rrcat.gov.in; panaik@rrcat.gov.in; chakera@rrcat.gov.in).
B. S. Rao is with the Center for Relativistic Laser Science, Institute of Basic the spectral interferometry detection technique [22], wherein the
Sciences, Daejeon 34126, South Korea, on leave from Raja Ramanna Centre for chirped probe carrying THz information is collinearly matched
Advanced Technology, Indore 452013, India (e-mail:,sunnyb@rrcat.gov.in). with a short transform-limited duration readout pulse sent after
Color versions of one or more of the figures in this paper are available online
at http://ieeexplore.ieee.org. a delay in a spectrograph. In this case, the temporal resolution
Digital Object Identifier 10.1109/TTHZ.2018.2851154 is defined by the duration of the readout pulse. In addition to
2156-342X © 2018 IEEE. Personal use is permitted, but republication/redistribution requires IEEE permission.
See http://www.ieee.org/publications standards/publications/rights/index.html for more information.
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SAXENA et al.: SINGLE-SHOT THz TIME PROFILING USING CURVED WAVEFRONT 529
for laser wavelength λ and focal spot size “w0 ” represents the
conventional meaning of the Rayleigh range of the focusing ge-
ometry. When this converging wavefront is incident on a plane
at a distance z, perpendicular to the propagation direction of the
beam, it is evident that the off-axial, i.e., marginal, rays will
arrive earlier than the axial rays. In other words, a finite time
delay δt exists between the arrival of marginal and axial rays.
The value of the delay δt is therefore governed by the wavefront
curvature ξ(z) = 1/R(z), where R(z) is the radius of curva-
ture of the wavefront at a distance z from the focal spot. For
a Gaussian beam, the radius of curvature can be conveniently
written as
z 2
R
R (z) = z 1 + (1)
z
and the corresponding beam radius at z can be written as
2
z
w (z) = w0 1 + . (2)
zR
Fig. 1. (a) Curved wavefront of converging laser beam at some plane perpen- Considering the instant at which the marginal rays just touch
dicular to the laser propagation direction, at z distance from the focal plane. the vertical plane at z, the spatial separation between the position
Wavefronts at other positions are shown as dotted lines. (b) Evolution of beam
radius and the radius of curvature are plotted with increasing distance from the of marginal rays and the axial ray can be written as
beam waist z. (c) Time delay between the fastest and the slowest part of the
curved wavefront with increasing defocussing distance. δz = R (z) (1 − cos θ) (3)
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530 IEEE TRANSACTIONS ON TERAHERTZ SCIENCE AND TECHNOLOGY, VOL. 8, NO. 5, SEPTEMBER 2018
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SAXENA et al.: SINGLE-SHOT THz TIME PROFILING USING CURVED WAVEFRONT 531
Fig. 5. (a) Temporal waveforms of the THz electric field obtained through
multishot and single-shot detection methods. (b) Spectra corresponding to mul-
tishot and single-shot detection techniques.
Fig. 3. (a) THz radiation captured as leakage intensity through the GT analyzer It should be noted that although the two-color laser-induced
prism. Intensity variation in image is directly proportional to the THz electric air plasma is a broadband source of THz radiation, the mea-
field amplitude observed at the spatial position in probe beam. (b) Line profile sured spectrum is limited because of the phase-mismatching in a
of the THz intensity taken through the image.
200-μm-thick ZnTe for frequencies beyond 5 THz [33]. Further,
the THz beam travels nearly 70 cm in air at 60% humidity level,
which curtails the spectrum even more. Dry nitrogen purging
in the THz beam path could have preserved the spectrum and
restricted the loss due to the properties of EO crystal. Non-
collinear phase-matching in the ZnTe crystal [34] plays no role
in determining the spectrum, as collinear geometry of multi-
shot EOS features a similar trend. Better temporal resolution of
the curved wavefront single-shot technique, on the other hand,
enhances the spectrum recorded.
There are two competing factors that determine the net tem-
poral resolution of this method. The laser pulse duration is the
obvious one, while the other is constituted by the effective “time
duration” of the probe pulse experienced by each CCD pixel.
The larger of these two factors limits the overall temporal res-
olution of this detection scheme. As the individual pixel size
Fig. 4. Pulse front of the probe beam at the surface of ZnTe crystal along the of the CCD camera employed is 4.65 μm2 , it therefore covers
vertical direction, as measured by the SHWS.
15.5 fs in time. Thus, the temporal resolution is governed by the
laser pulse duration itself, which is 45 fs. The temporal window
placed exactly at the place of the ZnTe crystal [31], [32]. Result scanned on single-shot basis is 2.8 ps, as is shown in Fig. 5(a).
of the SHWS measurement is displayed in Fig. 4, relating the Positioning and focal lengths of the OAPM and the lens in probe
time delay at various radial positions on the probe wavefront. beam path can be adjusted to regulate the temporal window.
The credibility and faithfulness of our single-shot THz tem- While the temporal characterization of THz radiation ob-
poral profile detection method is confirmed by comparing our tained from the current curved wavefront single-shot detection
results with those obtained from the conventional multishot EOS is commensurate with the conventional method, we now dis-
method. The same experimental setup is used for multishot de- cuss the spatial characterization conducted with this experi-
lay scanning by removing the positive lens from the probe beam mental setup. This is an additional and important advantage of
path and replacing the CCD camera with a balanced photode- our method compared to other single-shot-based techniques re-
tector. No further alignment was necessary for obtaining THz ported in literature. An indirect method of wavefront calibration
electric field trace with time in the multiple-shot mode. Fig. 5(a) requires recording of images at varying temporal delay (ΔT)
and (b) shows the multishot EOS plots in black and the traces given to the probe beam (see Fig. 2). Evidently, with varying
obtained from current single-shot detection technique in red. In probe delay, ΔT implies that the curved probe beam interacts
the multishot detection setup, an average of 20 shots at each time with different slices of the THz pulse at the surface of the ZnTe
delay was taken, because of which the error bars are also seen in crystal. Therefore, the region of spatial overlap of these two
the black plot. It is also observed that the THz temporal profile pulses shifts toward the radially outward direction. Thus, the
and spectrum obtained from the curved wavefront single-shot peak amplitude of the THz electric field is now recorded on
match closely with those obtained from the reference multishot a different radial position in the spatial extent of probe beam,
EOS technique. The negative THz electric field values could and the recorded peak intensity now depends on the profile of
be measured only because of the nonzero vertically polarized focused THz beam in space. Fig. 6 shows a schematic of the
leakage through the analyzer prism. interaction.
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532 IEEE TRANSACTIONS ON TERAHERTZ SCIENCE AND TECHNOLOGY, VOL. 8, NO. 5, SEPTEMBER 2018
V. CONCLUSION
Fig. 7. Spatial distribution of THz intensity in its focal plane as measured by
the (a) curved wavefront technique and the (b) knife-edge technique. In conclusion, we have devised a simple single-shot THz
electric field profile measurement technique based on the EOS
method. This was accomplished by addition of a positive lens
This implies that, when a smaller cross section of probe’s
to the conventional EOS experimental setup. The curved wave-
wavefront close to axis is coincident with the THz peak electric
front of the probe laser scans the entire THz electric field profile
field, the ring formed in images captured shall be smaller and
and generates a 2-D image with THz information encrypted as
brighter. Similarly, interaction of THz peak field amplitude with
intensity variation. This time-integrated image provides the THz
a larger (i.e., marginal) cross section of probe’s wavefront in the
field evolution with time as intensity variation along the radial
ZnTe crystal shall result in images with bigger and less intense
vector on a single-shot basis. Space vector in the image is related
rings. If the linear intensity profiles through each of these im-
to temporal delays in the probe’s wavefront. The space-to-time
ages are plotted together and their respective peak positions are
mapping is carried out in multiple steps by changing the probe
identified, the spatial profile of THz focal spot is reconstructed.
delay and recoding the variations. The mapping yields intensity
As shown in Fig. 7(a), the Gaussian curve fitted over the lin-
variation in spatial profile of the THz focal spot on a multishot
ear intensity profiles at varying probe delay features 1.94-mm
basis. This method is therefore capable of providing the THz
value of full-width at half-maximum (FWHM). Peak values of
spatial profile in multiple shots and the temporal profile in the
the line-cuts taken at probe delays ΔT equal to 200, 400, 600,
single-shot mode. Overall, this technique offers a straightfor-
and 800 fs are marked as green circles in the graph. A reference
ward option for real-time data acquisition for THz radiation and
study for spatial distribution of intensity in the THz focal spot
may be very useful for various applications.
was also conducted using the knife-edge method. A sharp knife-
edge is traversed across the focal plane of THz in one direction.
The transmitted THz energy, measured on a detector placed ACKNOWLEDGMENT
after the THz focal plane, keeps on increasing as the knife-edge The authors would like to thank R. A. Joshi and R. K. Bhat for
passes over the spatial extent of the THz focus. When whole of laser operation and S. Sebastin, R. P. Kushwaha, D. Karmakar,
the THz spot size is exposed, the measured energy gets satu- and K. C. Parmar for mechanical support during the experiment.
rated. A derivative of this trend depicts the spatial distribution The authors also thank S. A. Pai and S. Sendhil Raja for useful
of THz energy in its focal spot. Further measurement reveals discussions and for providing SHWS for measurements.
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SAXENA et al.: SINGLE-SHOT THz TIME PROFILING USING CURVED WAVEFRONT 533
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534 IEEE TRANSACTIONS ON TERAHERTZ SCIENCE AND TECHNOLOGY, VOL. 8, NO. 5, SEPTEMBER 2018
Bobbili Sanyasi Rao was born in Visakhapatnam, Juzer Ali Chakera was born in Mhow, India, on
India, on July 15, 1977. He received the Ph.D. de- February 3, 1967. He received the B.Sc. and M.Sc.
gree from the Homi Bhabha National Institute, Mum- degrees from Holkar Science College, Indore, India,
bai, India, upon submission of the thesis entitled in 1986 and 1988, respectively, the M.Tech. degree
“Laser Driven Plasma-Based Electron Acceleration” from Anna University, Chennai, India, in 1992,the
in 2013. Ph.D. degree from Devi Ahilya Vishwavidyalaya, In-
In 2003, he joined the Bhabha Atomic Re- dore, India, in 2005, and the Postdoctoral degree from
search Centre Training School, Raja Ramanna Centre the Department of Computer and Electrical Engineer-
for Advanced Technology (RRCAT), Indore, India. ing, University of Alberta, Edmonton, AB, Canada,
Since 2004, he has been a Permanent Staff Scientist in 2008.
with RRCAT, involved in the field of laser-produced In 1991, he was with the Bhabha Atomic Research
plasmas. He is currently a Scientific Officer (F) and a Member of the Laser Centre, Mumbai, India, where he was involved in the field of laser–plasma inter-
Plasma Section, RRCAT. Since August 2016, he has been a Research Fellow actions. In 1993, he joined the Raja Ramanna Centre for Advanced Technology
with the Center for Relativistic Laser Science, Institute of Basic Sciences, Dae- (RRCAT). He is currently the Head of the Laser Plasma Section, RRCAT. His
jeon, South Korea, where his areas of research involve using 4-pW laser to research interests include higher harmonic generation, physics at ultrahigh laser
demonstrate near 10-GeV electron beams and apply them to drive bright source intensities, laser-based electron acceleration, laser-based generation of positive
of muon pairs. His research interests include understanding the physics of in- and negative ions and neutral particles, time-resolved X-ray diffraction, attosec-
tense laser–matter interactions and development of compact and bright sources ond pulse generation, X-ray lasers, and THz generation.
of ultrashort pulsed high-energy electrons, X-rays, THz rays, and also exotic
particles like muon pairs using terawatt to multipetawatt lasers.
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