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2015 - Aerial Radiation Monitoring Around The Fukushima Dai-Ichi Nuclear Power Plant - Sanada
2015 - Aerial Radiation Monitoring Around The Fukushima Dai-Ichi Nuclear Power Plant - Sanada
2015 - Aerial Radiation Monitoring Around The Fukushima Dai-Ichi Nuclear Power Plant - Sanada
a r t i c l e i n f o a b s t r a c t
Article history: The Great East Japan Earthquake on March 11, 2011 generated a series of large tsunami that seriously
Received 2 December 2013 damaged the Fukushima Dai-ichi Nuclear Power Plant (FDNPP), which resulted in the release of radio-
Received in revised form active materials into the environment. To provide further details regarding the distribution of air dose
26 June 2014
rate and the distribution of radioactive cesium (134Cs and 137Cs) deposition on the ground within a radius
Accepted 26 June 2014
of approximately 5 km from the nuclear power plant, we carried out measurements using an unmanned
Available online 19 July 2014
helicopter equipped with a radiation detection system. The distribution of the air dose rate at a height of
1 m above the ground and the radioactive cesium deposition on the ground was calculated. Accordingly,
Keywords:
Unmanned helicopter
the footprint of radioactive plumes that extended from the FDNPP was illustrated.
Radiation measurement © 2014 Elsevier Ltd. All rights reserved.
Plastic scintillator
LaBr3:Ce scintillator
Fukushima Dai-ichi nuclear power plant
Radioactive cesium
http://dx.doi.org/10.1016/j.jenvrad.2014.06.027
0265-931X/© 2014 Elsevier Ltd. All rights reserved.
Y. Sanada, T. Torii / Journal of Environmental Radioactivity 139 (2015) 294e299 295
allowed for a safety check in operated automatically monitoring consideration of the safety and reliability of the data. A measure-
flights using a computer and a communication system that received ment at 80 m AGL means that the ARMS measured the average
radio waves (2.4 GHz) from a ground station in a vehicle. Based on gamma rays emitted from the ground within a circle 80 m in radius
information about the position of the helicopter obtained by a below the helicopter in the case of an infinite plate source (IAEA,
differential global positioning system (DGPS), the operator planned 2003). Furthermore, considering the 80 m AGL, we employed a
the flight program, including the flight path, speed and altitude of flight line spacing of 80 m.
the AUH. The AUH weighs 94 kg and has a maximum payload ca-
pacity of 10 kg. Its maximum speed is 72 km/h (about 40 knots). The
2.4. Calibration parameter
flight duration is 1.5 h in a filled-up fuels.
To convert the total count rate measured in the air into the air
2.2. Radiation measurement system dose rate at 1 m AGL, we measured the air dose rate at a height of
1 m using a NaI survey meter (TGS-172B, Hitachi Aloka Medical, Ltd,
We employed three LaBr3:Ce scintillation detectors (38.1 mm in Tokyo Japan) at 30 locations in a test area within the evacuation
diameter 38.1 mm in length), packaged with supporting electronics zones near the FDNPP. This survey meter was calibrated based on a
to create the 6.5 kg Aerial Radiation Measurement System (ARMS), Japanese standard (JIS, 2014). The test area was selected for its flat
which was installed under the helicopter. The ARMS was electrically topography and little variation in air dose-rate results. At the test
insulated by the AUH to reduce the occurrence of mutual in- area, the helicopter hovered at 10 m or 20 m AGL intervals from
terferences. Noise derived from the AUH was not detected in ARMS 10 m to 100 m AGL, and we measured the total count rate at each
data. The count rate of the three detectors, and the spectral and po- height. Fig. 2 shows the relationship between total count rates
sition data of the DGPS were acquired and stored in the ARMS every measured as a function of AGL altitudes. An effective attenuation
second. The pulse signal of the LaBr3:Ce scintillation detector from factor (AF) was selected from an exponential regression of each
0 keV to 3000 keV is preserved in each of the 1024 channels of the background-corrected count rate and height. Furthermore, the air
multi channel analyzer (MCA) in the ARMS. Any signal greater than dose-rate conversion factor (CDsd) was calculated as the ratio of the
3000 keV was only counted without information on gamma energy. total count rate of at 80 m AGL to the air dose rate at 1 m AGL in the
Any signal less than 50 keV was removed by the pulse height test area.
discriminator. The energy resolution (full width at half maximum over A background spectrum was collected at 80 m above the sea
the peak position) for the 662 keV photopeak was 2.8%. This resolution (gray line in Fig. 1). The background spectrum represents radio-
is sufficient to discriminate between the photopeaks of 605 keV logical contributions from (1) inherent contaminants within the
(134Cs) and 662 keV (137Cs). The gamma spectra of the three detectors LaBr3:Ce crystal, (2) any sources in/on the AUH and associated at-
were stored individually and summed after each flight. Detector tachments, and (3) cosmic radiation. The inherent-contamination
sensitivity dependency on temperature was corrected with a tem- of the LaBr3:Ce crystal is due to the presence of natural radionu-
perature compensation circuit. The output from the ARMS was down clides of the detector material itself, such as 138La, and contami-
linked to the ground station using a wireless local area network; thus nation by 227Ac, a chemical homolog of lanthanum (Nicolini et al.,
the count rate data were displayed in real time on a map. 2007). The influence of cosmic rays varies with the altitude of the
Samples of the gamma spectra measured in the evacuation zone flight. However, because variation of count rate due to cosmic rays
around the FDNPP are shown in Fig. 1. These spectra, representing a is smaller than the count rate of the radioactive cesium around the
period of 100 s, were obtained hovering at 100 m AGL and above the FDNPP, the influence of cosmic rays on the calibration parameter is
sea in December 2012. Both measurement areas were in Futaba- considered as negligible.
machi, which is 5 km north of the FDNPP. The spectrum repre-
sented by the black line was obtained in the area in where the air
2.5. Data analysis
dose rate at 1 m AGL was 10 mSv/h. Another spectrum represented by
a gray line was obtained above the sea 200 m from the shore.
2.5.1. Air dose rate
Although the gamma-ray energy spectrum can be collected with
2.3. Data acquisition the ARMS, we used the gross count rate for estimation of the air
dose rate, which includes the contribution from natural radiation.
Most of the flights were carried out at a speed of 8 m/s and 80 m
AGL. We selected this flight altitude as a standard altitude (Hsd) in
Fig. 2. Example of the relationship between the count rate of the ARMS and AGL flight
Fig. 1. Gamma spectra of the ARMS (three LaBr3:Ce detectors) above the ground and altitude. AF is the inclination of the exponential fitting curve. Air dose rate of this point
above the sea in Futaba-machi, 5 km from the FDNPP. Measurement time was 100 s. (in Namie-machi, 8 km from the FDNPP) was 0.6 mSv/h. The error was twice the
Measurement date was 22 December 2012. standard deviation of the measurement result.
296 Y. Sanada, T. Torii / Journal of Environmental Radioactivity 139 (2015) 294e299
We selected the total count rates of this background spectrum (gray point, because the data obtained by the unmanned helicopter are
line in Fig. 1) as the background count rate (BG). The air dose rate at an average value representing the area below the helicopter.
1 m AGL (D1m) was calculated from the airborne count rate by Moreover, the environmental effects pointed out by IAEA (2003)
subtracting BG from the gross count rate (GC). The AGL altitude was (e.g. shielding condition from source to detector, soil moisture, Rn
evaluated to subtract the altitude of the digital elevation model progeny in air and topographic effects) may also be responsible for
(DEM) data (GSI, 2011) of the 10 m mesh from the GPS altitude the slight data mismatch. Evaluation of these effects will be
(altitude above sea level). The difference of the real flight altitude necessary in the future.
(H) and Hsd was corrected using AF. The D1m is given by Eq. (1). The minimum detectable air dose rate (MDD) is 0.07 mSv/h at
80 m AGL. The MDD was calculated from the BG count rate obtained
above the sea, and the MDDs were converted into the air dose rate
D1m ¼ ðGC BGÞ CDsd exp½ AF ðH Hsd Þ (1) at 1 m AGL using Eq (1). To create a map of the air dose rate dis-
To evaluate the radioactive cesium deposition on the ground, we tribution, the air dose rate data obtained were interpolated using
used the method of calculating radioactive cesium deposition on the Kriging method (IAEA, 2003).
the ground from the air dose rate of the radioactive cesium. Here,
the air dose rate of the radioactive cesium was calculated by sub- 2.5.2. Radioactive cesium deposition on the ground
tracting the air dose rate by the cosmic ray and natural radionu- The radioactive cesium deposition on the ground (Rd) was
clides in AUH and ARMS from the measured air dose rate. The calculated from the air dose rate excluding the radiation from
relationship between the radioactive cesium deposition on the natural radionuclides in the ground. This is possible because those
ground and the air dose rate of the radioactive cesium was obtained from cesium are much lower than the gamma-ray energies from
using an in-situ Ge detector. radioactive cesium from the naturally occurring K, U, and Th at
Fig. 3a shows a comparison between the ground measurement 1471 keV, 1765 keV, and 2615 keV, respectively. Due to the inherent
results of 2500 points by the NaI survey meter at 1 m AGL and the contamination within the LaBr3:Ce crystal, it is difficult to correctly
ARMS measurements. These data all agreed well within the slope estimate the terrestrial component of natural radiation because the
range of 0.5e2, indicating that the two systems can accurately internal 138La emission (1436 keV) closely coincides with the nat-
measure the air dose rate distribution on the ground within an ural 40K emission (1461 keV). To overcome this challenge, the
uncertainty factor of 2. However, at certain points, the air dose rate contribution of the natural radionuclides to the air dose rate was
measured by the ARMS was higher or lower than that obtained by measured at 104 locations around the FDNPP using an in situ Ge
the ground measurement. This could be because such points are detector (Falcon 5000, CANBERRA Industries Inc., Meriden, CT), and
locations where the air dose rate is heterogeneous (for example the average air dose rate from natural radionuclides in the ground
1.0e10 mSv/h within 1 km2). The measurement results obtained by of 31.3 nSv/h, was estimated to be the background air dose rate
the ARMS may not match the ground measurement data at every (Dnat). The ratio of 134Cs/137Cs (B) was determined by the ratio of
Fig. 3. Comparison of AUH and measurement. Top left (a) shows results from the NaI survey meter. Top right (b) shows results of the in situ Ge measurement. Almost all plots are
between the two lines (y ¼ 0.5x, y ¼ 2.0x) shown in the figure. The figures on the bottom show the distributions of the ratios for the NaI survey meter (c) and in-situ Ge mea-
surement (d).
Y. Sanada, T. Torii / Journal of Environmental Radioactivity 139 (2015) 294e299 297
photopeak counts of 661 keV (137Cs) and 796 keV (134Cs) by using
the gamma-ray energy spectrum. The B on the measurement date
was similar to the value of the physical decay of the radioactive
cesium from the calibration date (the ratio of 134Cs/137Cs was 0.917
on Aug. 13, 2011 (MEXT, 2011)). The radioactive cesium deposition
on the ground was calculated using the conversion factor
(CF ¼ [kBq/m2][mSv/h]1) obtained from the air dose rate. The CF
was given by the relaxation mass per unit (b) of 1.0 g cm2 (ICRU,
1994). The b was used for consistency with the depth profile
measurements of the FDNPP (Kato et al., 2012). The Rd is shown in
Eq. (2).
B CF134 þ CF137
Rd ¼ ðD1m Dnat Þ (2)
Bþ1
where CF134 and CF137 are the conversion factors for 134Cs and 137Cs,
respectively.
A comparison between the ground measurement results ob-
tained by the in-situ Ge detector at 128 points that were 1 m AGL
and the analyzed results measured by the ARMS are shown in
Fig. 3c. These data agree well within the range of 0.5e2, indicating
that the ARMS can accurately measure the radioactive cesium
deposition on the ground. As shown by the preceding measure-
ment and the analysis, we can detect a minimum detectable ac-
tivity (MDA) of 4 kBq/m2 of radioactive cesium at 80 m AGL.
Fig. 4. Flight path of the AUH. There are gaps in the flight path because of a power Prior to this study, aerial monitoring using manned helicopters
transmission line. had only been used to measure data at a distance of 3 km or greater
Fig. 5. (a) Distribution map of the air dose-rate at 1 m AGL as measured by the AUH. The mesh of the map was 5 m. Data were decay-corrected to March 20, 2013. (b) Distribution
map of the air dose-rate at 1 m AGL as measured by the manned helicopter. The mesh of the map is 250 m. Data were decay-corrected to March 20, 2013. Black dots indicate the
flight path.
298 Y. Sanada, T. Torii / Journal of Environmental Radioactivity 139 (2015) 294e299
from the FDNPP due to the aviation regulations in Japan. However, rate distribution around the FDNPP obtained after the accident,
these regulations do not pertain to low altitude unmanned heli- providing important information for analysis of the accident.
copters, so we decided to measure the air dose rate within a 5 km
distance from FDNPP using the AUH. The entire survey was
3.2. Distribution of radioactive cesium deposition on the ground
completed over a period of 52 d from January 28, 2013 to March 20,
2013 using a line spacing of 80 m AGL. Fig. 4 shows the flight path of
The distribution of the radioactive cesium deposition on the
the AUH.
ground was obtained along with the air dose rate. The radioactive
Fig. 5a shows the distribution map of the air dose rate measured
cesium deposition on the ground was evaluated using the air dose
by the AUH. These data are decay-corrected to March 20, 2013 by
rate as previously mentioned, and the results are shown in Fig. 6.
the physical half-lives of radionuclides. Four deposition patterns in
The area with the greatest concentration of radioactive cesium was
which the air dose rate is particularly high extend from the FDNPP,
in the southern and western parts up to 3 km from the FDNPP site.
as clearly seen in the figure. This indicates that there were four
We were able to obtain the distribution of the radioactive cesium
unique releases of radioactive material during the accidents. High
deposition on the ground by this AUH monitoring.
air dose rate areas consist of four zones around the FDNPP. The
southern area had the highest air dose rate. The western area
seemed to be divided into two sections, and the high air dose-rate 4. Conclusion
area in the west appeared from a location several hundred meters
away from the boundary of the FDNPP site as shown in Fig. 5a. The To clarify the distribution of radioactive cesium deposition, we
air dose rate in the northwestern area was comparatively low. performed measurements over a wide area around the FDNPP us-
The distribution map produced from aerial monitoring using the ing the ARMS. This technique combines airborne monitoring and
manned helicopter is shown in Fig. 5b. These data were collected ground monitoring, and is useful in clarifying the detailed distri-
from October 31, 2012 to November 16, 2012 (MEXT, 2013) and are bution. This technique visually expressed the dispersion patterns of
decay-corrected to March 20, 2013 by the physical half life. Because the radioactive material around the FDNPP and clearly showed the
the spacing of the flight line with a manned helicopter (1.8 km) was deposition from the radioactive plumes emitted by the accident.
wider than that of the unmanned helicopter, the position resolution Because duplicate measurements are easily performed using AUH
of the map was relatively rough. Because flight conditions (altitude, monitoring, this method is effective for investigating the migration
speed and detector) are different, both maps do not completely of radioactive materials in the environment. In subsequent exper-
agree, but the tendency of the distribution maps was similar. iments, we will perform observational and analytical research on
Prior to this study, the air dose-rate distribution around the the migration of the radioactive cesium around the FDNPP.
FDNPP had not been measured by either airborne monitoring or
ground measurement. Our results show the first detailed air dose- Acknowledgment
References
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