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Exchange Magnon in Microwave Cavities
Exchange Magnon in Microwave Cavities
Yunshan Cao1 , Peng Yan1 , Hans Huebl2,3,4, Sebastian T.B. Goennenwein2,3,4, and Gerrit E.W. Bauer5,1
1
Kavli Institute of NanoScience, Delft University of Technology, Lorentzweg 1, 2628 CJ Delft, The Netherlands
2
Walther-Meißner-Institute, Bayerische Akademie der Wissenschaften, 85748 Garching, Germany
3
Nanosystems Initiative Munich, D-80799 München, Germany
4
Physik-Department, Technische Universität München, D-85748 Garching, Germany and
5
Institute for Materials Research and WPI-AIMR, Tohoku University, Sendai 980-8577, Japan
(Dated: March 25, 2015)
arXiv:1412.5809v3 [cond-mat.mes-hall] 24 Mar 2015
We formulate a scattering theory to study magnetic films in microwave cavities beyond the independent-spin
and rotating wave approximations of the Tavis-Cummings model. We demonstrate that strong coupling can be
realized not only for the ferromagnetic resonance (FMR) mode, but also for spin wave resonances (SWRs); the
coupling strengths are mode dependent and decrease with increasing mode index. The strong coupling regime
can be also accessed electrically by spin pumping into a metal contact.
II. MODEL fields, where, the exchange field Hex = J∇2 m with exchange
constant J. For wave vector k = k x̂, the coupled Eqs. (3) and
The weak to strong coupling transition can best be stud- (4) become,
ied in a simple configuration as shown in Fig. 1(a). The ! !
calculations for general configurations will be reported else- (1 + uk )kε2 −ivk kε2 hx
= 0. (5)
where. The magnetic film lies in the y-z plane between the ivk kε2 (1 + uk )kε2 − k2 hy
cavity defining mirrors. The equilibrium magnetization points
with ωM = γµ0 Ms , ωH = γµ0 H, ωk = ωH + JωM k2 − iαω
into the z-direction by crystal anisotropy, dipolar, and ex-
and
ternal magnetic fields. The incident microwave propagates
along x with rf magnetic field linearly polarized along y. ωk ωM ωωM
uk = 2 , vk = 2 . (6)
The cavity walls are modeled by the permeability µ(x) = ωk − ω2 ωk − ω2
µ0 [1 + 2ℓδ(x) + 2ℓδ(x − L)], where L is the cavity width and
ℓ models the wall opacity. In the absence of sources, the mi- The secular equation of Eq. (5) gives the dispersion relation
crowaves satisfy the Maxwell’s equation in frequency space, for the coupled microwave and spin wave modes or magnon-
polaritons [26–28]
µ(x) 2
∂2x h(x) +
h i
q h(x) = 0, (2) (1 + uk )k2 = (1 + uk )2 − v2k kε2 . (7)
µ0
√ III. RESULTS
where q = ω/c, with vacuum speed of light c = 1/ ε0 µ0 , and
ε0 , µ0 are the vacuum permittivity and permeability, respec-
A. Paramagnet (J = 0)
tively.
Inside the magnetic film, we consider small-amplitude spa- We first consider the simplest case of a paramagnet with un-
tiotemporal magnetizations M = Ms ẑ + m, where Ms is the coupled spins (J = 0), which is equivalent with the macrospin
saturation magnetization and m is driven by the rf magnetic model for unpinned ferromagnetic order. uk = u, vk = v are
field h, according to the Maxwell’s equation p
k independent and k = kε 1 + u − v2 /(1 + u) for a given fre-
quency ω. h x = −m x is the dipolar field. √ The susceptibil-
∇2 + kε2 h(x) = ∇(∇ · h(x)) − kε2 m(x), (3)
ity χ = ∂my /∂hy resonates at ωFMR = ωH (ωH + ωM ) with
linewidth ∆ωFMR ≃ α(2ωH + ωM ). Rewriting the hy (x, t) =
where ε is the permittivity of the magnet, kε2 ≡ εµ0 ω2 = ηq2 ,
ψ(x)e−iωt , the potentials ψ(x) in the five separated regimes
and dielectric constant η = ε/ε0 . M is governed by the LLG
marked in Fig.1(b) read
equation,
α ψ1 (x) = eiqx + Fe−iqx , ψ2 (x) = a1 eiqx + a2 e−iqx , (8a)
∂t M = −γµ0 M × Heff + M × ∂t M, (4)
Ms
ψ3 (x) = b1 eikx + b2 e−ikx , ψ4 (x) = c1 eiqx + c2 e−iqx , (8b)
where γ, α are the gyromagnetic ratio and Gilbert damping
constant, respectively. The effective magnetic field Heff =
Hẑ + Hex + h, consists of external, exchange, and rf magnetic ψ5 (x) = S eiqx . (8c)
3
The coefficients {S , F, a1 , a2 , b1 , b2 , c1 , c2 } are determined by ∝ d and by the dielectric constant η. Anti-crossings be-
the electromagnetic boundary conditions of continuity and tween magnetic andqcavity modes occur at ωFMR = ωc,n or
flux conservation at each interface. The transmission coeffi- µ0 Hres,n = (−ωM + ω2M + 4ω2c,n )/ (2γ). When not stated oth-
cient is
erwise, we use the parameters for YIG, with η = 15 [29],
1 − β2 tc2 ei(k−q)d γ/(2π) = 28 GHz/T and µ0 Ms = 175 mT [30], while reported
S = , (9) α’s range from 10−5 ∼ 10−3 [9, 31, 32]. The resonance fre-
1 − βrc eiφ 2 − e2ikd β − rc eiφ 2
quency ωc and loss rate κc of the cavity is governed by its
where φ = q(L − d), β = (ηq − k)/(ηq + k), introducing the width L and opacity ℓ. We choose L = 46 mm to be much
scattering coefficients of a single cavity wall tc = i/(i+qℓ) and larger than the film thickness d and the n = 3 cavity mode
rc = −qℓ/(i + qℓ). We first inspect the resonant cavity modes (around 10 GHz) as well as a κc,3 of the order of MHz, both of
identified by the maxima of the transmission probability |S |2 which can be tuned by ℓ.
for non-magnetic loads at
|S|2
(a) 9.91 (b) d=5μm
0.2
n = 1, 2, .... It follows from Eqs. (7) and (10) that the res- 9 n=3
9.76 Hres,3
0
onance frequencies ωc,n depend on both loading fraction d/L 0 2 4 6 8 10 0.25 0.27 0.29 0.31
Loading d/L (%) Magne"c field μ0H [T]
and dielectric constant η. The cavity mode frequencies for a
|S|2
nonmagnetic load are shown in Fig. 2(a). Odd modes ωc,2 j−1 13 (c) d=1mm 2.0 (d) g3 g4
1.0
1.6 80
p=1
p=1
at the edges y = 0. The magnetization dynamics at the in-
g(p)/2π [MHz]
30 30 40
1 2 3 4 5 6 7 terface then injects a spin current into the Pt film that gener-
sp
20 0.5 20 ates a Hall voltage VISHE = DISHE js over the Pt wire, with
p=3
DISHE ≡ (2e/~)θξ(d/σdy) tanh(dy /2ξ). We illustrate strong
10 10
p=5 coupling in the VISHE spectrum here for the paramagnetic (un-
d=10μm
0 0
1 3 5 7 9 0.5 0.7 0.9 1.1 1.3 pinned macrospin) limit J = 0. The pumped spin current can
Mode number p d [μm1/2] be written
# Z L+d
~g↑↓ v2 iv∗
" !
sp r ω 2
js = 2
Im u − ∗
dx|ψ3 (x)|2 . (14)
FIG. 3. (a,b) : Transmission for d = 1 µm and d = 5 µm; (c,d): 4πdMs 1+u 1+u L−d
2
Mode-dependent coupling strengths. In the calculations we used cav- We assume that the Pt wire has the width dy = 10 nm with
ity opacity ℓ/L = 2, Gilbert damping α = 10−5 , and ferromagnetic
exchange constant J = 3 × 10−16 m2 [8].
conductivity σ = 107 (m · Ω)−1 , spin mixing conductance
g↑↓ 19 −2
r = 10 m , spin Hall angle θ = 0.11 and spin diffusion
length ξ = 1.5 nm [36]. The spin back-flow contributes a mi-
The magnetization dynamics now becomes sensitive to the
nor correction that we disregard since ξ ≪ dy . The rf magnetic
surface boundary conditions. Kittel [33] has shown that
amplitude is chosen as µ0 h0 = 10 µT. The microwave power
pinning of the magnetization at the surface is required for
absorption is defined as the integration of the Poynting vector
SWR (the absorption of spatially homogeneous microwaves
enclosed by a section of the volume of the sample reads,
by higher order spin waves), and the symmetrically pinned
! Z L+d
boundaries merely render odd modes observable. Here µ0 dy dz ω v2 2
we adopt boundary conditions m((L ± d) /2) = 0, which Pabs = Im u − dx|ψ3 (x)|2 . (15)
2 1 + u L−d 2
can be justified by sufficiently strong surface anisotropies
(p) sp
[34, 35]. The standing spin wave frequencies are ωSWR = By substituting u and v, we find that js /Pabs ∝ ωM (ωM +
p
(ωH + 2JωM (pπ/d)2)(ωM + ωH + 2JωM (pπ/d)2) where p ∈ ωH )/α[ω2 + (ωM + ωH )2 ] is almost a constant near the reso-
N0 . We consider in the following magnetic film thicknesses nance, which proves that the spin pumping is a reliable mea-
in the range 0.1 ∼ 5 µm. Naively, exchange effects are sure of the microwave absorption. VISHE as a function of rf
5
VISHE /(25nV)
9.85 0.6 2954/1, GO 944/4) and the collaborative research center
ωc,3 SFB631 (C3).
9.82 0.4
9.79 0.2
9.76 Hres,3 0
d=10μm
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for Scientific Research (Grant Nos. 25247056, 25220910, 85, 043815 (2012).
6
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