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Environ. Eng. Res.

2024; 29(1): 230166 pISSN 1226-1025


https://doi.org/10.4491/eer.2023.166 eISSN 2005-968X

Research

Utilization of methane from municipal solid waste landfills


Abiy Tadesse1, , Jechan Lee2,
1
National Research Development and Nuclear Reactor Research, Ministry of Innovation and Technology, Arada Sub-city, Churchel Road, 2490, Addis
Ababa, Ethiopia
2
Department of Global Smart City & School of Civil, Architectural Engineering, and Landscape Architecture, Sungkyunkwan University, 2066
Seobu-ro, Suwon, 16419, Republic of Korea

Received March 24, 2023 Revised May 17, 2023 Accepted May 17, 2023

ABSTRACT
Here, we analyzed the utilization efficiency of methane (CH4) gas from landfill sites associated with its power generation potential in different
systems; in addition, we analyzed the reduction in the amount of CH4 emitted from landfills of untreated waste, proposed an effective method
for site selection, and investigated the environmental issues caused by landfilling solid waste. Furthermore, we evaluated the geographical and
chemical characteristics, iteration variables of landfill operations, application of CH4, efficiencies of energy-converting systems, and reduction
in the CO2 emissions from other energy sources, with the landfill gas (LFG) being considered as the fuel. For efficient and quality extraction
of CH4 from LFG, we investigated the ideal landfill conditions (e.g., construction, geometry, weather, temperature, moisture, pH, and biodegradable
matter) and hydrogeological parameters that influence the generation of LFG and landfill leachate. The first order decay equation was used
to predict the CH4 generation from a single bulk municipal solid waste stream for various characteristic interims of geography and CH4 generation
capacity and potential. More CH4 is generated in the conventional clean air act condition than wet and arid conditions. Based on the analysis,
we suggest efficient and economical power generation systems for using the CH4 emissions from landfills.

Keywords: Energy converting efficiency, Landfill technology, Methane (CH4) gas, Municipal solid waste


This is an Open Access article distributed under the terms Corresponding author
of the Creative Commons Attribution Non-Commercial License E-mail: abiy0120@yahoo.com (A.T.), jechanlee@skku.edu (J.L.)
(http://creativecommons.org/licenses/by-nc/3.0/) which per-
Tel: +251920719936 (A.T.), +82-31-290-7512 (J.L.)
mits unrestricted non-commercial use, distribution, and reproduction in any
medium, provided the original work is properly cited. ORCID: 0000-0002-8568-7520 (A.T.), 0000-0002-9759-361X (J.L)
Copyright © 2024 Korean Society of Environmental Engineers

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Abiy Tadesse and Jechan Lee

Graphical Abstract

1. Introduction
2. Global Scenario of Landfill Technology for
In most countries, rapid economic growth and urbanization cause Waste Management and Energy Recovery
shortage of energy and infrastructure and limit the available land
and applicable methods for managing solid waste. In several devel- In accordance with a World Bank report, globally the average
oping countries, the increasing rate of urbanization has resulted daily waste generation reached 0.74 kg per capita [7]. Economic
in issues related to energy shortage and municipal solid waste development, in terms of the entity variables that have proportion-
(MSW) management [1]. Landfilling is one of the most convenient ally increased historically, has increased the global waste gen-
MSW management method that is widely used in both developed eration, with 2.01 billion tons of MSW being annually generated
and developing countries [2]. Landfill gas (LFG) is a byproduct globally in 2018. Based on a projection (business as usual), this
of landfilling MSW, naturally produced through the decomposition number is expected to increase to 3.4 billion tons MSW by 2050
of organic matter in landfills [3]. As indicated in previous studies, [7].
LFG has been used as a renewable energy source for local power As shown in Fig. 1, the average global landfill content consists
generation (via grid-connected energy systems) [4]. There are more of 37% of disposed waste, 33% dumped untreated waste, 19%
than 1000 LFG plants worldwide, with the majority of them being of waste hat undergoes compositing and recycling, and 11% that
in Europe and the United States of America (USA). At present, undergoes partial thermal recovery, through modern mass burn
South Africa has four LFG plants, and the demand for LFG technol- incinerators. Upper-middle income countries carry out waste treat-
ogy is increasing [5]. The Global Methane Initiative (GMI) offers ment and disposal in controlled landfill facilities. However, in
technical assistance for the deployment of energy projects that countries that have low incomes, 93% of the waste is disposed
use methane (CH4) gas worldwide, enabling partner nations develop via open dumping; while, in high-income countries, 2% of the
and implement programs for the recovery and utilization of CH4 waste is disposed via open dumping [7].
[6]. The World Bank data indicates that the global picture of LFG
In this study, we examined the global perspective of LFG con- technology mostly spread after the industrial revolution.
sumption and provide an overview of the CH4 generation and Approximately 45% of the total waste generated in the European
utilization technologies. We focused on the potential for LFG to Union (EU) is disposed in the landfill site. In China, landfilling
produce energy and the possible social and economic effects of is the most actively chosen technology, and approximately 89%
using CH4. In addition, we analyzed the geographical and economic of the country’s total solid waste is landfilled [8]. In England,
growth implications on the characteristics and techno-economic 361 LFG utilization facilities were operational in 2015, over double
feasibility of LFG generation projects. the number of facilities that operated in 2001. In 2015, these plants
produced 4106.4 GWh, using LFG technology. The LFG utilization
technology continued to advance, primarily in wealthy countries.

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Environmental Engineering Research 29(1) 230166

Fig. 1. Waste disposal method for countries of different income levels (data source: [7])

However, the introduction of the Clean Development Mechanism sanitary landfills yearly produce LFG between 5 L/kg and 40 L/kg.
programs stimulated the development of LFG utilization technology The MSW generated in major Indian cities is rich in organic matter
in underdeveloped countries as well [9]. In South Korea, the waste and has the potential to produce 15–25 L/kg of gas annually, during
sector contributes to 37.6% of the total CH4 emissions. In 2001, the course of its life (most LFG projects operate up to 30 years)
approximately 465,000 tons of the total annual CH4 emissions [13]. The gas collected from smaller landfills can be supplied
were from the waste sector [10]. to nearby enterprises for direct use in internal combustion engines,
Open dump, partially controlled, and sanitary landfills are the gas turbines, micro turbines, steam boilers, and other facilities.
most common types of landfills [11]. An open dump landfill is Furthermore, the gas collected from large landfills can be ad-
a piece of land where MSW is dumped in the open, with the vantageously used as a clean fuel for power generation [15].
area having access to fresh air. Most developing nations have The LFGcost-Web LFG Energy Cost Model [16] portrays the
open dump landfills where the MSW is carelessly thrown into overall economic analysis used to compare the costs of treatment
low-lying open regions. Based on the type of wastes, the locations of waste (waste conversion) and the levelized cost of electricity,
of landfills and treatment facilities were discussed in detail in or cost of fuel to determine the suitable layout configurations
previous studies (e.g., toxic chemicals, biohazards, household, for all ranges of LFG plants. The data on the capital, operational,
biomedical, and radioactive wastes, as well as construction, demoli- and maintenance costs were collected from literature survey and
tion, and renovation wastes) [12]. Notably, the essential parts of estimated by considering the costs of existing technological facili-
a landfill include its foundation, bottom liner, and barrier cover, ties in Ethiopia and through energy and mass balances as well.
collection systems for LFG and landfill leachate, gas flaring station,
and soil layers on the top of the landfill area, which provide minerals
and organic chemicals that can improve CH4 quality and quantity. 3. LFG Production and Characteristics
In general, LFG is removed from MSW dumps, using a blow-
er/flare system and several wells [5, 13]. Depending on the gas’s In general, LFG is a naturally occurring gas that is produced from
intended use, this system routes the gathered gas to a central the breakdown of organic matter in landfills. CO2, CH4 (the main
location, where it can be processed. The gas can be vented at component of natural gas), and trace amounts of organic chemicals
this point or utilized advantageously in various LFG energy projects. make up the majority of LFG [17]. The CO2 contained in LFG
Numerous industrialized nations, including England, China, should be sequestrated [18], and landfill leachate needs to be
Uruguay, Mexico, and the USA, harvest the gases produced from carefully treated [19]. The conversion of landfilled waste substances
landfills [3]. According to the Landfill Methane Outreach Program into LFG occurs via waste decomposition and degradation. The
(LMOP) by the United States Environmental Protection Agency time duration and stage of CH4 generation amount generally have
(US EPA), the CH4 generation potential (L0) denotes the CH4 (m3) many intrinsic and environmental determinant variables. Those
available for the site-specific variables per ton of waste. The compo- determinant variables are, temperature, moisture level, waste com-
sition of the waste, and to some extent, that of the organic matter position, and a variety of substrates for microbial degradation are
fraction of the waste are the determining factors of the CH4 gen- some of the variables that have an impact on this process. The
eration rate (k). Notably, the L0 value can be determined based LFG synthesis process involves several chemical events, including
on the carbon content of the waste, stoichiometric conversion hydrolysis, acidogenesis, methanogenesis, and maturation [20, 21].
factor, and biodegradable carbon fraction. The typical values for The overall LFG maturation cycle has five basic phases (shown
L0 range from 125 m3/t to 310 m3/t. The US EPA uses a default Fig. S1), as follows:
L0 value of 170 m3/t. According to an analysis carried out in a I. Aerobic decomposition: Aerobic decomposition involves
previous study [14], the production of LFG begins a few months bacteria that digest garbage in the presence of oxygen. O2
after the MSW is disposed and typically lasts for 10 years or longer, is used to form CO2, as heat is created. The active duration
depending on the composition of the waste and the amount and of the process can be anywhere between a few months
distribution of moisture in the MSW. In several nations, full-size and a year, depending on the circumstances. Organic waste

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Abiy Tadesse and Jechan Lee

Table 1. Characteristics of LFG components and their effect on the environment and human health (source: [22-24])
Component Volume (%) Characteristics Effects
• Methane is a gas that occurs naturally.
• It has no color or smell.
CH4 45–60 • Landfill fire primarily caused by global warming
• It is the most significant greenhouse gas (GHG) and highly
combustible landfill gas (LFG) released from landfills
• Colorless, odorless, and mildly acidic gas
• It is present in the Earth’s atmosphere at a volumetric quantity • A significant contributor to ocean acidity and
CO2 40–60
of 0.04 (400 ppm). accelerates global warming
• It is a GHG.
• Approximately 80% of the atmosphere is made up of nitrogen • Nitrogen oxides (NOx) are harmful gases that
N2 2–5 (N). cause lung damage and respiratory issues and
• It doesn't have any color and is odorless. are a major contributor to smog and acid rain
• Iron rusts and landfill fire. Excessive oxygen
• Approximately 21% of the atmosphere is made up of oxygen.
O2 0.1–1 at partial pressure can cause serious health is-
• It doesn't have any color and is odorless.
sues
• Ammonia is a colorless gas that has a strong smell. • Coughing, skin irritation, eye irritation, and
NH3 0.1–1
• The gas is irritating and corrosive. nose, throat, and respiratory-tract burning
• NMOCs can form naturally or artificially through chemical
processes.
Non-meth- • Headaches, nausea, leukemia, and carcinogenic
• NMOCs typically found in landfills include acrylonitrile,
ane organic effects.
0.01–0.6 benzene, 1,1-dichloroethane, 1,2-cis trichloroethylene, di-
compounds • Several of the gases have a strong smell and
chloromethane, carbonyl sulfide, ethyl-benzene, hexane,
(NMOCs) are highly combustible
methyl ethyl ketone, tetrachloroethylene, toluene, trichloro-
ethylene, vinyl chloride, and xylenes.
• Sulfides, which include hydrogen sulfide, dimethyl sulfide,
and mercaptans, are naturally occurring gases that are re-
• Breathing issues, poor memory, throat, eye, na-
Sulfides 0–1 sponsible for the “rotten-egg” odor of the LFG mixture.
sal irritation, and fatigue
• Even at very small amounts, sulfides can produce dis-
agreeable odor.
H2 0–0.2 • A tasteless, odorless, colorless, and highly-flammable gas • It is highly inflammable and explosive in nature
• Reduces the body’s ability to absorb oxygen,
which can lead to mortality.
CO 0–0.2 • A colorless and odorless gas • Can cause the production of smog, as well as
issues related to vision (eyesight) and motor
dexterity

is broken down into its lengthy molecular chains of complex oxygen demand (COD). The organic acids produced in phase
carbohydrates, proteins, and lipids by aerobic bacteria, II are broken down by anaerobic bacteria into acetate, anoth-
which can only exist in the presence of oxygen. CO2 is er organic acid. By consuming the CO2 and acetate, this
the main byproduct of this process. Phase 1 continues until process transforms the garbage into a more neutral environ-
there is no more oxygen left. ment, wherein the bacteria that produce CH4 can flourish.
II. Acidogenic: Anaerobic conditions are established during IV. Methanogenesis: CH4 and CO2 are produced as byproducts
this stage, resulting in the formation of organic acids, CO2, of the acetogenesis phase, and H2 is consumed. The available
H2O, and hydrogen (H2). The anaerobic conditions cause substrates have an impact on the CH4 content. The pro-
a low rate of energy release. The pH of the leachate can duction rates and composition of LFG remain largely
go below 5, as a result of acid production. The anaerobic consistent. Notably, LFG typically comprises of 50–55% CH4
bacteria transform substances produced by aerobic bacteria by volume, 45–50% CO2, and 2–5% other gases, such as
into acetic, lactic, and formic acids, as well as alcohol prod- sulfides. In phase IV, LFG is generated steadily for 20 years
ucts, such as methanol and ethanol, without the need for (on average).
oxygen. As the acids react with the moisture in the landfill V. Maturation: At this phase, the gas production decreases
and nitrogen (N) is consumed, CO2 and H2 are formed. due to substrate depletion.
III. Acetogenesis: At this stage, acids and alcohols are converted Table 1 provides an overview of each LFG component’s impact
to acetic acids, and CO2 and H2 are also formed. The acid on the environment and human health.
and leachate contents cause a noticeable rise in the chemical

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Environmental Engineering Research 29(1) 230166

4. LFG Design, Operation, and Characteristic (2)


Parameters
where QTotal is the total production of LFG.
A blower/flare (or vacuum) system and a series of wells can be Compared to natural gas, LFG is cheaper and contains nearly
used to recover the LFG from MSW dumps [13]. Depending on 50% of the calorific value (16,78–20,495 kJ/m3) of natural gas (35,406
the gas’s intended use, this system routes the gathered gas to kJ/m3) [28]. Thus, if we extract large amounts of LFG, the electricity
a central location, where it can be processed. From here, the gas production using turbine or internal combustion engines would
can either be flared or utilized profitably in an LFG energy pro- be safe and efficient. Furthermore, we can improve the LFG heating
duction plant. The production of LFG often begins a few months value by decreasing the contents of O2, N2, and CO2 in the LFG
after waste disposal and lasts for 10 years, or even longer, depending [29].
on the composition and characteristics of the waste and the avail- For LFG generation estimation, we employed the LandGEM
ability and dispersion of moisture. Full-size sanitary landfills typi- spreadsheet software. This model can estimate LFG accurately
cally produce LFG of 5–40 L/kg. and determine the amounts of CH4 and CO2 generation, with respect
Several nations base their estimates of LFG emissions primarily to opening and closure year of the landfill site. According to the
on the first-order decomposition of organic matter in MSW [25]. LandGEM software specification, the generation rate of CH4 during
LandGEM, which is a spreadsheet tool [26], has been used to annual MSW disposal can be used to calculate or estimate the
determine the total amount of CH4, CO2, and other miscellaneous annual amount of CH4. The CH4 generation rate, k, is a country
organic compounds produced through landfill waste decomposition. and site-specific value used to determine the CH4 generation poten-
First order decay equation is the most useful equation for estimating tial of MSW on specific landfill area. Thus, a higher k value indicates
LFG generation [27]. To measure the emissions from the breakdown a high volume of CH4 per kg of MSW [30]. Note that the L0 and
of landfilled waste in MSW landfills, the scholars used a first-order k values are strongly dependent on the landfill type (Table S1).
decomposition rate equation in the LandGEM model. The software The capacity of CH4 generation of the waste also depends on
offers a comparatively straightforward method for calculating the the characteristics of the MSW (Table S2). Site specific parameters
LFG emissions, as reported by various LFG initiatives around the (e.g., inert-decomposable and semi-decomposable) are generally
world. used to characterize the MSW and its potential for CH4 generation
Theoretically, the first order decay methodologies can be ex- [2]. Each waste body has its own value of CH4 generation potential.
pressed as Eq. (1) [27]: Food and yard waste are considered decomposable.
The LFG rate-of-generation value has different variables, which
determine its level of potential. For example, decomposable MSW
have higher CH4 generation potential than inert and semi decom-
(1) posable solid waste in the landfill. The waste stream, temperature,
annual precipitation (moisture), and pH value of the soil in the
where waste accepted in the year (megagram, Mg), , landfill are considered to be the general determining factors of
annual methane generation (m3/year), i = 1 󰠚 year time increment, the generation rate of LFG [2].
n = (year of the calculation) 󰠚 (initial year of waste acceptance), The required area for the landfill site and its depth, together
j = 1 󰠚 year time increment, k = methan generation rate per with the level of bed in the lower end layer of the surface, were
year, Lo = potential methane generation capacity (m3/Mg), = calculated according to Eq. (3).
section waste, Mi, accepted in ithyear.
The input data for LandGEM spreadsheet [26] can be correlated (3)
directly with the specific geographical conditions of the landfill
region. LandGEM assumes that methane production peaks quickly where Wcollected average is the average annual collected waste in the
after the first disposal of waste (after a brief delay while anaerobic year of calculation, and V is the weight of the waste after compaction,
conditions are created in the landfill). The model also predicts with the typical value being 800 kg/m3.
that when organic material decomposes, the rate of landfill methane The required thickness of the cover and mixture soil for the
generation will drop exponentially (first-order decay). desired biological decomposition was assumed to be 20% of the
The estimated CH4 content was 40–60%. The first-order decom- desired average 20-m depth of the desired solid-waste landfill
position rate equation applied in the LandGEM model could be site. As indicated by a previous study [31], the overall size of
used to calculate the emissions; however, the results may not the landfill site was estimated using the volume of the waste after
be accurate if the content was lower or higher than 40–60%. The compaction, while considering 20% additional volume on the layer
production of CO2 was highly determined or affected by the concen- and mixing soil, as shown in Eq. (4):
tration of CH4 generation.
Eq. (2) was used to determine the production of CO2 (QCO2) (4)
from the production of CH4 (QCH4) and the proportion of CH4 in
the atmosphere (PCH4) [27]: The area of the landfill site was estimated using the total landfill
volume and its depth was also calculated, using Eq. (5):

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Abiy Tadesse and Jechan Lee

Fig. 2. Comparison of CH4 generation potential between Conditions I, II, and III

eration from the total LFG generation in the closing year of the
(5)
landfill site, as per the CAA conditions. For the closing year, the
optimum ranges was based on the data acquired from ([22]). The
After carrying out the geometrical analysis of the desired landfill
overall amount of produced LFG relies on the type of waste, environ-
site, we estimated the LandGEM model parameters, based on the
ment of the site, and effectiveness of the LFG collection system.
waste amount and area.
Moreover, there are important sources that can determine the un-
certainties in the LFG generation, which are often related to the
data on the waste properties and site conditions.
5. CH4 Generation Potential Condition II: In this condition, the L0 value is similar to Condition
I conventional CAA value and k values is lower than CAA conven-
To estimate the CH4 generation potential at different CH4 generation tional condition which determines the amount of CH4 obtained.
capacities and rates, we selected the following parameters and Climatic factors, like as rainfall, have a significant impact on the
year of optimum landfill operation. For the analysis, we assumed production and properties of landfill leachate. The leachate pro-
that the annual MSW disposed in the landfill area was 100,000 duced in arid climates contain higher levels of contaminants than
tons. Furthermore, we assumed that the total landfill-site operating that produced in humid settings [22]. Based on the LMOP, in
duration was 30 years, based on the standard range from the US terms of the area-specific parameters for arid areas, we used the
EPA and LMOP. The analysis was carried out using a first order k value of 0.02/year and L0 value of 170 m3/Mg. The total LFG
decay equation and the LandGEM spreadsheet tool [26]. Notably, generation was directly proportional to the CH4 gas amount ob-
three scenarios, Conditions I, II, and III, were considered. The tained from the total collected LFG, as shown in Fig. S4. Note
three scenarios are explained as follows. that the primary sources of leachate depend on biological processes
Condition I: According to the EPA, standard values for CH4 and are impacted by the waste, rather than runoff and precipitation
generation rate (k) and L0 for the case of Controlled Air Act (CAA) (type, amount, moisture, and degree of compaction). As shown
conventional value have a huge potential of CH4 generation. in Fig. S5, the amount of CH4 utilization increased until the max-
According to the LMOP, the geographical area and MSW that imum capacity (in the closing year of the landfill area). Furthermore,
have conventional values of k (0.05/year) and L0 (170 m3/Mg) have the CH4 production increased at higher k values (as long as the
better potential of generating CH4, compared to arid and wet landfill was still accepting new waste) and decreased swiftly once
conditions. The projects in this condition have an efficient economy the landfill closed. The amount of moisture in the waste, availability
of scale, due to mass CH4 gas generation potential for power gen- of nutrients for the bacteria that produce CH4, pH, and temperature
eration due to large amount methane generation through efficient affected the k value. As shown in Fig. S5, after closing the landfill
and matured decomposition cycle. In this condition, the soil and site, the total amount of CH4 obtained from the landfill decreased
environmental condition (moisture, soil characteristics and heat) rapidly.
provides efficient generation of CH4. Condition III: In this scenario, we assumed inventory wet con-
As shown in Fig. S2, the CH4 generation potential of MSW dition had a L0 value of 96 m3/Mg and k value of 0.7/year. The
in the CAA conditions indicates and increase until the closing dissimilated organic fraction and degradable organic carbon (DOC)
year of operation, with a sharp decline in the closing year. The were transformed into LFG constantly (beginning in 2030) as in-
estimated duration for the CH4 gas generation potential was consid- dicated in Fig. S6. The total amount of CH4 gas generated in the
ered to be 30 years. In general, the k value depends on the soil inventory wet condition decreased sharply when the landfill site
characteristics and moisture (average annual rainfall level) and reached closing year of the landfill, as shown in Fig. S7. Notably,
organic contents of the MSW [32]. Fig. S3 portrays the CH4 gen- the power generated using this condition was less sustainable,

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Environmental Engineering Research 29(1) 230166

Table 2. Advantages and disadvantages of using LFG as fuel for power generation
Application Discussion Advantages Disadvantages
• This entails converting LFG to natural gas grade
• Can be used as a source of heat • Costly and necessitates the ap-
[36].
Source of natural gas in enterprises and for cooking plication of LFG processing
• The natural gas network can be used to supply
at home methods
refined LFG for domestic use
• The second most frequent method for using LFG.
• Cost and pipeline length are
Boiler system • LFG is used by boilers as a fuel source, to create • Relatively cheaper
related
steam and hot water [37]
Furnace, dryers, and • This involves using landfill gas directly as a fuel • Limitations in LFG usage, if
• Cheap and easy to install
kilns [36] used seasonally
• According to a study, raw LFG can be collected, • Due to the cost of refining, the
• Use as a fuel source for cars
Vehicle fuel cleaned, dried, and compressed to a suitable pres- raw LFG converted to motor
and trucks
sure gauge for use as car fuel [38] fuels may be expensive
• Reciprocating internal combustion engines, steam • Operational costs are rela-
turbines, organic Rankine cycles, Stirling cycle en- • Can be a source of electricity tively higher
Source of electricity
gines, molten carbonate, and solid oxide fuel cells for global energy systems • High degree of skill and tech-
are all used to generate electricity [39] nology required

in terms of the utilization of CH4 gas, at the end of the landfill 6.1. LFG Power Generation Potential
site in the closing year, with no CH4 generation potential, compared
The economics in the selection of electricity-generation LFG tech-
to that in the CAA arid and conventional conditions.
nologies mostly rely on external factors, such as the available
In Conditions I, II, and III, we observed variable CH4 generation
tax credits (e.g., renewable revenue streams and certificates on
potentials and capacities for the same landfill area. As shown
renewable energy technologies) and the price at which electricity
in Fig. 2, the CAA conventional condition provides more CH4
can be sold [22]. The power purchase agreement is a convenient
gas than that obtained in the CAA arid and inventory wet conditions.
way of receiving more revenue, with renewable portfolio standards.
From this comparison, we can deduce that the CH4 gas generation
Several systems, including internal combustion engines (ICEs),
potentials and rates at different conditions varies significantly;
turbines, micro turbines, and gradual oxidizers (GOs), have been
thus, LFG projects need to consider the characteristic parameters
used to generate energy from LFG [40]. The Brayton cycle is the
of LFG sites and the chemical properties of MSWs. According
underlying mechanism of the operation of gas and micro turbines
to the US EPA, the recommended value for L0 is 56.6–198.2 m3/Mg.
[41]. It was computed the gross power generation potential in
The value for the L0 largely depends on the type and characteristics
a particular year after predicting the yearly LFG generation [13]
of garbage present in the landfill, with the exception of arid areas,
using Eq. (6):
wherein a lack of moisture may limit the CH4 generation.

(6)
6. LFG Power Generation and Environmental
where GPGPT is the gross power generation potential, is the system
Benefits collection system (the average value is 85%), is LFG energy content
LFG is used as a power generation energy source, especially in (calorific value, typically 500 BTU/ft3), and is the heat rate of
large-scale power plants, for economic gain. The LFG with a CH4 equipment. Then, by directly considering the parasitic load, we
content of approximately 40–65% in volume can be employed determined the net potential of power generation. We assumed
to produce electricity, using internal combustion engines (1–3 that the auxiliary equipment energy loss was 6% for steam/gas
MW), turbines (greater than 5 MW), micro-turbines (30–250 kW), turbine and 2% for reciprocating combustion engine [13].
and fuel cells. However, the gas must be flared if its CH4 content The LFGcost-Web [16] was employed to estimate the average
drops below 35–40 vol% [33, 34]. generation cost of the LFG, compared to other sources, such as
Several factors, such as technical and economic characteristics, steam, hydro, diesel, geothermal, combined cycle, and turbine
as well as environmental impacts, may influence the type of energy generation. The average electricity-generation cost of LFG from
technology applied at landfill sites [35]. Due to their numerous MSW was calculated as USD 0.0604/kWh, which is higher than
advantages and high electrical efficiency, internal combustion en- that of hydro power (USD 0.0018/kWh) and steam power (USD
gines are widely utilized to produce energy from LFG. Table 2 0.0415/kWh) generation, but lower than that of geothermal (USD
compares the benefits and drawbacks of several commonly used 0.0637/kWh), combined cycle power (USD 0.0763/kWh), diesel
LFG energy systems. (USD 0.1773/kWh), and gas turbine (USD 0.1966/kWh) generation
[42].
To produce electricity or convert the form of energy, the required

7
Abiy Tadesse and Jechan Lee

Table 3. Average power-generation cost for different technologies (source: [43])


Electricity generation technology Power generation capacity capital cost (USD/kW) in 2019
Gas or oil power plant (combined cycle) 1000
Photovoltaic (fixed) 1800
Onshore wind 1600
Conventional hydropower 2752
Coal (with SOx and NOx controls) 3500– 3800
Advanced nuclear 600
Fuel cells 7200

capital cost is the basic constrain when selecting the fuel technology ical risks [39]. Gas turbines is the most commonly used technology
[43]. We compared the cost of electricity production from different in LFG-to-energy projects, after ICEs, with lower performance and
technologies in Table 3; the LFG generation (CH4 is more advanta- higher loss than ICE, based on the same thermodynamic cycles.
geous than combined power cycle with oil and fuel cells with Moreover, ICEs are easy to transport and have a flexible design
economy of scale as well). International Methane Pledge (IMP) [28]. Based on the overall cost and efficiency correlation for the
suggests national to use methane gas for power generation due targeted application of LFG, ICEs are efficient at converting LFG
to its advantage when we use in large amount. into electricity [48], attaining electrical efficiency of 30–40%. Note
LFG yields lower CO2 emissions (0.27 × 10−9 kg/kWh) than that cogeneration, also known as combined heat and power (CHP)
others energy sources, such as fuel oil (0.85 kg/kWh), gas (0.85 applications, in which the waste heat from the engine cooling
kg/kWh), and coal (1.18 kg/kWh). Furthermore, LFG has lower system is recovered to produce hot water, or from the exhaust
CO2 emission, compared to other primary fuels in the global energy to produce low-pressure steam, offers a higher efficiency.
systems [44]. ICEs are commonly used electricity-generation auxil-
iary components for LFG projects. They have high efficiency and 6.2. Cost of Power Generation from LFG
low cost, when installed directly in the gas output of the LFG The price of producing electricity from CH4 gas depends on several
layout [22]. In the USA, more than two third (>66%) of landfills variables, e.g., whether a gas recovery system is present or not,
generate electricity using this technology. ICEs are highly efficient the size of the waste, and the conversion technology used. In
than gas turbine and can convert LFG (50% CH4) to electricity addition to the equipment costs, soft expenditures and grid con-
effectively. nectivity charges are frequently included in the project cost compo-
The steam and gas turbines applied for municipality LFG elec- nents [32]. In addition to these expenses, the collection system
tricity production use compressed gas and heat; the gas expands and generation equipment also have operation and maintenance
in the turbine then, rotates the generator, to produce electricity. costs.
Similar to reciprocating engines, gas turbines have a lifetime of The price of producing 1-kWh electricity can vary from as little
25 years and steam turbines have a lifetime of 50 years [45]. For as USD 3.4 to as much as USD 10. Where a collection infrastructure
large LFG-to-energy plants, with capacities more than 1 MW, tur- is in place, energy production is typically significantly more
bines are often employed. Micro turbines are ideal for small applica- cost-effective. Do reduce the cost of systems that convert CH4
tions and operate at low combustion temperatures and compression to energy, it is important to include government incentives, as
ratios [41]. Micro turbines have an electric yield of about 30%, such incentives can directly affect LFG utilization and thus, global
with an operational availability of up to 95% and the ability to and regional GHG emissions. According to the amount of CH4
use LFG with the CH4 concentration exceeding 35%; nonetheless, gas collected in each year, there is economy of scale (under conven-
they require expensive and substantial maintenance services every tional CAA condition there is incremental generation of methane
eight years for continuous operation [42]. gas until the closing year of the landfill), and additional reciprocat-
Gradual oxidizers (GOs) are recently developed appliances that ing engines are required each year on the existed connecting units
function at lower temperatures. They have 95% operational avail- assembled (additional ICs, gas turbines, and boilers installed in
ability, 29% electric energy production, and can function with the initial years of energy generation) for energy generation [49].
LFG containing CH4 at concentrations as low as 1.5%. Notably, The electricity generation from LFG gas can increase each year,
GOs need substantial and expensive servicing every 9 years, for due to population growth and the resulting increase in waste
continuous operation [45, 46]. Without a doubt, GOs seem to be generation. Therefore, the total annual cost for each income-level
the only practical replacements for LFGs (i.e., LFG with low CH4 of the population and the amount of CH4 gas from the collected
concentration that cannot be used with traditional technologies). MSW will vary significantly.
With the application of controlled heat pump, it is possible to
achieve a higher efficiency, using the exhaust heat to heat water, 6.3. Environmental Benefits of LFG Power Generation
and the low-pressure steam from the engine cooling system heat
With an atmospheric life of only approximately 12 years, CH4
exchanger can also be used to produce electricity [47].
is a powerful GHG (more than 25 times stronger than carbon dioxide
ICEs may be viable for LFG-to-electricity generation, due to
over a 100-year span). Thus, one of the best strategies to limit
its low capital cost compared to gas turbine and boiler. This technol-
human influence on global climate change is to reduce the CH4
ogy comprises of a consolidated advantage, with minimum econom-

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Environmental Engineering Research 29(1) 230166

emissions from MSW landfills. Also, as CH4 is produced in all produce the same amount of energy as that produced from LFG.
landfills, there is higher potential in reducing the CH4 emissions Gradual LFG use and collection at landfills can enhance regional
by flaring or collecting the LFG for energy production. air quality which can allow the global targeted protocols and agree-
In general, the LFG from MSW landfill is collected using a ments to maintain the global temperature.
connection of blowers and series of walls in general vacuum Low amounts of NMOCs in LFG are eliminated or transformed
systems. The gas collected through this system and accumulated during burning, thus, lowering the potential health hazards asso-
in the central unit point undergoes treatment according to the ciated with LFG. If fossil-fuel combustion at utility power plants
final target of LFG utilization. In most cases, LFG projects use is avoided, there will be less pollution; thus, the emissions of
this gas for direct flaring, for electricity or non-electricity generating SO2 (a major contributor to acid rain), particulate matter (a respira-
units [50]. The environmental benefits of LFG can be calculated tory health concern), nitrogen oxides (which can contribute to
separately for the projects that consider and do not consider elec- local ozone and smog formation), and trace hazardous air pollu-
tricity generation, as follows: tants, which are released into the air from the power plants, can
CH4 collected and destroyed: The total amount of CH4 collected be reduced.
each year (m3/Year), which is either burned by flaring or used
in the LFG energy project, can be calculated using Eq. (7):
7. Summary and Outlook
=
In general, LFG is a result of the breaking down of organic waste
(7) in landfills. LFG consists of a minor quantity of non- CH4 chemical
molecules, 50% CO2, and 50% CH4 (the main component of natural
Direct CH4 reduction: The total amount of CH4 collected each gas). CH4, which is a powerful GHG, traps the heat in the atmosphere
year, measured in million metric tons of carbon dioxide equivalents for up to 28–36 times longer than CO2. The implication of CH4
per year, (MMTCO2E/Year), is either burned by flaring or used generation potential is dependent on soil characteristics, moisture,
in the LFG energy project and can be calculated using Eq. (8): decomposable portion of MSW in the landfill, temperature, and
CH4 generation potential and capacity in arid, conventional, and
wet areas. In CAA, conventional landfill (Condition I) operation
= generates massive amounts of CH4 gas, compared to Conditions
II and III in arid and wet conditions, with variable k (CH4 generating
potential) and L0 (CH4 generation capacity) of each geographical
(8) condition.
The LFG market share is expected to reach approximately USD
where, is methane gas global warming potential which is directly 3178.3 million, projected to register a compound annual growth
reduced with the volume utilized and this direct methane reduction rate of 8.1% from 2022 to 2030. With the concomitant loss of
have an indirect methane reduction advantage by energy sub- production, significant unanticipated expenses, and, in some cir-
stitution through the energy system (fossil fuel or biomass). cumstances, loss of life, the occurrence of catastrophic operational
CH4 utilized: This is the amount of CH4 that the LFG energy failures resulting from garbage slides, long-lasting fires, and flood-
project or other end goals use in one million metric tons per year, ing conditions could be less likely with the use of this strategy.
(MMTCO2E/Year), which can be calculated using Eq. (9): Notably, LFG generation has a higher operating and maintenance
cost than other feedstock types. Because of the high capital and
operational expenses associated with LFG generation, we can an-
ticipate a decline in the market’s demand for LFG throughout
the projected period.
The future landfill might be a better instrumented structure
(9) that updates the operator on its performance and status in real-time
monitoring and optimization features. This strategy may assist
where GWP of CH4 in utilized methane is global warming potential in lowering the likelihood of significant failures, loss of pro-
through direct emission in the open landfill area to the environment. ductivity, and fatalities. Furthermore, LFG can be used as a low-car-
CH4 utilized for energy or other end target is calculated through bon and environment-friendly substitute for traditional fossil fuels.
actual gas utilized in the project and its amount of direct relieved Upon combustion, LFG creates bioenergy, which is a clean fuel
effect on the environment. for energy production. In the future, the generation of bioenergy
Depending on the efficiency and design of the system, during from biomass and LFG will most likely increase with the energy
its operational lifetime, an LFG energy project will likely capture demand, which expand the market. Therefore, governments and
between 60% and 90% of the CH4 produced by a landfill. As decision makers must encourage the use of CH4 emissions from
the gas is burned to produce electricity or heat, the CH4 collected landfills for power generation because it is a renewable source
will be converted to water and carbon dioxide [24]. Furthermore, of energy and can reduce the emissions of GHGs.
non-renewable resources (such as coal, oil, and natural gas) can

9
Abiy Tadesse and Jechan Lee

Conflict-of-Interest Statement 1-54.


13. Jaramillo P, Matthews HS. Landfill-gas-to-energy projects: anal-
ysis of net private and social benefits. Environ. Sci. Technol.
The authors declare that they have no conflict of interest.
2005;39:7365-7373. https://doi.org/10.1021/es050633j.
14. Wikramanayake ED, Ozkan O, Bahadur V. Landfill gas-powered
atmospheric water harvesting for oilfield operations in the
Author contributions United States. Energy 2017;138:647-658. https://doi.org/10.1016/
j.energy.2017.07.062.
A.T. (Product Engineer) collected and analyzed data and wrote
15. Sinha S. What India needs: landfill gas recovery and its
the manuscript. J.L. (Associate Professor) wrote and revised the
utilization. Int. J. Eng. Res. Technol. 2013;2:1981-1984. https://
manuscript. doi.org/10.17577/ijertv2is80817.
16. LFGcost-Web — landfill gas energy cost model (ver. 3.5)
[Internet]. 2021 [cited 23 February 2023]. Available from:
References https://www.epa.gov/lmop/lfgcost-web-landfill-gas-energy-cost-
model#three.
1. Marshall RE, Farahbakhsh K. Systems approaches to integrated 17. Gour AA, Singh SK. Solid waste management in India: a
solid waste management in developing countries. Waste state-of-the-art review. Environ. Eng. Res. 2023;28:220249-0.
Manage. 2013;33:988-1003. https://doi.org/10.1016/j.wasman. https://doi.org/10.4491/eer.2022.249.
2012.12.023. 18. Ko D. Comparison of carbon molecular sieve and zeolite 5A
2. Ebert EE, Gallus WA. Toward better understanding of the con- for CO2 sequestration from CH4/CO2 mixture gas using vacuum
tiguous rain area (CRA) method for spatial forecast verification. pressure swing adsorption. Korean J. Chem. Eng. 2021;38:
Weather Forecast. 2009;24:1401-1415. https://doi.org/10.1175/ 1043-1051. https://doi.org/10.1007/s11814-021-0771-y.
2009WAF2222252.1. 19. Ghanbari F, Khatebasreh M, Mahdavianpour M et al. Evaluation
3. Mokhtari M, Ebrahimi AA, Rezaeinia S. Prediction of green- of peroxymonosulfate/O3/UV process on a real polluted water
house gas emissions in municipal solid waste landfills using with landfill leachate: feasibility and comparative study.
LandGEM and IPCC methods in Yazd, Iran. J. Environ. Health Korean J. Chem. Eng. 2021;38:1416-1424. https://doi.org/10.
Sustain. Develop. 2020;5:1145-1154. https://doi.org/10.18502/ 1007/s11814-021-0782-8.
jehsd.v5i4.4964. 20. Popov V, Power H. Landfill emission of gases into the atmos-
4. Han J, Byun J, Kwon O, Lee J. Climate variability and food phere: boundary element analysis. WIT Press; 1999.
waste treatment: analysis for bioenergy sustainability. Renew. 21. White J, Robinson J, Ren Q. Modelling the biochemical degrada-
Sust. Energ. Rev. 2022;160:112336. https://doi.org/10.1016/ tion of solid waste in landfills. Waste Manage. 2004;24:227-240.
j.rser.2022.112336. https://doi.org/10.1016/j.wasman.2003.11.009.
5. Urase T, Okumura H, Panyosaranya S, Inamura A. Emission 22. LFG energy project development handbook. Washington, DC,
of volatile organic compounds from solid waste disposal sites USA: United States Environmental Protection Agency; 2021.
and importance of heat management. Waste Manage. Res. 23. Schulte-Uebbing L, Hansen G, Hernández AM, Winter M.
2008;26:534-538. https://doi.org/10.1177/0734242x07084321. Chapter scientists in the IPCC AR5—experience and lessons
6. Global Methane Initiative (GMI) [Internet]. 2021 [cited 23 learned. Curr. Opin. Environ. Sustain. 2015;14:250-256.
February 2023]. Available from: https://www. globalmethane.org. https://doi.org/10.1016/j.cosust.2015.06.012.
7. Kaza S, Yao L, Bhada-Tata P, van Woerden F. What a waste 24. 2006 IPCC guidelines for national greenhouse gas inventories
2.0: a global snapshot of solid waste management to 2050. - volume 5. waste. Institute for Global Environmental Strategies.
In: Urban Development Series. Washington, DC, USA: World Hayama, Japan: Intergovernmental Panel on Climate Change;
Bank Group; 2018. 2006.
8. Hoornweg D, Lam P. Solid waste management in China: issues 25. Aghdam EF, Fredenslund AM, Chanton J, Kjeldsen P, Scheutz
and options. Waste: The Social Context 2005:261-271. C. Determination of gas recovery efficiency at two Danish land-
9. Karekezi S. Poverty and energy in Africa—a brief review. Energy fills by performing downwind methane measurements and sta-
Policy 2002;30:915-919. https://doi.org/10.1016/s0301-4215 ble carbon isotopic analysis. Waste Manage. 2018;73:220-229.
(02)00047-2. https://doi.org/10.1016/j.wasman.2017.11.049.
10. Larney C, Heil M, Ha G-A. Case studies from the climate technol- 26. US EPA, Landfill gas emissions model (LandGEM) (ver. 3.03).
ogy partnership: landfill gas projects in South Korea and lessons 2020, https://www.epa.gov/catc/clean-air-technology-center-
learned. Golden, CO, USA: National Renewable Energy products#software (accessed on Feb. 23, 2023).
Laboratory; 2006. 27. Scharff H, Jacobs J. Applying guidance for methane emission
11. Narayana T. Municipal solid waste management in India: from estimation for landfills. Waste Manage. 2006;26:417-429.
waste disposal to recovery of resources? Waste Manage. 2009; https://doi.org/10.1016/j.wasman.2005.11.015.
29:1163-1166. https://doi.org/10.1016/j.wasman.2008.06.038. 28. Bade Shrestha SO, Narayanan G. Landfill gas with hydrogen
12. Haeming H, Bretthauer F, Heyer K-U, Stegmann R, Quicker addition – a fuel for SI engines. Fuel 2008;87:3616-3626.
P. Waste, 8. landfilling and deposition. In: Ullmann's https://doi.org/10.1016/j.fuel.2008.06.019.
Encyclopedia of Industrial Chemistry. Wiley-VCH; 2021. p. 29. Wang Y, Levis JW, Barlaz MA. Life-cycle assessment of a regu-

10
Environmental Engineering Research 29(1) 230166

latory compliant U.S. municipal solid waste landfill. Environ. 40. Manasaki V, Palogos I, Chourdakis I, Tsafantakis K, Gikas P.
Sci. Technol. 2021;55:13583-13592. https://doi.org/10.1021/acs.est. Techno-economic assessment of landfill gas (LFG) to electric
1c02526. energy: selection of the optimal technology through field-study
30. Njoku PO, Odiyo JO, Durowoju OS, Edokpayi JN. A review and model simulation. Chemosphere 2021;269:128688. https://
of landfill gas generation and utilisation in Africa. Open Environ. doi.org/10.1016/j.chemosphere.2020.128688.
Sci. 2018;10:1-15. https://doi.org/10.2174/1876325101810010001. 41. Catalog of CHP technologies: section 5. technology character-
31. Hatzichristos T, Giaoutzi M. Landfill siting using GIS, fuzzy ization - microturbines. Washington, DC, USA: United States
logic and the Delphi method. Int. J. Environ. Technol. Manage. Environmental Protection Agency; 2015.
2006;6:218-231. https://doi.org/10.1504/ijetm.2006.008263. 42. Darrow K, Tidball R, Wang J, Hampson A, Catalog of CHP
32. SCS Engineers, Economic and financial aspects of landfill gas technologies. Washington, DC, USA: United States Environmental
to energy project development in California. Sacramento, CA, Protection Agency; 2017.
USA: California Energy Commission; 2002. 43. Vimmerstedt L, Akar S, Mirletz B et al. Annual technology
33. Lombardi L, Carnevale EA. Analysis of an innovative process baseline: the 2021 electricity update. Golden, CO, USA:
for landfill gas quality improvement. Energy 2016;109:1107- National Renewable Energy Laboratory; 2021.
1117. https://doi.org/10.1016/j.energy.2016.05.071. 44. Swaminathan R, Johannes I. Power generation from landfill
34. Aguilar-Virgen Q, Taboada-González P, Ojeda-Benítez S, gas and a case study. Int. J. Energy Power Eng. 2020;9:81-85.
Cruz-Sotelo S. Power generation with biogas from municipal https://doi.org/10.11648/j.ijepe.20200905.12.
solid waste: prediction of gas generation with in situ parameters. 45. Hansen TA, Ringler E. Demonstration and verification of a
Renew. Sust. Energ. Rev. 2014;30:412-419. https://doi.org/ turbine power generation system utilizing renewable fuel: land-
10.1016/j.rser.2013.10.014. fill gas. Durham, NC, USA: Southern Research Institute; 2013.
35. Colpan CO, Dincer I, Hamdullahpur F. The reduction of green- 46. Ener-Core [Internet]. 2018 [cited 23 February 2023]. Available
house gas emissions using various thermal systems in a landfill from: https://www.ener-core.com.
site. Int. J. Glob. Warm. 2009;1:89-105. https://doi.org/10.1504/ 47. Barisano D, Canneto G, Nanna F et al. Steam/oxygen biomass
ijgw.2009.027083. gasification at pilot scale in an internally circulating bubbling
36. Hans C. Energy recovery from landfill gas in Denmark and fluidized bed reactor. Fuel Process. Technol. 2016;141:74-81.
worldwide. Corpus ID: 52888272; 2002. https://doi.org/10.1016/j.fuproc.2015.06.008.
37. International best practices guide for landfill gas energy 48. Kohn MP, Lee J, Basinger ML, Castaldi MJ. Performance of
projects. Washington, DC, USA: Global Methane Initiative, an internal combustion engine operating on landfill gas and
International Solid Waste Association, & United States the effect of syngas addition. Ind. Eng. Chem. Res. 2011;50:
Environmental Protection Agency; 2012. 3570-3579. https://doi.org/10.1021/ie101937s.
38. Borray E, Smith G, Deane G. Process and apparatus for purifica- 49. Chen C. Is landfill gas green energy?. New York, NY, USA:
tion and compression of raw landfill gas for vehicle fuel. US Natural Resources Defense Council; 2003.
Patent No. 5,727,903; 1998. 50. Hajinezhad A, Ziaee Halimehjani E. Study landfill development
39. Bove R, Lunghi P. Electric power generation from landfill gas in Rasht And latex management in order to reduce pollution
using traditional and innovative technologies. Energy Convers. Anzali Lagoon. Iranian J. Ecohydrol. 2015;2:11-22. https://do-
Manage. 2006;47:1391-1401. https://doi.org/10.1016/j.enconman. i.org/10.22059/ije.2015.55125.
2005.08.017.

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