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Monoblock Fuel Retention
Monoblock Fuel Retention
Monoblock Fuel Retention
E-mail: rdelaportemathurin@gmail.com
Abstract
The influence of the input power (IP), puffing rate and neutral pressure on the fuel (hydrogen
isotopes) inventory of the WEST and ITER divertors is investigated. For the chosen range of
parameters (relatively low temperature at the strike points), the inventory of the WEST
divertor evolves as the power 0.2 of the puffing rate and as the power 0.3 of the IP. The
inventory at the strike points is highly dominated by ions whereas it is dominated by neutrals
in the private zone. Increasing the fuelling rate increases the retention in the private zone and
decreases slightly the retention at the strike points. Increasing the IP increases the inventory at
the strike points and does not affect much the inventory at the private flux region. The
inventory of the ITER divertor is not strongly dependent on the divertor neutral pressure. The
inventory increases from 0 Pa to 7 Pa and then decreases slightly from 7 Pa to 10 Pa. After
107 s of continuous exposure, the maximum inventory in the ITER divertor was found to be
14 g. The inventory is not maximum at the strike points due to the high surface temperature of
the monoblocks in this region. The maximum accumulation of H in the ITER divertor is below
5 mg per 400 s discharge and below 2 mg per 400 s discharge after 200 discharges.
Keywords: hydrogen transport, divertor, SolEdge3X-EIRENE, SOLPS, FESTIM
(Some figures may appear in colour only in the online journal)
Figure 1. Geometry of WEST and ITER divertors showing the divertors in red, the plasma seperatrix and the location of the strike points.
IVT and OVT stand for inner and outer vertical target, respectively. For WEST, the pump position (in blue) is under the baffle.
Figure 2. Evolution of the implantation range and the reflection coefficient as a function of incident energy E and angle of incidence
computed from SRIM simulations.
by experimental work to determine key properties of fusion In a previous study [4], the finite element code FESTIM
materials. H transport in monoblocks has been studied in 1D [5, 9] was employed to simulate H isotopes transport in ITER-
[8]. However, it was shown in [9] that the 2D edge effects had like monoblocks with the geometry given in [11] coupled to
to be considered to have a better estimate of the H retention in heat transfer. A novel method was developed to rapidly esti-
the actively cooled divertor monoblocks. A recent major effort mate the H inventory in the whole ITER divertor from plasma
has been devoted to perform multi-dimensional simulations [4, code results without having to run additional finite element
5, 9, 10]. simulation. Instead, a behaviour law relying on a data base
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Nucl. Fusion 61 (2021) 126001 R. Delaporte-Mathurin et al
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Nucl. Fusion 61 (2021) 126001 R. Delaporte-Mathurin et al
Figure 4. Distribution of heat flux, particle flux and particle energy along the WEST divertor computed by SOLEDGE3X-EIRENE with IPs
varying from 0.49 MW to 2.0 MW with a puffing rate of 2.5 × 1021 molecule s−1 .
Figure 5. Distribution of surface temperature T surface , surface concentration csurface and inventory along the WEST divertor with IPs varying
from 0.49 MW to 2.0 MW with a puffing rate of 2.5 × 1021 molecule s−1 .
temperature T surface and surface hydrogen concentration csurface The relation between the heat flux ϕheat and the surface tem-
by equations (1) and (2). perature T surface (see equation (1)) has been obtained from heat
Tsurface = 1.1 × 10−4ϕheat + Tcoolant , (1) transfer simulations of ITER monoblocks [4].
The relation between the surface concentration of mobile
where ϕheat is the surface heat flux in W m−2 and T coolant = H csurface (m−3), the particle flux ϕi∈{ions,atoms} (m−2 s−1 ) and
323 K is the coolant temperature. T surface (K) is given by:
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Nucl. Fusion 61 (2021) 126001 R. Delaporte-Mathurin et al
Figure 6. H inventory at the strike points and in the private zone as a function of the SOL IP with a puffing rate of 2.5 × 1021 molecule s−1 .
Figure 7. Evolution of the WEST divertor inventory as a function of SOL IP for several puffing rates.
Rp,atoms ϕatoms (see figure 2) and computed with SRIM [20], ϕi are the parti-
csurface = (1 − ratoms ) + (2)
D(Tsurface ) cles fluxes in m−2 s−1 and D(T ) is the H diffusion coefficient
Rp,ions ϕions in m2 s−1 . The implantation ranges and reflection coefficients
(1 − rions ) , were calculated with deuterium ions (mass of 2.014 and hydro-
D(Tsurface )
gen species) on a W target. The deviation between protium,
where the reflection coefficients ri and implantation depths Rp,i deuterium and tritium was below the angstrom for the energy
in m depend on the particle energy and angle of incidence range used in this work.
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Nucl. Fusion 61 (2021) 126001 R. Delaporte-Mathurin et al
Figure 8. Distribution of heat flux, particle flux and particle energy along the WEST divertor computed by SOLEDGE3X-EIRENE with a
puffing rate varying from 4.4 × 1020 s−1 to 4.7 × 1021 s−1 with 0.45 MW of IP.
Figure 9. Distribution of surface temperature T surface , surface concentration csurface and inventory along the WEST divertor with a puffing
rate varying from 4.4 × 1020 s−1 to 4.7 × 1021 s−1 with 0.45 MW of IP.
According to the behaviour law obtained in [4], the tempo- The relation between the implantation range Rp and the inci-
ral evolution of the H inventory along the divertors can be esti- dent energy and angle of incidence can be obtained from SRIM
mated from the surface concentration of mobile H and surface [20] results (see figure 2(a)). It was found that the angle of inci-
temperature (see figure 3). dence had low influence on the implantation range. Rp can then
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Nucl. Fusion 61 (2021) 126001 R. Delaporte-Mathurin et al
Figure 10. H retention in WEST at the strike points and in the private zone as a function of puffing rate with 0.45 MW of SOL IP.
Figure 11. Evolution of the WEST divertor inventory as a function of puffing rate.
be expressed (in m) as a function of the incident energy only cient varies from around 0.5 at 0◦ to 0.8 at 80◦ (see figure 2(b)).
(see equation (3)). According to [18], the incident angles for ions and atoms were
assumed to be 60◦ and 45◦, respectively. It should be noted that
Rp = 1.9 × 10−10E0.59 , (3)
since SRIM is based on the binary collision approximation,
where E is the incident energy in eV. values around 10 eV might not be fully valid.
The evolution of the reflection coefficient r can also be esti- The source-code of the tool described in this work (divHre-
mated with SRIM for a perfect surface. The reflection coeffi- tention) is under version control and openly available via
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Nucl. Fusion 61 (2021) 126001 R. Delaporte-Mathurin et al
Figure 12. Heat flux, particle flux and particle energy along ITER divertor computed by SOLPS with neutral pressures varying from 2 Pa to
11 Pa.
Figure 13. Surface temperature, surface concentration and inventory along ITER divertor with neutral pressures varying from 2 Pa to 11 Pa.
Area corresponds to the 95% confidence interval.
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Nucl. Fusion 61 (2021) 126001 R. Delaporte-Mathurin et al
Figure 14. Hydrogen inventory in the ITER divertor as a function of neutral pressure after 107 s of exposure (approximately 25 000
discharges).
plasma facing surface, it was shown in [15] that the evolution The total inventory in the WEST divertor is computed as
of the monoblock inventory with the fluence was not affected. follows:
Moreover, it can be shown that the divertors inventories evolve invdivertor = NPFU · invPFU (x) dx, (4)
with a power law dependence of time.
where N PFU = 480 is the number of plasma facing units (PFU)
3.1. WEST in WEST, invPFU is the inventory per unit thickness in H m−1
Two parametric studies were performed on the WEST diver- (see figure 5) and x the distance along the target in m.
tor varying the input power (IP) and the puffing rate. In this At the strike points, the retention is dominated by the
section, the inner and outer strike points are located at 0.2 m ion flux whereas neutrals are dominant in the private zone
and 0.36 m respectively (see figure 1). (see figure 6(b)). The contribution of ions at the strike points
increased with the IP but remained approximately constant in
3.1.1. Power scan. The scrape off layer IP was varied the private zone.
between 0.45 MW and 2.0 MW. Two puffing rate values were The divertor inventory increased with the IP (see figure 7)
used: 2.5 × 1021 molecule s−1 and 4.4 × 1021 molecule s−1 . and evolved as the power 0.3 of the IP. The maximum divertor
The heat flux at the strike points increased with the IP from inventory was 8.8 × 1023 H at 2.0 MW of scrape off layer IP.
0.1 MW m−2 to 10 MW m−2 (see figure 4). The incident flux This value of IP is still relatively low. Increasing the puffing
of particle was not significantly affected by the IP variation. rate lead to an increase in the inventory. This will be explained
The particle incident energy however increased up to 100 eV more thoroughly in section 3.1.2.
at the strike points. The divertor inventory was found to increase as a square
The maximum retention was found to be located at the root of time.
strike points (see figure 5). The inventory at the outer strike
point was higher than at the inner strike point. The retention 3.1.2. Density scan. A parametric study on the puffing
at the strike points was found to increase with the SOL IP rate was performed. The puffing rate was varied between
whereas it slightly decreased in the private zone (see figure 4.4 × 1020 molecule s−1 and 4.7 × 1021 molecule s−1 . The
6(a)). This was explained by an attachment of the plasma scrape off layer IP was fixed to 0.45 MW.
decreasing the particle flux in the private zone. Since the sur- The heat flux was found to increase with the puffing rate
face temperature is constant, this leads to a decrease in the in the private region, whereas it decreases at the strike points
surface concentration of hydrogen as seen on figure 5. On the (see figure 8). The particle flux on the other hand, increases
other hand, the increasing temperature at the strike points only with the puffing rate in every region, especially for the neutral
enhanced the diffusion process while remaining low enough particles. The incident energy of particles decreased with the
so that hydrogen could get trapped. puffing rate.
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Nucl. Fusion 61 (2021) 126001 R. Delaporte-Mathurin et al
Figure 15. H retention at the strike points (defined as maximum temperature) as a function of the divertor neutral pressure.
The maximum retention was again located at the strike energy was found to be at least one order of magnitude lower
points for all puffing rates values (see figure 9). The inven- than that of the ions.
tory at the outer strike point was higher than at the inner strike Peak temperatures at strike points increased when decreas-
point. The inventory in the private zone was found to increase ing the divertor neutral pressure (see figure 13). The peak tem-
with the puffing rate whereas it was almost constant at the perature at the outer strike point reached 2000 K at 2 Pa and
strike points (see figure 10(a)). As for the power scan, the more than 1000 K at the inner strike point which is in accor-
ions contribution to the inventory is rather low in the private dance with the results obtained by Pitts et al [19]. This is con-
zone (see figure 10(b)). Moreover, the contribution of ions sistent with the higher heat flux observed at the outer strike
decreases rapidly at the strike points and represents only half point (see figure 12). The inventory in the whole divertor is
of the surface concentration at 4 × 1021 molecule s−1 . computed as follow:
The inventory in the whole WEST divertor is computed
from equation (4). As for the power scan, the divertor inven-
invdivertor = Ncassettes · NPFU−IVT · invIVT (x) dx
tory increased as the power 0.2 of the puffing rate (see figure
11). The maximum inventory was found to be 5 × 1023 H at (5)
4.7 × 1021 molecule s−1 . + NPFU−OVT · invOVT (x) dx
The divertor inventory was found to increase as a square
root of time.
with N cassettes = 54 the number of cassettes, N PFU−IVT = 16
and N PFU−OVT = 22 the number of plasma facing units per
3.2. ITER
cassette in the inner and outer targets respectively, invIVT and
The heat flux was maximum at the outer strike point reaching invOVT the hydrogen inventory profile along the inner and outer
20 MW m−2 (see figure 12). The neutral particles incident targets respectively and x the distance along the targets.
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Nucl. Fusion 61 (2021) 126001 R. Delaporte-Mathurin et al
Figure 16. Evolution of the H inventory of the ITER divertor with the number of 400 s discharges.
The inventory in the outer target was found to be nearly For all divertor neutral pressures, the temporal evolution of
twice that of the inner target. This is greatly explained by the divertor inventory is approximately the same (see figure
the larger number of plasma facing units in the outer target 16). The additional inventory per 400 s discharge was found to
and therefore a greater exposed surface. The global inventory decrease with time. Past 300 discharges, the additional inven-
increases with the divertor neutral pressure and a slight roll- tory per discharge decreases with the number of discharges.
over is observed above 7 Pa (see figure 14). This roll-over is The maximum is around 5 mg/discharge between 30 and 100
consistent with the results obtained in [19]. It is mainly due to discharges.
the surface temperature variations near the outer strike point
inducing variation in the near strike point inventory (see figure 4. Conclusion
13(b)).
The inventory increase was found to be more important in Fuel retention of both the WEST and the ITER divertors was
the outer vertical target. This was explained by the fact that studied. The technique developed in [4] has been applied
the plasma is more detached at the inner target. Therefore the to various divertor exposures. The influence of key control
surface temperature reduction is more significant in the outer parameters such as the scrape off layer IP, the puffing rate and
vertical target and the surface concentration is increased (see the divertor neutral pressure was investigated. This technique
figure 13(b)). can be applied to any reactor using the monoblock concept to
The maximum inventory was found at around 7 Pa and was shield the divertor/limiter. However, some reactors like JET do
approximately 14 g of H which is well below the ITER in- not use the monoblock design and this technique is therefore
vessel safety limit of tritium (1 kg), especially considering only not applicable.
half of this quantity will be tritium. This is especially true con- It was shown that the inventory in WEST increases as the
sidering that this was for a very long exposure time of 107 s power 0.3 of the SOL IP and as the power 0.2 of the puff-
which corresponds to 25 000 pulses of 400 s. ing rate. The inventory in the ITER divertor was found to first
The inventory at the inner and outer strike points globally increase with the neutral pressure up to 7 Pa then decrease,
increases with the divertor neutral pressure (see figure 15(a)). though the variation was smoother. The inventory in the outer
The contribution of ions to the surface concentration at the vertical target of the ITER divertor is twice that of the inner
inner strike point is around 50% and tends to decrease with vertical target. These results were in good agreement with the
increasing neutral pressure (see figure 15(b)). At low diver- observations made in [19].
tor neutral pressure, the contribution of ions at the outer strike However, it should be noted that for these simulations both
point is around 90% and tends to decrease with increasing neu- machines do not operate in the same regime. While WEST
tral pressure. This can be explained by the fact that in both operates at low SOL IP, ITER operates at high IP with a high
inner and outer targets, the integrated flux of ions decreases recycling divertor. These differences in the operation regime
with increasing neutral pressure whereas the integrated flux can explain different trends.
of atoms increases, leading to a greater proportion of neutral The underlying monoblock model has also a few limita-
particles. tions, as detailed in [4]. First, the set of trapping parameters
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Nucl. Fusion 61 (2021) 126001 R. Delaporte-Mathurin et al
that was used may not be relevant for every region of the at the ITER divertor vertical targets Plasma Phys. Control.
divertor. These properties can however be estimated from Fusion 60 044018
experimental work [23, 24]. The accuracy of the results could [2] Grisolia C. 1999 Plasma wall interaction during long
pulse operation in Tore Supra J. Nucl. Mater. 266–269
therefore be improved by running a new batch of FESTIM 146–52
monoblock simulations with different trapping parameters like [3] Dwivedi S.K. and Vishwakarma M. 2018 Hydrogen embrittle-
neutron-induced traps. The impact of edge localised modes is ment in different materials: a review Int. J. Hydrog. Energy
assumed to be negligible for very long exposure times [25]. 43 21603–16
Then, this model does not take into account retention in Be [4] Delaporte-Mathurin R., Hodille E., Mougenot J.,
De Temmerman G., Charles Y. and Grisolia C. 2020
co-deposited layers. These are expected to be the main driver Parametric study of hydrogenic inventory in the ITER
for H retention in ITER [26]. Estimations of the retention rate divertor based on machine learning Sci. Rep. 10
in these layers range from 100 mg to 300 mg per 400 s shot 17798
[27]. The retention rate computed in this study is much lower [5] Delaporte-Mathurin R., Hodille E.A., Mougenot J., Charles Y.,
and remains below 5 mg per discharge. However, this work is De Temmerman G., Leblond F. and Grisolia C. 2021 Influ-
still relevant for full-W environments like WEST and DEMO. ence of interface conditions on hydrogen transport studies
Nucl. Fusion 61 036038
Additionally, the FESTIM results used in this model are [6] Denis J. et al 2019 Dynamic modelling of local fuel inventory
2D simulations. It could be argued that 3D edge effects due and desorption in the whole tokamak vacuum vessel for auto-
to desorption from the gaps between the monoblocks would consistent plasma-wall interaction simulations Nucl. Mater.
decrease the estimated inventory. The current assumption is Energy 19 550–7
therefore conservative and is a worst-case scenario. However, [7] Dark J., Delaporte-Mathurin R., Charles Y., Hodille E.A.,
Grisolia C. and Mougenot J. 2021 Influence of hydrogen trap-
the influence of 3D edge effects on the monoblock inventory
ping on WCLL breeding blanket performances Nucl. Fusion
and outgassing fluxes will be investigated in future work. https://doi.org/10.1088/1741-4326/ac28b0
[8] Hodille E.A., Bernard E., Markelj S., Mougenot J., Becquart
Acknowledgments C.S., Bisson R. and Grisolia C. 2017 Estimation of the
tritium retention in ITER tungsten divertor target using
macroscopic rate equations simulations Phys. Scr. T170
The project leading to this publication has received funding 014033
from Excellence Initiative of Aix-Marseille Univer- [9] Delaporte-Mathurin R., Hodille E.A., Mougenot J., Charles Y.
sity—A∗ Midex, a French ‘Investissements d’Avenir’ and Grisolia C. 2019 Finite element analysis of hydrogen
programme as well as from the French National Research retention in ITER plasma facing components using FESTIM
Agency (Grant No. ANR-18-CE05-0012). This work has Nucl. Mater. Energy 21 100709
[10] Benannoune S., Charles Y., Mougenot J., Gaspérini M. and
been carried out within the framework of the EUROfusion De Temmerman G. 2020 Multidimensional finite-element
Consortium and has received funding from the Euratom simulations of the diffusion and trapping of hydrogen
research and training programme 2014–2018 and 2019–2020 in plasma-facing components including thermal expansion
under Grant Agreement No. 633053. The views and opinions Phys. Scr. T171 014011
expressed herein do not necessarily reflect those of the Euro- [11] Richou M. et al 2017 Realization of high heat flux tungsten
monoblock type target with graded interlayer for application
pean Commission. The views and opinions expressed herein to DEMO divertor Phys. Scr. T170 014022
do not necessarily reflect those of the ITER Organization. [12] Bowman C. 2020 C-Bowman/inference-tools: 0.5.3 release
https://doi.org/10.5281/zenodo.3757497
[13] Bufferand H. et al 2019 Three-dimensional modelling of edge
ORCID iDs multi-component plasma taking into account realistic wall
geometry Nucl. Mater. Energy 18 82–6
Rémi Delaporte-Mathurin https://orcid.org/0000-0003- [14] Kaveeva E. et al 2020 SOLPS-ITER modelling of ITER edge
plasma with drifts and currents Nucl. Fusion 60 046019
1064-8882 [15] Hodille E.A. et al 2021 Modelling of hydrogen trapping, dif-
Julien Denis https://orcid.org/0000-0002-1478-0269 fusion and permeation in divertor monoblocks under ITER-
James Dark https://orcid.org/0000-0002-0456-7210 like conditions Nucl. Fusion https://doi.org/10.1088/1741-
Etienne A. Hodille https://orcid.org/0000-0002-0859- 4326/ac2abc
390X [16] Ciraolo G. et al 2019 First modeling of strongly radiating WEST
plasmas with SOLEDGE-EIRENE Nucl. Mater. Energy 20
Gregory De Temmerman https://orcid.org/0000-0002- 100685
4173-0961 [17] Imbeaux F. et al 2015 Design and first applications of the
Xavier Bonnin https://orcid.org/0000-0002-6743-1062 ITER integrated modelling & analysis suite Nucl. Fusion 55
Jonathan Mougenot https://orcid.org/0000-0001-7397- 123006
0102 [18] Park J.-S., Bonnin X. and Pitts R. 2020 Assessment of ITER
divertor performance during early operation phases Nucl.
Yann Charles https://orcid.org/0000-0001-8185-7126 Fusion 61 016021
Christian Grisolia https://orcid.org/0000-0002-3038-9593 [19] Pitts R.A. et al 2019 Physics basis for the first ITER tungsten
divertor Nucl. Mater. Energy 20 100696
References [20] Ziegler J.F., Ziegler M.D. and Biersack J.P. 2010 SRIM—the
stopping and range of ions in matter Nucl. Instrum. Methods
Phys. Res. B 268 1818–23
[1] De Temmerman G., Hirai T. and Pitts R.A. 2018 The influence [21] Delaporte-Mathurin R., Dark J., Yang H. and Hodille E.A.
of plasma-surface interaction on the performance of tungsten 2021 IRFM/divHretention Source Code Github Repository
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