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A R T I C L E I N F O A B S T R A C T
Handling Editor: Dr S Nanda Hydrogen has a high diffusion rate and a wide range of combustion, making it essential to take safety precautions
against leakage during storage. We investigate the change in hydrogen concentration in confined spaces due to
Keywords: hydrogen leakage through experimental and numerical methods assuming the worst-case scenario. The vent area
Hydrogen consists of 12 %, 24 %, and 36 % of the floor area and is installed in the ceiling of the concrete enclosure. We
Leakage
confirm that the improvement of ventilation performance is insignificant just by increasing the ventilation area
Natural ventilation
above a certain standard during emergency ventilation. Moreover, the improvement of ventilation performance
Forced ventilation
Performance by forced ventilation is more effective as the natural ventilation area is smaller. Still, the effect decreases as the
natural ventilation area becomes larger. In conclusion, we confirm that ventilation efficiency is determined by
the natural ventilation area rather than forced ventilation.
* Corresponding author.
** Corresponding author.
E-mail addresses: kkpp9810@kict.re.kr (J. Kim), yangkyunkim@kict.re.kr (Y. Kim), templer83@kict.re.kr (B. Park), yoonunggi@kict.re.kr (U. Yoon), safetyfirst@
hknu.ac.kr (C. Kang).
https://doi.org/10.1016/j.ijhydene.2023.11.048
Received 23 August 2023; Received in revised form 17 October 2023; Accepted 4 November 2023
Available online 15 November 2023
0360-3199/© 2023 The Authors. Published by Elsevier Ltd on behalf of Hydrogen Energy Publications LLC. This is an open access article under the CC BY license
(http://creativecommons.org/licenses/by/4.0/).
J. Kim et al. International Journal of Hydrogen Energy 50 (2024) 1395–1405
ceiling, the more effectively it prevents hydrogen buildup. Lee et al. [19] close to the leakage source for hydrogen removal. In addition, studies on
conducted a CFD simulation of the hydrogen pressure regulation in hydrogen dispersion and removal based on ventilation types were con
Ulsan City’s hydrogen town in South Korea to investigate small-scale ducted for hydrogen refueling stations [29], nuclear facilities [30], and
leakage scenarios. They suggested an optimal vent location configura hydrogen-powered ship fuel cell rooms [31].
tion and compared different ventilation capacities by vent size relative The aforementioned studies confirmed that hydrogen behavior and
to floor area. Additionally, a hydrogen leakage management strategy ventilation performance vary depending on the location and shape of the
was proposed using forced-nitrogen purging. Barley et al. [20] investi vent when a hydrogen leak occurs. Additionally, these studies analyzed
gated the relationship between leakage rate, vent design, and hydrogen the ventilation effect in scenarios where natural ventilation is always
concentration through laboratory tests and CFD modeling. Their setup present, with variables comprising only vent shape and location and the
consisted of two vents, a lower and an upper one, while the degree of presence or absence of forced ventilation. However, it is equally
ventilation varied according to the opening of the vents; their experi important to consider the possibility of mechanical defects in the safety
mental results were compared to computational data to validate their measures set in advance. From a safety perspective, installing appro
model. Matsuura [21] also used CFD simulations to study hydrogen priate protective devices and buffers in any system is essential to reduce
dispersion and accumulation in a semi-confined space with natural and the likelihood of an accident or damage caused by one [32]. James
forced ventilation. Various combinations of roof vents and door vents Reason’s Swiss cheese model describes deficiencies in safeguards as the
were considered by changing their size and location, and their effec cause of accidents by analogizing them to randomly punctured cheese.
tiveness was compared with that of natural and forced ventilation. Ji In these terms, accidents occur when safeguards deficiencies fall in a
et al. [22] investigated hydrogen leakage and diffusion characteristics straight line. This analogy applies equally well to mitigating damage
by installing a 1.8 m × 2.2 m × 2.9 m room with 0.12 m3 of vents on after an accident has occurred and is compounded to produce results
three sides of the room and ventilation fans on the remaining side. [33,34]. Ultimately, no single safeguard can completely prevent an ac
Hydrogen concentrations were measured as the vent, ventilation fans, cident, so safeguards should be layered as much as possible to ensure
and supply shut-off valves operated. Moreover, Xie et al. [23] compared safety [35]. Indeed, it is possible scenarios for natural and forced
the effectiveness of different ventilation fan geometries on hydrogen ventilation systems to develop defects and fail to provide adequate
leakage in a garage with vehicles based on CFD simulations. ventilation. Due to the low minimum ignition energy of hydrogen
Studies comparing natural and forced ventilation have also been (mixed with air) (approximately 0.019 mJ), any ventilation method that
actively conducted. Cerchiara et al. [24] evaluated the effect of natural has the potential to release electrical energy, such as forced ventilation
ventilation based on the leakage rate to maintain hydrogen concentra with fans, could result in an explosion [19,36].
tion within 2 vol% inside a 25 m3 enclosure, including a fuel cell, and Studies so far have been conducted to create designs in which the
reported an increase in ventilation efficiency with additional forced concentration of hydrogen does not exceed the allowable value in the
ventilation. Prasad [25] compared the natural ventilation and forced event of hydrogen leakage through continuous ventilation. However, as
ventilation effects of compartmentalized spaces during the blowdown described above, consideration should be given to contingency plans to
situation of high-pressure hydrogen tanks, investigating the volume flow safely eliminate leaks in situations where ventilation is restricted (e.g.,
and behavior of released hydrogen. Merilo et al. [26] compared the in the event of ventilation system failure) and concentrations have
natural ventilation and forced ventilation effects in a hydrogen fuel cell already built up. This study aims to experimentally investigate ventila
vehicle garage concerning hydrogen leakage. They reported that me tion effectiveness using natural ventilation by deploying a vent that can
chanical ventilation was efficient in reducing hydrogen concentration in serve as an explosion panel in the event of an emergency; a scenario is
the garage in terms of hydrogen emission rate and ventilation rate. assumed in which a hydrogen leak occurs (due to, for example, irre
Additionally, Huang et al. [27] compared the ventilation effects of versible damage to a storage container) that results in an accumulating
hydrogen leakage from fuel cell vehicles in an underground parking lot hydrogen concentration. As a result, the ventilation efficiency by size of
using three modes (natural ventilation, forced ventilation after 300 s of the upper vent was compared to derive the appropriate ventilation size
leakage, continuous forced ventilation) and various ventilation layout for accident situations. This provides practical new designs and pa
configurations. Matsuura et al. [28] investigated the impact of different rameters to prevent and mitigate damage caused by hydrogen leakage
roof ventilation locations and areas on hydrogen accumulation and when designing enclosed spaces where hydrogen can exist. It can also
dispersion in partially open spaces from a natural ventilation perspec contribute to the development of a safer hydrogen infrastructure by
tive. They highlighted the effectiveness of selectively opening roof vents proposing new safety measures that are different from previous views.
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J. Kim et al. International Journal of Hydrogen Energy 50 (2024) 1395–1405
Fig. 1. (a) Images of the experimental setup, and (b) Schematic of the experimental setup.
This experiment aimed to determine the extent to which an internal where Av0 is the vent area calculated in m2, As is the enclosure internal
hydrogen concentration could reach below a reference value in the surface area in m2, Pred is the maximum pressure developed in a vented
event of a hydrogen leak in a confined space that is mitigated via the enclosure during a vented deflagration in barg, Su is the fundamental
deployment of an upper natural vent. The average temperature on the burning velocity of gas-air mixture in m/s, ρu is the mass density of
day of the experiment was 23.5 ◦ C, and the average wind speed was 1.6 unburned gas-air mixture in kg/m3, λ is the ratio of gas-air mixture
m/s. The experimental setup consisted of a 4.2 × 2.8 × 2.8 m burning velocity, Gu is the unburned gas-air mixture sonic flow mass flux
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J. Kim et al. International Journal of Hydrogen Energy 50 (2024) 1395–1405
Table 3
Investigated cases in the experiment (Cases E1-E9) and numerical analysis (Cases N1–N4).
Vents in the open position Total natural vent Vent area as a ratio of the Size of leakage hole Leak flow rate Ventilation fan flow rate
area (m2) floor area (%) (inches) (L/min) (m3/min)
in kg/m2-s, Cd is the vent flow discharge coefficient, Pmax is the different parameters. The overall setup for the thirteen cases is sum
maximum pressure in bar-g, and γb is the ratio of enclosure pressure marized in Table 3.
before ignition in bar-g, P0 is the enclosure pressure prior to ignition in
barg, Pstat is the nominal vent deployment or burst pressure in barg.
The internal space was completely sealed off until the hydrogen 2.2. Conditions for computational analysis
reached the target concentration. The size of each vent comprised 12 %
of the floor area. The experiment was conducted by varying the open 2.2.1. Governing equations
vent area (two and three times the base area, Case E1~E9). Four cases A nonlinear simultaneous differential equation was used to analyze
were selected for the computational analysis. In Cases N1 and N2, both the fluid and energy movements obtained after applying the laws of
vents were opened, a ventilation fan was installed in the center vent, and conservation of mass, momentum, and energy.
the capacity of the ventilation fan was set to different parameters. In As there are variations in velocity and pressure at each point in a
Cases N3 and N4, the center vent was closed, a ventilation fan was general turbulent flow situation, Reynolds Average Navier-Stokes
installed on one vent, and the capacity of the ventilation fan was set to (RANS) equation was utilized to analyze the momentum. In this study,
the k-ω model considering two equations among RANS-based models
Fig. 2. Grid information: (a) overall grid domain, (b) number of volume grid on the vent surface, and (c) size of volume grid on the vent surface.
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J. Kim et al. International Journal of Hydrogen Energy 50 (2024) 1395–1405
Fig. 4. Hydrogen concentration change over time for a vent area corresponding to 12 % of the floor are: (a) Case E1, (b) Case E2, and (c) Case E3.
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J. Kim et al. International Journal of Hydrogen Energy 50 (2024) 1395–1405
Table 4
Time to reach the target concentration by case (s).
12 % 24 % 36 %
Fig. 5. Hydrogen concentration change over time for a vent area corresponding to 24 % of the floor size: (a) Case E4, (b) Case E5, and (c) Case E6.
( ) ( )
⃒ ⃒
ln f3 − f2/f − f ln 1.36724 − 1.36676/1.36676 − 1.34769 ⃒1.36724 − 1.36676⃒/
2 1 = ⃒⃒ ⃒ ( −
⃒ 1.5 9.069
)
− 1 ×100% = − 0.036% (6)
p= = = − 9.069 1.36676
ln r ln 1.5
(5) ⃒ ⃒
⃒f2 − f1 ⃒⃒/
GCI1,2 = ⃒⃒ ⃒ (rp − 1) ×100%
Where f 1, f 2, f 3 is average hydrogen volume fraction by location (coarse, f1
medium, fine) respectively. Through the r and p value obtained in
⃒ ⃒
equation (5), the GCI was obtained as follows Eqs. (6) and (7). ⃒1.36676 − 1.34769⃒/
= ⃒⃒ ⃒ ( −
⃒ 1.5 9.069
)
− 1 ×100% = − 1.452% (7)
⃒ ⃒ 1.34769
⃒f3 − f2 ⃒/
GCI2,3 = ⃒⃒ ⃒ p ×100%
f2 ⃒ (r − 1) Grid dependence shown in equation (8) is 0.986, which is approxi
mately 1. Therefore, it was concluded that results obtained with current
grid structure are within the asymptotic range of convergence.
Fig. 6. Hydrogen concentration change over time for a vent area corresponding to 36 % of the floor size: (a) Case 3, (b) Case 6, and (c) Case 9.
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Fig. 8. Comparison of hydrogen concentrations per monitoring location (a) Left side of enclosure (S1, S2, S3) and (b) Center side of enclosure (S4, S5, S6).
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J. Kim et al. International Journal of Hydrogen Energy 50 (2024) 1395–1405
Fig. 9. Comparison of hydrogen concentrations per monitoring location for Case N1 and Case N2. (a) Left side of enclosure (S1, S2, S3 of Case N1), (b) Center side of
enclosure (S4, S5, S6 of Case N1), (c) Left side of enclosure (S1, S2, S3 of Case N2), and (d) Center side of enclosure (S4, S5, S6 of Case N2).
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J. Kim et al. International Journal of Hydrogen Energy 50 (2024) 1395–1405
Fig. 10. Comparison of hydrogen concentrations per monitoring location for Case N3 and Case N4. (a) Left side of enclosure (S1, S2, S3 of Case N3), (b) Center side
of enclosure (S4, S5, S6 of Case N3), (c) Left side of enclosure (S1, S2, S3 of Case N4), and (d) Center side of enclosure (S4, S5, S6 of Case N4).
3.3. Characteristics of forced ventilation concentration, like the method used in the previous experiment, the
time when all monitoring points were below the target concentration
Based on the simulation that confirmed validity, the results of the was measured, as shown in Table 5.
simultaneous application of natural and forced ventilation were shown In the case in which a fan with a capacity of 22 m3/min (Case N1)
below. The final target concentration was set as 4 vol% which is the LFL was installed in the center vent within a natural ventilation area cor
of hydrogen, in the computational analysis. To measure the target responding to 24 % of the floor area, it took 46.2 s to reach the target
Fig. 11. Overall comparison. (a) Concentration changes of the sensor [C-top] that fell below 4 % at the latest per case, and (b) Comparison of ventilation time below
4 % per case.
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concentration (LFL) (Table 5, Fig. 9). This finding is close (only 3 s 4. Conclusions
difference) to the fastest ventilation time (43.2 s) in cases E4, E5, and E6,
in which only natural ventilation (24 % of the floor area) was applied in This study experimentally investigated the efficiency of natural
the previous experiment. Considering that the simulation was analyzed ventilation in mitigating the effects of a hydrogen concentration buildup
conservatively, it is judged that the internal ventilation pattern (intake in a confined space with limited ventilation by deploying a vent that
and exhaust) formed under the influence of forced ventilation increased serves as an explosion panel. We reached the following conclusions.
ventilation efficiency. The formation of such a ventilation pattern can be
expected to maintain a constant ventilation efficiency, unlike natural i) As for experimental ventilation time, it was difficult to predict the
ventilation, which varies depending on the surrounding environment general ventilation time required to reach safe conditions in the
[43,44]. However, there was no considerable decrease in ventilation case of the smallest vent area (Kv = 6.62) because it was highly
time due to the addition of forced ventilation. affected by the external environment.
Under Case N2, similar to Case N1, in which a fan with a capacity of ii) The required ventilation time tended to decrease as the vent area
44 m3/min was installed in the center vent within a natural ventilation increased. But the ventilation time (to LFL) for the medium and
area corresponding to 24 % of the floor area, it required 44.8 s to reach large vents was similar. These results revealed that selecting an
the LFL (Table 5, Fig. 9). Compared to this result with Case N1 with the area below Kv = 3.31 is reasonable when designing a roof vent.
capacity of 22 m3/min, a slight difference of 1.4s was found. This may be iii) As a result of the numeric analysis, the time required for venti
due to the saturation of ventilation efficiency. In the previous experi lation decreased as fan capacity increased. We found that this
mental part, the ventilation efficiency of natural vents, which have an effect was larger when the natural ventilation area was smaller.
area equivalent to 24 % and 36 % of the floor area, was similar. This This implies that the ventilation performance depended on forced
indicates that when an appropriate natural ventilation area is secured in ventilation factors like the capacity of fans as the natural venti
forced ventilation, the natural ventilation area is dominant in deter lation area decreased.
mining ventilation efficiency rather than forced ventilation factors such iv) Higher ventilation efficiency can be expected with forced venti
as fan capacity. Therefore, if natural ventilation area had already pro lation under the condition that the vent area is larger than Kv =
vided optimal ventilation efficiency, further increases in forced venti 3.31; however, in the case where it is smaller than Kv = 3.31, the
lation capacity may not have a real effect. ventilation time will be dominated by natural ventilation area,
Under Case N3, in which there was a fan with a capacity of 22 m3/ which would make it difficult to expect a higher ventilation ef
min within a natural ventilation area corresponding to 12 % of the floor ficiency after adding forced ventilation.
area, it took 102.6 s to reach the LFL (Table 5, Fig. 10). Compared with
Case N1, with the fan with the same capacity, and the difference in the This study proposed a practical and novel method to design safety
natural ventilation area by 12 %, two cases showed a difference of 56.4 measures for areas where hydrogen is stored. This method can be
s; this finding is close (6.2 s difference) to the fastest ventilation time applied as an emergency measure when designing a ventilation system
(108.8 s) in Cases E1, E2, and E3, in which only natural ventilation (12 for a confined space. However, it may be challenging to maximize
% of the floor area) was applied in the previous experiment. Compared ventilation efficiency by using only the method proposed in this study as
to the results of 297.6 s and 228.4 s, it was 2.9 times smaller. It was also an emergency ventilation system. Designs such as the addition of forced
confirmed that the ventilation time, compared to Case N1, was more ventilation with nitrogen proposed in Ref. [19] can help design safer
influenced by the natural ventilation area than the fan capacity. hydrogen facilities. Therefore, further research is needed to increase
Case N4, similar to Case N3, in which there was a fan with a capacity ventilation efficiency by applying additional methods.
of 44 m3/min within the natural ventilation area corresponding to the
floor area, required 63.4 s to reach the LFL (Table 5, Fig. 10). Compared
to the difference between Cases N1 and N2 with 12 % additional natural Declaration of competing interest
ventilation areas, the difference between Cases N3 and N4 significantly
increased by approximately 37.8 s. This finding confirms that depen The authors declare that they have no known competing financial
dence on forced ventilation via fan increased in a smaller natural interests or personal relationships that could have appeared to influence
ventilation area. If the area of the natural ventilation where air is being the work reported in this paper.
drawn in is small, hydrogen tends to move downward due to the pro
motion of global circulation within the confined space, making it diffi Acknowledgements
cult for the hydrogen to be discharged through the roof vent [41]. This
directly affects the ventilation rate, and the more stringent these re This work is supported by the Ministry of the Interior and Safety
strictions become, the more efficient it is to apply forced ventilation. (20018517). The funding agency had no role in study design; in the
Therefore, if the vent size was 12 % of the floor area, forced ventilation collection, analysis and interpretation of data; in the writing of the
(fan capacity) greatly affected the ventilation efficiency. report; and in the decision to submit the article for publication.
Fig. 11 indicates the comparison of entire cases. We found that the
last point falling below 4 % among six monitoring points in all cases was
the center-top point (C-top), which is revealed in Fig. 11 (a), while the References
total ventilation time can be found in Fig. 11 (b). As for the overall
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