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PhysRevC 52 1348
PhysRevC 52 1348
The levels in' "" Ru have been investigated in the spontaneous fission of 2Cf using y-y-y-, y-y-, x-x-,
bands have been identified with very little energy staggering in ' "" Ru. The ground bands in ' "
x-y-, and x-y-y-coincidence techniques. The levels up to 16+ and 9+ in the yrast bands and y-vibrational
Ru
have identical y-ray transition energies up to 8+. These are the lightest observed even-even nuclei with
extended identical ground bands. Calculations in a collective model which includes rotations and vibrations
reproduce the level energies and y band branching ratios above the 3+ state rather we11, while rigid triaxial
rotor model calculations reproduce the branching ratios for the 2+ and 3+ states.
12.5 x 104 the lightest even-even nuclei with extended identical ground
10. 0— 0 '
N
}( 1 10RU p+ o+
"OSRu: 2+-0+
""
bands. The y-vibrational bands observed to 9+ in
Ru are the first y bands extended above 3+ in
N
"
neutron-rich nuclei in this region. While the 2 bandhead
energies are almost 100 keV apart in ' Ru, many of the
transitions in their y bands have nearly similar energies
O
5. 0— (0.7 —3% differences). The levels from 2+ to 9+ in the y
bands of all three nuclei exhibit very little signature splitting
in contrast to the strong splitting expected for triaxial nuclei.
Because of the additional parameters associated with signa-
0.0 I I
ture splitting and bandhead energies, the observation of simi-
225 230 235 240 260 265
lar energy transitions in y bands in neighboring even-even
Energy (keV)
nuclei raises additional questions regarding the explanation
of identical bands.
FIG. 1. The 2+~0+ transition in the high resolution x-ray de- The energies of the ground-band transitions in ' Ru and
tector in the x-y coincidence setup. " Ru are so close all the way up to 8 that only the
2+ ~0+ and 8+ — +6+ transitions can be separated to provide
events from 10 keV up to several hundred keV so that x-rays independent gates for investigating these bands. The
from Sr to Eu along with transitions above 300 keV were 2+ — +0+ transitions observed in a high resolution x-ray de-
observed with intensities sufficient to set gates on the x rays tector in the x-y-coincidence setup are shown in Fig. 1. A
and observe the low energy y rays. The triple-coincidence spectrum obtained by summing all the double gated spectra
that can result when gates are set on the first four members of
technique is particularly powerful in eliminating or reducing
background. This technique becomes very useful especially the yrast cascade in "
Ru is shown in Fig. 2(a). Figure 2(b)
shows a double gate set on the 14+~12+ and 10+ — +8+
if y-ray energies from different nuclei fall within the energy
gate set on a single y ray in a y-y-coincidence experiment. transitions in "
Ru. The level schemes based on y-y,
The x-x- and x-y-coincidence spectra were particularly help- y-y-y, and x-y coincidences are shown in Figs. 3(a), 3(b),
ful in unraveling the transitions in the identical bands in and 3(c). In the present work we have extended the ground
108, 110Ru bands in the three nuclei up to 16+. An unusual feature of
the" Ru level scheme is the sequence of three new transi-
tions feeding the 6+, 8+, and 10+ levels but with no observ-
III. RESULTS AND CONCLUSIONS able transitions connecting them.
""
The ground bands have been extended from 10 [8,9] up 10+ levels in the ground bands of ' "
The transitions up to the 8+ levels and essentially to the
Ru are among the
"
to 16+ in ' Ru. The ground band transitions in
Ru are found to be remarkably identical up to 8+ and "
most identical in energies and in moments of inertia, J1 and
J2. The ' Ru nuclei extend our knowledge of identical
essentially so up to 10+ but are not identical to those in
" Ru which has an even larger moment of inertia. These are
bands into new regions: those neighboring even-even nuclei
have the lowest mass number of any such neutron-rich
""'Ru
+
30000- Sum Double Gate on
~+ (244, 422, 576 and 705 keV)
(a)
20000-
C)
+
00
r x
10000—
200 400 600 800 the transitions out of the yrast cascade from 2+ to
CL
"'ORu 14+ in " Ru. (b) A double gate on the 705 —815-
Qj
0 900
Double Gate on 705—815 keV
keV transition in " Ru.
(b)
500
I
I
100
I
16+ 6512
16+ 5150.1
(865)
14~ i 4288.2 108 14+ 5211
798.6
64
12+ 3974 14+ )r 4351.5
Ru
762.1 44 66
12+ i ) 3526.1 12+ 4011
705.0
3158 0 36999 + ~r 3646 5
787.8
(9+) 2908.9 10+ 2921.5 10+ 3109.0
10+ i~ 2738.3 87.4
776.7 8+ 9+ 3004.0
2619.9 2892 8
(8+) 10+ 2947.0
2419.1 10+ it 2759.1 (9+) 2776.8 8+ 2411.0
7983
2269.0
2132.2 7+ 2 149.0
8+ (8+i 2397. 1
8~ 1941.6 6363 2011.7 814.7 755.9
l& 8+ 2031.0
(6 ) ii 1761.3 1841.4 (7+) ir 2020 6+ 1717.0
+ ir 1944.4
7018 ?12.8
) 1495.7
it
5+ (6+} ir 1684
578.8 1526.4 705, 7
521.1 645.4 5+ 1428.0
6+ i I1240.0 +) 1( 1182.5
'
1247.9 4+ 119L6
5+) ir l375.6 6+ 1260.0
6+ ir 1238. 515.4 599.7
974.6 3+ 4+) i 1084.3 1097 0
5755 942.2 r
475.0 2+
4+ it 6640 702.2 575.6 3+ i r859.8 3+ 854.4
707$
638.4 4+ ir 663. 247.6 471.7
2+ irir 612,6 2+ 606 3
4225
2+ 206, 1 y band 422, .3
lt 242.0 240.
0+ i t242.0 0.0 0+ 0.0
Z+ sr
240. 8
208.7
0.0
y- band
0.0
1 12Ru
44 68 16+ 6612.0
16+ 495 3.0
83 6. IQ
14+ 5241 0
14+ ir 4118.0
791.9 12+ 4033.0
12+ ir 3326.1
"
"
neighbors having extended identical bands. The transition esting that Ru with a larger moment of inertia is not iden-
"
energies in Ru are all considerably smaller than in
Ru, and the moments of inertia extracted from the en-
tical. If these nuclei are rigid triaxial rotors as recently re-
ported [9], this would make the identical nature of these
ergies are larger and increase more rapidly with spin [see
" bands even more unusual. Such identical energies are not
"" ""
Table I and Fig. 4]. The deformation of
presumably larger than that of ' "
Ru is therefore
Ru. The neutron number
seen in N=64, 66 Pd [3, 11]. However, the
have considerably smaller deformation, p2=0. 21(2) and
Pd
"
(N=64, 68) to either side. The deformations, p2=0. 28(2)
0. 12(2), respectively.
The clearly identified y bands up to 9+ in ' Ru ""
for ' Ru obtained from lifetime measurements, are sig- here, and also in [9], are the first extended y-vibrational
nificant [4 —6]. If saturation of collectivity is the explanation bands seen in neutron-rich nuclei. They have low energy
for the identical ground bands in &08Ru and rioRu as f~~~d
in ' '
Hg by Bindra et al. , [10] it is interesting to find this ""
2 band heads. The 612.6- and 523.4-keV bandheads in
Ru are the next lowest in energy of all known y bands,
effect still operative in this lighter mass neutron-rich region. second only to the 558.0- and 489. l-keV bandheads in
Also, if saturation of collectivity is the reason why the Os [12,13]. What is more surprising is that apart from
N = 64, 66 nuclei have identical energies„ it is likewise inter- the lowest transitions between the 3+ and 2+ levels, the
STRUCTURE OF ' "" Ru IDENTICAL BANDS IN . . . 1351
"" ""
TABLE I. The kinetic and dynamic moments of inertia J1 and J2 for the ground bands of
Ru. Notice the identical values for J1 and J2 for ' Ru because of their identical
energies.
transitions out of the 4+ to 9+ levels in ' Ru have en-" model t7j. In a rigid asymmetric rotor model the 2+ energy
""
+
ergies within 0.7 to 3.4% of each other (see Table II; the drops below the 4, ground level for y=22 . Since this oc-
3+~2+ energies differ by nearly 10%). The energies and curs for Ru and the fact that F2++ F2+ =E3+ are con-
1 2 1
relative intensities of y transitions in ' '
Ru are given sistent with the earlier reported y values Pj. Recently, the
in Table III. One can see from Table III that the two branching ratios for the extended side bands have provided
additional support for a rigid triaxial rotor interpretation of
y-vibrational bands in neighboring nuclei have nearly similar
energies. While the ratio R = E(4+)-E(2+)lE(3+)-E(2+) is "
Ru with y= 22. 6', 24.0', and 25.9', respectively I9].
somewhat different (1.78 in ' Ru and 1.90 in Ru) be- " However, the new levels above 3+ do not show the strong
cause of the different E(3 )-E(2+) energies, there is very signature splitting expected for a rigid y where the
little odd-even spin staggering through the 9 levels. Thus, (2+, 3 ), (4+, 5 ), (6,
7 ) pairs should be close in energy
the nearly identical dynamical moments of inertia are related for such a rigid triaxial rotor (RTR) interpretation. Likewise
neither to the bandhead energies nor to their signature split- the y-soft model, which is closely related to the IBA-I O(6)
"
Without information on the extended y bands, the
Ru nuclei have been treated using an interacting boson
2+ bandheads, little or no odd-even spin [12,13j staggerings
are also observed.
200
(a)
40
Ru
100—
35 08RU
1oRu
) 30 I
CU 0
FIG. 4. Moments of inertia J1 added J2 for
108, 110,112R
25 CU
20—
-100
15—
I I I I I
To see how well the energies of the two bands can be symmetry axis, and n~ and n& are the number of y- and
reproduced in a standard collective model, we carried out an P-vibrational phonons present. In order to obtain conver-
analysis in the rotation-vibration model [15,16]. The Hamil- gence of the energy levels up to spin 12 to four significant
tonian consists of three parts: a rotational part H„„, a P- and digits, we found that 140 basis states are required in
y-vibrational part H„b, and a third term which contains the the diag onalization. Specifically, our basis contains all
rotation-vibration interaction H . The last term arises from eigenstates with quantum numbers: K = 0,2,4, . . . , 12;
the dependence of the moments of inertia of the nucleus on n =0, 1, 2, 3, and n&=0, 1,2, 3,4. The three energy param-
the vibrational amplitudes. eters used in the rotation-vibration model are E„,=0.15,
We have diagonalized the interaction term H', numeri- 0. 15, 0. 15 MeV, E~=0.62, 0.52, 0.42 MeV, and E&=1.2,
cally in terms of the eigenstates ~K, n~, n&) of the basis 1.4, 1.4 MeV for &os, &io, ii2Ru respectively. The results are
Hamiltonian Ho= H, , + H„b. Here, K denotes the projection shown in Figs. 3(a), 3(b), and 3(c). It is surprising how well
of the total angular momentum onto the intrinsic nuclear this simple collective model reproduces the experimentally
observed level schemes in contrast to a RTR model. The
"."
TABLE III. Energies and relative intensities of y-transitions in
Ru. The uncertainties in the transition intensities range
generalized collective model (see Ref. [16]) would almost
certainly yield an even better agreement with the data, but
from 5% for strong transitions to 50% for very weak transitions.
only at the expense of introducing additional model param-
108R 1108 112R eters. This does not seem worthwhile, given the relatively
E (keV) I E (keV) I small number of experimentally observed levels and the ab-
(%) IC (keV) I~ (%) (%)
sence of other data such as B(E2) values.
242. 0 100 240. 8 100 236.6 100 Shannon et al. [9] compared the branching ratios with
422. 5 74 422. 3 74 408.4 77 those predicted by a rigid triaxial rotor (RTR) model. Under
575.5 46 575.6 44 544.9 53 the assumption that all transitions are pure E2, reasonable
701.6 12 705.7 16 649.5 17 agreement was found between the experimental branching
798.3 4 814.7 6 723.3 10 ratios and RTR calculated values for the 2+, 3+ levels as
787.8 2 887.4 2 763.4 6 seen in Table IV. However, for the 4 and 5+ levels dis-
762. 1 1 705.0 1 791.9 4 agreements by a factor of 2 —100 are observed compared to
865 0.3 798.6 0.7 836.0 2 RTR values. Shannon et al. [9] suggested that a small Ml
707.5 8 612.6 12 523.6 12 —
admixture in the 5+ &4+ transition could bring agreement,
267. 1 2 247. 6 6 224. 0 7 but such an approach seems insufficient to alter such a large
521.1 12 515.4 23 487.9 20 disagreement. They concluded that the branching ratios are
636.5
776.7
7
2
645.4
755.9
8
2
605.4
693.3
10
2
""
the most convincing evidence for rigid triaxial shapes for
Ru. They deduced y values of 22. 5', 24. 2', 26.4
for &os, i o, i i2Ru, respectively, from the excitation energies of
&
TABLE IV. B(E2) branching ratios. The theoretical results were calculated in a generalized collective model [15,16] and in a rigid triaxial
rotor model [17].
B(E2) ratios
2 -2: 3+ 2+ 3+ 2+, 4+ 2+ 4+ 2+ 5+ 3+ 6+ —+4+,
2+ 0+ 3+ 4+ 3+ 2+ 4+ 2+ 5+ 4+ 6+ +6+,
energies and the branching ratios from the 3+ levels. How- by a rigid triaxial rotor model which was able to provide a
ever, the 2+ branching ratios do not provide a unique test to good fit for the relative B(E2)'s from the decay of the 2+
claim that a nucleus is a rigid triaxial rotor. A possible inter- and 3+ levels. To explain both the level energies and branch-
pretation of these results is that the 2+ and 3+ states have a ing ratios requires additions to either model or a change from
triaxial shape or are soft to y deformation and that the nuclei RTR to an axially symmetric shape below the 4+ state.
take on a more axially syrrunetric shape by the 4+ state. To
ACKNOWLEDGMENTS
say the least, the new extended bands built on the 2 levels
in these nuclei present an interesting challenge for nuclear Work at Vanderbilt University and the Idaho National En-
Hlodels. gineering Laboratory was supported in part by the U. S. De-
In summary, the levels in the ground bands were observed partment of Energy under Grant No. DE-F605-88ER40407
up to 16+, spins being assigned tentatively from systematics and Contract No. DE-AC07-76ID01570, respectively. One of
9+ in ' "
in &08, »0, &12Ru, and the y-vibrational band was observed to
"
Ru. The ground band transitions and moments of
inertia are remarkably identical in '
the authors (V.E.O. ) acknowledges the support from the De-
partment of Energy under Grant No. DE-F605-87ER40376.
" Ru but not in the Work at the Lawrence Berkeley Laboratory was supported
"
more deformed Ru. The y band transition energies in
Ru are also very nearly identical. While somewhat less
identical than the ground bands, these are the first nearly
by the U. S. Department of Energy under Contract Nos. DE-
FG03-87ER40323, W-7405-EN 648, and DE-AC03-
76SF00098. Oak Ridge National Laboratory is managed by
identical y-vibrational bands reported. An analysis of the en- Martin Marietta Energy Systems for the U. S. Department of
ergies of the ground and y bands in a rotation-vibration Energy under Contract No. DE-AC05-84OR21400. Work at
model yielded rather good agreement between the predicted the Joint Institute for Nuclear Research was supported in part
and observed energy values and relative B(E2) values above by Grant No. 94-02-05584-a of the Russian Federal Founda-
3+ . This result is in contrast to the poor agreement yielded tion of Basic Sciences.
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