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Wang 2
Wang 2
W.-H. Wang
Abstract Introduction
Scintillation counters have widespread uses in The scintillation detector with a NaI crystal
measuring gamma rays and low-energy beta rays. doped with thallium [NaI(Tl)] as activation
The sodium iodide (NaI) scintillator has a high impurities is one of the best instruments for
attenuation coefficient for the interaction of counting gamma rays. The most prominent
gamma rays and gives high efficiency and good property of NaI(Tl) is its excellent light yield. The
resolution of gamma rays. When the analyzer of high atomic number of iodine in NaI results in
the counting system is in the differential mode, high efficiency for gamma ray detection. The best
both lower and upper discriminators are used and resolution achievable is about 7% for the 662-keV
the scintillation counting system is called a single gamma ray from Cs-137 for a 3-inch diameter by
channel analyzer (SCA). The primary application 3-inch long NaI crystal. Besides, NaI(Tl) is almost
of an SCA is to discriminate between a desired linear in its energy response.[1] It has come to be
radiation and other radiation that may be con- accepted as the standard scintillation material for
sidered noise. In this article, the principles and routine gamma ray spectroscopy. For a scintil-
components of a typical single channel analyzer lation counter, a gamma ray with a given energy
will be discussed. Also, five typical operating will deposit this energy in the NaI(Tl) crystal by
procedures will be described regarding: excitation and ionization. Only the amount of
excitation which causes electronic transitions to
1. determination of the operating voltage for the
excited states in the luminescent material is
photomultiplier (PM) tube;
proportional to the energy of the gamma ray. The
2. calibration of a spectrometer for excited states decay by emitting flashes of light
a particular gamma-ray energy; known as scintillation photons in 0.23 micro-
3. establishment of a differential spectrum of a second.[2] After the scintillation photons strike the
gamma-ray emitter; photocathode, photoelectrons are ejected at the
photocathode. Again, the number of photo-
4. computation of the energy resolution of the electrons is proportional to the energy of the
NaI detector; and gamma ray. Then the electrons are accelerated to a
5. calculation of the counting efficiency of the dynode. When the photo-multiplier tube is
single channel analyzer. operated at a high voltage, there will be multi-
plication of the photoelectrons. The degree of
multiplication depends upon the voltage applied.
The higher the voltage, the greater the
multiplication, and so the greater
60000
40000
20000
0
0 200 400 600 800 1000 1200
voltage (volts)
14. Correct the counts in the Cs-137 spectrum for After the analyzer has been calibrated for the
background. desired energy range and the spectrum of the Cs-
137 to be counted is known, the relative counting
15. Plot the net count rate of Cs-137 on the efficiency of the NaI detector should be
ordinate versus the base discriminator setting determined using a calibrated source. Counting
on the abscissa of linear graph paper. efficiency can be calculated using the ratio of the
16. Draw a smooth curve through the points. net count rate to the absolute activity of a
Check to ensure the peak is at 652. radionuclide. The geometry of the detector and
source arrangements must be fixed in order to
have a constant counting efficiency.
Results
Results for this typical operating procedure are Typical Operating Procedure
shown in Table 2 on the following page (result
B).When the coarse-gain and fine-gain settings 1. Use Cs-137 as a calibrated gamma source.
were 8 and 50 individually, there were almost no 2. Set the coarse gain and fine gain as
counts registered. The scaler started registering determined previously (8 and 337,
counts when the voltage was increased to 820 respectively in this case).
volts.
3. Set the high voltage as determined previously
(820 volts in this case).
Resolution 4. Set the analyzer in the differential mode.
The quality of a given scintillation counting 5. Choose a window of 0.2 V which straddles
system is often characterized by the magnitude of the photopeak for the source.
its energy resolution. The system resolution is a
measure of the photopeak sharpness. Resolution is 6. Take five successive one-minute counts
defined as the ratio of the full width at half- 7. Calculate the average count rate.
maximum (FWHM) of the full energy peak
(called the “photopeak” when dealing with photon 8. Calculate the current absolute activity.
detectors) to the energy midpoint of the full 9. Calculate the counting efficiency.
energy peak.[3] Thus, the resolution is dimen-
sionless fraction conventionally expressed as a
percentage. With a small resolution, the detector is
able to separate two radiations whose energies are
close together.
712 367 56,565 1,170 2,053 4,307 7,085 5,610 6,300 6,032
692 452 42,970 1,307 3,290 13,462 22,158 18,118 19,585 19,362
672 480 20,158 1,422 8,915 36,873 48,672 44,732 46,717 46,088
652 627 9,312 1,548 28,630 60,798 61,677 61,917 61,708 61,753
632 702 3,493 1,795 57,822 53,283 41,412 46,878 44,050 45,092
612 838 2,193 2,345 60,353 25,363 16,235 19,525 17,905 18,648
592 1,028 2,185 4,705 31,520 7,838 5,053 6,037 5,375 5,442
From the above experimental data, the optimal operating conditions for this counting system are coarse gain of 8,
fine gain of 337, and high voltage of 820 volts.
Determination of Cs-137 Spectrum (counts per minute)
Cs-137 Spectrum
500000
NET COUNT RATE
400000
count rate (cpm)
300000
200000
100000
0
0 200 400 600 800 1000
base discriminator setting
Results
A = A0 e -λt
The data of five successive one-minute counts dis
are follows: 3.7 × 10 4
= 7.0 µCi × sec
1µCi
Gross BKG Net
− 0.693
(cpm) (cpm (cpm) 60 sec 30yr
× 21.9yr
× ×e
) 1 min
dis
365,378 1 365,377 = 9,370,134
min
376,941 3 376,938
363,190 4 363,186 where:
371,007 1 371,006 A is the amount of activity left after time t;
357,600 3 357,597 A0 is the initial quantity of activity;
Average =
366,823 λ is the transformation constant (= 0.693 / half-
cpm life ); and
t is the decay time.