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G. Hazra Radioactive Pollution: An Overview
All content following this page was uploaded by Goutam Hazra on 15 July 2018.
GOUTAM HAZRA
The civilian radioactive waste encompasses a wide range of materials, most of the current debate focuses on highly radioactive
spent fuel from nuclear power plants. Other types of civilian radioactive waste have also generated by nuclear power plants,
medical institutions, industrial operations, and research activities. Disposal of radioactive waste will be a key issue in the
continuing nuclear power debate. Without a national disposal system, spent fuel from nuclear power plants must be stored on-site
indefinitely. the strategy for the management and disposal of used nuclear fuel and high-level radioactive waste has highlighted
agreement with many of the principles of the IAEA recommendations and has outlined actions that, with legislative authorization
by Congress, can lead to a safe and responsible solution to managing the nation‘s nuclear waste. Indeed, action by Congress in
the form of new authorizing legislation and appropriations is necessary. Key words: radioactive spent, nuclear power plants,
radioactive waste.
Radioaktivno onečišćenje: Pregled. Civilni radioaktivni otpad obuhvaća široki raspon materijala; većina aktualne rasprave
usmjerena je na visoko radioaktivno istrošeno gorivo iz nuklearnih elektrana. Druge vrste civilnog radioaktivnog otpada također
generiraju nuklearne elektrane, medicinske ustanove, industrijski procesi i istraživačke aktivnosti. Zbrinjavanje radioaktivnog
otpada bit će ključno pitanje u kontinuiranoj raspravi o nuklearnoj energiji. Bez nacionalnog sustava zbrinjavanja, istrošeno gorivo
iz nuklearnih elektrana mora se pohraniti na neodređeno vrijeme. Strategija upravljanja i zbrinjavanja korištenog nuklearnog
goriva i visokoradioaktivnog otpada istaknula je suglasnost s mnogim načelima preporuka IAEA (Međunarodna agencija za
atomsku energiju) i opisala aktivnosti koje uz zakonodavno odobrenje Kongresa mogu dovesti do sigurnog i odgovornog rješenja
za upravljanje nacionalnim nuklearnim otpadom. Doista, Kongres treba poduzeti aktivnosti u obliku nove legislative i izdvajanja
proračunskih sredstava.
Ključne riječi: radioaktivno onečišćenje, nuklearne elektrane, radioaktivni otpad.
INTRODUCTION
Certain elements that compose matter radiation with shorter wavelengths than any
emit particles and radiations spontaneously. X-rays. These ‗rays‘ can penetrate living
This phenomenon is referred to as tissues for short distances and affect the
‗radioactivity‘; it cannot be altered by tissue cells. But because they can disrupt
application of heat, electricity or any other chemical bonds in the molecules of
force and remains unchangeable. Three important chemicals within the cells, they
different kinds of rays, known as alpha, beta help in treating cancers and other diseases.
and gamma rays are associated with Every element can be made to emit such rays
radioactivity. The alpha rays consist of artificially. If such radioactive elements are
particles (nuclei of helium atoms) carrying a placed in the body through food or by other
The Holistic Approach to Environment 8(2018)2, 48-65 Page 48
G. Hazra Radioactive Pollution: An Overview
positive charge, beta rays particles have methods, the rays can be traced through the
negative charge (streams of electrons) and body. This use of tracer elements is
gamma rays are charge less electromagnetic extremely helpful in monitoring life
processes. Geologists use radioactivity to problem for handling and protecting the
determine the age of rocks. As atoms lose environment to be safe to the present and future
particles as heavy as nuclei of helium, they generations. This article deals with this global
become atoms of some other element. That is, problem in its varied aspects and discusses the
the elements change or ‗transmute‘ into other cause for concern, the magnitude of the waste
elements until the series ends with a stable involved and various solutions proposed and
element. Radioactive elements decay at being practised. As nuclear power and arsenal
different rates. Rates are measured as halflives – grow, continuous monitoring and
that is, the time it takes for one half of any given immobilization of the waste over several
quantity of a radioactive element to disintegrate. decades and centuries and deposition in safe
238
The longest half-life is that of the ‗isotope‘ U repositories, assumes great relevance and
of uranium is 4.5 billion years [1]. Some importance [3]. Methods for the safe disposal of
isotopes have halflives of years, months, days, nuclear waste materials will also be discussed.
minutes, seconds, or even less than millionths of This method is the state-of-theart in nuclear
a second. Every inhabitant on this planet is waste disposal technology. It is the single viable
constantly exposed to naturally occurring means of disposing radioactive waste that
ionizing radiation called back- ground radiation. ensures non return of the relegated material to
Sources of background radiation include cosmic the biosphere. At the same time, it affords
rays from the Sun and stars, naturally occurring inaccessibility to eliminated weapons material.
radioactive materials in rocks and soil, The principle involved is the removal of the
radionuclide normally incorporated into our material from the biosphere faster than it can
body‘s tissues, and radon and its products, return. It is considered that ‗the safest, the most
which we inhale. We are also exposed to sensible, the most eco- nominal, the most stable
ionizing radiation from man-made sources, longterm, the most environmentally benign, the
mostly through medical procedures like X-ray most utterly obvious places to get rid of nuclear
diagnostics. Radiation therapy is usually waste, high-level waste or low- level waste is in
targeted only to the affected tissues [2]. the deep oceans that cover 70% of the
In this lesson we will discuss about the planet‘[4].
radiations which are the cause of radioactive
pollution. These radiations are emitted by
radioactive decay of unstable heavy atoms
nuclei. Exposure of these radiations can cause
damage to living cells and environment.
Concern for radioactive pollution increased after
the discovery of artificial radioactivity,
development of nuclear weapons and installation
of nuclear reactors for generating electricity. We
shall discuss the possible threat to human health
and environment due to nuclear radiations both
from natural and anthropogenic (manmade)
sources. Radioactive waste, arising from civilian Page
nuclear activities as well as from defence-related
nu- clear-weapon activities, poses a formidable
The Holistic Approach to Environment 8(2018)2, 48-65 49
G. Hazra Radioactive Pollution: An Overview
[6].
RADIOACTIVE pollution. There are two types of sources
POLLUTION & THEIR [7].
SOURCES 1. Natural sources
Cosmic rays
Living organisms are continuously Terrestrial radiation
exposed to a variety of radiations called 2. Man-Made sources
background radiations. If the level of the Medical sources
radioactive radiations increases above a certain Industrial sources
limit it causes harmful effects to living beings.
Nuclear Explorations
This harmful level of radiations emitted by
Nuclear Power
radioactive elements is called radioactive
Nuclear & Radiation accidents
Throughout the history of life on earth,
organisms continuously have been exposed
Natural sources to cosmic rays, radionuclide produced by
cosmic ray interactions in the atmosphere,
and radiation from naturally occurring
substances which are ubiquitously distributed
in all living and nonliving components of the contributor to the total cosmic flux since
environment. It is clear that contemporary diurnal variations are very small. Cosmic
life have adjusted or are doing so to all rays may be termed "primary" or
features and limitations of the environment, "secondary". Those, which have not yet
including the natural radiation background. interacted with matter in the earth's
Although high levels of radiation are atmosphere, lithosphere, or hydrosphere, are
definitely harmful to organisms, some termed primary. These consist principally of
environmental radiation is of importance to protons (≈85%) and alpha particles (≈14%),
life, as we know it. For example, background with much smaller fluxes (<1%) of heavier
radiation has contributed, though we do not nuclei. Secondary cosmic rays, which are
know how much, to the fundamental produced by interactions of the primary rays
processes of chemical and biological and atmosphere, consist largely of subatomic
evolution. Of clearer importance is the fact particles such as pions, muons, and electrons.
that the earth's heat content is principally At sea level, nearly all the observed cosmic
provided and maintained by the heat of decay radiation consists of secondary cosmic rays,
of primordial, naturally occurring with some 68% of the flux accounted for by
radionuclide. moons‘ and 30% by electrons. Less than 1%
Cosmic rays of the flux at sea level consists of protons.
Radiation of extraterrestrial origin, which Terrestrial Radiation
rain continuously upon the earth, is termed Radionuclide‘s, which appeared on the
"cosmic rays". The fact that this highly Earth at the time of formation of the Earth,
penetrating radiation was impinging upon the are termed "primordial". Of the many
earth from space, rather than emanating from radionuclides that must have been formed
the earth, was deduced from balloon with the Earth, only a few have half-lives
experiments in which ionization sufficiently long to explain their current
measurements were made at various altitudes existence. If the Earth was formed about 6
from sea level to 9,000 m. It was found that 109 years ago, a primordial radionuclide
the ionizing radiation rate decreased for some would need a half-life of at least 108 years
700 m and from that point increased quite to still be present in measurable quantities.
rapidly with elevation. The initial decrease Of the primordial radionuclide that are still
could be explained by a decreased intensity detectable, three are of overwhelming
of terrestrial gamma rays, while the significance. These are K-40, U-238 and
increasing component was due to cosmic Th232. Uranium and thorium each initiate
rays. The likely origin of cosmic rays is the a chain of radioactive progeny, which are
almost infinite number of stars in the nearly always found in the presence of the
Universe. Evidence for this is the increased parent nuclides (Table 2). Although many
cosmic ray intensity observed on earth of the daughter radionuclide are short-
following solar flares. However, it is clear lived, they are distributed in the
that the sun is not normally a major environment because they are continually
being forming from long-lived precursors.
Radiations are employed for diagnostic
and therapeutic applications. X-rays are
Man-maide sources used in general radiology and CT scan.
Gamma rays are used in treatment of
Medical source
cancer. In all these procedures we are given off during nuclear test affect the human
exposed to varying doses of radiations. body.
Industrial source Nuclear & Radiation Accidents
Radioisotopes are much more widely used in Radiations may leak from nuclear reactors
industry than is generally recognized and and other nuclear facilities even when they
represent a significant component in the are operating normally. It is often feared that
man-made radiation environment. even with the best design, proper handling
The principal applications include and techniques; some radioactivity is
industrial radiography, radiation routinely released into the air and water.
gauging, smoke detectors and However, dangers of radiation leakage are
self-luminous materials. Because most of
from possibility of accidents that could result
these applications entail the utilization of
in the release of radioactive material which
encapsulated sources, radiation exposures
raises the level of radioactive (ionizing)
would be expected to occur mainly externally
radiations. Such accidents took place at the
during shipment, transfer, maintenance, and
disposal. In the past decade, radiation ‗Chernobyl nuclear power plant‘ in USSR in
exposures in research and industrial 1986 and at the ‗Three Mile Island Power
applications were roughly half those due to
medical occupational exposure; hence, their
contribution to the direct population dose is
substantial.
Nuclear explorations
Nuclear explosions are a serious source
of radiations hazard. The effects of
atomic explosions in Nagasaki and
Hiroshima are still not forgotten.
Nuclear power
Nuclear explosion tests especially when
carried out in the atmosphere are a major
cause of radiation pollution. It is responsible
for increasing the background level of
radiation throughout the world. During
atmospheric nuclear explosion tests, a
number of long-lived radionuclides are
released into the atmosphere. This
radioactive dust (also known as radioactive
fallout) gets suspended in air at a height of 6
to 7 km above the earth‘s surface and is
dispersed over long distances by winds from
the test site. This radionuclide‘s often settle
down by rain and get mixed with soil and
water. From there they can easily enter the
food chain and finally get deposited in the
human body where they cause serious health
hazards. Some of the radioactive isotopes
RADIOACTIVE
CONTAMINATION
structure could helps avoid unnecessary of the natural radiation to which we are
medical X-rays. If we are all being struck by exposed has one chance in 1000
a million particles of radiation every minute, (30million/30 billion) of causing a cancer.
why don‘t we all develop cancer at an early Statistics show that our overall chance of
age? The reason we don‘t is not because this dying from cancer is one in five, so only one
level of radiation is ‗safe.‘‘ Even single in200 of all cancers may be due to natural
particle of radiation can cause cancer, but the radiation. The average exposure from a
probability for it to do so is very small, about nuclear power plant to those who live closest
one chance in 30 quadrillion (i.e., 30 million to it is about one percent of their exposure to
billion). Hence, the million particles that natural radiation; hence, if they live there for
strike us each minute have only one chance a lifetime, there is one chance in 100,000 that
in 30 billion of causing a cancer. A human they will die of cancer as a result of exposure
lifespan is about 30 million minutes; thus, all to radiation from the nuclear plant [12].
absorption. In addition, gamma radiation
external to the body can enter the skin and
RADIATION produce a dose various tissues [14]. Non
EFFECTS ionizing radiation refers to radioactive
energy which as opposed to produce charged
Radiation is the emission of particle or ions when passing through matters has
energy in wave form. This is stated as enough energy only for excitation. However
electromagnetic radiation. Examples consist it is known to cause biological effects. Non
of: visible light, radio waves, microwaves, ionizing radiations usually work together
infrared and ultraviolet lights, X-rays, and with tissue through the generation of heat.
gamma-rays [13]. Radiation can be described The hazard depends on the ability to go
as two basic types, ionizing and non-ionizing through the human body and the absorption
radiation. The discussion will include a characteristics of different tissues [15]. If
review of radiation of radioactivity. There are each and every one of these types of
three main kinds of ionizing radiation which radiation added by human activities can
are included alpha particles, beta particles cause radiation pollution. The meaning of
and gamma rays. Beside these there forms of radiation pollution is that while there are
ionizing also we have neutrons, protons, omnipresent sources of radiation, generally
heavy charged particles, X-ray and others. the high-energy radiations cause radiation
Radioactive substance can penetrate into the pollution with a serious health risk (such as
body by inhalation, in-gestation or dermal cancer or death) [16]. As has been mentioned
(
air pollution can caused by radioactivity control and mitigation of nuclear accidents,
which are in the air as gas or aerosols that as well as the control and minimization of
emit such ionizing radiation as alpha and personal expo-sure to radiation at an
beta particles, gamma rays, neutrons and individual level .Apart from being an
other high energy quanta. From the inevitable series of negative effects of
beginning of the life story the man has been radiations, it is the duty of humans with
exposed to ionizing radiations from regard to Radiation Standards Organizations
radioactive isotopes and other sources by to help in reducing the harmful effects of this
development of atomic reactor. This kind of kind of pollution. Radiation effects are also
pollution has been raised considerably classified in two other ways, namely somatic
[17,18]. Exposure radiation can cause tissue and genetic effects. Somatic effects appear in
and organ injury unless suitable precautions the exposed person. The delayed somatic
are taken. The more important health effects effects have a potential for the development
described as being caused by radioactive of cancer and cataracts. Acute somatic effects
isotopes are blood abnormalities, skin of radiation include skin burns, vomiting,
changes, bon changes and so forth. Physical hair loss, temporary sterility or sub fertility in
half-life of radioactive isotopes causes the men, and blood changes. Chronic somatic
amount of injury in human body. The most in effects include the development of eye
danger part of body is where have many cataracts and cancers. The second class of
actively dividing cells such as the skins, effects, namely genetic or heritable effects
intestine, gonads and tissues that grow blood appears in the future generations of the
cells [19]. The Radiation has most damaging exposed person as a result of radiation
effect on single celled organisms because a damage to the reproductive cells, but risks
single cell damaged by radiation can in a from genetic effects in humans are seen to be
roundabout way affect other cells in the considerably smaller than the risks for
individual. Cells which exposed with low somatic effects [20].
energy radioactivity can have biochemical RADIOACTIVE
repair system which can repeal some WASTE
damage. Actually it is good to mention that
all humans during their life are exposed to Radioactive waste, arising from
radiation in really small doses. Radioactive civilian nuclear activities as well as from
pollution is a vital ecological crisis. It could defence-related nu-clear-weapon activities,
be much worse if extreme caution is not poses a formidable problem for handling and
utilized in the handling and use of protecting the environment to be safe to t-he
radioactive material, and in the design and present and future generations. This article
operation of nuclear power plants .There are deals with this global problem in its varied
three basic tools that can provide protection aspects and discusses the cause for concern,
against a radiation source. These are time, the magnitude of the waste involved and
distance and shielding. The goal of the various solutions proposed and being
protection is to prevent over exposure from practised. As nuclear power and arsenal
external radiation and to minimize the en-try grow, continuous monitoring and
of radionuclides into the body or minimize immobilization of the waste over several
internal radiation. Controlling Radiation decades and centuries and deposition in safe
Pollution can be done at various levels, such repositories, assumes great relevance and
as usage and treatment of radiation waste, the importance [21].
lead-iron phosphate system loaded with highly radioactive spent fuel that must
simulated nuclear waste, were melted in the be regularly removed from operating
temperature range 750-950 degree. IAEA reactors. Low-level radioactive waste
published procedure for conducting generated by nuclear power plants,
probabilistic safety assessment for industry, hospitals, and other activities is
nonreactor nuclear facilities. This procedure also a long-standing issue because the
is consist of six interlinked steps, which spent fuel removed from a nuclear
include reactor is highly radioactive, it must be
Management and organization, disposed of in a way that protects the
Identification of source of radioactive environment from contamination and
releases, exposure and accident living organisms from exposure.
initiator Radioactive isotopes can be spread by
Scenario modelling, air or water, and can also become part of
Sequence quantification, the food chain. While the radioactivity
of spent fuel drops with time, according
Documentation of the analysis and
to a 1995 National Academy of Sciences
interpretation of the results
study, the ―peak risks [from a
Quality assurance
repository] might occur tens to hundreds
Figure 5. Protection against radioactive
of thou-sands of years or even farther
radiation.
The Holistic Approach to Environment 8(2018)2, 48-65 Page 62
G. Hazra Radioactive Pollution: An Overview
into thefuture.‖96 Isolating spent fuel June 3, 2008, and projected that the
from the environment is therefore a repository could begin receiving waste
highly demanding task—for in 2020, about 22 years later than the
comparison, human civilization has 1998 goal established by NWPA.
existed for only some 10,000 years. However, the Obama Administration
Several potential ways of handling spent had made a policy decision that the
fuel in the long term have been Yucca Mountain repository should not
proposed—none of which are ideal. be opened, largely because of Nevada‘s
These include burying the waste below continuing opposition, although it
the seabed, launching it into outer space, requested FY2010 funding to continue
and storing it on remote islands. the NRC licensing process. But the
However, the international scientific Administration‘s FY2011 budget
consensus is that spent fuel and other request reversed the previous year‘s
high-level waste should be stored plan to continue licensing the repository
underground in a ―geologic‖ repository, and called for a complete halt in funding
where the geological properties of the and elimination of the Office of Civilian
surrounding area would provide the Radioactive Waste Management
long-term stability needed to isolate the (OCRWM), which had run the program.
waste from the environment. The waste In line with the request, the FY2011
would sit inside tunnels drilled deep into Continuing Appropriations Act (P.L.
the earth. UCS concurs with this 11210) provided no DOE funding for
consensus, and believes that such a the program. DOE shut down the Yucca
repository—if properly sited and Mountain project at the end of FY2010 and
constructed—can protect the public and transferred OCRWM‘s remaining functions
the environment for tens of thousands of to the Office of Nuclear Energy. DOE filed a
years [28]. The Nuclear Waste Policy motion to withdraw the Yucca Mountain
Act of 1982 (NWPA, P.L. 97-425), as license application on March 3, 2010, ―with
amended in 1987, required the prejudice,‖ meaning the application could not
Department of Energy (DOE) to focus be resubmitted to NRC in the future [30].
on Yucca Mountain, Nevada, as the site
of a deep underground repository for
spent nuclear fuel and other highly
radioactive waste. The state of Nevada
has strongly opposed DOE‘s efforts on
the grounds that the site is unsafe,
pointing to potential volcanic activity,
earthquakes, water infiltration,
underground flooding, nuclear chain
reactions, and fossil fuel and mineral
deposits that might encourage future
human intrusion. Under the George W.
Bush Administration, DOE determined
that Yucca Mountain was suitable for a
repository and that licensing of the site
by the Nuclear Regulatory Commission
(NRC) should proceed, as specified by
NWPA [29]. DOE submitted a license
application for the repository to NRC on
The Holistic Approach to Environment 8(2018)2, 48-65 Page 63
G. Hazra Radioactive Pollution: An Overview
Figure 6.
if hot particles are present. Doses of several location can be very substantially different.
millisieverts a year could result from some of There is also no simple correlation with
the most contaminated sites. The levels of contamination levels and distance from the
floodplain contamination are very variable; discharge.
samples taken at the same approximate
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