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Sounds Waves and Fluctuations in One-Dimensional Supersolids
Sounds Waves and Fluctuations in One-Dimensional Supersolids
ations, and phase fluctuations of the two gapless bands. Our results are presented for two distinct supersolid
models: a dipolar Bose-Einstein condensate in an infinite tube and a dilute Bose gas of atoms with soft-core in-
teractions. Characteristic energy scales are identified, highlighting that these two models approximately realize
the bulk incompressible and rigid lattice supersolid limits.
ing transition, leading to a relatively rigid lattice. These two occurs depends on ω and ρ, and the transition can be contin-
cases are conveniently distinguished by comparing the energy uous or discontinuous. In the results we present here are for
164
scales associated with the isothermal compressibility at con- Dy atoms with add = 130.8 a0 and ω/2π = 150 Hz.
stant strain and the longitudinal elastic modulus of the lattice.
The outline of the paper is as follows. In Sec. II we briefly
introduce the dipolar and soft-core systems we use in this B. 1D soft-core Bose gas
work. The supersolid Lagrangian is introduced in Sec. III
and we discuss the how to obtained the elastic parameters that Our second system is a BEC of atoms free to move in 1D,
appear in the Lagrangian. In Sec. IV we derive the hydro- but interacting via a soft-core interaction potential Usc (x) =
dynamic behavior of the excitations from the Lagrangian and U0 θ(asc − |x|), where asc is the core radius and U0 is the
use this to determine the speeds of sound. We then make a potential strength [see Fig. 1(b)]. It conventional to define the
detailed comparison to calculations of the two models, and dimensionless interaction parameter
explore the limiting behavior of the predictions. The density
fluctuations are discussed in Sec. V. Here a focus is on the 2ma3sc U0 ρ
decomposition of the fluctuations into components related to Λ= , (3)
ℏ2
tunneling of atoms between sites (defect density fluctuations)
and due movement of the crystal lattice (lattice strain fluctu- and continuous transition occurs from a uniform to a modu-
ations). Finally, in Sec. VI we discuss the phase fluctuations lated state at the critical value Λc = 21.05. Further details
before concluding in Sec. VII. about this model are given in Appendix A 2.
We consider two zero-temperature systems that undergo a By solving the (generalized) Gross-Pitaevskii equations for
transition to a 1D crystalline state. The models are briefly in- these models we determine the energy minimising wavefunc-
troduced in the following two subsections. Additional details tion ψ0 . These solutions can be found in a single unit cell of
of the models and numerical solution method are given in Ap- length a along x. If the state is crystalline, then a is the lattice
pendix A. Apart from the microscopic parameters particular constant (for uniform states the energy is independent of a).
to each model, we consider both systems in a thermodynamic Take E to be the energy per unit length of this state for den-
limit with a specified density per unit length ρ. sity ρ and lattice constant a (as defined in Appendix A). In the
thermodynamic limit where the system is free to choose the
microscopic length a to minimise the energy, the ground state
A. Dipolar Bose gas in a tube potential is
Our first system is a Bose gas of magnetic atoms confined E0 (ρ) = min E(ρ, a), (4)
a
in a tube shaped potential [see Fig. 1(a)]. The single particle
Hamiltonian is which can be used to implicitly determine a(ρ) as the value of
a that minimises E at density ρ.
ℏ2 ∇ 2 1
Hsp = − + mω 2 (y 2 + z 2 ), (1)
2m 2
III. SUPERSOLID LAGRANGIAN
where ω is the transverse harmonic confinement angular fre-
quency, and the atoms are free to move along the x-axis. The
atomic dipole moments are polarized along z by a bias field A. Quadratic Lagrangian density
and the interactions are described by the potential
Here our interest is in a Lagrangian description of the low-
4πas ℏ2 3add ℏ2 z2
energy, long-wavelength features of a system where 1D crys-
U (r) = δ(r) + 1−3 2 , (2)
m mr3 r talline order can occur along the x-direction. We work in a
thermodynamic limit where the ground state is determined by
where as is the s-wave scattering length, add = the average linear number density ρ in addition to the inter-
mµ0 µ2m /12πℏ2 is the dipole length, and µm is the atomic action and relevant transverse confinement parameters. Long-
magnetic moment. The ratio ϵdd = add /as characterises wavelength perturbations of the ground state can be character-
the relative strength of the dipole-dipole to s-wave interac- ized by three fields: {δρ(x, t), u(x, t), ϕ(x, t)}. Here δρ(x, t)
tions. When this parameter is sufficiently large the ground denotes variations in the average density, u denotes the defor-
state undergoes a transition to a crystalline state with mod- mation field of the crystal lattice along the x direction (relative
ulation along x. Quantum fluctuation effects are necessary to the unstrained ground state), and ϕ denotes the superfluid
to stabilize this state and further details about this model are phase field. For treating small departures from equilibrium
given in Appendix A 1. The value of ϵdd where the transition the Lagrangian density can be expanded to quadratic order in
3
these fields as dimensional crystals the αuu term generalizes to the elastic
αρρ αuu tensor. For the 1D crystal αuu can also be identified as the
L = − ℏ δρ ∂t ϕ − (δρ)2 − (∂x u)2 − αρu δρ ∂x u layer-compressibility used to characterize smectic materials
2 2
1 ℏ 2 ℏ2 [19, 35]. Finally, we define the density-strain coupling pa-
+ mρn ∂t u − ∂x ϕ − ρ (∂x ϕ)2 , (5) rameter by the mixed partial derivative
2 m 2m
2
where ρn is the normal density, with ρ = ρs + ρn , and ρs be- ∂ E
αρu = a . (11)
ing the superfluid density. Similar forms of Lagrangian den- ∂ρ∂a
sities have been obtained by other authors (e.g. see [18–22]),
although here we follow the approach of Yoo and Dorsey [18].
A discussion about the relationship between these treatments IV. EXCITATIONS AND SPEEDS OF SOUND
is given in Refs. [18, 19]. The phase gradient relates to the
ℏ In this section we consider the collective excitations of the
superfluid velocity as vs = m ∂x ϕ and the normal velocity
relates to the time-derivative of the lattice deformation field gapless energy bands. We begin by deriving hydrodynamic
vn = ∂t u [17, 18]. results for the collective modes, and the associated speeds of
sound. We then compare these to results for our two models,
and consider the limiting behavior.
B. Generalized elastic parameters
In addition to the superfluid density, which determines the A. Hydrodynamic equations of motion and collective modes
rigidity of the state to twists in the phase ϕ [31], three other
generalized elastic parameters of the system {αρρ , αρu , αuu } The Euler-Lagrange equations obtained from Eq. (5) are
also appear in Eq. (5). Here we discuss how these can be
obtained from ground state calculations. ℏ∂t ϕ = −αρρ δρ − αρu ∂x u, (12)
For 1D crystals the superfluid fraction fs = ρs /ρ has ρn (m∂t2 u − ℏ∂tx ϕ) = αuu ∂x2 u+ αρu ∂x δρ, (13)
−1 ℏ
∂t δρ = −ρn ∂tx u − ρs ∂x2 ϕ.
Z
a dx (14)
fs+ = R , (6) m
ρ uc dy dz |ψ0 |2
Z Z −1 These describe the hydrodynamic evolution for small depar-
a dx
fs− = dy dz 2
, (7) tures from equilibrium.
ρ uc |ψ0 | We look for normal mode solutions of Eqs. (12) - (14) of
as upper and lower bounds, respectively [32, 33]. Hereon, the form X(x, t) = Xw ei(qx−ωt) , where X denotes our three
we neglect the transverse coordinates (y, z) when applying fields appearing in the Lagrangian and q is a quasimomentum.
results to the soft-core case. Both bounds are identical for The resulting linear system is
the soft-core case, and provide the exact superfluid fraction
δρw
(e.g. see [27]). For the dipolar case the bounds are close to M ϕw = 0, (15)
each other and taking fs = 12 (fs+ + fs− ) provides an accurate uw
estimate of the superfluid fraction (see [34]).
The other generalized elastic parameters can be determined where
from the energy density E(ρ, a), for the ground state under
the constraint of lattice constant being a and the mean density αρρ −iℏω iqαρu
being ρ. The first elastic parameter is defined by M = iℏω ℏ2 q 2 ρs /m −ℏωqρn . (16)
2 2
2 iqαρu ℏωqρn ω ρn m − q αuu
∂ E
αρρ = , (8) Nontrivial solutions require the matrix M to be singular, i.e. its
∂ρ2 a
determinant ∆M must be zero, where
and relates to the isothermal compressibility at constant strain:
∆M = mℏρn (ω 2 − c2+ q 2 )(ω 2 − c2− q 2 ). (17)
1
κ̃ = 2 . (9) Here we have introduced
ρ αρρ
1
q
The second parameter describes the effects of straining a site mc2± = (a∆ ± a2∆ − 4b∆ ), (18)
at constant density 2
2 where
2 ∂ E
αuu = a . (10) αuu
∂a2 ρ a∆ = ραρρ − 2αρu + , (19)
ρn
Noting that lattice strain, given by ∂x u, relates to changes ρs 2
b∆ = (αρρ αuu − αρu ). (20)
in the lattice constant according to δa/a = ∂x u. In higher ρn
4
0.5
ω± = c± q, (21)
1
We compare the speeds of sound determined from direct
calculation of the excitations to the hydrodynamic result of 0.8
Eq. (18) in Figs. 2 and 3 for the dipolar and soft-core systems,
respectively. The direct calculation of the excitations involves 0.6
1 ters are shown in Figs. 2(d) and 3(d). These results reveal that
(a) the crystal-dependent elastic terms αρu and αuu both vanish
as we approach the transition from the modulated side. For
0.5
both systems we find that ραρu is typically smaller than αuu ,
suggesting that neglecting this parameter can be a reasonable
0 first approximation. The parameter αρρ is non-zero in both
16
(b) phases, but changes discontinuously at the transition (also see
[37]).
14
12
C. Supersolid sound limiting behavior
10
0.4
being the bulk compressibility and lattice compressibility
energies, respectively, defining the associated characteristic
0.2
speeds cκ and cu . Here
0
αuu
-0.2 κ= , (25)
ρ2 (αρρ αuu − αρu
2 )
For the dipolar case cκ > cu , while the soft-core case instead 1.5
has cκ < cu [see Figs. 2(d) and 3(d)]. (a)
These results emphasize an important difference between
the two models we consider. The crystalline phase of
the dipolar system is dominated by the compressive energy 1
(i.e. mc2κ > mc2u ), while the soft-core system is dominated by
the lattice compressive energy.
140 the frequency of the upper excitation band for dipolar (soft-
core) model. These results confirm that the excitations in this
120
band are closely related to the classical crystal phonon modes.
100
80 V. DENSITY FLUCTUATIONS
4
60 2
We are interested in the density fluctuations caused by the
40 0 quasiparticles of the gapless bands. To do this we examine the
-4 -2 0 2 4
effect of adding an excitation with band index ν and quasimo-
20 mentum q to the condensate with a small coherent amplitude
cνq , i.e.
0
25
ψ(x) = ψ0 (x) + cνq uνq (x) − c∗νq vνq
∗
(x). (38)
20 In particular, we will consider the changes in the linear density
Z
15 ϱ(x) = dy dz |ψ(x)|2 , (39)
4
0
0 0.1 0.2 0.3 0.4 0.5 A. Total density fluctuation
5000
4000
3000
2000
1000
0
0.2
0.1
4500
0
4000
-0.1 3500
-0.2 3000
5.3 5.4 5.5 5.6 5.7 5.8 5.9 6 6.1 6.2
100
-100
-10 -5 0 5 10
0.3 1 1
200
150 0.2
0 0 0 0
0 0.1 0.2 0.3 0.4 0 0.1 0.2 0.3 0.4 0 0.1 0.2 0.3 0.4 0 0.1 0.2 0.3 0.4
FIG. 6. Effect of an excitation on the density fluctuations of a dipolar supersolid with ϵdd = 1.43. (a) The ground state density ϱ0 (x) (black)
and density ϱ(x) (red) when perturbed by a ν = 1 excitation with q = 2π/9a and cνq = 5. The purely-deformed density profile ϱu (x)
(blue) using the deformation field determined from the quasiparticle. Vertical lines indicate the lattice locations for the ground state (x0j ,
grey lines) and the perturbed state (xj , light red lines). (b) The deformation field u(x) associated with the perturbed state from (a). Small
circle markers indicate the deformation of the density maxima of ϱ(x). Inset: close up of a density peak showing the identification of u(x).
(c) A comparison of the total, lattice deformation, and defect density fluctuations projected to the first Brillouin zone (see Appendix B). (d)
Excitations frequencies for the lowest two bands comparing BdG (solid) and hydrodynamic [i.e. ωνq = cν q] (dashed) results. Marker identifies
the excitation used in subplots (a)-(c). (e)-(f) The density fluctuations comparing the BdG (solid) and hydrodynamic (dashed) results.
(i.e. maxima of ϱ). The displacement field can be expressed on a supersolid state with equilibrium density profile ϱ0 (x).
as Assuming that the atom number in each cell remains constant
then the purely-deformed density profile is given by
u(x) = 2Re{cνq uνq eiqx }. (42)
where the amplitude uνq is a measure of how the quasiparticle ϱu (x) = ϱ0 (x − u(x))(1 − ∂x u(x)), (43)
displaces the site at the origin3 . In Fig. 6(b) we show (42) for
where the first factor describes the displaced density profile
the perturbed density of Fig. 6(a), and give an example of its
and second factor adjusts the envelope of density profile to
relationship to the site displacements [inset to Fig. 6(b)].
keep the atom number per cell constant. The change in cell
To understand the effect of lattice deformation on the den-
width, i.e. strain, leads to a change in density across the sys-
sity we consider a weak displacement field of the form (42)
tem, giving rise to the lattice strain density fluctuation. Fourier
transforming δϱu (x) ≡ ϱu (x) − ϱ0 (x) for a single quasipar-
ticle yields [cf. Eq. (41)]
3 In calculations we evaluate uνq = −δρ′νq (0)/ϱ′′ (0), where the prime is
R 0
derivative with respect to x and δρνq (x) = dy dz ψ0 [uνq − vνq ] δ ρ̃u,νq = −iqρuνq L, (44)
9
and δ ρ̃u,ν−q = δ ρ̃∗u,νq as the nonzero contributions in the first band (ν = +, red) has weak defect density fluctuations, and
Brillouin zone. In Eq. (44) L is the length of the x region the strain density fluctuation makes the dominant contribution
integrated over. to the total density fluctuation. Hence the second band can be
We illustrate the lattice strain density fluctuation construc- considered a crystal-like excitation, consistent with the con-
tion in Fig. 6. Using the identified deformation field u(x) clusions from the linear-chain model presented in Sec. IV D.
[Fig. 6(b)], in Fig. 6(a) we show the purely-deformed den-
sity profile ϱu (x), with associated density fluctuation shown
in Fig. 6(c). 10 1
0.25
10 0
0.2
In Figs. 9(a) and (b) we show examples of Sϕ,ν (q) com-
10 -1 0.15
puted from the BdG results for the dipolar and soft-core super-
0.1 solid states, respectively. We also confirm that the hydrody-
10 -2
0.05 namic results agree in the q → 0 limit. In Figs. 9(c)-(f) we ex-
10 -3 0 amine the hydrodynamic limiting behavior of the fluctuations
1.5
[i.e. comparing ξϕν to limq→0 q/2Sϕ,ν (q)] crossing the transi-
10 1
tion for both models. In the uniform superfluid state ξϕ+ → ξκ ,
1 being identical to the length scale for the total density fluctua-
10 0
tions in the same regime. In the dipolar supersolid the ν = −
band exhibits stronger phase fluctuations close to the transi-
0.5 10 -1
tion, but as ϵdd increases the phase fluctuations of the ν = +
band eventually dominates. For the soft-core supersolid the
10 -2
0
1.4 1.45 1.5 20 40 60 80
ν = + band dominates the phase fluctuations everywhere.
We note that the Fourier component of the superfluid ve-
locity field is revealed from the phase fluctuations as vνq =
FIG. 9. Phase fluctuations. (a), (b) Comparison of the phase fluctu- iℏqϕq /m, and thus our results are trivially extendible to de-
ations as a function of q obtained from the BdG calculations (solid) scribe the superfluid velocity fluctuations (also see [39]). The
to the hydrodynamic limit ξϕ± (dashed) for the lowest two bands (a) character of quasiparticle effect on the phase or velocity has
dipolar and (b) soft-core supersolids. (c)-(f) Strengths of the hydro- been employed to characterise the bands and excitations of
dynamic regime total density ξρ± (black line) and phase ξϕ± (green dipolar supersolids (e.g. see [5, 42]). However, these char-
line) correlation lengths for a dipolar supersolid, compared to the acterizations involve quantifying the phase variations distin-
relevant limits limq→0 1/[2qSϕ,ν (q)] (markers). Results for the (c) guishing between the high and low density regions of the su-
ν = −1 and (e) ν = +1 bands of a dipolar supersolid, with other persolid within the unit cell, and are thus beyond the hydro-
parameters as in Fig. 2. In both subplots we show ξκ for reference. dynamic description.
Results for (d) ν = −1 and (f) ν = +1 bands of a soft-core super-
solid, with other parameters as in Fig. 3. In (e) and (f) the ξϕ+ and
ξρ+ are identical for the uniform phase, and are indicated by dashed
VII. OUTLOOK AND CONCLUSIONS
lines. Also, the modulated results from (c) and (d) are repeated as
light dash-dot lines.
In this study, we have demonstrated the effectiveness of the
supersolid Lagrangian formalism in providing a quantitative
For a single quasiparticle, the only non-zero fluctuations are description of the hydrodynamic characteristics of dipolar and
at wavevectors q and −q, with [cf. Eq. (41)] soft-core supersolids. The Lagrangian description depends on
Z a number of elastic parameters and we have discussed how
uνq (x) + vνq (x) these can be extracted from ground state calculations. Our
ϕ̃νq = dx e−iqx . (57)
2iψ0 (x) findings include a comparative analysis of the Lagrangian the-
ory to the BdG excitations for the speeds of sound, density and
The strength of the phase fluctuations are given by the dimen- phase fluctuations. The excellent agreement shows that the
sionless quantity hydrodynamic behaviour is well-described by the Lagrangian.
ρ Also, these results underscore the distinct behaviors exhibited
Sϕ,ν (q) = |ϕ̃νq |2 . (58) by dipolar and soft-core models.
L
To unravel these distinctions, we have considered various
Similar to the treatment of density functions, from the limiting properties of the Lagrangian theory and how these
quadratic Lagrangian we obtain the phase response function apply to the two models. This has brought to light the signif-
1 X 1 icance of two energy scales, mc2κ and mc2u , which delineate
χ′′ϕ (q, ω) = Nπ [δ(ω − cν q) − δ(ω + cν q)], (59) the relative impacts of bulk and lattice compressibility, respec-
2 ξϕν q
ν tively. The incompressible limit (mc2κ ≫ mc2u ) applies to the
12
dipolar supersolid, while the rigid lattice limit (mc2κ ≪ mc2u ) where
applies to the soft-core supersolid. Our results illuminate how Z
these distinct limits manifest in the excitation spectrum, den- Φ(x) = dx′ U (x − x′ )|ψ(x′ )|2 , (A2)
sity, and phase fluctuations.
It is interesting to consider how our predictions can be ver- and the effects of quantum fluctuations p are described by
ified in experiments. Recently, the work of Šindik et al. [25] the term with coefficient γQF = 32 3 gs a3s /πQ5 (ϵdd ), with
proposed a scheme for measuring the excitations and density R1
Q5 (x) = ℜ{ 0 du[1+x(3u2 −1)]5/2 } [49]. The energy func-
response of a dipolar supersolid with minimal finite size ef- tional is evaluated in a single unit cell of length a along x (and
fects. Their scheme involves the use of a toroidal potential integrated over all space in the transverse directions). The ef-
for confinement with a well-defined mean density, and an az- fective potential arising from interactions, Φ(x), is evaluated
imuthally varying perturbing potential to excite q → 0 excita- using a truncated interaction kernel (see Ref. [34] for details).
tions. Observing the density oscillations following the sudden The energy minimising wavefunction for (A1) is determined
removal of the potential can be used to determine the speeds using the gradient flow (or imaginary time) evolution [50, 51],
of sound and the amplitude of the density response. Deter- noting that the average density condition enforces the follow-
mining the lattice strain and defect density fluctuations may ing normalization constrain on the wavefunction
be possible with high-resolution in situ imaging which have Z
already been used in experiments to characterize excitations
[11] (also see [43, 44]). dx |ψ(x)|2 = ρa. (A3)
uc
Our results describe the zero temperature fluctuations and
an important extension of this work is to include finite tem- As a result we obtain E(ρ, a), i.e. the minimising energy as
perature effects (see Refs. [18, 19]). Another area of inter- a function of density and cell size. We discuss the energy
est is higher dimensional supersolids where an elastic tensor density function and identifying the ground state in Sec. A 3.
describes the crystal, and the shear modulus will become rele-
vant. Of interest is the two-dimensional supersolid that has re-
cently been produced in experiments with a dipolar BEC [45]. 2. 1D soft-core formalism
In the thermodynamic limit the ground state phase diagram
for this case has been determined [46, 47], yet the excitations The stationary states are determining by minimising the
remain largely unexplored. This system is expected to have meanfield functional of the state
three gapless branches [6] (cf. [7]) with the emergence of a Z
ℏ2 d2 1
transverse crystal mode. E[ψ, a] = dx ψ ∗ − + Φ sc (x) ψ, (A4)
uc 2m dx2 2
Note added. As we were about to submit, the preprint
Ref. [48] appeared, which also considers the elastic proper- where the integration is over a unit cell along x of length a,
ties of softcore supersolids. and
Z
Φsc (x) = dx′ Usc (x − x′ )|ψ(x′ )|2 . (A5)
ACKNOWLEDGMENTS
To implement the average density constraint on the stationary
PBB acknowledges useful discussions with J. Hofmann and states ψ has the normalization condition
use of New Zealand eScience Infrastructure (NeSI) high per- Z
formance computing facilities. LMP, DB and PBB, acknowl- dx |ψ(x)|2 = ρa. (A6)
edge support from the Marsden Fund of the Royal Society of uc
New Zealand. Identical to the dipolar case, we obtain the minimum energy
per unit cell E(ρ, a), by applying gradient flow algorithm op-
timise the energy functional Eq. (A4) against the wavefunc-
Appendix A: Additional details on supersolid models tion.
We only need to obtain E(ρ, a) for values of a close to the is the (constant) mean linear density. We also define the pro-
ground state value at each density, since the elastic param- jected total density fluctuation [shown in Fig. 6(c)]
eters involve derivatives evaluated at the ground state value.
We also note that in situations where the stationary state is δ ϱ̄(x) = PBZ δϱ(x), (B2)
uniform E independent of a.
where for an excitation of quasimomentum q only the ±q
wavevectors contribute following projection, i.e.
Appendix B: Projected density fluctuations
δ ϱ̄(x) = 2Re{cνq δ ρ̃νq eiqx /L}, (B3)
We reveal the long-wavelength character of the density fluc- with δ ρ̃νq as defined in Eq. (41). We can similarly project the
tuations by projecting them to the first Brillouin zone with the density fluctuations δϱu (x) and δϱ∆ (x) to obtain δ ϱ̄u (x) and
operation δ ϱ̄∆ (x), respectively [also shown in Fig. 6(c)]. These satisfy
X 1Z ′
similar relations to (B3) but in terms of δ ρ̃u,νq and δ ρ̃∆,νq ,
PBZ f (x) = dx′ eik(x−x ) f (x′ ), (B1) respectively. For lattice strain density fluctuation this is
L
k∈BZ
δ ϱ̄u (x) = 2Re{−iqρcνq uνq eiqx }, (B4)
where BZ denotes wavevectors in the range [−π/a, π/a]. For
the unperturbed linear density only the constant (k = 0) term where we have used (44). From this we see that δ ϱ̄u (x) =
survives projection ρ = PBZ ϱ0 (x), i.e., the projected density −ρ ∂x u with u given by Eq. (42) [52].
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