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270-3
Selected Values of Chemical

Thermodynamic Properties
Tables for the First Thirty-Four Elements
In the Standard Order of Arrangement
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U.S. DEPARTMENT OF COMMERCE
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THE NATIONAL BUREAU OF STANDARDS
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maximum application of the physical and engineering sciences to the advancement of technology in
industry and commerce. Its responsibilities include development and maintenance of the national stand-
ards of measurement, and the provisions of means for making measurements consistent with those
standards; determination of physical constants and properties of materials; development of methods
for testing materials, mechanisms, and structures, and making such tests as may be necessary, particu-
larly for government agencies; cooperation in the establishment of standard practices for incorpora-
tion in codes and specifications; advisory service to government agencies on scientific and technical
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to industry, business, and consumers in the development and acceptance of commercial standards and
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UNITED STATES DEPARTMENT OF COMMERCE
Alexander B. Trowbridge, Secretary
NATIONAL BUREAU OF STANDARDS • A. V. Astin, Director
NBS TECHNICAL NOTE 270-3

ISSUED JANUARY 1968
Selected Values of Chemical Thermodynamic Properties
Tables for the First Thirty-Four Elements

in the Standard Order of Arrangement
D. D. Wagman, W. H. Evans, V. B. Parker,
I. Halow, S. M. Bailey, and R. H. Schumm
Institute for Basic Standards

National Bureau of Standards
Washington, D.C. 20234
This Technical Note supersedes Technical Notes 270-1 and 270-2

|_ J
NBS Technical Notes are designed to supplement the

Bureau's regular publications program. They provide a
means for making available scientific data that are of
transient or limited interest. Technical Notes may be
listed or referred to in the open literature.
For sale by the Superintendent of Documents, U.S. Government Printing Office

Washington, D.C, 20402 - Price $1.25
^
PREFACE
Technical Note 270-3 is the third in a series of publications
containing material prepared as a revision of the tables of Series I
of National Bureau of Standards Circular 500, Selected Values of
Chemical Thermodynamic Properties, by F. D. Rossini, D. D.
Wagman, "W. H. Evans, S. Levine, and I. Jaffe. This Note extends
the revision to Tables 23, 33, and 34, covering the compounds
of the elements carbon, zinc, and cadmium in the Standard Order of
Arrangement. In addition this Note contains all of the Tables of
Technical Note 270-1 and 270-2, including corrections for a number
of minor errors. Thus this Note supersedes Technical Notes
270-1 and 270-2.
Donald D. Wagman, Chief

Thermochemistry Section.
Ill
CONTENTS
Preface III
Introduction 1
Table A Conversion Factors „ 7

Table 1 Oxygen 1 1
Table 2 Hydrogen 12
Table 3 Helium 15
Table 4 Neon 16
Table 5 Argon 17
Table 6 Krypton 18
Table 7 Xenon 19
Table 8 Radon 20
Table 9 Fluorine 21
Table 10 Chlorine 24
Table 11 Bromine 31
Table 12 Iodine 36
Table 13 Astatine 42
Table 14 Sulfur ___ 43
Table 15 Selenium 56
Table 16 Tellurium 58
Table 17 Polonium . 60
Table 18 Nitrogen 61
Table 19 Phosphorus 84
Table 20 Arsenic 95
Table 21 Antimony 99
Table 22 Bismuth 103
Table 23 Carbon 106
Table 24 Silicon 171
Table 25 Germanium 177
Table 26 Tin 181
Table 27 Lead 187
Table 28 Boron 196
Table 29 Aluminum 207
Table 30 Gallium 2 18
Table 31 Indium 223
Table 32 Thallium 227
Table 33 Zinc 233
Table 34 Cadmium 248
Appendix 262
Table B 263
Index 264
W
SELECTED VALUES OF CHEMICAL THERMODYNAMIC PROPERTIES
by
Donald D. Wagman, William H. Evans, Vivian B. Parker,

Iva Halow, Sylvia M„ Bailey, and Richard H. Schurnm
INTRODUCTION
Substances and Properties Included in the Tables
The tables contain values where known of the enthalpy and Gibbs
energy of formation, enthalpy, entropy and heat capacity at 298.15°K
(2 5°C), and the enthalpy of formation at 0°K, for all inorganic substances
and organic molecules containing not more than two carbon atoms. In
some instances such as metal-organic compounds, data are given for
substances in which each organic radical contains one or two carbon
atoms.
No values are given in these tables for metal alloys or other
solid solutions, fused salts, or for substances of undefined chemical
composition.
Physical States
The physical state of each substance is indicated in the column

headed "State" as crystalline solid (c), liquid (liq), glassy or amorphous
(amorp), or gaseous (g). Solutions in water are listed as aqueous (aq).
For non -aqueous systems the physical state is that normal for the
indicated solvent at 298.15°K.
Definition of Symbols
The symbols used in these tables are defined as follows: P =

pressure; V = volume; T = absolute temperature; E = intrinsic or
internal energy; S = entropy; H = E + PV = enthalpy (heat content);
G = H - TS = Gibbs energy (formerly the free energy); C p = (dH/dT)p =
heat capacity at constant pressure.
Conventions Regarding Pure Substances
The values of the thermodynamic properties of the pure substances

given in these tables are for the substances in their standard states
(indicated by the superscript c on the thermodynamic symbol). These
standard states are defined as follows:
For a pure solid or liquid, the standard state is the substance
in the condensed phase under a pressure of one atmosphere.
For a gas the standard state is the hypothetical ideal gas at unit
fugacity, in which state the enthalpy is that of the real gas at the same
temperature and at zero pressure.
The values of A Hf c and AGf° given in the tables represent the change
in the appropriate thermodynamic quantity when one gram -formula
weight of the substance in its standard state is formed, isothermally at
the indicated temperature, from the elements, each in its appropriate
standard reference state. The standard reference state at 25 °C for
each element except phosphorus has been chosen to be the standard
state that is thermodynamically stable at 25 °C and at one atmosphere
pressure. For phosphorus the standard reference state is the crystalline
white form; the more stable forms have not been well characterized
thermochemically. The same reference states have been maintained for
the elements at °K except for the liquid elements bromine and mercury,
for which the reference states have been chosen as the stable crystalline
forms. The standard reference states are indicated in the tables by the
fact that the values of A Hf° and A Gf ° are exactly zero.
The values of H^ q „ -Hq represent the enthalpy difference for the
given substance between 298.15 C K and 0°K. If the indicated standard
state at 25 °C is the gas, the corresponding state at C
K is the hypo-
thetical ideal gas; if the state at 25 °C is solid or liquid, the corres-
ponding state at C
K thermodynamically "stable crystalline
is the
solid, unless otherwise specifically indicated.
The values of S represent the virtual or "thermal" entropy of the
c
substance in the standard state at 298.15°K, omitting contributions from

nuclear spins. Isotope mixing effects, etc. are also excluded except
,
in the case of the hydrogen-deuterium ( H- H) system. Where data have

been available only for a particular isotope, they have been corrected
when possible to the normal isotopic composition.
The values of the enthalpies of formation of gaseous ionic species
are computed on the convention that the value of &Hf ° for the electron
is zero. Conversions between and 2 Q 8.15°K are calculated using
the value of H^ng-HA = 1. 481 kcal per mole of electrons, and assuming
that the values of H^gg-Hg for the ionized and un-ionized molecules are
the same.
Conventions Regarding Solutions
Solutions in water are designated as aqueous (aq); other solvents

are designated by name or chemical formula. The concentration of the
solution is expressed in terms of the number of moles of solvent asso-
ciated with one mole of the solute. If no concentration is indicated, the
solution is assumed to be "dilute".
The standard state for a solute in aqueous solution is taken as the
hypothetical ideal solution of unit molality (indicated as "std. state,
m = 1"). In this state the partial molal enthalpy and heat capacity of the
solute are the same as in the infinitely dilute real solution. For non-
aqueous solutions the standard state of the solute is the hypothetical
ideal solution of unit mole fraction of solute ("std. state, X£ = 1").
The value of A Hf ° given in the tables for a solute in its standard
state is the apparent molal enthalpy of formation of the substance in
the infinitely dilute real solution. At this dilution the partial molal
enthalpy is equal to the apparent molal quantity. At concentrations
other than the standard state, the value of A Hf ° represents the apparent
enthalpy of the reaction of formation of the solution from the elements
comprising the solute, each in its standard reference state, and the
appropriate total number of moles of solvent. In this representation
the value of A Hf ° for the solvent is not required. The experimental value
for a heat of dilution is obtained directly as the difference between the
two values of A Hf ° at the corresponding concentrations.
The values of the thermodynamic properties tabulated for the
individual ions in aqueous solution are based on the usual convention
p
1
that the values of AHf°, AGf°, S° and C ° for H" (aq, std. state,
"
m = 1)
are zero. The properties of a neutral electrolyte in aqueous solution
in the standard state are equal to the algebraic sum of these values for
the appropriate kinds and number of individual ions assumed to constitute
the molecule of the given electrolyte. When the undissociated species,
rather than the sum of the ions, is meant, the notation "undissociated"
or "un-ionized" is used. For an ionic species the properties tabulated
refer to that undissociated ion. By adopting the above convention with
respect to aqueous H , it follows that the thermodynamic relation A Gf
°
= A Hf ° - T A Sf ° will not hold for an individual ionic species. However

no problem arises when neutral chemical systems are considered.
Unit of Energy and Fundamental Constants
All of the energy values given in these tables are expressed in terms
of the thermochemical calorie. This unit, defined as equal to 4.1840
joules, is generally accepted for the presentation of chemical thermo-
dynamic data. Values reported in other units have been converted to
calories by means of the conversion factors for molecular energy given
in Table A.
The following values of the fundamental physical constants have
been used in these calculations:
R = gas constant = 8. 3143 + 0. 0012 J/deg mol =, 1.98717 + 0. 00029
cal/deg mol
F = Faraday constant = 96487.0 + 1. 6 coulombs/mol
±0.4 cal/volt equivalent
= 23060.9
Z = Nhc = 11. 00107 J/cm" 1 mol = 2. 85912 ± 0. 00026 cal/cm" 1
96258 + 0. r
C£ = second radiation constant = hc/k = 1.43879 i 0.00015 cm deg
C = 273.15°K
C
These constants are consistent with those given in the Table of General
Physical Constants, recommended by the National Academy of Sciences -
National Research Council The formula weights in the tables have
.
been calculated for the molecular formula given in the Formula and
Description column using the 1961 Table of Relative Atomic Weights based
on the atomic mass of i(i C = 12 exactly .
Internal Consistency of the Tables
All of the values given in these tables have been calculated from
the original articles, using consistent values for all subsidiary and
auxiliary quantities. The original data were corrected where possible
for differences in energy units, molecular weights, temperature scales,
etc. Thus we have sought to maintain a uniform scale of energies for
all thesubstances in the tables. In addition the tabulated values of the
properties of a substance satisfy all the known physical and thermodynamic
relationships among these properties. The quantities A Hf °, A Gf°, and
S° at 298.15°K satisfy the relation:
A Gf° = A Hf° - T A Sf°.
NBS Technical News Bulletin, October 1963.

>
'A. E. Cameron and E. Wichers, J. Am. Chem. Soc. 84, 4192 (1962).
Furthermore any thermodynamic quantity for a
the calculated value of
reaction is independent of the path chosen for the evaluation.
In some cases newer data may have become available on certain
substances after the values were selected for these tables. Because
of the need to maintain the internal consistency of the tables, it is not
always possible to incorporate these newer data into the tables without
a detailed analysis of the effect of such a change. Unless great care is
used, relatively significant errors in calculated values of A H° or A G°
for specific reactions may result from the introduction of such data.
Uncertainties
The uncertainty any value in the tables depends on the uncertain-

in
ties of all the determinations in the total chain of reactions used to
establish the value.
A discussion of the uncertainties will be included in the final
publication of these tables in the National Standard Reference Data
System. However we have followed certain rules with respect to
significant figures to indicate these uncertainties. Values are tabulated
in general such that the overall uncertainty lies between 2 and 20 units
of the last figure. On the other hand, values are given so that the
experimental data from which they are derived may be recovered with
an accuracy equal to that of the original quantities. Thus the number
of significant figures for any one value in the tables need not represent
the absolute accuracy of that value. For solutions of varying composition
values are frequently tabulated to more figures to make possible the
recovery of enthalpies of solution and dilution. Similarly values of
A HfQ and ^Hfôn c may be given to different numbers of significant
i
figures. In this instance the quantity with the lesser number of figures
is used to represent the uncertainty estimate. The larger number of
figures is used for the other quantity to retain the significance of the
temperature correction term.
Arrangement of the Tables
The compounds in the tables are entered according to the Standard

Order of Arrangement, (see Figure 1), by the principle of latest position.
In this scheme, a compound is listed under the element occurring latest
in the list; water of hydration is neglected. Within a given element
table will be found all of the compounds of that element with elements
occurring earlier in the order; the arrangement within a table follows
the same ordering. An exception occurs in the carbon tables (Table 23),
which is divided into subgroups consisting of all compounds with one
carbon atom, then all with two carbon atoms, etc.
STANDARD ORDER OF ARRANGEMENT
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SERIES I
Enthalpy of Formation at 0°K

Enthalpy of Formation at 298. 15°K
Gibbs Energy of Formation at 298. 15°K
Enthalpy at 298. 15°K
Entropy at 298. 15 °K
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APPENDIX
The order in which the tables of Series I of National
Bureau of Standards Circular 500 are revised follows the
Standard Order of Arrangement. However it has been

necessary to evaluate the data on certain additional sub-
stances in order to complete the calculations for the
tables given in this part. The values obtained for some

of these compounds are given in the following Table B.
262
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263
Index of Contents
Chemical Element Table Page

Symbol Number
Al Aluminum 29 207
Ar Argon 5 17
As Arsenic 20 95
At Astatine 13 42
B Boron 28 196
Bi Bismuth 22 103
Br Bromine 11 31
C Carbon 23 106
Cd Cadmium 34 248
CI Chlorine 10 24
F Fluorine 9 21
Ga Gallium 30 2 18
Ge Germanium 25 177
H Hydrogen 2 12
He Helium 3 15
I Iodine 12 36
In Indium 31 223
Kr Krypton 6 18
N Nitrogen 1 8 61
Ne Neon 4 16
O Oxygen 1 1 1
P Phosphorus 19 84
Pb Lead 27 187
Po Polonium 17 60
Rn Radon 8 20
S Sulfur 14 43
Sb Antimony 21 99
Se Selenium 15 56
Si Silicon 24 171
Sn Tin 26 181
Te Tellurium 16 58
Tl Thallium 32 227
Xe Xenon 7 19
Zn Zinc 33 233
-
U. S. GOVERNMENT PRINTING OFFICE: 1967 — 301-022/68

264
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WASHINGTON, D.C. 20230 U.S. DEPARTMENT OF COMMERCE
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NATL INST.

OF STAND & TECH

Selected Values of Chemical

Central Radio Propagation Laboratory.* Ionospheric Telecommunications. Tropospheric Tele-

* Located at Boulder, Colorado 80301.

NBS TECHNICAL NOTE 270-3

Selected Values of Chemical Thermodynamic Properties

Tables for the First Thirty-Four Elements

D. D. Wagman, W. H. Evans, V. B. Parker,

I. Halow, S. M. Bailey, and R. H. Schumm

Institute for Basic Standards

This Technical Note supersedes Technical Notes 270-1 and 270-2

NBS Technical Notes are designed to supplement the

For sale by the Superintendent of Documents, U.S. Government Printing Office

Technical Note 270-3 is the third in a series of publications

containing material prepared as a revision of the tables of Series I

of National Bureau of Standards Circular 500, Selected Values of

Chemical Thermodynamic Properties, by F. D. Rossini, D. D.

Wagman, "W. H. Evans, S. Levine, and I. Jaffe. This Note extends

of the elements carbon, zinc, and cadmium in the Standard Order of

Arrangement. In addition this Note contains all of the Tables of

Technical Note 270-1 and 270-2, including corrections for a number

of minor errors. Thus this Note supersedes Technical Notes

270-1 and 270-2.

Donald D. Wagman, Chief

Table A Conversion Factors „ 7

Donald D. Wagman, William H. Evans, Vivian B. Parker,

Substances and Properties Included in the Tables

The physical state of each substance is indicated in the column

The symbols used in these tables are defined as follows: P =

The values of the thermodynamic properties of the pure substances

substance in the standard state at 298.15°K, omitting contributions from

in the case of the hydrogen-deuterium ( H- H) system. Where data have

Solutions in water are designated as aqueous (aq); other solvents

= A Hf ° - T A Sf ° will not hold for an individual ionic species. However

Internal Consistency of the Tables

A Gf° = A Hf° - T A Sf°.

NBS Technical News Bulletin, October 1963.

The uncertainty any value in the tables depends on the uncertain-

Arrangement of the Tables

The compounds in the tables are entered according to the Standard

Enthalpy of Formation at 0°K

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