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Lorenzo Torrisi
Università degli Studi di Messina
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The laser irradiation of thin foils may induce resonant between 0 and 30 . The schematic view of the experimental
absorption effects if the wavelength is comparable with the arrangement is reported in Fig. 1(a).
spherulite particle sizes or with other nanoparticles or nucle- Generally, the focal point of the laser was maintained at
ation centers embedded in the polymer. In these cases, high 100 lm in front of the target surface, in order to induce
laser energy is absorbed in the thin polymer and transferred preplasma and possible self-focusing effects, by using micro-
to the plasma particles, permitting the enhancement of the metric step motors controlled in a vacuum. This focalization
ponderomotive energy transferred to the electrons and conse- guarantees high plasma temperature production and high for-
quently the electric field driving the ion acceleration devel- ward ion acceleration, as demonstrated in previous
oped in the TNSA regime. The value of this electric field measurements.9
depends on the following parameters:4 The targets consist of thin polymeric films of semicrys-
rffiffiffiffiffiffiffiffiffiffiffi talline PET. The preparation of thin films was accomplished
~ kTe ne kTe by the formation of spherulites associated with the crystalli-
E¼ ¼ ; (1)
ekD e0 zation conduced in the viscous state from the melt (264 C)
with a high undercooling process controlled by the cooling
where kTe is the electron temperature of the plasma, e the rate.
electron charge, kD the Debye length, ne the electron density, In the polymeric fuse, Au spherical nanoparticles of
and e0 the dielectric constant in a vacuum. Increasing the 0.5% in weight with 100 nm average size were added. The
electron density and the plasma temperature, the electric diameter of spherulites in the polymers was measured by
field generated between the emitted electrons and the target optical microscopy in polarized light, obtaining a size distri-
ions increases. Generally, in polymers the electron density is bution varying in a wide range, from a fraction of micron to
low; thus, in order to enhance the electric field driving the about 2.5 lm. The polymer crystallization process was
ion acceleration, it is necessary to increase the plasma tem-
perature, i.e., the laser energy transferred to the target, or
embedding the polymer with metallic additives to enhance
the mean electron density. Gold nanoparticles (Au NPs) can
be embedded uniformly in the polymeric fuse in order to
enhance the electron density of the material and the absorp-
tion coefficient to the light. Metallic nanoparticles in insula-
tors induce surface plasmon resonance (SPR) absorption at
large wavelength bands depending on their nature, dimen-
sion, shape, and dielectric medium, producing high ion
acceleration in laser-generated plasmas, as reported in the
literature.2,5
In the standard description of the TNSA mechanism, a
laser pulse heats electrons in a target and creates charge sep-
aration on a femtosecond time scale. The laser accelerated
electrons emitted from the rear side of the thin foil (target)
generate a high electric field able to ionize the target surface
and to drive hydrogen and carbon ions. In the experiment
reported in this manuscript, the laser illumination time-scale
and the target thickness are favorable to produce a strong
heating of the electrons that are pushed away from the focus,
followed by a Coulomb explosion of the target due to the
strong ion charge density. Thus, although the TNSA regime
occurs mainly for fs lasers at intensity higher than 1018 W/
cm2, the mechanism involved using 300 ps laser pulses at an
intensity of about 1016 W/cm2 producing high ion accelera-
tion is very similar and it can be called “TNSA-like”
regime.6,7
10
M. Cutroneo, P. Musumeci, M. Zimbone, L. Torrisi, F. La Via, D. Meyroneinc, P. Mora, J. Schreiber, T. Toncian, P. Audebert, and H. Pepin,
Margarone, A. Velyhan, J. Ullschmied, and L. Calcagno, J. Mater. Res. Nat. Phys. 2, 48–54 (2006).
17
28(01), 87–93 (2013). R. Nave, See http://hyperphysics.phy-astr.gsu.edu/hbase/quantum/
11
M. Cutroneo, L. Torrisi, L. Ando, S. Cavallaro, J. Ullschmied, J. Krasa, D. wien3.html#c1 for Wien’s displacement law and other ways to character-
Margarone, A. Velyhan, E. Krousky, and M. Pfeifer, Acta Polytech. 53(2), ize the peak of blackbody radiation, 2017.
18
138–141 (2013). NIST, National Institute of Standards and Technology, See http://physics.-
12
NIST, National Institute of Standards and Technology, See http:// nist.gov/PhysRefData/ASD/ionEnergy.html for Atomic spectra database
www.nist.gov/pml/data/xraycoef/ for X-ray attenuation database, 2017. ionization energies form, 2017.
13 19
L. Laska, J. Badziak, K. Jungwirth, M. Kalal, J. Krasa, E. Krousk y, P. L. Torrisi, S. Gammino, L. And o, L. Laska, J. Krasa, K. Rohlena, J.
Kubes, D. Margarone, P. Parys, M. Pfeifer, K. Rohlena, M. Rosinski, L. Ullschmied, J. Wolowski, J. Badziak, and P. Parys, J. Appl. Phys. 99,
Ryc, J. Skala, L. Torrisi, J. Ullschmied, A. Velyhan, and J. Wolowski, 083301 (2006).
20
Radiat. Eff. Defects Solids 165(6–10), 463–471 (2010). L. Torrisi and M. Cutroneo, J. Appl. Phys. 115, 083105 (2014).
14 21
Z. Huang, L. Bi, Z. Zhang, and Y. Han, Mol. Med. Rep. 6(4), 709–715 L. Torrisi, D. Margarone, L. Laska, J. Krasa, A. Velyhan, M.
(2012). Pfeifer, J. Ullschmied, and L. Ryc, Laser Part. Beams 26, 379–387
15
L. Torrisi, M. Cutroneo, L. And o, and J. Ullschmied, Phys. Plasmas 20, (2008).
22
023106 (2013). A. Picciotto, L. Torrisi, S. Gammino, A. M. Mezzasalma, F. Caridi, D.
16
J. Fuchs, P. Antici, E. D’Humieres, E. Lefebvre, M. Borghesi, E. Margarone, L. And o, J. Krasa, L. Laska, and J. Wolowski, Radiat. Eff.
Brambrink, C. A. Cecchetti, M. Kaluza, V. Malka, M. Manclossi, S. Defects Solids 160(10–12), 705–713 (2005).