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Theory of Robust Quantum Many-Body Scars in Long-Range Interacting Systems
Theory of Robust Quantum Many-Body Scars in Long-Range Interacting Systems
Theory of Robust Quantum Many-Body Scars in Long-Range Interacting Systems
Alessio Lerose ,1, ∗ Tommaso Parolini,2, 3, † Rosario Fazio ,2, 4 Dmitry A. Abanin,1, 5 and Silvia Pappalardi 6
1
Department of Theoretical Physics, University of Geneva,
Quai Ernest-Ansermet 30, 1205 Geneva, Switzerland
2
The Abdus Salam International Centre for Theoretical Physics (ICTP), Strada Costiera 11, 34151 Trieste, Italy
3
Scuola Internazionale di Studi Superiori Avanzati, Via Bonomea, 265, 34136 Trieste, Italy
4
Dipartimento di Fisica, Università di Napoli “Federico II”, Monte S. Angelo, I-80126 Napoli, Italy
5
Department of Physics, Princeton University, Princeton, New Jersey 08544, USA
6
Institut für Theoretische Physik, Universität zu Köln, Zülpicher Straße 77, 50937 Köln, Germany
(Dated: September 25, 2023)
Quantum many-body scars (QMBS) are exceptional energy eigenstates of quantum many-body
arXiv:2309.12504v1 [cond-mat.str-el] 21 Sep 2023
systems associated with violations of thermalization for special non-equilibrium initial states. Their
various systematic constructions require fine-tuning of local Hamiltonian parameters. In this work
we demonstrate that the setting of long-range interacting quantum spin systems generically hosts
robust QMBS. We analyze spectral properties upon raising the power-law decay exponent α of spin-
spin interactions from the solvable permutationally-symmetric limit α = 0. First, we numerically
establish that despite spectral signatures of chaos appear for infinitesimal α, the towers of α = 0
energy eigenstates with large collective spin are smoothly deformed as α is increased, and exhibit
characteristic QMBS features. To elucidate the nature and fate of these states in larger systems, we
introduce an analytical approach based on mapping the spin Hamiltonian onto a relativistic quantum
rotor non-linearly coupled to an extensive set of bosonic modes. We exactly solve for the eigenstates
of this interacting impurity model, and show their self-consistent localization in large-spin sectors
of the original Hamiltonian for 0 < α < d. Our theory unveils the stability mechanism of such
QMBS for arbitrary system size and predicts instances of its breakdown e.g. near dynamical critical
points or in presence of semiclassical chaos, which we verify numerically in long-range quantum
Ising chains. As a byproduct, we find a predictive criterion for presence or absence of heating
under periodic driving for 0 < α < d, beyond existing Floquet-prethermalization theorems. Broader
perspectives of this work range from independent applications of the technical toolbox developed
here to informing experimental routes to metrologically useful multipartite entanglement.
are known to give rise to anomalous dynamical phenom- lap with product states (Sec. IV). We identify
ena [55–65]. This behavior can be traced back to a pecu- these eigenstates as candidate QMBS-like states,
liar form of integrability breaking. In the limit of all-to- smoothly deformed from the large-spin eigenstates
all infinite-range interactions the full permutational sym- of the permutationally-symmetric (solvable) mean-
metry allows to reduce the quantum many-body dynam- field limit α = 0. Using a refined numerical ap-
ics to the semiclassical dynamics of few collective degrees proach which involves a projection of the Hamilto-
of freedom. As the range of interactions is decreased, nian onto large-spin subspaces (App. B), we find
all other degrees of freedom associated with gradually evidence for robustness of the QMBS for arbitrary
shorter wavelengths get “activated” and interact with L when 0 < α ≲ d, and for their eventual hybridiza-
the collective ones. This tunable decoupling gives rise a tion when α ≫ d.
scenario that interpolates between few-body and many-
body physics. As a consequence, non-equilibrium behav-
• We formulate a self-consistent analytical theory of
ior shows resilience over long prethermal stages of dy-
eigenstate localization in Hilbert space that fully
namics [62, 66–69], whose duration increases with the
backs our numerical observations (Sec. V). First,
interaction range and grows unbounded in the thermo-
we introduce a procedure to map an interacting
dynamic limit when interactions decay slower than 1/rd
spin lattice onto a collective spin coupled to an en-
(d = system dimensionality) [56, 64, 70]. The occurrence
semble of bosonic modes, physically representing
of thermalization at longer times remains, however, an
magnon excitations with non-vanishing momenta.
open question.
The coupling strength is controlled by α and d and
In this paper we demonstrate the occurrence of robust it is vanishingly small in the mean-field limit. In
QMBS arising from long-range interactions in isotropic a Hilbert space shell with fixed energy density and
quantum spin lattices. This finding implies thermaliza- large collective spin, the exact spin-boson descrip-
tion breakdown at arbitrarily long times in this large tion reduces to a simpler but still interacting quan-
class of quantum many-body systems. As key point tum impurity model: a relativistic quantum rotor
of our analysis, we unveil an emergent exact solvabil- parametrically coupled to a quadratic bosonic bath.
ity of eigenstates originating from high-permutational- We find an exact solution to this effective Hamil-
symmetry sectors in these systems. We show that such tonian, which allows us to compute the degree of
eigenstates get smoothly deformed upon changing Hamil- eigenstate delocalization in Hilbert space and hence
tonian parameters as long as the decay of spin-spin inter- to check self-consistency. We find that the eigen-
actions remains sufficiently slow. The energy eigenvalues states of this rotor-magnon Hamiltonian are self-
associated with such QMBS form unequally spaced regu- consistent QMBS of the original spin Hamiltonian
lar towers, labelled by the collective spin quantum num- only for 0 < α < d. Figure 1 visually summa-
bers and by the occupation numbers of quasiparticle ex- rizes the steps of our eigenstate localization theory,
citations emerging from our analytical construction. To- which relies on two fundamental ingredients:
gether with the numerical observation of quantum chaos
signatures in level statistics for arbitrary decaying inter-
actions, our findings establish QMBS as a generic fea- 1. sufficiently slow interaction decay 0 < α < d;
ture of long-range interacting spin lattices. Our theory
2. classical integrability of the mean-field limit.
gives stringent quantitative criteria for the stability of
QMBS, which we numerically illustrate in the variable-
range quantum Ising chain. These QMBS thus possess, by construction, a clear
fingerprint from semiclassical periodic orbit – some-
times considered a defining feature of QMBS.
II. OVERVIEW
• We predict and classify instabilities of the QMBS,
The results of this paper apply to general quantum spin arising from violations of the two conditions above.
lattices with spin-spin interactions decaying algebraically Eigenstate delocalization most notably occurs in
as 1/rα with the distance r. For the sake of concrete- presence of discrete-symmetry breaking or of mean-
ness we work with a variable-range Ising-like quantum field chaotic dynamics. We accurately test these
spin chain, introduced in Sec. III. The following Sections predictions for the long-range quantum Ising chain,
present the main contributions of this work: respectively in the ordered phase or in presence of
periodic kicks (Sec. VI). Figure 2 reports represen-
• Performing an extensive study of numerical energy tative examples.
spectra of variable-range quantum Ising chains,
we show that random-matrix-like level repulsion
appears for infinitesimal α along with resilient The results of this work have a number of broader con-
anomalous eigenstates, characterized by large col- sequences, which we briefly elaborate on in the conclusive
lective spin size, low entanglement, and high over- Sec. VII.
3
quantum
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X
numbers eiF̂ eiŜ Ĥ↵,e↵ e iŜ iF̂
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e = ! N̂ + !k (↵) n̂k
collective spin size S
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Ĥ↵,e↵ k6=0
−π 0
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k6=0 π
k
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N ω̄
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fk(α)
S
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FIG. 1. Graphical summary of the theory of robust quantum many-body scars developed in this work. (Left panel) The
starting point is the solvable semiclassical spectrum of the mean-field limit of interacting spin lattices (α = 0), labelled by the
exact quantum numbers S = sLd − δS (collective spin size) and N (quantized classical action). Spin depletion δS is associated
with increasing degeneracy, which can be resolved in terms of magnon excitations with non-zero momentum. (Central panel)
We express the finite-range spin Hamiltonian with α ̸= 0 in terms of these degrees of freedom. This yields a reformulation as an
effective quantum impurity model: a relativistic quantum rotor parametrically coupled to an ensemble of bosons. In the dilute
sector δS ≪ L/2 of a given energy shell the effective rotor-magnon Hamiltonian simplifies to the extent that we can find a
(non-trivial) exact solution for its spectrum and eigenstates. (Right panel) Self-consistency of this solution is satisfied only for
0 < α < d, in agreement with our numerical data analysis for small system size. Our theory unveils the mechanism of eigenstate
localization underlying the robust quantum many-body scars. It also predicts and classifies instances of its breakdown, which
we verify numerically.
Classical limit
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Exact spectrum
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Eigenstate (de)localization
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↵=0 0<↵<d
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0<↵<d
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|hEn(0) |E ⇤ i|2
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collective spin size S
Ising model
|hEn(0) |E ⇤ i|2
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collective spin size S
Kicked Ising model
FIG. 2. Relation between classical mean-field trajectories for α = 0 (left column) and many-body energy eigenstates for α ̸= 0
(center and right columns). Classical integrability gives room to robust quantum many-body scars localized in the large-spin
sectors of Hilbert space, coexisting with a bulk of repelling energy levels for 0 < α < d (top row). Classical chaos, instead,
prevents quantum many-body scarring for arbitrarily small α > 0 (bottom row). The figure illustrates this dichotomy with
data for the quantum Ising model, Eq. (4) with γ = 1. We report: classical collective-spin trajectories ⟨Ŝ(t)⟩/L for α = 0 and
L → ∞ (left); exact energy spectra resolved in terms of the average collective spin size ⟨|Ŝ|⟩ for α = 0.5 and L = 18 (center);
(0)
weights on the unperturbed α = 0 basis {|En ⟩} of the representative eigenstate |E ∗ ⟩ highlighted in red in the center column
(right); with time-independent Hamiltonian (top) or subject to strong periodic driving (bottom) — in the latter case we report
stroboscopic trajectories and Floquet spectra. Quantum many-body scarring is here highlighted by wavefunction concentration
in large collective-spin size sectors (details are given further below in the paper).
4
1+γ x x 1−γ y y ∆ z z
X Å ã X
Ĥα = − Ji,j σ̂i σ̂j + σ̂i σ̂j + σ̂i σ̂j − h σ̂jz (1)
2 2 2
i,j j
where γ and ∆ parametrize the XY and XXZ Such prescription is necessary to have a well defined ther-
anisotropies, respectively. In this equation σ̂rx,y,z = modynamic limit for α ≤ d: The system-size divergent
ŝx,y,z
j /s are rescaled spin-s operators acting on the spin rescaling factor Nα,L ∼ Ld−α ensures that the energy per
at site j = (j1 , . . . , jd ) of the lattice, where ja = 1, . . . , L spin remains finite.
for a = 1, . . . , d. For spins-1/2 these are the standard
Pauli matrices.
We will consider interactions depending only on the
distance between spins, with algebraic decay:
J For definiteness, we will assume ferromagnetic inter-
Ji,j ≡ Ji−j = . (2) actions J0 > 0 throughout, and we set s = 1/2 [72].
||i − j||α
Increasing the range of interactions (i.e. decreasing α)
»P
d weakens spatial fluctuations, leading the system toward
where ||i − j|| ≡ a=1 [Min(|ia − ja |, L − |ia − ja |)]
2
its mean-field limit, analogously to increasing the system
realizes periodic boundary conditions. The constant J is dimensionality [73, 74]. It is thus convenient to perform
chosen to make the mean-field energy independent of the our theoretical analysis with fixed d and study the prop-
decay exponent α (Kac normalization [71]), erties of the model upon varying α. As the effects of
J0 1X 1 spatial fluctuations are strongest in one dimension, we
J= , Nα,L = . (3) will work with a variable-range XY quantum spin chain
2Nα,L 2 ||r||α
r̸=0
L L/2 L
J0 X X 1 1 + γ x x 1−γ y y
Å ã X
Ĥα = − σ̂j σ̂j+r + σ̂j σ̂j+r − h σ̂jz (4)
Nα,L j=1 r=1 rα 2 2 j=1
(periodic boundary conditions are understood). We an- limit with all-to-all interactions (α = 0). For α → 0
ticipate that our results do not rely at all on any of the Eq. (4) reduces to a Hamiltonian describing dynamics
model restrictions above, as we will explicitly show in of a single collective spin, completely decoupled from all
Sec. V H. the other degrees of freedom — realizing the mean-field
For α = ∞ the Hamiltonian (4) reduces to the XY description of the system. The effect of spatially mod-
quantum spin chain with nearest-neighbor interactions. ulated interactions α ̸= 0 is then to dynamically couple
This model is exactly solvable by mapping to a quadratic this collective degree of freedom to all the other finite-
fermionic chain via Jordan-Wigner transformation [75]. wavelength modes describing spatial fluctuations, result-
For finite α integrability is broken by couplings beyond ing in complex quantum many-body dynamics.
the nearest neighbors, as the associated Jordan-Wigner For later purpose we show how to make this picture
string turns into multi-fermion interactions. As α is de- explicit. We express the finite-range Hamiltonian Ĥα as
creased, longer-range interactions cooperate to suppress a perturbation to Ĥα=0 by rewriting it in momentum
spatial fluctuations, resulting in a qualitative enhance- space. Let us define the Fourier transform the spin oper-
ment of the system’s ability to order in excited states for ators (recall ŝµj = σ̂jµ /2 for µ = x, y, z)
α < 2 [76].
The tendency to sustain collective spin alignment be-
comes increasingly prominent as α is decreased. This is L
conveniently understood by viewing a long-range inter-
X
S̃kµ = eikj ŝµj , (5)
acting system as a “perturbation” to the infinite-range j=1
5
J0 X h i
−
Ĥα = − fk (α) S̃k+ S̃−k + S̃k− S̃−k
+
+ γ S̃k+ S̃−k
+
+ S̃k− S̃−k
−
− 2hS̃k=0
z
, (7)
L
k
J0 X h i
−
Ĥα = Ĥα=0 (Ŝ) + V̂α , with V̂α = − fk (α) S̃k+ S̃−k + S̃k− S̃−k
+
+ γ S̃k+ S̃−k
+ −
+ S̃k− S̃−k . (9)
L
k̸=0
Note that the term V̂α is in general an extensive pertur- The splitting in Eq. (9) thus gives us an intuitive phys-
bation [77]. ical picture of dynamics for α > 0 in terms of a collective
The quantity fk (α) controls how strongly spin fluctua- spin weakly coupled to finite-wavelength spin excitations.
tion modes with various wavelengths come into play, thus This representation can be expected to provide a starting
determining the physical properties of Ĥα . Its behavior point for a meaningful perturbation theory when fk̸=0 (α)
upon varying α is summarized in Fig. 3. Its shape shrinks is small. The precise notion of smallness will be clarified
from fk (α → ∞) = cos k to in this paper.
fk (α → 0) = δk,0 , (10)
IV. NUMERICAL ANALYSIS
becoming increasingly singular at k = 0 as α is decreased:
We analyze spectral properties of highly excited energy
fk (α) ∼ 1 − c(α)k 2 for α > 3; eigenstates
fk (α) ∼ 1 − c(α)|k|α−1 for 1 < α < 3;
Ĥα |En ⟩ = En |En ⟩ (12)
fkℓ (α) ≡ fℓ (α) ∼ c(α)|ℓ|−(1−α)
for α < 1.
(11) for finite 0 < α < ∞. While dynamical relaxation to
These and other properties of fk (α) are derived in thermal equilibrium is known to become slow as α is
App. A. The last case is the most interesting for this pa- decreased (see Introduction), it is generally believed
per: For α < 1, fk (α) squeezes onto the vertical axis as that thermalization is ultimately attained at long times
L → ∞; upon zooming near k = 0 one finds that the val- for any 0 < α < ∞, as the system is non-integrable. Ac-
ues f2πℓ/L converge as L → ∞ to a discrete sequence of fi- cordingly, the energy spectrum is believed to satisfy the
nite values, denoted fℓ , which fall off as |ℓ|−(1−α) , cf. the eigenstate thermalization hypothesis (ETH) [78, 79]. In
right panel of Fig. 3 [60, 64]. Thus, for small 0 < α < 1, this Section, we report extensive numerical simulations
only modes with extensive wavelengths kℓ ∝ 1/L do non- which show that the actual scenario may be subtler.
trivially participate in dynamics and interact; physically, While we find level statistics compatible with ETH down
in this regime interactions vary so slowly with the spatial to very small values of α ≳ 0.001 (in agreement with
distance that the system behaves as a permutationally Ref. [80], see also Ref. [81]), we will show that a relevant
invariant system over finite length scales, and it is thus subset of eigenstates exhibits remarkable deviations,
unable to resolve finite wavelengths. As α is increased characterized by anomalous QMBS-like properties such
further, all k ̸= 0 get eventually activated. as large collective spin size, low entanglement, and large
6
1.0 1
0.50
0.5 α = 0.5 L=250
fℓ (0.5)
fk(α ) α =1 L=1000
0.0 0.10
α = 1.5 L=4000
0.05
- 0.5 α =3 L=16000
- 1.0 α =6 L=64000
0.01
- 1.0 - 0.5 0.0 0.5 1.0 1 2 5 10 20
k/π ℓ
FIG. 3. Left panel: Couplings fk in Eq. (8) for a range of values of α; here we set L = 1000. Right panel: convergence of the
discrete sequence fℓ (α) for α = 0.5 as L → ∞; the dashed line highlights the asymptotics ∼ ℓ−(1−α) from Eq. (11).
p(r)
1.0
For definiteness, in this Section, we set γ = 1 in Eq. (4)
(quantum Ising chain). We further set J0 = h = 1 so as
to avoid signatures of the thermal phase transition (or of 0.5
the excited-state quantum phase transition [82]) in highly
excited states. In Sec. VI B below we will comment on 0.0
0.0 0.5 1.00.0 0.5 1.0
how these phenomena affect our results. r r
The Hamiltonian (4) has translation, spatial reflection,
and spin-flip symmetries, with associated quantum num-
bers K = 0, 2π/L, . . . , 2π(L−1)/L, I = ±1, and Pz = ±1
respectively. In our exact diagonalization (ED) results,
we fix for definiteness K = 0, I = 1, and Pz = 1.
A. Level repulsion
ˆ
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|hEn | *i|2
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FIG. 5. QMBS in the long-range quantum Ising chain. We report numerical energy spectra of the model in Eq. (4) with L = 18,
γ = 1 and h = 1, restricted to the translation-invariant, parity and spin-flip symmetric sector. Scatter plot of the observables
⟨δS ⟩ (row a), half-chain entanglement entropy SL/2 (En ) (row b), and overlap with the polarized state |⟨↑ |En ⟩|2 (row c) of each
eigenstate |En ⟩ as a function of the energy density En /L. Columns (1-4) correspond to increasing values of α = 0, 0.2, 0.5, 0.8.
ligible fraction of atypical non-thermal eigenstates run- In the limit α = 0 the Hamiltonian conserves the col-
ning througout the many-body energy spectrum. lective spin size [Ĥα=0 , Ŝ2 ] = 0 and hence δS = L/2−S is
In Fig. 5 we plot, for all energy eigenstates {|En ⟩}: an exact quantum number. The energy spectrum forms
a) the average depletion of the total spin Ŝ2 = |Ŝ|(|Ŝ|+1) unequally spaced towers (Peres lattice [86]) labelled by
from its maximal value, i.e. δS – the horizontal rows in Fig. 5a1. The degeneracy
of the eigenspaces increases exponentially with δS , i.e.,
L as the collective spin size gets smaller. The so-called
⟨δ̂S ⟩En = − ⟨|Ŝ|⟩En , (14)
2 Dicke manifold [87] spanned by the L + 1 non-degenerate
eigenstates with maximum collective spin size δS = 0 is
b) the half-chain entanglement entropy: the permutationally symmetric subspace. This tower of
eigenstates corresponds to the large orange dots in the
SL/2 = Tr(ρ̂L/2 ln ρ̂L/2 ),ρ̂L/2 = TrL/2+1,...,L |En ⟩⟨En | , figure. Their bipartite entanglement entropy is known to
(15) scale logarithmically with system size, i.e., SL/2 ∼ ln L,
c) the overlap with the fully polarized state away from the edges of the spectrum [88]. The fully po-
larized state | ⇑⟩ has non-vanishing overlap with them
|⟨En | ⇑⟩|2 , (16)
only. Note that some states are missing in the plot due
where | ⇑ ⟩ ≡ | ↑1 ↑2 . . . ↑L ⟩. to our symmetry restrictions [89].
The anomalous structure of the many-body energy spec- As α is increased from 0 the degeneracies are lifted.
trum is highlighted by either of these three quantities in While the splitting of the exponentially degenerate sec-
Fig. 5. tors having δS = O(L) dominate the level spacing statis-
8
The dynamic counterpart of the spectral structure of In this Section we analyze spectral properties at fi-
QMBS found above is given by out-of-equilibrium dy- nite α using an analytical approach we develop. This
namics depending strongly on the initial condition. For allows us to formulate a predictive theory for the stabil-
completeness we report evidence of this behavior, exem- ity of non-thermal eigenstates observed in numerics.
plified by Fig. 8, where we contrast initialization in a Taking the exact solution of the α = 0 model as start-
polarized state (blue) to a random product state (red), ing point (Secs. V A), we interpret the spectral degener-
subject to evolution governed by a long-range quantum acy in terms of magnon excitations (Sec. V B). Hence, we
Ising Hamiltonian, (4) with γ = 1 and α = 0.7. provide basic intuition for the persistence of a few non-
Polarized states, such as |⇑⟩ = |↑ . . . ↑⟩, have a large thermal eigenstates for small finite α (Sec. V C). Building
overlap with the QMBS [cf. Fig. 5]. Consequently, they on this intuition we systematically map the original spin
display anomalous dynamics of local observables such as Hamiltonian to that of a collective spin interacting with
the single-site spin polarization ⟨σ̂1z (t)⟩, see Fig. 8a, ex- L − 1 bosonic modes (Sec. V D), and we demonstrate
hibiting strong revivals over time scales that grow with that this mapping takes a particularly simple and physi-
L. This is accompanied by slow logarithmic growth of cally suggestive form in the large-spin sectors (Sec. V E).
the entanglement entropy, which eventually saturates to Remarkably, we show that the resulting effective model
a value scaling only logarithmically with the volume, is an interacting impurity model, for which we find an
see Fig. 8b. This phenomenology, detected numerically exact solution (Sec. V F), and we compute the spread-
in Refs. [95, 96], was explained via a semiclassical the- ing of energy eigenstates in Hilbert space as α is in-
ory [64] valid at long but finite times. (Qualitatively creased (Sec. V G). These results show that non-thermal
different behavior occurs in proximity to semiclassical in- eigenstates are stable for arbitrary system size L when
stabilities [56, 64], as we discuss in Sec. VI B.) 0 < α < 1 in absence of semi-classical chaos. We con-
We contrast this behavior with dynamics initialized in clude this Section by expounding the generality of our
a random product state such as |ψ0 ⟩ = | ↑1 ⟩|s2 ⟩ . . . |sL ⟩ theory (Sec. V H). We make reference to Fig. 1 for a vi-
where the first spin points along z while other spins point sual summary of the main steps of this Section.
in random uncorrelated directions on the Bloch sphere, We note that a related rotor-magnon description of
|si ⟩ = cos(θi /2)| ↑⟩i + eiϕi sin(θi /2)| ↓⟩i with θi ∈ [0, π) the low-energy spectrum has been recently developed by
and ϕi ∈ [0, 2π). In this case, the initial collective spin Roscilde et al. [97, 98].
10
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S ⋮ ⋮ ⋮
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limit (α = 0) L/2
⋮
!
¯
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⋮
with infinite interaction range (α = 0) [99–103], which
plays a central role in the following theory.
⋮
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!
The Hamiltonian Ĥα=0 is invariant under all spin per- E
<latexit sha1_base64="kMrIg88zv9vFXFvsZ29D8EiAanA=">AAACH3icdVDLSgNBEJz1bXxFBS9eBoPgQcJs8JWbKIInUTQqJGHpnbQ6OPtgplcJaz5Gr/of3sSrv+EXuLtGUNE6FVXdVFF+rJUlId6cgcGh4ZHRsfHSxOTU9Ex5du7URomR2JCRjsy5Dxa1CrFBijSexwYh8DWe+de7uX92g8aqKDyhboztAC5DdaEkUCZ55YU9L211UBN4x6u8zw56Xrkiqq6or4tNnpMNsSUKUqvXBXerokCF9XHold9bnUgmAYYkNVjbdEVM7RQMKamxV2olFmOQ13CJzYyGEKBtp0X/Hl9OLFDEYzRcaV6I+P0jhcDabuBnlwHQlf3t5eJfXjOhi612qsI4IQxlHkRKYxFkpVHZMMg7yiAR5M2Rq5BLMECERnGQMhOTbKkfgbdgu1mbXikb6WsJ/j85rVXdjer60Vple6c/1xhbZEtshblsk22zfXbIGkyyO/bAHtmTc+88Oy/O6+fpgNP/mWc/4Lx9AIbFo3U=</latexit>
S, N
mutations. It reduces to a function of the collective spin
PL
components Ŝ x,y,z = 12 j=1 σ̂jx,y,z :
4J0 1 + γ x 2 1 − γ y 2
ï ò
Ĥα=0 = − Ŝ + Ŝ −2hŜ z . (17)
…
L 2 2
1
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S ,N
size Ŝ2 = (Ŝ x )2 + (Ŝ y )2 + (Ŝ z )2 . The eigenvalues of Ŝ2 0
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is simply defined by N̂ |N ⟩ = N |N ⟩, and the quantum for M = 0, 1, . . . , L − 2δS . On varying ⃗n(Ω) on the unit
operators e±iφ̂ associated with the classical conjugated sphere, spin-coherent states span the full tower (“over-
angle act as raising and lowering operators on the ladder complete basis”): one can show that
of eigenstates. On the other hand, the collective spin size
ρ is also similarly quantized, ρ = S/(L/2) = 1 − 2δS /L. L−2δ
XS
Taking δS ≪ L/2 we can consistently neglect O(1/L2 ) 1δS ,κ = |δS , κ; M⇑ ⟩⟨δS , κ; M⇑ |
corrections in n and obtain a formula for the semiclassi- M =0 (31)
cal spectrum to leading order in ℏeff = 2/L: L − 2δS + 1
Z
= dΩ |δS , κ; Ω⟩⟨δS , κ; Ω|
L
Å
2N 2δS
ã 4π
EδS ,N ∼ H ;1 − . (26)
2 L L R 2π Rπ
where dΩ ≡ 0 dϕ 0 dθ sin θ. Thus, every state in
R
This is illustrated in Fig. 9. the tower can be written as a linear combination of spin-
The level spacing EδS ,N −EδS ,N −1 within a tower has a coherent states [104]. In particular, for the eigenstates of
semiclassical interpretation as ℏω(n; ρ), where ω = ∂n H Hα=0 we can write
is the frequency of the classical orbit at the correspond-
ing energy. This quantity varies smoothly as N runs
Z
through a tower (at least away from isolated phase-space |δS , κ; N ⟩ = dΩ ψδS ,N (Ω)|δS , κ; Ω⟩. (32)
separatrices where ω = 0, corresponding to singularities
of the action-angle representation of H). To make the lo- Here we introduced the coherent-state wave function
cal structure of the semiclassical spectrum manifest, we ψδS ,N (Ω) ∝ ⟨δS , κ; Ω|δS , κ; N ⟩ of the unperturbed eigen-
focus on a given energy shell and set N = n L/2 + δN , state, which is efficiently accessible to both semiclassical
with δN integer. Expanding in 1/L, we obtain and numerical computations (see App. C).
2δN 2δS
Å ã
L
EδS ,δN ∼ H n + ;1 − In this work we will consider the α = 0 spectrum and
2 L L
Å ã (27) eigenbasis as known input data, which can be computed
1 either analytically (via a large-L asymptotic expansion)
∼ L E(n) + ω(n) δN + ω̄(n) δS + O .
L or numerically (via exact diagonalization of the single-
Thus, the energy spectrum around the energy density spin problem for S ≤ L/2 ≈ 105 ). We briefly mention in
E(n) = H(n; 1)/2 is built by combining integer multiples passing that the considered family of models is equivalent
of two (positive) fundamental frequencies, ω ≡ ∂n H in the limit α = 0 to the Lipkin-Meshkov-Glick model
and ω̄ ≡ −∂ρ H, which vary smoothly with n. This is of nuclear physics [99], which is actually Bethe-ansatz
illustrated in the inset of Fig. 9. solvable [105]; however, this solution is not practically
useful for large L, and semiclassical/numerical techniques
For later convenience, we note that the α = 0 give much easier access to the relevant information.
eigenstates can be expressed in the language of spin-
coherent states. Here we synthetically report the nec-
essary information on this formalism; a minimalistic self- B. Bosonic labelling of α = 0 eigenstates
contained review is in App. C. Considering the SU (2)
tower identified by (δS , κ), we define the spin-coherent For α = 0 the many-body Hilbert space fragments into
state with spherical angle Ω ≡ (θ, ϕ) as the state many single-spin Hilbert spaces. Each such SU (2) irre-
with maximal spin projection in the direction ⃗n(Ω) = ducible representation is associated with a regular en-
(sin θ cos ϕ, sin θ sin ϕ, cos θ) within the tower: ergy tower, identified by the collective spin size S and
by an additional quantum number κ [cf. Eq. (21)] that
⃗ˆ |δS , κ; Ω⟩ = L − δS |δS , κ; Ω⟩.
Å ã
⃗n(Ω) · S (28) parametrizes the degeneracy of the towers with equal S.
2
As soon as interactions acquire a non-trivial spatial struc-
The freedom in the choice of relative phases of spin- ture, e.g. for α ̸= 0, different towers get coupled and the
coherent states can be fixed by choosing a reference one degeneracy gets lifted. To understand how the perturba-
— usually in the ⃗z direction (θ = 0), i.e. |δS , κ; ⇑⟩ — tion affects the eigenstates, we first need to make sense
and a particular rotation protocol — usually the rota- of κ in terms of additional physical degrees of freedom,
tion by θ in the plane generated by ⃗z and ⃗n(Ω): denoting which are “inert” for α = 0 and get activated as α ̸= 0.
⃗r(Ω) ≡ |⃗⃗zz×⃗
n(Ω)
n(Ω)| , one has
×⃗ In this Subsection we show how the degeneracy of Ĥα=0
ˆ
can be resolved in terms of bosonic excitations (physically
⃗
|δS , κ; Ω⟩ = Û (Ω)|δS , κ; ⇑⟩, Û (Ω) ≡ e−iθ ⃗r(Ω)·S . (29) interpreted as magnons or quantized spin waves) with
non-vanishing momenta. This way, each α = 0 eigenstate
For every choice of Ω we denote the ladder of eigenstates
can be identified by the collective spin state – specified
of the corresponding collective spin projection as
by the quantized classical action N = 0, 1, . . . , L − 2δS –
ˆ and by the magnon content of the state – specified e.g.
Å ã
L
⃗n(Ω) · S |δS , κ; MΩ ⟩ =
⃗ − δS − M |δS , κ; MΩ ⟩ (30)
2 by δS non-vanishing momenta. This allows us to replace
12
z
S
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<latexit sha1_base64="cJYR4Lv/UCE0YBlJ2BaU2F2o2LU=">AAACLXicbVDLSgNBEJyN7/iKevQyGAUPEnbFF3gRvXhUMCpkQ+gdO3HI7Oww06uEmB/wZ/Sq/+FBEK/e/QJ3Yw5qrMNQVHVTPRUZJR35/qtXGBkdG5+YnCpOz8zOzZcWFs9dklqBVZGoxF5G4FBJjVWSpPDSWIQ4UngRtY9y/+IGrZOJPqOOwXoMLS2bUgBlUqO0ehdibKjjkHi4wffzx2+EVQPWJrehBd1S2CiV/YrfBx8mwYCU2QAnjdJneJWINEZNQoFztcA3VO+CJSkU9oph6tCAaEMLaxnVEKOrd/u/6fG11AEl3KDlUvG+iD83uhA714mjbDIGunZ/vVz8z6ul1Nyrd6U2KaEWeRBJhf0gJ6zMakJ+JS0SQX45cqm5AAtEaCUHITIxzXr7FXgLrpNd0ytmJQV/Kxkm55uVYKeyfbpVPjgc1DXJltkKW2cB22UH7JidsCoT7J49sif27D14L96b9/49WvAGO0vsF7yPL4JEqII=</latexit>
Standard
Ŝk=0 −
ator S̃k=0 to it, we generate the entire δS = 0
<latexit sha1_base64="CDMBqum9idBHKT89JXbgQ12lE2g=">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</latexit>
and S z = S − M ). The eigenstates of the desired Ĥα=0 • This procedure can be iterated to break down
are linear combinations of the eigenstates of Ŝ z within the full multi-spin Hilbert space into simultane-
individual SU (2) towers, i.e. of states with different M ous eigenspaces of Ŝ 2 and Ŝ z : For arbitrary δS
but fixed magnon content, as we describe at the end. we define the normalized states |{k1 , . . . , kδS }; ⇑⟩ ∝
P̂δS S̃k−δ . . . S̃k−1 | ⇑ ⟩ where k1 , . . . , kδS ̸= 0. Such
S
We start from the spin-coherent state | ⇑ ⟩ ≡ | ↑1 ↑2 states span the full eigenspace with fixed δS and
. . . ↑L ⟩ and act with lowering operators Sk− [cf. Eq. (5)], maximal S z = L/2 − δS . By repeatedly apply-
−
generalizing the procedure leading to Clebsch-Gordan co- ing the collective lowering operator S̃k=0 to each of
efficients [106]. To follow the construction it is helpful to them we generate the entire towers that compose
make reference to the illustration in Fig. 10: the δS eigenspace. We normalize such states and
13
h i
⟨{k1′ , . . . , kδ′ ′ }; M⇑′ | {k1 , . . . , kδS }; M⇑ ⟩ = δδS ,δS′ δM,M ′ δ{k1 ,...,kδS },{k1′ ,...,kδ′ } + O δS /L . (35)
S S
This property can be traced back to the correspondence δS ≪ L/2 but also M ≪ L, the correspondence between
between nearly polarized spin states with large S z and spin states and bosonic states is one-to-one:
dilute bosonic states, realized by the Holstein-Primakoff
transformation. To see this, let us define the mapping ⟨{nk }|{k1 , . . . , kδS }; M⇑ ⟩ =
† † † 1 δnk=0 ,M δ{nk }k̸=0 ,{k1 ,...,kδS } + O (M + δS )/L . (39)
ŝ−
j 7→ b̂j (1 − b̂j b̂j ), ŝj 7→ (1 − b̂j b̂j )b̂j , ŝj 7→
+ z
− b̂†j b̂j ,
2
(36) In other words, when the spin state is close to fully polar-
where b̂j , b̂†j are canonical bosonic annihilation and cre- ized (L/2−S z ≪ L), the quantum number M can simply
be identified with the occupation of the k = 0 bosonic
ation operators. [Note that this is an equivalent sim-
mode. In this corner of the multi-spin Hilbert space
pler version of the standard exact Holstein-Primakoff
(blue-shaded area in Fig. 10), the correspondence be-
transformation for s = 1/2, see e.g. Ref. [107].] The
tween nearly fully polarized spin states and dilute bosonic
mapping (36) should be understood as an embedding of
Fock states is complete.
the two-dimensional Hilbert space of a spin-1/2 in the
Equation (35) shows however that spin states
infinite-dimensional Hilbert space of a bosonic mode,
|{k1 , . . . , kδS }; M⇑ ⟩ with δS ≪ L/2 but arbitrarily large
with | ↑ ⟩ and | ↓ ⟩ mapped onto |0⟩ ≡ |∅⟩ and |1⟩ ≡ b† |∅⟩
M can also be accurately labelled by their magnon con-
respectively. It is useful to define bosonic Fock states
tent {nk }k̸=0 (red-shaded area in Fig. 10). Loosely speak-
Y b̃† nk ing, Eq. (35) allows us to factorize the Hilbert space of
|{nk }⟩ ≡ √k |∅⟩ , (37) L spins as direct product of a large spin and a Fock
nk !
k space of L − 1 bosonic modes, which is accurate in the
√ P subspace δS ≪ L/2 with dilute bosons. It is tempt-
where b̃†k = (1/ L) j eikj b†j creates a boson with mo-
ing to picture the state |{k1 , . . . , kδS }; M⇑ ⟩ as a macro-
mentum k and {nk } is a string of occupation numbers. In scopic “condensate” of M collective magnon excitations
App. D we show that, in the dilute regime, the maximally with k = 0 accompanied by dilute magnons with non-
polarized (i.e. M = 0) spin states |{k1 , . . . , kδS }; ⇑⟩ de- vanishing momenta k1 , . . . , kδS ̸= 0, as suggested by the
fined above are close to the corresponding bosonic Fock expression in Eq. (34). One must keep in mind, how-
states with unoccupied k = 0 mode: ever, that for extensive M = O(L) the total popula-
⟨{nk }|{k1 , . . . , kδS }; ⇑⟩ = δ{nk },{k1 ,...,kδS } + O δS /L . tion M + δS = O(L) of Holstein-Primakoff bosons is
−
(38) far from dilute, making the naive replacement of S̃k=0
(Here, with a little abuse of notation, the Kronecker (the actual creation operator of collective spin excita-
delta on the right-hand side forces the set of momenta tions) by b̃†k=0 (the Holstein-Primakoff creation operator)
counted with their multiplicities to be that identified by highly inaccurate. The spin state |{k1 , . . . , kδS }; M⇑ ⟩ ac-
the string of occupation numbers.) Since Fock states are tually has exponentially-small-in-M overlap with its can-
orthonormal, Eq. (38) immediately implies Eq. (35) for didate bosonic partner |n0 = M, {nk }k̸=0 ⟩. [In fact, it is
M = M ′ = 0. Hence, crucially, the quasi-orthonormality straightforward to check that only an exponentially small
of the parent maximally polarized states is transferred fraction of the latter bosonic Fock state belongs to the
down throughout the respective SU (2) towers, to states physical spin space!]
|{k1 , . . . , kδS }; M⇑ ⟩ with arbitrary M . ThePset of non-vanishing momenta {nk }k̸=0 determines
As illustrated in Fig. 10, the construction above non- δS = k̸=0 nk and the silent quantum number κ appear-
trivially extends the standard Holstein-Primakoff map- ing in Eq. (21), with accuracy O δS /L . In the construc-
ping between spins and bosons. Indeed, when not only tion above, states within each SU (2) tower are identified
14
by the eigenvalue of the collective operator Ŝ z . As an- on the (δS , δN )-lattice. Furthermore, since the two fun-
ticipated above, the role of Ŝ z can however be played as damental frequencies ω, ω̄ that locally define the lattice
well by the quantized action operator N̂ associated with smoothly vary with n, for a generic choice of energy shell
an arbitrary collective Hamiltonian Ĥα=0 . Correspond- they are typically non-resonant (i.e. incommensurate).
−
ingly, the role of S̃k=0 is played by eiφ̂ . This way, states This condition prevents energy denominators to become
within each tower are identified by N = 0, 1, . . . , L − 2δS , arbitrarily small at any given order in perturbation the-
ory [109]. The simultaneous suppression of matrix ele-
|{k1 , . . . , kδS }; N ⟩ (40) ments for small α thus prevents the occurrence of energy
resonances to all orders, hindering the delocalization of
in place of the collective z-magnetization depletion M = perturbed eigenstates over the graph in Fig. 9.
0, 1, . . . , L − 2δS . This labelling is equivalent to Eq. (21) Remarkably, the basic mechanism illustrated above
upon identifying (δS , κ) ↔ {k1 , . . . , kδS } ↔ {nk }k̸=0 . finds a natural counterpart in an emergent exact solvabil-
This is the conclusion we aimed for. ity of the perturbed energy eigenstates originating from
the subspaces δS ≪ L/2. The rest of this Section is de-
voted to this demonstration, which constitutes the main
C. Eigenstate localization for 0 < α ≪ 1 theoretical result of this paper. Combined with the solid
observation of level repulsion at arbitrarily small α > 0
The fully connected Hamiltonian Ĥα=0 features an ex- reported in Sec. IV, this result proves the coexistence of
tensive tower of “ground-state-like” wavefunctions — the robust QMBS and a quantum-chaotic bulk many-body
δS = 0 states — running throughout the many-body en- spectrum in long-range interacting systems, which is the
ergy spectrum. From a thermodynamic viewpoint, such main message of this paper.
states are anomalous highly-excited states with large
overlap with product states, low entanglement, and reg-
ular energy level spacing. Each such state finds exponen- D. Matrix elements of Ĥα
tially many other states of non-collective character — i.e.
with δS = O(L) — at equal energy density. As α > 0
states with different collective spin length get dynami- In Sec. V A we reviewed how Ĥα=0 dynamically acti-
cally connected, and hybridization of the “few” anoma- vates a single collective degree of freedom, and in Sec. V B
lous states with small δS with the “many” normal states we showed how the remaining L − 1 dynamically frozen
with δS = O(L) becomes a priori favorable. As discussed degrees of freedom can be conveniently expressed as
in Sec. IV, the numerical results indicate a different sce- bosonic modes — physically associated with magnon or
nario, showing a weak or suppressed tendency towards spin-wave excitations with non-vanishing momenta. It is
hybridization. natural to ask how the variable-range perturbation V̂α fits
into this framework. Considering the unperturbed spec-
We argue here — and demonstrate below via ex-
trum as in Fig. 11, transitions between different towers
plicit analytical arguments — that hybridization of non-
generated by V̂α (shaded arrows) correspond to creation
thermal eigenstates is hindered for small α by a combi-
or destruction of few magnons simultaneously with jumps
nation of two crucial ingredients:
of the collective spin quantum number N . The goal of
i) the suppression of matrix elements ∝ fk (α), as- this and the next Subsection is to derive an explicit rep-
cribed to the long range of the interactions; resentation of the Hamiltonian Ĥα as a large spin inter-
acting with an ensemble of bosonic modes. We will infer
ii) the absence of energy resonances in the subspaces this representation by computing matrix elements.
δS ≪ L/2, ascribed to the classical integrability of Starting from the expression of Ĥα in Eq. (7), we insert
the mean-field limit. on both sides resolutions of the identity with unperturbed
eigenstates (21). The infinite-range Hamiltonian is by
This mechanism is pictorially illustrated in Fig. 11. construction diagonal,
The graph therein shows the energy levels of Ĥα=0 ar-
ranged in a smoothly varying 2d lattice spanned by the XX
Ĥα=0 = EδS ,N |δS , κ; N ⟩⟨δS , κ; N |, (41)
integers quantum numbers (δS , δN ), cf. Eq. (27), con-
δS ,κ N
nected by shaded arrows representing matrix elements
for α ̸= 0. As the interaction operator flips at most two
with EδS ,N given by Eq. (26). The variable-range per-
spins, each matrix element connects states with δS differ-
turbation can be written as V̂α = L1 k̸=0 fk (α)V̂k , with
P
ing by at most 2 — and we will interpret the change in
δS as creation and annihilation of magnons [108]. At the
−
same time, the dependency of matrix elements on the col- V̂k = −J0 (S̃k+ S̃−k + S̃k− S̃−k
+
) + γ(S̃k+ S̃−k
+
+ S̃k− S̃−k
−
) .
lective spin variables is rooted in semiclassics, resulting in (42)
analytic functions of n = N/L and φ (which will be rig- We need to compute the matrix elements
orously shown below). These remarks show that transi-
tions generated by the perturbation α ̸= 0 are quasi-local ⟨δS′ , κ′ ; N ′ |V̂k |δS , κ; N ⟩. (43)
15
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S S
…
//
//
⇝
…
…
…
E E
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S ,N S ,N
FIG. 11. Sketch of the intuitive argument for eigenstate localization in the main text. Left panel: Transitions generated by V̂α
are quasilocal on the unperturbed spectrum graph. The shading of the arrows denotes the amount of hybridization generated
at the perturbative order for which the corresponding transition comes into play. Right panel: For α < 1, we demonstrate that
an exact eigenstate originating from the δS ≪ L/2 subspace stays localized in a local neighbourhood.
where we defined (omitting Ω-dependency for simplicity) Here comes the crucial point: We have now isolated the
amplitudes of the collective spin’s and the magnons’ tran-
h sitions in the expression of the matrix element. Putting
J µ,ν ≡ −J0 R+,µ R−,ν + R−,µ R+,ν
everything together and performing the integrals over the
i spherical angles we obtain
+ γ R+,µ R+,ν + R−,µ R−,ν . (52)
4 å1/2
L − 2δS S̃kµ S̃−k
ν
Ç
X X X
⟨δS′ , κ′ ; N ′ |V̂α |δS , κ; N ⟩ = fk (α) Jδµ,ν
′ ,N ′ ;δ ,N ;(M ) ⟨δS , κ ; M⇑ |
′ ′
|δS , κ; ⇑⟩ , (53)
µ,ν=+,−,z M =0
M S S L
k̸=0
This is an exact expression for the matrix elements of Holstein-Primakoff mapping (36),
the finite-range perturbation V̂α between arbitrary eigen-
states of an infinite-range Hamiltonian Ĥα=0 (no relation 1
S̃k− 7→ L1/2 b̃†k −
X
b̃†q1 b̃†q2 b̃q1 +q2 −k ,
between the two has to be assumed). The computation L1/2 q1 ,q2
of the matrix element is reduced to a finite sum of ma- 1
b̃†q1 +q2 +k b̃q1 b̃q2 ,
X
trix elements of two-spin operators between maximally S̃k+ 7→ L1/2 b̃−k − (55)
(ket) and a nearly-maximally (bra) polarized states in L1/2 q1 ,q2
the corresponding SU (2) towers, with coefficients com- L X †
puted from the single-spin α = 0 solution, i.e. by taking S̃kz 7→ δk,0 − b̃q+k b̃q .
2
integrals of simple trigonometric polynomials and the two q
indeed, in this case the extra factor L1/2 in Eq. (53) App. C. It follows that the matrices Jδµ,ν
′ ,N ′ ;δ ,N ;(M ) are
S
compensates the 1/L1/2 in the right-hand sides.
S
independent of the spin size and only sensitive to δS − δS′
• Similarly, for M = 2, 3, 4, contributions of the same to leading order in 1/L. Furthermore, these matrices
have characteristic semiclassical structure, which is best
leading order are given by terms with (b̃†0 )M and a
appreciated upon expressing the spin components as an-
zero-momentum pair. Here the factors L−M/2 on alytic functions of the action and angle variables of the
the right-hand sides are exactly compensated by unperturbed problem: The analytic dependency on the
the extra factors LM/2 in Eq. (53). As it turns angle φ translates into an (at most) exponential decay
out, only the following term with M = 2 con- of the matrix elements in N ′ − N away from the diago-
tributes: [111] nal, and the analytic dependency on the action n trans-
1 − − 1 lates into a smooth variation with (N + N ′ )/L along the
S̃k S̃−k 7→ − (b̃†0 )2 b̃†k b̃k + b̃−k b̃†−k . (59) diagonal. (These standard general properties can eas-
L L
ily be checked numerically for an arbitrary polynomial
We conclude that the transitions in magnon space are collective operator P (Ŝ/S) and an arbitrary single-spin
described by a quadratic bosonic Hamiltonian (up to cor- Hamiltonian Ĥα=0 eigenbasis.)
rections of higher order in the magnon density δS /L).
What about the simultaneous transitions in collective- Putting everything together, we have found a remark-
spin space? Here the crucial observation is that the coef- able result: for δS ≪ L/2, the matrix elements of the
ficients Jδ±,±
′ ,N ′ ;δ ,N ;(M ) can be identified with matrix ele-
S finite-range Hamiltonian Ĥα coincide with those of an
S
ments of a certain polynomial collective operator P (Ŝ/S) effective Hamiltonian describing a large spin coupled to
between eigenstates of the α = 0 problem, as derived in bosons,
X ïL Å N ã Å
N
ãX ò
Ĥα,eff = H ; 1 − ω̄ ;1 b̃†k b̃k |N ⟩⟨N |
2 L/2 L/2
N k̸=0
" #
1 X X N + N′ † N + N′ N + N′ † †
Å ã Å ã Å ã
†
+ fk (α) JN ′ −N b̃k b̃k +b̃−k b̃−k +KN ′ −N b̃−k b̃k +KN ′ −N
∗
b̃k b̃−k |N ′ ⟩⟨N |,
2 ′
L L L
N,N k̸=0
(60)
′ +,− z,− −,− ′ +,+
where JN ′ −N N +N L ≡ 2 J0,N ′ ;0,N ;(0) − J0,N ′ ;0,N ;(1) − J0,N ′ ;0,N ;(2) and KN ′ −N N +N
L ≡ 2J0,N ′ ;2,N ;(0) . This
equation is our first main result: We have rewritten our finite-range Hamiltonian as an effective model of a semiclassical
particle (the collective spin), described by states {|N ⟩}, coupled to an ensemble of bosonic modes associated with
magnon excitations with non-vanishing momentum (k ̸= 0).
While the Hamiltonian (60) is quadratic in the bosons, the coupling is highly non-linear as the coefficients of the
quadratic bosonic Hamiltonian depend on the configuration of the collective spin. Since the semiclassical particle
spans macroscopically different energies, we can simplify the expression by focusing on a given energy shell, and
rewrite the effective Hamiltonian therein. Setting N = nL/2 + δN , N ′ = nL/2 + δN + r, and consistently neglecting
O(1/L) terms, we obtain the following quantum rotor-magnon Hamiltonian:
b̃†k b̃k
X X
Ĥα,eff (n) = LE(n) + ω(n) δN |δN ⟩⟨δN | + ω̄(n)
δN k̸=0
" #
1X X
† † † †
+ fk (α) Jr (n) b̃k b̃k + b̃−k b̃−k + Kr (n) b̃−k b̃k + Kr (n) b̃k b̃−k |δN + r⟩⟨δN | . (61)
∗
2
δN ,r k̸=0
Alternatively, introducing the collective action displacement δ̂N = δN |δN ⟩⟨δN | and angle e±iφ̂ =
P P
δN δN |δN ±1⟩⟨δN |
operators, we can rewrite the rotor-magnon Hamiltonian as
b̃†k b̃k
X
Ĥα,eff (n) = LE(n) + ω(n) δ̂N + ω̄(n)
k̸=0
1X h i
+ fk (α) J (n, φ̂) b̃†k b̃k + b̃−k b̃†−k + K(n, φ̂) b̃−k b̃k + K∗ (n, φ̂) b̃†k b̃†−k . (62)
2
k̸=0
18
the condensate fluctuations (associated with the collec- such a way that the transformed coefficients of b̃k b̃−k ,
tive phase φ̂) can be formally eliminated, and one is left b̃†−k b̃†k in the Hamiltonian get cancelled. Parametriz-
with an effective quadratic theory for k ̸= 0 excitations ing the hyperbolic rotation of modes (k, −k) by a ra-
(parametrically depending on the self-consistent conden- »
(+) 2 (−) 2
sate fraction) [112]. Crucially, in this case, the stability pidity ηk = Fk + Fk and an angle ξk with
(+) (−)
of the Bose-condensed long-range ordered ground state is tan ξk = −Fk /Fk , diagonalization imposes the fol-
a priori guaranteed by the U (1) symmetry. In our spin lowing pair of ordinary differential equations for ηk (φ),
system with γ = 0, the eigenstates with smallest δS are ξk (φ) (see App. E):
ω∂φ ηk sin ξk = +ω̄ sinh ηk cos ξk
h i
+ fk (α) J (0) (φ) sinh ηk cos ξk + J (+) (φ) cosh ηk cos2 ξk + sin2 ξk + 2J (−) (φ) sinh2 (ηk /2) cos ξk sin ξk , (64)
ω∂φ ηk cos ξk = −ω̄ sinh ηk sin ξk
h i
− fk (α) J (0) (φ) sinh ηk sin ξk + 2J (+) (φ) sinh2 (ηk /2) cos ξk sin ξk + J (−) (φ) cosh ηk sin2 ξk + cos2 ξk , (65)
19
where J (0) ≡ J , J (+) ≡ Re K, J (−) ≡ Im K. Note successfully decouples the rotor from the magnons if the
that we obtain differential equations rather than stan- (0)
generator satisfies ω∂φ Fk (φ) ≡ Gk (φ) for all k (see
dard equations because of the non-linear rotor-magnon App. E for more details). In this case, we find that the
interactions. sequential application of eiŜ and eiF̂ fully diagonalizes
To understand the existence conditions of analytic 2π- our effective rotor-magnon Hamiltonian (62):
periodic solutions to Eqs. (64), (65) we first observe that
for α → 0 the second lines vanish, and hence ηk ≡ 0; ˆN+ ω̄k (α)β̃k† β̃k ,
X
eiF̂ eiŜ Ĥα,eff e−iŜ e−iF̂ = LE(α)+ω ∆
linearization in ηk ∼ fk (α) yields the simplified equations k̸=0
(70)
ω∂φ ηk sin ξk = +ω̄ ηk cos ξk + fk (α)J (+) (φ) ,
with a reference energy E(α) = E + 21 k̸=0 (ω̄k (α) − ω̄)
P
(66)
ω∂φ ηk cos ξk = −ω̄ ηk sin ξk − fk (α)J (−) (φ) , dressed by zero-point fluctuations and a nontrivial “dis-
persion relation” for dressed magnons,
which are equivalent (upon renaming P ≡ ηk sin ξk ,
Q ≡ ηk cos ξk , and rescaling the “time” variable φ ≡ ωt) ω̄k (α) ≡ Gk (φ), (71)
to a fictitious harmonic oscillator with natural frequency R 2π
ω̄ externally driven at frequency ω. As is well known, where ·(φ) = 0 dφ 2π · (φ). Here, ω̄k (α) replaces the flat
there always exists a unique periodic trajectory of this band ω̄ of the limit α = 0, cf. Eq. (27); it may be inter-
system with the same frequency ω of the drive (i.e., a 2π- preted as a spectrum of quasiparticle excitations on top
periodic solution in φ), provided ω̄ ̸= rω, for all integers r of a highly excited eigenstate.
appearing in the Fourier representation of J (±) . In corre- The many-body spectrum thus P takes the form
spondence of such resonances {ω̄ = rω}, all solutions are E{nk },δN (α) = LE(α) + ω δN + k̸=0 ω̄k (α)nk : the
unbounded. Remarkably, the existence and uniqueness many-body eigenstates are labelled by the integer quan-
of a solution with the same periodicity as the drive per- tum numbers δN and {nk }k̸=0 continuously from α = 0
sists under a general weak non-linearity [113]. The main to α (away from resonances!). Importantly, however, in
qualitative effect of the non-linearity is to thicken the res- the original unperturbed basis the eigenstates feature
onances from discrete points to finite intervals {|ω̄−rω| ≤ non-trivial quantum entanglement between the rotor
δr } of width depending on the driving amplitude, thus and the magnons, encoded in the inverse canonical
upper bounded as δr ≤ δ0 e−σ|r| Maxk̸=0 |fk (α)| for some transformation e−iŜ e−iF̂ , as is manifest in the expres-
constant σ > 0. This condition provides a theoretical sions (63) and (69).
guarantee of the existence of a finite range of parame-
ter values for which the ansatz (63) successfully diag-
onalizes the magnon part of the effective Hamiltonian.
From a practical point of view, the non-linear equa- G. Self-consistency of localized eigenstates for
0<α<1
tions (64), (65) are known explicitly for a given model,
and one can numerically determine its range of solvability
throughout the parameter space. In the previous Subsection we determined the ex-
Diagonalization of the magnon part of the Hamiltonian act eigenstates of the effective rotor-magnon Hamilto-
brings us within a stone’s throw from the full solution of nian (62) for arbitrary α. An important property of
our problem. The transformed Hamiltonian reads these eigenstates is the extent of delocalization — i.e.
the amount of bare rotor and bare magnon excitations
Xï 1
Å ã ò
† ω̄ they contain — as a function of α. These quantities
iŜ
e Ĥα,eff e −iŜ
= LE +ω δ̂N +
′
Gk (φ̂) β̃k β̃k + − ,
2 2 can be evaluated explicitly and play a crucial role to es-
k̸=0
(67) tablish the regime of self-consistency of the theory, i.e.
where ′
δ̂N and β̃k , β̃k†
denote the dressed (i.e. trans- consistency with the assumptions leading to the effective
formed) rotor and magnon operators, respectively, and Hamiltonian (62): An eigenstate of the effective Hamilto-
nian can represent a legitimate eigenstate of the original
long-range XY spin chain only if its wavefunction remains
Gk (φ̂) ≡ cosh ηk (φ̂) ω̄ + fk (α)J (0) (φ̂)
localized in the subspace δS ≪ L/2, |δN | ≪ L (associ-
+ sinh ηk (φ̂) cos ξk (φ̂) fk (α)J (+) (φ̂) ated with the “vertical” and “horizontal” delocalizations
+ sinh ηk (φ̂) sin ξk (φ̂) fk (α)J (−) (φ̂) . (68) in Fig. 11, respectively).
Both these quantities can be computed within the ex-
As the magnon part is now diagonal, we can diagonal- act solution above. Considering for simplicity an eigen-
ize the rotor part separately in each sector defined by a state in the magnon vacuum tower {nk }k̸D=0 = E ∅ (calcu-
Fock occupation {nk }k̸=0 of dressed magnon modes. In
lation is analogous for other eigenstates), δ̂S is readily
fact, it can be checked that a magnon-diagonal canonical
transformation eiF̂ ansatz, with evaluated as (see App. E)
* +
X (0) Å † 1
ã D E X † X
F̂ = Fk (φ̂) β̃k β̃k + , (69) δ̂S = b̃k b̃k = sinh2 ηk (φ) (72)
2
k̸=0 k̸=0 k̸=0
20
On the other hand, the amount of rotor fluctuations we just replace k fk (α) . . . with k fk (α) . . . every-
P P
in
D an E eigenstate can be estimated by evaluating, e.g., where. As shown in App. A, the properties of fk (α) for
2
δ̂N . Calculation yields an explicit expression, reported α < 1 directly generalize to fk (α) for α < d; in partic-
ular, f squeezes toward k = 0 as L → ∞, and becomes
in App. E.
a function of the discrete wavenumbers kL = 2πℓ, de-
The case 0 < α < 1 is particularly interesting, as the
caying algebraically as |ℓ|−(d−α) . By analogy we denote
values fkℓ (α) ≡ fℓ (α) are discrete and decay as ℓ−(1−α)
fkℓ ≡ fℓ .
(see App. A). Hence, for sufficiently large ℓ we are always
in the linear regime where ηℓ ∝ fℓ (α). This directly leads It follows that the collective spin depletion ⟨δ̂S ⟩ of solv-
to the estimates: able eigenstates is
D E L/2 O(1) for 0 < α < 1/2 ,
D E X O(1) for 0 < α < d/2 ,
log L for α = 1/2 ,
X
δ̂S ∼ |fℓ (α)|2 ∼ δ̂S ∼ |fℓ (α)| ∼
2 log L for α = d/2 ,
2α−1
ℓ=−L/2 L for 1/2 < α < 1 . ℓ L2α−d for d/2 < α < d
(73) (75)
…D E
In this regime, one finds the same qualitative behavior for
…D E Similar estimates apply to 2 . This shows self-
δ̂N
2
δ̂N (see App. E). This prediction for ⟨δ̂S ⟩ has been
consistency of QMBS for 0 < α < d.
shown in Fig.6 above and Fig.15 below, along with the
numerical data. The plot shows complete compatibility
even for finite system size. The joint occurrence 2. General spin-spin interactions
D E …D E
δ̂S ≪ L/2 , 2
δ̂N ≪ L , for 0 < α < 1 (74) Our stability result applies equally well to arbitrary
type of (long-range) spin interactions. For example, con-
graphically illustrated in the right panel of Fig. 11, con- cerning the XYZ spin interactions with ∆ ̸= 0 in Eq. (1),
stitutes a solid analytical argument for our description of our derivation can be straightforwardly generalized. The
QMBS being self-consistent for 0 < α < 1. only addition we need is for terms arising from S̃kz S̃−k
z
in
On the other hand, for α ≳ 1, the delocalization of V̂k : The additional rotated operators read
eigenstates extends to sectors D withE extensively depleted
R π dk −
collective spin δS = O(L), as δ̂S ∼ L −π 2π |fk (α)|2 . z
S̃±k (Ω) = Rz,+ (Ω)S̃±k
+
+ Rz,− (Ω)S̃±k + Rz,z (Ω)S̃±k
z
The small but finite density of magnons breaks the eigen- (76)
state self-consistency, and full hybridization of the QMBS with coefficients computed analogously:
with the thermal bulk may be expected for large L. The
dynamical counterpart of this expectation is that non- Rz,+ (Ω) =Rz,−
∗
(Ω) = − sin(θ)eiϕ ,
(77)
linear magnon-magnon interactions come into play and Rz,z (Ω) = + cos(θ).
trigger the eventual thermalization of initial states with
large collective spin. As such processes are suppressed These extra terms just result in the addition
with the magnon density, thermalization is (at least) +2∆Rz,µ Rz,ν inside the square brackets in Eq. (52). The
parametrically slow as α is decreased toward 1, in agree- rest of the discussion is unchanged.
ment with previous numerical observations [62, 66, 67].
We stress, however, that we are not in a position to rule
out other possible subtler effects which may further delay 3. Higher spins
(or even suppress) thermalization for α ≳ 1.
Our stability result becomes stronger when individual
spins are larger. In fact, an equivalent analysis can be
H. Generality of the theory performed when spins-1/2 are replaced by spins-s with
arbitrary s. This replacement gives more room to the
Here we comment on the generalization of the results accuracy of the bosonic description of spin states, which
of this Section, covering the full range of parameters of requires δS ≪ Ls.
model (1). The only important caveat here is the absence of
self-interactions Jr,r = 0 (which model e.g. single-ion
anisotropy in magnetic materials with higher local
1. Higher dimension spins). We will comment on their effect in Sec. VI below.
Our stability result becomes stronger for higher dimen- To summarize, our analysis straightforwardly carries
sional spin lattices. The only change we need is from over to arbitrary lattices, multi-spin interactions, and
fk (α) to the analogous function fk (α) defined in the d- spin sizes, resulting in the same qualitative conclusion
dimensional Brillouin zone. Throughout our derivation, in all cases.
21
A. Accidental resonances
The theory of Sec. V predicts the stability of QMBS In this Section, we discuss another effect leading to
with i) sufficiently long range of interactions and ii) ab- instability of QMBS: mean-field criticality at finite en-
sence of spectral resonances for α = 0. This theory ra- ergy density. This happens whenever the classical mean-
tionalizes the numerical findings of Sec. IV for the long- field Hamiltonian H has saddle points, which are accom-
range quantum Ising chain with α < 1 and h ≥ J0 , which panied by isolated unstable trajectories terminating on
generically satisfies both conditions. them (phase-space separatrices) with diverging period.
What if conditions i) or ii) fail? In Sec. IV we al- These systems are thus characterized by singularities of
ready presented evidence that violation of the condition the density of states at some finite energy density Ecr /L.
i) (i.e. α > 1) results in asymptotic hybridization of the Such mean-field criticality can (but does not necessarily)
seemingly anomalous finite-size eigenstates. Concerning result from the spontaneous breaking of a discrete sym-
condition ii), the representation of the Hamiltonian in metry. In this case the critical energy separates ordered
Sec. V E in terms of a collective spin coupled to magnon eigenstates (below) from disordered ones (above).
modes gives us a clear and predictive understanding of Such excited-state quantum phase transitions (ES-
QMBS stability. In this Section we explore situations QPTs) [82] have been discussed at mean-field level, see
where, according to our theory, stability is challenged by also Refs. [114–116]. The accumulation of energy eigen-
resonances in the mean-field energy spectrum. values at a given energy density is necessarily associated
with resonances – in the language of Sec. V E one has
We begin by discussing proximity to rare accidental ω(n) = 0. This leads to the failure of eigenstate localiza-
resonances in Sec.VI A, which generically exist for large tion theory. We are thus led to conjecture that quantum
system size. Afterwards, we demonstrate how exponen- many-body chaos develops for α > 0 near the location of
tially diverging classical trajectories of the mean-field a mean-field ESQPT.
Hamiltonian result in instability of QMBS. This happens We numerically assess the impact of finite-range inter-
in correspondence of isolated phase-space separatrices actions on an ESQPT. In Fig. 13 we consider the quan-
(often associated with ESQPT) discussed in Sec. VI B, as tum Ising chain Hamiltonian in Eq. (4) with γ = 1 and
well as of fully developed classical chaos, e.g. generated in the ordered phase h < J0 . In this range of parameters
by strong periodic drives, which we analyze in Sec. VI C. the level spacing distribution agrees with Wigner-Dyson
In all these cases numerical data indicate instability of statistics for α > 0, in agreement with the findings of
QMBS in agreement with our theory predictions. Refs. [80, 81]. In Fig. 13 we take h = 0.4J0 and α = 0.7
22
and check the stability of QMBS for L = 14, 16, 18. In caused by the breaking of classical integrability at mean-
the energy region corresponding to the transition, QMBS field level α = 0. The tight relationship between classical
are unstable and hybridize with the rest of the spectrum, trajectories and semiclassical eigenstates is well estab-
while states well above or below the transition remain lished [117]. When the mean-field integrability-breaking
stable. We find indications of scars hybridization even perturbation is small, Kolmogorov-Arnold-Moser (KAM)
for small α > 0. theory [109] guarantees that the most classical trajec-
tories are deformed tori. In this case the semiclassical
spectrum is regular. Our theory thus predicts generic
stability of QMBS for finite 0 < α < d. Conversely, for
stronger integrability breaking the classical phase space
gradually crosses over to fully developed chaos. In this
case the semiclassical spectrum for α = 0 is well-known
to display statistical properties compatible with random-
matrix universality. As energy eigenvalues are randomly
arranged according to Wigner-Dyson statistics and un-
correlated between adjacent towers in δS , low-order res-
onances become generic, and we expect full eigenstate
delocalization for small α > 0.
We numerically verify the above prediction by studying
the kicked version of the quantum Ising model, with a
time-periodic Hamiltonian defined by the following two-
step protocol,
L L/2
J0 X X σ̂jx σ̂j+r
x ï ã
T T
− t∈ − , mod T
FIG. 13. Fate of the ESQPT for finite-range interactions Nα,L
j=1 r=1
rα 4 4
α > 0. Scatter plot of the observables ⟨δS ⟩En (first row) and Ĥα (t) =
L
entanglement entropy SL/2 (En ) (second row) of each eigen- T 3
ï ã
X
state |En ⟩ versus energy density En /L, for α = 0.7, h = 0.4,
−h
z
σ̂j t∈ , T mod T ,
with L = 14, 16, 18 from left to right. The dashed vertical j=1
4 4
line indicates the location Ecr /L of the ESQPT in the mean- (78)
field limit α = 0. where T is the period of the drive. The evolution over
one period reads
Interestingly, we observe that the energy window of Ç Z T å
instability of QMBS shows a marked asymmetry, ly-
T zT T
Û = Tt exp −i H(t)dt = eiŴα 4 eihŜ 2 eiŴα 4 ,
ing entirely above the mean-field energy density value 0
Ecr /L associated with the ESQPT (dashed vertical lines (79)
in Fig. 13). This global displacement towards higher en- PL PL/2 σ̂jx σ̂j+r
x
ergies can be attributed to finite-size effects, as the win- where Ŵα = NJα,L0
j=1 r=1 . In our numerical
r α
dow slowly drifts downwards in energy (i.e. leftwards in simulations, we fix T = 1 and h = π/2. For α = 0 this is
the Figure) upon increasing L. However, in the weak cou- a textbook model of quantum chaos known as quantum
pling regime (small α), one can give an intuitive physical kicked top. Depending on the value of the interaction
argument for the persistence of the asymmetry for large strength J0 , the model exhibits a transition between a
L based on energy conservation as follows. As the col- regular phase-space – described by KAM theory – and
lective spin is weakly coupled to empty bosonic modes, a chaotic one [118, 119]. Its dynamical properties and
the latter subtract energy from the former, pushing it their relations to quantum information dynamics have
downward in the mean-field energy landscape. Thus, for been intensively investigated [120–134].
energy slightly below Ecr /L, interactions push the collec- We perform exact diagonalization of the unitary oper-
tive spin away from the resonance, leading to stability; ator in Eq. (79) and study the Floquet spectrum
instead, for energy above Ecr /L, they push it towards the
resonance, leading to instability [58, 59]. Û |ϕn ⟩ = eiϕn |ϕn ⟩ , (80)
with ϕn ∈ (−π, π]. We examine the behaviour of Floquet
eigenstates as a function of the chaoticity parameter J0
C. Semiclassical chaos: Periodic kicking and of α. This is illustrated in Fig. 14, where – paral-
leling the analysis of the time-independent Hamiltonian
A cornerstone of our stability theory in Sec. V is clas- version in Fig. 5 – we report a scatter plot the collective
sical integrability of the mean-field Hamiltonian, which spin depletion, the entanglement entropy, and the overlap
implies generic absence of resonances in the unperturbed with a fully polarized state, for each Floquet eigenstate,
spectrum. We here discuss the effects on QMBS for α > 0 versus the Floquet quasi-energy ϕn /π, with fixed L = 18.
23
J0 = 0.5 J0 = 8
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ˆ
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|hEn | *i|2
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FIG. 14. Fate of QMBS in the kicked variable-range quantum Ising model. Here L = 18. Scatter plot of the observables ⟨δS ⟩En
(row a), entanglement entropy SL/2 (En ) (row b), and overlap with the polarized state |⟨↑ |En ⟩|2 (row c), for each eigenstate
|En ⟩, versus energy density En /L. Column 1 has J0 = 0.5, corresponding to the weak-integrability breaking (KAM) regime,
and α = 0.8. Columns 2-5 have J0 = 8, corresponding to the fully chaotic regime of the mean-field dynamics, and increasing
α = 0, 0.2, 0.5, 0.8, respectively.
Results are remarkably sharp even for the small system As shown in the left panel, in the strongly chaotic regime
size we can simulate. ⟨δ̂S ⟩ increases rapidly with L, while the growth is strongly
For small J0 = 0.5 the mean-field classical phase-space suppressed in the regular regime. In this case the scal-
is regular. Correspondingly, the spectral properties in ing of ⟨δ̂S ⟩ with L looks roughly compatible with the
this regime (column 1 of Fig. 14) show clear signatures behavior predicted by the theory of eigenstate localiza-
of stability of QMBS for all 0 < α ≲ 1. The conditions tion, Eq. (73), highlighted by the dashed lines in the right
identified by our theory in Sec. V thus appear necessary panel.
and sufficient for robust QMBS to exist. By contrast, As an important byproduct of our analysis, we have
for J0 = 8 and α = 0, the classical phase-space is fully demonstrated that in periodically driven quantum many-
chaotic. The quantized single-spin spectra within sectors body systems with slowly decaying interactions and non-
labelled by δS thus exhibit random-matrix features (while chaotic mean-field dynamics, energy absorption from the
retaining exact degeneracy among equal-weight SU (2) drive and entropy growth (“heating”) is suppressed for
irreducible representation spaces). This is shown in col- arbitrarily long times. Conversely, in presence of chaotic
umn 2 of Fig. 14. As soon as permutational symmetry mean-field dynamics, heating is fast even for small α > 0.
is broken by finite α > 0 (columns 3-5 of Fig. 14) we This demonstration underlies the findings of Ref. [70].
observe that the eigenstates quickly hybridize, in a way Suppression of heating opens the door to hosting long-
compatible with the onset of strong ETH. In particular, range ordered non-equilibrium phases of matter such as
no signatures of QMBS phenomena appear. We conclude discrete time crystals [135, 136] protected by QMBS sta-
that classical chaos at the mean-field level completely de- bility, similarly to Refs. [137, 138]. See also Ref. [139].
stroys the mechanism of eigenstate localization and sup-
presses all signatures of QMBS, for arbitrarily slow decay
of the interactions. D. Higher spin models
We further analyze the behavior upon increasing the
system size L. In Fig. 15 we plot the collective spin deple- Higher spin Hamiltonians with s > 1/2 can exhibit
tion ⟨δ̂S ⟩ = L/2 − ⟨|Ŝ|⟩ averaged over the L/4 + 1 eigen- chaotic mean-field dynamics even without an external
states with minimum ⟨δ̂S ⟩ (i.e., the candidate QMBS). drive. This happens when the Hamiltonian features ad-
24
dipolar lattices in two but not in three dimensions, of Excellence Matter and Light for Quantum Computing
as the strong anisotropy of interactions has been (ML4Q) EXC 2004/1 -390534769 (S.P.). Views and opin-
theoretically and experimentally shown to cause ions expressed are however those of the authors only and
rapid thermalization [148, 149]. do not necessarily reflect those of the European Union or
the European Research Council. Neither the European
This work furthermore opens future avenues of inves-
Union nor the granting authority can be held responsible
tigation:
for them.
- Our approach — more specifically Eqs. (53)
and (60) — may form the basis of a new class
of computational methods to study non-equilibrium Appendix A: Properties of fk (α)
quantum spin dynamics for arbitrary α. At vari-
ance with other non-equilibrium spin-wave ap- Here we review the properties of the Fourier transform
proaches [58, 59, 64], which inevitably lose accuracy
√ of 1/||r||α on a periodic d-dimensional lattice of V = Ld
over the Ehrenfest time scale (usually TEh ∼ Ld ), sites [same conventions as for Eq. (1)], which we denote
the new method promises to remain accurate at fk (α):
long times, its accuracy being only controlled by α. ,
As it fully takes into account the quantum nature X e−ik·r X 1
of the collective spin wavefunction, subtle long- fk (α) = α
. (A1)
||r|| ||r||α
time non-classicality effects are expected to be ac- r̸=0 r̸=0
1011
109 Krylov time evolution
L=30
dim ℋNshell
107 L=40
105 full ED
L=60
1000 L=90
10
1 2 3 4 5 6 7 8
Nshell
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1/
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1s/2
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1/s2
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1/
s
2
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1s <latexit sha1_base64="cff0vYK4x1PwOF7jkumW5Bj1oow=">AAACCnicbVDJTgJBFOzBDXFDPXrpSEw8kRnjwpHoxSNGWRIg5E3zwA49S7rfaMiEP9Cr/oc349Wf8Df8AmdGDgLWqVL1XqpSbqikIdv+snJLyyura/n1wsbm1vZOcXevYYJIC6yLQAW65YJBJX2skySFrVAjeK7Cpju6Sv3mA2ojA/+OxiF2PRj6ciAFUCLdml6lVyzZZTsDXyTOlJTYFLVe8bvTD0TkoU9CgTFtxw6pG4MmKRROCp3IYAhiBENsJ9QHD003zqpO+FFkgAIeouZS8UzEvx8xeMaMPTe59IDuzbyXiv957YgGlW4s/TAi9EUaRFJhFmSElskGyPtSIxGkzZFLnwvQQIRachAiEaNklJnARzDjpM2kkIzkzE+ySBonZee8fHZzWqpeTufKswN2yI6Zwy5YlV2zGqszwYbsmb2wV+vJerPerY/f05w1/dlnM7A+fwAPxJtD</latexit>
with Nshell ∼ L2α−d for d/2 < α < d, see Eq. (75).
1 2 3 4 5 6 7 8
In the main text, we used this method as a numerical
tool to check the stability of the tower of QMBS with
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ss04
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ss60
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ss002
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for M = 0, 1, . . . , 2S. They can be generated by applying The representation (C10) is non-unique for every finite
M times the rotated lowering operator S: the null vector |ψ⟩ = 0 can be represented with non-
vanishing functions ψ(Ω) (the vector space of complex
U (Ω)Ŝ − U † (Ω) = functions on the sphere is infinite-dimensional, and the
map ψ(Ω) 7→ |ψ⟩ is a projection.)
cos2 (θ/2) Ŝ + − sin2 (θ/2)e−2iϕ Ŝ − − sin(θ)eiϕ Ŝ z (C5)
In Eq. (45) of the main text the coherent-state wave
to the vector |Ω⟩ ≡ |0Ω ⟩. functions of the eigenstates |M⇑ ⟩ of Ŝ z appear. To com-
The overlap between two spin-coherent states is pute them, we can proceed as follows. First, we can write
tion, first observe that the operator dΩ |Ω⟩⟨Ω| com- of the eigenstate of Ŝ z as a classical trajectory on the
mutes with all rotations, hence it is proportional to the sphere.
identity (Schur’s lemma). The proportionality factor can
be found e.g. by taking the expectation value on |⃗z⟩:
d. Semiclassical limit of spin-coherent kernels
ã2S
1 + cos θ 4π
Z 2π Z π Å
dϕ dθ sin θ = . (C9) In Eq. (54) we encounter an expression of the form
0 0 2 2S + 1
Z Z
′
dΩ ′
dΩ ψδ∗ (Ω′ )ψ0 (Ω) K(Ω′ , Ω) J(Ω) ⟨Ω|Ω′ ⟩ ,
c. Coherent-state wave functions (C16)
where the braket is between spin-S coherent states, and
The overcomplete basis property implies that every ψ0 , ψδ′ are the coherent-state wavefunctions of two eigen-
state in Hilbert space can be written as a linear com- ⃗ˆ
states of a Hamiltonian H(S/S) of a single spin of size S
bination of spin-coherent states:
and S 7→ S + δ, respectively, and K and J are analytic
functions on the sphere. We want to show for fixed δ this
Z
|ψ⟩ = dΩ ψ(Ω)|Ω⟩ . (C10) expression is equivalent to
b. Second step
a. First step
1 X † †
R̂ = − b̃0 b̃q1 b̃q2 b̃q1 +q2 + b̃†q1 b̃†q2 b̃q1 +q2 b̃0 + H.c.
2 q ,q
1 2
1 X †
+ b̃q1 +q2 b̃q1 b̃q2 b̃†q3 b̃†q4 b̃q3 +q4
2L q ,q ,q ,q
Å ãÅ ã
L X † L X †
Ŝ 2 = − b̃k b̃k − b̃k b̃k + 1 1 2 3 4
2 2
+ b̃†q1 b̃†q2 b̃q1 +q2 b̃†q3 +q4 b̃q3 b̃q4 . (D14)
k̸=0 k̸=0
X † †
X †
+ b̃k b̃k + 2b̃k=0 b̃k=0 b̃k b̃k + R̂ . (D12)
k̸=0 k̸=0 Now, let us evaluate the action of these operators on
the state |{nk }⟩ with δS bosons with non-vanishing mo-
menta. It is straightforward to see that terms in the first
line generate δS2 block-off-diagonal contributions (they
scatter two k ̸= 0 magnons to one k ̸= 0 magnon plus one
From the first line we recognize the leading-order identi- k = 0 magnon). The perturbative dressing of the state
|{nk }⟩, i.e. (matrix element/eigenvalue mismatch)2 , is
P
fication of the collective spin size eigenvalue
thus of order O(δS2 /L2 ). The remaining terms give both
block-diagonal contributions (which do not affect the pro-
jection space) and δS3 block-off-diagonal contributions.
By the same line of argument, the latter yield a per-
turbative dressing of the state |{nk }⟩ of order O(δS3 /L4 ).
L X † □
b̃†k b̃k .
X
S= − b̃k b̃k , i.e. δS = (D13)
2 We finally note that the exact projector is also harm-
k̸=0 k̸=0 −
less for states with M > 0, as S̃k=0 commutes with the
projector. This immediately implies Eq. (39).
1X h i
b̃†k b̃k + fk J (φ̂) b̃†k b̃k + J (φ̂) b̃−k b̃†−k + K(φ̂) b̃−k b̃k + K∗ (φ̂) b̃†k b̃†−k , (E1)
X
Ĥ = ω δ̂N + ω̄
2
k̸=0 k̸=0
describing a quantum rotor with quantized angular momentum δˆN and conjugate phase φ̂, interacting with an ensemble
of bosonic modes labelled by k, described by canonical annihilation and creation operators b̃k , b̃†k .
Such a Hamiltonian can be diagonalized using a sequence of two canonical transformation. First, we introduce a
canonical transformation eiŜ with a generator of the form
⃗ˆk
X ï (0) (0) (+) (+) (−) (−)
ò X
Ŝ = Fk (φ̂) Âk + Fk (φ̂) Âk + Fk (φ̂) Âk ≡ F⃗k (φ̂) · A (E2)
k̸=0 k̸=0
31
These operators are hermitian generators of the two- implementing the adjoint representation of the SO(2, 1)
boson quadratic algebra for each pair (k, −k): algebra.
(0) (∓) (−) (0)
[Âk , Â(±)
q ] = ±iÂk δk,q ,[Âk , Â(+)
q ] = +iÂk δk,q
(E4)
(here we recognize SO(2, 1) commutation relations). The With these ingredients at hand we can compute the
generator (E2) has the following properties: i) it is inde- transformed Hamiltonian:
pendent of δ̂N ; ii) it is quadratic in the bosonic operators;
iii) it does not mix pairs of bosonic modes with different
momentum. Basically, the ansatz (E2) represents a kind
of generalized Bogolubov transformation where the “an-
gles” depend on the collective operator φ̂. Our goal is
to determine functions F⃗k (φ̂) which cancel the last two
terms in Eq. (E1). eiŜ Ĥ e−iŜ = −ω δ̂N
To this aim, let us compute the transformed effective
⃗ˆk ,
Xï ò
+ − ω∂φ F⃗k (φ̂) + ω̄⃗e1 + fk J⃗ (φ̂) eFk (φ̂) · A
Hamiltonian Ĥ 7→ eiŜ Ĥe−iŜ . First of all, we rewrite Ĥ
in the compact form k̸=0
(E11)
T
X (0)
X
⃗ˆk , (E5) where ⃗e1 ≡ 1 0 0 . We see that, compared to
Ĥ = ω δ̂N + ω̄ Âk + fk J⃗ (φ̂) · A
Eq. (E5), the effect of the transformation is to mix the
⃗ˆk via the matrix eFk
k̸=0 k̸=0
coefficients of the operator vector A
where we omitted the constant −Lω̄/2 for simplicity, and transposed and to add −ω∂φ Fk . Our ansatz is successful
⃗
if we can choose functions F⃗k (φ) such that the trans-
J (0) (φ) ≡ J (φ), (±)
formed coefficients of Âk become zero, i.e. the magnon
J (+) (φ) ≡ Re K(φ), (E6) Hamiltonian becomes diagonal.
J (−) (φ) ≡ Im K(φ).
Hence, we need the following ingredients: As we have two equations and three variables per mo-
(0) (±)
mentum to play with (i.e. Fk , Fk ), we can restrict
eiŜ δ̂N e−iŜ = δ̂N − ∂φ Ŝ ; (E7) (0)
the ansatz. A convenient choice is to set Fk ≡ 0.
eiŜ J⃗ (φ̂)e−iŜ = J⃗ (φ̂) ; (E8) In this case the matrix e Fk
becomes a hyperbolic ro-
⃗ˆk e−iŜ = exp Fk (φ̂) · A
⃗ˆk ; tation»(or Lorentz boost) parametrized by a rapidity
eiŜ A (E9) (+) 2 (−) 2
ηk = Fk + Fk and an angle ξk with tan ξk =
(+) (−)
here we defined the matrix −Fk /Fk . Imposing the vanishing of the second and
Ö
(−) (+)
è third coefficients yields the following pair of ordinary
0 −Fk +Fk differential equations for the unknown functions ηk (φ),
Fk (φ̂) ≡ −Fk(−) 0 −Fk
(0)
(E10) ξk (φ):
(+) (0)
+Fk +Fk 0
ω∂φ ηk sin ξk = +ω̄ sinh ηk cos ξk
h i
+ fk J (0) (φ) sinh ηk cos ξk + J (+) (φ) cosh ηk cos2 ξk + sin2 ξk + 2J (−) (φ) sinh2 (ηk /2) cos ξk sin ξk ; (E12)
ω∂φ ηk cos ξk = −ω̄ sinh ηk sin ξk
h i
− fk J (0) (φ) sinh ηk sin ξk + 2J (+) (φ) sinh2 (ηk /2) cos ξk sin ξk + J (−) (φ) cosh ηk sin2 ξk + cos2 ξk . (E13)
32
We look for analytic 2π-periodic solutions. To convince Importantly, the functions Gk are analytic in φ (and
ourselves that such solutions exist, we can proceed as smoothly vary with n).
follows. First, a quick inspection of the equations reveals From Eq. (E15) we can read off the eigenvalues and
that for fk → 0 the second lines vanish, and hence ηk ≡ 0 eigenstates of the Hamiltonian. As the bosonic part is
solves the equations. (Indeed, in this limit the effective now diagonal, we can choose a factorized ansatz for the
Hamiltonian is already in diagonal form, as we know.) eigenstate wavefunction
Thus, for small fk we have ηk ∼ fk , and it makes sense to
linearize the equations in fk . This gives us the simplified |Ψ{nk }k̸=0 ⟩ ≡ |ψ⟩ ⊗ |{nk }k̸=0 ⟩. (E17)
pair of equations
where the bosonic part is a Fock state in the Bogolubov-
ω∂φ ηk sin ξk = +ω̄ ηk cos ξk + fk J (+) (φ) , rotated basis. The rotor wavefunction |ψ⟩ is subject to
(E14) a reduced Hamiltonian with a potential that parametri-
ω∂φ ηk cos ξk = −ω̄ ηk sin ξk − fk J (−) (φ) . cally depends on the Fock state:
Now, renaming the variables as P ≡ ηk sin ξk , Q ≡ ⟨{nk }k̸=0 |Ĥ|{nk }k̸=0 ⟩ = ω δ̂N
′
+ G{nk } (φ̂) (E18)
ηk cos ξk , and rescaling the “time” variable φ ≡ ωt, we
recognize equivalence with a fictitious harmonic oscilla- where we defined
tor with coordinate Q, momentum P , and natural fre-
quency ω̄, externally driven at frequency ω. As it is well 1
X Å ã
G{nk } (φ̂) ≡ Gk (φ̂) nk + . (E19)
known, there always exists a unique periodic trajectory 2
k̸=0
of this system with the same frequency ω of the drive
(i.e., a 2π-periodic solution in the original variable φ), This Hamiltonian is equivalent to a Wannier-Stark lad-
provided the natural frequency ω̄ does not equal any fre- der, i.e. a single particle hopping on a chain and subject
quency component of the drive, i.e. provided ω̄ ̸= rω, for to a linear potential. Here the integer δN plays the role
all integers r appearing in the Fourier representation of of the chain sites, ω̄ plays the role of the potential slope,
J (±) . In correspondence of such resonances {ω̄ = rω}, and the Fourier components of G{nk } (φ) play the role
all solutions are unbounded. of hopping amplitudes; analyticity guarantees that the
Remarkably, the analysis of the linearized regime en- hopping amplitudes decay exponentially for all choices of
lightens the general scenario, as the existence and unique- {nk }. This problem can be easily diagonalized by a uni-
ness of a solution with the same periodicity as the drive
tary transformation of the form eiF{nk } (φ̂) , upon choosing
persists under a general weak non-linearity: see, e.g.,
the function F{nk } (φ) so as to remove the oscillating part
Chapter 2 of the book in Ref. [113]. The main qualita-
of G{nk } . To this aim, let us define the averaging symbol
tive effect of the non-linearity is to thicken the resonances R 2π
from discrete points to finite intervals {|ω̄ − rω| ≤ δr } of ·(φ) = 0 dφ 2π · (φ), and split
width depending on the driving amplitude, thus upper
bounded as δr ≤ δ0 e−σ|r| Maxk̸=0 |fk |. This condition G{nk } (φ) = E{nk } + T{nk } (φ) (E20)
provides a theoretical guarantee of the existence of a fi-
nite range of parameter values for which our generalized where
Bogolubov transformation successfully diagonalizes the X Å
1
ã
bosonic part of the Hamiltonian. From a practical point E{nk } ≡ G{nk } (φ) = Gk (φ) nk + (E21)
2
of view, the non-linear equations (E12), (E13) are known k̸=0
explicitly for a given model, and one can numerically de-
termine its range of solvability throughout the parameter is a constant and T{nk } (φ) is an oscillating function with
space. zero average, T{nk } (φ) = 0. Now, we can pick a gen-
Diagonalization of the bosonic Hamiltonian brings us erating function F{nk } such that ω∂φ F{nk } = T{nk } (φ)
within a stone’s throw from the full solution of our prob- [cf. Eq. (E7)]. After this transformation, the reduced
lem. The transformed Hamiltonian reads Hamiltonian becomes diagonal. The spectrum is still an
equi-spaced ladder with spacing ω, rigidly shifted by the
1
Å ã
Gk (φ̂) β̃k† β̃k + quantity E{nk } depending on the magnon state.
X
eiŜ Ĥ e−iŜ = ω δ̂N
′
+ , (E15)
2 We can thus assemble a unitary transformation eiF̂ in
k̸=0
the full many-body Hilbert space by taking the direct
where δ̂N
′
and β̃k , β̃k† denote here the dressed (i.e. trans- product of the unitaries eiF{nk } (φ̂) in each sector with
formed) rotor and bosons, and fixed bosonic state |{nk }⟩. Explicitly, the rotor part of
eiŜ Ĥ e−iŜ in Eq. (E15) is diagonalized by the canonical
Gk (φ̂) ≡ cosh ηk (φ̂) ω̄ + fk J (0) (φ̂) transformation eiF̂ with generator
+ fk sinh ηk (φ̂) cos ξk (φ̂) J (+) (φ̂) Å
1
ã
†
X
F̂ = Fk (φ̂) β̃k β̃k + (E22)
+ fk sinh ηk (φ̂) sin ξk (φ̂) J (−) (φ̂) . (E16) 2
k̸=0
33
D E ã2
ˆ
Å X
δ̂N = ⟨0, ∅|e e δ̂N e e
2 iF̂ iŜ 2 −iŜ −iF̂
|0, ∅⟩ = ⟨0, ∅| ∂φ F∅ + ⃗ ⃗
∂φ Fk · Ak |0, ∅⟩
k̸=0
1 1X
(+) (+) (−) (−)
= 2 ⟨0, ∅|T∅2 (φ̂)|0, ∅⟩ + ⟨0, ∅| ∂φ Fk (φ̂)∂φ Fk (φ̂) + ∂φ Fk (φ̂)∂φ Fk (φ̂) |0, ∅⟩
ω 2
k̸=0
" #2
1 X 1X
Å ã
(+) (+) (−) (−)
= Gk (φ) − Gk (φ) + ∂φ Fk (φ)∂φ Fk (φ) + ∂φ Fk (φ)∂φ Fk (φ) (E28)
4ω 2 2
k̸=0 k̸=0
In the perturbative regime ηk (φ) ∼ fk one has Gk (φ) − general, it must be noted that in theP problem treated in
(±)
Gk (φ) ∼ fk as well as Fk (φ) ∼ fk (both the right- the main text one has the sum rule k fk = 0 (see the
hand sides implicitly contain a k-independent analytic definition in App. A). In this case, the leading contri-
function of φ). The first term thus gives a contribution bution to the first term is given by the next-to-leading
P 2 order expansion
∼ f , whereas the second term gives a contri- …DGk (φ)E
− Gk (φ) ∼ fk2 . Then one finds
k̸=0 k
the estimate 2
k̸=0 |fk | for the amount of
2
P
δ̂N ∼
bution ∼ k̸=0 |fk |2 . While the relative impact of these
P
two terms depends on the signs of the couplings {fk } in rotor excitations, qualitatively similar to the amount of
magnon excitations in Eq. (E27).
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