Professional Documents
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ingles 11-50
ingles 11-50
VENTILATION SYSTEMS*
-1 - bO(;UMiENT
DISCLAIMER
The HEPA filters used in the nuclear industry to remove radioactive airborne
contaminants are extremely effective and practical devices and will continue to be
so despite the large number of new control devices presently available. However,
HEPA filters generate a significant volume of radioactive waste and are costly to
purchase and operate. The actual cost of materials and labor to buy, change,
test, and dispose of a HEPA filter is several times its initial purchase price.
In an effort to reduce the HEPA's operational cost and the volume of radioactive
waste it generates, the Nuclear Fuel Cycle and Waste Management Division of DOE
has contracted with LLNL to develop an enhanced filtration system that will extend
the service life of HEPA filters. The approach selectedlbyLLNL consists of using 4
an electrofibrous prefilter to take the load off the HEPA filter, since it appears
to have a greater potential for success than other methods, such as scrubbers and
electrostatic precipitators.
The electrofibrous filter represents the best technology for removing
airborne particles. Compared to a conventional fibrous f'ilter, the electrofibrous
filter has a much higher efficiency and significantly lower pressure drop at the
same level of particle loading. This dramatic increase iln filter performance due
to the added electrical forces has recently created a world-wide interest in this
field. A symposium on F.ibers, Electrostatics and Filters that was held in
Princeton, New Jersey in November 1979, illustrated tne diversity of techniques
used to generate electrof i brous f i 1 ters( 1.
The concepts used in our electrofibrous prefilter are not new. Electrostatics
have been used to improve the performance of fibrous filters since 1930. Although
the electrofibrous filters can have a number of different configurations, all are
based on either charging or polarizing the filter fibers,, This generates an
electrical force between the fibers and particles and reqjults in a large increase
in the filter efficiency and filter life. The primary methods for generating
electrofibrous filters include precharging the aerosols, polarizing the filter
media with electric fields, a combination of these two methods an ermanently
?
charging the fibers. These methods have been reviewed previously 27 .
LLNL has established a comprehensive program to conduct theoretical
modelling, small-scale laboratory experiments, prototype development and field
evaluations of electrofibrous prefilters. The objective of our theory and
laboratory experiments is to understand the mechanical and electrical filtration
mechanisms for both clean and clogged filters in sufficient detail to optimize the
electrofibrous filter. Although we have not yet completed this optimization
study, we have identified the important parameters in thle prototye design and have
established general design criteria.
Using these design criteria, we have been developing prototype electrofibrous
prefilters for use in radioactive gloved boxes and in nuclear ventilation
systems. The design and field evaluation our prototype filters for gloved box 'I
-2-
ponents o f the
d in Fig. 1. A
s separated by
1'
charger upstream o
' Another class o
-3-
charged p a r t i c l e s o f r e s i n a r e s c a t t e r e d o v e r t h e s u r f a c e l o f t h e wool f i b e r s . The
r e s i n p a r t i c l e s become h i g h l y charged due t o f r i c t i o n a l cl;arging d u r i n g t h e
m a n u f a c t u r i n g process i n which t h e w o o l - r e s i n m i x t u r e i s (;:ombed on a t e x t i l e
c a r d i n g machine. S i n c e t h e r e s i n p a r t i c l e s have a h i g h r e s i s t i v i t y , t h e y can
r e t a i n t h e charge f o r l o n g p e r i o d s o f time. These h i g h l y l c h a r g e d r e s i n p a r t i c l e s
c a n a t t r a c t a e r o s o l s t h r o u g h e l e c t r o s t a t i c f o r c e s and a r e l r e s p o n s i b l e f o r t n e h i g h
e f f i c i e n c y o f tiansen f i l t e r s . U n f o r t u n a t e l y , t h e r e s i n p , ! r t i c l e s can be
d i s c h a r g e d when exposed t o i o n i z i n g r a d i a t i o n , c o n c e n t r a t e d o r g a n i c s o l v e n t s , o r
e x c e s s i v e h e a t . When t h i s happens, t h e Hansen f i l t e r bec#nes a v e r y p o o r f i l t e r .
Because o f t h e p o t e n t i a l d i s c h a r g i n g problem and t h e f l a m y a b i l i t y o f t h e wool
f i b e r s , we d i d n o t b e l i e v e t h a t t h e Hansen f i l t e r c o u l d be used i n n u c l e a r
v e n t i l a t i o n systems.
111. Theory o f E l e c t r o f i b r o u s F i l i-
ter
D e v e l o p i n g an a c c u r a t e t h e o r y o f t h e e l e c t r o f i b r o u s f i l t e r i s an i m p o r t a n t
p a r t o f o u r f i l t r a t i o n program. T h i s t h e o r y w i l l be used t o o p t i m i z e t h e d e s i g n
o f o u r p r o t o t y p e e l e c t r o f i b r o u s f i l t e r s . Since a d e t a i l e d d e s c r i p t i o n o f t h e
t h e o r y was I r e d p u b l i s h e d , we s h a l l D r i e f l y r e v i e w t h e e s s e n t i a l f e a t u r e s o f
t h e t h e ~ r y ( ~ , ~ , ~ The ~ T .dominant c h a r a c t e r i s t i c s o f t h e e l e c t r o f i b r o u s f i l t e r
t h a t must be t h e o r e t i c a l l y e x p l a i n e d a r e ( 1 ) t h e h i g h e r e f f i c i e n c y and ( 2 ) t h e
l o n g e r f i l t e r l i f e when compared t o a c o n v e n t i o n a l f i b r o u s f i l t e r . The i n c r e a s e d
f i l t e r e f f i c i e n c y due t o t h e a p p l i e d e l e c t r i c f i e l d was p r e v i o u s l y shown i n F i g . 1.
When an e x t e r n a l e l e c t r i c f i e l d i s f i r s t a p p l i e d t o t h e f i l t e r , t h e o n l y
c a p t u r e mechanism i s due t o t h e f o r c e s between a p o l a r i z e d f i b e r and a p o l a r i z e d
o r charged p a r t i c l e . The e l e c t r i c f i e l d i n s t a n t l y p o l a r i z e s t h e f i b e r , which t h e n
a t t r a c t s b o t h charged and p o l a r i z e d p a r t i c l e s . The charged p a r t i c l e s t h a t d e p o s i t
on t h e f i b e r t h e n g r a d u a l l y b u i l d up a f i b e r charge which i n t r o d u c e s t h e second
mechanism. T h i s mechanism i s based on t h e f o r c e between charged f i b e r s and
charged o r p o l a r i z e d p a r t i c l e s . The i n c r e a s e d f i l t e r e f f i c i e n c y i s t h u s due t o a
t i m e independent a t t r a c t i o n between p o l a r i z e d f i b e r s and a e r o s o l s , and a t i m e
dependent a t t r a c t i o n between charged f i b e r s and a e r o s o l s . An e q u i l i b r i u m charge
i s e s t a b l i s h e d on t h e f i b e r i n a dynamic process o f charge a c c u m u l a t i o n due t o t h e
p a r t i c l e d e p o s i t s and charge d i s s i p a t i o n due t o t h e f i b e r c o n d u c t i v i t y . Other
r e s e a r c h e r s have n o t c o n s i d e r e d t h e t i m e dependent mechanism i n v o l v i n g f i b e r '4
cnarge and c o u l d t h e r e f o r e n o t e x p l a i n many e x p e r i m e n t a l f i n d i n g s . 9
F i g u r e 2 i l l u s t r a t e s t h e two p a r t i c l e c a p t u r e mechanisms t h a t a r e r e s p o n s i b l e
f o r i n c r e a s i n g t h e f i l t e r e f f i c i e n c y . The l a r g e r and s m a l l e r c i r c l e s r e p r e s e n t
t n e c r o s s s e c t i o n s o f t h e f i b e r s and t h e charged p a r t i c l e s r e s p e c t i v e l y . The
s o l i d l i n e s a r e t h e e l e c t r i c a l l i n e s o f force, w h i l e theIdashed l i n e s a r e t h e
p a r t i c l e t r a j e c t o r i e s f o r t h e two c a p t u r e mechanisms. Triese c a p t u r e mechanisms
a r e due t o t h e i n t e r a c t i o n between a p o l a r i z e d f i b e r a n d l a charged p a r t i c l e , and
-4-
the interaction between a charged fiber and a charged particle. The same basic
mechanisms are also valid for uncharged particles, in which case, we must replace
the charged particles with polarized particles.
1.t
0.5
I
Charged fiber -'charged particle 0.0
(fiber charged from the deposition 0 1 2 3 4 5 6 7
of charged particles) Particle mass - g
Figure 2 Figure 3
Electrical capture mechanisms The appl ied electric fie1 d increases
responsible for the increased the filter service 1 ife,
filter efficiency.
-5-
c a p t u r e d by f i b e r s on t h e f r o n t f a c e o f t h e f i l t e r , where more p a r t i c l e d e p o s i t s
can be accommodated because t h e f i b e r p a c k i n g d e n s i t y is1 v e r y low. The i n c r e a s e d
f i b e r e f f i c i e n c y due t o t h e e l e c t r i c f i e l d i s r e s p o n s i b l e f o r t h e enhanced
p a r t i c l e c o l l e c t i o n on t h e f r o n t f a c e o f t h e f i l t e r . F i g . 4 shows t h a t t h e
p a r t i c l e d e p o s i t s on t h e f r o n t f a c e of t h e f i l t e r f o r m a~more open s t r u c t u r e ( F i g .
4B) t h a n t h e d e p o s i t s w i t h i n t h e f i l t e r volume ( F i g . 4A).
On a m i c r o s c o p i c s c a l e , t h e e f f e c t of t h e a p p l i e d e l l e c t r i c f i e l d i s t o extend
t h e p e r i o d i n which t h e p a r t i c l e d e p o s i t s a r e i n t h e f i r s t s t a g e o f f i l t e r
c l o g g i n g . Payatakes has c h a r a c t e r i z e d f i l t e r c l o g g i n g ajs a s e q u e n t i a l p
which t h e morphology o f p a r t i c l e d e p o s i t s goes t h r o u g h f o u r m a j o r stages
I n t h e f i r s t s t a g e p a r t i c l e s d e p o s i t d i r e c t l y on t h e f i b j e r and f o r m a random
c o v e r i n g o f i s o l a t e d p a r t i c l e s . I n t h e second stage, p a r t i c l e s d e p o s i t
p r e f e r e n t i a l l y on p r e v i o u s l y d e p o s i t e d p a r t i c l e s and f o r m extended p a r t i c l e c h a i n s
c a l l e d d e n d r i t e s . T h i s s t a g e o f f i l t e r c l o g g i n g i s i l l u s t r a t e d i n F i g . 5A where
t h e l a r g e and s m a l l c i r c l e s r e p r e s e n t t h e f i b e r and p a r t / i c l e d e p o s i t s
r e s p e c t i v e l y . The d e n d r i t e s i n t e r m e s h w i t h n e i g h b o r i n g d e n d r i t e s i n t h e t h i r d
s t a g e and b r i d g e between n e i g h b o r i n g f i b e r s i n t h e f o u r t l h and f i n a l s t a g e o f
f i l t e r c l o g g i n g . W i t h a superimposed e l e c t r i c f i e l d , t h e i n c r e a s e d c o l l e c t i o n
e f f i c i e n c y r e s u l t s i n a more dense and u n i f o r m s u r f a c e cloverage d u r i n g t h e e a r l y
stages o f f i l t e r c l o g g i n g as shown i n F i g . 5B. The e l e c l t r i c a l f o r c e s cause
p a r t i c l e s t o d e p o s i t on t h e downstream s i d e o f t h e f i b e q and f i l l i n t h e open
spaces on t h e upstream s i d e t h a t were i n a c c e s s i b l e t o mechanical c a p t u r e . Thus
f o r t h e same q u a n t i t y o f p a r t i c l e s t r a p p e d on a f i b e r , tihe d e p o s i t s formed due t o
e l e c t r i c a l c a p t u r e a r e i n s t a g e 1 ( F i g . 5 6 ) w h i l e t h e d e p o s i t s formed due t o
mechanical c a p t u r e a r e in s t a g e 2 ( F i g . 5A). The lower I a i r r e s i s t a n c e o f t h e
d e p o s i t s i n s t a g e 1 accounts f o r t h e decreased p r e s s u r e d r o p when f i l t e r s a r e
o p e r a t e d w i t h an e l e c t r i c f i e l d .
8a Figure 5
A Schematic of
p a r t i c l e deposits
on a f i b e r ( A )
w i t h o u t an e l e c t r i c
f i e l d and (B) w i t h
an e l e c t r i c f i e l d .
A B
Figure 4
Schematic o f t h e f i l t e r c r o s s s e c t i o n B
showing t h e p a r t i c l e d e p o s i t s [A) w i t h -
o u t an e l e c t r i c f i e l d and (B) w i t h an
electric field.
I V . Desisn C r i t e r i a f o r P r o t o t w e Electrol'ibrous F i l t e r s
The d e s i g n of a p r o t o t y p e e l e c t r o f i b r o u s f i l t e r fot; n u c l e a r v e n t i l a t i o n
systems r e q u i r e s making a number o f d e c i s i o n s on key f i l l t e r parameters. The
c r i t e r i a used f o r making t h e s e d e c i s i o n s a r e summarized i n T a b l e I .
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Tab e I . Des gn c r i t e r i a f o r e l e c t r o f i b r o u s f i l t e r s
D e s i g n parameter Criterion
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After the physical dimensions,
the most important design parameter
is the f.ilter face velocity, which
should h(;ve a minimum value. A lower
face velocity will decrease the
filter resistance and increase the
filter efficiency and dust holding
capacity, Figure 6 illustrates the
increased filter efficiency for
electrofibrous filters due to a
decreased face velocity. This figure
shows the efficiency as a function of
the applied electric field for the
same filcer operated at three
0 0.16 m/s different face velocities. A lower
0 0.32m/s face velocity produces a higher
filter efficiency because the
A 0.65 m/s electricdl forces have a longer time
to attract particles to the filter
fibers. The most common technique
for decreasing the face velocity is
to increase the filtering area by
pleating the filtering element; the
0.5 1.o 1.5 number o f pleats being governed Dy
the thickness of the filtering
Electric field, MV/m element and the ease o f r e p l a c i n g t h e
Figure 6 filter medium.
-8 -
I 1 I I C
electrofibrous filters during filter
12 I clogging. However, we believe that
0 Clean 8 Clogged far better results can be achieved by
designing a filter with the optimum
gradation in fiber packing density.
Another property of the filter
medium that is closely related to the
fiber packing density is the
compressibility of the filter mat.
Since compressing the filter mat will
increase the fiber packing density and
consequently the pressure drop, we
LL
want to have filter media that has a
0 minimum compressibility. Figure 7
0 20 40 60 80 100 shows the filter compression that
Velocity , cm/s occurs due to the air flow through the
media. We have plotted the filter
Figure 7 thickness as a function of the air
velocity for clean and clogged AF-4
Filter thickness as a function of air and AF-18 filters. We see that the
f l o w velocity for clean and clogged AF-18 medium is only moderately
AF-4 and AF-18 filters. compessed compared to the AF-4
medium. Figure 7 also shows that
there is an additional compression due
to the particle deposits in clogged
filters. Althouqh this additional
compression is insignificant for the AF-18 medium, it is very large for the AF-4
riiedium. The increased compression for the AF-4 medium is due to the smaller
diameter fibers that are easier to bend. The AF-4 filter has a median fiber
diameter of 0.73pm while the AF-18 filter has a median fiber diameter of
3.5 p m .
The final criterion listed in Table I for the ideal filter medium is a
minimum water adsorption. It is a well established phenomenon that water
adsorbed on an insulator will dramatically increase the surface conductivity. For
exa ple, the surface conductivity of soda lime glass increaf73)from 10-l' to
lo-' mhos as the relative humidity increases from 40 to 90% . This
i n c r e a s e d c o n d u c t i v i t y w i l l lead t o an increased c u r r e n t flow and e v e n t u a l l y s h o r t
circuiting across the high voltage electrodes.
This phenomenon is illustrated in Fig. 8 which shows the filter efficiency and
the electrode current as a function of the relative humidity. The data was
obtained using an AF-18 medium sandwiched between two electrode screens as shown
in Fig. 1. Since sodium chloride aerosols are hygroscopic, we used DOP aerosols
generated Dy nebulizing a solution o f DOP in alcohol. Efficiencies were
determined using a Sinclair-Phoenix light scattering photometer. Figure 8 shows
that the filter efficiency witn and without an applied voltage remains constant
over the relative humidities tested. Below 70% relative humidity, the electrode
current i's less than 0.5 PA. However, beyond 80% relative humidity, the current
rapidly increases until there is a snort circuiting across the electrodes at 90%
relative humidity. Since the water adsorption is much less for most plastics than
for glass (e.g., polypropylene absorbs about 0.02% water compared to 0.3% for
glass), we would expect that electrof brous filters made from plastic fibers can
operate at a much higher relative hum dity.
-9-
100 - 200
80 - = O r + : 150
5
c,
-
E
aJ
L
60 L
3 Figure 8
V
100
-0 F i l t e r e f f i c i e n c y and
0
L
40 c, e l e c t r o d e c u r r e n t as a f u n c t i o n
u o f re1,ative humidity f o r
50 EI
Q,
.
e l e c t r o f ib r o u s f i 1t e r
20
0 0
One o f t h e most i m p o r t a n t c r i t e r i a f o r t h e d e s i g n o f t h e h i g h v o l t a g e
e l e c t r o d e s i s a good e l e c t r i c a l c o n t a c t w i t h t h e f i l t e r medium. We have shown
t h a t i f t h e f i l t e r medium does n o t have good e l e c t r i c a l c o n t a c t W i t h t h e
e l e c t r o d e s , t h e e l e c t r o f ' b r us f i l t e r w i l l have t h e same performance as a f i l t e r
w i t h no a p p l i e d v o l t a g e.7'9'( T h i s phenomenon o c c u r s bec,:ause t h e f i b e r charge
m i g r a t e s across t h e f i l t e r bed and accumulates n e x t t o t h e e l e c t r o d e s i f t h e y a r e
n o t i n c o n t a c t w i t h t h e medium. The accumulated charge c r e a t e s an e l e c t r i c f i e l d
w i t h i n t h e f i l t e r medium t h a t c a n c e l s t h e f i e l d produced b y t h e h i g h v o l t a g e
e l e c t r o d e s . However, i f t h e e l e c t r o d e s a r e i n c o n t a c t w i t h t h e medium, t h e f i b e r
-1 0-
charge that migrates to the electrodes is neutralized and therefore can not reduce
the electric field generated by the electrodes. One of the primary causes for
losing electrode contact with the medium is the compression due to air flow as
seen in Fig. 7.
The criterion for designing the high voltage electrode for the optimum
electric field orientation is.not well established. All of our studies have been
conducted with the electric field either parallel or anti parallel to the air
flow. No change in the filter efficiency was observed with either orientation.
We chose to apply high voltage to the rear electrode in our prototype filters to
minimize the possibility of particle deposits creating a leak path or even a short
circuit between the high voltage and the grounded filter housing. Grounding the
front electrode also provides an additional safety feature against accidental
short circuits and electric shock hazard.
Lamb et a1 have performed a series of experimen n the effect of the
electric field orientation on the filter efficiencylf4?. They concluded that
the electric field perpendicular to the air flow produced a much higher filter
efficiency than the field parallel or anti parallel to the air flow.
Unfortunately the electrodes were not contacting the filter medium in the
experiments with the parallel and anti parallel configuration, thereby
invalidating the conclusions. The optimum field orientation for the maximum
filter efficiency must still be determined.
The criterion for having electrodes with a high electrical resistanc
established to minimize the potential for sparking across the electrodes h sa:
Sparking across the electrodes is undesirable because of the potential fire hazard
ana the decreased voltage a r s the electrodes which decreases the filter
efficiency. Thompson et a1 f1'7 have shown that the use o f high resistance
electrodes can significantly reduce the potential for sparKing across the
electrodes. High resistance electrodes also reduce the probability for accidental
short circuits and electric shock hazards. We should also point out that the high
resistance electrodes will not reduce the electric field compared to highly
conductive electrodes at the same applied voltage. However the high resistance
electrodes must have a sufficient conductivity to pass the currents due to the
particle c h a r g e ~ ( ~ 9 ~ ) .
In our design concept we considered the electrodes to be a permanent part of
the filter unit and the filter medium as a disposable element. We should point
out that the electrodes can also be fabricated as an integral part of the filter
medium. In this case the electrodes and filter medium are discarded as an
integrdl unit wnen the medium becomes clogged. Including the electrodes as part
of the filter medium will increase the cost o f the medium but will also reduce the
cust and coniplexity of trre filter housing. A variety of different mesh electrodes
can be used for this purpose. For example, the glass fiber scrim that is
routinely sewn over the glass fiber media in commerc filters can have a
conductive coating applied and serve as an electrode?f% . We should emphasize
tnat the criteria listed in Table I for the electrodes also apply for the case
where tne electrodes are an integral part of the filter medium.
The final component of the.electrofibrous filter that must be specified is the
high voltage power supply. Our previous studies have shown that much h
filter efficiencies can be obtained using d.c. rather than a.c. voltageiy;g.
The decreased filter efficiency with a.c. voltage i s due to the elimination of the
charged fiber mechanism (Fig. 2) that results from the periodic reversal of the
electric field. The power supply must be capable of delivering the maximum d.c.
electric field that can be applied across the filter medium without shorting. The
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e l e c t r i c f i e l d e q u a l s t h e a p p l i e d v o l t a g e d i v i d e d by t h e d i s t a n c e between t h e
e l e c t r o d e s . F o r t h e same e l e c t r i c f i e l d , t h e maximum ),oltage w i l l De low f o r
e l e c t r o d e s c l o s e l y spaced and h i g h f o r e l e c t r o d e s spaced f a r a p a r t . A compromise
must be reached between t h e g r e a t e r i n s u l a t i o n r e q u i r e i i e n t s a t h i g h e r v o l t a g e and
t h e i n c r e a s e d t o l e r a n c e r e q u i r e d f o r c l o s e l y spaced e l t x t r o d e s . We s e l e c t e d 10 mm
as t h e minimum e l e c t r o d e s e p a r a t i o n t h a t we c o u l d main1;ain a t r e a s o n a b l e
t o l e r a n c e s . A t t h i s s e p a r a t i o n , s p a r k i n g o c c u r s acres:: t h e e l e c t r o d e s a t 14-15 kV
d.c. w i t h t h e AF-18 medium.
I n a d d i t i o n t o t h e maximum o u t p u t v o l t a g e , we a l s o l n e e d t h e maximum e l e c t r o d e
c u r r e n t f o r s e l e c t i n g t h e p r o p e r power supply. A s see$ i n F i g . 8, t h e e l e c t r o d e
c u r r e n t i n c r e a s e s s i g n i f i c a n t l y above 80% r.h. u n t i l tl?e e l e c t r o d e s s h o r t c i r c u i t
a t 90% r.h. Below 70% r . h . t h e e l e c t r o d e c u r r e n t i s lflss t h a n 0.5 P A . Based o n
t h e s e c u r r e n t and v o l t a g e r e q u i r e m e n t s we s e l e c t e d a Spellman m i n i a t u r e d.c. power
s u p p l y t h a t was r a t e d up t o 15 kV a t 75 PA. However, t o p r o v i d e f o r a
s u f f i c i e n t s a f e t y f a c t o r a g a i n s t s h o r t i n g , we o n l y a p p l y 10 kV t o t h e h i g h v o l t a g e
e l e c t r o d e s i n o u r p r o t o t y p e f i l t e r s . We a l s o added a n l a u t o m a t i c s h u t - o f f d e v i c e
t o t h e power s u p p l y d u r i n g o v e r l o a d c o n d i t i o n s as an a d d i t i o n a l s a f e t y measure.
V. Stationary Electrofibrous P r e f i l t e r
-1 2 -
were used in a similar fashion t o
maintain the shape of the rear
electrode, Pushing in the spacer bars
would press the electrodes together
and make -a good contact with the
f i l t e r medium, A 10 rntn separation was
maintained between the front and r e a r
electrodes by three s t r i p s of rubber
t h a t were attached t o the rear
electrode.
The major d i f f i c u l t y i n t h i s
design i s I~iaintaining the proper
distance between the two electrodes t o
prevent sparking. This problem i s
i l l u s t r a t e d in Fig. 10 which s h o ~ san
enlarged view of the f i l t e r element.
B o t h of the electrodes would d i s t o r t
and buckle as the unit was assembled.
Although we t r i e d a riumber o f
different schemes t o maintain tne
proper electrode spacing, we were only
able t o a p p l y 6kV before sparking
occurred.
Anot~erprobletii with the design
i s the d i f f i c u l t y i n replacing the
f i l t e r medium. To remove the f i l t e r
medium, we have t o f i r s t reiiiove b o t h
s i d e panels, take o u t the three spacer
bars, gently pull o u t the f r o n t
electrode and f i n a l l y p u l l a u t the
~tiediurn. I t i s very d i f f i c u l t t o pull
o u t the front electrode because the
screen tends t o expand like a spring.
The rear electrode i s p e ~ i ~ a ~ i e n t l y
fastened t o the nousiig. Inserting a
new f i l t e r medium requires the reverse
of these steps, a l t h o u g h the process
i s more d i f f i c u l t . The f i l t e r mediui~i
f i r s t has t o be cdrefully tucked i n t o
a l l of the deep pleats, Inserting the
f r o n t electrode screen i s especially
d i f f i c u l t becpuse the screen does n o t
maintajn i t s form a n d tends t o behave
like an accordian. The f i l t e r med~ur~i
would frequently t e a r in t h i s step.
Thk-entire process f o r replacing t h e
f i l t e r mediuin takes up t o four hours,
~ r u g ~ l with
i n ~ minor design
nients t o reduce the Sparking
probleq and make the riredia r e p l a ~ e ~ ~ n ~
Figure 10 easier, we fina?ly ~ b a n d ~ n etdh e
design.
Enlarged view o f the pleated f i l t e r
element.
-1 3-
. - "_ "._.,..,.* ".. .x.. I ill
to the ASHRAE
our maximum
filter.
e lectrof i b r o
-1 5-
100
80
M
>,
. Figure 1 4
0
c 60
a
.r Filter efficiency o f the
V
-l-
0 AF-3 AP=431Pa stationary electrofibrous
re
w 40 a AF-4 AP=229Pa I prefil ter as a function
Q-
01 I I I I I 1
0 2 4 6 8 10 12 14
Appl ied Voltage, kV
VI. Rolling Electrofibrous Prerfilter
One of the most serious accidents that can occur i n a nuclear facility is a
fire. A critical factor that increases the severity of! a fire is the potential
loss of the ventilation system due to the plugging of tlEPA filters by smoke
aerosols. A recent report by Alvares et a1 summarizes the results of a ten year
study to develop o ntermeasures to protect HEPA filters from heat and smoke
generated by f iref7r. They identified the following three countermeasures to
mitigate the problem:
materials management to reduce the quantity of' combustible materials,
1)
conventional fire detection and fire suppression techniques,
2)
Smoke removal or treatment in the ventilation duct upstream of the HEPA
3)
filter.
Alvares et a1 concluded tnat facilities having a molderate quantity of
combustible material and conventional fire management systems would be adequate to
prevent the plugging of HEPA filters during potential fires. They also concluded
that an in-duct countermeasure is necessary in facilities hav ng a high fire risk.
We became interested in the smoke problem as an extension of our program to
develop electrofibrous prefilters for prolonging the l.ife of HEPA filters.
Although we were primarily concerned with protecting the HEPA filter from the
aerosols generated during normal operations, we could not ignore the problem of
smoke aerosols plugging the HEPA filter. Since our program was just beginning a
hardware development phase in 1978, we initiated a joint program with Alvares and
his collegues to develop a prefiltration system that hIid the potential for
effectively removing normal production aerosols as well as fire generated smoke
aerosols. The difficulty of the task had been well established in various
attempts to remove the smoke aerosols. Among the variyus hods examined were
wet scrubbers, afterburners, granular beds and prefi l t w s (T'j. Although
efficient prefilters appeared to stop the smoke aerosoils, they were also rapidly
plugged. Because of the tar like property of the smoke aerosols, cleanable
prefilters, like those used in bag houses, would not o,ffer any benefit. Once the
smoke aerosol deposited on a filter, the particle depo!;it could not be removed.
-1 6-
It became very for removing smoke
g the prefilter once
it had plugged. Two gene roaches can be taken for replacing the plugged
filter; replacing individ ter units in a batch'process or replacing the
filter medium in a continuous process. Since the filter industry had nothing
available fur replacing individual filter units but had an extensive selection of
rolling filters, we selected the rolling prefilter (KPF) concept for further
development. Two preliminary experiments were conducted to examine the
feasibility of the concept. Gaskill et a1 had previously evaluated the RPF
concept using three la of cheese cloth that were pulled across the ventilation
duct with a hand cranky7'8j. Although the smoke concentration was very low, the
test demonstrated the cycle of increasing and decreasing pressure drop across the
prefilter as the medium would be periodically advanced. Alvares et a1 conducted a
more string t evaluation using an automated RPF that was rented from t h e Andersen
CorporationTy9). This evaluation confirmed that the KPF concept was capaclle of
protecting the HEPA filter from extreme smoke concentrations. Unfortun~tely,
using the Andersen unit as a prefilter t o HEPA filters would require the
installation of hign pressure blowers and associated hardware, and therefore was
not considered practical for use in nuclear ventilation systems.
Our objective was to establish the feasibility of a RPF that could operate in
nuclear ventilation systems with a low pressure drop and still protect the HEPA
filter from plugging due to smoke aerosols. Since there were no commercial RPFs
that nad the required high efficiency and low pressure drop, our strategy was to
idodify the filter housing and filter media of commercial units until the desired
results were obtained. The modifications made to the filter housing corisisted of
removing sharp edges that could tear the filter media, sealing minor leak paths in
the reservoirs holding the filter supply and take-up spools, adding an additional
rear screen to support the filter tnedium and extending the blinders used to
prevent edge leakage(l7). Figure 15 shows the inlet side of the rolling filter
purchased froin American Air Filter after these modifications were made for our
evaluation.
Figure 15
Commercial roll ing
pref i 1ter ( R P F )
modified f o r h i g h
effi c i en cy.
-1 7-
Lami na ted f i 1
-
r 1 1
\ 1 I 1 L
1
fu 1 1- Baseline - no RPF
3.0 -
n 4
3i 4 2- RPF
n
m
3 3- AF-18 + W F
0
L 4 - AF-18 + AF-18 + RPF L Figure 17
U 5- AF-18 + AF-4 + E F
aJ
L
J
v)
m
C9 m l e n g t h )
6- AF-18 + AF-4 + FG'F - Effect of filter media
on the RPF's ability
aJ (18 m l e n g t h )
L to protect the HEPA
p. -. fi 1 ter from pl ugging
2 by smoke aerosols.
w
I -
6 -
0, I I L I I 1 1
4
RPF H EPA
1 I 1
ORPF Pressure drop - 600
1.2 O H E P A Pressure drop
i
l
u
CL
r:
a
m
0.8 400
0
L
U
01
L
1
v)
v)
aJ 0.4 200
L
e
0 I I 10
0 1 2
time, ks
-1 9-
250 Pa t o 400 Pa. A more e x t e n s i v e a n a l y s i s o f experim$nt number 6 i s shown i n
F i g . 18. T h i s f i g u r e shows t h e p r e s s u r e d r o p across the; HEPA f i l t e r and p r e f i l t e r
and t h e t o t a l a i r f l o w r a t e d u r i n g t h e f i r s t 2400 seconc,ls o f t h e burn. The
o s c i l l a t i o n s i n t h e p r e s s u r e d r o p across t h e p r e f i l t e r y e due t o r e p e a t e d c y c l e s
o f f i l t e r p l u g g i n g and f i l t e r advancement. Note t h a t tile p r e s s u r e f l u c t u a t i o n s
across t h e p r e f i l t e r a r e a l s o r e f l e c t e d i n t h e f l o w r a t e and t h e p r e s s u r e d r o p
a c r o s s t h e HEPA f i l t e r .
-20-
RPF, t h e r e b y exposing t h e HEPA f i l t e r d i r e c t l y t o t h e smoke a e r o s o l s . The r a p i d
p l u g g i n g o f t h e HEPA f i l t e r a t t h i s t i m e c o n f i r m s t h a t t h e RPF i s a l s o v e r y
e f f e c t i v e a t low f a c e v e l o c i t i e s . These t e s t s demonstrate t h a t t h e m u l t i - p a s s RPF
s h o u l d a l s o be v e r y e f f e c t i v e i n p r o t e c t i n g HEPA f i l t e r s f r o m smoke aerosols.
Develoment o f t h e K o l l i n a E l e c t r o f i b r o u s P r e f i l t e r
We a l s o r e p l a c e d t h e t h i c K , l a m i n a t e d f i l t e r media shown i n F i g . 16 w i t h a
t h i n n e r media o f equal e f f i c i e n c y . T h i s change was r e q u i r e d t o p r o v i d e a s t r o n g
e l e c t r i c f i e l d w i t h o u t t h e need f o r e x c e s s i v e l y h i g h v o l t a t g e s . The compromise
between f i l t e r t h i c k n e s s and h i g h v o l t a g e requirements was p r e v i o u s l y discussed i n
S e c t i o n I V o f t h i s r e p o r t . We were a b l e t o reduce t h e f i l t e r t h i c k n e s s by
e l i i n i n a t i n g t h e coarse RPF mdium w i t h o u t a f f e c t i n g t h e f i l t e r e f f i c i e n c y .
However, i n o r d e r t o make up f o r t h e l a s t t e n s i l e s t r e n g t h o f t h e RPF medium, we
had t o sew a l a y e r o f s c r i m m a t e r i a l o v e r t h e two r e m a i n i n g f i l t e r l a y e r s . The
s c r i m m a t e r i a l i s a v e r y t h i n c l o t h t h a t i s commonly used i n t h e f i l t e r i n d u s t r y
t o add s t r e n g t h t o f i b r o u s bag f i l t e r s . U n f o r t u n a t e l y , t h e s t r e n g t h of t h e
r e i n f o r c e d media i s s t i l l n o t comparable t o t h e KPF media.
-21 -
ototipe of the screen
rof i brous pref i
1
the P l e x i g l a s t o p i
... . . .. .... ... .~ . . . -. .-.
We began o u r e v a l u a t i o n w i t h a s e r i e s o f f i r e t e s t s $ s i n g a s i n g l e l a y e r o f
HF-4 medium t h a t was 13 mm t h i c k and had r e i n f o r c i n g scr-im o r n e t t i n g on b o t h
s i d e s . L a b o r a t o r y t e s t s w i t h sodium c h l o r i d e a e r o s o l s i n d i c a t e d t h a t t h i s medium
should be a t l e a s t 85% e f f i c i e n t . The f i l t e r medium w a s i c u t e x t r a wide so t h a t
t h e edges would p r e s s a g a i n s t t h e f i l t e r housing, therebly p r e v e n t i n g e x c e s s i v e
edge leakage. No o t h e r edge s e a l i n g mechanism was used 'in t h e s e i n i t i a l t e s t s .
A l t h o u g h t h e RPF f u n c t i o n e d v e r y smoothly i n t h e s e t e s t s ' , t h e HEPA f i l t e r was
plugged i n n e a r l y t h e same t i m e as i n t h e b a s e l i n e t e t s t i t h no RPF. We b e l i e v e d
t h a t t h e primary cause of t h e poor r e s u l t s was t h e inadecjuate e f f i c i e n c y o f t h e
f i l t e r media. We i n c r e a s e d t h e f i l t e r e f f i c i e n c y by u s i n g two l a y e r s o f f i l t e r
media i n s t e a d o f one. V a r i o u s c o m b i n a t i o n s o f AF-18, AF-4 and AF-3 f i l t e r media
were used, b u t w i t h o u t success. D u r i n g t h i s phase o f o u r e v a l u a t i o n , s e v e r a l t e s t s
were p r e m a t u r e l y t e r m i n a t e d because t h e d r i v e mechanism c o u l d n o t advance t h e
screen b e l t i n g . The problem was caused by t h e f a i l u r e of t h e screen b e l t i n g t o
s u p p o r t t h e more e f f i c i e n t media d u r i n g f i l t e r c l o g g i n g . A t i n c r e a s i n g p r e s s u r e
drop, t h e screen b e l t was s l i g h t l y d e f l e c t e d , and, o c c a s i o n a l l y , one o f t h e
s u p p o r t i n g r o d s would p u l l o u t f r o m t h e c h a i n l i n k s . The c h a i n l i n k would t h e n be
f r e e t o move and would become jammed i n t h e i n s u l a t i n g t r a c k . T h i s problem was
corrected by welding t h e supporting rods t o t h e chain l i n k s .
-24-
Figure 24. Experimental deflection Figure 25. F i l t e r media reinforced w i t h
plates used t o reduce a cloth enve ope,
the leak p a t h s around
the f i l t e r edges.
t o edge leakage,
Our f i r s t attempt a t
the screen belt
filter nousing onnected t o the
move unobstructed
was quickly fab
performance. T
f 1 1 t e r med iurn" ag
made an i~nprov~m The deflection plate
Other t e s t s
showed t h a t
~ e ~ ~w ni i c~h ikept
$ t h e f i l t e r media under s l i g n t compression. W
e repeated the DOP
leak t e s t s ana f o u n d t h a t the leaks were eliminated along the s t r a i g h t parts b u t
Here s t i l l substantial along the curved portions. We were n o t aole t o m a i n t a i n a
~ o ~ ~ p r e s s iseal
o n around the curved p o r t i o n of the f i l t e r p a t h because tne media
-25-
mechanism. An integral
er media awa
I
-26- I
.
r preventing e d g e
leakage. This
compressing the ropin
F i g . 25, would be sli
in the deflecti
sealing design was
significant edg
making crrdnges
these Changes bef
Lawrence L i verm
funded oy the U
filters in the am is to develop
prototype elect ers to reduce the
load on HEPA fi
prefilter, HEPA filt eduction in c o s t and volume o f
-27-
radioactive waste when compared to the present HEPA fiilter system alone. The
electrofibrous filter being developed at LLNL is generated by applying an electric
field across a conventional fibrous filter.
on the fibers result from a dynamic process of charge accumulation due to the
particle deposits and charge dissipation due to the fiber conductivity. We have
-28-
. . .. . .. . .. .. . . . . . .. . .. .. . . . . . .. . . . . . .. . . .
t h e f i l t e r medium. We conducted a s e r i e s o f f i r e t e s t s on t h e f i r s t p r o t o t y p e t o
e v a l u a t e t h e a b i l i t y o f t h e e l e c t r o f i b r o u s r o l l i n g p r e f i l t e r t o p r o t e c t HEPA
f i l t e r s f r o m p l u g g i n g by smoke aerosols. These t e s t s have i d e n t i f i e d problems
w i t h t h e screen b e l t jamming, t h e f i l t e r media t e a r i n g and edge leakage arund t h e
f i l t e r medium. We have c o r r e c t e d t h e problems w i t h t h e screen b e l t jamming and
t h e f i l t e r media t e a r i n g b u t have n o t y e t e l i m i n a t e d t h e edge leakage. To date,
we have been unable t o demonstrate t h a t t h e p l e a t e d r o l l i n g p r e f i l t e r can p r o t e c t
t h e HEPA f i l t e r f r o m p l u g g i n g . Excessive edge leakage was i d e n t i f i e d as t h e
p r i m a r y cause o f t h e unsuccessful f i r e t e s t s . We have b u i l t a second r o l l i n g
p r e f i l t e r t h a t has i n c o r p o r a t e d design m o d i f i c a t i o n s t o c o r r e c t t h e problems
encountered w i t h o u r f i r s t u n i t . DOP t e s t s have shown t h a t t h e edge leakage has
been s i g n i f i c a n t l y reduced i n t h e second p r o t o t y p e , b u t n o t e l i m i n a t e d . We p l a n
a d d i t i o n a l d e s i g n changes t o minimize t h e leakage problem b e f o r e c o n d u c t i n g f i r e
t e s t s on t h i s u n i t .
V I I I . Biblioarauhv
3. Bergman, W., T a y l o r , R.D., Hebard, H.D., Lum, B.Y., Kuhl, W.D., B o l i n g , R.M.
and B u t t e d a h l , O . I . , " E l e c t r o f i b r o u s p r e f i l t e r ' s f o r use i n t h e n u c l e a r
i n d u s t r y , " Proc. Second U.S. DOE Environmental C o n t r o l Symposium, Reston,
V i r g i n i a , pp. 334-371 (1980).
10. Bergman, W., Biermann, A.H., Hebard, H.D., Lum, B.Y., and Kuhl, W.D.,
" E l e c t r o s t a t i c a i r f i l t e r s generated by e l e c t r i c f i e l d s , " Proc. o f F i n e
P a r t i c l e S o c i e t y Meeting, Maryland (1980).
-29-
11. Lamb, G.E.R. and Costanza, P.A., "A low-energy e l e c t r i f i e d f i l t e r system,"
F i l t r a t i o n and Separation, Vol. 17, pp. 319-322 (19t,!O).
~
17. A l v a r e s , N., Beason, D., Bergman, W., C r e i g h t o n , J.,! Ford, H. and L i p s k a , A.,
" F i r e p r o t e c t i o n countermeasures f o r containment veqiti l a t i o n , " Lawrence
L i v e r m o r e N a t i o n a l L a b o r a t o r y r e p o r t UCID-18781, L i v e r m o r e , C a l i f o r n i a (1980).
Disclaimer
-30-