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2407.04744v1
2407.04744v1
We present Quantum Monte Carlo calculations of magnetic moments, form factors, and densities
of A ≤ 10 nuclei within a chiral effective field theory approach. We use the Norfolk two- and three-
body chiral potentials and their consistent electromagnetic one- and two-nucleon current operators.
We find that two-body contributions to the magnetic moment can be large (up to ∼ 33% in A = 9
arXiv:2407.04744v1 [nucl-th] 3 Jul 2024
systems). We study the model dependence of these observables and place particular emphasis
on investigating their sensitivity to using different cutoffs to regulate the many-nucleon operators.
Calculations of elastic magnetic form factors for A ≤ 10 nuclei show excellent agreement with the
data out to momentum transfers q ≈ 3 fm−1 .
the hyperspherical harmonics method, showed excellent where Ψ(J π ; T, Tz ) is a nuclear wave function with spe-
agreement with data for magnetic form factors of A ≤ 3 cific spin-parity J π , isospin T , and charge state Tz . The
nuclei up to momentum transfers q ∼ 4 fm−1 , which is Hamiltonian has the form
well beyond the region of convergence for χEFT. Here, we X X X
H= Ki + vij + Vijk , (2)
extend these calculations to nuclei with mass number up
i i<j i<j<k
to A = 10 with the VMC method to further investigate
this high-momentum behavior. We note that these are where Ki is the non-relativistic kinetic energy and vij and
the first QMC calculations of form factors in A = 7 − 10 Vijk are respectively two- and three-nucleon potentials.
systems. The QMC approach of this work is a two-step pro-
All together, the studies of electromagnetic proper- cess that begins with the variational Monte Carlo (VMC)
ties in this work provide a benchmark of electroweak method. In nuclear VMC calculations, the variational
current models against readily available data over a ansatz taken for the many-body wave function is [51]
wide range of kinematics. Such a wide-ranging valida-
tion is necessary, as an accurate electromagnetic current Y X
TNI
model is needed for studies of electromagnetic transi- |ΨT ⟩ = S 1 + Uij + U
eijk |ΨJ ⟩ (3)
i<j i<j̸=k
tions [8, 18–21], electron-nucleus scattering [22–28], and
radiative corrections to super-allowed beta decays [29– where S is the symmetrization operator, Uij is a two-
31]. These models are also needed to interpret future body correlation operator, U e TNI is a three-body cor-
ijk
searches for new physics [32], including precision beta- relation operator, and ΨJ is a Jastrow-like wave func-
decay at low energy- and momentum-transfer [32–37], tion. The antisymmetric state ΨJ encodes the long-range
neutrinoless double beta decay at moderate momentum- structure of the system and is constructed by acting on a
transfers [38–41], and long-baseline neutrino oscillation Slater determinant that places nucleons in s- and p-shell
experiments that will involve both high energy- and orbitals with correlation functions that encode the appro-
momentum-transfer neutrino-nucleus scattering [42–48]. priate cluster structure (e.g., 6 Li ∼ α + d) of the system.
These analyses rely on theoretical inputs in order to dis- The design of the two- and three-body correlation func-
entangle signals of new physics from nuclear physics ef- tions in Eq. 3 reflects the influence of the short-distance
fects; thus, an accurate understanding of the underlying nuclear interaction in the medium. The correlation oper-
nuclear dynamics is necessary. Therefore, the compu- ators contain embedded variational parameters that one
tation of electromagnetic properties for light nuclei and then optimizes to find a best variational state, ΨV , by
detailed analysis of model dependencies are pivotal for minimizing the expectation value
the future of programs in both nuclear and fundamental
science. ⟨ΨV |H|ΨV ⟩
EV = ≥ E0 (4)
This work is organized as follows: In Section II, we de- ⟨ΨV |ΨV ⟩
tail the theoretical basis for the calculation. We review where E0 is the true ground state energy of the system.
the QMC computational technique in Section II A and The VMC result is then further improved upon by us-
report on the NV2+3 interaction models and associated ing the Green’s function Monte Carlo (GFMC) method.
electromagnetic current used in this work in Sections II B The method leverages the fact that the real time (t)
and II C, respectively. Section II D contains the multi- Schrödinger Equation
pole analysis relating QMC matrix elements to electro-
magnetic observables. Magnetic moments and two-body ∂
i |Ψ(t)⟩ = (H − ET ) |Ψ(t)⟩ , (5)
magnetic densities computed in this formalism are pre- ∂t
sented in Section III A. This is followed, in Section III B, may be recast as a diffusion equation in imaginary time
by a detailed discussion of magnetic form factors that τ = it
supplements the results and extends the analysis of a ∂
PRL submitted concurrently to this article [49]. Finally, − |Ψ(τ )⟩ = (H − ET ) |Ψ(τ )⟩ , (6)
we give concluding remarks in Section IV. ∂τ
where ET is an energy offset that controls the normaliza-
tion of the wave function. Noting that one may expand
any state in a complete orthonormal basis, we can write
II. THEORY ΨV as a sum of the true eigenstates ψi of the Hamiltonian
∞
X
A. Quantum Monte Carlo methods |ΨV ⟩ = ci |ψi ⟩ . (7)
i=1
Quantum Monte Carlo (QMC) approaches [50] are a From Eq. (6), if the energy offset ET is taken to be the
suite of computational methods used to stochastically exact energy of the ground state E0 , it is clear that in
solve the Schrödinger equation the limit τ → ∞
⟨ΨV |O|Ψ(τ )⟩ ⟨ΨV |O|ΨV ⟩ FIG. 1: Diagrams illustrating the contributions to the
⟨O(τ )⟩ ≈ 2 − , (10) electromagnetic current up to N2LO. Nucleons,
⟨ΨV |Ψ(τ )⟩ ⟨ΨV |ΨV ⟩
∆-isobars, pions, and external fields are denoted by
derived assuming the GFMC wave function at τ is a small solid, thick-solid, dashed, and wavy lines, respectively.
improvement over the VMC state; i.e., Ψ(τ ) = ΨV + δΨ. The square in panel (d) represents relativistic
Since the variational wave functions are typically good corrections to the LO current. Figure from Ref. [6].
descriptions of light nuclei, this a valid approximation.
In principle, it is possible to calculate a matrix element
L
between two propagated states in GFMC; however, this where v12 is the long-range term consisting of OPE and
S
requires performing separate imaginary time propaga- TPE contributions to order N2LO, v12 is the short-range
EM
tions for each matrix element that one would like to com- term consisting of contact interactions, and v12 is an
pute [52], which makes an order-by-order analysis of the electromagnetic contribution. The electromagnetic term
magnetic moments and form factors quite costly. Thus, retains second-order Coulomb, Darwin-Foldy, vacuum
the mixed estimate is a necessary approximation to sys- polarization, and magnetic moment interaction terms [9].
L
tematically analyze the convergence of χEFT predictions The radial functions in v12 have ∼1/rn (with n ≤ 6)
for the magnetic structure of nuclei over a range of mo- singularities at the origin that are regulated with the
menta. function
1
CRL (r) = 1 − , (12)
B. The Norfolk interaction model (r/RL )6 e2(r−RL )/RL +1
where we express the magnetic form factor as a function The various multipole contribution to the magnetic
of the reduced matrix elements (RMEs) of the magnetic form factor for the nuclei considered in this work are sum-
multipole operators (ML ), and J is the total angular mo- marized in Table I. The number of independent matrix
mentum of the nucleus. elements with different directions of q (i.e., of different
The calculation of the magnetic multipole expansion is θ’s) that have to be computed is equal to the number of
carried out using standard techniques [64] implemented multipoles allowed. Clearly, any independent choice of
to expand the current operator j(q). As the reference the directions are equivalent; in Appendix B we present
frame, we adopt the one where ẑ is the spin-quantization the explicit formulas obtained for our specific choices.
axis of the nucleus, and the direction of q̂ is defined by From the small q behaviour of the magnetic form factor
the angles θ and ϕ, the polar and azimuthal angles with it is possible to extract the magnetic (dipole) moment of
respect to this axis, respectively. In what follows, we the nucleus. Starting from the definition of the magnetic
define q = |q|. The current, in terms of the magnetic moment, it is possible to show that [67]
and electric multipoles, MLML and ELML , reads
i q
⟨J||M1 (q)||J⟩ ≃ √ µ. (19)
Z
jλ (q) = dx eiq·x êλ · j(x) 2π⟨JJ, J −J|10⟩ 2mN
X p
=− 2π(2L + 1)iL DM
L
L ,λ
(−ϕ, −θ, ϕ) Therefore, considering that the higher-order multipoles
L≥1,ML have a negligible contribution to the magnetic moment
× [λMLML (q) + ELML (q)] , at small q we can select the matrix element computed for
(16) θ = π/2 (any choice is equivalent) and so the magnetic
where λ = ±1, and DM L
are the rotation matrices [65]. moment becomes
L ,λ
The unit vector êqλ indicates the linear combination 2mN
µ = lim −i ⟨JJ|jy (q x̂)|JJ⟩ . (20)
q→0 q
ê1 ± ê2
êλ=±1 =∓ √ , (17)
2 To extract µ, we evaluate ⟨JJ|jy (qx̂)|JJ⟩ for q ∈
[0.00, 0.25] fm−1 and fit the results to a polynomial, sim-
where ê3 = q̂, ê2 = ẑ×q̂, and ê1 = ê2 ×ê3 . Note that, for
ilarly to what was done for the multipole analysis of the
elastic scattering, the electric multipole operators (EL ) 6
He β-decay spectrum in Ref. [35]. The linear coefficient
vanish because of time reversal invariance [66], and the
is then used to determine the quantity of interest.
sum over L runs only on odd values because of parity
conservation.
As observed in Ref. [67], in VMC and GFMC calcula-
tions, it is more efficient to compute the matrix elements III. RESULTS AND DISCUSSION
of j(q) between states of a specific spin configuration MJ
(usually MJ = J) and then adjust the direction of q̂ to In this section, we summarize our calculations. Specif-
isolate the single RME contributions. In our case, it is ically, we report the results for i) magnetic moments; ii)
very convenient to select q to be in the x − z plane. This two-body magnetic densities; and iii) magnetic form fac-
makes ϕ = 0, and ê2 = ŷ. Leveraging this selection and tors of light nuclei.
6
TABLE II: VMC results in units of µN for magnetic moments of nuclei with mass number A = 3 − 7, computed
with the NV2+3 interaction and consistent electromagnetic current broken down order-by-order in the chiral
expansion. The column denoted by TOT is the sum of all contributions to the magnetic moment. The columns
denoted with LO and TOT-LO indicate the contribution to the magnetic moment from the electromagnetic current
at LO and the cumulative contribution from sub-leading electromagnetic currents, respectively. Statistical
uncertainties from the Monte Carlo integration, which are ≲ 2% for all contributions listed, have been omitted. The
experimental data are from the evaluations of Refs. [68–71].
TABLE III: Same as Tab. III but for nuclei with mass number A = 8 − 10.
4 9Li
tact contributions. This is made evident by the similarity
7Li of the two-body magnetic densities in Fig. 4, defined as
3 3H 9B Z
2 8Li 10B µ2b = drij 4π rij2 2b
ρM (rij ) . (21)
1 8B
6 Li
Here, µ2b denotes a generic two-body current contribu-
( N)
TABLE IV: GFMC calculations of magnetic moments of A ≤ 9 nuclei in units of µN computed for the NV2+3-Ia⋆
model and consistent electromagnetic current. The column denoted by TOT is the sum of all contributions to the
magnetic moment, while TOT-LO indicates the sub-leading current contribution to the result. The experimental
data are from the evaluations of [68–71].
tions in this case are still enhanced, making few percent very little model dependence. Now, two-body currents
contributions to the overall magnetic moment. There only account for ∼2% of the total magnetic moment.
is a ∼15% model dependence on the N3LO(MIN) con-
tribution that is driven by changing the cutoff, whereas
the N3LO(NM) contribution is much more stable across 2. VMC magnetic moments of A = 8 − 10 nuclei
models.
The N3LO(OPE), contrary to its behavior for A = 3 Due to the cutoff dependence found in the one-pion
and A = 7, contributes with a size that is consistent with range terms at NLO and N2LO, and the general model
its power counting. The N3LO(OPE) term also displays dependence observed in the N3LO terms, we focus on two
a large model dependence in 6 Li, though this term makes representative model classes, Ia⋆ and IIb⋆ , for the heavier
a rather small contribution to the overall matrix element. nuclei with A = 8 − 10 to streamline computations.
This model dependence is readily understood by looking The VMC results for the A = 8 − 10 systems are sum-
at Eq. (A16). As observed in Ref. [6], the N3LO(OPE) IS marized in Table III. Referring to this table, we begin
contribution exhibits a node stemming from the opposite our discussion with the case of the purely IS 10 B ground
signs of the correlation functions, I1 (x) and I2 (x), ap- state. Similar to 6 Li, the IV terms are suppressed relative
pearing in the current. This, combined with the cancel- to their expected power counting. The LO contribution
lation of the N3LO(MIN) IS and N3LO(NM) IS contact is once again rather stable, albeit differing slightly from
terms, leads to an overall small contribution from two- that of the deuteron at the same order primarily due to
body IS currents to the total magnetic moment. Similar additional contributions from the orbital magnetic mo-
observations persist when extending our analysis to the ments of the protons. The N3LO(MIN) and N3LO(OPE)
two-body IS magnetic densities across the remaining nu- contributions display model dependence and have a mag-
clei examined in this study, which are plotted in Fig. 5. nitude that would be consistent with one order lower in
The three IS terms plotted are the ‘N3LO(OPE) IS,’ as the power counting. However, this model dependence
well as the ‘N3LO(MIN) IS’ and ‘N3LO(NM) IS’ contact cancels out in the summed result, leading to an overall
currents of Eqs. (A29) and (A34). These are represented consistency between the two investigated model classes.
in the figure with the yellow crosses, pink triangles, and As for 6 Li, two-body currents only play a small role and
purple “x” symbols, respectively. make up ∼1% of the total magnetic moment.
Finally, the summed magnetic moment for 6 Li displays The addition of an unpaired p-shell neutron (proton)
9
0.20 7
0.15 H
3 Li 0.15 8Li
NLO OPE
( Nfm 1)
N2LO
0.15
N3LO MIN IV
N3LO NM IV
0.10
N3LO OPE IV d 08
0.10
N3LO OPE IV d 021 0.10
N3LO LOOP M1
0.10
M
0.10
0.15 7Be
4 rij2
0.15 He
3 8B
0.15
0.0 0.5 1.0 1.5 2.0 2.5 3.0 3.5 4.0 0.200.0 0.5 1.0 1.5 2.0 2.5 3.0 3.5 4.0 0.0 0.5 1.0 1.5 2.0 2.5 3.0 3.5 4.0
rij (fm) rij (fm) rij (fm)
FIG. 4: VMC calculations of two-body IV magnetic densities for A = 3, 7, and 8 systems computed with the
NV2+3-IIb⋆ model as a function of interparticle spacing rij . Contributions from the ‘NLO’, ‘N2LO(∆)’, ‘N3LO
OPE IV d′8 ’ and ‘N3LO OPE IV d′21 ’ currents of one-pion range are represented by blue circles, red squares, light
brown triangles, and green octagons, respectively. Contributions from the short-range ‘N3LO(MIN) IV’ and
‘N3LO(NM) IV’ currents are represented by olive green stars and cyan diamonds, respectively; while the TPE IV
contribution is indicated by brown hexagons. See text for explanations. Statistical uncertainties are included but
smaller than the markers representing the central value at a given rij .
N3LO NM IS
N3LO OPE IS
0.05
0.025
0.000
0.00
2b
M
0.025
4 rij2
0.0500 1 2 3 0.050 1 2 3
rij (fm) rij (fm)
FIG. 5: VMC calculations of two-body IS magnetic densities for 6 Li and 10 B computed with the NV2+3-IIb⋆ model
as a function of interparticle spacing rij . Contributions from the ‘N3LO(MIN) IS’, ‘N3LO(NM) IS’, and
‘N3LO(OPE) IS’ currents are represented by pink triangles, yellow crosses, and purple times symbols, respectively.
See text for explanations. Statistical uncertainties are included but smaller than the markers representing the
central value at a given rij .
to 7 Li (7 Be) forms the predominantly [431] spatial sym- short-range contributions at N3LO remain enhanced rel-
metry ground state of 8 Li (8 B). At LO, the uncoupled ative to their power counting, and are found to be model
valence nucleon quenches the magnitude of the magnetic dependent. For 8 B, two-body currents quench the mag-
moment. Interestingly, the NLO and N2LO contribu- netic moment by ∼ 30%. In 8 Li, instead, they enhance
tions are not greatly altered by this additional nucleon. it by ∼ 20%.
In these nuclei, there is little additional binding from For A = 9 systems, the differences between the T =
the OPE NN interaction with the added nucleon [72]. 3/2 ground state of 9 Li and the T = 1/2 ground state
Consequently, the dominant one-pion range current con- of 9 Be lead to interesting physics in the two-body cur-
tribution at NLO stays roughly the same in A = 8 as in rents’ effect. As discussed in the previous QMC evalu-
A = 7 systems. The similarity is also true for the two- ation within the hybrid approach [8], the [432] spatial
body density, as seen in Fig. 4. This carries over also into symmetry dominates the 9 Li ground state, giving it a
the long-range N2LO and N3LO contributions, while the α + t + 2n cluster structure. On the other hand, 9 Be
10
N2LO
N3LO MIN IV 0.2
0.04 T = 3/2 nuclei, the N3LO(NM) contribution whose mag-
4 rij2
N3LO NM IV
9Be N3LO OPE IV d
0
8 9C
0.06 N3LO OPE IV d
21
0
N3LO LOOP M1
0.3 nitude would be more consistent with roughly NLO in
0.06 9B 9Li the power counting. Comparatively, in T = 1/2 systems,
( Nfm 1)
serve a behaviour consistent with the findings of Ref. [17]. spin correlations in the system. We stress that while the
During the GFMC propagation, the point proton (neu- GFMC provides the most accurate calculation within a
tron) radius increases monotonically even after conver- model, this does not imply it will provide better agree-
gence is reached for the energy calculation, which typi- ment with data than the VMC. Thus, further attention is
cally occurs at τ ≈ 0.1 MeV−1 . This may be interpreted merited to understand the inability of the Norfolk model
as the nucleus dissolving into a 7 Be (7 Li) and a proton to obtain few percent agreement with the data in these
(neutron). For these systems, we treat τ = 0.1 MeV−1 specific cases and to improve nuclear models based on
as the imaginary time at which spurious contamination χEFT moving forward.
has been removed from the VMC wave function, and av- We note that two-body currents still play a large role
erage for a small number of time steps around this point; in the total GFMC magnetic moments for all but the IS
namely, in the windows τ ∈ [0.06, 0.14] MeV−1 . We es- nuclei. As expected, the overall two-body correction still
timated the systematic uncertainty by doubling the size provides a small change to the LO result. Finally, in some
of the window to find the change in the average. cases, the two-body current contribution can change sign.
For the A = 9, T = 3/2 cases, we also have a large un- These cases all correspond to currents whose two-body
certainty on the GFMC calculations. In this case, how- densities show the presence of a node due to an interplay
ever, the uncertainty is statistical rather than system- of operators with opposite signs.
atic. While the total and beyond leading order results are
stable after convergence, there is a large error on these
matrix elements. Two matrix elements–namely the NLO 4. Scaled two-body magnetic densities
and N3LO(MIN)– have large uncertainties while the sum
of the subleading currents is stable. This results in a 5%
error for 9 Li, but for 9 C, there is a more striking 14% er- 3H
1.00 N3LO MIN IS N3LO NM IS 3He
M /|rij M |max
ror. In the later case, the LO contribution only has a 3% 6Li
error but the overall uncertainty is dominated by the two- 2b 2 2b 0.75 7Li
7Be
8Li
body term; however, as we treat the uncertainties on the 0.50 8B
9Be
total and total subleading matrix elements as a quadra- 0.25 9Li
rij2
M /|rij M |max
7Li
2b 2 2b 0.75 7Be
8Li
0.50 8B
9Be
0.25 9Li
rij2
0.00
0.5
0.0
rij2
0.75
2b 2 2b
0.50
0.25
0.00
rij2
0.0 0.5 1.0 1.5 2.0 2.5 3.0 3.5 4.0 0.0 0.5 1.0 1.5 2.0 2.5 3.0 3.5 4.0
rij (fm) rij (fm)
FIG. 8: Scaled two-body VMC IV magnetic densities for different nuclei computed with model IIb⋆ as a function of
interparticle spacing rij . Different colors represent different nuclei.
The explanation for the universal behavior of the mag- of the nucleus.
netic densities follows a similar logic. At short distances
(rij ≲ 1/mπ ), there are very few pairs in relative P -waves
due to the repulsive nature of the nuclear force in odd 5. Model dependencies in two-body magnetic densities
partial waves and the centrifugal barrier. Thus, IS pairs
at short distances tend to be predominantly ST = 10
and IV pairs ST = 01. Both the ST = 01 and ST = 10
0.15 H
pair distributions in nuclei have similar shapes and dif- 3 NLO OPE
fer only by an overall scaling factor [80, 81]. Therefore, N2LO
N3LO NM IV
this universal behavior is a result of the short-range cor-
0.10
2b
M
FIG. 10: Two-body VMC magnetic densities arising B. Magnetic form factors and high-momentum
from the N3LO(MIN) IS (blue circles), and the structure
N3LO(OPE) IS (orange squares) contributions for 6 Li
computed with model Ia⋆ (filled symbols) and IIb⋆
The magnetic form factor has been computed using
(open symbols) as a function of interparticle spacing rij .
the same interactions and currents used for the magnetic
moments. In Fig. 11, we present the results for all the
Up to this point, we have analyzed the densities only nuclei showing the contributions of the currents order-by-
for one model; however, it is important to assess the cut- order for the NV2+3-IIb⋆ interaction compared to data
off dependence, which is evidently important in the inte- where available. We also include predicted magnetic form
grated two-body contributions. To that end, we compare factors of radioactive isotopes, because while there are
the dominant IV contributions to the 3 H magnetic mo- presently are no data for comparison, novel techniques
ment in Fig. 9. The effect of the softer cutoff in the Ia⋆ have recently made it possible to study electron scatter-
regulator on the NLO(OPE) and N2LO(∆) currents is, ing from radioactive nuclei [84].
unsurprisingly, to reduce the two-body magnetic density In Fig. 12 we present the multipole contributions to
at short distances; however, the tail of the density is un- the magnetic form factors for the nuclei with J > 1 com-
affected by the cutoff function. Thus, taking a softer puted with the full currents at N3LO and the NV2+3-
cutoff quenches the overall magnitude of the matrix el- IIb⋆ . Similar results are obtained for the other interac-
ement. This particularly impacts the N2LO(∆) current tion and current models considered.
which is of shorter-range than the NLO contribution due Finally, we estimated the truncation error, limiting our
to the presence of the intermediate ∆-isobar. The soft analysis to the error associated with the chiral expan-
cutoff removes strength from the N2LO(∆) magnetic mo- sion of the electromagnetic currents, assuming the power
ment around its peak, resulting in a large quenching of counting adopted in Refs. [6, 7, 11–14]. The calculation
the contribution in model Ia⋆ relative to model IIb⋆ . The of the full chiral truncation error would require an anal-
N3LO(NM) contribution, however, is enhanced when us- ysis of the chiral expansion in both the interaction and
ing the softer cutoff of model Ia⋆ . The contact density currents, together; however, for the nuclear interactions
is broadened for the softer cutoff while preserving the considered in this work, this is not presently possible.
overall magnitude. This effect is likely due to a combina-
In order to estimate the truncation error we use the
tion of having a broader Gaussian representation of the
prescription of Ref. [85, 86] applied to
δ-function and a larger density of short-range IV pairs.
A similar broadening of the contact densities is ob-
served in Fig. 10 which shows the IS densities plotted
p 2mN
F̃M (q) = 2π(2J + 1) ⟨JJ, J −J|10⟩FM (q) . (22)
for 6 Li. For the long-range N3LO(OPE) IS contribution, q
the correlation functions I1 (x) and I2 (x) are particularly
sensitive to the choice of regulator, as was previously ob- For this analysis, we select a value of Λb = 700 MeV and,
served in Ref. [6]. This can move the node in the density for the characteristic scale of momentum Q, we follow
and change the overall sign of the contribution to the Ref. [87] by setting it to the typical momentum trans-
magnetic moment from this current, as shown in the fig- fer (A − 1)/A q, to the nucleus of mass number A. In
ure. Fig. 13, we plot the error bands at LO (orange), NLO
From the model comparison, it is clear that altering (green), N2LO (blue) and N3LO(red). Note that we do
the short-range dynamics with different cutoffs signifi- not renormalize the results to a specific value of the mag-
cantly impacts two-body magnetic moments. Clearly, netic moment.
if one takes a cutoff that is too small, it will spoil the Below we discuss in detail the results obtained for each
convergence behavior of the higher-order contributions nucleus studied.
14
10−2 10−2
10−4
10−3 10−3
10−4 10−4
|FM (q)|2
|FM (q)|2
|FM (q)|2
10−5
10−5 10−5
10−3
|FM (q)|2
10−4
10−4
10−5
Lichtenstadt 1983
Van Niftrik 1971
Goldemberg 1963
10−6
Peterson 1962
10−5 10−5
0.0 0.5 1.0 1.5 2.0 2.5 3.0 0.0 0.5 1.0 1.5 2.0 2.5 3.0 0.0 0.5 1.0 1.5 2.0 2.5 3.0
q [fm−1 ] q [fm−1 ] q [fm−1 ]
10−4
10−3
10−4
|FM (q)|2
|FM (q)|2
|FM (q)|2
10−5
10−4
Lapikas 1975
Rand 1966
Vanpraet 1965
Goldemberg 1963
10−6 10−5 10−5
0.0 0.5 1.0 1.5 2.0 2.5 3.0 0.0 0.5 1.0 1.5 2.0 2.5 3.0 0.0 0.5 1.0 1.5 2.0 2.5 3.0
q [fm−1 ] q [fm−1 ] q [fm−1 ]
|FM (q)|2
|FM (q)|2
10−4 10−5
10−4
10−6
FIG. 11: Magnetic form factors computed with the NV2+3-IIb⋆ interaction and consistent electromagnetic current.
In the figure we show the contribution of the currents up to LO (dotted blue), NLO (dashed yellow), N2LO (dot
dashed green) and N3LO (full red) in the chiral expansion. We compare our calculations with the available world
experimental data. See the text for more details.
15
10−3
10−3
10−4
|FM (q)|2
|FM (q)|2
|FM (q)|2
10−4
10−4
10−5
Lichtenstadt 1983
Van Niftrik 1971
Goldemberg 1963
10−6
Peterson 1962
10−5 10−5
0.0 0.5 1.0 1.5 2.0 2.5 3.0 0.0 0.5 1.0 1.5 2.0 2.5 3.0 0.0 0.5 1.0 1.5 2.0 2.5 3.0
q [fm−1 ] q [fm−1 ] q [fm−1 ]
10−4
10−3
10−4
|FM (q)|2
|FM (q)|2
|FM (q)|2
10−5
10−4
Lapikas 1975
Rand 1966
Vanpraet 1965
Goldemberg 1963
10−6 10−5 10−5
0.0 0.5 1.0 1.5 2.0 2.5 3.0 0.0 0.5 1.0 1.5 2.0 2.5 3.0 0.0 0.5 1.0 1.5 2.0 2.5 3.0
q [fm−1 ] q [fm−1 ] q [fm−1 ]
|FM (q)|2
|FM (q)|2
10−4 10−5
10−4
10−6
FIG. 12: Multipole contribution to the form factors computed with the NV2+3-IIb∗ interaction and consistent
electromagnetic current at N3LO for nuclei with J > 1. In the figure we show the contribution of the multipoles M1
(dashed blue line), M3 (dotted green), and M5 (dashed dot purple). The red line represents the full result.
16
1. Tritium and Helium-3 quired to describe the tail of the magnetic f.f.; however,
they generate too much strength for the M1 peak, de-
The experimental magnetic form factors (shortened to spite accurately predicting the magnetic moment. In the
f.f.’s, throughout the reminder of this section) of 3 H and region with q ≥ 1 fm−1 , the magnetic f.f. is reasonably
3
He [88, 89] are well reproduced by the VMC calculation reproduced, taking into account the theoretical errors.
as can be seen in Figs. 11a and 11b. The contribution of We note that, with none of the NV2+3 models consid-
the N3LO(NM) and N3LO(OPE) fitted terms are able to ered are we able to reproduce the experimental strength
fill in the diffraction minimum appearing at q ≃ 3 fm−1 of the first peak (see Fig. 11d), which we overpredict by
in the magnetic f.f.’s of 3 He. The 3 H diffraction is not ∼25 − 40%. For all the interactions considered, two-body
visible in the figure but a similar effect is present. We currents give a correction of ∼25% in the region of the
refer to Ref. [7] for a more detailed discussion. Similar first peak, and up to over ∼50% in the tail. This is in
results are obtained for all the other NV2+3 interactions. line with the findings of Ref. [63], which are based on
Note that the VMC calculations are in perfect agreement phenomenological models. In that study, contributions
with the Hyperspherical Harmonics results of Ref. [7]. from two-body meson exchange are found to be of the
order of 7 − 15% over most of the q region.
In 7 Be, the contribution from NLO two-body currents
2. Lithium-6 enhances the LO magnetic f.f. by a factor of ∼2, this
enhancement is even more pronounced when adding the
The 6 Li experimental magnetic form factor presents N3LO currents, almost uniformly across the 0.5 ≲ q ≲
two peaks at q ≃ 0.5 and 2 fm−1 [90–94]. Our calcu- 2.5 fm−1 region. This would make the 7 Be magnetic f.f.
lations are able to reproduce the two peaks even if, for a perfect candidate for validating models of two-body
all the interactions considered, the zero tends to come a currents, if that experimental data were available.
little too early, and the second peak contains too much
strength. This is evidenced when comparing the theoret-
ical error bands with the experimental data in Fig. 13c. 4. Lithium-8 and Boron-8
This is in line with the results of Ref. [18] obtained using
VMC together with phenomenological interactions and There are no experimental data for the magnetic f.f.’s
currents; however, the phenomenological interactions are of the A = 8 systems; however, from our calculations, we
able to reproduce the strength of the first peak [18], while observe again a large contribution from two-body cur-
all the models used in this work underpredict the strength rents (Figs. 11, panels (f) and (g)). This is particu-
of the first peak (see Fig. 11c). Since 6 Li is a T = 0 nu- larly striking in 8 B, where two-body currents reduce the
cleus, only two-body IS currents contribute to the mag- strength of the form factor for all q. It is also worth not-
netic f.f.. These contributions are negligible in the low ing the difference in the structure imprinted on the calcu-
q region (see Ref. [18, 63]) and become sizable only at lations. 8 B only has a single dominant peak at low q gen-
large values of q; indeed the IS corrections at N3LO are erated by the M1 multipole and a quenched M3 contribu-
visible only for q ≳ 1.5 fm−1 , seen in Fig. 11c. tion at higher q with a double peak structure. Instead,
8
Li exhibits a slightly two-peaked structure, where the
second peak generated by the M3 multipole is strongly
3. Lithium-7 and Beryllium-7 suppressed. Should advancements in electron scattering
on radioisotopes progress enough to measure these form
The 7 Li and 7 Be magnetic f.f.’s receive contributions factors, they would also provide interesting cases to bet-
from M1 and M3 multipoles, as can be seen in Figs. 12a ter understand two-body currents.
and 12b. The M3 contribution becomes dominant in the
region 1.0 ≤ q ≤ 2.5 fm−1 where it fills in the diffraction
minimum appearing in M1 . This is consistent with the 5. A = 9 nuclei
findings of Ref. [63] and references there in, where 7 Li is
analyzed using phenomenological models. The M1 and For A = 9 systems, there are data only for the 9 Be
M3 contributions are different in the two mirror nuclei. magnetic f.f. [91, 92, 97, 98]. The data present a plateau
In 7 Be, M3 has more strength than M1 , in contrast to in the 0.3 ≲ q ≲ 1 fm−1 region, and a peak around
what is observed in 7 Li. q ∼ 1.7 fm−1 . In Fig. 11i, we compare our results with
The available data for 7 Li are obtained from Refs. [90, the data. Referring to this figure, we note that the NLO
91, 95, 96]. As can be seen in Fig. 11d, we are able and N3LO two-body currents correct the strength of the
to explain the shape and magnitude of the experimental plateau obtained with the LO current alone, leading to
magnetic f.f.’s. The cumulative contribution from LO an improved agreement with the data. This finding con-
and NLO currents is sufficient to reproduce the peak firms the hypothesis that two body currents are crucial
at q ≃ 0.5 fm−1 . Conversely, the region where q ≥ 1 to describe the plateau as conjectured in Ref. [63]. On
fm−1 is significantly underestimated, unless N3LO cur- the other hand, they (in particular, the NLO current) sig-
rents are incorporated. The N3LO contributions are re- nificantly contribute to the second peak, resulting in an
17
F̃M (q)
F̃M (q)
F̃M (q)
10−1 10−1 10−1
Bergstrom 1982
10−2 10−2 10−2 Lapikas 1978
Rand 1966
Goldemberg 1963
Sick 2001 Sick 2001 Peterson 1962
0.0 0.5 1.0 1.5 2.0 2.5 3.0 0.0 0.5 1.0 1.5 2.0 2.5 3.0 0.0 0.5 1.0 1.5 2.0 2.5 3.0
q [fm−1 ] q [fm−1 ] q [fm−1 ]
100
100
100
10−1
F̃M (q)
F̃M (q)
F̃M (q)
10−1
10−1
F̃M (q)
F̃M (q)
Lapikas 1975
10−2 10−2 10−2 Rand 1966
Vanpraet 1965
Goldemberg 1963
0 1 2 3 0 1 2 3 0 1 2 3
q [fm−1 ] q [fm−1 ] q [fm−1 ]
100
0
10 100
F̃M (q)
F̃M (q)
F̃M (q)
10−1
10−1 10−1
LO
NLO
N2LO
−2 N3LO
10−2 10 10−2 Lapikas 1978
Rand 1966
Vanpraet 1965
0 1 2 3 0 1 2 3 0 1 2 3
q [fm−1 ] q [fm−1 ] q [fm−1 ]
FIG. 13: Errors generated by the truncation of the chiral current (only) for the magnetic form factors computed with
the NV2+3-IIb∗ interaction. In the figure the bands represent the error computed at LO (orange), NLO (green),
N2LO (blue) and N3LO (red). Note that for this figure we used the definition of the form factor as in Eq. 22.
18
Multipole
the secondary peak is overestimated even when two-body 0.00
currents are not included.
In Figs. 11i, 11j, and 11k, we show the results for the −0.01
remaining A = 9 nuclei. While in 9 B the two-body cor-
rections are minimal over all the q range, both 9 Li and 9 C −0.02 9
receive large contributions form the NLO and N3LO two- Be
body currents, and, therefore, these systems are good −0.03
candidates for studies of higher order corrections in the 0.0 0.5 1.0 1.5 2.0 2.5 3.0 3.5
currents.
q [fm−1 ]
As per the multipole contributions displayed in
Figs. 12e–12h, we note that all the A = 9 present a sim-
0.04
ilar structure. A first peak, dominated by M1 , is found
around q ∼ 0.5 fm−1 , and a second peak, dominated by
M3 , appears at q ∼ 1.5 − 1.8 fm−1 . The latter fills in 0.02
the diffraction minimum observed in M1 . The strength
of the second peak is larger for 9 Be and 9 C, while in 9 Li
Multipole
and 9 B the first peak is dominant. A similar feature is 0.00
also observed for the mirror systems 7 Li and 7 Be, where
the former is dominated by M1 and the latter by M3 .
This pattern is generated by the interference between −0.02
6. Boron-10
IV. CONCLUSIONS
10
The experimental data for the B magnetic f.f. are
provided for 0.5 ≲ q ≲ 2.0 fm−1 region [91–93, 98, 100]. In this work we presented the QMC calculations of
We did not include the data of Refs. [91, 100] in the plots magnetic moments and magnetic form factors of nuclei
because of the strong disagreement with the more recent for A ≤ 10 based on chiral effective field theory. For
experimental results reported in Ref. [63]. The VMC the calculation we used the Norfolk two- and three- body
calculation has a very nice agreement with the data in interaction and consistent one- and two-body current op-
the region of the main peak (see Fig. 11l). Contributions erators.
19
The computation of magnetic moments in light nuclei ror systems, this represents a prediction of this effect.
displayed the important role of two-body contributions. Finally, our calculations of the magnetic form factor
Consistent with previous QMC studies [8, 15], two-body also included an analysis of the contributions from two-
currents can make up a significant fraction (≈30% – 40%) body currents. As for the magnetic moments, two-body
of the total magnetic moments in light systems. The currents make a sizeable contribution to the form factors.
analysis of two-body currents in this work was supple- Over the range of momenta studied, two-body currents
mented by the computation of two-body magnetic densi- can be as large as ≈20% – 50%.
ties in a microscopic framework. These densities not only Because of the interesting structural features and the
corroborated the understanding of the two-body contri- insights provided on two-body currents, it is our view
butions on the basis of the dominant cluster structures that a renewed interest in studying elastic magnetic form
in nuclear systems, but also further illuminated our un- factors would spark further improvements in the χEFT
derstanding of how the short-range dynamics impact the framework. Until recently, it was only possible to mea-
system. As for transition densities associated with β- sure these data for stable systems; however, novel tech-
decay [17], magnetic densities display a striking univer- niques were recently used to perform the first electron
sal behavior at short distances. The long-range structure, scattering measurement for a radioisotope [84]. In the
however, is sensitive to the details of pair formation inside future, a synergy between experimentalists and theorists
the nucleus which is driven by the tensor component of could identify which systems represent feasible and inter-
the nuclear force. Finally, these densities displayed how esting candidates for such a study. This type of effort,
changing the cutoff in the Norfolk model influences the aided by the current and future capabilities of state-of-
short-range dynamics associated with this observable. the-art rare isotope beam facilities, will only serve to en-
Consistent with the studies of Refs. [7, 15], we find that hance our understanding of models of nuclear structure,
fitting the LECs appearing at N3LO in the electromag- interactions, and currents.
netic current can lead to unnaturally large contributions
compared to the expectation from naive dimensional
analysis. In the Norfolk model, this is driven by a rather ACKNOWLEDGMENTS
large contribution from the short-range N3LO(NM) dia-
gram. This enhancement spoils the order-by-order con- The authors would like to thank Josh Martin,
vergence in these calculation in the Norfolk model, as is Emanuele Mereghetti, and Ingo Tews for useful dis-
also the case for the other chiral potentials appearing in cussions at various stages in the preparation of this
the previous QMC studies. manuscript.
We investigated the impact of different regulators in This work is supported by the US Department of En-
the χEFT approach by looking at different Norfolk mod- ergy under Contracts No. DE-SC0021027 (G. C.-W.,
els. As in the calculations performed in Ref. [16], a regu- G. B. K. and S. P.), DE-AC02-06CH11357 (R.B.W.), DE-
lator dependence at NLO also appears in our calcula- AC05-06OR23177 (A.G. and R.S.), a 2021 Early Career
tions. Combined with the lack of convergence in the Award number DE-SC0022002 (M. P.), the FRIB Theory
power counting, these results merit further scrutiny to Alliance award DE-SC0013617 (M. P.), and the NUCLEI
better understand the physics responsible for these phe- SciDAC program (S.P., M.P., and R.B.W.). G. B. K.
nomena. A detailed investigation of the regulator depen- would like to acknowledge support from the U.S. DOE
dence in long-range terms could illuminate whether this NNSA Stewardship Science Graduate Fellowship under
behavior is due to power corrections from the choice of Cooperative Agreement DE-NA0003960. G. C.-W. ac-
cutoff or to a lack of renormalization in the framework. knowledges support from the NSF Graduate Research
To validate away from zero momentum transfer, we Fellowship Program under Grant No. DGE-213989. We
performed the calculation of magnetic form factors. In thank the Nuclear Theory for New Physics Topical Col-
A = 3 systems, our results represent a benchmark with laboration, supported by the U.S. Department of Energy
Ref. [7] and we find good agreement with the previous under contract DE-SC0023663, for fostering dynamic col-
evaluation and the data. We additionally performed the laborations. A.G. acknowledges the direct support of Nu-
first microscopic calculations of magnetic form factors in clear Theory for New Physics Topical collaboration.
6 ≤ A ≤ 10 nuclei using a χEFT model, which we pre- The many-body calculations were performed on the
sented in a companion [49]. We observed good qualita- parallel computers of the Laboratory Computing Re-
tive agreement with the data in most cases, reproducing source Center, Argonne National Laboratory, the com-
the strength and position of peaks in the measured form puters of the Argonne Leadership Computing Facil-
factor. We also observed for the first time that, in the ity (ALCF) via the INCITE grant “Ab-initio nuclear
mirror nuclei, there is an inversion of the strength of the structure and nuclear reactions”, the 2019/2020 ALCC
M1 and M3 multipoles. Here, we supplemented the dis- grant “Low Energy Neutrino-Nucleus interactions” for
cussion of Ref. [49] by demonstrating that this inversion the project NNInteractions, the 2020/2021 ALCC grant
is due to an interference between the LO orbital and spin- “Chiral Nuclear Interactions from Nuclei to Nucleonic
magnetization contributions to the M1 multipole. As no Matter” for the project ChiralNuc, the 2021/2022 ALCC
experiments or previous calculations exist for these mir- grant “Quantum Monte Carlo Calculations of Nuclei up
20
to 16 O and Neutron Matter” for the project QMCNuc, in Ref. [7], which are given by
and by the National Energy Research Scientific Comput-
ing Center, a DOE Office of Science User Facility sup- GpE (qµ2 ) = GD (qµ2 ) ,
ported by the Office of Science of the U.S. Department GnE (qµ2 ) = −µn χGD (qµ2 )(1 + 4χ)−1 ,
of Energy under Contract No. DE-AC02-05CH11231 us-
ing NERSC award NP-ERCAP0027147. GpM (qµ2 ) = µp GD (qµ2 ) ,
GnM (qµ2 ) = µn GD (qµ2 ) ,
which depend on qµ = q 2 − ω 2 , with ω being the energy In the preceding expressions, gA = 1.29 is the nu-
transfer. Though the form factors, which appear in all cleon axial coupling constant corrected to account for
order of the the current, themselves have a power series the Goldberger-Treiman discrepancy [101, 102].
expansion in Q, this is typically neglected and they are The N2LO (Q0 ) current involves a one-body relativis-
treated as multiplicative factors. The form factors in this tic correction (RC), shown in panel (d) of Fig. 1, and an
work are not taken from chiral perturbation theory, but IV term of one-pion range involving the excitation of an
rather from experimental fits of elastic scattering on the intermediate ∆-isobar, displayed in panel (e) of Fig. 1.
proton and deuteron. We adopt the same form factors as Their expressions are
21
ϵi (qµ2 ) q2
jN2LO 2 iq·ri
RC (q) = − 2 p i + 2 p i + i σi × q + pi · q (q + 2 i σi × pi ) , e
16 m3 4 +
µi (qµ2 ) − ϵi (qµ2 )
−i pi · q 4 σi × pi − i q
16 m3
q2
− (2 i pi − σi × q) + 2 (pi × q) σi · pi , eiq·ri , (A11)
2 +
j∆ (q) = −iGγN ∆ (qmu ) eiq·ri τj,z I1∆ (xij ) σj + I2∆ (xij ) σj · r̂ij r̂ij
N2LO 2
1 q
− ei q·ri (τi × τj )z I1∆ (xij ) σi × σj + I2∆ (xij ) σj · r̂ij σi × r̂ij
×
4 mπ
+(i ⇌ j) , (A12)
with the correlation functions Ik∆ (x) defined as follows, where the transition magnetic moment µγN ∆ = 3µN is
taken from an analysis of γN data in the ∆ resonance
gA hA 1 m2π m2π
∆ region [103] and we adopt Λ∆,1 = 0.84 GeV and Λ∆,2 =
I1 (x) = −
18 π 2 m m∆N fπ2 1.2 GeV from the same analysis.
e−x
×(1 + x) 3 , (A13)
x
2 2
gA hA 1 mπ mπ
I2∆ (x) =
18 π 2 m m∆N fπ2
e−x
×(3 + 3 x + x2 ) 3 , (A14)
x
where m∆N = 0.2931 GeV is the delta-nucleon mass dif- At N3LO (Q1 ), the long-range current operator con-
ference and hA = 2.73 is the πN ∆ coupling constant. sists of an isocalar (IS) and an isovector (IV) OPE terms
The N -to-∆ transition form factor is defined as, generated by the diagram illustrated in panel (f) of Fig. 2.
µγN ∆ The N3LO IS current of one-pion range is proportional
2
GγN ∆ (qmu )= q , (A15) to the d′9 LEC, and it reads
(1 + qµ2 /Λ2∆,1 ) 1 + qµ2 /Λ2∆,2
q
jN3LO iq·ri
Gγπρ (qµ2 ) τi · τj I1S (xij ) σj + I2S (xij ) σj · r̂ij r̂ij ×
IS OPE (q) = −i e + (i ⇌ j) , (A16)
mπ
where the correlation functions, namely I1S (x) and I2S (x), where mω is the ω-meson mass.
may be obtained from the following rescaling of the The N3LO IV current of one-pion range is composed
N2LO(∆) correlation functions of Eqs. (A13)-(A14) by two terms proportional to the d′8 and d′21 LECs, re-
spectively:
gA hA 1 m2π m2π gA m2π 2 ′
−→ m d ,
18 π 2 m m∆N fπ2 16 π fπ2 π 9
N3LO, d′8 N3LO, d′21
jN3LO
IV OPE (q) = jIV OPE (q) + jIVOPE (q) , (A18)
and the transition form factor is defined as,
1
Gγπρ (qµ2 ) = , (A17) where
1 + qµ2 /m2ω
In the expressions above, the IV correlation functions while the correlation functions Ie1V (x) and Ie2V (x) can be
I1V (x) and I2V (x) are obtained from the correlation func- obtained by making the substitution,
tions of Eqs. (A13)-(A14) by substituting,
gA hA 1 m2π m2π gA m2π 2 ′
−→ m d .
18 π 2 m m∆N fπ2 16 π fπ2 π 21
(A22)
gA hA 1 m2π m2π gA m2π 2 ′
−→ m d . The N3LO TPE loop term coming from the contribu-
18 π 2 m m∆N fπ2 16 π fπ2 π 8 tions shown in panels (g)-(k) of Fig. 2 has the following
(A21) form
h
(0) (1)
i
(2)
q
jN3LO
LOOP (q) = i τj,z e iq·Rij
GVE (qµ2 ) F0 (λij ) + F2 (λij ) σi + F2 (λij ) σi · r̂ij r̂ij ×
2 mπ
1 ṽ 2π (λij )
− (τi × τj )z eiq·Rij r̂ij λij + (i ⇌ j) . (A23)
2 2 mπ
A detailed derivation of the loop functions F (n) (λij ), where λij = 2mπ rij , can be found in Ref. [6]. Here, we
limit ourselves to listing their expressions,
4 −λ
4
1 1 1 − e−λ(αz −1)
(2 mπ ) e 1 1 1
Z
(0) gA (−)
F0 (λ) = 1+ dz − 2 + 1 − E1 (λ)
256 π 3 fπ4 λ 2 0 αz2 − 1 gA λ 2
1 1 1 (+)
− 2 + 1 λ + 2 E1 (λ) ,
gA
4
4
1 1 1 − e−λ(αz −1)
(2 mπ ) 1 1
Z
(2) gA −λ
F1 (λ) = e + 1 + dz
256 π 3 fπ4 λ3 λ2 2 0 αz2 − 1
1 1 1 1 (−) 1 1 1 1 (+)
− 2 +2 + 2 − E (λ) − 2 +2 − 2 − E (λ)
gA λ3 λ 2λ 1 gA λ3 λ 2λ 1
Z 1
1 1 (0) 4 1 1 −λαz
+ − 2 E (λ) − dz + e ,
2
gA λ3 1 0 λ3 αz + 1 2 λ2
4
4
1 1 1 − e−λ(αz −1)
(2 mπ ) 3 3 1
Z
(2) gA −λ
F2 (λ) = − e + 2+ 1+ dz
256 π 3 fπ4 λ3 λ λ 2 0 α2 − 1
z
1 3 3 1 1 1 (−)
− 2 +2 3
+ 2+ − 1+ E1 (λ)
gA λ λ λ 2 λ
1 3 3 1 1 1 (+) 1 3 (0)
− +2 − 2+ + 1− E1 (λ) + −2 E (λ)
2
gA λ 3 λ λ 2 λ gA2 λ3 1
Z 1
16 3 1 1 −λαz
− dz 3 + 4 αz + e ,
0 λ 2 αz + 1 λ2
where the following definitions have been employed, The N3LO LOOP two-body currents satisfy the con-
tinuity equation with the NV2 potential at N2LO in the
αz = (1 − z 2 )−1/2 , (A24) limit of momentum transfer going to zero. This is re-
Z ∞
e−t flected by the presence of the ṽ2π (λij ) = v2π (λij )τi · τj
E1 (x) = dt , (A25) term in Eq. (A23). The v2π (λij ) term indicates contribu-
x t
tions to the NV2 potential coming from TPE diagrams.
e±λ 1
Z
(±) In the present study, it accounts for TPE terms at both
E1 (λ) = dzE1 (λαz + λ) (A26)
2 0 NLO and N2LO, therefore it includes two-pion loops with
Z 1
(0) and without ∆-isobar intermediate states (see Ref. [6] for
E1 (λ) = dzE1 (λαz ) (A27)
0
23
1 4 h
(0) q i
jN3LO
MIN IS (q) = − m C 5 eiq·Rij S
G (q 2
) i C (zij ) (σ i + σj ) × , (A29)
8 π E µ RS
mπ
1 (1)
h
jN3LO
MIN IV (q) = (τi × τj )z eiq·Rij GVE (qµ2 ) CRS (zij ) m4π (C2 + 3 C4 + C7 ) r̂ij
8 i
+m4π (C2 − C4 − C7 ) r̂ij σi · σj + m4π C7 (σi · r̂ij σj + σj · r̂ij σi )
1 h
(1)
i
− m4π C5 eiq·Rij (τi,z − τj,z ) CRS (zij ) (σi + σj ) × r̂ij . (A30)
8
In the equations above are the same that appear in the contact terms of the NV2
2
potential at N2LO.
(0) e−z The N3LO(NM) contact term is also broken into IS
CRS = , (A31)
π (mπ RS )3
3/2 and IV components as
(0)
(1) 1 dCRS
CRS = , (A32) jN3LO N3LO N3LO
NM (q) = jNM IS (q) + jNM IV (q) , (A33)
mπ RS dz
where zij = rij /RS . The Ci LECs in Eqs. (A29)-(A30) where
(0) q
jN3LO
NM IS (q) = −i e
iq·Rij
CRS (zij ) m4π GSE (qµ2 ) C15
′
(σi + σj ) × , (A34)
mπ
(0) q
jN3LO
NM IV (q) = −i e
iq·Rij
CRS (zij ) m4π GVE (qµ2 ) C16
′
(τi,z − τj,z ) (σi − σj ) × . (A35)
mπ
The last N3LO contact term, originating from the regu- larization scheme in configuration space adopted for the
TPE currents [6], reads:
(0) q
jN3LO V 2
CT (q) = iGE (qµ ) τj,z e
iq·Rij
F0 (zij ; ∞) σi × + (i ⇌ j) , (A36)
2 mπ
For the unknown LECs of non-minimal nature, namely, Appendix B: Evaluation of the magnetic multipoles
d′8 , d′9 , d′21 , C15
′ ′
and C16 , we take the values obtained
in Ref. [7] that use the deuteron and the three-nucleon Using Eq. (18) we can evaluate the value of the reduced
systems’ magnetic moments, as well as deuteron photo- matrix elements for the magnetic multipole operators. To
disintegration data at backward angles to constrain them. do that we need a number of linear equations equal to the
These values are provided in Table V. number of the multipoles allowed by the transition.
As stated in Ref. [67] for VMC and GFMC, in order
to obtain the linear equations we need for the extraction
of the reduced matrix elements, is more computationally
efficient to change the direction of q̂ rather than repeat-
ing the calculation of the matrix elements for different
24
′
Class C16 m4π d′8 m2π d′21 m2π ′
C15 m4π d′9 m2π The final result reads
NVIa⋆ −0.050(2) 0.49(7) 0.094(4) 0.012(1) 0.023(7) " √ #
NVIb⋆ −0.055(3) 0.09(5) 0.073(3) 0.025(2) 0.030(6) 3 2 2 2
NVIIa⋆ −0.066(2) 0.01(7) 0.069(4) 0.011(1) 0.019(7)
M12= √ 2
Xπ/2 + Xπ/4 , (B6)
2 5π 3
NVIIb⋆ −0.049(2) 0.09(4) 0.048(3) 0.017(1) 0.018(3) √
2 4 2 h 2 √ 2 i
M3 = √ Xπ/2 − 2Xπ/4 . (B7)
TABLE V: Values of the LECs corresponding to the 15π
NV2+3 Hamiltonians Ia⋆ , Ib⋆ , IIa⋆ , and IIb⋆ obtained
in Ref. [7] from fits to the deuteron and the trinucleon For J = 3 three different multipoles with L = 1, 3,
systems’ magnetic moments, as well as deuteron and 5 can be excited. Therefore, we need to have three
photo-disintegration at backward angles data. independent linear equations that
√ we obtain selecting θ =
π/2, θ = π/4 and cos θ = 2 2/3. The solution of the
linear equations reads
r
3 1 53 3 232 3 81 3
projection of the total angular momentum. Therefore, if M1 = √ X + X − √ X ,
we have n possible multipoles, we select n values for the 7π 280 2 π/2 735 π/4 1960 2 1/3
angle θ (that is the angle between the ẑ axis and the di- (B8)
rection of q̂) obtaining n linear equations to invert. The " √ √ #
1 13 2 3 32 3 81 2 3
choice of θ is arbitrary: we choose the ones that simplify M33 = √ Xπ/2 − Xπ/4 − X ,
as much as possible the solution of the linear equations. π 20 35 140 1/3
Below we report the solution of the linear equations for (B9)
the cases studied in this work. To simplify the notation r "√ √ #
35 2 3 32 3 27 2 3
we indicate the matrix element computed using Monte M53 = 6 X − X + X ,
Carlo as π 35 π/2 245 π/4 245 1/3
(B10)
XθJ = ⟨J J |jγ,y (q(θ))| J J⟩ , (B1)
3
where X1/3 = ⟨3 3| jγ,y (q(cos θ = 1/3)) |3 3⟩.
and by
MLJ = ⟨J||ML ||J⟩ , (B2) Appendix C: Note on the magnetic form factors data
the reduced matrix elements of the magnetic multipole The experimental data of the magnetic form factors
L among states J. shown in this work have been obtained directly the orig-
For nuclei with J = 1/2 and J = 1 only the multi- inal references. The definitions used in some of the ex-
pole with L = 1 is allowed. In this case we need only perimental works for the magnetic f.f. are different com-
one equation for which we chose θ = π/2 (q̂ ∥ x̂). The pared to the one used in this work, therefore we renor-
resultant reduced matrix element for J = 1/2 and J = 1 malize them with an appropriate factor given by the ratio
2∗
is among the experimental values FM (q) in the paper and
the one defined in Eq. (15). For example, in the cases of
1/2,1 1 1/2,1 Refs. [92, 95, 98], this ratio is given by
M1 = √ Xπ/2 . (B3)
π
2
FM (q) 1 2 q 2 J + 1
2∗ = µ , (C1)
The situation for the J = 23 case is more involved since FM (q) 2π 2M 3J
both the M1 and M3 multipoles contributes to the mag-
netic f.f. In order to obtain the two magnetic multipoles where µ is the magnetic moment and J the total angular
we have to compute two matrix elements changing the di- momentum of the nucleus.
rection of q̂. For this case we select θ = π/2 and θ = π/4. Note that Refs. [90, 91, 97, 100] report only the elastic
By inverting the linear equations we obtain the magnetic scattering cross section data from which we obtain the
multipoles as function of the computed matrix elements, values of the magnetic f.f. with the following formula
as " 2 #−1
2 dσ α
r " √ # FM (q) = 4π , (C2)
3/2 2 3/2 2 2 3/2 dΩ Exp 2E0
M1 = Xπ/2 + Xπ/4 , (B4)
5π 3
where α is the fine structure constant, and E0 the
3/2 8 h 3/2 √ 3/2 i energy of the electron beam. Note that the data of
M3 = √ Xπ/2 − 2Xπ/4 . (B5)
15π Refs. [90, 91, 100] tend to overestimate the other experi-
mental data sets. Indeed we excluded them in the plots
For the J = 2 case we use the same angle as J = 3/2. of 10 B magnetic f.f., following what was done in Ref. [63].
25
Nucleus Reference Data type ratio/method The data for 3 H and 3 He are from a global fit per-
3
H Sick 2001 [89] N 1 formed in Ref. [88] of the electron scattering cross sec-
tions at different angles applying the Rosenbluth separa-
3
He Sick 2001 [89] N 1 tion, which was then reused in [89] where the data are
6
taken from. For Refs. [93, 95], no numerical values were
Li Peterson 1962 [90] N Eq. (C2) available, and therefore we digitized directly the plots on
Goldemberg 1963 [91] N Eq. (C2) the paper using Web Plot Digitizer [104]. In Table VI,
Rand 1966 [92] N Eq. (C1)
we report for each nucleus and experimental data set the
Lapikas 1978 [93] D 1/4π
Bergstrom 1982 [94] N Z 2 /4π reference, the normalization compared to our definition
of the magnetic f.f. or the formula used to extract from
7
Li Peterson 1962 [90] N Eq. (C2) the cross section respect to the original reference, and
Goldemberg 1963 [91] N Eq. (C2) if the data have been digitized (D) or taken as numeric
Van Niftrik 1971 [95] D Eq. (C1) (N). The digitized data sets are available as Supplemental
Lichtenstadt 1983 [96] N Z 2 /4π Material to this paper.
9
Be Goldemberg 1963 [91] N Eq. (C2)
Vanpraet 1965 [98] N Eq. (C1)
Rand 1966 [92] N Eq. (C1)
Lapikas 1975 [97] N Eq. (C2)
10
B Goldemberg 1963 [91] N Eq. (C2)
Goldemberg 1965 [100] N Eq. (C2)
Vanpraet 1965 [98] N Eq. (C1)
Rand 1966 [92] N Eq. (C1)
Lapikas 1978 [93] D 1/4π
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