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Phonons Phonons: Longitudinal Lattice Wave (Phonon)
Phonons Phonons: Longitudinal Lattice Wave (Phonon)
MSE/ECE 310
Phonons
Longitudinal Lattice Wave (phonon)
Phonons
vg =
s+p = specific plane us+p = displacement
Knowlton
p = whole number
1
Knowlton
MSE/ECE 310
MSE/ECE 310
Phonons
Phonons
Phonon Dispersion Relation for Diatomic Linear Lattice
1 1 2 2c + m1 m2
2c m2 2c m1
McKelvey, Solid State Physics for Engineering & Materials Science, (Krieger, 1993) Ch. 3
Knowlton
Knowlton
MSE/ECE 310
MSE/ECE 310
Phonons
Phonons
u k
u & k Are perpendicular for a transverse phonon
Whether a vibrational mode is longitudinal or transverse, a given atomic amplitude of motion requires much more energy for a long wave optical than acoustic mode. Why? B/c optical modes minimize changes in 2nd n.n. separation by maximizing separation between n.n.s. N.n. interaction greater than any other n.n. interaction, therefore, energy required for n.n. separation greater than any other separation. KnowltonU = dF/dx integrate under curves to get energy.
Knowlton
MSE/ECE 310
MSE/ECE 310
Phonons
Knowlton
Knowlton
MSE/ECE 310
MSE/ECE 310
Phonons
Phonon Combination Bands (two phonon overtone bands)
Phonon Imaging
Phonon Transmission study:
65% transmission of ballistic phonons
fast transverse <111>
unbonded side
Knowlton
10
MSE/ECE 310
MSE/ECE 310
Phonon Imaging
Phonon Transmission study:
Sample configuration
2750 2500 2250
Phonon Imaging
Phonon Transmission study:
Time of flight
Integration: FTA Spectrum - Side Without Interface Area Peak at Width Height 377.64547 1.57617 0.21094 1269 Integration: FTA Spectrum - Side With Interface Area Peak at Width Height 693.59764 1.49414 0.19922 2515 % Phonon Transmission = Area1/Area2 x 100 = 55%
3mm
Laser Pulse
E In utec te ti rfa c ce
4mm
380m
Ballistic
900m
1.0
1.5
2.0
2.5
3.0
3.5
4.0
4.5
5.0
5.5
6.0
Time (s)
Fast tranverse optical phonon Slow transverse optical phonon If we examine TOF data from phonon imaging study Notice that time at peak max is no more than 1 s
11
Knowlton
12
MSE/ECE 310
MSE/ECE 310
Phonon Imaging
Phonon Transmission study:
Prototype Dark Matter Detector Really a phonon detector
Si Si Si [111]
Energy (meV)
62 100 150 200 250 300 350 400 450 496
(m)
20 15 6000
Transmittance (arb. units)
10
5
4000
2.5
3500
5000
3000
2500
2000 1100
1110
1120
1130
1140
1150
1160
1170
1136.4 cm
-1
Knowlton
500
Knowlton LVM of O
1000
1500
2000
2500
-1
3000
3500
4000
13
Knowlton
14